Effect of different electronegative oxygen atoms of cellulose nanofibrils on the formation and photocatalytic property of ZnO/cellulose composite
Cellulose is widely employed as a template in supporting and dispersing ZnO. The oxygen atom of the hydroxyl (–OH) groups of cellulose have a significant impact on the morphology and photocatalytic property of ZnO. This work aims to investigate the effect of different electronegative oxygen atoms of...
Ausführliche Beschreibung
Autor*in: |
Yan, Ming [verfasserIn] An, Bihui [verfasserIn] Li, Xin [verfasserIn] Zai, Zhenqiang [verfasserIn] Wu, Shufang [verfasserIn] Ma, Jinxia [verfasserIn] Zhang, Lili [verfasserIn] |
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Format: |
E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2023 |
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Schlagwörter: |
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Übergeordnetes Werk: |
Enthalten in: Applied surface science - Amsterdam : Elsevier, 1985, 637 |
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Übergeordnetes Werk: |
volume:637 |
DOI / URN: |
10.1016/j.apsusc.2023.157974 |
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Katalog-ID: |
ELV060575182 |
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520 | |a Cellulose is widely employed as a template in supporting and dispersing ZnO. The oxygen atom of the hydroxyl (–OH) groups of cellulose have a significant impact on the morphology and photocatalytic property of ZnO. This work aims to investigate the effect of different electronegative oxygen atoms of cellulose nanofibrils (CNF) on the formation and photocatalytic properties of ZnO/cellulose composites. The interaction between cellulose and ZnO has been achieved by controlling cellulose fiber size and regulating the electronegativity of oxygen atoms on the CNF surface. The results indicate that etherized CNF (ECNF) with the highest degree of etherification substitution (1.7) and the best electronegativity (−34.6 mV) can synthesize the ZnO/cellulose composite with the largest loading content of ZnO (58.9%) and the best photocatalytic activity for MO degradation (91.1%). It can be concluded that the intenser electrostatic interaction between oxygen atoms on the CNF surface and ZnO can facilitate the fixation and growth of more high-quality ZnO nanoflowers, thus improving the photocatalytic property. In a word, this work can provide a novel perspective for the efficient preparation of ZnO/cellulose composites with designable morphology and structure. | ||
650 | 4 | |a Cellulose | |
650 | 4 | |a Electronegative oxygen atoms | |
650 | 4 | |a ZnO | |
650 | 4 | |a Morphology | |
650 | 4 | |a Photocatalytic property | |
700 | 1 | |a An, Bihui |e verfasserin |4 aut | |
700 | 1 | |a Li, Xin |e verfasserin |4 aut | |
700 | 1 | |a Zai, Zhenqiang |e verfasserin |4 aut | |
700 | 1 | |a Wu, Shufang |e verfasserin |4 aut | |
700 | 1 | |a Ma, Jinxia |e verfasserin |4 aut | |
700 | 1 | |a Zhang, Lili |e verfasserin |0 (orcid)0000-0002-8328-4648 |4 aut | |
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10.1016/j.apsusc.2023.157974 doi (DE-627)ELV060575182 (ELSEVIER)S0169-4332(23)01653-7 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Yan, Ming verfasserin aut Effect of different electronegative oxygen atoms of cellulose nanofibrils on the formation and photocatalytic property of ZnO/cellulose composite 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Cellulose is widely employed as a template in supporting and dispersing ZnO. The oxygen atom of the hydroxyl (–OH) groups of cellulose have a significant impact on the morphology and photocatalytic property of ZnO. This work aims to investigate the effect of different electronegative oxygen atoms of cellulose nanofibrils (CNF) on the formation and photocatalytic properties of ZnO/cellulose composites. The interaction between cellulose and ZnO has been achieved by controlling cellulose fiber size and regulating the electronegativity of oxygen atoms on the CNF surface. The results indicate that etherized CNF (ECNF) with the highest degree of etherification substitution (1.7) and the best electronegativity (−34.6 mV) can synthesize the ZnO/cellulose composite with the largest loading content of ZnO (58.9%) and the best photocatalytic activity for MO degradation (91.1%). It can be concluded that the intenser electrostatic interaction between oxygen atoms on the CNF surface and ZnO can facilitate the fixation and growth of more high-quality ZnO nanoflowers, thus improving the photocatalytic property. In a word, this work can provide a novel perspective for the efficient preparation of ZnO/cellulose composites with designable morphology and structure. Cellulose Electronegative oxygen atoms ZnO Morphology Photocatalytic property An, Bihui verfasserin aut Li, Xin verfasserin aut Zai, Zhenqiang verfasserin aut Wu, Shufang verfasserin aut Ma, Jinxia verfasserin aut Zhang, Lili verfasserin (orcid)0000-0002-8328-4648 aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 637 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:637 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 637 |
spelling |
10.1016/j.apsusc.2023.157974 doi (DE-627)ELV060575182 (ELSEVIER)S0169-4332(23)01653-7 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Yan, Ming verfasserin aut Effect of different electronegative oxygen atoms of cellulose nanofibrils on the formation and photocatalytic property of ZnO/cellulose composite 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Cellulose is widely employed as a template in supporting and dispersing ZnO. The oxygen atom of the hydroxyl (–OH) groups of cellulose have a significant impact on the morphology and photocatalytic property of ZnO. This work aims to investigate the effect of different electronegative oxygen atoms of cellulose nanofibrils (CNF) on the formation and photocatalytic properties of ZnO/cellulose composites. The interaction between cellulose and ZnO has been achieved by controlling cellulose fiber size and regulating the electronegativity of oxygen atoms on the CNF surface. The results indicate that etherized CNF (ECNF) with the highest degree of etherification substitution (1.7) and the best electronegativity (−34.6 mV) can synthesize the ZnO/cellulose composite with the largest loading content of ZnO (58.9%) and the best photocatalytic activity for MO degradation (91.1%). It can be concluded that the intenser electrostatic interaction between oxygen atoms on the CNF surface and ZnO can facilitate the fixation and growth of more high-quality ZnO nanoflowers, thus improving the photocatalytic property. In a word, this work can provide a novel perspective for the efficient preparation of ZnO/cellulose composites with designable morphology and structure. Cellulose Electronegative oxygen atoms ZnO Morphology Photocatalytic property An, Bihui verfasserin aut Li, Xin verfasserin aut Zai, Zhenqiang verfasserin aut Wu, Shufang verfasserin aut Ma, Jinxia verfasserin aut Zhang, Lili verfasserin (orcid)0000-0002-8328-4648 aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 637 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:637 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 637 |
allfields_unstemmed |
10.1016/j.apsusc.2023.157974 doi (DE-627)ELV060575182 (ELSEVIER)S0169-4332(23)01653-7 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Yan, Ming verfasserin aut Effect of different electronegative oxygen atoms of cellulose nanofibrils on the formation and photocatalytic property of ZnO/cellulose composite 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Cellulose is widely employed as a template in supporting and dispersing ZnO. The oxygen atom of the hydroxyl (–OH) groups of cellulose have a significant impact on the morphology and photocatalytic property of ZnO. This work aims to investigate the effect of different electronegative oxygen atoms of cellulose nanofibrils (CNF) on the formation and photocatalytic properties of ZnO/cellulose composites. The interaction between cellulose and ZnO has been achieved by controlling cellulose fiber size and regulating the electronegativity of oxygen atoms on the CNF surface. The results indicate that etherized CNF (ECNF) with the highest degree of etherification substitution (1.7) and the best electronegativity (−34.6 mV) can synthesize the ZnO/cellulose composite with the largest loading content of ZnO (58.9%) and the best photocatalytic activity for MO degradation (91.1%). It can be concluded that the intenser electrostatic interaction between oxygen atoms on the CNF surface and ZnO can facilitate the fixation and growth of more high-quality ZnO nanoflowers, thus improving the photocatalytic property. In a word, this work can provide a novel perspective for the efficient preparation of ZnO/cellulose composites with designable morphology and structure. Cellulose Electronegative oxygen atoms ZnO Morphology Photocatalytic property An, Bihui verfasserin aut Li, Xin verfasserin aut Zai, Zhenqiang verfasserin aut Wu, Shufang verfasserin aut Ma, Jinxia verfasserin aut Zhang, Lili verfasserin (orcid)0000-0002-8328-4648 aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 637 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:637 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 637 |
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10.1016/j.apsusc.2023.157974 doi (DE-627)ELV060575182 (ELSEVIER)S0169-4332(23)01653-7 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Yan, Ming verfasserin aut Effect of different electronegative oxygen atoms of cellulose nanofibrils on the formation and photocatalytic property of ZnO/cellulose composite 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Cellulose is widely employed as a template in supporting and dispersing ZnO. The oxygen atom of the hydroxyl (–OH) groups of cellulose have a significant impact on the morphology and photocatalytic property of ZnO. This work aims to investigate the effect of different electronegative oxygen atoms of cellulose nanofibrils (CNF) on the formation and photocatalytic properties of ZnO/cellulose composites. The interaction between cellulose and ZnO has been achieved by controlling cellulose fiber size and regulating the electronegativity of oxygen atoms on the CNF surface. The results indicate that etherized CNF (ECNF) with the highest degree of etherification substitution (1.7) and the best electronegativity (−34.6 mV) can synthesize the ZnO/cellulose composite with the largest loading content of ZnO (58.9%) and the best photocatalytic activity for MO degradation (91.1%). It can be concluded that the intenser electrostatic interaction between oxygen atoms on the CNF surface and ZnO can facilitate the fixation and growth of more high-quality ZnO nanoflowers, thus improving the photocatalytic property. In a word, this work can provide a novel perspective for the efficient preparation of ZnO/cellulose composites with designable morphology and structure. Cellulose Electronegative oxygen atoms ZnO Morphology Photocatalytic property An, Bihui verfasserin aut Li, Xin verfasserin aut Zai, Zhenqiang verfasserin aut Wu, Shufang verfasserin aut Ma, Jinxia verfasserin aut Zhang, Lili verfasserin (orcid)0000-0002-8328-4648 aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 637 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:637 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 637 |
allfieldsSound |
10.1016/j.apsusc.2023.157974 doi (DE-627)ELV060575182 (ELSEVIER)S0169-4332(23)01653-7 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Yan, Ming verfasserin aut Effect of different electronegative oxygen atoms of cellulose nanofibrils on the formation and photocatalytic property of ZnO/cellulose composite 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Cellulose is widely employed as a template in supporting and dispersing ZnO. The oxygen atom of the hydroxyl (–OH) groups of cellulose have a significant impact on the morphology and photocatalytic property of ZnO. This work aims to investigate the effect of different electronegative oxygen atoms of cellulose nanofibrils (CNF) on the formation and photocatalytic properties of ZnO/cellulose composites. The interaction between cellulose and ZnO has been achieved by controlling cellulose fiber size and regulating the electronegativity of oxygen atoms on the CNF surface. The results indicate that etherized CNF (ECNF) with the highest degree of etherification substitution (1.7) and the best electronegativity (−34.6 mV) can synthesize the ZnO/cellulose composite with the largest loading content of ZnO (58.9%) and the best photocatalytic activity for MO degradation (91.1%). It can be concluded that the intenser electrostatic interaction between oxygen atoms on the CNF surface and ZnO can facilitate the fixation and growth of more high-quality ZnO nanoflowers, thus improving the photocatalytic property. In a word, this work can provide a novel perspective for the efficient preparation of ZnO/cellulose composites with designable morphology and structure. Cellulose Electronegative oxygen atoms ZnO Morphology Photocatalytic property An, Bihui verfasserin aut Li, Xin verfasserin aut Zai, Zhenqiang verfasserin aut Wu, Shufang verfasserin aut Ma, Jinxia verfasserin aut Zhang, Lili verfasserin (orcid)0000-0002-8328-4648 aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 637 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:637 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 637 |
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Oberflächen Dünne Schichten Grenzflächen Kolloidchemie Grenzflächenchemie Oberflächentechnik Wärmebehandlung |
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Cellulose Electronegative oxygen atoms ZnO Morphology Photocatalytic property |
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Yan, Ming @@aut@@ An, Bihui @@aut@@ Li, Xin @@aut@@ Zai, Zhenqiang @@aut@@ Wu, Shufang @@aut@@ Ma, Jinxia @@aut@@ Zhang, Lili @@aut@@ |
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Yan, Ming ddc 670 bkl 33.68 bkl 35.18 bkl 52.78 misc Cellulose misc Electronegative oxygen atoms misc ZnO misc Morphology misc Photocatalytic property Effect of different electronegative oxygen atoms of cellulose nanofibrils on the formation and photocatalytic property of ZnO/cellulose composite |
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effect of different electronegative oxygen atoms of cellulose nanofibrils on the formation and photocatalytic property of zno/cellulose composite |
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Effect of different electronegative oxygen atoms of cellulose nanofibrils on the formation and photocatalytic property of ZnO/cellulose composite |
abstract |
Cellulose is widely employed as a template in supporting and dispersing ZnO. The oxygen atom of the hydroxyl (–OH) groups of cellulose have a significant impact on the morphology and photocatalytic property of ZnO. This work aims to investigate the effect of different electronegative oxygen atoms of cellulose nanofibrils (CNF) on the formation and photocatalytic properties of ZnO/cellulose composites. The interaction between cellulose and ZnO has been achieved by controlling cellulose fiber size and regulating the electronegativity of oxygen atoms on the CNF surface. The results indicate that etherized CNF (ECNF) with the highest degree of etherification substitution (1.7) and the best electronegativity (−34.6 mV) can synthesize the ZnO/cellulose composite with the largest loading content of ZnO (58.9%) and the best photocatalytic activity for MO degradation (91.1%). It can be concluded that the intenser electrostatic interaction between oxygen atoms on the CNF surface and ZnO can facilitate the fixation and growth of more high-quality ZnO nanoflowers, thus improving the photocatalytic property. In a word, this work can provide a novel perspective for the efficient preparation of ZnO/cellulose composites with designable morphology and structure. |
abstractGer |
Cellulose is widely employed as a template in supporting and dispersing ZnO. The oxygen atom of the hydroxyl (–OH) groups of cellulose have a significant impact on the morphology and photocatalytic property of ZnO. This work aims to investigate the effect of different electronegative oxygen atoms of cellulose nanofibrils (CNF) on the formation and photocatalytic properties of ZnO/cellulose composites. The interaction between cellulose and ZnO has been achieved by controlling cellulose fiber size and regulating the electronegativity of oxygen atoms on the CNF surface. The results indicate that etherized CNF (ECNF) with the highest degree of etherification substitution (1.7) and the best electronegativity (−34.6 mV) can synthesize the ZnO/cellulose composite with the largest loading content of ZnO (58.9%) and the best photocatalytic activity for MO degradation (91.1%). It can be concluded that the intenser electrostatic interaction between oxygen atoms on the CNF surface and ZnO can facilitate the fixation and growth of more high-quality ZnO nanoflowers, thus improving the photocatalytic property. In a word, this work can provide a novel perspective for the efficient preparation of ZnO/cellulose composites with designable morphology and structure. |
abstract_unstemmed |
Cellulose is widely employed as a template in supporting and dispersing ZnO. The oxygen atom of the hydroxyl (–OH) groups of cellulose have a significant impact on the morphology and photocatalytic property of ZnO. This work aims to investigate the effect of different electronegative oxygen atoms of cellulose nanofibrils (CNF) on the formation and photocatalytic properties of ZnO/cellulose composites. The interaction between cellulose and ZnO has been achieved by controlling cellulose fiber size and regulating the electronegativity of oxygen atoms on the CNF surface. The results indicate that etherized CNF (ECNF) with the highest degree of etherification substitution (1.7) and the best electronegativity (−34.6 mV) can synthesize the ZnO/cellulose composite with the largest loading content of ZnO (58.9%) and the best photocatalytic activity for MO degradation (91.1%). It can be concluded that the intenser electrostatic interaction between oxygen atoms on the CNF surface and ZnO can facilitate the fixation and growth of more high-quality ZnO nanoflowers, thus improving the photocatalytic property. In a word, this work can provide a novel perspective for the efficient preparation of ZnO/cellulose composites with designable morphology and structure. |
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score |
7.4011383 |