Engineering multi-pathway graphene oxide membranes toward ultrafast water purification
Graphene oxide (GO) membranes hold great promise in molecular separation owing to the ultrathin thickness as well as precisely controllable interlayer distance. However, the tortuous mass transport pathway along stacked nanosheets hinders the availability of high-flux GO membranes. Herein, we design...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Guan, Jingyuan [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2021transfer abstract |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Steering charge kinetics in W - Yue, Xin-Zheng ELSEVIER, 2019, the official journal of the North American Membrane Society, New York, NY [u.a.] |
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| Übergeordnetes Werk: |
volume:638 ; year:2021 ; day:15 ; month:11 ; pages:0 |
| Links: |
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| DOI / URN: |
10.1016/j.memsci.2021.119706 |
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| 520 | |a Graphene oxide (GO) membranes hold great promise in molecular separation owing to the ultrathin thickness as well as precisely controllable interlayer distance. However, the tortuous mass transport pathway along stacked nanosheets hinders the availability of high-flux GO membranes. Herein, we design multi-pathway GO membranes to afford fast water transport through in-plane and interlayer pathways. The in-plane pathway is introduced by the porous GO (pGO) nanosheets and the interlayer pathway is enlarged by intercalating hydrophilic halloysite nanotubes (HNTs) into adjacent pGO nanosheets, jointly contributing to the enhanced water permeance. Through manipulating the intercalator amount, the optimized membrane displays ultrahigh water permeance of 206.7 L m−2 h−1 bar−1 and dye rejections over 98.5%. Furthermore, the resultant membranes exhibit resistance against broad-spectrum oil-in-water emulsions. Our study can pave a facile and prospective way to fabricating high-performance two-dimensional laminated membranes. | ||
| 520 | |a Graphene oxide (GO) membranes hold great promise in molecular separation owing to the ultrathin thickness as well as precisely controllable interlayer distance. However, the tortuous mass transport pathway along stacked nanosheets hinders the availability of high-flux GO membranes. Herein, we design multi-pathway GO membranes to afford fast water transport through in-plane and interlayer pathways. The in-plane pathway is introduced by the porous GO (pGO) nanosheets and the interlayer pathway is enlarged by intercalating hydrophilic halloysite nanotubes (HNTs) into adjacent pGO nanosheets, jointly contributing to the enhanced water permeance. Through manipulating the intercalator amount, the optimized membrane displays ultrahigh water permeance of 206.7 L m−2 h−1 bar−1 and dye rejections over 98.5%. Furthermore, the resultant membranes exhibit resistance against broad-spectrum oil-in-water emulsions. Our study can pave a facile and prospective way to fabricating high-performance two-dimensional laminated membranes. | ||
| 650 | 7 | |a Multiple mass transport pathways |2 Elsevier | |
| 650 | 7 | |a Ultrafast water transport |2 Elsevier | |
| 650 | 7 | |a Graphene oxide membrane |2 Elsevier | |
| 650 | 7 | |a Acid etching |2 Elsevier | |
| 650 | 7 | |a Halloysite nanotube intercalating |2 Elsevier | |
| 700 | 1 | |a You, Xinda |4 oth | |
| 700 | 1 | |a Shi, Benbing |4 oth | |
| 700 | 1 | |a Liu, Yanan |4 oth | |
| 700 | 1 | |a Yuan, Jinqiu |4 oth | |
| 700 | 1 | |a Yang, Chao |4 oth | |
| 700 | 1 | |a Pang, Xiao |4 oth | |
| 700 | 1 | |a Wu, Hong |4 oth | |
| 700 | 1 | |a Shen, Jianliang |4 oth | |
| 700 | 1 | |a Fan, Chunyang |4 oth | |
| 700 | 1 | |a Long, Mengying |4 oth | |
| 700 | 1 | |a Zhang, Runnan |4 oth | |
| 700 | 1 | |a Jiang, Zhongyi |4 oth | |
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10.1016/j.memsci.2021.119706 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001500.pica (DE-627)ELV055068766 (ELSEVIER)S0376-7388(21)00652-9 DE-627 ger DE-627 rakwb eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Guan, Jingyuan verfasserin aut Engineering multi-pathway graphene oxide membranes toward ultrafast water purification 2021transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Graphene oxide (GO) membranes hold great promise in molecular separation owing to the ultrathin thickness as well as precisely controllable interlayer distance. However, the tortuous mass transport pathway along stacked nanosheets hinders the availability of high-flux GO membranes. Herein, we design multi-pathway GO membranes to afford fast water transport through in-plane and interlayer pathways. The in-plane pathway is introduced by the porous GO (pGO) nanosheets and the interlayer pathway is enlarged by intercalating hydrophilic halloysite nanotubes (HNTs) into adjacent pGO nanosheets, jointly contributing to the enhanced water permeance. Through manipulating the intercalator amount, the optimized membrane displays ultrahigh water permeance of 206.7 L m−2 h−1 bar−1 and dye rejections over 98.5%. Furthermore, the resultant membranes exhibit resistance against broad-spectrum oil-in-water emulsions. Our study can pave a facile and prospective way to fabricating high-performance two-dimensional laminated membranes. Graphene oxide (GO) membranes hold great promise in molecular separation owing to the ultrathin thickness as well as precisely controllable interlayer distance. However, the tortuous mass transport pathway along stacked nanosheets hinders the availability of high-flux GO membranes. Herein, we design multi-pathway GO membranes to afford fast water transport through in-plane and interlayer pathways. The in-plane pathway is introduced by the porous GO (pGO) nanosheets and the interlayer pathway is enlarged by intercalating hydrophilic halloysite nanotubes (HNTs) into adjacent pGO nanosheets, jointly contributing to the enhanced water permeance. Through manipulating the intercalator amount, the optimized membrane displays ultrahigh water permeance of 206.7 L m−2 h−1 bar−1 and dye rejections over 98.5%. Furthermore, the resultant membranes exhibit resistance against broad-spectrum oil-in-water emulsions. Our study can pave a facile and prospective way to fabricating high-performance two-dimensional laminated membranes. Multiple mass transport pathways Elsevier Ultrafast water transport Elsevier Graphene oxide membrane Elsevier Acid etching Elsevier Halloysite nanotube intercalating Elsevier You, Xinda oth Shi, Benbing oth Liu, Yanan oth Yuan, Jinqiu oth Yang, Chao oth Pang, Xiao oth Wu, Hong oth Shen, Jianliang oth Fan, Chunyang oth Long, Mengying oth Zhang, Runnan oth Jiang, Zhongyi oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:638 year:2021 day:15 month:11 pages:0 https://doi.org/10.1016/j.memsci.2021.119706 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 638 2021 15 1115 0 |
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10.1016/j.memsci.2021.119706 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001500.pica (DE-627)ELV055068766 (ELSEVIER)S0376-7388(21)00652-9 DE-627 ger DE-627 rakwb eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Guan, Jingyuan verfasserin aut Engineering multi-pathway graphene oxide membranes toward ultrafast water purification 2021transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Graphene oxide (GO) membranes hold great promise in molecular separation owing to the ultrathin thickness as well as precisely controllable interlayer distance. However, the tortuous mass transport pathway along stacked nanosheets hinders the availability of high-flux GO membranes. Herein, we design multi-pathway GO membranes to afford fast water transport through in-plane and interlayer pathways. The in-plane pathway is introduced by the porous GO (pGO) nanosheets and the interlayer pathway is enlarged by intercalating hydrophilic halloysite nanotubes (HNTs) into adjacent pGO nanosheets, jointly contributing to the enhanced water permeance. Through manipulating the intercalator amount, the optimized membrane displays ultrahigh water permeance of 206.7 L m−2 h−1 bar−1 and dye rejections over 98.5%. Furthermore, the resultant membranes exhibit resistance against broad-spectrum oil-in-water emulsions. Our study can pave a facile and prospective way to fabricating high-performance two-dimensional laminated membranes. Graphene oxide (GO) membranes hold great promise in molecular separation owing to the ultrathin thickness as well as precisely controllable interlayer distance. However, the tortuous mass transport pathway along stacked nanosheets hinders the availability of high-flux GO membranes. Herein, we design multi-pathway GO membranes to afford fast water transport through in-plane and interlayer pathways. The in-plane pathway is introduced by the porous GO (pGO) nanosheets and the interlayer pathway is enlarged by intercalating hydrophilic halloysite nanotubes (HNTs) into adjacent pGO nanosheets, jointly contributing to the enhanced water permeance. Through manipulating the intercalator amount, the optimized membrane displays ultrahigh water permeance of 206.7 L m−2 h−1 bar−1 and dye rejections over 98.5%. Furthermore, the resultant membranes exhibit resistance against broad-spectrum oil-in-water emulsions. Our study can pave a facile and prospective way to fabricating high-performance two-dimensional laminated membranes. Multiple mass transport pathways Elsevier Ultrafast water transport Elsevier Graphene oxide membrane Elsevier Acid etching Elsevier Halloysite nanotube intercalating Elsevier You, Xinda oth Shi, Benbing oth Liu, Yanan oth Yuan, Jinqiu oth Yang, Chao oth Pang, Xiao oth Wu, Hong oth Shen, Jianliang oth Fan, Chunyang oth Long, Mengying oth Zhang, Runnan oth Jiang, Zhongyi oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:638 year:2021 day:15 month:11 pages:0 https://doi.org/10.1016/j.memsci.2021.119706 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 638 2021 15 1115 0 |
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10.1016/j.memsci.2021.119706 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001500.pica (DE-627)ELV055068766 (ELSEVIER)S0376-7388(21)00652-9 DE-627 ger DE-627 rakwb eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Guan, Jingyuan verfasserin aut Engineering multi-pathway graphene oxide membranes toward ultrafast water purification 2021transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Graphene oxide (GO) membranes hold great promise in molecular separation owing to the ultrathin thickness as well as precisely controllable interlayer distance. However, the tortuous mass transport pathway along stacked nanosheets hinders the availability of high-flux GO membranes. Herein, we design multi-pathway GO membranes to afford fast water transport through in-plane and interlayer pathways. The in-plane pathway is introduced by the porous GO (pGO) nanosheets and the interlayer pathway is enlarged by intercalating hydrophilic halloysite nanotubes (HNTs) into adjacent pGO nanosheets, jointly contributing to the enhanced water permeance. Through manipulating the intercalator amount, the optimized membrane displays ultrahigh water permeance of 206.7 L m−2 h−1 bar−1 and dye rejections over 98.5%. Furthermore, the resultant membranes exhibit resistance against broad-spectrum oil-in-water emulsions. Our study can pave a facile and prospective way to fabricating high-performance two-dimensional laminated membranes. Graphene oxide (GO) membranes hold great promise in molecular separation owing to the ultrathin thickness as well as precisely controllable interlayer distance. However, the tortuous mass transport pathway along stacked nanosheets hinders the availability of high-flux GO membranes. Herein, we design multi-pathway GO membranes to afford fast water transport through in-plane and interlayer pathways. The in-plane pathway is introduced by the porous GO (pGO) nanosheets and the interlayer pathway is enlarged by intercalating hydrophilic halloysite nanotubes (HNTs) into adjacent pGO nanosheets, jointly contributing to the enhanced water permeance. Through manipulating the intercalator amount, the optimized membrane displays ultrahigh water permeance of 206.7 L m−2 h−1 bar−1 and dye rejections over 98.5%. Furthermore, the resultant membranes exhibit resistance against broad-spectrum oil-in-water emulsions. Our study can pave a facile and prospective way to fabricating high-performance two-dimensional laminated membranes. Multiple mass transport pathways Elsevier Ultrafast water transport Elsevier Graphene oxide membrane Elsevier Acid etching Elsevier Halloysite nanotube intercalating Elsevier You, Xinda oth Shi, Benbing oth Liu, Yanan oth Yuan, Jinqiu oth Yang, Chao oth Pang, Xiao oth Wu, Hong oth Shen, Jianliang oth Fan, Chunyang oth Long, Mengying oth Zhang, Runnan oth Jiang, Zhongyi oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:638 year:2021 day:15 month:11 pages:0 https://doi.org/10.1016/j.memsci.2021.119706 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 638 2021 15 1115 0 |
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10.1016/j.memsci.2021.119706 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001500.pica (DE-627)ELV055068766 (ELSEVIER)S0376-7388(21)00652-9 DE-627 ger DE-627 rakwb eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Guan, Jingyuan verfasserin aut Engineering multi-pathway graphene oxide membranes toward ultrafast water purification 2021transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Graphene oxide (GO) membranes hold great promise in molecular separation owing to the ultrathin thickness as well as precisely controllable interlayer distance. However, the tortuous mass transport pathway along stacked nanosheets hinders the availability of high-flux GO membranes. Herein, we design multi-pathway GO membranes to afford fast water transport through in-plane and interlayer pathways. The in-plane pathway is introduced by the porous GO (pGO) nanosheets and the interlayer pathway is enlarged by intercalating hydrophilic halloysite nanotubes (HNTs) into adjacent pGO nanosheets, jointly contributing to the enhanced water permeance. Through manipulating the intercalator amount, the optimized membrane displays ultrahigh water permeance of 206.7 L m−2 h−1 bar−1 and dye rejections over 98.5%. Furthermore, the resultant membranes exhibit resistance against broad-spectrum oil-in-water emulsions. Our study can pave a facile and prospective way to fabricating high-performance two-dimensional laminated membranes. Graphene oxide (GO) membranes hold great promise in molecular separation owing to the ultrathin thickness as well as precisely controllable interlayer distance. However, the tortuous mass transport pathway along stacked nanosheets hinders the availability of high-flux GO membranes. Herein, we design multi-pathway GO membranes to afford fast water transport through in-plane and interlayer pathways. The in-plane pathway is introduced by the porous GO (pGO) nanosheets and the interlayer pathway is enlarged by intercalating hydrophilic halloysite nanotubes (HNTs) into adjacent pGO nanosheets, jointly contributing to the enhanced water permeance. Through manipulating the intercalator amount, the optimized membrane displays ultrahigh water permeance of 206.7 L m−2 h−1 bar−1 and dye rejections over 98.5%. Furthermore, the resultant membranes exhibit resistance against broad-spectrum oil-in-water emulsions. Our study can pave a facile and prospective way to fabricating high-performance two-dimensional laminated membranes. Multiple mass transport pathways Elsevier Ultrafast water transport Elsevier Graphene oxide membrane Elsevier Acid etching Elsevier Halloysite nanotube intercalating Elsevier You, Xinda oth Shi, Benbing oth Liu, Yanan oth Yuan, Jinqiu oth Yang, Chao oth Pang, Xiao oth Wu, Hong oth Shen, Jianliang oth Fan, Chunyang oth Long, Mengying oth Zhang, Runnan oth Jiang, Zhongyi oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:638 year:2021 day:15 month:11 pages:0 https://doi.org/10.1016/j.memsci.2021.119706 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 638 2021 15 1115 0 |
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10.1016/j.memsci.2021.119706 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001500.pica (DE-627)ELV055068766 (ELSEVIER)S0376-7388(21)00652-9 DE-627 ger DE-627 rakwb eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Guan, Jingyuan verfasserin aut Engineering multi-pathway graphene oxide membranes toward ultrafast water purification 2021transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Graphene oxide (GO) membranes hold great promise in molecular separation owing to the ultrathin thickness as well as precisely controllable interlayer distance. However, the tortuous mass transport pathway along stacked nanosheets hinders the availability of high-flux GO membranes. Herein, we design multi-pathway GO membranes to afford fast water transport through in-plane and interlayer pathways. The in-plane pathway is introduced by the porous GO (pGO) nanosheets and the interlayer pathway is enlarged by intercalating hydrophilic halloysite nanotubes (HNTs) into adjacent pGO nanosheets, jointly contributing to the enhanced water permeance. Through manipulating the intercalator amount, the optimized membrane displays ultrahigh water permeance of 206.7 L m−2 h−1 bar−1 and dye rejections over 98.5%. Furthermore, the resultant membranes exhibit resistance against broad-spectrum oil-in-water emulsions. Our study can pave a facile and prospective way to fabricating high-performance two-dimensional laminated membranes. Graphene oxide (GO) membranes hold great promise in molecular separation owing to the ultrathin thickness as well as precisely controllable interlayer distance. However, the tortuous mass transport pathway along stacked nanosheets hinders the availability of high-flux GO membranes. Herein, we design multi-pathway GO membranes to afford fast water transport through in-plane and interlayer pathways. The in-plane pathway is introduced by the porous GO (pGO) nanosheets and the interlayer pathway is enlarged by intercalating hydrophilic halloysite nanotubes (HNTs) into adjacent pGO nanosheets, jointly contributing to the enhanced water permeance. Through manipulating the intercalator amount, the optimized membrane displays ultrahigh water permeance of 206.7 L m−2 h−1 bar−1 and dye rejections over 98.5%. Furthermore, the resultant membranes exhibit resistance against broad-spectrum oil-in-water emulsions. Our study can pave a facile and prospective way to fabricating high-performance two-dimensional laminated membranes. Multiple mass transport pathways Elsevier Ultrafast water transport Elsevier Graphene oxide membrane Elsevier Acid etching Elsevier Halloysite nanotube intercalating Elsevier You, Xinda oth Shi, Benbing oth Liu, Yanan oth Yuan, Jinqiu oth Yang, Chao oth Pang, Xiao oth Wu, Hong oth Shen, Jianliang oth Fan, Chunyang oth Long, Mengying oth Zhang, Runnan oth Jiang, Zhongyi oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:638 year:2021 day:15 month:11 pages:0 https://doi.org/10.1016/j.memsci.2021.119706 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 638 2021 15 1115 0 |
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Graphene oxide (GO) membranes hold great promise in molecular separation owing to the ultrathin thickness as well as precisely controllable interlayer distance. However, the tortuous mass transport pathway along stacked nanosheets hinders the availability of high-flux GO membranes. Herein, we design multi-pathway GO membranes to afford fast water transport through in-plane and interlayer pathways. The in-plane pathway is introduced by the porous GO (pGO) nanosheets and the interlayer pathway is enlarged by intercalating hydrophilic halloysite nanotubes (HNTs) into adjacent pGO nanosheets, jointly contributing to the enhanced water permeance. Through manipulating the intercalator amount, the optimized membrane displays ultrahigh water permeance of 206.7 L m−2 h−1 bar−1 and dye rejections over 98.5%. Furthermore, the resultant membranes exhibit resistance against broad-spectrum oil-in-water emulsions. Our study can pave a facile and prospective way to fabricating high-performance two-dimensional laminated membranes. |
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Graphene oxide (GO) membranes hold great promise in molecular separation owing to the ultrathin thickness as well as precisely controllable interlayer distance. However, the tortuous mass transport pathway along stacked nanosheets hinders the availability of high-flux GO membranes. Herein, we design multi-pathway GO membranes to afford fast water transport through in-plane and interlayer pathways. The in-plane pathway is introduced by the porous GO (pGO) nanosheets and the interlayer pathway is enlarged by intercalating hydrophilic halloysite nanotubes (HNTs) into adjacent pGO nanosheets, jointly contributing to the enhanced water permeance. Through manipulating the intercalator amount, the optimized membrane displays ultrahigh water permeance of 206.7 L m−2 h−1 bar−1 and dye rejections over 98.5%. Furthermore, the resultant membranes exhibit resistance against broad-spectrum oil-in-water emulsions. Our study can pave a facile and prospective way to fabricating high-performance two-dimensional laminated membranes. |
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Graphene oxide (GO) membranes hold great promise in molecular separation owing to the ultrathin thickness as well as precisely controllable interlayer distance. However, the tortuous mass transport pathway along stacked nanosheets hinders the availability of high-flux GO membranes. Herein, we design multi-pathway GO membranes to afford fast water transport through in-plane and interlayer pathways. The in-plane pathway is introduced by the porous GO (pGO) nanosheets and the interlayer pathway is enlarged by intercalating hydrophilic halloysite nanotubes (HNTs) into adjacent pGO nanosheets, jointly contributing to the enhanced water permeance. Through manipulating the intercalator amount, the optimized membrane displays ultrahigh water permeance of 206.7 L m−2 h−1 bar−1 and dye rejections over 98.5%. Furthermore, the resultant membranes exhibit resistance against broad-spectrum oil-in-water emulsions. Our study can pave a facile and prospective way to fabricating high-performance two-dimensional laminated membranes. |
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