A review on the development of supported non-noble metal catalysts for the endothermic high temperature sulfuric acid decomposition step in the Iodine–Sulfur cycle for hydrogen production
The decomposition of sulfuric acid to sulfur dioxide is an important reaction section in both the thermochemical Iodine–Sulfur (IS) cycle and the Hybrid (Hybs) cycle for hydrogen production. This decomposition reaction is a high temperature, highly endothermic reaction whose activation barrier needs...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Pathak, Shailesh [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2022transfer abstract |
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| Umfang: |
25 |
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| Übergeordnetes Werk: |
Enthalten in: External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs - Dedhia, Kavita ELSEVIER, 2018, official journal of the International Association for Hydrogen Energy, New York, NY [u.a.] |
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| Übergeordnetes Werk: |
volume:47 ; year:2022 ; number:31 ; day:12 ; month:04 ; pages:14186-14210 ; extent:25 |
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| DOI / URN: |
10.1016/j.ijhydene.2022.02.165 |
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| 245 | 1 | 0 | |a A review on the development of supported non-noble metal catalysts for the endothermic high temperature sulfuric acid decomposition step in the Iodine–Sulfur cycle for hydrogen production |
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| 520 | |a The decomposition of sulfuric acid to sulfur dioxide is an important reaction section in both the thermochemical Iodine–Sulfur (IS) cycle and the Hybrid (Hybs) cycle for hydrogen production. This decomposition reaction is a high temperature, highly endothermic reaction whose activation barrier needs to be reduced by a highly active catalyst. The catalysts reported in this reaction are either exorbitantly expensive, synthesized using noble metals, or exhibiting low activity and stability. Hence, the development of non-noble active and stable catalysts in this reaction is a significant challenge. This review comprehensively discusses the recent developments and activity trends of supported non-noble catalysts including their synthesis, activity & stability trends, mechanistic and kinetic aspects. The catalytic activity of nano-catalysts in sulfuric acid decomposition is largely affected by the size of the metal nanoparticles, dispersion, oxygen vacancies, and metal-support interaction. Herein, we report an in-depth theoretical and experimental understanding of the catalytic challenges and solutions that leads to designing a cost-effective, efficient and stable catalyst in this reaction. The role of catalyst support modification for long run stability is also discussed. Further, literature considering reaction kinetics over various catalysts is also reviewed. | ||
| 520 | |a The decomposition of sulfuric acid to sulfur dioxide is an important reaction section in both the thermochemical Iodine–Sulfur (IS) cycle and the Hybrid (Hybs) cycle for hydrogen production. This decomposition reaction is a high temperature, highly endothermic reaction whose activation barrier needs to be reduced by a highly active catalyst. The catalysts reported in this reaction are either exorbitantly expensive, synthesized using noble metals, or exhibiting low activity and stability. Hence, the development of non-noble active and stable catalysts in this reaction is a significant challenge. This review comprehensively discusses the recent developments and activity trends of supported non-noble catalysts including their synthesis, activity & stability trends, mechanistic and kinetic aspects. The catalytic activity of nano-catalysts in sulfuric acid decomposition is largely affected by the size of the metal nanoparticles, dispersion, oxygen vacancies, and metal-support interaction. Herein, we report an in-depth theoretical and experimental understanding of the catalytic challenges and solutions that leads to designing a cost-effective, efficient and stable catalyst in this reaction. The role of catalyst support modification for long run stability is also discussed. Further, literature considering reaction kinetics over various catalysts is also reviewed. | ||
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10.1016/j.ijhydene.2022.02.165 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001733.pica (DE-627)ELV05737371X (ELSEVIER)S0360-3199(22)00779-0 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Pathak, Shailesh verfasserin aut A review on the development of supported non-noble metal catalysts for the endothermic high temperature sulfuric acid decomposition step in the Iodine–Sulfur cycle for hydrogen production 2022transfer abstract 25 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The decomposition of sulfuric acid to sulfur dioxide is an important reaction section in both the thermochemical Iodine–Sulfur (IS) cycle and the Hybrid (Hybs) cycle for hydrogen production. This decomposition reaction is a high temperature, highly endothermic reaction whose activation barrier needs to be reduced by a highly active catalyst. The catalysts reported in this reaction are either exorbitantly expensive, synthesized using noble metals, or exhibiting low activity and stability. Hence, the development of non-noble active and stable catalysts in this reaction is a significant challenge. This review comprehensively discusses the recent developments and activity trends of supported non-noble catalysts including their synthesis, activity & stability trends, mechanistic and kinetic aspects. The catalytic activity of nano-catalysts in sulfuric acid decomposition is largely affected by the size of the metal nanoparticles, dispersion, oxygen vacancies, and metal-support interaction. Herein, we report an in-depth theoretical and experimental understanding of the catalytic challenges and solutions that leads to designing a cost-effective, efficient and stable catalyst in this reaction. The role of catalyst support modification for long run stability is also discussed. Further, literature considering reaction kinetics over various catalysts is also reviewed. The decomposition of sulfuric acid to sulfur dioxide is an important reaction section in both the thermochemical Iodine–Sulfur (IS) cycle and the Hybrid (Hybs) cycle for hydrogen production. This decomposition reaction is a high temperature, highly endothermic reaction whose activation barrier needs to be reduced by a highly active catalyst. The catalysts reported in this reaction are either exorbitantly expensive, synthesized using noble metals, or exhibiting low activity and stability. Hence, the development of non-noble active and stable catalysts in this reaction is a significant challenge. This review comprehensively discusses the recent developments and activity trends of supported non-noble catalysts including their synthesis, activity & stability trends, mechanistic and kinetic aspects. The catalytic activity of nano-catalysts in sulfuric acid decomposition is largely affected by the size of the metal nanoparticles, dispersion, oxygen vacancies, and metal-support interaction. Herein, we report an in-depth theoretical and experimental understanding of the catalytic challenges and solutions that leads to designing a cost-effective, efficient and stable catalyst in this reaction. The role of catalyst support modification for long run stability is also discussed. Further, literature considering reaction kinetics over various catalysts is also reviewed. Kinetics and reaction mechanism Elsevier Iodine–Sulfur process Elsevier Sulfuric acid decomposition Elsevier Non-noble based catalysts Elsevier Hydrogen production Elsevier Catalysts for sulfuric acid decomposition Elsevier Upadhyayula, Sreedevi oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:47 year:2022 number:31 day:12 month:04 pages:14186-14210 extent:25 https://doi.org/10.1016/j.ijhydene.2022.02.165 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 47 2022 31 12 0412 14186-14210 25 |
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10.1016/j.ijhydene.2022.02.165 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001733.pica (DE-627)ELV05737371X (ELSEVIER)S0360-3199(22)00779-0 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Pathak, Shailesh verfasserin aut A review on the development of supported non-noble metal catalysts for the endothermic high temperature sulfuric acid decomposition step in the Iodine–Sulfur cycle for hydrogen production 2022transfer abstract 25 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The decomposition of sulfuric acid to sulfur dioxide is an important reaction section in both the thermochemical Iodine–Sulfur (IS) cycle and the Hybrid (Hybs) cycle for hydrogen production. This decomposition reaction is a high temperature, highly endothermic reaction whose activation barrier needs to be reduced by a highly active catalyst. The catalysts reported in this reaction are either exorbitantly expensive, synthesized using noble metals, or exhibiting low activity and stability. Hence, the development of non-noble active and stable catalysts in this reaction is a significant challenge. This review comprehensively discusses the recent developments and activity trends of supported non-noble catalysts including their synthesis, activity & stability trends, mechanistic and kinetic aspects. The catalytic activity of nano-catalysts in sulfuric acid decomposition is largely affected by the size of the metal nanoparticles, dispersion, oxygen vacancies, and metal-support interaction. Herein, we report an in-depth theoretical and experimental understanding of the catalytic challenges and solutions that leads to designing a cost-effective, efficient and stable catalyst in this reaction. The role of catalyst support modification for long run stability is also discussed. Further, literature considering reaction kinetics over various catalysts is also reviewed. The decomposition of sulfuric acid to sulfur dioxide is an important reaction section in both the thermochemical Iodine–Sulfur (IS) cycle and the Hybrid (Hybs) cycle for hydrogen production. This decomposition reaction is a high temperature, highly endothermic reaction whose activation barrier needs to be reduced by a highly active catalyst. The catalysts reported in this reaction are either exorbitantly expensive, synthesized using noble metals, or exhibiting low activity and stability. Hence, the development of non-noble active and stable catalysts in this reaction is a significant challenge. This review comprehensively discusses the recent developments and activity trends of supported non-noble catalysts including their synthesis, activity & stability trends, mechanistic and kinetic aspects. The catalytic activity of nano-catalysts in sulfuric acid decomposition is largely affected by the size of the metal nanoparticles, dispersion, oxygen vacancies, and metal-support interaction. Herein, we report an in-depth theoretical and experimental understanding of the catalytic challenges and solutions that leads to designing a cost-effective, efficient and stable catalyst in this reaction. The role of catalyst support modification for long run stability is also discussed. Further, literature considering reaction kinetics over various catalysts is also reviewed. Kinetics and reaction mechanism Elsevier Iodine–Sulfur process Elsevier Sulfuric acid decomposition Elsevier Non-noble based catalysts Elsevier Hydrogen production Elsevier Catalysts for sulfuric acid decomposition Elsevier Upadhyayula, Sreedevi oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:47 year:2022 number:31 day:12 month:04 pages:14186-14210 extent:25 https://doi.org/10.1016/j.ijhydene.2022.02.165 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 47 2022 31 12 0412 14186-14210 25 |
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10.1016/j.ijhydene.2022.02.165 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001733.pica (DE-627)ELV05737371X (ELSEVIER)S0360-3199(22)00779-0 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Pathak, Shailesh verfasserin aut A review on the development of supported non-noble metal catalysts for the endothermic high temperature sulfuric acid decomposition step in the Iodine–Sulfur cycle for hydrogen production 2022transfer abstract 25 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The decomposition of sulfuric acid to sulfur dioxide is an important reaction section in both the thermochemical Iodine–Sulfur (IS) cycle and the Hybrid (Hybs) cycle for hydrogen production. This decomposition reaction is a high temperature, highly endothermic reaction whose activation barrier needs to be reduced by a highly active catalyst. The catalysts reported in this reaction are either exorbitantly expensive, synthesized using noble metals, or exhibiting low activity and stability. Hence, the development of non-noble active and stable catalysts in this reaction is a significant challenge. This review comprehensively discusses the recent developments and activity trends of supported non-noble catalysts including their synthesis, activity & stability trends, mechanistic and kinetic aspects. The catalytic activity of nano-catalysts in sulfuric acid decomposition is largely affected by the size of the metal nanoparticles, dispersion, oxygen vacancies, and metal-support interaction. Herein, we report an in-depth theoretical and experimental understanding of the catalytic challenges and solutions that leads to designing a cost-effective, efficient and stable catalyst in this reaction. The role of catalyst support modification for long run stability is also discussed. Further, literature considering reaction kinetics over various catalysts is also reviewed. The decomposition of sulfuric acid to sulfur dioxide is an important reaction section in both the thermochemical Iodine–Sulfur (IS) cycle and the Hybrid (Hybs) cycle for hydrogen production. This decomposition reaction is a high temperature, highly endothermic reaction whose activation barrier needs to be reduced by a highly active catalyst. The catalysts reported in this reaction are either exorbitantly expensive, synthesized using noble metals, or exhibiting low activity and stability. Hence, the development of non-noble active and stable catalysts in this reaction is a significant challenge. This review comprehensively discusses the recent developments and activity trends of supported non-noble catalysts including their synthesis, activity & stability trends, mechanistic and kinetic aspects. The catalytic activity of nano-catalysts in sulfuric acid decomposition is largely affected by the size of the metal nanoparticles, dispersion, oxygen vacancies, and metal-support interaction. Herein, we report an in-depth theoretical and experimental understanding of the catalytic challenges and solutions that leads to designing a cost-effective, efficient and stable catalyst in this reaction. The role of catalyst support modification for long run stability is also discussed. Further, literature considering reaction kinetics over various catalysts is also reviewed. Kinetics and reaction mechanism Elsevier Iodine–Sulfur process Elsevier Sulfuric acid decomposition Elsevier Non-noble based catalysts Elsevier Hydrogen production Elsevier Catalysts for sulfuric acid decomposition Elsevier Upadhyayula, Sreedevi oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:47 year:2022 number:31 day:12 month:04 pages:14186-14210 extent:25 https://doi.org/10.1016/j.ijhydene.2022.02.165 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 47 2022 31 12 0412 14186-14210 25 |
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10.1016/j.ijhydene.2022.02.165 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001733.pica (DE-627)ELV05737371X (ELSEVIER)S0360-3199(22)00779-0 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Pathak, Shailesh verfasserin aut A review on the development of supported non-noble metal catalysts for the endothermic high temperature sulfuric acid decomposition step in the Iodine–Sulfur cycle for hydrogen production 2022transfer abstract 25 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The decomposition of sulfuric acid to sulfur dioxide is an important reaction section in both the thermochemical Iodine–Sulfur (IS) cycle and the Hybrid (Hybs) cycle for hydrogen production. This decomposition reaction is a high temperature, highly endothermic reaction whose activation barrier needs to be reduced by a highly active catalyst. The catalysts reported in this reaction are either exorbitantly expensive, synthesized using noble metals, or exhibiting low activity and stability. Hence, the development of non-noble active and stable catalysts in this reaction is a significant challenge. This review comprehensively discusses the recent developments and activity trends of supported non-noble catalysts including their synthesis, activity & stability trends, mechanistic and kinetic aspects. The catalytic activity of nano-catalysts in sulfuric acid decomposition is largely affected by the size of the metal nanoparticles, dispersion, oxygen vacancies, and metal-support interaction. Herein, we report an in-depth theoretical and experimental understanding of the catalytic challenges and solutions that leads to designing a cost-effective, efficient and stable catalyst in this reaction. The role of catalyst support modification for long run stability is also discussed. Further, literature considering reaction kinetics over various catalysts is also reviewed. The decomposition of sulfuric acid to sulfur dioxide is an important reaction section in both the thermochemical Iodine–Sulfur (IS) cycle and the Hybrid (Hybs) cycle for hydrogen production. This decomposition reaction is a high temperature, highly endothermic reaction whose activation barrier needs to be reduced by a highly active catalyst. The catalysts reported in this reaction are either exorbitantly expensive, synthesized using noble metals, or exhibiting low activity and stability. Hence, the development of non-noble active and stable catalysts in this reaction is a significant challenge. This review comprehensively discusses the recent developments and activity trends of supported non-noble catalysts including their synthesis, activity & stability trends, mechanistic and kinetic aspects. The catalytic activity of nano-catalysts in sulfuric acid decomposition is largely affected by the size of the metal nanoparticles, dispersion, oxygen vacancies, and metal-support interaction. Herein, we report an in-depth theoretical and experimental understanding of the catalytic challenges and solutions that leads to designing a cost-effective, efficient and stable catalyst in this reaction. The role of catalyst support modification for long run stability is also discussed. Further, literature considering reaction kinetics over various catalysts is also reviewed. Kinetics and reaction mechanism Elsevier Iodine–Sulfur process Elsevier Sulfuric acid decomposition Elsevier Non-noble based catalysts Elsevier Hydrogen production Elsevier Catalysts for sulfuric acid decomposition Elsevier Upadhyayula, Sreedevi oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:47 year:2022 number:31 day:12 month:04 pages:14186-14210 extent:25 https://doi.org/10.1016/j.ijhydene.2022.02.165 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 47 2022 31 12 0412 14186-14210 25 |
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10.1016/j.ijhydene.2022.02.165 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001733.pica (DE-627)ELV05737371X (ELSEVIER)S0360-3199(22)00779-0 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Pathak, Shailesh verfasserin aut A review on the development of supported non-noble metal catalysts for the endothermic high temperature sulfuric acid decomposition step in the Iodine–Sulfur cycle for hydrogen production 2022transfer abstract 25 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The decomposition of sulfuric acid to sulfur dioxide is an important reaction section in both the thermochemical Iodine–Sulfur (IS) cycle and the Hybrid (Hybs) cycle for hydrogen production. This decomposition reaction is a high temperature, highly endothermic reaction whose activation barrier needs to be reduced by a highly active catalyst. The catalysts reported in this reaction are either exorbitantly expensive, synthesized using noble metals, or exhibiting low activity and stability. Hence, the development of non-noble active and stable catalysts in this reaction is a significant challenge. This review comprehensively discusses the recent developments and activity trends of supported non-noble catalysts including their synthesis, activity & stability trends, mechanistic and kinetic aspects. The catalytic activity of nano-catalysts in sulfuric acid decomposition is largely affected by the size of the metal nanoparticles, dispersion, oxygen vacancies, and metal-support interaction. Herein, we report an in-depth theoretical and experimental understanding of the catalytic challenges and solutions that leads to designing a cost-effective, efficient and stable catalyst in this reaction. The role of catalyst support modification for long run stability is also discussed. Further, literature considering reaction kinetics over various catalysts is also reviewed. The decomposition of sulfuric acid to sulfur dioxide is an important reaction section in both the thermochemical Iodine–Sulfur (IS) cycle and the Hybrid (Hybs) cycle for hydrogen production. This decomposition reaction is a high temperature, highly endothermic reaction whose activation barrier needs to be reduced by a highly active catalyst. The catalysts reported in this reaction are either exorbitantly expensive, synthesized using noble metals, or exhibiting low activity and stability. Hence, the development of non-noble active and stable catalysts in this reaction is a significant challenge. This review comprehensively discusses the recent developments and activity trends of supported non-noble catalysts including their synthesis, activity & stability trends, mechanistic and kinetic aspects. The catalytic activity of nano-catalysts in sulfuric acid decomposition is largely affected by the size of the metal nanoparticles, dispersion, oxygen vacancies, and metal-support interaction. Herein, we report an in-depth theoretical and experimental understanding of the catalytic challenges and solutions that leads to designing a cost-effective, efficient and stable catalyst in this reaction. The role of catalyst support modification for long run stability is also discussed. Further, literature considering reaction kinetics over various catalysts is also reviewed. Kinetics and reaction mechanism Elsevier Iodine–Sulfur process Elsevier Sulfuric acid decomposition Elsevier Non-noble based catalysts Elsevier Hydrogen production Elsevier Catalysts for sulfuric acid decomposition Elsevier Upadhyayula, Sreedevi oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:47 year:2022 number:31 day:12 month:04 pages:14186-14210 extent:25 https://doi.org/10.1016/j.ijhydene.2022.02.165 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 47 2022 31 12 0412 14186-14210 25 |
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Enthalten in External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs New York, NY [u.a.] volume:47 year:2022 number:31 day:12 month:04 pages:14186-14210 extent:25 |
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Enthalten in External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs New York, NY [u.a.] volume:47 year:2022 number:31 day:12 month:04 pages:14186-14210 extent:25 |
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a review on the development of supported non-noble metal catalysts for the endothermic high temperature sulfuric acid decomposition step in the iodine–sulfur cycle for hydrogen production |
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A review on the development of supported non-noble metal catalysts for the endothermic high temperature sulfuric acid decomposition step in the Iodine–Sulfur cycle for hydrogen production |
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The decomposition of sulfuric acid to sulfur dioxide is an important reaction section in both the thermochemical Iodine–Sulfur (IS) cycle and the Hybrid (Hybs) cycle for hydrogen production. This decomposition reaction is a high temperature, highly endothermic reaction whose activation barrier needs to be reduced by a highly active catalyst. The catalysts reported in this reaction are either exorbitantly expensive, synthesized using noble metals, or exhibiting low activity and stability. Hence, the development of non-noble active and stable catalysts in this reaction is a significant challenge. This review comprehensively discusses the recent developments and activity trends of supported non-noble catalysts including their synthesis, activity & stability trends, mechanistic and kinetic aspects. The catalytic activity of nano-catalysts in sulfuric acid decomposition is largely affected by the size of the metal nanoparticles, dispersion, oxygen vacancies, and metal-support interaction. Herein, we report an in-depth theoretical and experimental understanding of the catalytic challenges and solutions that leads to designing a cost-effective, efficient and stable catalyst in this reaction. The role of catalyst support modification for long run stability is also discussed. Further, literature considering reaction kinetics over various catalysts is also reviewed. |
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The decomposition of sulfuric acid to sulfur dioxide is an important reaction section in both the thermochemical Iodine–Sulfur (IS) cycle and the Hybrid (Hybs) cycle for hydrogen production. This decomposition reaction is a high temperature, highly endothermic reaction whose activation barrier needs to be reduced by a highly active catalyst. The catalysts reported in this reaction are either exorbitantly expensive, synthesized using noble metals, or exhibiting low activity and stability. Hence, the development of non-noble active and stable catalysts in this reaction is a significant challenge. This review comprehensively discusses the recent developments and activity trends of supported non-noble catalysts including their synthesis, activity & stability trends, mechanistic and kinetic aspects. The catalytic activity of nano-catalysts in sulfuric acid decomposition is largely affected by the size of the metal nanoparticles, dispersion, oxygen vacancies, and metal-support interaction. Herein, we report an in-depth theoretical and experimental understanding of the catalytic challenges and solutions that leads to designing a cost-effective, efficient and stable catalyst in this reaction. The role of catalyst support modification for long run stability is also discussed. Further, literature considering reaction kinetics over various catalysts is also reviewed. |
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The decomposition of sulfuric acid to sulfur dioxide is an important reaction section in both the thermochemical Iodine–Sulfur (IS) cycle and the Hybrid (Hybs) cycle for hydrogen production. This decomposition reaction is a high temperature, highly endothermic reaction whose activation barrier needs to be reduced by a highly active catalyst. The catalysts reported in this reaction are either exorbitantly expensive, synthesized using noble metals, or exhibiting low activity and stability. Hence, the development of non-noble active and stable catalysts in this reaction is a significant challenge. This review comprehensively discusses the recent developments and activity trends of supported non-noble catalysts including their synthesis, activity & stability trends, mechanistic and kinetic aspects. The catalytic activity of nano-catalysts in sulfuric acid decomposition is largely affected by the size of the metal nanoparticles, dispersion, oxygen vacancies, and metal-support interaction. Herein, we report an in-depth theoretical and experimental understanding of the catalytic challenges and solutions that leads to designing a cost-effective, efficient and stable catalyst in this reaction. The role of catalyst support modification for long run stability is also discussed. Further, literature considering reaction kinetics over various catalysts is also reviewed. |
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