Excellent electromagnetic wave absorption of MOF/SiBCN nanomaterials at high temperature
Electromagnetic wave absorbing materials at high-temperature are urgently needed for stealth aircrafts or aero-engines worked in harsh environments. In this contribution, cobalt-containing siliconboron carbonitride (MOF/SiBCN) nanomaterials were prepared by pyrolyzing metal–organic framework, i.e. c...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
LUO, Chunjia [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2021transfer abstract |
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| Schlagwörter: |
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| Umfang: |
15 |
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| Übergeordnetes Werk: |
Enthalten in: Computable convergence bounds of series expansions for infinite dimensional linear-analytic systems and application - Hélie, Thomas ELSEVIER, 2014transfer abstract, Amsterdam [u.a.] |
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| Übergeordnetes Werk: |
volume:34 ; year:2021 ; number:11 ; pages:277-291 ; extent:15 |
| Links: |
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| DOI / URN: |
10.1016/j.cja.2020.06.028 |
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| 520 | |a Electromagnetic wave absorbing materials at high-temperature are urgently needed for stealth aircrafts or aero-engines worked in harsh environments. In this contribution, cobalt-containing siliconboron carbonitride (MOF/SiBCN) nanomaterials were prepared by pyrolyzing metal–organic framework, i.e. cobalt 2-methylimidazole (ZIF-67), and hyperbranched polyborosilazane. The rhombic dodecahedral ZIF-67 and cobalt element promoted in situ formation of dielectric loss phases, including SiC nanocrystals, CoSi nanocrystals and turbostratic carbons. The ZIF-67/SiBCN nanomaterials showed excellent microwave absorption both at room and elevated temperature. The minimum reflection coefficient (RCmin) was −51.6 dB and effective absorption bandwidth (EAB) is 3.93 GHz at room temperature. At an elevated temperature of 600 °C, the RCmin reached −30.29 dB and EAB covered almost the whole X-band (3.95 GHz, 8.45–12.4 GHz). The ZIF-67/SiBCN nanocomposites are promising and useful platform for microwave absorbing materials at high-temperature. It may shed light on the downstream applications in designing next generation areo-engines and stealth aircrafts. | ||
| 520 | |a Electromagnetic wave absorbing materials at high-temperature are urgently needed for stealth aircrafts or aero-engines worked in harsh environments. In this contribution, cobalt-containing siliconboron carbonitride (MOF/SiBCN) nanomaterials were prepared by pyrolyzing metal–organic framework, i.e. cobalt 2-methylimidazole (ZIF-67), and hyperbranched polyborosilazane. The rhombic dodecahedral ZIF-67 and cobalt element promoted in situ formation of dielectric loss phases, including SiC nanocrystals, CoSi nanocrystals and turbostratic carbons. The ZIF-67/SiBCN nanomaterials showed excellent microwave absorption both at room and elevated temperature. The minimum reflection coefficient (RCmin) was −51.6 dB and effective absorption bandwidth (EAB) is 3.93 GHz at room temperature. At an elevated temperature of 600 °C, the RCmin reached −30.29 dB and EAB covered almost the whole X-band (3.95 GHz, 8.45–12.4 GHz). The ZIF-67/SiBCN nanocomposites are promising and useful platform for microwave absorbing materials at high-temperature. It may shed light on the downstream applications in designing next generation areo-engines and stealth aircrafts. | ||
| 650 | 7 | |a Electromagnetic wave absorption |2 Elsevier | |
| 650 | 7 | |a Polymer-derived ceramics |2 Elsevier | |
| 650 | 7 | |a High temperature resistance |2 Elsevier | |
| 650 | 7 | |a Metal-organic framework |2 Elsevier | |
| 650 | 7 | |a Siliconboron carbonitride |2 Elsevier | |
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| 700 | 1 | |a TANG, Yusheng |4 oth | |
| 700 | 1 | |a KONG, Jie |4 oth | |
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10.1016/j.cja.2020.06.028 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001541.pica (DE-627)ELV055157440 (ELSEVIER)S1000-9361(20)30317-4 DE-627 ger DE-627 rakwb eng 000 VZ 620 VZ 610 VZ 44.48 bkl LUO, Chunjia verfasserin aut Excellent electromagnetic wave absorption of MOF/SiBCN nanomaterials at high temperature 2021transfer abstract 15 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Electromagnetic wave absorbing materials at high-temperature are urgently needed for stealth aircrafts or aero-engines worked in harsh environments. In this contribution, cobalt-containing siliconboron carbonitride (MOF/SiBCN) nanomaterials were prepared by pyrolyzing metal–organic framework, i.e. cobalt 2-methylimidazole (ZIF-67), and hyperbranched polyborosilazane. The rhombic dodecahedral ZIF-67 and cobalt element promoted in situ formation of dielectric loss phases, including SiC nanocrystals, CoSi nanocrystals and turbostratic carbons. The ZIF-67/SiBCN nanomaterials showed excellent microwave absorption both at room and elevated temperature. The minimum reflection coefficient (RCmin) was −51.6 dB and effective absorption bandwidth (EAB) is 3.93 GHz at room temperature. At an elevated temperature of 600 °C, the RCmin reached −30.29 dB and EAB covered almost the whole X-band (3.95 GHz, 8.45–12.4 GHz). The ZIF-67/SiBCN nanocomposites are promising and useful platform for microwave absorbing materials at high-temperature. It may shed light on the downstream applications in designing next generation areo-engines and stealth aircrafts. Electromagnetic wave absorbing materials at high-temperature are urgently needed for stealth aircrafts or aero-engines worked in harsh environments. In this contribution, cobalt-containing siliconboron carbonitride (MOF/SiBCN) nanomaterials were prepared by pyrolyzing metal–organic framework, i.e. cobalt 2-methylimidazole (ZIF-67), and hyperbranched polyborosilazane. The rhombic dodecahedral ZIF-67 and cobalt element promoted in situ formation of dielectric loss phases, including SiC nanocrystals, CoSi nanocrystals and turbostratic carbons. The ZIF-67/SiBCN nanomaterials showed excellent microwave absorption both at room and elevated temperature. The minimum reflection coefficient (RCmin) was −51.6 dB and effective absorption bandwidth (EAB) is 3.93 GHz at room temperature. At an elevated temperature of 600 °C, the RCmin reached −30.29 dB and EAB covered almost the whole X-band (3.95 GHz, 8.45–12.4 GHz). The ZIF-67/SiBCN nanocomposites are promising and useful platform for microwave absorbing materials at high-temperature. It may shed light on the downstream applications in designing next generation areo-engines and stealth aircrafts. Electromagnetic wave absorption Elsevier Polymer-derived ceramics Elsevier High temperature resistance Elsevier Metal-organic framework Elsevier Siliconboron carbonitride Elsevier MIAO, Peng oth TANG, Yusheng oth KONG, Jie oth Enthalten in Elsevier Hélie, Thomas ELSEVIER Computable convergence bounds of series expansions for infinite dimensional linear-analytic systems and application 2014transfer abstract Amsterdam [u.a.] (DE-627)ELV017935458 volume:34 year:2021 number:11 pages:277-291 extent:15 https://doi.org/10.1016/j.cja.2020.06.028 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_63 GBV_ILN_70 44.48 Medizinische Genetik VZ AR 34 2021 11 277-291 15 |
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10.1016/j.cja.2020.06.028 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001541.pica (DE-627)ELV055157440 (ELSEVIER)S1000-9361(20)30317-4 DE-627 ger DE-627 rakwb eng 000 VZ 620 VZ 610 VZ 44.48 bkl LUO, Chunjia verfasserin aut Excellent electromagnetic wave absorption of MOF/SiBCN nanomaterials at high temperature 2021transfer abstract 15 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Electromagnetic wave absorbing materials at high-temperature are urgently needed for stealth aircrafts or aero-engines worked in harsh environments. In this contribution, cobalt-containing siliconboron carbonitride (MOF/SiBCN) nanomaterials were prepared by pyrolyzing metal–organic framework, i.e. cobalt 2-methylimidazole (ZIF-67), and hyperbranched polyborosilazane. The rhombic dodecahedral ZIF-67 and cobalt element promoted in situ formation of dielectric loss phases, including SiC nanocrystals, CoSi nanocrystals and turbostratic carbons. The ZIF-67/SiBCN nanomaterials showed excellent microwave absorption both at room and elevated temperature. The minimum reflection coefficient (RCmin) was −51.6 dB and effective absorption bandwidth (EAB) is 3.93 GHz at room temperature. At an elevated temperature of 600 °C, the RCmin reached −30.29 dB and EAB covered almost the whole X-band (3.95 GHz, 8.45–12.4 GHz). The ZIF-67/SiBCN nanocomposites are promising and useful platform for microwave absorbing materials at high-temperature. It may shed light on the downstream applications in designing next generation areo-engines and stealth aircrafts. Electromagnetic wave absorbing materials at high-temperature are urgently needed for stealth aircrafts or aero-engines worked in harsh environments. In this contribution, cobalt-containing siliconboron carbonitride (MOF/SiBCN) nanomaterials were prepared by pyrolyzing metal–organic framework, i.e. cobalt 2-methylimidazole (ZIF-67), and hyperbranched polyborosilazane. The rhombic dodecahedral ZIF-67 and cobalt element promoted in situ formation of dielectric loss phases, including SiC nanocrystals, CoSi nanocrystals and turbostratic carbons. The ZIF-67/SiBCN nanomaterials showed excellent microwave absorption both at room and elevated temperature. The minimum reflection coefficient (RCmin) was −51.6 dB and effective absorption bandwidth (EAB) is 3.93 GHz at room temperature. At an elevated temperature of 600 °C, the RCmin reached −30.29 dB and EAB covered almost the whole X-band (3.95 GHz, 8.45–12.4 GHz). The ZIF-67/SiBCN nanocomposites are promising and useful platform for microwave absorbing materials at high-temperature. It may shed light on the downstream applications in designing next generation areo-engines and stealth aircrafts. Electromagnetic wave absorption Elsevier Polymer-derived ceramics Elsevier High temperature resistance Elsevier Metal-organic framework Elsevier Siliconboron carbonitride Elsevier MIAO, Peng oth TANG, Yusheng oth KONG, Jie oth Enthalten in Elsevier Hélie, Thomas ELSEVIER Computable convergence bounds of series expansions for infinite dimensional linear-analytic systems and application 2014transfer abstract Amsterdam [u.a.] (DE-627)ELV017935458 volume:34 year:2021 number:11 pages:277-291 extent:15 https://doi.org/10.1016/j.cja.2020.06.028 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_63 GBV_ILN_70 44.48 Medizinische Genetik VZ AR 34 2021 11 277-291 15 |
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10.1016/j.cja.2020.06.028 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001541.pica (DE-627)ELV055157440 (ELSEVIER)S1000-9361(20)30317-4 DE-627 ger DE-627 rakwb eng 000 VZ 620 VZ 610 VZ 44.48 bkl LUO, Chunjia verfasserin aut Excellent electromagnetic wave absorption of MOF/SiBCN nanomaterials at high temperature 2021transfer abstract 15 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Electromagnetic wave absorbing materials at high-temperature are urgently needed for stealth aircrafts or aero-engines worked in harsh environments. In this contribution, cobalt-containing siliconboron carbonitride (MOF/SiBCN) nanomaterials were prepared by pyrolyzing metal–organic framework, i.e. cobalt 2-methylimidazole (ZIF-67), and hyperbranched polyborosilazane. The rhombic dodecahedral ZIF-67 and cobalt element promoted in situ formation of dielectric loss phases, including SiC nanocrystals, CoSi nanocrystals and turbostratic carbons. The ZIF-67/SiBCN nanomaterials showed excellent microwave absorption both at room and elevated temperature. The minimum reflection coefficient (RCmin) was −51.6 dB and effective absorption bandwidth (EAB) is 3.93 GHz at room temperature. At an elevated temperature of 600 °C, the RCmin reached −30.29 dB and EAB covered almost the whole X-band (3.95 GHz, 8.45–12.4 GHz). The ZIF-67/SiBCN nanocomposites are promising and useful platform for microwave absorbing materials at high-temperature. It may shed light on the downstream applications in designing next generation areo-engines and stealth aircrafts. Electromagnetic wave absorbing materials at high-temperature are urgently needed for stealth aircrafts or aero-engines worked in harsh environments. In this contribution, cobalt-containing siliconboron carbonitride (MOF/SiBCN) nanomaterials were prepared by pyrolyzing metal–organic framework, i.e. cobalt 2-methylimidazole (ZIF-67), and hyperbranched polyborosilazane. The rhombic dodecahedral ZIF-67 and cobalt element promoted in situ formation of dielectric loss phases, including SiC nanocrystals, CoSi nanocrystals and turbostratic carbons. The ZIF-67/SiBCN nanomaterials showed excellent microwave absorption both at room and elevated temperature. The minimum reflection coefficient (RCmin) was −51.6 dB and effective absorption bandwidth (EAB) is 3.93 GHz at room temperature. At an elevated temperature of 600 °C, the RCmin reached −30.29 dB and EAB covered almost the whole X-band (3.95 GHz, 8.45–12.4 GHz). The ZIF-67/SiBCN nanocomposites are promising and useful platform for microwave absorbing materials at high-temperature. It may shed light on the downstream applications in designing next generation areo-engines and stealth aircrafts. Electromagnetic wave absorption Elsevier Polymer-derived ceramics Elsevier High temperature resistance Elsevier Metal-organic framework Elsevier Siliconboron carbonitride Elsevier MIAO, Peng oth TANG, Yusheng oth KONG, Jie oth Enthalten in Elsevier Hélie, Thomas ELSEVIER Computable convergence bounds of series expansions for infinite dimensional linear-analytic systems and application 2014transfer abstract Amsterdam [u.a.] (DE-627)ELV017935458 volume:34 year:2021 number:11 pages:277-291 extent:15 https://doi.org/10.1016/j.cja.2020.06.028 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_63 GBV_ILN_70 44.48 Medizinische Genetik VZ AR 34 2021 11 277-291 15 |
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10.1016/j.cja.2020.06.028 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001541.pica (DE-627)ELV055157440 (ELSEVIER)S1000-9361(20)30317-4 DE-627 ger DE-627 rakwb eng 000 VZ 620 VZ 610 VZ 44.48 bkl LUO, Chunjia verfasserin aut Excellent electromagnetic wave absorption of MOF/SiBCN nanomaterials at high temperature 2021transfer abstract 15 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Electromagnetic wave absorbing materials at high-temperature are urgently needed for stealth aircrafts or aero-engines worked in harsh environments. In this contribution, cobalt-containing siliconboron carbonitride (MOF/SiBCN) nanomaterials were prepared by pyrolyzing metal–organic framework, i.e. cobalt 2-methylimidazole (ZIF-67), and hyperbranched polyborosilazane. The rhombic dodecahedral ZIF-67 and cobalt element promoted in situ formation of dielectric loss phases, including SiC nanocrystals, CoSi nanocrystals and turbostratic carbons. The ZIF-67/SiBCN nanomaterials showed excellent microwave absorption both at room and elevated temperature. The minimum reflection coefficient (RCmin) was −51.6 dB and effective absorption bandwidth (EAB) is 3.93 GHz at room temperature. At an elevated temperature of 600 °C, the RCmin reached −30.29 dB and EAB covered almost the whole X-band (3.95 GHz, 8.45–12.4 GHz). The ZIF-67/SiBCN nanocomposites are promising and useful platform for microwave absorbing materials at high-temperature. It may shed light on the downstream applications in designing next generation areo-engines and stealth aircrafts. Electromagnetic wave absorbing materials at high-temperature are urgently needed for stealth aircrafts or aero-engines worked in harsh environments. In this contribution, cobalt-containing siliconboron carbonitride (MOF/SiBCN) nanomaterials were prepared by pyrolyzing metal–organic framework, i.e. cobalt 2-methylimidazole (ZIF-67), and hyperbranched polyborosilazane. The rhombic dodecahedral ZIF-67 and cobalt element promoted in situ formation of dielectric loss phases, including SiC nanocrystals, CoSi nanocrystals and turbostratic carbons. The ZIF-67/SiBCN nanomaterials showed excellent microwave absorption both at room and elevated temperature. The minimum reflection coefficient (RCmin) was −51.6 dB and effective absorption bandwidth (EAB) is 3.93 GHz at room temperature. At an elevated temperature of 600 °C, the RCmin reached −30.29 dB and EAB covered almost the whole X-band (3.95 GHz, 8.45–12.4 GHz). The ZIF-67/SiBCN nanocomposites are promising and useful platform for microwave absorbing materials at high-temperature. It may shed light on the downstream applications in designing next generation areo-engines and stealth aircrafts. Electromagnetic wave absorption Elsevier Polymer-derived ceramics Elsevier High temperature resistance Elsevier Metal-organic framework Elsevier Siliconboron carbonitride Elsevier MIAO, Peng oth TANG, Yusheng oth KONG, Jie oth Enthalten in Elsevier Hélie, Thomas ELSEVIER Computable convergence bounds of series expansions for infinite dimensional linear-analytic systems and application 2014transfer abstract Amsterdam [u.a.] (DE-627)ELV017935458 volume:34 year:2021 number:11 pages:277-291 extent:15 https://doi.org/10.1016/j.cja.2020.06.028 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_63 GBV_ILN_70 44.48 Medizinische Genetik VZ AR 34 2021 11 277-291 15 |
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10.1016/j.cja.2020.06.028 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001541.pica (DE-627)ELV055157440 (ELSEVIER)S1000-9361(20)30317-4 DE-627 ger DE-627 rakwb eng 000 VZ 620 VZ 610 VZ 44.48 bkl LUO, Chunjia verfasserin aut Excellent electromagnetic wave absorption of MOF/SiBCN nanomaterials at high temperature 2021transfer abstract 15 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Electromagnetic wave absorbing materials at high-temperature are urgently needed for stealth aircrafts or aero-engines worked in harsh environments. In this contribution, cobalt-containing siliconboron carbonitride (MOF/SiBCN) nanomaterials were prepared by pyrolyzing metal–organic framework, i.e. cobalt 2-methylimidazole (ZIF-67), and hyperbranched polyborosilazane. The rhombic dodecahedral ZIF-67 and cobalt element promoted in situ formation of dielectric loss phases, including SiC nanocrystals, CoSi nanocrystals and turbostratic carbons. The ZIF-67/SiBCN nanomaterials showed excellent microwave absorption both at room and elevated temperature. The minimum reflection coefficient (RCmin) was −51.6 dB and effective absorption bandwidth (EAB) is 3.93 GHz at room temperature. At an elevated temperature of 600 °C, the RCmin reached −30.29 dB and EAB covered almost the whole X-band (3.95 GHz, 8.45–12.4 GHz). The ZIF-67/SiBCN nanocomposites are promising and useful platform for microwave absorbing materials at high-temperature. It may shed light on the downstream applications in designing next generation areo-engines and stealth aircrafts. Electromagnetic wave absorbing materials at high-temperature are urgently needed for stealth aircrafts or aero-engines worked in harsh environments. In this contribution, cobalt-containing siliconboron carbonitride (MOF/SiBCN) nanomaterials were prepared by pyrolyzing metal–organic framework, i.e. cobalt 2-methylimidazole (ZIF-67), and hyperbranched polyborosilazane. The rhombic dodecahedral ZIF-67 and cobalt element promoted in situ formation of dielectric loss phases, including SiC nanocrystals, CoSi nanocrystals and turbostratic carbons. The ZIF-67/SiBCN nanomaterials showed excellent microwave absorption both at room and elevated temperature. The minimum reflection coefficient (RCmin) was −51.6 dB and effective absorption bandwidth (EAB) is 3.93 GHz at room temperature. At an elevated temperature of 600 °C, the RCmin reached −30.29 dB and EAB covered almost the whole X-band (3.95 GHz, 8.45–12.4 GHz). The ZIF-67/SiBCN nanocomposites are promising and useful platform for microwave absorbing materials at high-temperature. It may shed light on the downstream applications in designing next generation areo-engines and stealth aircrafts. Electromagnetic wave absorption Elsevier Polymer-derived ceramics Elsevier High temperature resistance Elsevier Metal-organic framework Elsevier Siliconboron carbonitride Elsevier MIAO, Peng oth TANG, Yusheng oth KONG, Jie oth Enthalten in Elsevier Hélie, Thomas ELSEVIER Computable convergence bounds of series expansions for infinite dimensional linear-analytic systems and application 2014transfer abstract Amsterdam [u.a.] (DE-627)ELV017935458 volume:34 year:2021 number:11 pages:277-291 extent:15 https://doi.org/10.1016/j.cja.2020.06.028 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_63 GBV_ILN_70 44.48 Medizinische Genetik VZ AR 34 2021 11 277-291 15 |
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Enthalten in Computable convergence bounds of series expansions for infinite dimensional linear-analytic systems and application Amsterdam [u.a.] volume:34 year:2021 number:11 pages:277-291 extent:15 |
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Enthalten in Computable convergence bounds of series expansions for infinite dimensional linear-analytic systems and application Amsterdam [u.a.] volume:34 year:2021 number:11 pages:277-291 extent:15 |
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Excellent electromagnetic wave absorption of MOF/SiBCN nanomaterials at high temperature |
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Electromagnetic wave absorbing materials at high-temperature are urgently needed for stealth aircrafts or aero-engines worked in harsh environments. In this contribution, cobalt-containing siliconboron carbonitride (MOF/SiBCN) nanomaterials were prepared by pyrolyzing metal–organic framework, i.e. cobalt 2-methylimidazole (ZIF-67), and hyperbranched polyborosilazane. The rhombic dodecahedral ZIF-67 and cobalt element promoted in situ formation of dielectric loss phases, including SiC nanocrystals, CoSi nanocrystals and turbostratic carbons. The ZIF-67/SiBCN nanomaterials showed excellent microwave absorption both at room and elevated temperature. The minimum reflection coefficient (RCmin) was −51.6 dB and effective absorption bandwidth (EAB) is 3.93 GHz at room temperature. At an elevated temperature of 600 °C, the RCmin reached −30.29 dB and EAB covered almost the whole X-band (3.95 GHz, 8.45–12.4 GHz). The ZIF-67/SiBCN nanocomposites are promising and useful platform for microwave absorbing materials at high-temperature. It may shed light on the downstream applications in designing next generation areo-engines and stealth aircrafts. |
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Electromagnetic wave absorbing materials at high-temperature are urgently needed for stealth aircrafts or aero-engines worked in harsh environments. In this contribution, cobalt-containing siliconboron carbonitride (MOF/SiBCN) nanomaterials were prepared by pyrolyzing metal–organic framework, i.e. cobalt 2-methylimidazole (ZIF-67), and hyperbranched polyborosilazane. The rhombic dodecahedral ZIF-67 and cobalt element promoted in situ formation of dielectric loss phases, including SiC nanocrystals, CoSi nanocrystals and turbostratic carbons. The ZIF-67/SiBCN nanomaterials showed excellent microwave absorption both at room and elevated temperature. The minimum reflection coefficient (RCmin) was −51.6 dB and effective absorption bandwidth (EAB) is 3.93 GHz at room temperature. At an elevated temperature of 600 °C, the RCmin reached −30.29 dB and EAB covered almost the whole X-band (3.95 GHz, 8.45–12.4 GHz). The ZIF-67/SiBCN nanocomposites are promising and useful platform for microwave absorbing materials at high-temperature. It may shed light on the downstream applications in designing next generation areo-engines and stealth aircrafts. |
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Electromagnetic wave absorbing materials at high-temperature are urgently needed for stealth aircrafts or aero-engines worked in harsh environments. In this contribution, cobalt-containing siliconboron carbonitride (MOF/SiBCN) nanomaterials were prepared by pyrolyzing metal–organic framework, i.e. cobalt 2-methylimidazole (ZIF-67), and hyperbranched polyborosilazane. The rhombic dodecahedral ZIF-67 and cobalt element promoted in situ formation of dielectric loss phases, including SiC nanocrystals, CoSi nanocrystals and turbostratic carbons. The ZIF-67/SiBCN nanomaterials showed excellent microwave absorption both at room and elevated temperature. The minimum reflection coefficient (RCmin) was −51.6 dB and effective absorption bandwidth (EAB) is 3.93 GHz at room temperature. At an elevated temperature of 600 °C, the RCmin reached −30.29 dB and EAB covered almost the whole X-band (3.95 GHz, 8.45–12.4 GHz). The ZIF-67/SiBCN nanocomposites are promising and useful platform for microwave absorbing materials at high-temperature. It may shed light on the downstream applications in designing next generation areo-engines and stealth aircrafts. |
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