Co-pyrolysis of pine sawdust with aluminum dross for immobilization of heavy metal and enhancing hydrogen generation

Co-pyrolysis of pine sawdust with aluminum dross (AD) for harvesting energy product and safely treated AD-biochar composite was investigated in this work. The catalytic pyrolysis experiment was carried out in a fixed bed reactor. The pyrolysis products were analyzed by gas chromatography (GC), gas c...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Liu, Peng [verfasserIn] Liu, Li [verfasserIn] Zhou, Zhengzhong [verfasserIn] Li, Yanling [verfasserIn] Yuan, Haoran [verfasserIn] Huhetaoli [verfasserIn] Lei, Tingzhou [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2021

Schlagwörter:	Aluminum dross Biomass pyrolysis Intermediate hybrid Hydrogen generation Carbon structure

Übergeordnetes Werk:	Enthalten in: Fuel - New York, NY [u.a.] : Elsevier, 1970, 305
Übergeordnetes Werk:	volume:305

DOI / URN:	10.1016/j.fuel.2021.121597

Katalog-ID:	ELV055350062

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520			\|a Co-pyrolysis of pine sawdust with aluminum dross (AD) for harvesting energy product and safely treated AD-biochar composite was investigated in this work. The catalytic pyrolysis experiment was carried out in a fixed bed reactor. The pyrolysis products were analyzed by gas chromatography (GC), gas chromatography coupled with a mass spectrometer (GC–MS), and solid C-13 Nuclear Magnetic Resonance (13C NMR). The results show that the heavy metals, such as Cu, were immobilized by organic metal-chelating structures as carbon–oxygen-metal (C–O–M) bonds in the AD-biochar composite. In addition, the hydrogen yield from catalytic pyrolysis of pine on AD reaches 131.86 ml/g, significantly higher than the 98.97 ml/g from pure pine pyrolysis. The enhanced hydrogen production is elaborated by the intermediate hybrid mechanism with formation of C–O–M intermediates between the metallic oxides in AD and the oxygen containing functional groups in biomass. Meanwhile, the CO2 yield decreases from 23.68 ml/g to 16.41 ml/g while the CO yield reduces from 49.72 ml/g to 46.85 ml/g. These results may guide to a new exploration on simultaneous treatment of hazardous industrial wastes and utilization of biomass.
650		4	\|a Aluminum dross
650		4	\|a Biomass pyrolysis
650		4	\|a Intermediate hybrid
650		4	\|a Hydrogen generation
650		4	\|a Carbon structure
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700	1		\|a Huhetaoli \|e verfasserin \|4 aut
700	1		\|a Lei, Tingzhou \|e verfasserin \|4 aut
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publishDate	2021
allfields	10.1016/j.fuel.2021.121597 doi (DE-627)ELV055350062 (ELSEVIER)S0016-2361(21)01478-2 DE-627 ger DE-627 rda eng 660 VZ 58.21 bkl Liu, Peng verfasserin aut Co-pyrolysis of pine sawdust with aluminum dross for immobilization of heavy metal and enhancing hydrogen generation 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Co-pyrolysis of pine sawdust with aluminum dross (AD) for harvesting energy product and safely treated AD-biochar composite was investigated in this work. The catalytic pyrolysis experiment was carried out in a fixed bed reactor. The pyrolysis products were analyzed by gas chromatography (GC), gas chromatography coupled with a mass spectrometer (GC–MS), and solid C-13 Nuclear Magnetic Resonance (13C NMR). The results show that the heavy metals, such as Cu, were immobilized by organic metal-chelating structures as carbon–oxygen-metal (C–O–M) bonds in the AD-biochar composite. In addition, the hydrogen yield from catalytic pyrolysis of pine on AD reaches 131.86 ml/g, significantly higher than the 98.97 ml/g from pure pine pyrolysis. The enhanced hydrogen production is elaborated by the intermediate hybrid mechanism with formation of C–O–M intermediates between the metallic oxides in AD and the oxygen containing functional groups in biomass. Meanwhile, the CO2 yield decreases from 23.68 ml/g to 16.41 ml/g while the CO yield reduces from 49.72 ml/g to 46.85 ml/g. These results may guide to a new exploration on simultaneous treatment of hazardous industrial wastes and utilization of biomass. Aluminum dross Biomass pyrolysis Intermediate hybrid Hydrogen generation Carbon structure Liu, Li verfasserin aut Zhou, Zhengzhong verfasserin aut Li, Yanling verfasserin aut Yuan, Haoran verfasserin aut Huhetaoli verfasserin aut Lei, Tingzhou verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 305 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:305 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe VZ AR 305
spelling	10.1016/j.fuel.2021.121597 doi (DE-627)ELV055350062 (ELSEVIER)S0016-2361(21)01478-2 DE-627 ger DE-627 rda eng 660 VZ 58.21 bkl Liu, Peng verfasserin aut Co-pyrolysis of pine sawdust with aluminum dross for immobilization of heavy metal and enhancing hydrogen generation 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Co-pyrolysis of pine sawdust with aluminum dross (AD) for harvesting energy product and safely treated AD-biochar composite was investigated in this work. The catalytic pyrolysis experiment was carried out in a fixed bed reactor. The pyrolysis products were analyzed by gas chromatography (GC), gas chromatography coupled with a mass spectrometer (GC–MS), and solid C-13 Nuclear Magnetic Resonance (13C NMR). The results show that the heavy metals, such as Cu, were immobilized by organic metal-chelating structures as carbon–oxygen-metal (C–O–M) bonds in the AD-biochar composite. In addition, the hydrogen yield from catalytic pyrolysis of pine on AD reaches 131.86 ml/g, significantly higher than the 98.97 ml/g from pure pine pyrolysis. The enhanced hydrogen production is elaborated by the intermediate hybrid mechanism with formation of C–O–M intermediates between the metallic oxides in AD and the oxygen containing functional groups in biomass. Meanwhile, the CO2 yield decreases from 23.68 ml/g to 16.41 ml/g while the CO yield reduces from 49.72 ml/g to 46.85 ml/g. These results may guide to a new exploration on simultaneous treatment of hazardous industrial wastes and utilization of biomass. Aluminum dross Biomass pyrolysis Intermediate hybrid Hydrogen generation Carbon structure Liu, Li verfasserin aut Zhou, Zhengzhong verfasserin aut Li, Yanling verfasserin aut Yuan, Haoran verfasserin aut Huhetaoli verfasserin aut Lei, Tingzhou verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 305 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:305 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe VZ AR 305
allfields_unstemmed	10.1016/j.fuel.2021.121597 doi (DE-627)ELV055350062 (ELSEVIER)S0016-2361(21)01478-2 DE-627 ger DE-627 rda eng 660 VZ 58.21 bkl Liu, Peng verfasserin aut Co-pyrolysis of pine sawdust with aluminum dross for immobilization of heavy metal and enhancing hydrogen generation 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Co-pyrolysis of pine sawdust with aluminum dross (AD) for harvesting energy product and safely treated AD-biochar composite was investigated in this work. The catalytic pyrolysis experiment was carried out in a fixed bed reactor. The pyrolysis products were analyzed by gas chromatography (GC), gas chromatography coupled with a mass spectrometer (GC–MS), and solid C-13 Nuclear Magnetic Resonance (13C NMR). The results show that the heavy metals, such as Cu, were immobilized by organic metal-chelating structures as carbon–oxygen-metal (C–O–M) bonds in the AD-biochar composite. In addition, the hydrogen yield from catalytic pyrolysis of pine on AD reaches 131.86 ml/g, significantly higher than the 98.97 ml/g from pure pine pyrolysis. The enhanced hydrogen production is elaborated by the intermediate hybrid mechanism with formation of C–O–M intermediates between the metallic oxides in AD and the oxygen containing functional groups in biomass. Meanwhile, the CO2 yield decreases from 23.68 ml/g to 16.41 ml/g while the CO yield reduces from 49.72 ml/g to 46.85 ml/g. These results may guide to a new exploration on simultaneous treatment of hazardous industrial wastes and utilization of biomass. Aluminum dross Biomass pyrolysis Intermediate hybrid Hydrogen generation Carbon structure Liu, Li verfasserin aut Zhou, Zhengzhong verfasserin aut Li, Yanling verfasserin aut Yuan, Haoran verfasserin aut Huhetaoli verfasserin aut Lei, Tingzhou verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 305 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:305 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe VZ AR 305
allfieldsGer	10.1016/j.fuel.2021.121597 doi (DE-627)ELV055350062 (ELSEVIER)S0016-2361(21)01478-2 DE-627 ger DE-627 rda eng 660 VZ 58.21 bkl Liu, Peng verfasserin aut Co-pyrolysis of pine sawdust with aluminum dross for immobilization of heavy metal and enhancing hydrogen generation 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Co-pyrolysis of pine sawdust with aluminum dross (AD) for harvesting energy product and safely treated AD-biochar composite was investigated in this work. The catalytic pyrolysis experiment was carried out in a fixed bed reactor. The pyrolysis products were analyzed by gas chromatography (GC), gas chromatography coupled with a mass spectrometer (GC–MS), and solid C-13 Nuclear Magnetic Resonance (13C NMR). The results show that the heavy metals, such as Cu, were immobilized by organic metal-chelating structures as carbon–oxygen-metal (C–O–M) bonds in the AD-biochar composite. In addition, the hydrogen yield from catalytic pyrolysis of pine on AD reaches 131.86 ml/g, significantly higher than the 98.97 ml/g from pure pine pyrolysis. The enhanced hydrogen production is elaborated by the intermediate hybrid mechanism with formation of C–O–M intermediates between the metallic oxides in AD and the oxygen containing functional groups in biomass. Meanwhile, the CO2 yield decreases from 23.68 ml/g to 16.41 ml/g while the CO yield reduces from 49.72 ml/g to 46.85 ml/g. These results may guide to a new exploration on simultaneous treatment of hazardous industrial wastes and utilization of biomass. Aluminum dross Biomass pyrolysis Intermediate hybrid Hydrogen generation Carbon structure Liu, Li verfasserin aut Zhou, Zhengzhong verfasserin aut Li, Yanling verfasserin aut Yuan, Haoran verfasserin aut Huhetaoli verfasserin aut Lei, Tingzhou verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 305 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:305 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe VZ AR 305
allfieldsSound	10.1016/j.fuel.2021.121597 doi (DE-627)ELV055350062 (ELSEVIER)S0016-2361(21)01478-2 DE-627 ger DE-627 rda eng 660 VZ 58.21 bkl Liu, Peng verfasserin aut Co-pyrolysis of pine sawdust with aluminum dross for immobilization of heavy metal and enhancing hydrogen generation 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Co-pyrolysis of pine sawdust with aluminum dross (AD) for harvesting energy product and safely treated AD-biochar composite was investigated in this work. The catalytic pyrolysis experiment was carried out in a fixed bed reactor. The pyrolysis products were analyzed by gas chromatography (GC), gas chromatography coupled with a mass spectrometer (GC–MS), and solid C-13 Nuclear Magnetic Resonance (13C NMR). The results show that the heavy metals, such as Cu, were immobilized by organic metal-chelating structures as carbon–oxygen-metal (C–O–M) bonds in the AD-biochar composite. In addition, the hydrogen yield from catalytic pyrolysis of pine on AD reaches 131.86 ml/g, significantly higher than the 98.97 ml/g from pure pine pyrolysis. The enhanced hydrogen production is elaborated by the intermediate hybrid mechanism with formation of C–O–M intermediates between the metallic oxides in AD and the oxygen containing functional groups in biomass. Meanwhile, the CO2 yield decreases from 23.68 ml/g to 16.41 ml/g while the CO yield reduces from 49.72 ml/g to 46.85 ml/g. These results may guide to a new exploration on simultaneous treatment of hazardous industrial wastes and utilization of biomass. Aluminum dross Biomass pyrolysis Intermediate hybrid Hydrogen generation Carbon structure Liu, Li verfasserin aut Zhou, Zhengzhong verfasserin aut Li, Yanling verfasserin aut Yuan, Haoran verfasserin aut Huhetaoli verfasserin aut Lei, Tingzhou verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 305 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:305 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe VZ AR 305
language	English
source	Enthalten in Fuel 305 volume:305
sourceStr	Enthalten in Fuel 305 volume:305
format_phy_str_mv	Article
bklname	Brennstoffe Kraftstoffe Explosivstoffe
institution	findex.gbv.de
topic_facet	Aluminum dross Biomass pyrolysis Intermediate hybrid Hydrogen generation Carbon structure
dewey-raw	660
isfreeaccess_bool	false
container_title	Fuel
authorswithroles_txt_mv	Liu, Peng @@aut@@ Liu, Li @@aut@@ Zhou, Zhengzhong @@aut@@ Li, Yanling @@aut@@ Yuan, Haoran @@aut@@ Huhetaoli @@aut@@ Lei, Tingzhou @@aut@@
publishDateDaySort_date	2021-01-01T00:00:00Z
hierarchy_top_id	300898584
dewey-sort	3660
id	ELV055350062
language_de	englisch
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author	Liu, Peng
spellingShingle	Liu, Peng ddc 660 bkl 58.21 misc Aluminum dross misc Biomass pyrolysis misc Intermediate hybrid misc Hydrogen generation misc Carbon structure Co-pyrolysis of pine sawdust with aluminum dross for immobilization of heavy metal and enhancing hydrogen generation
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topic_title	660 VZ 58.21 bkl Co-pyrolysis of pine sawdust with aluminum dross for immobilization of heavy metal and enhancing hydrogen generation Aluminum dross Biomass pyrolysis Intermediate hybrid Hydrogen generation Carbon structure
topic	ddc 660 bkl 58.21 misc Aluminum dross misc Biomass pyrolysis misc Intermediate hybrid misc Hydrogen generation misc Carbon structure
topic_unstemmed	ddc 660 bkl 58.21 misc Aluminum dross misc Biomass pyrolysis misc Intermediate hybrid misc Hydrogen generation misc Carbon structure
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title	Co-pyrolysis of pine sawdust with aluminum dross for immobilization of heavy metal and enhancing hydrogen generation
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title_full	Co-pyrolysis of pine sawdust with aluminum dross for immobilization of heavy metal and enhancing hydrogen generation
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title_sort	co-pyrolysis of pine sawdust with aluminum dross for immobilization of heavy metal and enhancing hydrogen generation
title_auth	Co-pyrolysis of pine sawdust with aluminum dross for immobilization of heavy metal and enhancing hydrogen generation
abstract	Co-pyrolysis of pine sawdust with aluminum dross (AD) for harvesting energy product and safely treated AD-biochar composite was investigated in this work. The catalytic pyrolysis experiment was carried out in a fixed bed reactor. The pyrolysis products were analyzed by gas chromatography (GC), gas chromatography coupled with a mass spectrometer (GC–MS), and solid C-13 Nuclear Magnetic Resonance (13C NMR). The results show that the heavy metals, such as Cu, were immobilized by organic metal-chelating structures as carbon–oxygen-metal (C–O–M) bonds in the AD-biochar composite. In addition, the hydrogen yield from catalytic pyrolysis of pine on AD reaches 131.86 ml/g, significantly higher than the 98.97 ml/g from pure pine pyrolysis. The enhanced hydrogen production is elaborated by the intermediate hybrid mechanism with formation of C–O–M intermediates between the metallic oxides in AD and the oxygen containing functional groups in biomass. Meanwhile, the CO2 yield decreases from 23.68 ml/g to 16.41 ml/g while the CO yield reduces from 49.72 ml/g to 46.85 ml/g. These results may guide to a new exploration on simultaneous treatment of hazardous industrial wastes and utilization of biomass.
abstractGer	Co-pyrolysis of pine sawdust with aluminum dross (AD) for harvesting energy product and safely treated AD-biochar composite was investigated in this work. The catalytic pyrolysis experiment was carried out in a fixed bed reactor. The pyrolysis products were analyzed by gas chromatography (GC), gas chromatography coupled with a mass spectrometer (GC–MS), and solid C-13 Nuclear Magnetic Resonance (13C NMR). The results show that the heavy metals, such as Cu, were immobilized by organic metal-chelating structures as carbon–oxygen-metal (C–O–M) bonds in the AD-biochar composite. In addition, the hydrogen yield from catalytic pyrolysis of pine on AD reaches 131.86 ml/g, significantly higher than the 98.97 ml/g from pure pine pyrolysis. The enhanced hydrogen production is elaborated by the intermediate hybrid mechanism with formation of C–O–M intermediates between the metallic oxides in AD and the oxygen containing functional groups in biomass. Meanwhile, the CO2 yield decreases from 23.68 ml/g to 16.41 ml/g while the CO yield reduces from 49.72 ml/g to 46.85 ml/g. These results may guide to a new exploration on simultaneous treatment of hazardous industrial wastes and utilization of biomass.
abstract_unstemmed	Co-pyrolysis of pine sawdust with aluminum dross (AD) for harvesting energy product and safely treated AD-biochar composite was investigated in this work. The catalytic pyrolysis experiment was carried out in a fixed bed reactor. The pyrolysis products were analyzed by gas chromatography (GC), gas chromatography coupled with a mass spectrometer (GC–MS), and solid C-13 Nuclear Magnetic Resonance (13C NMR). The results show that the heavy metals, such as Cu, were immobilized by organic metal-chelating structures as carbon–oxygen-metal (C–O–M) bonds in the AD-biochar composite. In addition, the hydrogen yield from catalytic pyrolysis of pine on AD reaches 131.86 ml/g, significantly higher than the 98.97 ml/g from pure pine pyrolysis. The enhanced hydrogen production is elaborated by the intermediate hybrid mechanism with formation of C–O–M intermediates between the metallic oxides in AD and the oxygen containing functional groups in biomass. Meanwhile, the CO2 yield decreases from 23.68 ml/g to 16.41 ml/g while the CO yield reduces from 49.72 ml/g to 46.85 ml/g. These results may guide to a new exploration on simultaneous treatment of hazardous industrial wastes and utilization of biomass.
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title_short	Co-pyrolysis of pine sawdust with aluminum dross for immobilization of heavy metal and enhancing hydrogen generation
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author2	Liu, Li Zhou, Zhengzhong Li, Yanling Yuan, Haoran Huhetaoli Lei, Tingzhou
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doi_str	10.1016/j.fuel.2021.121597
up_date	2024-07-06T17:18:15.003Z
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score	7.398551

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Co-pyrolysis of pine sawdust with aluminum dross for immobilization of heavy metal and enhancing hydrogen generation

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