Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation

Nonlinear optical (NLO) crystals are an essential support for laser applications, as they could extend the tunable range of all-solid-state lasers. NLO inorganic sulfates always exhibit a large band gap and a moderate second harmonic generation response, which should be a rich source of NLO material...
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Autor*in:	Shang, Yanran [verfasserIn] Xu, Junxin [verfasserIn] Sha, Hongyuan [verfasserIn] Wang, Zujian [verfasserIn] He, Chao [verfasserIn] Su, Rongbing [verfasserIn] Yang, Xiaoming [verfasserIn] Long, Xifa [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Nonlinear optical materials Inorganic sulfate Phase matching ability Birefringence phase matching Quasi-phase matching

Übergeordnetes Werk:	Enthalten in: Coordination chemistry reviews - Amsterdam [u.a.] : Elsevier Science, 1966, 494
Übergeordnetes Werk:	volume:494

DOI / URN:	10.1016/j.ccr.2023.215345

Katalog-ID:	ELV062105094

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245	1	0	\|a Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation
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520			\|a Nonlinear optical (NLO) crystals are an essential support for laser applications, as they could extend the tunable range of all-solid-state lasers. NLO inorganic sulfates always exhibit a large band gap and a moderate second harmonic generation response, which should be a rich source of NLO materials. However, due to the high symmetry of the [SO4] tetrahedron, most of the inorganic sulfates present insufficient phase matching ability, the improvement of which will bring the rapid advance of NLO materials. Therefore, in this review, the development of NLO inorganic sulfates is briefly discussed and the structures with a good phase matching ability are carefully investigated. On the basis of the structure–property relationships, four design strategies to improve their phase matching ability are summarized, including (1) the combination of the planar group; (2) the cooperation of highly polarized cations; (3) the synergy of multiple functional motifs such as [IO3] triangular pyramids and highly polarized cations; (4) the development of polar structures with ferroelectricity. All these strategies effectively improve the phase matching ability of sulfates, while most of them also bring the reduction of the band gap. In order to give full play of the large band gap of sulfates and develop deep-ultraviolet NLO inorganic sulfates, we propose that much attention should be paid to the combination of the planar group based on the birefringence phase matching and the polar structures with ferroelectricity based on the quasi-phase matching. Finally, we hope that this review could provide some inspiration for the design of NLO crystals.
650		4	\|a Nonlinear optical materials
650		4	\|a Inorganic sulfate
650		4	\|a Phase matching ability
650		4	\|a Birefringence phase matching
650		4	\|a Quasi-phase matching
700	1		\|a Xu, Junxin \|e verfasserin \|4 aut
700	1		\|a Sha, Hongyuan \|e verfasserin \|4 aut
700	1		\|a Wang, Zujian \|e verfasserin \|4 aut
700	1		\|a He, Chao \|e verfasserin \|4 aut
700	1		\|a Su, Rongbing \|e verfasserin \|4 aut
700	1		\|a Yang, Xiaoming \|e verfasserin \|0 (orcid)0000-0001-5733-7622 \|4 aut
700	1		\|a Long, Xifa \|e verfasserin \|4 aut
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Indexfelder

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publishDate	2023
allfields	10.1016/j.ccr.2023.215345 doi (DE-627)ELV062105094 (ELSEVIER)S0010-8545(23)00334-X DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Shang, Yanran verfasserin aut Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Nonlinear optical (NLO) crystals are an essential support for laser applications, as they could extend the tunable range of all-solid-state lasers. NLO inorganic sulfates always exhibit a large band gap and a moderate second harmonic generation response, which should be a rich source of NLO materials. However, due to the high symmetry of the [SO4] tetrahedron, most of the inorganic sulfates present insufficient phase matching ability, the improvement of which will bring the rapid advance of NLO materials. Therefore, in this review, the development of NLO inorganic sulfates is briefly discussed and the structures with a good phase matching ability are carefully investigated. On the basis of the structure–property relationships, four design strategies to improve their phase matching ability are summarized, including (1) the combination of the planar group; (2) the cooperation of highly polarized cations; (3) the synergy of multiple functional motifs such as [IO3] triangular pyramids and highly polarized cations; (4) the development of polar structures with ferroelectricity. All these strategies effectively improve the phase matching ability of sulfates, while most of them also bring the reduction of the band gap. In order to give full play of the large band gap of sulfates and develop deep-ultraviolet NLO inorganic sulfates, we propose that much attention should be paid to the combination of the planar group based on the birefringence phase matching and the polar structures with ferroelectricity based on the quasi-phase matching. Finally, we hope that this review could provide some inspiration for the design of NLO crystals. Nonlinear optical materials Inorganic sulfate Phase matching ability Birefringence phase matching Quasi-phase matching Xu, Junxin verfasserin aut Sha, Hongyuan verfasserin aut Wang, Zujian verfasserin aut He, Chao verfasserin aut Su, Rongbing verfasserin aut Yang, Xiaoming verfasserin (orcid)0000-0001-5733-7622 aut Long, Xifa verfasserin aut Enthalten in Coordination chemistry reviews Amsterdam [u.a.] : Elsevier Science, 1966 494 Online-Ressource (DE-627)306655020 (DE-600)1499984-5 (DE-576)081985002 0010-8545 nnns volume:494 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 494
spelling	10.1016/j.ccr.2023.215345 doi (DE-627)ELV062105094 (ELSEVIER)S0010-8545(23)00334-X DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Shang, Yanran verfasserin aut Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Nonlinear optical (NLO) crystals are an essential support for laser applications, as they could extend the tunable range of all-solid-state lasers. NLO inorganic sulfates always exhibit a large band gap and a moderate second harmonic generation response, which should be a rich source of NLO materials. However, due to the high symmetry of the [SO4] tetrahedron, most of the inorganic sulfates present insufficient phase matching ability, the improvement of which will bring the rapid advance of NLO materials. Therefore, in this review, the development of NLO inorganic sulfates is briefly discussed and the structures with a good phase matching ability are carefully investigated. On the basis of the structure–property relationships, four design strategies to improve their phase matching ability are summarized, including (1) the combination of the planar group; (2) the cooperation of highly polarized cations; (3) the synergy of multiple functional motifs such as [IO3] triangular pyramids and highly polarized cations; (4) the development of polar structures with ferroelectricity. All these strategies effectively improve the phase matching ability of sulfates, while most of them also bring the reduction of the band gap. In order to give full play of the large band gap of sulfates and develop deep-ultraviolet NLO inorganic sulfates, we propose that much attention should be paid to the combination of the planar group based on the birefringence phase matching and the polar structures with ferroelectricity based on the quasi-phase matching. Finally, we hope that this review could provide some inspiration for the design of NLO crystals. Nonlinear optical materials Inorganic sulfate Phase matching ability Birefringence phase matching Quasi-phase matching Xu, Junxin verfasserin aut Sha, Hongyuan verfasserin aut Wang, Zujian verfasserin aut He, Chao verfasserin aut Su, Rongbing verfasserin aut Yang, Xiaoming verfasserin (orcid)0000-0001-5733-7622 aut Long, Xifa verfasserin aut Enthalten in Coordination chemistry reviews Amsterdam [u.a.] : Elsevier Science, 1966 494 Online-Ressource (DE-627)306655020 (DE-600)1499984-5 (DE-576)081985002 0010-8545 nnns volume:494 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 494
allfields_unstemmed	10.1016/j.ccr.2023.215345 doi (DE-627)ELV062105094 (ELSEVIER)S0010-8545(23)00334-X DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Shang, Yanran verfasserin aut Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Nonlinear optical (NLO) crystals are an essential support for laser applications, as they could extend the tunable range of all-solid-state lasers. NLO inorganic sulfates always exhibit a large band gap and a moderate second harmonic generation response, which should be a rich source of NLO materials. However, due to the high symmetry of the [SO4] tetrahedron, most of the inorganic sulfates present insufficient phase matching ability, the improvement of which will bring the rapid advance of NLO materials. Therefore, in this review, the development of NLO inorganic sulfates is briefly discussed and the structures with a good phase matching ability are carefully investigated. On the basis of the structure–property relationships, four design strategies to improve their phase matching ability are summarized, including (1) the combination of the planar group; (2) the cooperation of highly polarized cations; (3) the synergy of multiple functional motifs such as [IO3] triangular pyramids and highly polarized cations; (4) the development of polar structures with ferroelectricity. All these strategies effectively improve the phase matching ability of sulfates, while most of them also bring the reduction of the band gap. In order to give full play of the large band gap of sulfates and develop deep-ultraviolet NLO inorganic sulfates, we propose that much attention should be paid to the combination of the planar group based on the birefringence phase matching and the polar structures with ferroelectricity based on the quasi-phase matching. Finally, we hope that this review could provide some inspiration for the design of NLO crystals. Nonlinear optical materials Inorganic sulfate Phase matching ability Birefringence phase matching Quasi-phase matching Xu, Junxin verfasserin aut Sha, Hongyuan verfasserin aut Wang, Zujian verfasserin aut He, Chao verfasserin aut Su, Rongbing verfasserin aut Yang, Xiaoming verfasserin (orcid)0000-0001-5733-7622 aut Long, Xifa verfasserin aut Enthalten in Coordination chemistry reviews Amsterdam [u.a.] : Elsevier Science, 1966 494 Online-Ressource (DE-627)306655020 (DE-600)1499984-5 (DE-576)081985002 0010-8545 nnns volume:494 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 494
allfieldsGer	10.1016/j.ccr.2023.215345 doi (DE-627)ELV062105094 (ELSEVIER)S0010-8545(23)00334-X DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Shang, Yanran verfasserin aut Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Nonlinear optical (NLO) crystals are an essential support for laser applications, as they could extend the tunable range of all-solid-state lasers. NLO inorganic sulfates always exhibit a large band gap and a moderate second harmonic generation response, which should be a rich source of NLO materials. However, due to the high symmetry of the [SO4] tetrahedron, most of the inorganic sulfates present insufficient phase matching ability, the improvement of which will bring the rapid advance of NLO materials. Therefore, in this review, the development of NLO inorganic sulfates is briefly discussed and the structures with a good phase matching ability are carefully investigated. On the basis of the structure–property relationships, four design strategies to improve their phase matching ability are summarized, including (1) the combination of the planar group; (2) the cooperation of highly polarized cations; (3) the synergy of multiple functional motifs such as [IO3] triangular pyramids and highly polarized cations; (4) the development of polar structures with ferroelectricity. All these strategies effectively improve the phase matching ability of sulfates, while most of them also bring the reduction of the band gap. In order to give full play of the large band gap of sulfates and develop deep-ultraviolet NLO inorganic sulfates, we propose that much attention should be paid to the combination of the planar group based on the birefringence phase matching and the polar structures with ferroelectricity based on the quasi-phase matching. Finally, we hope that this review could provide some inspiration for the design of NLO crystals. Nonlinear optical materials Inorganic sulfate Phase matching ability Birefringence phase matching Quasi-phase matching Xu, Junxin verfasserin aut Sha, Hongyuan verfasserin aut Wang, Zujian verfasserin aut He, Chao verfasserin aut Su, Rongbing verfasserin aut Yang, Xiaoming verfasserin (orcid)0000-0001-5733-7622 aut Long, Xifa verfasserin aut Enthalten in Coordination chemistry reviews Amsterdam [u.a.] : Elsevier Science, 1966 494 Online-Ressource (DE-627)306655020 (DE-600)1499984-5 (DE-576)081985002 0010-8545 nnns volume:494 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 494
allfieldsSound	10.1016/j.ccr.2023.215345 doi (DE-627)ELV062105094 (ELSEVIER)S0010-8545(23)00334-X DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Shang, Yanran verfasserin aut Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Nonlinear optical (NLO) crystals are an essential support for laser applications, as they could extend the tunable range of all-solid-state lasers. NLO inorganic sulfates always exhibit a large band gap and a moderate second harmonic generation response, which should be a rich source of NLO materials. However, due to the high symmetry of the [SO4] tetrahedron, most of the inorganic sulfates present insufficient phase matching ability, the improvement of which will bring the rapid advance of NLO materials. Therefore, in this review, the development of NLO inorganic sulfates is briefly discussed and the structures with a good phase matching ability are carefully investigated. On the basis of the structure–property relationships, four design strategies to improve their phase matching ability are summarized, including (1) the combination of the planar group; (2) the cooperation of highly polarized cations; (3) the synergy of multiple functional motifs such as [IO3] triangular pyramids and highly polarized cations; (4) the development of polar structures with ferroelectricity. All these strategies effectively improve the phase matching ability of sulfates, while most of them also bring the reduction of the band gap. In order to give full play of the large band gap of sulfates and develop deep-ultraviolet NLO inorganic sulfates, we propose that much attention should be paid to the combination of the planar group based on the birefringence phase matching and the polar structures with ferroelectricity based on the quasi-phase matching. Finally, we hope that this review could provide some inspiration for the design of NLO crystals. Nonlinear optical materials Inorganic sulfate Phase matching ability Birefringence phase matching Quasi-phase matching Xu, Junxin verfasserin aut Sha, Hongyuan verfasserin aut Wang, Zujian verfasserin aut He, Chao verfasserin aut Su, Rongbing verfasserin aut Yang, Xiaoming verfasserin (orcid)0000-0001-5733-7622 aut Long, Xifa verfasserin aut Enthalten in Coordination chemistry reviews Amsterdam [u.a.] : Elsevier Science, 1966 494 Online-Ressource (DE-627)306655020 (DE-600)1499984-5 (DE-576)081985002 0010-8545 nnns volume:494 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 494
language	English
source	Enthalten in Coordination chemistry reviews 494 volume:494
sourceStr	Enthalten in Coordination chemistry reviews 494 volume:494
format_phy_str_mv	Article
bklname	Chemie: Allgemeines
institution	findex.gbv.de
topic_facet	Nonlinear optical materials Inorganic sulfate Phase matching ability Birefringence phase matching Quasi-phase matching
dewey-raw	540
isfreeaccess_bool	false
container_title	Coordination chemistry reviews
authorswithroles_txt_mv	Shang, Yanran @@aut@@ Xu, Junxin @@aut@@ Sha, Hongyuan @@aut@@ Wang, Zujian @@aut@@ He, Chao @@aut@@ Su, Rongbing @@aut@@ Yang, Xiaoming @@aut@@ Long, Xifa @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	306655020
dewey-sort	3540
id	ELV062105094
language_de	englisch
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author	Shang, Yanran
spellingShingle	Shang, Yanran ddc 540 bkl 35.00 misc Nonlinear optical materials misc Inorganic sulfate misc Phase matching ability misc Birefringence phase matching misc Quasi-phase matching Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation
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topic_title	540 VZ 35.00 bkl Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation Nonlinear optical materials Inorganic sulfate Phase matching ability Birefringence phase matching Quasi-phase matching
topic	ddc 540 bkl 35.00 misc Nonlinear optical materials misc Inorganic sulfate misc Phase matching ability misc Birefringence phase matching misc Quasi-phase matching
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title	Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation
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title_full	Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation
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title_sort	nonlinear optical inorganic sulfates: the improvement of the phase matching ability driven by the structural modulation
title_auth	Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation
abstract	Nonlinear optical (NLO) crystals are an essential support for laser applications, as they could extend the tunable range of all-solid-state lasers. NLO inorganic sulfates always exhibit a large band gap and a moderate second harmonic generation response, which should be a rich source of NLO materials. However, due to the high symmetry of the [SO4] tetrahedron, most of the inorganic sulfates present insufficient phase matching ability, the improvement of which will bring the rapid advance of NLO materials. Therefore, in this review, the development of NLO inorganic sulfates is briefly discussed and the structures with a good phase matching ability are carefully investigated. On the basis of the structure–property relationships, four design strategies to improve their phase matching ability are summarized, including (1) the combination of the planar group; (2) the cooperation of highly polarized cations; (3) the synergy of multiple functional motifs such as [IO3] triangular pyramids and highly polarized cations; (4) the development of polar structures with ferroelectricity. All these strategies effectively improve the phase matching ability of sulfates, while most of them also bring the reduction of the band gap. In order to give full play of the large band gap of sulfates and develop deep-ultraviolet NLO inorganic sulfates, we propose that much attention should be paid to the combination of the planar group based on the birefringence phase matching and the polar structures with ferroelectricity based on the quasi-phase matching. Finally, we hope that this review could provide some inspiration for the design of NLO crystals.
abstractGer	Nonlinear optical (NLO) crystals are an essential support for laser applications, as they could extend the tunable range of all-solid-state lasers. NLO inorganic sulfates always exhibit a large band gap and a moderate second harmonic generation response, which should be a rich source of NLO materials. However, due to the high symmetry of the [SO4] tetrahedron, most of the inorganic sulfates present insufficient phase matching ability, the improvement of which will bring the rapid advance of NLO materials. Therefore, in this review, the development of NLO inorganic sulfates is briefly discussed and the structures with a good phase matching ability are carefully investigated. On the basis of the structure–property relationships, four design strategies to improve their phase matching ability are summarized, including (1) the combination of the planar group; (2) the cooperation of highly polarized cations; (3) the synergy of multiple functional motifs such as [IO3] triangular pyramids and highly polarized cations; (4) the development of polar structures with ferroelectricity. All these strategies effectively improve the phase matching ability of sulfates, while most of them also bring the reduction of the band gap. In order to give full play of the large band gap of sulfates and develop deep-ultraviolet NLO inorganic sulfates, we propose that much attention should be paid to the combination of the planar group based on the birefringence phase matching and the polar structures with ferroelectricity based on the quasi-phase matching. Finally, we hope that this review could provide some inspiration for the design of NLO crystals.
abstract_unstemmed	Nonlinear optical (NLO) crystals are an essential support for laser applications, as they could extend the tunable range of all-solid-state lasers. NLO inorganic sulfates always exhibit a large band gap and a moderate second harmonic generation response, which should be a rich source of NLO materials. However, due to the high symmetry of the [SO4] tetrahedron, most of the inorganic sulfates present insufficient phase matching ability, the improvement of which will bring the rapid advance of NLO materials. Therefore, in this review, the development of NLO inorganic sulfates is briefly discussed and the structures with a good phase matching ability are carefully investigated. On the basis of the structure–property relationships, four design strategies to improve their phase matching ability are summarized, including (1) the combination of the planar group; (2) the cooperation of highly polarized cations; (3) the synergy of multiple functional motifs such as [IO3] triangular pyramids and highly polarized cations; (4) the development of polar structures with ferroelectricity. All these strategies effectively improve the phase matching ability of sulfates, while most of them also bring the reduction of the band gap. In order to give full play of the large band gap of sulfates and develop deep-ultraviolet NLO inorganic sulfates, we propose that much attention should be paid to the combination of the planar group based on the birefringence phase matching and the polar structures with ferroelectricity based on the quasi-phase matching. Finally, we hope that this review could provide some inspiration for the design of NLO crystals.
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title_short	Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation
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All these strategies effectively improve the phase matching ability of sulfates, while most of them also bring the reduction of the band gap. In order to give full play of the large band gap of sulfates and develop deep-ultraviolet NLO inorganic sulfates, we propose that much attention should be paid to the combination of the planar group based on the birefringence phase matching and the polar structures with ferroelectricity based on the quasi-phase matching. 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Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation

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