Insights into the synergistic effect of methoxy functionalized halloysite nanotubes for dielectric elastomer with improved dielectric properties and actuated strain
The application of silicone rubber (SiR) as a dielectric elastomer acuator is limited by its poor actuated strain because of low dielectric constant (ε r ). Herein, we designed and synthesized SiR-based dielectric elastomer composites with high ε r and acuated strain by introducing an extraordinary...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Wang, Ruolin [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2023transfer abstract |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: No title available - an international journal, Amsterdam [u.a.] |
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| Übergeordnetes Werk: |
volume:231 ; year:2023 ; day:5 ; month:01 ; pages:0 |
| Links: |
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| DOI / URN: |
10.1016/j.compscitech.2022.109802 |
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ELV059584076 |
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| 245 | 1 | 0 | |a Insights into the synergistic effect of methoxy functionalized halloysite nanotubes for dielectric elastomer with improved dielectric properties and actuated strain |
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| 520 | |a The application of silicone rubber (SiR) as a dielectric elastomer acuator is limited by its poor actuated strain because of low dielectric constant (ε r ). Herein, we designed and synthesized SiR-based dielectric elastomer composites with high ε r and acuated strain by introducing an extraordinary designed filler, methoxy functionalized halloysite nanotubes (HNTs-IPTS). This novel filler exhibits synergistic effects: (i) Highly polar urethane groups modified on the surface of HNTs-IPTS endow the composites with excellent dielectric properties (ε r = 13.590.1 kHz). (ii) The covalent bonds formed between HNTs-IPTS and SiR provide the composites with enanced tensile strength, better filler dispersion, and lower dielectric loss. (iii) The tubular architecture of HNTs-IPTS promotes the efficient delivery of charge carriers, further improve the ε r and actuated strain of the composites. These merits allow the resulting actuator to be more sensitive to driving field. Finally, HNTs-IPTS/SiR composites at 9 phr filler content exhibited a quite large actuated strain of 22.7% at 36.37 kV/mm without any prestrain. This work establishs the efficient HNTs-IPTS via structure design strategy, and the HNTs-IPTS/SiR composites are of great potential for next-generation DE acuators. | ||
| 520 | |a The application of silicone rubber (SiR) as a dielectric elastomer acuator is limited by its poor actuated strain because of low dielectric constant (ε r ). Herein, we designed and synthesized SiR-based dielectric elastomer composites with high ε r and acuated strain by introducing an extraordinary designed filler, methoxy functionalized halloysite nanotubes (HNTs-IPTS). This novel filler exhibits synergistic effects: (i) Highly polar urethane groups modified on the surface of HNTs-IPTS endow the composites with excellent dielectric properties (ε r = 13.590.1 kHz). (ii) The covalent bonds formed between HNTs-IPTS and SiR provide the composites with enanced tensile strength, better filler dispersion, and lower dielectric loss. (iii) The tubular architecture of HNTs-IPTS promotes the efficient delivery of charge carriers, further improve the ε r and actuated strain of the composites. These merits allow the resulting actuator to be more sensitive to driving field. Finally, HNTs-IPTS/SiR composites at 9 phr filler content exhibited a quite large actuated strain of 22.7% at 36.37 kV/mm without any prestrain. This work establishs the efficient HNTs-IPTS via structure design strategy, and the HNTs-IPTS/SiR composites are of great potential for next-generation DE acuators. | ||
| 650 | 7 | |a Polymer composites |2 Elsevier | |
| 650 | 7 | |a Silicon elastomer |2 Elsevier | |
| 650 | 7 | |a Dielectric elastomer |2 Elsevier | |
| 650 | 7 | |a Halloysite nanotubes |2 Elsevier | |
| 650 | 7 | |a Synergistic effect |2 Elsevier | |
| 700 | 1 | |a Wang, Yu |4 oth | |
| 700 | 1 | |a Liang, Yufeng |4 oth | |
| 700 | 1 | |a Yang, Zhen |4 oth | |
| 700 | 1 | |a Bai, Yongping |4 oth | |
| 700 | 1 | |a He, Jinmei |4 oth | |
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10.1016/j.compscitech.2022.109802 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001973.pica (DE-627)ELV059584076 (ELSEVIER)S0266-3538(22)00544-9 DE-627 ger DE-627 rakwb eng Wang, Ruolin verfasserin aut Insights into the synergistic effect of methoxy functionalized halloysite nanotubes for dielectric elastomer with improved dielectric properties and actuated strain 2023transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The application of silicone rubber (SiR) as a dielectric elastomer acuator is limited by its poor actuated strain because of low dielectric constant (ε r ). Herein, we designed and synthesized SiR-based dielectric elastomer composites with high ε r and acuated strain by introducing an extraordinary designed filler, methoxy functionalized halloysite nanotubes (HNTs-IPTS). This novel filler exhibits synergistic effects: (i) Highly polar urethane groups modified on the surface of HNTs-IPTS endow the composites with excellent dielectric properties (ε r = 13.590.1 kHz). (ii) The covalent bonds formed between HNTs-IPTS and SiR provide the composites with enanced tensile strength, better filler dispersion, and lower dielectric loss. (iii) The tubular architecture of HNTs-IPTS promotes the efficient delivery of charge carriers, further improve the ε r and actuated strain of the composites. These merits allow the resulting actuator to be more sensitive to driving field. Finally, HNTs-IPTS/SiR composites at 9 phr filler content exhibited a quite large actuated strain of 22.7% at 36.37 kV/mm without any prestrain. This work establishs the efficient HNTs-IPTS via structure design strategy, and the HNTs-IPTS/SiR composites are of great potential for next-generation DE acuators. The application of silicone rubber (SiR) as a dielectric elastomer acuator is limited by its poor actuated strain because of low dielectric constant (ε r ). Herein, we designed and synthesized SiR-based dielectric elastomer composites with high ε r and acuated strain by introducing an extraordinary designed filler, methoxy functionalized halloysite nanotubes (HNTs-IPTS). This novel filler exhibits synergistic effects: (i) Highly polar urethane groups modified on the surface of HNTs-IPTS endow the composites with excellent dielectric properties (ε r = 13.590.1 kHz). (ii) The covalent bonds formed between HNTs-IPTS and SiR provide the composites with enanced tensile strength, better filler dispersion, and lower dielectric loss. (iii) The tubular architecture of HNTs-IPTS promotes the efficient delivery of charge carriers, further improve the ε r and actuated strain of the composites. These merits allow the resulting actuator to be more sensitive to driving field. Finally, HNTs-IPTS/SiR composites at 9 phr filler content exhibited a quite large actuated strain of 22.7% at 36.37 kV/mm without any prestrain. This work establishs the efficient HNTs-IPTS via structure design strategy, and the HNTs-IPTS/SiR composites are of great potential for next-generation DE acuators. Polymer composites Elsevier Silicon elastomer Elsevier Dielectric elastomer Elsevier Halloysite nanotubes Elsevier Synergistic effect Elsevier Wang, Yu oth Liang, Yufeng oth Yang, Zhen oth Bai, Yongping oth He, Jinmei oth Enthalten in Elsevier No title available an international journal Amsterdam [u.a.] (DE-627)ELV013958402 nnns volume:231 year:2023 day:5 month:01 pages:0 https://doi.org/10.1016/j.compscitech.2022.109802 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_40 AR 231 2023 5 0105 0 |
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10.1016/j.compscitech.2022.109802 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001973.pica (DE-627)ELV059584076 (ELSEVIER)S0266-3538(22)00544-9 DE-627 ger DE-627 rakwb eng Wang, Ruolin verfasserin aut Insights into the synergistic effect of methoxy functionalized halloysite nanotubes for dielectric elastomer with improved dielectric properties and actuated strain 2023transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The application of silicone rubber (SiR) as a dielectric elastomer acuator is limited by its poor actuated strain because of low dielectric constant (ε r ). Herein, we designed and synthesized SiR-based dielectric elastomer composites with high ε r and acuated strain by introducing an extraordinary designed filler, methoxy functionalized halloysite nanotubes (HNTs-IPTS). This novel filler exhibits synergistic effects: (i) Highly polar urethane groups modified on the surface of HNTs-IPTS endow the composites with excellent dielectric properties (ε r = 13.590.1 kHz). (ii) The covalent bonds formed between HNTs-IPTS and SiR provide the composites with enanced tensile strength, better filler dispersion, and lower dielectric loss. (iii) The tubular architecture of HNTs-IPTS promotes the efficient delivery of charge carriers, further improve the ε r and actuated strain of the composites. These merits allow the resulting actuator to be more sensitive to driving field. Finally, HNTs-IPTS/SiR composites at 9 phr filler content exhibited a quite large actuated strain of 22.7% at 36.37 kV/mm without any prestrain. This work establishs the efficient HNTs-IPTS via structure design strategy, and the HNTs-IPTS/SiR composites are of great potential for next-generation DE acuators. The application of silicone rubber (SiR) as a dielectric elastomer acuator is limited by its poor actuated strain because of low dielectric constant (ε r ). Herein, we designed and synthesized SiR-based dielectric elastomer composites with high ε r and acuated strain by introducing an extraordinary designed filler, methoxy functionalized halloysite nanotubes (HNTs-IPTS). This novel filler exhibits synergistic effects: (i) Highly polar urethane groups modified on the surface of HNTs-IPTS endow the composites with excellent dielectric properties (ε r = 13.590.1 kHz). (ii) The covalent bonds formed between HNTs-IPTS and SiR provide the composites with enanced tensile strength, better filler dispersion, and lower dielectric loss. (iii) The tubular architecture of HNTs-IPTS promotes the efficient delivery of charge carriers, further improve the ε r and actuated strain of the composites. These merits allow the resulting actuator to be more sensitive to driving field. Finally, HNTs-IPTS/SiR composites at 9 phr filler content exhibited a quite large actuated strain of 22.7% at 36.37 kV/mm without any prestrain. This work establishs the efficient HNTs-IPTS via structure design strategy, and the HNTs-IPTS/SiR composites are of great potential for next-generation DE acuators. Polymer composites Elsevier Silicon elastomer Elsevier Dielectric elastomer Elsevier Halloysite nanotubes Elsevier Synergistic effect Elsevier Wang, Yu oth Liang, Yufeng oth Yang, Zhen oth Bai, Yongping oth He, Jinmei oth Enthalten in Elsevier No title available an international journal Amsterdam [u.a.] (DE-627)ELV013958402 nnns volume:231 year:2023 day:5 month:01 pages:0 https://doi.org/10.1016/j.compscitech.2022.109802 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_40 AR 231 2023 5 0105 0 |
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10.1016/j.compscitech.2022.109802 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001973.pica (DE-627)ELV059584076 (ELSEVIER)S0266-3538(22)00544-9 DE-627 ger DE-627 rakwb eng Wang, Ruolin verfasserin aut Insights into the synergistic effect of methoxy functionalized halloysite nanotubes for dielectric elastomer with improved dielectric properties and actuated strain 2023transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The application of silicone rubber (SiR) as a dielectric elastomer acuator is limited by its poor actuated strain because of low dielectric constant (ε r ). Herein, we designed and synthesized SiR-based dielectric elastomer composites with high ε r and acuated strain by introducing an extraordinary designed filler, methoxy functionalized halloysite nanotubes (HNTs-IPTS). This novel filler exhibits synergistic effects: (i) Highly polar urethane groups modified on the surface of HNTs-IPTS endow the composites with excellent dielectric properties (ε r = 13.590.1 kHz). (ii) The covalent bonds formed between HNTs-IPTS and SiR provide the composites with enanced tensile strength, better filler dispersion, and lower dielectric loss. (iii) The tubular architecture of HNTs-IPTS promotes the efficient delivery of charge carriers, further improve the ε r and actuated strain of the composites. These merits allow the resulting actuator to be more sensitive to driving field. Finally, HNTs-IPTS/SiR composites at 9 phr filler content exhibited a quite large actuated strain of 22.7% at 36.37 kV/mm without any prestrain. This work establishs the efficient HNTs-IPTS via structure design strategy, and the HNTs-IPTS/SiR composites are of great potential for next-generation DE acuators. The application of silicone rubber (SiR) as a dielectric elastomer acuator is limited by its poor actuated strain because of low dielectric constant (ε r ). Herein, we designed and synthesized SiR-based dielectric elastomer composites with high ε r and acuated strain by introducing an extraordinary designed filler, methoxy functionalized halloysite nanotubes (HNTs-IPTS). This novel filler exhibits synergistic effects: (i) Highly polar urethane groups modified on the surface of HNTs-IPTS endow the composites with excellent dielectric properties (ε r = 13.590.1 kHz). (ii) The covalent bonds formed between HNTs-IPTS and SiR provide the composites with enanced tensile strength, better filler dispersion, and lower dielectric loss. (iii) The tubular architecture of HNTs-IPTS promotes the efficient delivery of charge carriers, further improve the ε r and actuated strain of the composites. These merits allow the resulting actuator to be more sensitive to driving field. Finally, HNTs-IPTS/SiR composites at 9 phr filler content exhibited a quite large actuated strain of 22.7% at 36.37 kV/mm without any prestrain. This work establishs the efficient HNTs-IPTS via structure design strategy, and the HNTs-IPTS/SiR composites are of great potential for next-generation DE acuators. Polymer composites Elsevier Silicon elastomer Elsevier Dielectric elastomer Elsevier Halloysite nanotubes Elsevier Synergistic effect Elsevier Wang, Yu oth Liang, Yufeng oth Yang, Zhen oth Bai, Yongping oth He, Jinmei oth Enthalten in Elsevier No title available an international journal Amsterdam [u.a.] (DE-627)ELV013958402 nnns volume:231 year:2023 day:5 month:01 pages:0 https://doi.org/10.1016/j.compscitech.2022.109802 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_40 AR 231 2023 5 0105 0 |
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10.1016/j.compscitech.2022.109802 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001973.pica (DE-627)ELV059584076 (ELSEVIER)S0266-3538(22)00544-9 DE-627 ger DE-627 rakwb eng Wang, Ruolin verfasserin aut Insights into the synergistic effect of methoxy functionalized halloysite nanotubes for dielectric elastomer with improved dielectric properties and actuated strain 2023transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The application of silicone rubber (SiR) as a dielectric elastomer acuator is limited by its poor actuated strain because of low dielectric constant (ε r ). Herein, we designed and synthesized SiR-based dielectric elastomer composites with high ε r and acuated strain by introducing an extraordinary designed filler, methoxy functionalized halloysite nanotubes (HNTs-IPTS). This novel filler exhibits synergistic effects: (i) Highly polar urethane groups modified on the surface of HNTs-IPTS endow the composites with excellent dielectric properties (ε r = 13.590.1 kHz). (ii) The covalent bonds formed between HNTs-IPTS and SiR provide the composites with enanced tensile strength, better filler dispersion, and lower dielectric loss. (iii) The tubular architecture of HNTs-IPTS promotes the efficient delivery of charge carriers, further improve the ε r and actuated strain of the composites. These merits allow the resulting actuator to be more sensitive to driving field. Finally, HNTs-IPTS/SiR composites at 9 phr filler content exhibited a quite large actuated strain of 22.7% at 36.37 kV/mm without any prestrain. This work establishs the efficient HNTs-IPTS via structure design strategy, and the HNTs-IPTS/SiR composites are of great potential for next-generation DE acuators. The application of silicone rubber (SiR) as a dielectric elastomer acuator is limited by its poor actuated strain because of low dielectric constant (ε r ). Herein, we designed and synthesized SiR-based dielectric elastomer composites with high ε r and acuated strain by introducing an extraordinary designed filler, methoxy functionalized halloysite nanotubes (HNTs-IPTS). This novel filler exhibits synergistic effects: (i) Highly polar urethane groups modified on the surface of HNTs-IPTS endow the composites with excellent dielectric properties (ε r = 13.590.1 kHz). (ii) The covalent bonds formed between HNTs-IPTS and SiR provide the composites with enanced tensile strength, better filler dispersion, and lower dielectric loss. (iii) The tubular architecture of HNTs-IPTS promotes the efficient delivery of charge carriers, further improve the ε r and actuated strain of the composites. These merits allow the resulting actuator to be more sensitive to driving field. Finally, HNTs-IPTS/SiR composites at 9 phr filler content exhibited a quite large actuated strain of 22.7% at 36.37 kV/mm without any prestrain. This work establishs the efficient HNTs-IPTS via structure design strategy, and the HNTs-IPTS/SiR composites are of great potential for next-generation DE acuators. Polymer composites Elsevier Silicon elastomer Elsevier Dielectric elastomer Elsevier Halloysite nanotubes Elsevier Synergistic effect Elsevier Wang, Yu oth Liang, Yufeng oth Yang, Zhen oth Bai, Yongping oth He, Jinmei oth Enthalten in Elsevier No title available an international journal Amsterdam [u.a.] (DE-627)ELV013958402 nnns volume:231 year:2023 day:5 month:01 pages:0 https://doi.org/10.1016/j.compscitech.2022.109802 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_40 AR 231 2023 5 0105 0 |
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10.1016/j.compscitech.2022.109802 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001973.pica (DE-627)ELV059584076 (ELSEVIER)S0266-3538(22)00544-9 DE-627 ger DE-627 rakwb eng Wang, Ruolin verfasserin aut Insights into the synergistic effect of methoxy functionalized halloysite nanotubes for dielectric elastomer with improved dielectric properties and actuated strain 2023transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The application of silicone rubber (SiR) as a dielectric elastomer acuator is limited by its poor actuated strain because of low dielectric constant (ε r ). Herein, we designed and synthesized SiR-based dielectric elastomer composites with high ε r and acuated strain by introducing an extraordinary designed filler, methoxy functionalized halloysite nanotubes (HNTs-IPTS). This novel filler exhibits synergistic effects: (i) Highly polar urethane groups modified on the surface of HNTs-IPTS endow the composites with excellent dielectric properties (ε r = 13.590.1 kHz). (ii) The covalent bonds formed between HNTs-IPTS and SiR provide the composites with enanced tensile strength, better filler dispersion, and lower dielectric loss. (iii) The tubular architecture of HNTs-IPTS promotes the efficient delivery of charge carriers, further improve the ε r and actuated strain of the composites. These merits allow the resulting actuator to be more sensitive to driving field. Finally, HNTs-IPTS/SiR composites at 9 phr filler content exhibited a quite large actuated strain of 22.7% at 36.37 kV/mm without any prestrain. This work establishs the efficient HNTs-IPTS via structure design strategy, and the HNTs-IPTS/SiR composites are of great potential for next-generation DE acuators. The application of silicone rubber (SiR) as a dielectric elastomer acuator is limited by its poor actuated strain because of low dielectric constant (ε r ). Herein, we designed and synthesized SiR-based dielectric elastomer composites with high ε r and acuated strain by introducing an extraordinary designed filler, methoxy functionalized halloysite nanotubes (HNTs-IPTS). This novel filler exhibits synergistic effects: (i) Highly polar urethane groups modified on the surface of HNTs-IPTS endow the composites with excellent dielectric properties (ε r = 13.590.1 kHz). (ii) The covalent bonds formed between HNTs-IPTS and SiR provide the composites with enanced tensile strength, better filler dispersion, and lower dielectric loss. (iii) The tubular architecture of HNTs-IPTS promotes the efficient delivery of charge carriers, further improve the ε r and actuated strain of the composites. These merits allow the resulting actuator to be more sensitive to driving field. Finally, HNTs-IPTS/SiR composites at 9 phr filler content exhibited a quite large actuated strain of 22.7% at 36.37 kV/mm without any prestrain. This work establishs the efficient HNTs-IPTS via structure design strategy, and the HNTs-IPTS/SiR composites are of great potential for next-generation DE acuators. Polymer composites Elsevier Silicon elastomer Elsevier Dielectric elastomer Elsevier Halloysite nanotubes Elsevier Synergistic effect Elsevier Wang, Yu oth Liang, Yufeng oth Yang, Zhen oth Bai, Yongping oth He, Jinmei oth Enthalten in Elsevier No title available an international journal Amsterdam [u.a.] (DE-627)ELV013958402 nnns volume:231 year:2023 day:5 month:01 pages:0 https://doi.org/10.1016/j.compscitech.2022.109802 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_40 AR 231 2023 5 0105 0 |
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Wang, Ruolin @@aut@@ Wang, Yu @@oth@@ Liang, Yufeng @@oth@@ Yang, Zhen @@oth@@ Bai, Yongping @@oth@@ He, Jinmei @@oth@@ |
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Herein, we designed and synthesized SiR-based dielectric elastomer composites with high ε r and acuated strain by introducing an extraordinary designed filler, methoxy functionalized halloysite nanotubes (HNTs-IPTS). This novel filler exhibits synergistic effects: (i) Highly polar urethane groups modified on the surface of HNTs-IPTS endow the composites with excellent dielectric properties (ε r = 13.590.1 kHz). (ii) The covalent bonds formed between HNTs-IPTS and SiR provide the composites with enanced tensile strength, better filler dispersion, and lower dielectric loss. (iii) The tubular architecture of HNTs-IPTS promotes the efficient delivery of charge carriers, further improve the ε r and actuated strain of the composites. These merits allow the resulting actuator to be more sensitive to driving field. Finally, HNTs-IPTS/SiR composites at 9 phr filler content exhibited a quite large actuated strain of 22.7% at 36.37 kV/mm without any prestrain. 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insights into the synergistic effect of methoxy functionalized halloysite nanotubes for dielectric elastomer with improved dielectric properties and actuated strain |
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Insights into the synergistic effect of methoxy functionalized halloysite nanotubes for dielectric elastomer with improved dielectric properties and actuated strain |
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The application of silicone rubber (SiR) as a dielectric elastomer acuator is limited by its poor actuated strain because of low dielectric constant (ε r ). Herein, we designed and synthesized SiR-based dielectric elastomer composites with high ε r and acuated strain by introducing an extraordinary designed filler, methoxy functionalized halloysite nanotubes (HNTs-IPTS). This novel filler exhibits synergistic effects: (i) Highly polar urethane groups modified on the surface of HNTs-IPTS endow the composites with excellent dielectric properties (ε r = 13.590.1 kHz). (ii) The covalent bonds formed between HNTs-IPTS and SiR provide the composites with enanced tensile strength, better filler dispersion, and lower dielectric loss. (iii) The tubular architecture of HNTs-IPTS promotes the efficient delivery of charge carriers, further improve the ε r and actuated strain of the composites. These merits allow the resulting actuator to be more sensitive to driving field. Finally, HNTs-IPTS/SiR composites at 9 phr filler content exhibited a quite large actuated strain of 22.7% at 36.37 kV/mm without any prestrain. This work establishs the efficient HNTs-IPTS via structure design strategy, and the HNTs-IPTS/SiR composites are of great potential for next-generation DE acuators. |
| abstractGer |
The application of silicone rubber (SiR) as a dielectric elastomer acuator is limited by its poor actuated strain because of low dielectric constant (ε r ). Herein, we designed and synthesized SiR-based dielectric elastomer composites with high ε r and acuated strain by introducing an extraordinary designed filler, methoxy functionalized halloysite nanotubes (HNTs-IPTS). This novel filler exhibits synergistic effects: (i) Highly polar urethane groups modified on the surface of HNTs-IPTS endow the composites with excellent dielectric properties (ε r = 13.590.1 kHz). (ii) The covalent bonds formed between HNTs-IPTS and SiR provide the composites with enanced tensile strength, better filler dispersion, and lower dielectric loss. (iii) The tubular architecture of HNTs-IPTS promotes the efficient delivery of charge carriers, further improve the ε r and actuated strain of the composites. These merits allow the resulting actuator to be more sensitive to driving field. Finally, HNTs-IPTS/SiR composites at 9 phr filler content exhibited a quite large actuated strain of 22.7% at 36.37 kV/mm without any prestrain. This work establishs the efficient HNTs-IPTS via structure design strategy, and the HNTs-IPTS/SiR composites are of great potential for next-generation DE acuators. |
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The application of silicone rubber (SiR) as a dielectric elastomer acuator is limited by its poor actuated strain because of low dielectric constant (ε r ). Herein, we designed and synthesized SiR-based dielectric elastomer composites with high ε r and acuated strain by introducing an extraordinary designed filler, methoxy functionalized halloysite nanotubes (HNTs-IPTS). This novel filler exhibits synergistic effects: (i) Highly polar urethane groups modified on the surface of HNTs-IPTS endow the composites with excellent dielectric properties (ε r = 13.590.1 kHz). (ii) The covalent bonds formed between HNTs-IPTS and SiR provide the composites with enanced tensile strength, better filler dispersion, and lower dielectric loss. (iii) The tubular architecture of HNTs-IPTS promotes the efficient delivery of charge carriers, further improve the ε r and actuated strain of the composites. These merits allow the resulting actuator to be more sensitive to driving field. Finally, HNTs-IPTS/SiR composites at 9 phr filler content exhibited a quite large actuated strain of 22.7% at 36.37 kV/mm without any prestrain. This work establishs the efficient HNTs-IPTS via structure design strategy, and the HNTs-IPTS/SiR composites are of great potential for next-generation DE acuators. |
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