Bridge-linking interfacial engineering of triple carbons for highly efficient and binder-free electrodes toward flexible Zn-air batteries
Reasonable modulation of catalyst/substrate interface still remains great challenge for binder-free and high-performance electrodes. Herein, interfacial engineering via bridge-linking is proposed to effectively integrate powdery catalysts with flexible substrates by in situ synthesized nanocarbon. C...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Zheng, Xiangjun [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2022transfer abstract |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Comparability studies of hemin from two different origins porcine and bovine in the production of - Beri, Suresh ELSEVIER, 2020, an international journal devoted to catalytic science and its applications, Amsterdam |
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| Übergeordnetes Werk: |
volume:319 ; year:2022 ; day:15 ; month:12 ; pages:0 |
| Links: |
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| DOI / URN: |
10.1016/j.apcatb.2022.121937 |
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| 520 | |a Reasonable modulation of catalyst/substrate interface still remains great challenge for binder-free and high-performance electrodes. Herein, interfacial engineering via bridge-linking is proposed to effectively integrate powdery catalysts with flexible substrates by in situ synthesized nanocarbon. Concretely, a binder-free CNTs on carbonized carbon cloth linked with N-doped nanocarbons (CNTs-NC-CCC) electrode is formed via self-assembly and covalent coupling. Experimental results and theoretical calculation disclose that the bridge-linking strategy not only enables the fast electron and mass transfer, but also modifies the charge distribution and optimizes the adsorption/desorption process of oxygenated intermediates. With these merits, this metal-free catalyst exhibits superb bifunctional ORR/OER electrocatalytic activity with a voltage gap of 0.78 V. Remarkably, when equipped in aqueous and flexible Zn-air batteries, high power density (288, 68 mW cm–2) and enhanced durability are obtained. This facile nanocarbon-linkage strategy opens up a new avenue for the application of powdery catalysts in wearable energy devices. | ||
| 520 | |a Reasonable modulation of catalyst/substrate interface still remains great challenge for binder-free and high-performance electrodes. Herein, interfacial engineering via bridge-linking is proposed to effectively integrate powdery catalysts with flexible substrates by in situ synthesized nanocarbon. Concretely, a binder-free CNTs on carbonized carbon cloth linked with N-doped nanocarbons (CNTs-NC-CCC) electrode is formed via self-assembly and covalent coupling. Experimental results and theoretical calculation disclose that the bridge-linking strategy not only enables the fast electron and mass transfer, but also modifies the charge distribution and optimizes the adsorption/desorption process of oxygenated intermediates. With these merits, this metal-free catalyst exhibits superb bifunctional ORR/OER electrocatalytic activity with a voltage gap of 0.78 V. Remarkably, when equipped in aqueous and flexible Zn-air batteries, high power density (288, 68 mW cm–2) and enhanced durability are obtained. This facile nanocarbon-linkage strategy opens up a new avenue for the application of powdery catalysts in wearable energy devices. | ||
| 650 | 7 | |a Binder-free electrode |2 Elsevier | |
| 650 | 7 | |a Flexible Zn-air batteries |2 Elsevier | |
| 650 | 7 | |a Interfacial engineering |2 Elsevier | |
| 650 | 7 | |a Nanocarbon |2 Elsevier | |
| 650 | 7 | |a Metal-free electrocatalysts |2 Elsevier | |
| 700 | 1 | |a Qian, Yuhang |4 oth | |
| 700 | 1 | |a Gong, Hongyu |4 oth | |
| 700 | 1 | |a Shi, Wenhua |4 oth | |
| 700 | 1 | |a Yan, Jin |4 oth | |
| 700 | 1 | |a Wang, Wentao |4 oth | |
| 700 | 1 | |a Guo, Xingmei |4 oth | |
| 700 | 1 | |a Zhang, Junhao |4 oth | |
| 700 | 1 | |a Cao, Xuecheng |4 oth | |
| 700 | 1 | |a Yang, Ruizhi |4 oth | |
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10.1016/j.apcatb.2022.121937 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001903.pica (DE-627)ELV058947736 (ELSEVIER)S0926-3373(22)00878-5 DE-627 ger DE-627 rakwb eng 570 VZ BIODIV DE-30 fid PHARM DE-84 fid 44.00 bkl Zheng, Xiangjun verfasserin aut Bridge-linking interfacial engineering of triple carbons for highly efficient and binder-free electrodes toward flexible Zn-air batteries 2022transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Reasonable modulation of catalyst/substrate interface still remains great challenge for binder-free and high-performance electrodes. Herein, interfacial engineering via bridge-linking is proposed to effectively integrate powdery catalysts with flexible substrates by in situ synthesized nanocarbon. Concretely, a binder-free CNTs on carbonized carbon cloth linked with N-doped nanocarbons (CNTs-NC-CCC) electrode is formed via self-assembly and covalent coupling. Experimental results and theoretical calculation disclose that the bridge-linking strategy not only enables the fast electron and mass transfer, but also modifies the charge distribution and optimizes the adsorption/desorption process of oxygenated intermediates. With these merits, this metal-free catalyst exhibits superb bifunctional ORR/OER electrocatalytic activity with a voltage gap of 0.78 V. Remarkably, when equipped in aqueous and flexible Zn-air batteries, high power density (288, 68 mW cm–2) and enhanced durability are obtained. This facile nanocarbon-linkage strategy opens up a new avenue for the application of powdery catalysts in wearable energy devices. Reasonable modulation of catalyst/substrate interface still remains great challenge for binder-free and high-performance electrodes. Herein, interfacial engineering via bridge-linking is proposed to effectively integrate powdery catalysts with flexible substrates by in situ synthesized nanocarbon. Concretely, a binder-free CNTs on carbonized carbon cloth linked with N-doped nanocarbons (CNTs-NC-CCC) electrode is formed via self-assembly and covalent coupling. Experimental results and theoretical calculation disclose that the bridge-linking strategy not only enables the fast electron and mass transfer, but also modifies the charge distribution and optimizes the adsorption/desorption process of oxygenated intermediates. With these merits, this metal-free catalyst exhibits superb bifunctional ORR/OER electrocatalytic activity with a voltage gap of 0.78 V. Remarkably, when equipped in aqueous and flexible Zn-air batteries, high power density (288, 68 mW cm–2) and enhanced durability are obtained. This facile nanocarbon-linkage strategy opens up a new avenue for the application of powdery catalysts in wearable energy devices. Binder-free electrode Elsevier Flexible Zn-air batteries Elsevier Interfacial engineering Elsevier Nanocarbon Elsevier Metal-free electrocatalysts Elsevier Qian, Yuhang oth Gong, Hongyu oth Shi, Wenhua oth Yan, Jin oth Wang, Wentao oth Guo, Xingmei oth Zhang, Junhao oth Cao, Xuecheng oth Yang, Ruizhi oth Enthalten in Elsevier Beri, Suresh ELSEVIER Comparability studies of hemin from two different origins porcine and bovine in the production of 2020 an international journal devoted to catalytic science and its applications Amsterdam (DE-627)ELV004775082 volume:319 year:2022 day:15 month:12 pages:0 https://doi.org/10.1016/j.apcatb.2022.121937 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV FID-PHARM SSG-OLC-PHA SSG-OPC-PHA 44.00 Medizin: Allgemeines VZ AR 319 2022 15 1215 0 |
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10.1016/j.apcatb.2022.121937 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001903.pica (DE-627)ELV058947736 (ELSEVIER)S0926-3373(22)00878-5 DE-627 ger DE-627 rakwb eng 570 VZ BIODIV DE-30 fid PHARM DE-84 fid 44.00 bkl Zheng, Xiangjun verfasserin aut Bridge-linking interfacial engineering of triple carbons for highly efficient and binder-free electrodes toward flexible Zn-air batteries 2022transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Reasonable modulation of catalyst/substrate interface still remains great challenge for binder-free and high-performance electrodes. Herein, interfacial engineering via bridge-linking is proposed to effectively integrate powdery catalysts with flexible substrates by in situ synthesized nanocarbon. Concretely, a binder-free CNTs on carbonized carbon cloth linked with N-doped nanocarbons (CNTs-NC-CCC) electrode is formed via self-assembly and covalent coupling. Experimental results and theoretical calculation disclose that the bridge-linking strategy not only enables the fast electron and mass transfer, but also modifies the charge distribution and optimizes the adsorption/desorption process of oxygenated intermediates. With these merits, this metal-free catalyst exhibits superb bifunctional ORR/OER electrocatalytic activity with a voltage gap of 0.78 V. Remarkably, when equipped in aqueous and flexible Zn-air batteries, high power density (288, 68 mW cm–2) and enhanced durability are obtained. This facile nanocarbon-linkage strategy opens up a new avenue for the application of powdery catalysts in wearable energy devices. Reasonable modulation of catalyst/substrate interface still remains great challenge for binder-free and high-performance electrodes. Herein, interfacial engineering via bridge-linking is proposed to effectively integrate powdery catalysts with flexible substrates by in situ synthesized nanocarbon. Concretely, a binder-free CNTs on carbonized carbon cloth linked with N-doped nanocarbons (CNTs-NC-CCC) electrode is formed via self-assembly and covalent coupling. Experimental results and theoretical calculation disclose that the bridge-linking strategy not only enables the fast electron and mass transfer, but also modifies the charge distribution and optimizes the adsorption/desorption process of oxygenated intermediates. With these merits, this metal-free catalyst exhibits superb bifunctional ORR/OER electrocatalytic activity with a voltage gap of 0.78 V. Remarkably, when equipped in aqueous and flexible Zn-air batteries, high power density (288, 68 mW cm–2) and enhanced durability are obtained. This facile nanocarbon-linkage strategy opens up a new avenue for the application of powdery catalysts in wearable energy devices. Binder-free electrode Elsevier Flexible Zn-air batteries Elsevier Interfacial engineering Elsevier Nanocarbon Elsevier Metal-free electrocatalysts Elsevier Qian, Yuhang oth Gong, Hongyu oth Shi, Wenhua oth Yan, Jin oth Wang, Wentao oth Guo, Xingmei oth Zhang, Junhao oth Cao, Xuecheng oth Yang, Ruizhi oth Enthalten in Elsevier Beri, Suresh ELSEVIER Comparability studies of hemin from two different origins porcine and bovine in the production of 2020 an international journal devoted to catalytic science and its applications Amsterdam (DE-627)ELV004775082 volume:319 year:2022 day:15 month:12 pages:0 https://doi.org/10.1016/j.apcatb.2022.121937 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV FID-PHARM SSG-OLC-PHA SSG-OPC-PHA 44.00 Medizin: Allgemeines VZ AR 319 2022 15 1215 0 |
| allfields_unstemmed |
10.1016/j.apcatb.2022.121937 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001903.pica (DE-627)ELV058947736 (ELSEVIER)S0926-3373(22)00878-5 DE-627 ger DE-627 rakwb eng 570 VZ BIODIV DE-30 fid PHARM DE-84 fid 44.00 bkl Zheng, Xiangjun verfasserin aut Bridge-linking interfacial engineering of triple carbons for highly efficient and binder-free electrodes toward flexible Zn-air batteries 2022transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Reasonable modulation of catalyst/substrate interface still remains great challenge for binder-free and high-performance electrodes. Herein, interfacial engineering via bridge-linking is proposed to effectively integrate powdery catalysts with flexible substrates by in situ synthesized nanocarbon. Concretely, a binder-free CNTs on carbonized carbon cloth linked with N-doped nanocarbons (CNTs-NC-CCC) electrode is formed via self-assembly and covalent coupling. Experimental results and theoretical calculation disclose that the bridge-linking strategy not only enables the fast electron and mass transfer, but also modifies the charge distribution and optimizes the adsorption/desorption process of oxygenated intermediates. With these merits, this metal-free catalyst exhibits superb bifunctional ORR/OER electrocatalytic activity with a voltage gap of 0.78 V. Remarkably, when equipped in aqueous and flexible Zn-air batteries, high power density (288, 68 mW cm–2) and enhanced durability are obtained. This facile nanocarbon-linkage strategy opens up a new avenue for the application of powdery catalysts in wearable energy devices. Reasonable modulation of catalyst/substrate interface still remains great challenge for binder-free and high-performance electrodes. Herein, interfacial engineering via bridge-linking is proposed to effectively integrate powdery catalysts with flexible substrates by in situ synthesized nanocarbon. Concretely, a binder-free CNTs on carbonized carbon cloth linked with N-doped nanocarbons (CNTs-NC-CCC) electrode is formed via self-assembly and covalent coupling. Experimental results and theoretical calculation disclose that the bridge-linking strategy not only enables the fast electron and mass transfer, but also modifies the charge distribution and optimizes the adsorption/desorption process of oxygenated intermediates. With these merits, this metal-free catalyst exhibits superb bifunctional ORR/OER electrocatalytic activity with a voltage gap of 0.78 V. Remarkably, when equipped in aqueous and flexible Zn-air batteries, high power density (288, 68 mW cm–2) and enhanced durability are obtained. This facile nanocarbon-linkage strategy opens up a new avenue for the application of powdery catalysts in wearable energy devices. Binder-free electrode Elsevier Flexible Zn-air batteries Elsevier Interfacial engineering Elsevier Nanocarbon Elsevier Metal-free electrocatalysts Elsevier Qian, Yuhang oth Gong, Hongyu oth Shi, Wenhua oth Yan, Jin oth Wang, Wentao oth Guo, Xingmei oth Zhang, Junhao oth Cao, Xuecheng oth Yang, Ruizhi oth Enthalten in Elsevier Beri, Suresh ELSEVIER Comparability studies of hemin from two different origins porcine and bovine in the production of 2020 an international journal devoted to catalytic science and its applications Amsterdam (DE-627)ELV004775082 volume:319 year:2022 day:15 month:12 pages:0 https://doi.org/10.1016/j.apcatb.2022.121937 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV FID-PHARM SSG-OLC-PHA SSG-OPC-PHA 44.00 Medizin: Allgemeines VZ AR 319 2022 15 1215 0 |
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10.1016/j.apcatb.2022.121937 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001903.pica (DE-627)ELV058947736 (ELSEVIER)S0926-3373(22)00878-5 DE-627 ger DE-627 rakwb eng 570 VZ BIODIV DE-30 fid PHARM DE-84 fid 44.00 bkl Zheng, Xiangjun verfasserin aut Bridge-linking interfacial engineering of triple carbons for highly efficient and binder-free electrodes toward flexible Zn-air batteries 2022transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Reasonable modulation of catalyst/substrate interface still remains great challenge for binder-free and high-performance electrodes. Herein, interfacial engineering via bridge-linking is proposed to effectively integrate powdery catalysts with flexible substrates by in situ synthesized nanocarbon. Concretely, a binder-free CNTs on carbonized carbon cloth linked with N-doped nanocarbons (CNTs-NC-CCC) electrode is formed via self-assembly and covalent coupling. Experimental results and theoretical calculation disclose that the bridge-linking strategy not only enables the fast electron and mass transfer, but also modifies the charge distribution and optimizes the adsorption/desorption process of oxygenated intermediates. With these merits, this metal-free catalyst exhibits superb bifunctional ORR/OER electrocatalytic activity with a voltage gap of 0.78 V. Remarkably, when equipped in aqueous and flexible Zn-air batteries, high power density (288, 68 mW cm–2) and enhanced durability are obtained. This facile nanocarbon-linkage strategy opens up a new avenue for the application of powdery catalysts in wearable energy devices. Reasonable modulation of catalyst/substrate interface still remains great challenge for binder-free and high-performance electrodes. Herein, interfacial engineering via bridge-linking is proposed to effectively integrate powdery catalysts with flexible substrates by in situ synthesized nanocarbon. Concretely, a binder-free CNTs on carbonized carbon cloth linked with N-doped nanocarbons (CNTs-NC-CCC) electrode is formed via self-assembly and covalent coupling. Experimental results and theoretical calculation disclose that the bridge-linking strategy not only enables the fast electron and mass transfer, but also modifies the charge distribution and optimizes the adsorption/desorption process of oxygenated intermediates. With these merits, this metal-free catalyst exhibits superb bifunctional ORR/OER electrocatalytic activity with a voltage gap of 0.78 V. Remarkably, when equipped in aqueous and flexible Zn-air batteries, high power density (288, 68 mW cm–2) and enhanced durability are obtained. This facile nanocarbon-linkage strategy opens up a new avenue for the application of powdery catalysts in wearable energy devices. Binder-free electrode Elsevier Flexible Zn-air batteries Elsevier Interfacial engineering Elsevier Nanocarbon Elsevier Metal-free electrocatalysts Elsevier Qian, Yuhang oth Gong, Hongyu oth Shi, Wenhua oth Yan, Jin oth Wang, Wentao oth Guo, Xingmei oth Zhang, Junhao oth Cao, Xuecheng oth Yang, Ruizhi oth Enthalten in Elsevier Beri, Suresh ELSEVIER Comparability studies of hemin from two different origins porcine and bovine in the production of 2020 an international journal devoted to catalytic science and its applications Amsterdam (DE-627)ELV004775082 volume:319 year:2022 day:15 month:12 pages:0 https://doi.org/10.1016/j.apcatb.2022.121937 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV FID-PHARM SSG-OLC-PHA SSG-OPC-PHA 44.00 Medizin: Allgemeines VZ AR 319 2022 15 1215 0 |
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10.1016/j.apcatb.2022.121937 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001903.pica (DE-627)ELV058947736 (ELSEVIER)S0926-3373(22)00878-5 DE-627 ger DE-627 rakwb eng 570 VZ BIODIV DE-30 fid PHARM DE-84 fid 44.00 bkl Zheng, Xiangjun verfasserin aut Bridge-linking interfacial engineering of triple carbons for highly efficient and binder-free electrodes toward flexible Zn-air batteries 2022transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Reasonable modulation of catalyst/substrate interface still remains great challenge for binder-free and high-performance electrodes. Herein, interfacial engineering via bridge-linking is proposed to effectively integrate powdery catalysts with flexible substrates by in situ synthesized nanocarbon. Concretely, a binder-free CNTs on carbonized carbon cloth linked with N-doped nanocarbons (CNTs-NC-CCC) electrode is formed via self-assembly and covalent coupling. Experimental results and theoretical calculation disclose that the bridge-linking strategy not only enables the fast electron and mass transfer, but also modifies the charge distribution and optimizes the adsorption/desorption process of oxygenated intermediates. With these merits, this metal-free catalyst exhibits superb bifunctional ORR/OER electrocatalytic activity with a voltage gap of 0.78 V. Remarkably, when equipped in aqueous and flexible Zn-air batteries, high power density (288, 68 mW cm–2) and enhanced durability are obtained. This facile nanocarbon-linkage strategy opens up a new avenue for the application of powdery catalysts in wearable energy devices. Reasonable modulation of catalyst/substrate interface still remains great challenge for binder-free and high-performance electrodes. Herein, interfacial engineering via bridge-linking is proposed to effectively integrate powdery catalysts with flexible substrates by in situ synthesized nanocarbon. Concretely, a binder-free CNTs on carbonized carbon cloth linked with N-doped nanocarbons (CNTs-NC-CCC) electrode is formed via self-assembly and covalent coupling. Experimental results and theoretical calculation disclose that the bridge-linking strategy not only enables the fast electron and mass transfer, but also modifies the charge distribution and optimizes the adsorption/desorption process of oxygenated intermediates. With these merits, this metal-free catalyst exhibits superb bifunctional ORR/OER electrocatalytic activity with a voltage gap of 0.78 V. Remarkably, when equipped in aqueous and flexible Zn-air batteries, high power density (288, 68 mW cm–2) and enhanced durability are obtained. This facile nanocarbon-linkage strategy opens up a new avenue for the application of powdery catalysts in wearable energy devices. Binder-free electrode Elsevier Flexible Zn-air batteries Elsevier Interfacial engineering Elsevier Nanocarbon Elsevier Metal-free electrocatalysts Elsevier Qian, Yuhang oth Gong, Hongyu oth Shi, Wenhua oth Yan, Jin oth Wang, Wentao oth Guo, Xingmei oth Zhang, Junhao oth Cao, Xuecheng oth Yang, Ruizhi oth Enthalten in Elsevier Beri, Suresh ELSEVIER Comparability studies of hemin from two different origins porcine and bovine in the production of 2020 an international journal devoted to catalytic science and its applications Amsterdam (DE-627)ELV004775082 volume:319 year:2022 day:15 month:12 pages:0 https://doi.org/10.1016/j.apcatb.2022.121937 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV FID-PHARM SSG-OLC-PHA SSG-OPC-PHA 44.00 Medizin: Allgemeines VZ AR 319 2022 15 1215 0 |
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Bridge-linking interfacial engineering of triple carbons for highly efficient and binder-free electrodes toward flexible Zn-air batteries |
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Reasonable modulation of catalyst/substrate interface still remains great challenge for binder-free and high-performance electrodes. Herein, interfacial engineering via bridge-linking is proposed to effectively integrate powdery catalysts with flexible substrates by in situ synthesized nanocarbon. Concretely, a binder-free CNTs on carbonized carbon cloth linked with N-doped nanocarbons (CNTs-NC-CCC) electrode is formed via self-assembly and covalent coupling. Experimental results and theoretical calculation disclose that the bridge-linking strategy not only enables the fast electron and mass transfer, but also modifies the charge distribution and optimizes the adsorption/desorption process of oxygenated intermediates. With these merits, this metal-free catalyst exhibits superb bifunctional ORR/OER electrocatalytic activity with a voltage gap of 0.78 V. Remarkably, when equipped in aqueous and flexible Zn-air batteries, high power density (288, 68 mW cm–2) and enhanced durability are obtained. This facile nanocarbon-linkage strategy opens up a new avenue for the application of powdery catalysts in wearable energy devices. |
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Reasonable modulation of catalyst/substrate interface still remains great challenge for binder-free and high-performance electrodes. Herein, interfacial engineering via bridge-linking is proposed to effectively integrate powdery catalysts with flexible substrates by in situ synthesized nanocarbon. Concretely, a binder-free CNTs on carbonized carbon cloth linked with N-doped nanocarbons (CNTs-NC-CCC) electrode is formed via self-assembly and covalent coupling. Experimental results and theoretical calculation disclose that the bridge-linking strategy not only enables the fast electron and mass transfer, but also modifies the charge distribution and optimizes the adsorption/desorption process of oxygenated intermediates. With these merits, this metal-free catalyst exhibits superb bifunctional ORR/OER electrocatalytic activity with a voltage gap of 0.78 V. Remarkably, when equipped in aqueous and flexible Zn-air batteries, high power density (288, 68 mW cm–2) and enhanced durability are obtained. This facile nanocarbon-linkage strategy opens up a new avenue for the application of powdery catalysts in wearable energy devices. |
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Reasonable modulation of catalyst/substrate interface still remains great challenge for binder-free and high-performance electrodes. Herein, interfacial engineering via bridge-linking is proposed to effectively integrate powdery catalysts with flexible substrates by in situ synthesized nanocarbon. Concretely, a binder-free CNTs on carbonized carbon cloth linked with N-doped nanocarbons (CNTs-NC-CCC) electrode is formed via self-assembly and covalent coupling. Experimental results and theoretical calculation disclose that the bridge-linking strategy not only enables the fast electron and mass transfer, but also modifies the charge distribution and optimizes the adsorption/desorption process of oxygenated intermediates. With these merits, this metal-free catalyst exhibits superb bifunctional ORR/OER electrocatalytic activity with a voltage gap of 0.78 V. Remarkably, when equipped in aqueous and flexible Zn-air batteries, high power density (288, 68 mW cm–2) and enhanced durability are obtained. This facile nanocarbon-linkage strategy opens up a new avenue for the application of powdery catalysts in wearable energy devices. |
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