Influence of relative humidity on the structure, swelling and electrical conductivity of PEDOT:PSS fibers

PEDOT:PSS is a conducting polymer with a wide variety of applications in the field of organic electronics. Over the past few years our group has developed PEDOT:PSS fibers with high electrical conductivity and robust mechanical properties, and we have observed changes in their properties that seemed...
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Gespeichert in:

Autor*in:	Sarabia-Riquelme, Ruben [verfasserIn] Schimpf, Warren C. [verfasserIn] Kuhn, Danielle L. [verfasserIn] Weisenberger, Matthew C. [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	PEDOT:PSS fiber Electrical conductivity Relative humidity Swelling Degradation Stability WAXS

Übergeordnetes Werk:	Enthalten in: Synthetic metals - Amsterdam [u.a.] : Elsevier Science, 1979, 297
Übergeordnetes Werk:	volume:297

DOI / URN:	10.1016/j.synthmet.2023.117399

Katalog-ID:	ELV061159476

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245	1	0	\|a Influence of relative humidity on the structure, swelling and electrical conductivity of PEDOT:PSS fibers
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520			\|a PEDOT:PSS is a conducting polymer with a wide variety of applications in the field of organic electronics. Over the past few years our group has developed PEDOT:PSS fibers with high electrical conductivity and robust mechanical properties, and we have observed changes in their properties that seemed to stem from seasonal changes in atmospheric relative humidity. In this work, we report the influence of relative humidity on the swelling, electrical conductivity and structure of wet-spun PEDOT:PSS fibers. The diameter of the fibers linearly increased with relative humidity up to the 70–80% range where the increase became exponential. The electrical conductivity reversibly decreased with increasing relative humidity with a similar linear and then exponential behavior. Additionally, an irreversible decrease (aging) in electrical conductivity was also observed. To gain more insight into the structural origin of these changes, wide angle x-ray scattering of the PEDOT:PSS fibers were gathered at different relative humidities in the 10–90% range so that the changes in structure could be observed in situ. On one hand, the lamella stacking distance of PEDOT and PSS chains increased linearly up to the 70–80% relative humidity range where the increase became exponential. On the other hand, the π-π stacking distance between PEDOT chains remained unaltered. We found that the changes in the lamella stacking distance were closely correlated to the changes observed for the diameter and electrical conductivity.
650		4	\|a PEDOT:PSS fiber
650		4	\|a Electrical conductivity
650		4	\|a Relative humidity
650		4	\|a Swelling
650		4	\|a Degradation
650		4	\|a Stability
650		4	\|a WAXS
700	1		\|a Schimpf, Warren C. \|e verfasserin \|4 aut
700	1		\|a Kuhn, Danielle L. \|e verfasserin \|4 aut
700	1		\|a Weisenberger, Matthew C. \|e verfasserin \|4 aut
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allfields	10.1016/j.synthmet.2023.117399 doi (DE-627)ELV061159476 (ELSEVIER)S0379-6779(23)00121-2 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl 51.50 bkl 58.00 bkl Sarabia-Riquelme, Ruben verfasserin aut Influence of relative humidity on the structure, swelling and electrical conductivity of PEDOT:PSS fibers 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier PEDOT:PSS is a conducting polymer with a wide variety of applications in the field of organic electronics. Over the past few years our group has developed PEDOT:PSS fibers with high electrical conductivity and robust mechanical properties, and we have observed changes in their properties that seemed to stem from seasonal changes in atmospheric relative humidity. In this work, we report the influence of relative humidity on the swelling, electrical conductivity and structure of wet-spun PEDOT:PSS fibers. The diameter of the fibers linearly increased with relative humidity up to the 70–80% range where the increase became exponential. The electrical conductivity reversibly decreased with increasing relative humidity with a similar linear and then exponential behavior. Additionally, an irreversible decrease (aging) in electrical conductivity was also observed. To gain more insight into the structural origin of these changes, wide angle x-ray scattering of the PEDOT:PSS fibers were gathered at different relative humidities in the 10–90% range so that the changes in structure could be observed in situ. On one hand, the lamella stacking distance of PEDOT and PSS chains increased linearly up to the 70–80% relative humidity range where the increase became exponential. On the other hand, the π-π stacking distance between PEDOT chains remained unaltered. We found that the changes in the lamella stacking distance were closely correlated to the changes observed for the diameter and electrical conductivity. PEDOT:PSS fiber Electrical conductivity Relative humidity Swelling Degradation Stability WAXS Schimpf, Warren C. verfasserin aut Kuhn, Danielle L. verfasserin aut Weisenberger, Matthew C. verfasserin aut Enthalten in Synthetic metals Amsterdam [u.a.] : Elsevier Science, 1979 297 Online-Ressource (DE-627)320525953 (DE-600)2015168-8 (DE-576)09861522X nnns volume:297 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ 51.50 Metallische Werkstoffe: Allgemeines VZ 58.00 Chemische Technik: Allgemeines VZ AR 297
spelling	10.1016/j.synthmet.2023.117399 doi (DE-627)ELV061159476 (ELSEVIER)S0379-6779(23)00121-2 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl 51.50 bkl 58.00 bkl Sarabia-Riquelme, Ruben verfasserin aut Influence of relative humidity on the structure, swelling and electrical conductivity of PEDOT:PSS fibers 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier PEDOT:PSS is a conducting polymer with a wide variety of applications in the field of organic electronics. Over the past few years our group has developed PEDOT:PSS fibers with high electrical conductivity and robust mechanical properties, and we have observed changes in their properties that seemed to stem from seasonal changes in atmospheric relative humidity. In this work, we report the influence of relative humidity on the swelling, electrical conductivity and structure of wet-spun PEDOT:PSS fibers. The diameter of the fibers linearly increased with relative humidity up to the 70–80% range where the increase became exponential. The electrical conductivity reversibly decreased with increasing relative humidity with a similar linear and then exponential behavior. Additionally, an irreversible decrease (aging) in electrical conductivity was also observed. To gain more insight into the structural origin of these changes, wide angle x-ray scattering of the PEDOT:PSS fibers were gathered at different relative humidities in the 10–90% range so that the changes in structure could be observed in situ. On one hand, the lamella stacking distance of PEDOT and PSS chains increased linearly up to the 70–80% relative humidity range where the increase became exponential. On the other hand, the π-π stacking distance between PEDOT chains remained unaltered. We found that the changes in the lamella stacking distance were closely correlated to the changes observed for the diameter and electrical conductivity. PEDOT:PSS fiber Electrical conductivity Relative humidity Swelling Degradation Stability WAXS Schimpf, Warren C. verfasserin aut Kuhn, Danielle L. verfasserin aut Weisenberger, Matthew C. verfasserin aut Enthalten in Synthetic metals Amsterdam [u.a.] : Elsevier Science, 1979 297 Online-Ressource (DE-627)320525953 (DE-600)2015168-8 (DE-576)09861522X nnns volume:297 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ 51.50 Metallische Werkstoffe: Allgemeines VZ 58.00 Chemische Technik: Allgemeines VZ AR 297
allfields_unstemmed	10.1016/j.synthmet.2023.117399 doi (DE-627)ELV061159476 (ELSEVIER)S0379-6779(23)00121-2 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl 51.50 bkl 58.00 bkl Sarabia-Riquelme, Ruben verfasserin aut Influence of relative humidity on the structure, swelling and electrical conductivity of PEDOT:PSS fibers 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier PEDOT:PSS is a conducting polymer with a wide variety of applications in the field of organic electronics. Over the past few years our group has developed PEDOT:PSS fibers with high electrical conductivity and robust mechanical properties, and we have observed changes in their properties that seemed to stem from seasonal changes in atmospheric relative humidity. In this work, we report the influence of relative humidity on the swelling, electrical conductivity and structure of wet-spun PEDOT:PSS fibers. The diameter of the fibers linearly increased with relative humidity up to the 70–80% range where the increase became exponential. The electrical conductivity reversibly decreased with increasing relative humidity with a similar linear and then exponential behavior. Additionally, an irreversible decrease (aging) in electrical conductivity was also observed. To gain more insight into the structural origin of these changes, wide angle x-ray scattering of the PEDOT:PSS fibers were gathered at different relative humidities in the 10–90% range so that the changes in structure could be observed in situ. On one hand, the lamella stacking distance of PEDOT and PSS chains increased linearly up to the 70–80% relative humidity range where the increase became exponential. On the other hand, the π-π stacking distance between PEDOT chains remained unaltered. We found that the changes in the lamella stacking distance were closely correlated to the changes observed for the diameter and electrical conductivity. PEDOT:PSS fiber Electrical conductivity Relative humidity Swelling Degradation Stability WAXS Schimpf, Warren C. verfasserin aut Kuhn, Danielle L. verfasserin aut Weisenberger, Matthew C. verfasserin aut Enthalten in Synthetic metals Amsterdam [u.a.] : Elsevier Science, 1979 297 Online-Ressource (DE-627)320525953 (DE-600)2015168-8 (DE-576)09861522X nnns volume:297 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ 51.50 Metallische Werkstoffe: Allgemeines VZ 58.00 Chemische Technik: Allgemeines VZ AR 297
allfieldsGer	10.1016/j.synthmet.2023.117399 doi (DE-627)ELV061159476 (ELSEVIER)S0379-6779(23)00121-2 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl 51.50 bkl 58.00 bkl Sarabia-Riquelme, Ruben verfasserin aut Influence of relative humidity on the structure, swelling and electrical conductivity of PEDOT:PSS fibers 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier PEDOT:PSS is a conducting polymer with a wide variety of applications in the field of organic electronics. Over the past few years our group has developed PEDOT:PSS fibers with high electrical conductivity and robust mechanical properties, and we have observed changes in their properties that seemed to stem from seasonal changes in atmospheric relative humidity. In this work, we report the influence of relative humidity on the swelling, electrical conductivity and structure of wet-spun PEDOT:PSS fibers. The diameter of the fibers linearly increased with relative humidity up to the 70–80% range where the increase became exponential. The electrical conductivity reversibly decreased with increasing relative humidity with a similar linear and then exponential behavior. Additionally, an irreversible decrease (aging) in electrical conductivity was also observed. To gain more insight into the structural origin of these changes, wide angle x-ray scattering of the PEDOT:PSS fibers were gathered at different relative humidities in the 10–90% range so that the changes in structure could be observed in situ. On one hand, the lamella stacking distance of PEDOT and PSS chains increased linearly up to the 70–80% relative humidity range where the increase became exponential. On the other hand, the π-π stacking distance between PEDOT chains remained unaltered. We found that the changes in the lamella stacking distance were closely correlated to the changes observed for the diameter and electrical conductivity. PEDOT:PSS fiber Electrical conductivity Relative humidity Swelling Degradation Stability WAXS Schimpf, Warren C. verfasserin aut Kuhn, Danielle L. verfasserin aut Weisenberger, Matthew C. verfasserin aut Enthalten in Synthetic metals Amsterdam [u.a.] : Elsevier Science, 1979 297 Online-Ressource (DE-627)320525953 (DE-600)2015168-8 (DE-576)09861522X nnns volume:297 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ 51.50 Metallische Werkstoffe: Allgemeines VZ 58.00 Chemische Technik: Allgemeines VZ AR 297
allfieldsSound	10.1016/j.synthmet.2023.117399 doi (DE-627)ELV061159476 (ELSEVIER)S0379-6779(23)00121-2 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl 51.50 bkl 58.00 bkl Sarabia-Riquelme, Ruben verfasserin aut Influence of relative humidity on the structure, swelling and electrical conductivity of PEDOT:PSS fibers 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier PEDOT:PSS is a conducting polymer with a wide variety of applications in the field of organic electronics. Over the past few years our group has developed PEDOT:PSS fibers with high electrical conductivity and robust mechanical properties, and we have observed changes in their properties that seemed to stem from seasonal changes in atmospheric relative humidity. In this work, we report the influence of relative humidity on the swelling, electrical conductivity and structure of wet-spun PEDOT:PSS fibers. The diameter of the fibers linearly increased with relative humidity up to the 70–80% range where the increase became exponential. The electrical conductivity reversibly decreased with increasing relative humidity with a similar linear and then exponential behavior. Additionally, an irreversible decrease (aging) in electrical conductivity was also observed. To gain more insight into the structural origin of these changes, wide angle x-ray scattering of the PEDOT:PSS fibers were gathered at different relative humidities in the 10–90% range so that the changes in structure could be observed in situ. On one hand, the lamella stacking distance of PEDOT and PSS chains increased linearly up to the 70–80% relative humidity range where the increase became exponential. On the other hand, the π-π stacking distance between PEDOT chains remained unaltered. We found that the changes in the lamella stacking distance were closely correlated to the changes observed for the diameter and electrical conductivity. PEDOT:PSS fiber Electrical conductivity Relative humidity Swelling Degradation Stability WAXS Schimpf, Warren C. verfasserin aut Kuhn, Danielle L. verfasserin aut Weisenberger, Matthew C. verfasserin aut Enthalten in Synthetic metals Amsterdam [u.a.] : Elsevier Science, 1979 297 Online-Ressource (DE-627)320525953 (DE-600)2015168-8 (DE-576)09861522X nnns volume:297 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ 51.50 Metallische Werkstoffe: Allgemeines VZ 58.00 Chemische Technik: Allgemeines VZ AR 297
language	English
source	Enthalten in Synthetic metals 297 volume:297
sourceStr	Enthalten in Synthetic metals 297 volume:297
format_phy_str_mv	Article
bklname	Chemie: Allgemeines Metallische Werkstoffe: Allgemeines Chemische Technik: Allgemeines
institution	findex.gbv.de
topic_facet	PEDOT:PSS fiber Electrical conductivity Relative humidity Swelling Degradation Stability WAXS
dewey-raw	540
isfreeaccess_bool	false
container_title	Synthetic metals
authorswithroles_txt_mv	Sarabia-Riquelme, Ruben @@aut@@ Schimpf, Warren C. @@aut@@ Kuhn, Danielle L. @@aut@@ Weisenberger, Matthew C. @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	320525953
dewey-sort	3540
id	ELV061159476
language_de	englisch
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author	Sarabia-Riquelme, Ruben
spellingShingle	Sarabia-Riquelme, Ruben ddc 540 bkl 35.00 bkl 51.50 bkl 58.00 misc PEDOT:PSS fiber misc Electrical conductivity misc Relative humidity misc Swelling misc Degradation misc Stability misc WAXS Influence of relative humidity on the structure, swelling and electrical conductivity of PEDOT:PSS fibers
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topic_title	540 VZ 35.00 bkl 51.50 bkl 58.00 bkl Influence of relative humidity on the structure, swelling and electrical conductivity of PEDOT:PSS fibers PEDOT:PSS fiber Electrical conductivity Relative humidity Swelling Degradation Stability WAXS
topic	ddc 540 bkl 35.00 bkl 51.50 bkl 58.00 misc PEDOT:PSS fiber misc Electrical conductivity misc Relative humidity misc Swelling misc Degradation misc Stability misc WAXS
topic_unstemmed	ddc 540 bkl 35.00 bkl 51.50 bkl 58.00 misc PEDOT:PSS fiber misc Electrical conductivity misc Relative humidity misc Swelling misc Degradation misc Stability misc WAXS
topic_browse	ddc 540 bkl 35.00 bkl 51.50 bkl 58.00 misc PEDOT:PSS fiber misc Electrical conductivity misc Relative humidity misc Swelling misc Degradation misc Stability misc WAXS
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title	Influence of relative humidity on the structure, swelling and electrical conductivity of PEDOT:PSS fibers
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title_full	Influence of relative humidity on the structure, swelling and electrical conductivity of PEDOT:PSS fibers
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author_browse	Sarabia-Riquelme, Ruben Schimpf, Warren C. Kuhn, Danielle L. Weisenberger, Matthew C.
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title_sort	influence of relative humidity on the structure, swelling and electrical conductivity of pedot:pss fibers
title_auth	Influence of relative humidity on the structure, swelling and electrical conductivity of PEDOT:PSS fibers
abstract	PEDOT:PSS is a conducting polymer with a wide variety of applications in the field of organic electronics. Over the past few years our group has developed PEDOT:PSS fibers with high electrical conductivity and robust mechanical properties, and we have observed changes in their properties that seemed to stem from seasonal changes in atmospheric relative humidity. In this work, we report the influence of relative humidity on the swelling, electrical conductivity and structure of wet-spun PEDOT:PSS fibers. The diameter of the fibers linearly increased with relative humidity up to the 70–80% range where the increase became exponential. The electrical conductivity reversibly decreased with increasing relative humidity with a similar linear and then exponential behavior. Additionally, an irreversible decrease (aging) in electrical conductivity was also observed. To gain more insight into the structural origin of these changes, wide angle x-ray scattering of the PEDOT:PSS fibers were gathered at different relative humidities in the 10–90% range so that the changes in structure could be observed in situ. On one hand, the lamella stacking distance of PEDOT and PSS chains increased linearly up to the 70–80% relative humidity range where the increase became exponential. On the other hand, the π-π stacking distance between PEDOT chains remained unaltered. We found that the changes in the lamella stacking distance were closely correlated to the changes observed for the diameter and electrical conductivity.
abstractGer	PEDOT:PSS is a conducting polymer with a wide variety of applications in the field of organic electronics. Over the past few years our group has developed PEDOT:PSS fibers with high electrical conductivity and robust mechanical properties, and we have observed changes in their properties that seemed to stem from seasonal changes in atmospheric relative humidity. In this work, we report the influence of relative humidity on the swelling, electrical conductivity and structure of wet-spun PEDOT:PSS fibers. The diameter of the fibers linearly increased with relative humidity up to the 70–80% range where the increase became exponential. The electrical conductivity reversibly decreased with increasing relative humidity with a similar linear and then exponential behavior. Additionally, an irreversible decrease (aging) in electrical conductivity was also observed. To gain more insight into the structural origin of these changes, wide angle x-ray scattering of the PEDOT:PSS fibers were gathered at different relative humidities in the 10–90% range so that the changes in structure could be observed in situ. On one hand, the lamella stacking distance of PEDOT and PSS chains increased linearly up to the 70–80% relative humidity range where the increase became exponential. On the other hand, the π-π stacking distance between PEDOT chains remained unaltered. We found that the changes in the lamella stacking distance were closely correlated to the changes observed for the diameter and electrical conductivity.
abstract_unstemmed	PEDOT:PSS is a conducting polymer with a wide variety of applications in the field of organic electronics. Over the past few years our group has developed PEDOT:PSS fibers with high electrical conductivity and robust mechanical properties, and we have observed changes in their properties that seemed to stem from seasonal changes in atmospheric relative humidity. In this work, we report the influence of relative humidity on the swelling, electrical conductivity and structure of wet-spun PEDOT:PSS fibers. The diameter of the fibers linearly increased with relative humidity up to the 70–80% range where the increase became exponential. The electrical conductivity reversibly decreased with increasing relative humidity with a similar linear and then exponential behavior. Additionally, an irreversible decrease (aging) in electrical conductivity was also observed. To gain more insight into the structural origin of these changes, wide angle x-ray scattering of the PEDOT:PSS fibers were gathered at different relative humidities in the 10–90% range so that the changes in structure could be observed in situ. On one hand, the lamella stacking distance of PEDOT and PSS chains increased linearly up to the 70–80% relative humidity range where the increase became exponential. On the other hand, the π-π stacking distance between PEDOT chains remained unaltered. We found that the changes in the lamella stacking distance were closely correlated to the changes observed for the diameter and electrical conductivity.
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title_short	Influence of relative humidity on the structure, swelling and electrical conductivity of PEDOT:PSS fibers
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author2	Schimpf, Warren C. Kuhn, Danielle L. Weisenberger, Matthew C.
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up_date	2024-07-06T17:17:39.022Z
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Influence of relative humidity on the structure, swelling and electrical conductivity of PEDOT:PSS fibers

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