High-efficient and scalable solar-driven MOF-based water collection unit: From module design to concrete implementation

MOF-based atmospheric water harvesting technology is a straightforward and practical strategy for producing safe drinking water. However, separate designs of high-adsorption desiccant skeletons and efficient photothermal layers are required to maximize water production efficiency. This work presents...
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Gespeichert in:

Autor*in:	Luo, Fan [verfasserIn] Liang, Xianghui [verfasserIn] Chen, Weicheng [verfasserIn] Wang, Shuangfeng [verfasserIn] Gao, Xuenong [verfasserIn] Zhang, Zhengguo [verfasserIn] Fang, Yutang [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Atmospheric water harvesting Hybridized MOF skeleton Monolithic adsorbent Light-heat conversion High-efficient water collection

Übergeordnetes Werk:	Enthalten in: The chemical engineering journal - Amsterdam : Elsevier, 1997, 465
Übergeordnetes Werk:	volume:465

DOI / URN:	10.1016/j.cej.2023.142891

Katalog-ID:	ELV059901403

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520			\|a MOF-based atmospheric water harvesting technology is a straightforward and practical strategy for producing safe drinking water. However, separate designs of high-adsorption desiccant skeletons and efficient photothermal layers are required to maximize water production efficiency. This work presents an integrated design of a multifunctional monolithic adsorbent through the layer-by-layer assembly of chitosan/polydopamine layers and hybridized MOF backbones on a glass fiber support. The hydrophilic hybridized MOF consisting of MIL-160(Al) and MOF-303 obtains the higher specific surface area (917.59 m2/g) and pore volume (0.44 cm3/g) through morphological reorganization for facilitating water capture and storage capacity. Especially in arid environments (RH ≤ 30 %), the resultant MOF has a superior moisture adsorption capacity (0.44 g/g) than parental MOF and other potential MOFs. The polymeric photothermal layer of adsorbent enables high solar thermal conversion in sunlight to assist the release of collected water. With fast sorption–desorption kinetics, an impressive outdoor water production of 0.94 g/g per day is observed in the designed monolithic adsorbent, indicating its enormous potential for safe, sustainable and scalable atmospheric water collection technology.
650		4	\|a Atmospheric water harvesting
650		4	\|a Hybridized MOF skeleton
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650		4	\|a Light-heat conversion
650		4	\|a High-efficient water collection
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700	1		\|a Gao, Xuenong \|e verfasserin \|4 aut
700	1		\|a Zhang, Zhengguo \|e verfasserin \|4 aut
700	1		\|a Fang, Yutang \|e verfasserin \|4 aut
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allfields	10.1016/j.cej.2023.142891 doi (DE-627)ELV059901403 (ELSEVIER)S1385-8947(23)01622-4 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Luo, Fan verfasserin aut High-efficient and scalable solar-driven MOF-based water collection unit: From module design to concrete implementation 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier MOF-based atmospheric water harvesting technology is a straightforward and practical strategy for producing safe drinking water. However, separate designs of high-adsorption desiccant skeletons and efficient photothermal layers are required to maximize water production efficiency. This work presents an integrated design of a multifunctional monolithic adsorbent through the layer-by-layer assembly of chitosan/polydopamine layers and hybridized MOF backbones on a glass fiber support. The hydrophilic hybridized MOF consisting of MIL-160(Al) and MOF-303 obtains the higher specific surface area (917.59 m2/g) and pore volume (0.44 cm3/g) through morphological reorganization for facilitating water capture and storage capacity. Especially in arid environments (RH ≤ 30 %), the resultant MOF has a superior moisture adsorption capacity (0.44 g/g) than parental MOF and other potential MOFs. The polymeric photothermal layer of adsorbent enables high solar thermal conversion in sunlight to assist the release of collected water. With fast sorption–desorption kinetics, an impressive outdoor water production of 0.94 g/g per day is observed in the designed monolithic adsorbent, indicating its enormous potential for safe, sustainable and scalable atmospheric water collection technology. Atmospheric water harvesting Hybridized MOF skeleton Monolithic adsorbent Light-heat conversion High-efficient water collection Liang, Xianghui verfasserin aut Chen, Weicheng verfasserin aut Wang, Shuangfeng verfasserin aut Gao, Xuenong verfasserin aut Zhang, Zhengguo verfasserin aut Fang, Yutang verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 465 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:465 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 465
spelling	10.1016/j.cej.2023.142891 doi (DE-627)ELV059901403 (ELSEVIER)S1385-8947(23)01622-4 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Luo, Fan verfasserin aut High-efficient and scalable solar-driven MOF-based water collection unit: From module design to concrete implementation 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier MOF-based atmospheric water harvesting technology is a straightforward and practical strategy for producing safe drinking water. However, separate designs of high-adsorption desiccant skeletons and efficient photothermal layers are required to maximize water production efficiency. This work presents an integrated design of a multifunctional monolithic adsorbent through the layer-by-layer assembly of chitosan/polydopamine layers and hybridized MOF backbones on a glass fiber support. The hydrophilic hybridized MOF consisting of MIL-160(Al) and MOF-303 obtains the higher specific surface area (917.59 m2/g) and pore volume (0.44 cm3/g) through morphological reorganization for facilitating water capture and storage capacity. Especially in arid environments (RH ≤ 30 %), the resultant MOF has a superior moisture adsorption capacity (0.44 g/g) than parental MOF and other potential MOFs. The polymeric photothermal layer of adsorbent enables high solar thermal conversion in sunlight to assist the release of collected water. With fast sorption–desorption kinetics, an impressive outdoor water production of 0.94 g/g per day is observed in the designed monolithic adsorbent, indicating its enormous potential for safe, sustainable and scalable atmospheric water collection technology. Atmospheric water harvesting Hybridized MOF skeleton Monolithic adsorbent Light-heat conversion High-efficient water collection Liang, Xianghui verfasserin aut Chen, Weicheng verfasserin aut Wang, Shuangfeng verfasserin aut Gao, Xuenong verfasserin aut Zhang, Zhengguo verfasserin aut Fang, Yutang verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 465 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:465 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 465
allfields_unstemmed	10.1016/j.cej.2023.142891 doi (DE-627)ELV059901403 (ELSEVIER)S1385-8947(23)01622-4 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Luo, Fan verfasserin aut High-efficient and scalable solar-driven MOF-based water collection unit: From module design to concrete implementation 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier MOF-based atmospheric water harvesting technology is a straightforward and practical strategy for producing safe drinking water. However, separate designs of high-adsorption desiccant skeletons and efficient photothermal layers are required to maximize water production efficiency. This work presents an integrated design of a multifunctional monolithic adsorbent through the layer-by-layer assembly of chitosan/polydopamine layers and hybridized MOF backbones on a glass fiber support. The hydrophilic hybridized MOF consisting of MIL-160(Al) and MOF-303 obtains the higher specific surface area (917.59 m2/g) and pore volume (0.44 cm3/g) through morphological reorganization for facilitating water capture and storage capacity. Especially in arid environments (RH ≤ 30 %), the resultant MOF has a superior moisture adsorption capacity (0.44 g/g) than parental MOF and other potential MOFs. The polymeric photothermal layer of adsorbent enables high solar thermal conversion in sunlight to assist the release of collected water. With fast sorption–desorption kinetics, an impressive outdoor water production of 0.94 g/g per day is observed in the designed monolithic adsorbent, indicating its enormous potential for safe, sustainable and scalable atmospheric water collection technology. Atmospheric water harvesting Hybridized MOF skeleton Monolithic adsorbent Light-heat conversion High-efficient water collection Liang, Xianghui verfasserin aut Chen, Weicheng verfasserin aut Wang, Shuangfeng verfasserin aut Gao, Xuenong verfasserin aut Zhang, Zhengguo verfasserin aut Fang, Yutang verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 465 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:465 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 465
allfieldsGer	10.1016/j.cej.2023.142891 doi (DE-627)ELV059901403 (ELSEVIER)S1385-8947(23)01622-4 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Luo, Fan verfasserin aut High-efficient and scalable solar-driven MOF-based water collection unit: From module design to concrete implementation 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier MOF-based atmospheric water harvesting technology is a straightforward and practical strategy for producing safe drinking water. However, separate designs of high-adsorption desiccant skeletons and efficient photothermal layers are required to maximize water production efficiency. This work presents an integrated design of a multifunctional monolithic adsorbent through the layer-by-layer assembly of chitosan/polydopamine layers and hybridized MOF backbones on a glass fiber support. The hydrophilic hybridized MOF consisting of MIL-160(Al) and MOF-303 obtains the higher specific surface area (917.59 m2/g) and pore volume (0.44 cm3/g) through morphological reorganization for facilitating water capture and storage capacity. Especially in arid environments (RH ≤ 30 %), the resultant MOF has a superior moisture adsorption capacity (0.44 g/g) than parental MOF and other potential MOFs. The polymeric photothermal layer of adsorbent enables high solar thermal conversion in sunlight to assist the release of collected water. With fast sorption–desorption kinetics, an impressive outdoor water production of 0.94 g/g per day is observed in the designed monolithic adsorbent, indicating its enormous potential for safe, sustainable and scalable atmospheric water collection technology. Atmospheric water harvesting Hybridized MOF skeleton Monolithic adsorbent Light-heat conversion High-efficient water collection Liang, Xianghui verfasserin aut Chen, Weicheng verfasserin aut Wang, Shuangfeng verfasserin aut Gao, Xuenong verfasserin aut Zhang, Zhengguo verfasserin aut Fang, Yutang verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 465 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:465 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 465
allfieldsSound	10.1016/j.cej.2023.142891 doi (DE-627)ELV059901403 (ELSEVIER)S1385-8947(23)01622-4 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Luo, Fan verfasserin aut High-efficient and scalable solar-driven MOF-based water collection unit: From module design to concrete implementation 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier MOF-based atmospheric water harvesting technology is a straightforward and practical strategy for producing safe drinking water. However, separate designs of high-adsorption desiccant skeletons and efficient photothermal layers are required to maximize water production efficiency. This work presents an integrated design of a multifunctional monolithic adsorbent through the layer-by-layer assembly of chitosan/polydopamine layers and hybridized MOF backbones on a glass fiber support. The hydrophilic hybridized MOF consisting of MIL-160(Al) and MOF-303 obtains the higher specific surface area (917.59 m2/g) and pore volume (0.44 cm3/g) through morphological reorganization for facilitating water capture and storage capacity. Especially in arid environments (RH ≤ 30 %), the resultant MOF has a superior moisture adsorption capacity (0.44 g/g) than parental MOF and other potential MOFs. The polymeric photothermal layer of adsorbent enables high solar thermal conversion in sunlight to assist the release of collected water. With fast sorption–desorption kinetics, an impressive outdoor water production of 0.94 g/g per day is observed in the designed monolithic adsorbent, indicating its enormous potential for safe, sustainable and scalable atmospheric water collection technology. Atmospheric water harvesting Hybridized MOF skeleton Monolithic adsorbent Light-heat conversion High-efficient water collection Liang, Xianghui verfasserin aut Chen, Weicheng verfasserin aut Wang, Shuangfeng verfasserin aut Gao, Xuenong verfasserin aut Zhang, Zhengguo verfasserin aut Fang, Yutang verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 465 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:465 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 465
language	English
source	Enthalten in The chemical engineering journal 465 volume:465
sourceStr	Enthalten in The chemical engineering journal 465 volume:465
format_phy_str_mv	Article
bklname	Verfahrenstechnik: Allgemeines
institution	findex.gbv.de
topic_facet	Atmospheric water harvesting Hybridized MOF skeleton Monolithic adsorbent Light-heat conversion High-efficient water collection
dewey-raw	660
isfreeaccess_bool	false
container_title	The chemical engineering journal
authorswithroles_txt_mv	Luo, Fan @@aut@@ Liang, Xianghui @@aut@@ Chen, Weicheng @@aut@@ Wang, Shuangfeng @@aut@@ Gao, Xuenong @@aut@@ Zhang, Zhengguo @@aut@@ Fang, Yutang @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	320500322
dewey-sort	3660
id	ELV059901403
language_de	englisch
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author	Luo, Fan
spellingShingle	Luo, Fan ddc 660 bkl 58.10 misc Atmospheric water harvesting misc Hybridized MOF skeleton misc Monolithic adsorbent misc Light-heat conversion misc High-efficient water collection High-efficient and scalable solar-driven MOF-based water collection unit: From module design to concrete implementation
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topic_title	660 VZ 58.10 bkl High-efficient and scalable solar-driven MOF-based water collection unit: From module design to concrete implementation Atmospheric water harvesting Hybridized MOF skeleton Monolithic adsorbent Light-heat conversion High-efficient water collection
topic	ddc 660 bkl 58.10 misc Atmospheric water harvesting misc Hybridized MOF skeleton misc Monolithic adsorbent misc Light-heat conversion misc High-efficient water collection
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title	High-efficient and scalable solar-driven MOF-based water collection unit: From module design to concrete implementation
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title_full	High-efficient and scalable solar-driven MOF-based water collection unit: From module design to concrete implementation
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title_sort	high-efficient and scalable solar-driven mof-based water collection unit: from module design to concrete implementation
title_auth	High-efficient and scalable solar-driven MOF-based water collection unit: From module design to concrete implementation
abstract	MOF-based atmospheric water harvesting technology is a straightforward and practical strategy for producing safe drinking water. However, separate designs of high-adsorption desiccant skeletons and efficient photothermal layers are required to maximize water production efficiency. This work presents an integrated design of a multifunctional monolithic adsorbent through the layer-by-layer assembly of chitosan/polydopamine layers and hybridized MOF backbones on a glass fiber support. The hydrophilic hybridized MOF consisting of MIL-160(Al) and MOF-303 obtains the higher specific surface area (917.59 m2/g) and pore volume (0.44 cm3/g) through morphological reorganization for facilitating water capture and storage capacity. Especially in arid environments (RH ≤ 30 %), the resultant MOF has a superior moisture adsorption capacity (0.44 g/g) than parental MOF and other potential MOFs. The polymeric photothermal layer of adsorbent enables high solar thermal conversion in sunlight to assist the release of collected water. With fast sorption–desorption kinetics, an impressive outdoor water production of 0.94 g/g per day is observed in the designed monolithic adsorbent, indicating its enormous potential for safe, sustainable and scalable atmospheric water collection technology.
abstractGer	MOF-based atmospheric water harvesting technology is a straightforward and practical strategy for producing safe drinking water. However, separate designs of high-adsorption desiccant skeletons and efficient photothermal layers are required to maximize water production efficiency. This work presents an integrated design of a multifunctional monolithic adsorbent through the layer-by-layer assembly of chitosan/polydopamine layers and hybridized MOF backbones on a glass fiber support. The hydrophilic hybridized MOF consisting of MIL-160(Al) and MOF-303 obtains the higher specific surface area (917.59 m2/g) and pore volume (0.44 cm3/g) through morphological reorganization for facilitating water capture and storage capacity. Especially in arid environments (RH ≤ 30 %), the resultant MOF has a superior moisture adsorption capacity (0.44 g/g) than parental MOF and other potential MOFs. The polymeric photothermal layer of adsorbent enables high solar thermal conversion in sunlight to assist the release of collected water. With fast sorption–desorption kinetics, an impressive outdoor water production of 0.94 g/g per day is observed in the designed monolithic adsorbent, indicating its enormous potential for safe, sustainable and scalable atmospheric water collection technology.
abstract_unstemmed	MOF-based atmospheric water harvesting technology is a straightforward and practical strategy for producing safe drinking water. However, separate designs of high-adsorption desiccant skeletons and efficient photothermal layers are required to maximize water production efficiency. This work presents an integrated design of a multifunctional monolithic adsorbent through the layer-by-layer assembly of chitosan/polydopamine layers and hybridized MOF backbones on a glass fiber support. The hydrophilic hybridized MOF consisting of MIL-160(Al) and MOF-303 obtains the higher specific surface area (917.59 m2/g) and pore volume (0.44 cm3/g) through morphological reorganization for facilitating water capture and storage capacity. Especially in arid environments (RH ≤ 30 %), the resultant MOF has a superior moisture adsorption capacity (0.44 g/g) than parental MOF and other potential MOFs. The polymeric photothermal layer of adsorbent enables high solar thermal conversion in sunlight to assist the release of collected water. With fast sorption–desorption kinetics, an impressive outdoor water production of 0.94 g/g per day is observed in the designed monolithic adsorbent, indicating its enormous potential for safe, sustainable and scalable atmospheric water collection technology.
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title_short	High-efficient and scalable solar-driven MOF-based water collection unit: From module design to concrete implementation
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author2	Liang, Xianghui Chen, Weicheng Wang, Shuangfeng Gao, Xuenong Zhang, Zhengguo Fang, Yutang
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High-efficient and scalable solar-driven MOF-based water collection unit: From module design to concrete implementation

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