Enhanced photoelectrochemical performances in photocatalytic pollutant degradation and water splitting by direct Z-scheme Bi2Sn2O7/TiO2 NTAs
The construction of ternary metal oxide to improve photoelectrochemical performances of TiO2 photocatalysts is the hot topic in environmental and resource applications. Herein, Bi2Sn2O7 nanoparticles were deposited on TiO2 nanotube arrays (TiO2 NTAs) by the solvothermal technology only by changing r...
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Hou, Junwei [verfasserIn] |
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Enthalten in: Soil and water bioengineering: Practice and research needs for reconciling natural hazard control and ecological restoration - Rey, F. ELSEVIER, 2018, Amsterdam [u.a.] |
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Übergeordnetes Werk: |
volume:48 ; year:2022 ; number:3 ; day:1 ; month:02 ; pages:3941-3953 ; extent:13 |
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DOI / URN: |
10.1016/j.ceramint.2021.10.181 |
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ELV056290519 |
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245 | 1 | 0 | |a Enhanced photoelectrochemical performances in photocatalytic pollutant degradation and water splitting by direct Z-scheme Bi2Sn2O7/TiO2 NTAs |
264 | 1 | |c 2022transfer abstract | |
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520 | |a The construction of ternary metal oxide to improve photoelectrochemical performances of TiO2 photocatalysts is the hot topic in environmental and resource applications. Herein, Bi2Sn2O7 nanoparticles were deposited on TiO2 nanotube arrays (TiO2 NTAs) by the solvothermal technology only by changing reagent concentration. The solar absorption region of TiO2 NTAs was obviously extended into visible light after Bi2Sn2O7 sensitization, and the photoelectric performance was also significantly improved. The high visible light photocurrent density and photovoltage achieved 30.24 μA/cm2 and -0.19 V, and the interface resistance was reduced that benefited the rapid electron transportation. The photocatalytic performances of methyl orange (MO), rhodamine b (RhB), methylene blue (MB) and Cr (VI) removal were enhanced, and 63.76%, 77.34%, 100% and 100% of these pollutants were photoremoved under solar irradiation. Moreover, the construction of direct Z-scheme Bi2Sn2O7/TiO2 NTAs heterojunction was beneficial to the photoelectron transfer and active radical formation, and the experimental results indicated that •OH and •O2 - were the decisive species for the dye degradation. The samples also exhibited outstanding photocatalytic water splitting for H2 evolution, and the high efficiency (306.36 μmol·cm−2·h−1) and stability were confirmed. The excellent photocatalytic performances of the Bi2Sn2O7/TiO2 NTAs photoelectrodes showed extensive potential applications in environmental pollution and green resource exploitation. | ||
520 | |a The construction of ternary metal oxide to improve photoelectrochemical performances of TiO2 photocatalysts is the hot topic in environmental and resource applications. Herein, Bi2Sn2O7 nanoparticles were deposited on TiO2 nanotube arrays (TiO2 NTAs) by the solvothermal technology only by changing reagent concentration. The solar absorption region of TiO2 NTAs was obviously extended into visible light after Bi2Sn2O7 sensitization, and the photoelectric performance was also significantly improved. The high visible light photocurrent density and photovoltage achieved 30.24 μA/cm2 and -0.19 V, and the interface resistance was reduced that benefited the rapid electron transportation. The photocatalytic performances of methyl orange (MO), rhodamine b (RhB), methylene blue (MB) and Cr (VI) removal were enhanced, and 63.76%, 77.34%, 100% and 100% of these pollutants were photoremoved under solar irradiation. Moreover, the construction of direct Z-scheme Bi2Sn2O7/TiO2 NTAs heterojunction was beneficial to the photoelectron transfer and active radical formation, and the experimental results indicated that •OH and •O2 - were the decisive species for the dye degradation. The samples also exhibited outstanding photocatalytic water splitting for H2 evolution, and the high efficiency (306.36 μmol·cm−2·h−1) and stability were confirmed. The excellent photocatalytic performances of the Bi2Sn2O7/TiO2 NTAs photoelectrodes showed extensive potential applications in environmental pollution and green resource exploitation. | ||
650 | 7 | |a Water splitting |2 Elsevier | |
650 | 7 | |a Bi2Sn2O7 nanoparticles |2 Elsevier | |
650 | 7 | |a Photocatalytic technology |2 Elsevier | |
650 | 7 | |a TiO2 NTAs |2 Elsevier | |
700 | 1 | |a Kong, Lingcong |4 oth | |
700 | 1 | |a Xie, Yu |4 oth | |
700 | 1 | |a Ma, Jingui |4 oth | |
700 | 1 | |a Liu, Yansheng |4 oth | |
700 | 1 | |a Chen, Mengmeng |4 oth | |
700 | 1 | |a Wang, Qingyao |4 oth | |
773 | 0 | 8 | |i Enthalten in |n Elsevier Science |a Rey, F. ELSEVIER |t Soil and water bioengineering: Practice and research needs for reconciling natural hazard control and ecological restoration |d 2018 |g Amsterdam [u.a.] |w (DE-627)ELV000899798 |
773 | 1 | 8 | |g volume:48 |g year:2022 |g number:3 |g day:1 |g month:02 |g pages:3941-3953 |g extent:13 |
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10.1016/j.ceramint.2021.10.181 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001621.pica (DE-627)ELV056290519 (ELSEVIER)S0272-8842(21)03323-X DE-627 ger DE-627 rakwb eng 333.7 610 VZ 43.12 bkl 43.13 bkl 44.13 bkl Hou, Junwei verfasserin aut Enhanced photoelectrochemical performances in photocatalytic pollutant degradation and water splitting by direct Z-scheme Bi2Sn2O7/TiO2 NTAs 2022transfer abstract 13 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The construction of ternary metal oxide to improve photoelectrochemical performances of TiO2 photocatalysts is the hot topic in environmental and resource applications. Herein, Bi2Sn2O7 nanoparticles were deposited on TiO2 nanotube arrays (TiO2 NTAs) by the solvothermal technology only by changing reagent concentration. The solar absorption region of TiO2 NTAs was obviously extended into visible light after Bi2Sn2O7 sensitization, and the photoelectric performance was also significantly improved. The high visible light photocurrent density and photovoltage achieved 30.24 μA/cm2 and -0.19 V, and the interface resistance was reduced that benefited the rapid electron transportation. The photocatalytic performances of methyl orange (MO), rhodamine b (RhB), methylene blue (MB) and Cr (VI) removal were enhanced, and 63.76%, 77.34%, 100% and 100% of these pollutants were photoremoved under solar irradiation. Moreover, the construction of direct Z-scheme Bi2Sn2O7/TiO2 NTAs heterojunction was beneficial to the photoelectron transfer and active radical formation, and the experimental results indicated that •OH and •O2 - were the decisive species for the dye degradation. The samples also exhibited outstanding photocatalytic water splitting for H2 evolution, and the high efficiency (306.36 μmol·cm−2·h−1) and stability were confirmed. The excellent photocatalytic performances of the Bi2Sn2O7/TiO2 NTAs photoelectrodes showed extensive potential applications in environmental pollution and green resource exploitation. The construction of ternary metal oxide to improve photoelectrochemical performances of TiO2 photocatalysts is the hot topic in environmental and resource applications. Herein, Bi2Sn2O7 nanoparticles were deposited on TiO2 nanotube arrays (TiO2 NTAs) by the solvothermal technology only by changing reagent concentration. The solar absorption region of TiO2 NTAs was obviously extended into visible light after Bi2Sn2O7 sensitization, and the photoelectric performance was also significantly improved. The high visible light photocurrent density and photovoltage achieved 30.24 μA/cm2 and -0.19 V, and the interface resistance was reduced that benefited the rapid electron transportation. The photocatalytic performances of methyl orange (MO), rhodamine b (RhB), methylene blue (MB) and Cr (VI) removal were enhanced, and 63.76%, 77.34%, 100% and 100% of these pollutants were photoremoved under solar irradiation. Moreover, the construction of direct Z-scheme Bi2Sn2O7/TiO2 NTAs heterojunction was beneficial to the photoelectron transfer and active radical formation, and the experimental results indicated that •OH and •O2 - were the decisive species for the dye degradation. The samples also exhibited outstanding photocatalytic water splitting for H2 evolution, and the high efficiency (306.36 μmol·cm−2·h−1) and stability were confirmed. The excellent photocatalytic performances of the Bi2Sn2O7/TiO2 NTAs photoelectrodes showed extensive potential applications in environmental pollution and green resource exploitation. Water splitting Elsevier Bi2Sn2O7 nanoparticles Elsevier Photocatalytic technology Elsevier TiO2 NTAs Elsevier Kong, Lingcong oth Xie, Yu oth Ma, Jingui oth Liu, Yansheng oth Chen, Mengmeng oth Wang, Qingyao oth Enthalten in Elsevier Science Rey, F. ELSEVIER Soil and water bioengineering: Practice and research needs for reconciling natural hazard control and ecological restoration 2018 Amsterdam [u.a.] (DE-627)ELV000899798 volume:48 year:2022 number:3 day:1 month:02 pages:3941-3953 extent:13 https://doi.org/10.1016/j.ceramint.2021.10.181 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO 43.12 Umweltchemie VZ 43.13 Umwelttoxikologie VZ 44.13 Medizinische Ökologie VZ AR 48 2022 3 1 0201 3941-3953 13 |
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10.1016/j.ceramint.2021.10.181 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001621.pica (DE-627)ELV056290519 (ELSEVIER)S0272-8842(21)03323-X DE-627 ger DE-627 rakwb eng 333.7 610 VZ 43.12 bkl 43.13 bkl 44.13 bkl Hou, Junwei verfasserin aut Enhanced photoelectrochemical performances in photocatalytic pollutant degradation and water splitting by direct Z-scheme Bi2Sn2O7/TiO2 NTAs 2022transfer abstract 13 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The construction of ternary metal oxide to improve photoelectrochemical performances of TiO2 photocatalysts is the hot topic in environmental and resource applications. Herein, Bi2Sn2O7 nanoparticles were deposited on TiO2 nanotube arrays (TiO2 NTAs) by the solvothermal technology only by changing reagent concentration. The solar absorption region of TiO2 NTAs was obviously extended into visible light after Bi2Sn2O7 sensitization, and the photoelectric performance was also significantly improved. The high visible light photocurrent density and photovoltage achieved 30.24 μA/cm2 and -0.19 V, and the interface resistance was reduced that benefited the rapid electron transportation. The photocatalytic performances of methyl orange (MO), rhodamine b (RhB), methylene blue (MB) and Cr (VI) removal were enhanced, and 63.76%, 77.34%, 100% and 100% of these pollutants were photoremoved under solar irradiation. Moreover, the construction of direct Z-scheme Bi2Sn2O7/TiO2 NTAs heterojunction was beneficial to the photoelectron transfer and active radical formation, and the experimental results indicated that •OH and •O2 - were the decisive species for the dye degradation. The samples also exhibited outstanding photocatalytic water splitting for H2 evolution, and the high efficiency (306.36 μmol·cm−2·h−1) and stability were confirmed. The excellent photocatalytic performances of the Bi2Sn2O7/TiO2 NTAs photoelectrodes showed extensive potential applications in environmental pollution and green resource exploitation. The construction of ternary metal oxide to improve photoelectrochemical performances of TiO2 photocatalysts is the hot topic in environmental and resource applications. Herein, Bi2Sn2O7 nanoparticles were deposited on TiO2 nanotube arrays (TiO2 NTAs) by the solvothermal technology only by changing reagent concentration. The solar absorption region of TiO2 NTAs was obviously extended into visible light after Bi2Sn2O7 sensitization, and the photoelectric performance was also significantly improved. The high visible light photocurrent density and photovoltage achieved 30.24 μA/cm2 and -0.19 V, and the interface resistance was reduced that benefited the rapid electron transportation. The photocatalytic performances of methyl orange (MO), rhodamine b (RhB), methylene blue (MB) and Cr (VI) removal were enhanced, and 63.76%, 77.34%, 100% and 100% of these pollutants were photoremoved under solar irradiation. Moreover, the construction of direct Z-scheme Bi2Sn2O7/TiO2 NTAs heterojunction was beneficial to the photoelectron transfer and active radical formation, and the experimental results indicated that •OH and •O2 - were the decisive species for the dye degradation. The samples also exhibited outstanding photocatalytic water splitting for H2 evolution, and the high efficiency (306.36 μmol·cm−2·h−1) and stability were confirmed. The excellent photocatalytic performances of the Bi2Sn2O7/TiO2 NTAs photoelectrodes showed extensive potential applications in environmental pollution and green resource exploitation. Water splitting Elsevier Bi2Sn2O7 nanoparticles Elsevier Photocatalytic technology Elsevier TiO2 NTAs Elsevier Kong, Lingcong oth Xie, Yu oth Ma, Jingui oth Liu, Yansheng oth Chen, Mengmeng oth Wang, Qingyao oth Enthalten in Elsevier Science Rey, F. ELSEVIER Soil and water bioengineering: Practice and research needs for reconciling natural hazard control and ecological restoration 2018 Amsterdam [u.a.] (DE-627)ELV000899798 volume:48 year:2022 number:3 day:1 month:02 pages:3941-3953 extent:13 https://doi.org/10.1016/j.ceramint.2021.10.181 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO 43.12 Umweltchemie VZ 43.13 Umwelttoxikologie VZ 44.13 Medizinische Ökologie VZ AR 48 2022 3 1 0201 3941-3953 13 |
allfields_unstemmed |
10.1016/j.ceramint.2021.10.181 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001621.pica (DE-627)ELV056290519 (ELSEVIER)S0272-8842(21)03323-X DE-627 ger DE-627 rakwb eng 333.7 610 VZ 43.12 bkl 43.13 bkl 44.13 bkl Hou, Junwei verfasserin aut Enhanced photoelectrochemical performances in photocatalytic pollutant degradation and water splitting by direct Z-scheme Bi2Sn2O7/TiO2 NTAs 2022transfer abstract 13 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The construction of ternary metal oxide to improve photoelectrochemical performances of TiO2 photocatalysts is the hot topic in environmental and resource applications. Herein, Bi2Sn2O7 nanoparticles were deposited on TiO2 nanotube arrays (TiO2 NTAs) by the solvothermal technology only by changing reagent concentration. The solar absorption region of TiO2 NTAs was obviously extended into visible light after Bi2Sn2O7 sensitization, and the photoelectric performance was also significantly improved. The high visible light photocurrent density and photovoltage achieved 30.24 μA/cm2 and -0.19 V, and the interface resistance was reduced that benefited the rapid electron transportation. The photocatalytic performances of methyl orange (MO), rhodamine b (RhB), methylene blue (MB) and Cr (VI) removal were enhanced, and 63.76%, 77.34%, 100% and 100% of these pollutants were photoremoved under solar irradiation. Moreover, the construction of direct Z-scheme Bi2Sn2O7/TiO2 NTAs heterojunction was beneficial to the photoelectron transfer and active radical formation, and the experimental results indicated that •OH and •O2 - were the decisive species for the dye degradation. The samples also exhibited outstanding photocatalytic water splitting for H2 evolution, and the high efficiency (306.36 μmol·cm−2·h−1) and stability were confirmed. The excellent photocatalytic performances of the Bi2Sn2O7/TiO2 NTAs photoelectrodes showed extensive potential applications in environmental pollution and green resource exploitation. The construction of ternary metal oxide to improve photoelectrochemical performances of TiO2 photocatalysts is the hot topic in environmental and resource applications. Herein, Bi2Sn2O7 nanoparticles were deposited on TiO2 nanotube arrays (TiO2 NTAs) by the solvothermal technology only by changing reagent concentration. The solar absorption region of TiO2 NTAs was obviously extended into visible light after Bi2Sn2O7 sensitization, and the photoelectric performance was also significantly improved. The high visible light photocurrent density and photovoltage achieved 30.24 μA/cm2 and -0.19 V, and the interface resistance was reduced that benefited the rapid electron transportation. The photocatalytic performances of methyl orange (MO), rhodamine b (RhB), methylene blue (MB) and Cr (VI) removal were enhanced, and 63.76%, 77.34%, 100% and 100% of these pollutants were photoremoved under solar irradiation. Moreover, the construction of direct Z-scheme Bi2Sn2O7/TiO2 NTAs heterojunction was beneficial to the photoelectron transfer and active radical formation, and the experimental results indicated that •OH and •O2 - were the decisive species for the dye degradation. The samples also exhibited outstanding photocatalytic water splitting for H2 evolution, and the high efficiency (306.36 μmol·cm−2·h−1) and stability were confirmed. The excellent photocatalytic performances of the Bi2Sn2O7/TiO2 NTAs photoelectrodes showed extensive potential applications in environmental pollution and green resource exploitation. Water splitting Elsevier Bi2Sn2O7 nanoparticles Elsevier Photocatalytic technology Elsevier TiO2 NTAs Elsevier Kong, Lingcong oth Xie, Yu oth Ma, Jingui oth Liu, Yansheng oth Chen, Mengmeng oth Wang, Qingyao oth Enthalten in Elsevier Science Rey, F. ELSEVIER Soil and water bioengineering: Practice and research needs for reconciling natural hazard control and ecological restoration 2018 Amsterdam [u.a.] (DE-627)ELV000899798 volume:48 year:2022 number:3 day:1 month:02 pages:3941-3953 extent:13 https://doi.org/10.1016/j.ceramint.2021.10.181 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO 43.12 Umweltchemie VZ 43.13 Umwelttoxikologie VZ 44.13 Medizinische Ökologie VZ AR 48 2022 3 1 0201 3941-3953 13 |
allfieldsGer |
10.1016/j.ceramint.2021.10.181 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001621.pica (DE-627)ELV056290519 (ELSEVIER)S0272-8842(21)03323-X DE-627 ger DE-627 rakwb eng 333.7 610 VZ 43.12 bkl 43.13 bkl 44.13 bkl Hou, Junwei verfasserin aut Enhanced photoelectrochemical performances in photocatalytic pollutant degradation and water splitting by direct Z-scheme Bi2Sn2O7/TiO2 NTAs 2022transfer abstract 13 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The construction of ternary metal oxide to improve photoelectrochemical performances of TiO2 photocatalysts is the hot topic in environmental and resource applications. Herein, Bi2Sn2O7 nanoparticles were deposited on TiO2 nanotube arrays (TiO2 NTAs) by the solvothermal technology only by changing reagent concentration. The solar absorption region of TiO2 NTAs was obviously extended into visible light after Bi2Sn2O7 sensitization, and the photoelectric performance was also significantly improved. The high visible light photocurrent density and photovoltage achieved 30.24 μA/cm2 and -0.19 V, and the interface resistance was reduced that benefited the rapid electron transportation. The photocatalytic performances of methyl orange (MO), rhodamine b (RhB), methylene blue (MB) and Cr (VI) removal were enhanced, and 63.76%, 77.34%, 100% and 100% of these pollutants were photoremoved under solar irradiation. Moreover, the construction of direct Z-scheme Bi2Sn2O7/TiO2 NTAs heterojunction was beneficial to the photoelectron transfer and active radical formation, and the experimental results indicated that •OH and •O2 - were the decisive species for the dye degradation. The samples also exhibited outstanding photocatalytic water splitting for H2 evolution, and the high efficiency (306.36 μmol·cm−2·h−1) and stability were confirmed. The excellent photocatalytic performances of the Bi2Sn2O7/TiO2 NTAs photoelectrodes showed extensive potential applications in environmental pollution and green resource exploitation. The construction of ternary metal oxide to improve photoelectrochemical performances of TiO2 photocatalysts is the hot topic in environmental and resource applications. Herein, Bi2Sn2O7 nanoparticles were deposited on TiO2 nanotube arrays (TiO2 NTAs) by the solvothermal technology only by changing reagent concentration. The solar absorption region of TiO2 NTAs was obviously extended into visible light after Bi2Sn2O7 sensitization, and the photoelectric performance was also significantly improved. The high visible light photocurrent density and photovoltage achieved 30.24 μA/cm2 and -0.19 V, and the interface resistance was reduced that benefited the rapid electron transportation. The photocatalytic performances of methyl orange (MO), rhodamine b (RhB), methylene blue (MB) and Cr (VI) removal were enhanced, and 63.76%, 77.34%, 100% and 100% of these pollutants were photoremoved under solar irradiation. Moreover, the construction of direct Z-scheme Bi2Sn2O7/TiO2 NTAs heterojunction was beneficial to the photoelectron transfer and active radical formation, and the experimental results indicated that •OH and •O2 - were the decisive species for the dye degradation. The samples also exhibited outstanding photocatalytic water splitting for H2 evolution, and the high efficiency (306.36 μmol·cm−2·h−1) and stability were confirmed. The excellent photocatalytic performances of the Bi2Sn2O7/TiO2 NTAs photoelectrodes showed extensive potential applications in environmental pollution and green resource exploitation. Water splitting Elsevier Bi2Sn2O7 nanoparticles Elsevier Photocatalytic technology Elsevier TiO2 NTAs Elsevier Kong, Lingcong oth Xie, Yu oth Ma, Jingui oth Liu, Yansheng oth Chen, Mengmeng oth Wang, Qingyao oth Enthalten in Elsevier Science Rey, F. ELSEVIER Soil and water bioengineering: Practice and research needs for reconciling natural hazard control and ecological restoration 2018 Amsterdam [u.a.] (DE-627)ELV000899798 volume:48 year:2022 number:3 day:1 month:02 pages:3941-3953 extent:13 https://doi.org/10.1016/j.ceramint.2021.10.181 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO 43.12 Umweltchemie VZ 43.13 Umwelttoxikologie VZ 44.13 Medizinische Ökologie VZ AR 48 2022 3 1 0201 3941-3953 13 |
allfieldsSound |
10.1016/j.ceramint.2021.10.181 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001621.pica (DE-627)ELV056290519 (ELSEVIER)S0272-8842(21)03323-X DE-627 ger DE-627 rakwb eng 333.7 610 VZ 43.12 bkl 43.13 bkl 44.13 bkl Hou, Junwei verfasserin aut Enhanced photoelectrochemical performances in photocatalytic pollutant degradation and water splitting by direct Z-scheme Bi2Sn2O7/TiO2 NTAs 2022transfer abstract 13 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The construction of ternary metal oxide to improve photoelectrochemical performances of TiO2 photocatalysts is the hot topic in environmental and resource applications. Herein, Bi2Sn2O7 nanoparticles were deposited on TiO2 nanotube arrays (TiO2 NTAs) by the solvothermal technology only by changing reagent concentration. The solar absorption region of TiO2 NTAs was obviously extended into visible light after Bi2Sn2O7 sensitization, and the photoelectric performance was also significantly improved. The high visible light photocurrent density and photovoltage achieved 30.24 μA/cm2 and -0.19 V, and the interface resistance was reduced that benefited the rapid electron transportation. The photocatalytic performances of methyl orange (MO), rhodamine b (RhB), methylene blue (MB) and Cr (VI) removal were enhanced, and 63.76%, 77.34%, 100% and 100% of these pollutants were photoremoved under solar irradiation. Moreover, the construction of direct Z-scheme Bi2Sn2O7/TiO2 NTAs heterojunction was beneficial to the photoelectron transfer and active radical formation, and the experimental results indicated that •OH and •O2 - were the decisive species for the dye degradation. The samples also exhibited outstanding photocatalytic water splitting for H2 evolution, and the high efficiency (306.36 μmol·cm−2·h−1) and stability were confirmed. The excellent photocatalytic performances of the Bi2Sn2O7/TiO2 NTAs photoelectrodes showed extensive potential applications in environmental pollution and green resource exploitation. The construction of ternary metal oxide to improve photoelectrochemical performances of TiO2 photocatalysts is the hot topic in environmental and resource applications. Herein, Bi2Sn2O7 nanoparticles were deposited on TiO2 nanotube arrays (TiO2 NTAs) by the solvothermal technology only by changing reagent concentration. The solar absorption region of TiO2 NTAs was obviously extended into visible light after Bi2Sn2O7 sensitization, and the photoelectric performance was also significantly improved. The high visible light photocurrent density and photovoltage achieved 30.24 μA/cm2 and -0.19 V, and the interface resistance was reduced that benefited the rapid electron transportation. The photocatalytic performances of methyl orange (MO), rhodamine b (RhB), methylene blue (MB) and Cr (VI) removal were enhanced, and 63.76%, 77.34%, 100% and 100% of these pollutants were photoremoved under solar irradiation. Moreover, the construction of direct Z-scheme Bi2Sn2O7/TiO2 NTAs heterojunction was beneficial to the photoelectron transfer and active radical formation, and the experimental results indicated that •OH and •O2 - were the decisive species for the dye degradation. The samples also exhibited outstanding photocatalytic water splitting for H2 evolution, and the high efficiency (306.36 μmol·cm−2·h−1) and stability were confirmed. The excellent photocatalytic performances of the Bi2Sn2O7/TiO2 NTAs photoelectrodes showed extensive potential applications in environmental pollution and green resource exploitation. Water splitting Elsevier Bi2Sn2O7 nanoparticles Elsevier Photocatalytic technology Elsevier TiO2 NTAs Elsevier Kong, Lingcong oth Xie, Yu oth Ma, Jingui oth Liu, Yansheng oth Chen, Mengmeng oth Wang, Qingyao oth Enthalten in Elsevier Science Rey, F. ELSEVIER Soil and water bioengineering: Practice and research needs for reconciling natural hazard control and ecological restoration 2018 Amsterdam [u.a.] (DE-627)ELV000899798 volume:48 year:2022 number:3 day:1 month:02 pages:3941-3953 extent:13 https://doi.org/10.1016/j.ceramint.2021.10.181 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO 43.12 Umweltchemie VZ 43.13 Umwelttoxikologie VZ 44.13 Medizinische Ökologie VZ AR 48 2022 3 1 0201 3941-3953 13 |
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enhanced photoelectrochemical performances in photocatalytic pollutant degradation and water splitting by direct z-scheme bi2sn2o7/tio2 ntas |
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Enhanced photoelectrochemical performances in photocatalytic pollutant degradation and water splitting by direct Z-scheme Bi2Sn2O7/TiO2 NTAs |
abstract |
The construction of ternary metal oxide to improve photoelectrochemical performances of TiO2 photocatalysts is the hot topic in environmental and resource applications. Herein, Bi2Sn2O7 nanoparticles were deposited on TiO2 nanotube arrays (TiO2 NTAs) by the solvothermal technology only by changing reagent concentration. The solar absorption region of TiO2 NTAs was obviously extended into visible light after Bi2Sn2O7 sensitization, and the photoelectric performance was also significantly improved. The high visible light photocurrent density and photovoltage achieved 30.24 μA/cm2 and -0.19 V, and the interface resistance was reduced that benefited the rapid electron transportation. The photocatalytic performances of methyl orange (MO), rhodamine b (RhB), methylene blue (MB) and Cr (VI) removal were enhanced, and 63.76%, 77.34%, 100% and 100% of these pollutants were photoremoved under solar irradiation. Moreover, the construction of direct Z-scheme Bi2Sn2O7/TiO2 NTAs heterojunction was beneficial to the photoelectron transfer and active radical formation, and the experimental results indicated that •OH and •O2 - were the decisive species for the dye degradation. The samples also exhibited outstanding photocatalytic water splitting for H2 evolution, and the high efficiency (306.36 μmol·cm−2·h−1) and stability were confirmed. The excellent photocatalytic performances of the Bi2Sn2O7/TiO2 NTAs photoelectrodes showed extensive potential applications in environmental pollution and green resource exploitation. |
abstractGer |
The construction of ternary metal oxide to improve photoelectrochemical performances of TiO2 photocatalysts is the hot topic in environmental and resource applications. Herein, Bi2Sn2O7 nanoparticles were deposited on TiO2 nanotube arrays (TiO2 NTAs) by the solvothermal technology only by changing reagent concentration. The solar absorption region of TiO2 NTAs was obviously extended into visible light after Bi2Sn2O7 sensitization, and the photoelectric performance was also significantly improved. The high visible light photocurrent density and photovoltage achieved 30.24 μA/cm2 and -0.19 V, and the interface resistance was reduced that benefited the rapid electron transportation. The photocatalytic performances of methyl orange (MO), rhodamine b (RhB), methylene blue (MB) and Cr (VI) removal were enhanced, and 63.76%, 77.34%, 100% and 100% of these pollutants were photoremoved under solar irradiation. Moreover, the construction of direct Z-scheme Bi2Sn2O7/TiO2 NTAs heterojunction was beneficial to the photoelectron transfer and active radical formation, and the experimental results indicated that •OH and •O2 - were the decisive species for the dye degradation. The samples also exhibited outstanding photocatalytic water splitting for H2 evolution, and the high efficiency (306.36 μmol·cm−2·h−1) and stability were confirmed. The excellent photocatalytic performances of the Bi2Sn2O7/TiO2 NTAs photoelectrodes showed extensive potential applications in environmental pollution and green resource exploitation. |
abstract_unstemmed |
The construction of ternary metal oxide to improve photoelectrochemical performances of TiO2 photocatalysts is the hot topic in environmental and resource applications. Herein, Bi2Sn2O7 nanoparticles were deposited on TiO2 nanotube arrays (TiO2 NTAs) by the solvothermal technology only by changing reagent concentration. The solar absorption region of TiO2 NTAs was obviously extended into visible light after Bi2Sn2O7 sensitization, and the photoelectric performance was also significantly improved. The high visible light photocurrent density and photovoltage achieved 30.24 μA/cm2 and -0.19 V, and the interface resistance was reduced that benefited the rapid electron transportation. The photocatalytic performances of methyl orange (MO), rhodamine b (RhB), methylene blue (MB) and Cr (VI) removal were enhanced, and 63.76%, 77.34%, 100% and 100% of these pollutants were photoremoved under solar irradiation. Moreover, the construction of direct Z-scheme Bi2Sn2O7/TiO2 NTAs heterojunction was beneficial to the photoelectron transfer and active radical formation, and the experimental results indicated that •OH and •O2 - were the decisive species for the dye degradation. The samples also exhibited outstanding photocatalytic water splitting for H2 evolution, and the high efficiency (306.36 μmol·cm−2·h−1) and stability were confirmed. The excellent photocatalytic performances of the Bi2Sn2O7/TiO2 NTAs photoelectrodes showed extensive potential applications in environmental pollution and green resource exploitation. |
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Moreover, the construction of direct Z-scheme Bi2Sn2O7/TiO2 NTAs heterojunction was beneficial to the photoelectron transfer and active radical formation, and the experimental results indicated that •OH and •O2 - were the decisive species for the dye degradation. The samples also exhibited outstanding photocatalytic water splitting for H2 evolution, and the high efficiency (306.36 μmol·cm−2·h−1) and stability were confirmed. 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ELSEVIER</subfield><subfield code="t">Soil and water bioengineering: Practice and research needs for reconciling natural hazard control and ecological restoration</subfield><subfield code="d">2018</subfield><subfield code="g">Amsterdam [u.a.]</subfield><subfield code="w">(DE-627)ELV000899798</subfield></datafield><datafield tag="773" ind1="1" ind2="8"><subfield code="g">volume:48</subfield><subfield code="g">year:2022</subfield><subfield code="g">number:3</subfield><subfield code="g">day:1</subfield><subfield code="g">month:02</subfield><subfield code="g">pages:3941-3953</subfield><subfield code="g">extent:13</subfield></datafield><datafield tag="856" ind1="4" ind2="0"><subfield code="u">https://doi.org/10.1016/j.ceramint.2021.10.181</subfield><subfield code="3">Volltext</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_USEFLAG_U</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ELV</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SYSFLAG_U</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SSG-OLC-PHA</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SSG-OPC-GGO</subfield></datafield><datafield tag="936" ind1="b" ind2="k"><subfield code="a">43.12</subfield><subfield code="j">Umweltchemie</subfield><subfield code="q">VZ</subfield></datafield><datafield tag="936" ind1="b" ind2="k"><subfield code="a">43.13</subfield><subfield code="j">Umwelttoxikologie</subfield><subfield code="q">VZ</subfield></datafield><datafield tag="936" ind1="b" ind2="k"><subfield code="a">44.13</subfield><subfield code="j">Medizinische Ökologie</subfield><subfield code="q">VZ</subfield></datafield><datafield tag="951" ind1=" " ind2=" "><subfield code="a">AR</subfield></datafield><datafield tag="952" ind1=" " ind2=" "><subfield code="d">48</subfield><subfield code="j">2022</subfield><subfield code="e">3</subfield><subfield code="b">1</subfield><subfield code="c">0201</subfield><subfield code="h">3941-3953</subfield><subfield code="g">13</subfield></datafield></record></collection>
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