Volatilization behavior of polycyclic aromatic hydrocarbons from the oil-based residues of shale drill cuttings
Shale gas, an emerging oil-bearing and pillar industry at home and abroad, has a very large impact on economic development and industry, but the resulting emerging pollutants pose a serious threat to the environment. Drilling cuttings, the primary byproduct of the exploration and mining of shale gas...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Wang, Shu [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2022transfer abstract |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: MPI vs Fortran coarrays beyond 100k cores: 3D cellular automata - Shterenlikht, Anton ELSEVIER, 2019, chemistry, biology and toxicology as related to environmental problems, Amsterdam [u.a.] |
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| Übergeordnetes Werk: |
volume:288 ; year:2022 ; pages:0 |
| Links: |
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| DOI / URN: |
10.1016/j.chemosphere.2021.132455 |
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ELV056034245 |
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| 520 | |a Shale gas, an emerging oil-bearing and pillar industry at home and abroad, has a very large impact on economic development and industry, but the resulting emerging pollutants pose a serious threat to the environment. Drilling cuttings, the primary byproduct of the exploration and mining of shale gas, are potentially hazardous types of waste that seriously deplete land resources and pose environmental safety problems. In this paper, a long-term static volatilization experiment was conducted to study the volatilization of polycyclic aromatic hydrocarbons (PAHs) in the oil-based residue of shale gas drill cuttings. Furthermore, the effects of some relevant environmental factors controlling the volatilization behavior were evaluated, including different particle sizes, temperatures and illuminances. The results showed that (1) the volatilization concentrations of PAHs gradually increased with prolonged volatilization time. PAHs with smaller ring numbers were present at the highest concentrations among the detected PAHs, and they were more readily volatilized and could be detected earlier. (2) The C-history method was found to significantly describe the kinetic process of the volatilization of PAHs. (3) Different environmental factors had different effects on the volatilization of PAHs. We found that increasing the temperature and illuminance and decreasing the particle size increased volatility. Through canonical correspondence analysis, PAHs volatilization was found to be a complex process, so volatilization tests under simulated environmental conditions are of scientific and environmental interest. | ||
| 520 | |a Shale gas, an emerging oil-bearing and pillar industry at home and abroad, has a very large impact on economic development and industry, but the resulting emerging pollutants pose a serious threat to the environment. Drilling cuttings, the primary byproduct of the exploration and mining of shale gas, are potentially hazardous types of waste that seriously deplete land resources and pose environmental safety problems. In this paper, a long-term static volatilization experiment was conducted to study the volatilization of polycyclic aromatic hydrocarbons (PAHs) in the oil-based residue of shale gas drill cuttings. Furthermore, the effects of some relevant environmental factors controlling the volatilization behavior were evaluated, including different particle sizes, temperatures and illuminances. The results showed that (1) the volatilization concentrations of PAHs gradually increased with prolonged volatilization time. PAHs with smaller ring numbers were present at the highest concentrations among the detected PAHs, and they were more readily volatilized and could be detected earlier. (2) The C-history method was found to significantly describe the kinetic process of the volatilization of PAHs. (3) Different environmental factors had different effects on the volatilization of PAHs. We found that increasing the temperature and illuminance and decreasing the particle size increased volatility. Through canonical correspondence analysis, PAHs volatilization was found to be a complex process, so volatilization tests under simulated environmental conditions are of scientific and environmental interest. | ||
| 650 | 7 | |a Oil-based residues of shale drill cuttings |2 Elsevier | |
| 650 | 7 | |a Volatilization |2 Elsevier | |
| 650 | 7 | |a C-history method |2 Elsevier | |
| 650 | 7 | |a PAHs |2 Elsevier | |
| 700 | 1 | |a Qin, Jihong |4 oth | |
| 700 | 1 | |a Xie, Bingxin |4 oth | |
| 700 | 1 | |a Sun, Hui |4 oth | |
| 700 | 1 | |a Li, Xin |4 oth | |
| 700 | 1 | |a Chen, Wenqing |4 oth | |
| 773 | 0 | 8 | |i Enthalten in |n Elsevier Science |a Shterenlikht, Anton ELSEVIER |t MPI vs Fortran coarrays beyond 100k cores: 3D cellular automata |d 2019 |d chemistry, biology and toxicology as related to environmental problems |g Amsterdam [u.a.] |w (DE-627)ELV002112701 |
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10.1016/j.chemosphere.2021.132455 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001596.pica (DE-627)ELV056034245 (ELSEVIER)S0045-6535(21)02927-1 DE-627 ger DE-627 rakwb eng 004 620 VZ 54.25 bkl Wang, Shu verfasserin aut Volatilization behavior of polycyclic aromatic hydrocarbons from the oil-based residues of shale drill cuttings 2022transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Shale gas, an emerging oil-bearing and pillar industry at home and abroad, has a very large impact on economic development and industry, but the resulting emerging pollutants pose a serious threat to the environment. Drilling cuttings, the primary byproduct of the exploration and mining of shale gas, are potentially hazardous types of waste that seriously deplete land resources and pose environmental safety problems. In this paper, a long-term static volatilization experiment was conducted to study the volatilization of polycyclic aromatic hydrocarbons (PAHs) in the oil-based residue of shale gas drill cuttings. Furthermore, the effects of some relevant environmental factors controlling the volatilization behavior were evaluated, including different particle sizes, temperatures and illuminances. The results showed that (1) the volatilization concentrations of PAHs gradually increased with prolonged volatilization time. PAHs with smaller ring numbers were present at the highest concentrations among the detected PAHs, and they were more readily volatilized and could be detected earlier. (2) The C-history method was found to significantly describe the kinetic process of the volatilization of PAHs. (3) Different environmental factors had different effects on the volatilization of PAHs. We found that increasing the temperature and illuminance and decreasing the particle size increased volatility. Through canonical correspondence analysis, PAHs volatilization was found to be a complex process, so volatilization tests under simulated environmental conditions are of scientific and environmental interest. Shale gas, an emerging oil-bearing and pillar industry at home and abroad, has a very large impact on economic development and industry, but the resulting emerging pollutants pose a serious threat to the environment. Drilling cuttings, the primary byproduct of the exploration and mining of shale gas, are potentially hazardous types of waste that seriously deplete land resources and pose environmental safety problems. In this paper, a long-term static volatilization experiment was conducted to study the volatilization of polycyclic aromatic hydrocarbons (PAHs) in the oil-based residue of shale gas drill cuttings. Furthermore, the effects of some relevant environmental factors controlling the volatilization behavior were evaluated, including different particle sizes, temperatures and illuminances. The results showed that (1) the volatilization concentrations of PAHs gradually increased with prolonged volatilization time. PAHs with smaller ring numbers were present at the highest concentrations among the detected PAHs, and they were more readily volatilized and could be detected earlier. (2) The C-history method was found to significantly describe the kinetic process of the volatilization of PAHs. (3) Different environmental factors had different effects on the volatilization of PAHs. We found that increasing the temperature and illuminance and decreasing the particle size increased volatility. Through canonical correspondence analysis, PAHs volatilization was found to be a complex process, so volatilization tests under simulated environmental conditions are of scientific and environmental interest. Oil-based residues of shale drill cuttings Elsevier Volatilization Elsevier C-history method Elsevier PAHs Elsevier Qin, Jihong oth Xie, Bingxin oth Sun, Hui oth Li, Xin oth Chen, Wenqing oth Enthalten in Elsevier Science Shterenlikht, Anton ELSEVIER MPI vs Fortran coarrays beyond 100k cores: 3D cellular automata 2019 chemistry, biology and toxicology as related to environmental problems Amsterdam [u.a.] (DE-627)ELV002112701 volume:288 year:2022 pages:0 https://doi.org/10.1016/j.chemosphere.2021.132455 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 54.25 Parallele Datenverarbeitung VZ AR 288 2022 0 |
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10.1016/j.chemosphere.2021.132455 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001596.pica (DE-627)ELV056034245 (ELSEVIER)S0045-6535(21)02927-1 DE-627 ger DE-627 rakwb eng 004 620 VZ 54.25 bkl Wang, Shu verfasserin aut Volatilization behavior of polycyclic aromatic hydrocarbons from the oil-based residues of shale drill cuttings 2022transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Shale gas, an emerging oil-bearing and pillar industry at home and abroad, has a very large impact on economic development and industry, but the resulting emerging pollutants pose a serious threat to the environment. Drilling cuttings, the primary byproduct of the exploration and mining of shale gas, are potentially hazardous types of waste that seriously deplete land resources and pose environmental safety problems. In this paper, a long-term static volatilization experiment was conducted to study the volatilization of polycyclic aromatic hydrocarbons (PAHs) in the oil-based residue of shale gas drill cuttings. Furthermore, the effects of some relevant environmental factors controlling the volatilization behavior were evaluated, including different particle sizes, temperatures and illuminances. The results showed that (1) the volatilization concentrations of PAHs gradually increased with prolonged volatilization time. PAHs with smaller ring numbers were present at the highest concentrations among the detected PAHs, and they were more readily volatilized and could be detected earlier. (2) The C-history method was found to significantly describe the kinetic process of the volatilization of PAHs. (3) Different environmental factors had different effects on the volatilization of PAHs. We found that increasing the temperature and illuminance and decreasing the particle size increased volatility. Through canonical correspondence analysis, PAHs volatilization was found to be a complex process, so volatilization tests under simulated environmental conditions are of scientific and environmental interest. Shale gas, an emerging oil-bearing and pillar industry at home and abroad, has a very large impact on economic development and industry, but the resulting emerging pollutants pose a serious threat to the environment. Drilling cuttings, the primary byproduct of the exploration and mining of shale gas, are potentially hazardous types of waste that seriously deplete land resources and pose environmental safety problems. In this paper, a long-term static volatilization experiment was conducted to study the volatilization of polycyclic aromatic hydrocarbons (PAHs) in the oil-based residue of shale gas drill cuttings. Furthermore, the effects of some relevant environmental factors controlling the volatilization behavior were evaluated, including different particle sizes, temperatures and illuminances. The results showed that (1) the volatilization concentrations of PAHs gradually increased with prolonged volatilization time. PAHs with smaller ring numbers were present at the highest concentrations among the detected PAHs, and they were more readily volatilized and could be detected earlier. (2) The C-history method was found to significantly describe the kinetic process of the volatilization of PAHs. (3) Different environmental factors had different effects on the volatilization of PAHs. We found that increasing the temperature and illuminance and decreasing the particle size increased volatility. Through canonical correspondence analysis, PAHs volatilization was found to be a complex process, so volatilization tests under simulated environmental conditions are of scientific and environmental interest. Oil-based residues of shale drill cuttings Elsevier Volatilization Elsevier C-history method Elsevier PAHs Elsevier Qin, Jihong oth Xie, Bingxin oth Sun, Hui oth Li, Xin oth Chen, Wenqing oth Enthalten in Elsevier Science Shterenlikht, Anton ELSEVIER MPI vs Fortran coarrays beyond 100k cores: 3D cellular automata 2019 chemistry, biology and toxicology as related to environmental problems Amsterdam [u.a.] (DE-627)ELV002112701 volume:288 year:2022 pages:0 https://doi.org/10.1016/j.chemosphere.2021.132455 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 54.25 Parallele Datenverarbeitung VZ AR 288 2022 0 |
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10.1016/j.chemosphere.2021.132455 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001596.pica (DE-627)ELV056034245 (ELSEVIER)S0045-6535(21)02927-1 DE-627 ger DE-627 rakwb eng 004 620 VZ 54.25 bkl Wang, Shu verfasserin aut Volatilization behavior of polycyclic aromatic hydrocarbons from the oil-based residues of shale drill cuttings 2022transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Shale gas, an emerging oil-bearing and pillar industry at home and abroad, has a very large impact on economic development and industry, but the resulting emerging pollutants pose a serious threat to the environment. Drilling cuttings, the primary byproduct of the exploration and mining of shale gas, are potentially hazardous types of waste that seriously deplete land resources and pose environmental safety problems. In this paper, a long-term static volatilization experiment was conducted to study the volatilization of polycyclic aromatic hydrocarbons (PAHs) in the oil-based residue of shale gas drill cuttings. Furthermore, the effects of some relevant environmental factors controlling the volatilization behavior were evaluated, including different particle sizes, temperatures and illuminances. The results showed that (1) the volatilization concentrations of PAHs gradually increased with prolonged volatilization time. PAHs with smaller ring numbers were present at the highest concentrations among the detected PAHs, and they were more readily volatilized and could be detected earlier. (2) The C-history method was found to significantly describe the kinetic process of the volatilization of PAHs. (3) Different environmental factors had different effects on the volatilization of PAHs. We found that increasing the temperature and illuminance and decreasing the particle size increased volatility. Through canonical correspondence analysis, PAHs volatilization was found to be a complex process, so volatilization tests under simulated environmental conditions are of scientific and environmental interest. Shale gas, an emerging oil-bearing and pillar industry at home and abroad, has a very large impact on economic development and industry, but the resulting emerging pollutants pose a serious threat to the environment. Drilling cuttings, the primary byproduct of the exploration and mining of shale gas, are potentially hazardous types of waste that seriously deplete land resources and pose environmental safety problems. In this paper, a long-term static volatilization experiment was conducted to study the volatilization of polycyclic aromatic hydrocarbons (PAHs) in the oil-based residue of shale gas drill cuttings. Furthermore, the effects of some relevant environmental factors controlling the volatilization behavior were evaluated, including different particle sizes, temperatures and illuminances. The results showed that (1) the volatilization concentrations of PAHs gradually increased with prolonged volatilization time. PAHs with smaller ring numbers were present at the highest concentrations among the detected PAHs, and they were more readily volatilized and could be detected earlier. (2) The C-history method was found to significantly describe the kinetic process of the volatilization of PAHs. (3) Different environmental factors had different effects on the volatilization of PAHs. We found that increasing the temperature and illuminance and decreasing the particle size increased volatility. Through canonical correspondence analysis, PAHs volatilization was found to be a complex process, so volatilization tests under simulated environmental conditions are of scientific and environmental interest. Oil-based residues of shale drill cuttings Elsevier Volatilization Elsevier C-history method Elsevier PAHs Elsevier Qin, Jihong oth Xie, Bingxin oth Sun, Hui oth Li, Xin oth Chen, Wenqing oth Enthalten in Elsevier Science Shterenlikht, Anton ELSEVIER MPI vs Fortran coarrays beyond 100k cores: 3D cellular automata 2019 chemistry, biology and toxicology as related to environmental problems Amsterdam [u.a.] (DE-627)ELV002112701 volume:288 year:2022 pages:0 https://doi.org/10.1016/j.chemosphere.2021.132455 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 54.25 Parallele Datenverarbeitung VZ AR 288 2022 0 |
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10.1016/j.chemosphere.2021.132455 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001596.pica (DE-627)ELV056034245 (ELSEVIER)S0045-6535(21)02927-1 DE-627 ger DE-627 rakwb eng 004 620 VZ 54.25 bkl Wang, Shu verfasserin aut Volatilization behavior of polycyclic aromatic hydrocarbons from the oil-based residues of shale drill cuttings 2022transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Shale gas, an emerging oil-bearing and pillar industry at home and abroad, has a very large impact on economic development and industry, but the resulting emerging pollutants pose a serious threat to the environment. Drilling cuttings, the primary byproduct of the exploration and mining of shale gas, are potentially hazardous types of waste that seriously deplete land resources and pose environmental safety problems. In this paper, a long-term static volatilization experiment was conducted to study the volatilization of polycyclic aromatic hydrocarbons (PAHs) in the oil-based residue of shale gas drill cuttings. Furthermore, the effects of some relevant environmental factors controlling the volatilization behavior were evaluated, including different particle sizes, temperatures and illuminances. The results showed that (1) the volatilization concentrations of PAHs gradually increased with prolonged volatilization time. PAHs with smaller ring numbers were present at the highest concentrations among the detected PAHs, and they were more readily volatilized and could be detected earlier. (2) The C-history method was found to significantly describe the kinetic process of the volatilization of PAHs. (3) Different environmental factors had different effects on the volatilization of PAHs. We found that increasing the temperature and illuminance and decreasing the particle size increased volatility. Through canonical correspondence analysis, PAHs volatilization was found to be a complex process, so volatilization tests under simulated environmental conditions are of scientific and environmental interest. Shale gas, an emerging oil-bearing and pillar industry at home and abroad, has a very large impact on economic development and industry, but the resulting emerging pollutants pose a serious threat to the environment. Drilling cuttings, the primary byproduct of the exploration and mining of shale gas, are potentially hazardous types of waste that seriously deplete land resources and pose environmental safety problems. In this paper, a long-term static volatilization experiment was conducted to study the volatilization of polycyclic aromatic hydrocarbons (PAHs) in the oil-based residue of shale gas drill cuttings. Furthermore, the effects of some relevant environmental factors controlling the volatilization behavior were evaluated, including different particle sizes, temperatures and illuminances. The results showed that (1) the volatilization concentrations of PAHs gradually increased with prolonged volatilization time. PAHs with smaller ring numbers were present at the highest concentrations among the detected PAHs, and they were more readily volatilized and could be detected earlier. (2) The C-history method was found to significantly describe the kinetic process of the volatilization of PAHs. (3) Different environmental factors had different effects on the volatilization of PAHs. We found that increasing the temperature and illuminance and decreasing the particle size increased volatility. Through canonical correspondence analysis, PAHs volatilization was found to be a complex process, so volatilization tests under simulated environmental conditions are of scientific and environmental interest. Oil-based residues of shale drill cuttings Elsevier Volatilization Elsevier C-history method Elsevier PAHs Elsevier Qin, Jihong oth Xie, Bingxin oth Sun, Hui oth Li, Xin oth Chen, Wenqing oth Enthalten in Elsevier Science Shterenlikht, Anton ELSEVIER MPI vs Fortran coarrays beyond 100k cores: 3D cellular automata 2019 chemistry, biology and toxicology as related to environmental problems Amsterdam [u.a.] (DE-627)ELV002112701 volume:288 year:2022 pages:0 https://doi.org/10.1016/j.chemosphere.2021.132455 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 54.25 Parallele Datenverarbeitung VZ AR 288 2022 0 |
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10.1016/j.chemosphere.2021.132455 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001596.pica (DE-627)ELV056034245 (ELSEVIER)S0045-6535(21)02927-1 DE-627 ger DE-627 rakwb eng 004 620 VZ 54.25 bkl Wang, Shu verfasserin aut Volatilization behavior of polycyclic aromatic hydrocarbons from the oil-based residues of shale drill cuttings 2022transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Shale gas, an emerging oil-bearing and pillar industry at home and abroad, has a very large impact on economic development and industry, but the resulting emerging pollutants pose a serious threat to the environment. Drilling cuttings, the primary byproduct of the exploration and mining of shale gas, are potentially hazardous types of waste that seriously deplete land resources and pose environmental safety problems. In this paper, a long-term static volatilization experiment was conducted to study the volatilization of polycyclic aromatic hydrocarbons (PAHs) in the oil-based residue of shale gas drill cuttings. Furthermore, the effects of some relevant environmental factors controlling the volatilization behavior were evaluated, including different particle sizes, temperatures and illuminances. The results showed that (1) the volatilization concentrations of PAHs gradually increased with prolonged volatilization time. PAHs with smaller ring numbers were present at the highest concentrations among the detected PAHs, and they were more readily volatilized and could be detected earlier. (2) The C-history method was found to significantly describe the kinetic process of the volatilization of PAHs. (3) Different environmental factors had different effects on the volatilization of PAHs. We found that increasing the temperature and illuminance and decreasing the particle size increased volatility. Through canonical correspondence analysis, PAHs volatilization was found to be a complex process, so volatilization tests under simulated environmental conditions are of scientific and environmental interest. Shale gas, an emerging oil-bearing and pillar industry at home and abroad, has a very large impact on economic development and industry, but the resulting emerging pollutants pose a serious threat to the environment. Drilling cuttings, the primary byproduct of the exploration and mining of shale gas, are potentially hazardous types of waste that seriously deplete land resources and pose environmental safety problems. In this paper, a long-term static volatilization experiment was conducted to study the volatilization of polycyclic aromatic hydrocarbons (PAHs) in the oil-based residue of shale gas drill cuttings. Furthermore, the effects of some relevant environmental factors controlling the volatilization behavior were evaluated, including different particle sizes, temperatures and illuminances. The results showed that (1) the volatilization concentrations of PAHs gradually increased with prolonged volatilization time. PAHs with smaller ring numbers were present at the highest concentrations among the detected PAHs, and they were more readily volatilized and could be detected earlier. (2) The C-history method was found to significantly describe the kinetic process of the volatilization of PAHs. (3) Different environmental factors had different effects on the volatilization of PAHs. We found that increasing the temperature and illuminance and decreasing the particle size increased volatility. Through canonical correspondence analysis, PAHs volatilization was found to be a complex process, so volatilization tests under simulated environmental conditions are of scientific and environmental interest. Oil-based residues of shale drill cuttings Elsevier Volatilization Elsevier C-history method Elsevier PAHs Elsevier Qin, Jihong oth Xie, Bingxin oth Sun, Hui oth Li, Xin oth Chen, Wenqing oth Enthalten in Elsevier Science Shterenlikht, Anton ELSEVIER MPI vs Fortran coarrays beyond 100k cores: 3D cellular automata 2019 chemistry, biology and toxicology as related to environmental problems Amsterdam [u.a.] (DE-627)ELV002112701 volume:288 year:2022 pages:0 https://doi.org/10.1016/j.chemosphere.2021.132455 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 54.25 Parallele Datenverarbeitung VZ AR 288 2022 0 |
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volatilization behavior of polycyclic aromatic hydrocarbons from the oil-based residues of shale drill cuttings |
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Volatilization behavior of polycyclic aromatic hydrocarbons from the oil-based residues of shale drill cuttings |
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Shale gas, an emerging oil-bearing and pillar industry at home and abroad, has a very large impact on economic development and industry, but the resulting emerging pollutants pose a serious threat to the environment. Drilling cuttings, the primary byproduct of the exploration and mining of shale gas, are potentially hazardous types of waste that seriously deplete land resources and pose environmental safety problems. In this paper, a long-term static volatilization experiment was conducted to study the volatilization of polycyclic aromatic hydrocarbons (PAHs) in the oil-based residue of shale gas drill cuttings. Furthermore, the effects of some relevant environmental factors controlling the volatilization behavior were evaluated, including different particle sizes, temperatures and illuminances. The results showed that (1) the volatilization concentrations of PAHs gradually increased with prolonged volatilization time. PAHs with smaller ring numbers were present at the highest concentrations among the detected PAHs, and they were more readily volatilized and could be detected earlier. (2) The C-history method was found to significantly describe the kinetic process of the volatilization of PAHs. (3) Different environmental factors had different effects on the volatilization of PAHs. We found that increasing the temperature and illuminance and decreasing the particle size increased volatility. Through canonical correspondence analysis, PAHs volatilization was found to be a complex process, so volatilization tests under simulated environmental conditions are of scientific and environmental interest. |
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Shale gas, an emerging oil-bearing and pillar industry at home and abroad, has a very large impact on economic development and industry, but the resulting emerging pollutants pose a serious threat to the environment. Drilling cuttings, the primary byproduct of the exploration and mining of shale gas, are potentially hazardous types of waste that seriously deplete land resources and pose environmental safety problems. In this paper, a long-term static volatilization experiment was conducted to study the volatilization of polycyclic aromatic hydrocarbons (PAHs) in the oil-based residue of shale gas drill cuttings. Furthermore, the effects of some relevant environmental factors controlling the volatilization behavior were evaluated, including different particle sizes, temperatures and illuminances. The results showed that (1) the volatilization concentrations of PAHs gradually increased with prolonged volatilization time. PAHs with smaller ring numbers were present at the highest concentrations among the detected PAHs, and they were more readily volatilized and could be detected earlier. (2) The C-history method was found to significantly describe the kinetic process of the volatilization of PAHs. (3) Different environmental factors had different effects on the volatilization of PAHs. We found that increasing the temperature and illuminance and decreasing the particle size increased volatility. Through canonical correspondence analysis, PAHs volatilization was found to be a complex process, so volatilization tests under simulated environmental conditions are of scientific and environmental interest. |
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Shale gas, an emerging oil-bearing and pillar industry at home and abroad, has a very large impact on economic development and industry, but the resulting emerging pollutants pose a serious threat to the environment. Drilling cuttings, the primary byproduct of the exploration and mining of shale gas, are potentially hazardous types of waste that seriously deplete land resources and pose environmental safety problems. In this paper, a long-term static volatilization experiment was conducted to study the volatilization of polycyclic aromatic hydrocarbons (PAHs) in the oil-based residue of shale gas drill cuttings. Furthermore, the effects of some relevant environmental factors controlling the volatilization behavior were evaluated, including different particle sizes, temperatures and illuminances. The results showed that (1) the volatilization concentrations of PAHs gradually increased with prolonged volatilization time. PAHs with smaller ring numbers were present at the highest concentrations among the detected PAHs, and they were more readily volatilized and could be detected earlier. (2) The C-history method was found to significantly describe the kinetic process of the volatilization of PAHs. (3) Different environmental factors had different effects on the volatilization of PAHs. We found that increasing the temperature and illuminance and decreasing the particle size increased volatility. Through canonical correspondence analysis, PAHs volatilization was found to be a complex process, so volatilization tests under simulated environmental conditions are of scientific and environmental interest. |
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