Chloride ion with ferric ion in boosting zero-valent copper activated peroxydisulfate for efficiently removing tetracycline

The Cu0-stimulated PDS system, which produces reactive oxygen species (ROS) to decompose environmental pollutants, has been widely studied. Although Cu+ is produced in the Cu0-stimulated PDS system, its susceptibility to disproportionate and easy oxidized by O2 must be considered. To improve the uti...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Xu, Peng [verfasserIn] Zhu, Pengfei [verfasserIn] Yang, Zhuoyu [verfasserIn] Liu, Xin [verfasserIn] Wu, Ruoxi [verfasserIn] Hou, Baolin [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Cl Tetracycline Sulfate radical Reactive chlorine species Hydroxyl radical

Übergeordnetes Werk:	Enthalten in: The chemical engineering journal - Amsterdam : Elsevier, 1997, 471
Übergeordnetes Werk:	volume:471

DOI / URN:	10.1016/j.cej.2023.144773

Katalog-ID:	ELV061367516

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520			\|a The Cu0-stimulated PDS system, which produces reactive oxygen species (ROS) to decompose environmental pollutants, has been widely studied. Although Cu+ is produced in the Cu0-stimulated PDS system, its susceptibility to disproportionate and easy oxidized by O2 must be considered. To improve the utilization of Cu+, Cl− and Fe3+ were considered for strengthening the Cu0-stimulated PDS process. With the addition of Cl− and Fe3+ in the Cu0-stimulated PDS system (Cl−/Fe3+/Cu0/PDS system), the decomposition of tetracycline was greatly increased within 8 min. In the Cl−/Fe3+/Cu0/PDS system, Cl− limited the disproportionation reaction of Cu+ by promoting Cu0 and Cu2+ reaction with Cl− and increased Cu+ utilization rate. Fe3+ promoted the recycling of Fe2+/Fe3+ and contributed to reducing the invalid oxidation of Cu+ by O2. Sulfate radical, reactive chlorine species and hydroxyl radical were generated in the Cl−/Fe3+/Cu0/PDS system. NO3 − and SO4 2− had no influence on decomposing tetracycline in the Cl−/Fe3+/Cu0/PDS system, but humic acid inhibited tetracycline decomposition. Moreover, the Cl−/Fe3+/Cu0/PDS system had great performance on the experimental water samples with the removal rate of tetracycline was higher than 80%. Furthermore, when the final solution pH was adjusted to 8.0, only 0.88 mg/L total dissolved copper remained after precipitation and filtering.
650		4	\|a Cl
650		4	\|a Tetracycline
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700	1		\|a Wu, Ruoxi \|e verfasserin \|4 aut
700	1		\|a Hou, Baolin \|e verfasserin \|4 aut
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936	b	k	\|a 58.10 \|j Verfahrenstechnik: Allgemeines \|q VZ
951			\|a AR
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allfields	10.1016/j.cej.2023.144773 doi (DE-627)ELV061367516 (ELSEVIER)S1385-8947(23)03504-0 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Xu, Peng verfasserin aut Chloride ion with ferric ion in boosting zero-valent copper activated peroxydisulfate for efficiently removing tetracycline 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The Cu0-stimulated PDS system, which produces reactive oxygen species (ROS) to decompose environmental pollutants, has been widely studied. Although Cu+ is produced in the Cu0-stimulated PDS system, its susceptibility to disproportionate and easy oxidized by O2 must be considered. To improve the utilization of Cu+, Cl− and Fe3+ were considered for strengthening the Cu0-stimulated PDS process. With the addition of Cl− and Fe3+ in the Cu0-stimulated PDS system (Cl−/Fe3+/Cu0/PDS system), the decomposition of tetracycline was greatly increased within 8 min. In the Cl−/Fe3+/Cu0/PDS system, Cl− limited the disproportionation reaction of Cu+ by promoting Cu0 and Cu2+ reaction with Cl− and increased Cu+ utilization rate. Fe3+ promoted the recycling of Fe2+/Fe3+ and contributed to reducing the invalid oxidation of Cu+ by O2. Sulfate radical, reactive chlorine species and hydroxyl radical were generated in the Cl−/Fe3+/Cu0/PDS system. NO3 − and SO4 2− had no influence on decomposing tetracycline in the Cl−/Fe3+/Cu0/PDS system, but humic acid inhibited tetracycline decomposition. Moreover, the Cl−/Fe3+/Cu0/PDS system had great performance on the experimental water samples with the removal rate of tetracycline was higher than 80%. Furthermore, when the final solution pH was adjusted to 8.0, only 0.88 mg/L total dissolved copper remained after precipitation and filtering. Cl Tetracycline Sulfate radical Reactive chlorine species Hydroxyl radical Zhu, Pengfei verfasserin (orcid)0000-0001-9515-1490 aut Yang, Zhuoyu verfasserin aut Liu, Xin verfasserin aut Wu, Ruoxi verfasserin aut Hou, Baolin verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 471 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:471 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 471
spelling	10.1016/j.cej.2023.144773 doi (DE-627)ELV061367516 (ELSEVIER)S1385-8947(23)03504-0 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Xu, Peng verfasserin aut Chloride ion with ferric ion in boosting zero-valent copper activated peroxydisulfate for efficiently removing tetracycline 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The Cu0-stimulated PDS system, which produces reactive oxygen species (ROS) to decompose environmental pollutants, has been widely studied. Although Cu+ is produced in the Cu0-stimulated PDS system, its susceptibility to disproportionate and easy oxidized by O2 must be considered. To improve the utilization of Cu+, Cl− and Fe3+ were considered for strengthening the Cu0-stimulated PDS process. With the addition of Cl− and Fe3+ in the Cu0-stimulated PDS system (Cl−/Fe3+/Cu0/PDS system), the decomposition of tetracycline was greatly increased within 8 min. In the Cl−/Fe3+/Cu0/PDS system, Cl− limited the disproportionation reaction of Cu+ by promoting Cu0 and Cu2+ reaction with Cl− and increased Cu+ utilization rate. Fe3+ promoted the recycling of Fe2+/Fe3+ and contributed to reducing the invalid oxidation of Cu+ by O2. Sulfate radical, reactive chlorine species and hydroxyl radical were generated in the Cl−/Fe3+/Cu0/PDS system. NO3 − and SO4 2− had no influence on decomposing tetracycline in the Cl−/Fe3+/Cu0/PDS system, but humic acid inhibited tetracycline decomposition. Moreover, the Cl−/Fe3+/Cu0/PDS system had great performance on the experimental water samples with the removal rate of tetracycline was higher than 80%. Furthermore, when the final solution pH was adjusted to 8.0, only 0.88 mg/L total dissolved copper remained after precipitation and filtering. Cl Tetracycline Sulfate radical Reactive chlorine species Hydroxyl radical Zhu, Pengfei verfasserin (orcid)0000-0001-9515-1490 aut Yang, Zhuoyu verfasserin aut Liu, Xin verfasserin aut Wu, Ruoxi verfasserin aut Hou, Baolin verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 471 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:471 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 471
allfields_unstemmed	10.1016/j.cej.2023.144773 doi (DE-627)ELV061367516 (ELSEVIER)S1385-8947(23)03504-0 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Xu, Peng verfasserin aut Chloride ion with ferric ion in boosting zero-valent copper activated peroxydisulfate for efficiently removing tetracycline 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The Cu0-stimulated PDS system, which produces reactive oxygen species (ROS) to decompose environmental pollutants, has been widely studied. Although Cu+ is produced in the Cu0-stimulated PDS system, its susceptibility to disproportionate and easy oxidized by O2 must be considered. To improve the utilization of Cu+, Cl− and Fe3+ were considered for strengthening the Cu0-stimulated PDS process. With the addition of Cl− and Fe3+ in the Cu0-stimulated PDS system (Cl−/Fe3+/Cu0/PDS system), the decomposition of tetracycline was greatly increased within 8 min. In the Cl−/Fe3+/Cu0/PDS system, Cl− limited the disproportionation reaction of Cu+ by promoting Cu0 and Cu2+ reaction with Cl− and increased Cu+ utilization rate. Fe3+ promoted the recycling of Fe2+/Fe3+ and contributed to reducing the invalid oxidation of Cu+ by O2. Sulfate radical, reactive chlorine species and hydroxyl radical were generated in the Cl−/Fe3+/Cu0/PDS system. NO3 − and SO4 2− had no influence on decomposing tetracycline in the Cl−/Fe3+/Cu0/PDS system, but humic acid inhibited tetracycline decomposition. Moreover, the Cl−/Fe3+/Cu0/PDS system had great performance on the experimental water samples with the removal rate of tetracycline was higher than 80%. Furthermore, when the final solution pH was adjusted to 8.0, only 0.88 mg/L total dissolved copper remained after precipitation and filtering. Cl Tetracycline Sulfate radical Reactive chlorine species Hydroxyl radical Zhu, Pengfei verfasserin (orcid)0000-0001-9515-1490 aut Yang, Zhuoyu verfasserin aut Liu, Xin verfasserin aut Wu, Ruoxi verfasserin aut Hou, Baolin verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 471 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:471 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 471
allfieldsGer	10.1016/j.cej.2023.144773 doi (DE-627)ELV061367516 (ELSEVIER)S1385-8947(23)03504-0 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Xu, Peng verfasserin aut Chloride ion with ferric ion in boosting zero-valent copper activated peroxydisulfate for efficiently removing tetracycline 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The Cu0-stimulated PDS system, which produces reactive oxygen species (ROS) to decompose environmental pollutants, has been widely studied. Although Cu+ is produced in the Cu0-stimulated PDS system, its susceptibility to disproportionate and easy oxidized by O2 must be considered. To improve the utilization of Cu+, Cl− and Fe3+ were considered for strengthening the Cu0-stimulated PDS process. With the addition of Cl− and Fe3+ in the Cu0-stimulated PDS system (Cl−/Fe3+/Cu0/PDS system), the decomposition of tetracycline was greatly increased within 8 min. In the Cl−/Fe3+/Cu0/PDS system, Cl− limited the disproportionation reaction of Cu+ by promoting Cu0 and Cu2+ reaction with Cl− and increased Cu+ utilization rate. Fe3+ promoted the recycling of Fe2+/Fe3+ and contributed to reducing the invalid oxidation of Cu+ by O2. Sulfate radical, reactive chlorine species and hydroxyl radical were generated in the Cl−/Fe3+/Cu0/PDS system. NO3 − and SO4 2− had no influence on decomposing tetracycline in the Cl−/Fe3+/Cu0/PDS system, but humic acid inhibited tetracycline decomposition. Moreover, the Cl−/Fe3+/Cu0/PDS system had great performance on the experimental water samples with the removal rate of tetracycline was higher than 80%. Furthermore, when the final solution pH was adjusted to 8.0, only 0.88 mg/L total dissolved copper remained after precipitation and filtering. Cl Tetracycline Sulfate radical Reactive chlorine species Hydroxyl radical Zhu, Pengfei verfasserin (orcid)0000-0001-9515-1490 aut Yang, Zhuoyu verfasserin aut Liu, Xin verfasserin aut Wu, Ruoxi verfasserin aut Hou, Baolin verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 471 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:471 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 471
allfieldsSound	10.1016/j.cej.2023.144773 doi (DE-627)ELV061367516 (ELSEVIER)S1385-8947(23)03504-0 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Xu, Peng verfasserin aut Chloride ion with ferric ion in boosting zero-valent copper activated peroxydisulfate for efficiently removing tetracycline 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The Cu0-stimulated PDS system, which produces reactive oxygen species (ROS) to decompose environmental pollutants, has been widely studied. Although Cu+ is produced in the Cu0-stimulated PDS system, its susceptibility to disproportionate and easy oxidized by O2 must be considered. To improve the utilization of Cu+, Cl− and Fe3+ were considered for strengthening the Cu0-stimulated PDS process. With the addition of Cl− and Fe3+ in the Cu0-stimulated PDS system (Cl−/Fe3+/Cu0/PDS system), the decomposition of tetracycline was greatly increased within 8 min. In the Cl−/Fe3+/Cu0/PDS system, Cl− limited the disproportionation reaction of Cu+ by promoting Cu0 and Cu2+ reaction with Cl− and increased Cu+ utilization rate. Fe3+ promoted the recycling of Fe2+/Fe3+ and contributed to reducing the invalid oxidation of Cu+ by O2. Sulfate radical, reactive chlorine species and hydroxyl radical were generated in the Cl−/Fe3+/Cu0/PDS system. NO3 − and SO4 2− had no influence on decomposing tetracycline in the Cl−/Fe3+/Cu0/PDS system, but humic acid inhibited tetracycline decomposition. Moreover, the Cl−/Fe3+/Cu0/PDS system had great performance on the experimental water samples with the removal rate of tetracycline was higher than 80%. Furthermore, when the final solution pH was adjusted to 8.0, only 0.88 mg/L total dissolved copper remained after precipitation and filtering. Cl Tetracycline Sulfate radical Reactive chlorine species Hydroxyl radical Zhu, Pengfei verfasserin (orcid)0000-0001-9515-1490 aut Yang, Zhuoyu verfasserin aut Liu, Xin verfasserin aut Wu, Ruoxi verfasserin aut Hou, Baolin verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 471 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:471 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 471
language	English
source	Enthalten in The chemical engineering journal 471 volume:471
sourceStr	Enthalten in The chemical engineering journal 471 volume:471
format_phy_str_mv	Article
bklname	Verfahrenstechnik: Allgemeines
institution	findex.gbv.de
topic_facet	Cl Tetracycline Sulfate radical Reactive chlorine species Hydroxyl radical
dewey-raw	660
isfreeaccess_bool	false
container_title	The chemical engineering journal
authorswithroles_txt_mv	Xu, Peng @@aut@@ Zhu, Pengfei @@aut@@ Yang, Zhuoyu @@aut@@ Liu, Xin @@aut@@ Wu, Ruoxi @@aut@@ Hou, Baolin @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	320500322
dewey-sort	3660
id	ELV061367516
language_de	englisch
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author	Xu, Peng
spellingShingle	Xu, Peng ddc 660 bkl 58.10 misc Cl misc Tetracycline misc Sulfate radical misc Reactive chlorine species misc Hydroxyl radical Chloride ion with ferric ion in boosting zero-valent copper activated peroxydisulfate for efficiently removing tetracycline
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topic_title	660 VZ 58.10 bkl Chloride ion with ferric ion in boosting zero-valent copper activated peroxydisulfate for efficiently removing tetracycline Cl Tetracycline Sulfate radical Reactive chlorine species Hydroxyl radical
topic	ddc 660 bkl 58.10 misc Cl misc Tetracycline misc Sulfate radical misc Reactive chlorine species misc Hydroxyl radical
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title	Chloride ion with ferric ion in boosting zero-valent copper activated peroxydisulfate for efficiently removing tetracycline
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title_full	Chloride ion with ferric ion in boosting zero-valent copper activated peroxydisulfate for efficiently removing tetracycline
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title_sort	chloride ion with ferric ion in boosting zero-valent copper activated peroxydisulfate for efficiently removing tetracycline
title_auth	Chloride ion with ferric ion in boosting zero-valent copper activated peroxydisulfate for efficiently removing tetracycline
abstract	The Cu0-stimulated PDS system, which produces reactive oxygen species (ROS) to decompose environmental pollutants, has been widely studied. Although Cu+ is produced in the Cu0-stimulated PDS system, its susceptibility to disproportionate and easy oxidized by O2 must be considered. To improve the utilization of Cu+, Cl− and Fe3+ were considered for strengthening the Cu0-stimulated PDS process. With the addition of Cl− and Fe3+ in the Cu0-stimulated PDS system (Cl−/Fe3+/Cu0/PDS system), the decomposition of tetracycline was greatly increased within 8 min. In the Cl−/Fe3+/Cu0/PDS system, Cl− limited the disproportionation reaction of Cu+ by promoting Cu0 and Cu2+ reaction with Cl− and increased Cu+ utilization rate. Fe3+ promoted the recycling of Fe2+/Fe3+ and contributed to reducing the invalid oxidation of Cu+ by O2. Sulfate radical, reactive chlorine species and hydroxyl radical were generated in the Cl−/Fe3+/Cu0/PDS system. NO3 − and SO4 2− had no influence on decomposing tetracycline in the Cl−/Fe3+/Cu0/PDS system, but humic acid inhibited tetracycline decomposition. Moreover, the Cl−/Fe3+/Cu0/PDS system had great performance on the experimental water samples with the removal rate of tetracycline was higher than 80%. Furthermore, when the final solution pH was adjusted to 8.0, only 0.88 mg/L total dissolved copper remained after precipitation and filtering.
abstractGer	The Cu0-stimulated PDS system, which produces reactive oxygen species (ROS) to decompose environmental pollutants, has been widely studied. Although Cu+ is produced in the Cu0-stimulated PDS system, its susceptibility to disproportionate and easy oxidized by O2 must be considered. To improve the utilization of Cu+, Cl− and Fe3+ were considered for strengthening the Cu0-stimulated PDS process. With the addition of Cl− and Fe3+ in the Cu0-stimulated PDS system (Cl−/Fe3+/Cu0/PDS system), the decomposition of tetracycline was greatly increased within 8 min. In the Cl−/Fe3+/Cu0/PDS system, Cl− limited the disproportionation reaction of Cu+ by promoting Cu0 and Cu2+ reaction with Cl− and increased Cu+ utilization rate. Fe3+ promoted the recycling of Fe2+/Fe3+ and contributed to reducing the invalid oxidation of Cu+ by O2. Sulfate radical, reactive chlorine species and hydroxyl radical were generated in the Cl−/Fe3+/Cu0/PDS system. NO3 − and SO4 2− had no influence on decomposing tetracycline in the Cl−/Fe3+/Cu0/PDS system, but humic acid inhibited tetracycline decomposition. Moreover, the Cl−/Fe3+/Cu0/PDS system had great performance on the experimental water samples with the removal rate of tetracycline was higher than 80%. Furthermore, when the final solution pH was adjusted to 8.0, only 0.88 mg/L total dissolved copper remained after precipitation and filtering.
abstract_unstemmed	The Cu0-stimulated PDS system, which produces reactive oxygen species (ROS) to decompose environmental pollutants, has been widely studied. Although Cu+ is produced in the Cu0-stimulated PDS system, its susceptibility to disproportionate and easy oxidized by O2 must be considered. To improve the utilization of Cu+, Cl− and Fe3+ were considered for strengthening the Cu0-stimulated PDS process. With the addition of Cl− and Fe3+ in the Cu0-stimulated PDS system (Cl−/Fe3+/Cu0/PDS system), the decomposition of tetracycline was greatly increased within 8 min. In the Cl−/Fe3+/Cu0/PDS system, Cl− limited the disproportionation reaction of Cu+ by promoting Cu0 and Cu2+ reaction with Cl− and increased Cu+ utilization rate. Fe3+ promoted the recycling of Fe2+/Fe3+ and contributed to reducing the invalid oxidation of Cu+ by O2. Sulfate radical, reactive chlorine species and hydroxyl radical were generated in the Cl−/Fe3+/Cu0/PDS system. NO3 − and SO4 2− had no influence on decomposing tetracycline in the Cl−/Fe3+/Cu0/PDS system, but humic acid inhibited tetracycline decomposition. Moreover, the Cl−/Fe3+/Cu0/PDS system had great performance on the experimental water samples with the removal rate of tetracycline was higher than 80%. Furthermore, when the final solution pH was adjusted to 8.0, only 0.88 mg/L total dissolved copper remained after precipitation and filtering.
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title_short	Chloride ion with ferric ion in boosting zero-valent copper activated peroxydisulfate for efficiently removing tetracycline
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author2	Zhu, Pengfei Yang, Zhuoyu Liu, Xin Wu, Ruoxi Hou, Baolin
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up_date	2024-07-06T17:33:45.663Z
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Chloride ion with ferric ion in boosting zero-valent copper activated peroxydisulfate for efficiently removing tetracycline

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