Improving the stability of NASICON-type electrolyte with Li metal anode by interfacial modification
Sodium super-ionic conductors (NASICON)-type electrolyte Li1.4Al0.4Ti1.6(PO4)3 (LATP), with high ionic conductivity and low cost, is considered as one of the most attractive alternatives to liquid electrolytes. However, the poor interfacial compatibilities of LATP electrolyte in lithium batteries le...
Ausführliche Beschreibung
Autor*in: |
Huang, Can [verfasserIn] |
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E-Artikel |
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Sprache: |
Englisch |
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2022transfer abstract |
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Übergeordnetes Werk: |
Enthalten in: Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method - Xiao, Hong ELSEVIER, 2013, the international journal on the science and technology of electrochemical energy systems, New York, NY [u.a.] |
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Übergeordnetes Werk: |
volume:536 ; year:2022 ; day:15 ; month:07 ; pages:0 |
Links: |
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DOI / URN: |
10.1016/j.jpowsour.2022.231491 |
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Katalog-ID: |
ELV057604797 |
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520 | |a Sodium super-ionic conductors (NASICON)-type electrolyte Li1.4Al0.4Ti1.6(PO4)3 (LATP), with high ionic conductivity and low cost, is considered as one of the most attractive alternatives to liquid electrolytes. However, the poor interfacial compatibilities of LATP electrolyte in lithium batteries lead to the failure, which hinders its further development. Herein, a MoS2 coating layer as an artificial solid electrolyte interphase (ASEI) is used for modifying the surface of LATP (MCLATP) via an economical and uncomplicated spin coating method, which not only effectively inhibits the decomposition of LATP, but also in-situ forms a conversion layer consisting of Li2S and Mo metal during cycling. The conversion layer can improve the interfacial charge transfer kinetics and decrease the charge transfer resistance. According to interfacial modification of MoS2, the symmetric cells show slight polarization, and the Li/MCLATP/LFP cells demonstrate excellent cycling performance over 300 cycles at 1 C. The enhanced batteries performance is ascribed to interfacial modification of MoS2 as an ASEI layer, which reduces interfacial concentration polarization caused by the formed microcracks around the surface during decomposition of LATP. This work provides a promising strategy to construct the interface between Li metal and solid-state electrolytes for other unstable electrolytes beyond NASICON. | ||
520 | |a Sodium super-ionic conductors (NASICON)-type electrolyte Li1.4Al0.4Ti1.6(PO4)3 (LATP), with high ionic conductivity and low cost, is considered as one of the most attractive alternatives to liquid electrolytes. However, the poor interfacial compatibilities of LATP electrolyte in lithium batteries lead to the failure, which hinders its further development. Herein, a MoS2 coating layer as an artificial solid electrolyte interphase (ASEI) is used for modifying the surface of LATP (MCLATP) via an economical and uncomplicated spin coating method, which not only effectively inhibits the decomposition of LATP, but also in-situ forms a conversion layer consisting of Li2S and Mo metal during cycling. The conversion layer can improve the interfacial charge transfer kinetics and decrease the charge transfer resistance. According to interfacial modification of MoS2, the symmetric cells show slight polarization, and the Li/MCLATP/LFP cells demonstrate excellent cycling performance over 300 cycles at 1 C. The enhanced batteries performance is ascribed to interfacial modification of MoS2 as an ASEI layer, which reduces interfacial concentration polarization caused by the formed microcracks around the surface during decomposition of LATP. This work provides a promising strategy to construct the interface between Li metal and solid-state electrolytes for other unstable electrolytes beyond NASICON. | ||
650 | 7 | |a Lithium metal batteries |2 Elsevier | |
650 | 7 | |a LATP |2 Elsevier | |
650 | 7 | |a Artificial SEI |2 Elsevier | |
650 | 7 | |a MoS2 |2 Elsevier | |
650 | 7 | |a NASICON |2 Elsevier | |
700 | 1 | |a Li, Zhuojie |4 oth | |
700 | 1 | |a Duan, Shanshan |4 oth | |
700 | 1 | |a Xie, Shuhong |4 oth | |
700 | 1 | |a Yuan, Shuoguo |4 oth | |
700 | 1 | |a Hou, Shuen |4 oth | |
700 | 1 | |a Cao, Guozhong |4 oth | |
700 | 1 | |a Jin, Hongyun |4 oth | |
773 | 0 | 8 | |i Enthalten in |n Elsevier |a Xiao, Hong ELSEVIER |t Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method |d 2013 |d the international journal on the science and technology of electrochemical energy systems |g New York, NY [u.a.] |w (DE-627)ELV00098745X |
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10.1016/j.jpowsour.2022.231491 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001808.pica (DE-627)ELV057604797 (ELSEVIER)S0378-7753(22)00498-0 DE-627 ger DE-627 rakwb eng 690 VZ 50.92 bkl Huang, Can verfasserin aut Improving the stability of NASICON-type electrolyte with Li metal anode by interfacial modification 2022transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Sodium super-ionic conductors (NASICON)-type electrolyte Li1.4Al0.4Ti1.6(PO4)3 (LATP), with high ionic conductivity and low cost, is considered as one of the most attractive alternatives to liquid electrolytes. However, the poor interfacial compatibilities of LATP electrolyte in lithium batteries lead to the failure, which hinders its further development. Herein, a MoS2 coating layer as an artificial solid electrolyte interphase (ASEI) is used for modifying the surface of LATP (MCLATP) via an economical and uncomplicated spin coating method, which not only effectively inhibits the decomposition of LATP, but also in-situ forms a conversion layer consisting of Li2S and Mo metal during cycling. The conversion layer can improve the interfacial charge transfer kinetics and decrease the charge transfer resistance. According to interfacial modification of MoS2, the symmetric cells show slight polarization, and the Li/MCLATP/LFP cells demonstrate excellent cycling performance over 300 cycles at 1 C. The enhanced batteries performance is ascribed to interfacial modification of MoS2 as an ASEI layer, which reduces interfacial concentration polarization caused by the formed microcracks around the surface during decomposition of LATP. This work provides a promising strategy to construct the interface between Li metal and solid-state electrolytes for other unstable electrolytes beyond NASICON. Sodium super-ionic conductors (NASICON)-type electrolyte Li1.4Al0.4Ti1.6(PO4)3 (LATP), with high ionic conductivity and low cost, is considered as one of the most attractive alternatives to liquid electrolytes. However, the poor interfacial compatibilities of LATP electrolyte in lithium batteries lead to the failure, which hinders its further development. Herein, a MoS2 coating layer as an artificial solid electrolyte interphase (ASEI) is used for modifying the surface of LATP (MCLATP) via an economical and uncomplicated spin coating method, which not only effectively inhibits the decomposition of LATP, but also in-situ forms a conversion layer consisting of Li2S and Mo metal during cycling. The conversion layer can improve the interfacial charge transfer kinetics and decrease the charge transfer resistance. According to interfacial modification of MoS2, the symmetric cells show slight polarization, and the Li/MCLATP/LFP cells demonstrate excellent cycling performance over 300 cycles at 1 C. The enhanced batteries performance is ascribed to interfacial modification of MoS2 as an ASEI layer, which reduces interfacial concentration polarization caused by the formed microcracks around the surface during decomposition of LATP. This work provides a promising strategy to construct the interface between Li metal and solid-state electrolytes for other unstable electrolytes beyond NASICON. Lithium metal batteries Elsevier LATP Elsevier Artificial SEI Elsevier MoS2 Elsevier NASICON Elsevier Li, Zhuojie oth Duan, Shanshan oth Xie, Shuhong oth Yuan, Shuoguo oth Hou, Shuen oth Cao, Guozhong oth Jin, Hongyun oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:536 year:2022 day:15 month:07 pages:0 https://doi.org/10.1016/j.jpowsour.2022.231491 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 536 2022 15 0715 0 |
spelling |
10.1016/j.jpowsour.2022.231491 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001808.pica (DE-627)ELV057604797 (ELSEVIER)S0378-7753(22)00498-0 DE-627 ger DE-627 rakwb eng 690 VZ 50.92 bkl Huang, Can verfasserin aut Improving the stability of NASICON-type electrolyte with Li metal anode by interfacial modification 2022transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Sodium super-ionic conductors (NASICON)-type electrolyte Li1.4Al0.4Ti1.6(PO4)3 (LATP), with high ionic conductivity and low cost, is considered as one of the most attractive alternatives to liquid electrolytes. However, the poor interfacial compatibilities of LATP electrolyte in lithium batteries lead to the failure, which hinders its further development. Herein, a MoS2 coating layer as an artificial solid electrolyte interphase (ASEI) is used for modifying the surface of LATP (MCLATP) via an economical and uncomplicated spin coating method, which not only effectively inhibits the decomposition of LATP, but also in-situ forms a conversion layer consisting of Li2S and Mo metal during cycling. The conversion layer can improve the interfacial charge transfer kinetics and decrease the charge transfer resistance. According to interfacial modification of MoS2, the symmetric cells show slight polarization, and the Li/MCLATP/LFP cells demonstrate excellent cycling performance over 300 cycles at 1 C. The enhanced batteries performance is ascribed to interfacial modification of MoS2 as an ASEI layer, which reduces interfacial concentration polarization caused by the formed microcracks around the surface during decomposition of LATP. This work provides a promising strategy to construct the interface between Li metal and solid-state electrolytes for other unstable electrolytes beyond NASICON. Sodium super-ionic conductors (NASICON)-type electrolyte Li1.4Al0.4Ti1.6(PO4)3 (LATP), with high ionic conductivity and low cost, is considered as one of the most attractive alternatives to liquid electrolytes. However, the poor interfacial compatibilities of LATP electrolyte in lithium batteries lead to the failure, which hinders its further development. Herein, a MoS2 coating layer as an artificial solid electrolyte interphase (ASEI) is used for modifying the surface of LATP (MCLATP) via an economical and uncomplicated spin coating method, which not only effectively inhibits the decomposition of LATP, but also in-situ forms a conversion layer consisting of Li2S and Mo metal during cycling. The conversion layer can improve the interfacial charge transfer kinetics and decrease the charge transfer resistance. According to interfacial modification of MoS2, the symmetric cells show slight polarization, and the Li/MCLATP/LFP cells demonstrate excellent cycling performance over 300 cycles at 1 C. The enhanced batteries performance is ascribed to interfacial modification of MoS2 as an ASEI layer, which reduces interfacial concentration polarization caused by the formed microcracks around the surface during decomposition of LATP. This work provides a promising strategy to construct the interface between Li metal and solid-state electrolytes for other unstable electrolytes beyond NASICON. Lithium metal batteries Elsevier LATP Elsevier Artificial SEI Elsevier MoS2 Elsevier NASICON Elsevier Li, Zhuojie oth Duan, Shanshan oth Xie, Shuhong oth Yuan, Shuoguo oth Hou, Shuen oth Cao, Guozhong oth Jin, Hongyun oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:536 year:2022 day:15 month:07 pages:0 https://doi.org/10.1016/j.jpowsour.2022.231491 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 536 2022 15 0715 0 |
allfields_unstemmed |
10.1016/j.jpowsour.2022.231491 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001808.pica (DE-627)ELV057604797 (ELSEVIER)S0378-7753(22)00498-0 DE-627 ger DE-627 rakwb eng 690 VZ 50.92 bkl Huang, Can verfasserin aut Improving the stability of NASICON-type electrolyte with Li metal anode by interfacial modification 2022transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Sodium super-ionic conductors (NASICON)-type electrolyte Li1.4Al0.4Ti1.6(PO4)3 (LATP), with high ionic conductivity and low cost, is considered as one of the most attractive alternatives to liquid electrolytes. However, the poor interfacial compatibilities of LATP electrolyte in lithium batteries lead to the failure, which hinders its further development. Herein, a MoS2 coating layer as an artificial solid electrolyte interphase (ASEI) is used for modifying the surface of LATP (MCLATP) via an economical and uncomplicated spin coating method, which not only effectively inhibits the decomposition of LATP, but also in-situ forms a conversion layer consisting of Li2S and Mo metal during cycling. The conversion layer can improve the interfacial charge transfer kinetics and decrease the charge transfer resistance. According to interfacial modification of MoS2, the symmetric cells show slight polarization, and the Li/MCLATP/LFP cells demonstrate excellent cycling performance over 300 cycles at 1 C. The enhanced batteries performance is ascribed to interfacial modification of MoS2 as an ASEI layer, which reduces interfacial concentration polarization caused by the formed microcracks around the surface during decomposition of LATP. This work provides a promising strategy to construct the interface between Li metal and solid-state electrolytes for other unstable electrolytes beyond NASICON. Sodium super-ionic conductors (NASICON)-type electrolyte Li1.4Al0.4Ti1.6(PO4)3 (LATP), with high ionic conductivity and low cost, is considered as one of the most attractive alternatives to liquid electrolytes. However, the poor interfacial compatibilities of LATP electrolyte in lithium batteries lead to the failure, which hinders its further development. Herein, a MoS2 coating layer as an artificial solid electrolyte interphase (ASEI) is used for modifying the surface of LATP (MCLATP) via an economical and uncomplicated spin coating method, which not only effectively inhibits the decomposition of LATP, but also in-situ forms a conversion layer consisting of Li2S and Mo metal during cycling. The conversion layer can improve the interfacial charge transfer kinetics and decrease the charge transfer resistance. According to interfacial modification of MoS2, the symmetric cells show slight polarization, and the Li/MCLATP/LFP cells demonstrate excellent cycling performance over 300 cycles at 1 C. The enhanced batteries performance is ascribed to interfacial modification of MoS2 as an ASEI layer, which reduces interfacial concentration polarization caused by the formed microcracks around the surface during decomposition of LATP. This work provides a promising strategy to construct the interface between Li metal and solid-state electrolytes for other unstable electrolytes beyond NASICON. Lithium metal batteries Elsevier LATP Elsevier Artificial SEI Elsevier MoS2 Elsevier NASICON Elsevier Li, Zhuojie oth Duan, Shanshan oth Xie, Shuhong oth Yuan, Shuoguo oth Hou, Shuen oth Cao, Guozhong oth Jin, Hongyun oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:536 year:2022 day:15 month:07 pages:0 https://doi.org/10.1016/j.jpowsour.2022.231491 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 536 2022 15 0715 0 |
allfieldsGer |
10.1016/j.jpowsour.2022.231491 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001808.pica (DE-627)ELV057604797 (ELSEVIER)S0378-7753(22)00498-0 DE-627 ger DE-627 rakwb eng 690 VZ 50.92 bkl Huang, Can verfasserin aut Improving the stability of NASICON-type electrolyte with Li metal anode by interfacial modification 2022transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Sodium super-ionic conductors (NASICON)-type electrolyte Li1.4Al0.4Ti1.6(PO4)3 (LATP), with high ionic conductivity and low cost, is considered as one of the most attractive alternatives to liquid electrolytes. However, the poor interfacial compatibilities of LATP electrolyte in lithium batteries lead to the failure, which hinders its further development. Herein, a MoS2 coating layer as an artificial solid electrolyte interphase (ASEI) is used for modifying the surface of LATP (MCLATP) via an economical and uncomplicated spin coating method, which not only effectively inhibits the decomposition of LATP, but also in-situ forms a conversion layer consisting of Li2S and Mo metal during cycling. The conversion layer can improve the interfacial charge transfer kinetics and decrease the charge transfer resistance. According to interfacial modification of MoS2, the symmetric cells show slight polarization, and the Li/MCLATP/LFP cells demonstrate excellent cycling performance over 300 cycles at 1 C. The enhanced batteries performance is ascribed to interfacial modification of MoS2 as an ASEI layer, which reduces interfacial concentration polarization caused by the formed microcracks around the surface during decomposition of LATP. This work provides a promising strategy to construct the interface between Li metal and solid-state electrolytes for other unstable electrolytes beyond NASICON. Sodium super-ionic conductors (NASICON)-type electrolyte Li1.4Al0.4Ti1.6(PO4)3 (LATP), with high ionic conductivity and low cost, is considered as one of the most attractive alternatives to liquid electrolytes. However, the poor interfacial compatibilities of LATP electrolyte in lithium batteries lead to the failure, which hinders its further development. Herein, a MoS2 coating layer as an artificial solid electrolyte interphase (ASEI) is used for modifying the surface of LATP (MCLATP) via an economical and uncomplicated spin coating method, which not only effectively inhibits the decomposition of LATP, but also in-situ forms a conversion layer consisting of Li2S and Mo metal during cycling. The conversion layer can improve the interfacial charge transfer kinetics and decrease the charge transfer resistance. According to interfacial modification of MoS2, the symmetric cells show slight polarization, and the Li/MCLATP/LFP cells demonstrate excellent cycling performance over 300 cycles at 1 C. The enhanced batteries performance is ascribed to interfacial modification of MoS2 as an ASEI layer, which reduces interfacial concentration polarization caused by the formed microcracks around the surface during decomposition of LATP. This work provides a promising strategy to construct the interface between Li metal and solid-state electrolytes for other unstable electrolytes beyond NASICON. Lithium metal batteries Elsevier LATP Elsevier Artificial SEI Elsevier MoS2 Elsevier NASICON Elsevier Li, Zhuojie oth Duan, Shanshan oth Xie, Shuhong oth Yuan, Shuoguo oth Hou, Shuen oth Cao, Guozhong oth Jin, Hongyun oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:536 year:2022 day:15 month:07 pages:0 https://doi.org/10.1016/j.jpowsour.2022.231491 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 536 2022 15 0715 0 |
allfieldsSound |
10.1016/j.jpowsour.2022.231491 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001808.pica (DE-627)ELV057604797 (ELSEVIER)S0378-7753(22)00498-0 DE-627 ger DE-627 rakwb eng 690 VZ 50.92 bkl Huang, Can verfasserin aut Improving the stability of NASICON-type electrolyte with Li metal anode by interfacial modification 2022transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Sodium super-ionic conductors (NASICON)-type electrolyte Li1.4Al0.4Ti1.6(PO4)3 (LATP), with high ionic conductivity and low cost, is considered as one of the most attractive alternatives to liquid electrolytes. However, the poor interfacial compatibilities of LATP electrolyte in lithium batteries lead to the failure, which hinders its further development. Herein, a MoS2 coating layer as an artificial solid electrolyte interphase (ASEI) is used for modifying the surface of LATP (MCLATP) via an economical and uncomplicated spin coating method, which not only effectively inhibits the decomposition of LATP, but also in-situ forms a conversion layer consisting of Li2S and Mo metal during cycling. The conversion layer can improve the interfacial charge transfer kinetics and decrease the charge transfer resistance. According to interfacial modification of MoS2, the symmetric cells show slight polarization, and the Li/MCLATP/LFP cells demonstrate excellent cycling performance over 300 cycles at 1 C. The enhanced batteries performance is ascribed to interfacial modification of MoS2 as an ASEI layer, which reduces interfacial concentration polarization caused by the formed microcracks around the surface during decomposition of LATP. This work provides a promising strategy to construct the interface between Li metal and solid-state electrolytes for other unstable electrolytes beyond NASICON. Sodium super-ionic conductors (NASICON)-type electrolyte Li1.4Al0.4Ti1.6(PO4)3 (LATP), with high ionic conductivity and low cost, is considered as one of the most attractive alternatives to liquid electrolytes. However, the poor interfacial compatibilities of LATP electrolyte in lithium batteries lead to the failure, which hinders its further development. Herein, a MoS2 coating layer as an artificial solid electrolyte interphase (ASEI) is used for modifying the surface of LATP (MCLATP) via an economical and uncomplicated spin coating method, which not only effectively inhibits the decomposition of LATP, but also in-situ forms a conversion layer consisting of Li2S and Mo metal during cycling. The conversion layer can improve the interfacial charge transfer kinetics and decrease the charge transfer resistance. According to interfacial modification of MoS2, the symmetric cells show slight polarization, and the Li/MCLATP/LFP cells demonstrate excellent cycling performance over 300 cycles at 1 C. The enhanced batteries performance is ascribed to interfacial modification of MoS2 as an ASEI layer, which reduces interfacial concentration polarization caused by the formed microcracks around the surface during decomposition of LATP. This work provides a promising strategy to construct the interface between Li metal and solid-state electrolytes for other unstable electrolytes beyond NASICON. Lithium metal batteries Elsevier LATP Elsevier Artificial SEI Elsevier MoS2 Elsevier NASICON Elsevier Li, Zhuojie oth Duan, Shanshan oth Xie, Shuhong oth Yuan, Shuoguo oth Hou, Shuen oth Cao, Guozhong oth Jin, Hongyun oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:536 year:2022 day:15 month:07 pages:0 https://doi.org/10.1016/j.jpowsour.2022.231491 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 536 2022 15 0715 0 |
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Enthalten in Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method New York, NY [u.a.] volume:536 year:2022 day:15 month:07 pages:0 |
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Enthalten in Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method New York, NY [u.a.] volume:536 year:2022 day:15 month:07 pages:0 |
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Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method |
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improving the stability of nasicon-type electrolyte with li metal anode by interfacial modification |
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Improving the stability of NASICON-type electrolyte with Li metal anode by interfacial modification |
abstract |
Sodium super-ionic conductors (NASICON)-type electrolyte Li1.4Al0.4Ti1.6(PO4)3 (LATP), with high ionic conductivity and low cost, is considered as one of the most attractive alternatives to liquid electrolytes. However, the poor interfacial compatibilities of LATP electrolyte in lithium batteries lead to the failure, which hinders its further development. Herein, a MoS2 coating layer as an artificial solid electrolyte interphase (ASEI) is used for modifying the surface of LATP (MCLATP) via an economical and uncomplicated spin coating method, which not only effectively inhibits the decomposition of LATP, but also in-situ forms a conversion layer consisting of Li2S and Mo metal during cycling. The conversion layer can improve the interfacial charge transfer kinetics and decrease the charge transfer resistance. According to interfacial modification of MoS2, the symmetric cells show slight polarization, and the Li/MCLATP/LFP cells demonstrate excellent cycling performance over 300 cycles at 1 C. The enhanced batteries performance is ascribed to interfacial modification of MoS2 as an ASEI layer, which reduces interfacial concentration polarization caused by the formed microcracks around the surface during decomposition of LATP. This work provides a promising strategy to construct the interface between Li metal and solid-state electrolytes for other unstable electrolytes beyond NASICON. |
abstractGer |
Sodium super-ionic conductors (NASICON)-type electrolyte Li1.4Al0.4Ti1.6(PO4)3 (LATP), with high ionic conductivity and low cost, is considered as one of the most attractive alternatives to liquid electrolytes. However, the poor interfacial compatibilities of LATP electrolyte in lithium batteries lead to the failure, which hinders its further development. Herein, a MoS2 coating layer as an artificial solid electrolyte interphase (ASEI) is used for modifying the surface of LATP (MCLATP) via an economical and uncomplicated spin coating method, which not only effectively inhibits the decomposition of LATP, but also in-situ forms a conversion layer consisting of Li2S and Mo metal during cycling. The conversion layer can improve the interfacial charge transfer kinetics and decrease the charge transfer resistance. According to interfacial modification of MoS2, the symmetric cells show slight polarization, and the Li/MCLATP/LFP cells demonstrate excellent cycling performance over 300 cycles at 1 C. The enhanced batteries performance is ascribed to interfacial modification of MoS2 as an ASEI layer, which reduces interfacial concentration polarization caused by the formed microcracks around the surface during decomposition of LATP. This work provides a promising strategy to construct the interface between Li metal and solid-state electrolytes for other unstable electrolytes beyond NASICON. |
abstract_unstemmed |
Sodium super-ionic conductors (NASICON)-type electrolyte Li1.4Al0.4Ti1.6(PO4)3 (LATP), with high ionic conductivity and low cost, is considered as one of the most attractive alternatives to liquid electrolytes. However, the poor interfacial compatibilities of LATP electrolyte in lithium batteries lead to the failure, which hinders its further development. Herein, a MoS2 coating layer as an artificial solid electrolyte interphase (ASEI) is used for modifying the surface of LATP (MCLATP) via an economical and uncomplicated spin coating method, which not only effectively inhibits the decomposition of LATP, but also in-situ forms a conversion layer consisting of Li2S and Mo metal during cycling. The conversion layer can improve the interfacial charge transfer kinetics and decrease the charge transfer resistance. According to interfacial modification of MoS2, the symmetric cells show slight polarization, and the Li/MCLATP/LFP cells demonstrate excellent cycling performance over 300 cycles at 1 C. The enhanced batteries performance is ascribed to interfacial modification of MoS2 as an ASEI layer, which reduces interfacial concentration polarization caused by the formed microcracks around the surface during decomposition of LATP. This work provides a promising strategy to construct the interface between Li metal and solid-state electrolytes for other unstable electrolytes beyond NASICON. |
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title_short |
Improving the stability of NASICON-type electrolyte with Li metal anode by interfacial modification |
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Li, Zhuojie Duan, Shanshan Xie, Shuhong Yuan, Shuoguo Hou, Shuen Cao, Guozhong Jin, Hongyun |
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