Smart bifunctional covalent organic frameworks for water treatment: Reversible colorimetric pH detection and photocatalytic removal of pollutants

Covalent Organic Frameworks (COFs) with uniform aperture size, high surface area and tunable structure have been proposed as a potential material in water treatment. In this work, we utilized methoxy based covalent organic frameworks (COF–OMe) at room temperature as a dual-role smart material. For o...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Zhou, Zi-Wen [verfasserIn] Wu, Zhe-Ning [verfasserIn] Cai, Chun-Xian [verfasserIn] Lin, Ru-De [verfasserIn] Yu, Xiao-Qi [verfasserIn] Li, Kun [verfasserIn] Wang, Na [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Covalent organic frameworks Water treatment pH colorimetric detection Pollutants removal Light-controlled Oxidase-mimicking

Übergeordnetes Werk:	Enthalten in: Microporous and mesoporous materials - Amsterdam [u.a.] : Elsevier, 1998, 360
Übergeordnetes Werk:	volume:360

DOI / URN:	10.1016/j.micromeso.2023.112689

Katalog-ID:	ELV061206075

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100	1		\|a Zhou, Zi-Wen \|e verfasserin \|0 (orcid)0000-0001-5845-6762 \|4 aut
245	1	0	\|a Smart bifunctional covalent organic frameworks for water treatment: Reversible colorimetric pH detection and photocatalytic removal of pollutants
264		1	\|c 2023
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520			\|a Covalent Organic Frameworks (COFs) with uniform aperture size, high surface area and tunable structure have been proposed as a potential material in water treatment. In this work, we utilized methoxy based covalent organic frameworks (COF–OMe) at room temperature as a dual-role smart material. For one thing, it can respond to the pH of solutions by visual, colorimetric change. Due to the protonation effect of methoxy groups in its pore skeleton, the fluorescent intensity of COF–OMe went down and the color changed from yellow to black as the pH decreased reversibly. For another, the abundant pores and ordered conjugated structure endowed it with a large surface area and light absorption ability. Therefore, the light-triggered oxidase-mimic porous COF–OMe can be applied in the synergistic removal of organic pollutants with synergistic physical absorption and light degradation. The outstanding and sensitive response to pH, great removal efficiency and dual function made it applied in water treatment with great potential, achieving killing two birds with one stone.
650		4	\|a Covalent organic frameworks
650		4	\|a Water treatment
650		4	\|a pH colorimetric detection
650		4	\|a Pollutants removal
650		4	\|a Light-controlled
650		4	\|a Oxidase-mimicking
700	1		\|a Wu, Zhe-Ning \|e verfasserin \|4 aut
700	1		\|a Cai, Chun-Xian \|e verfasserin \|4 aut
700	1		\|a Lin, Ru-De \|e verfasserin \|4 aut
700	1		\|a Yu, Xiao-Qi \|e verfasserin \|4 aut
700	1		\|a Li, Kun \|e verfasserin \|4 aut
700	1		\|a Wang, Na \|e verfasserin \|0 (orcid)0000-0002-1703-1124 \|4 aut
773	0	8	\|i Enthalten in \|t Microporous and mesoporous materials \|d Amsterdam [u.a.] : Elsevier, 1998 \|g 360 \|h Online-Ressource \|w (DE-627)318368277 \|w (DE-600)2012505-7 \|w (DE-576)09529998X \|x 1387-1811 \|7 nnns
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publishDate	2023
allfields	10.1016/j.micromeso.2023.112689 doi (DE-627)ELV061206075 (ELSEVIER)S1387-1811(23)00265-2 DE-627 ger DE-627 rda eng 530 VZ 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 bkl Zhou, Zi-Wen verfasserin (orcid)0000-0001-5845-6762 aut Smart bifunctional covalent organic frameworks for water treatment: Reversible colorimetric pH detection and photocatalytic removal of pollutants 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Covalent Organic Frameworks (COFs) with uniform aperture size, high surface area and tunable structure have been proposed as a potential material in water treatment. In this work, we utilized methoxy based covalent organic frameworks (COF–OMe) at room temperature as a dual-role smart material. For one thing, it can respond to the pH of solutions by visual, colorimetric change. Due to the protonation effect of methoxy groups in its pore skeleton, the fluorescent intensity of COF–OMe went down and the color changed from yellow to black as the pH decreased reversibly. For another, the abundant pores and ordered conjugated structure endowed it with a large surface area and light absorption ability. Therefore, the light-triggered oxidase-mimic porous COF–OMe can be applied in the synergistic removal of organic pollutants with synergistic physical absorption and light degradation. The outstanding and sensitive response to pH, great removal efficiency and dual function made it applied in water treatment with great potential, achieving killing two birds with one stone. Covalent organic frameworks Water treatment pH colorimetric detection Pollutants removal Light-controlled Oxidase-mimicking Wu, Zhe-Ning verfasserin aut Cai, Chun-Xian verfasserin aut Lin, Ru-De verfasserin aut Yu, Xiao-Qi verfasserin aut Li, Kun verfasserin aut Wang, Na verfasserin (orcid)0000-0002-1703-1124 aut Enthalten in Microporous and mesoporous materials Amsterdam [u.a.] : Elsevier, 1998 360 Online-Ressource (DE-627)318368277 (DE-600)2012505-7 (DE-576)09529998X 1387-1811 nnns volume:360 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 38.30 Mineralogie VZ 35.68 Organische Verbindungen: Sonstiges VZ 33.61 Festkörperphysik VZ 35.90 Festkörperchemie VZ 51.45 Werkstoffe mit besonderen Eigenschaften VZ AR 360
spelling	10.1016/j.micromeso.2023.112689 doi (DE-627)ELV061206075 (ELSEVIER)S1387-1811(23)00265-2 DE-627 ger DE-627 rda eng 530 VZ 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 bkl Zhou, Zi-Wen verfasserin (orcid)0000-0001-5845-6762 aut Smart bifunctional covalent organic frameworks for water treatment: Reversible colorimetric pH detection and photocatalytic removal of pollutants 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Covalent Organic Frameworks (COFs) with uniform aperture size, high surface area and tunable structure have been proposed as a potential material in water treatment. In this work, we utilized methoxy based covalent organic frameworks (COF–OMe) at room temperature as a dual-role smart material. For one thing, it can respond to the pH of solutions by visual, colorimetric change. Due to the protonation effect of methoxy groups in its pore skeleton, the fluorescent intensity of COF–OMe went down and the color changed from yellow to black as the pH decreased reversibly. For another, the abundant pores and ordered conjugated structure endowed it with a large surface area and light absorption ability. Therefore, the light-triggered oxidase-mimic porous COF–OMe can be applied in the synergistic removal of organic pollutants with synergistic physical absorption and light degradation. The outstanding and sensitive response to pH, great removal efficiency and dual function made it applied in water treatment with great potential, achieving killing two birds with one stone. Covalent organic frameworks Water treatment pH colorimetric detection Pollutants removal Light-controlled Oxidase-mimicking Wu, Zhe-Ning verfasserin aut Cai, Chun-Xian verfasserin aut Lin, Ru-De verfasserin aut Yu, Xiao-Qi verfasserin aut Li, Kun verfasserin aut Wang, Na verfasserin (orcid)0000-0002-1703-1124 aut Enthalten in Microporous and mesoporous materials Amsterdam [u.a.] : Elsevier, 1998 360 Online-Ressource (DE-627)318368277 (DE-600)2012505-7 (DE-576)09529998X 1387-1811 nnns volume:360 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 38.30 Mineralogie VZ 35.68 Organische Verbindungen: Sonstiges VZ 33.61 Festkörperphysik VZ 35.90 Festkörperchemie VZ 51.45 Werkstoffe mit besonderen Eigenschaften VZ AR 360
allfields_unstemmed	10.1016/j.micromeso.2023.112689 doi (DE-627)ELV061206075 (ELSEVIER)S1387-1811(23)00265-2 DE-627 ger DE-627 rda eng 530 VZ 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 bkl Zhou, Zi-Wen verfasserin (orcid)0000-0001-5845-6762 aut Smart bifunctional covalent organic frameworks for water treatment: Reversible colorimetric pH detection and photocatalytic removal of pollutants 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Covalent Organic Frameworks (COFs) with uniform aperture size, high surface area and tunable structure have been proposed as a potential material in water treatment. In this work, we utilized methoxy based covalent organic frameworks (COF–OMe) at room temperature as a dual-role smart material. For one thing, it can respond to the pH of solutions by visual, colorimetric change. Due to the protonation effect of methoxy groups in its pore skeleton, the fluorescent intensity of COF–OMe went down and the color changed from yellow to black as the pH decreased reversibly. For another, the abundant pores and ordered conjugated structure endowed it with a large surface area and light absorption ability. Therefore, the light-triggered oxidase-mimic porous COF–OMe can be applied in the synergistic removal of organic pollutants with synergistic physical absorption and light degradation. The outstanding and sensitive response to pH, great removal efficiency and dual function made it applied in water treatment with great potential, achieving killing two birds with one stone. Covalent organic frameworks Water treatment pH colorimetric detection Pollutants removal Light-controlled Oxidase-mimicking Wu, Zhe-Ning verfasserin aut Cai, Chun-Xian verfasserin aut Lin, Ru-De verfasserin aut Yu, Xiao-Qi verfasserin aut Li, Kun verfasserin aut Wang, Na verfasserin (orcid)0000-0002-1703-1124 aut Enthalten in Microporous and mesoporous materials Amsterdam [u.a.] : Elsevier, 1998 360 Online-Ressource (DE-627)318368277 (DE-600)2012505-7 (DE-576)09529998X 1387-1811 nnns volume:360 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 38.30 Mineralogie VZ 35.68 Organische Verbindungen: Sonstiges VZ 33.61 Festkörperphysik VZ 35.90 Festkörperchemie VZ 51.45 Werkstoffe mit besonderen Eigenschaften VZ AR 360
allfieldsGer	10.1016/j.micromeso.2023.112689 doi (DE-627)ELV061206075 (ELSEVIER)S1387-1811(23)00265-2 DE-627 ger DE-627 rda eng 530 VZ 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 bkl Zhou, Zi-Wen verfasserin (orcid)0000-0001-5845-6762 aut Smart bifunctional covalent organic frameworks for water treatment: Reversible colorimetric pH detection and photocatalytic removal of pollutants 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Covalent Organic Frameworks (COFs) with uniform aperture size, high surface area and tunable structure have been proposed as a potential material in water treatment. In this work, we utilized methoxy based covalent organic frameworks (COF–OMe) at room temperature as a dual-role smart material. For one thing, it can respond to the pH of solutions by visual, colorimetric change. Due to the protonation effect of methoxy groups in its pore skeleton, the fluorescent intensity of COF–OMe went down and the color changed from yellow to black as the pH decreased reversibly. For another, the abundant pores and ordered conjugated structure endowed it with a large surface area and light absorption ability. Therefore, the light-triggered oxidase-mimic porous COF–OMe can be applied in the synergistic removal of organic pollutants with synergistic physical absorption and light degradation. The outstanding and sensitive response to pH, great removal efficiency and dual function made it applied in water treatment with great potential, achieving killing two birds with one stone. Covalent organic frameworks Water treatment pH colorimetric detection Pollutants removal Light-controlled Oxidase-mimicking Wu, Zhe-Ning verfasserin aut Cai, Chun-Xian verfasserin aut Lin, Ru-De verfasserin aut Yu, Xiao-Qi verfasserin aut Li, Kun verfasserin aut Wang, Na verfasserin (orcid)0000-0002-1703-1124 aut Enthalten in Microporous and mesoporous materials Amsterdam [u.a.] : Elsevier, 1998 360 Online-Ressource (DE-627)318368277 (DE-600)2012505-7 (DE-576)09529998X 1387-1811 nnns volume:360 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 38.30 Mineralogie VZ 35.68 Organische Verbindungen: Sonstiges VZ 33.61 Festkörperphysik VZ 35.90 Festkörperchemie VZ 51.45 Werkstoffe mit besonderen Eigenschaften VZ AR 360
allfieldsSound	10.1016/j.micromeso.2023.112689 doi (DE-627)ELV061206075 (ELSEVIER)S1387-1811(23)00265-2 DE-627 ger DE-627 rda eng 530 VZ 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 bkl Zhou, Zi-Wen verfasserin (orcid)0000-0001-5845-6762 aut Smart bifunctional covalent organic frameworks for water treatment: Reversible colorimetric pH detection and photocatalytic removal of pollutants 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Covalent Organic Frameworks (COFs) with uniform aperture size, high surface area and tunable structure have been proposed as a potential material in water treatment. In this work, we utilized methoxy based covalent organic frameworks (COF–OMe) at room temperature as a dual-role smart material. For one thing, it can respond to the pH of solutions by visual, colorimetric change. Due to the protonation effect of methoxy groups in its pore skeleton, the fluorescent intensity of COF–OMe went down and the color changed from yellow to black as the pH decreased reversibly. For another, the abundant pores and ordered conjugated structure endowed it with a large surface area and light absorption ability. Therefore, the light-triggered oxidase-mimic porous COF–OMe can be applied in the synergistic removal of organic pollutants with synergistic physical absorption and light degradation. The outstanding and sensitive response to pH, great removal efficiency and dual function made it applied in water treatment with great potential, achieving killing two birds with one stone. Covalent organic frameworks Water treatment pH colorimetric detection Pollutants removal Light-controlled Oxidase-mimicking Wu, Zhe-Ning verfasserin aut Cai, Chun-Xian verfasserin aut Lin, Ru-De verfasserin aut Yu, Xiao-Qi verfasserin aut Li, Kun verfasserin aut Wang, Na verfasserin (orcid)0000-0002-1703-1124 aut Enthalten in Microporous and mesoporous materials Amsterdam [u.a.] : Elsevier, 1998 360 Online-Ressource (DE-627)318368277 (DE-600)2012505-7 (DE-576)09529998X 1387-1811 nnns volume:360 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 38.30 Mineralogie VZ 35.68 Organische Verbindungen: Sonstiges VZ 33.61 Festkörperphysik VZ 35.90 Festkörperchemie VZ 51.45 Werkstoffe mit besonderen Eigenschaften VZ AR 360
language	English
source	Enthalten in Microporous and mesoporous materials 360 volume:360
sourceStr	Enthalten in Microporous and mesoporous materials 360 volume:360
format_phy_str_mv	Article
bklname	Mineralogie Organische Verbindungen: Sonstiges Festkörperphysik Festkörperchemie Werkstoffe mit besonderen Eigenschaften
institution	findex.gbv.de
topic_facet	Covalent organic frameworks Water treatment pH colorimetric detection Pollutants removal Light-controlled Oxidase-mimicking
dewey-raw	530
isfreeaccess_bool	false
container_title	Microporous and mesoporous materials
authorswithroles_txt_mv	Zhou, Zi-Wen @@aut@@ Wu, Zhe-Ning @@aut@@ Cai, Chun-Xian @@aut@@ Lin, Ru-De @@aut@@ Yu, Xiao-Qi @@aut@@ Li, Kun @@aut@@ Wang, Na @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	318368277
dewey-sort	3530
id	ELV061206075
language_de	englisch
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author	Zhou, Zi-Wen
spellingShingle	Zhou, Zi-Wen ddc 530 bkl 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 misc Covalent organic frameworks misc Water treatment misc pH colorimetric detection misc Pollutants removal misc Light-controlled misc Oxidase-mimicking Smart bifunctional covalent organic frameworks for water treatment: Reversible colorimetric pH detection and photocatalytic removal of pollutants
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topic_title	530 VZ 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 bkl Smart bifunctional covalent organic frameworks for water treatment: Reversible colorimetric pH detection and photocatalytic removal of pollutants Covalent organic frameworks Water treatment pH colorimetric detection Pollutants removal Light-controlled Oxidase-mimicking
topic	ddc 530 bkl 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 misc Covalent organic frameworks misc Water treatment misc pH colorimetric detection misc Pollutants removal misc Light-controlled misc Oxidase-mimicking
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topic_browse	ddc 530 bkl 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 misc Covalent organic frameworks misc Water treatment misc pH colorimetric detection misc Pollutants removal misc Light-controlled misc Oxidase-mimicking
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title	Smart bifunctional covalent organic frameworks for water treatment: Reversible colorimetric pH detection and photocatalytic removal of pollutants
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title_full	Smart bifunctional covalent organic frameworks for water treatment: Reversible colorimetric pH detection and photocatalytic removal of pollutants
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title_sort	smart bifunctional covalent organic frameworks for water treatment: reversible colorimetric ph detection and photocatalytic removal of pollutants
title_auth	Smart bifunctional covalent organic frameworks for water treatment: Reversible colorimetric pH detection and photocatalytic removal of pollutants
abstract	Covalent Organic Frameworks (COFs) with uniform aperture size, high surface area and tunable structure have been proposed as a potential material in water treatment. In this work, we utilized methoxy based covalent organic frameworks (COF–OMe) at room temperature as a dual-role smart material. For one thing, it can respond to the pH of solutions by visual, colorimetric change. Due to the protonation effect of methoxy groups in its pore skeleton, the fluorescent intensity of COF–OMe went down and the color changed from yellow to black as the pH decreased reversibly. For another, the abundant pores and ordered conjugated structure endowed it with a large surface area and light absorption ability. Therefore, the light-triggered oxidase-mimic porous COF–OMe can be applied in the synergistic removal of organic pollutants with synergistic physical absorption and light degradation. The outstanding and sensitive response to pH, great removal efficiency and dual function made it applied in water treatment with great potential, achieving killing two birds with one stone.
abstractGer	Covalent Organic Frameworks (COFs) with uniform aperture size, high surface area and tunable structure have been proposed as a potential material in water treatment. In this work, we utilized methoxy based covalent organic frameworks (COF–OMe) at room temperature as a dual-role smart material. For one thing, it can respond to the pH of solutions by visual, colorimetric change. Due to the protonation effect of methoxy groups in its pore skeleton, the fluorescent intensity of COF–OMe went down and the color changed from yellow to black as the pH decreased reversibly. For another, the abundant pores and ordered conjugated structure endowed it with a large surface area and light absorption ability. Therefore, the light-triggered oxidase-mimic porous COF–OMe can be applied in the synergistic removal of organic pollutants with synergistic physical absorption and light degradation. The outstanding and sensitive response to pH, great removal efficiency and dual function made it applied in water treatment with great potential, achieving killing two birds with one stone.
abstract_unstemmed	Covalent Organic Frameworks (COFs) with uniform aperture size, high surface area and tunable structure have been proposed as a potential material in water treatment. In this work, we utilized methoxy based covalent organic frameworks (COF–OMe) at room temperature as a dual-role smart material. For one thing, it can respond to the pH of solutions by visual, colorimetric change. Due to the protonation effect of methoxy groups in its pore skeleton, the fluorescent intensity of COF–OMe went down and the color changed from yellow to black as the pH decreased reversibly. For another, the abundant pores and ordered conjugated structure endowed it with a large surface area and light absorption ability. Therefore, the light-triggered oxidase-mimic porous COF–OMe can be applied in the synergistic removal of organic pollutants with synergistic physical absorption and light degradation. The outstanding and sensitive response to pH, great removal efficiency and dual function made it applied in water treatment with great potential, achieving killing two birds with one stone.
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title_short	Smart bifunctional covalent organic frameworks for water treatment: Reversible colorimetric pH detection and photocatalytic removal of pollutants
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author2	Wu, Zhe-Ning Cai, Chun-Xian Lin, Ru-De Yu, Xiao-Qi Li, Kun Wang, Na
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up_date	2024-07-06T17:20:21.144Z
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