In situ construction of rich oxygen vacancy Bi/Bi

Oxygen vacancy-rich Bi/Bi3TaO7 binary nanomaterials were obtained by a simple in situ reduction. The as-prepared composite exhibited superior photocatalytic activity for the degradation of RhB compared to the single material under the visible light range. The degradation rate of the optimal sample r...
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Autor*in:	Liu, Yuehui [verfasserIn] Li, Yueyi [verfasserIn] Liu, Xuguang [verfasserIn] Li, Jiaxin [verfasserIn] Feng, Yanjie [verfasserIn] Li, Xia [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Photocatalysis Oxygen vacancy Bi/Bi Bismuth metal Plasma resonance

Übergeordnetes Werk:	Enthalten in: International journal of hydrogen energy - New York, NY [u.a.] : Elsevier, 1976, 48
Übergeordnetes Werk:	volume:48

DOI / URN:	10.1016/j.ijhydene.2023.04.259

Katalog-ID:	ELV062136488

Internformat


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520			\|a Oxygen vacancy-rich Bi/Bi3TaO7 binary nanomaterials were obtained by a simple in situ reduction. The as-prepared composite exhibited superior photocatalytic activity for the degradation of RhB compared to the single material under the visible light range. The degradation rate of the optimal sample reached 92% within 120 min, 12.25 times that of the pure Bi3TaO7. XRD and HRTEM characterization showed that the Bi metal obtained through in situ reduction was loaded on the Bi3TaO7 nanostructure. In addition, XPS and EPR indicated a significant increase in the oxygen vacancy content of the composites. The time-resolved transient fluorescence spectroscopy and photocurrent results proved that the separation rate of photoexcited carriers and the corresponding ability of photoelectrons are greatly increased. It is due to the synergistic effect of the unique photo-reaction excitation pathway induced by bismuth metal plasma resonance and oxygen vacancies, which not only extends the photo-reaction to the infrared region but also increases the carrier residence time, and this is the fundamental reason for the excellent photocatalytic performance of the composite material. The h+ is the main reactive radical of the reaction, and •O2 − also plays a role. Based on the above characterization study, we propose a possible photoreaction mechanism for the synergistic oxygen vacancy and Bi metal of Bi/Bi3TaO7.
650		4	\|a Photocatalysis
650		4	\|a Oxygen vacancy
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700	1		\|a Liu, Xuguang \|e verfasserin \|4 aut
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700	1		\|a Feng, Yanjie \|e verfasserin \|4 aut
700	1		\|a Li, Xia \|e verfasserin \|4 aut
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publishDate	2023
allfields	10.1016/j.ijhydene.2023.04.259 doi (DE-627)ELV062136488 (ELSEVIER)S0360-3199(23)02088-8 DE-627 ger DE-627 rda eng 660 620 VZ 52.56 bkl Liu, Yuehui verfasserin aut In situ construction of rich oxygen vacancy Bi/Bi 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Oxygen vacancy-rich Bi/Bi3TaO7 binary nanomaterials were obtained by a simple in situ reduction. The as-prepared composite exhibited superior photocatalytic activity for the degradation of RhB compared to the single material under the visible light range. The degradation rate of the optimal sample reached 92% within 120 min, 12.25 times that of the pure Bi3TaO7. XRD and HRTEM characterization showed that the Bi metal obtained through in situ reduction was loaded on the Bi3TaO7 nanostructure. In addition, XPS and EPR indicated a significant increase in the oxygen vacancy content of the composites. The time-resolved transient fluorescence spectroscopy and photocurrent results proved that the separation rate of photoexcited carriers and the corresponding ability of photoelectrons are greatly increased. It is due to the synergistic effect of the unique photo-reaction excitation pathway induced by bismuth metal plasma resonance and oxygen vacancies, which not only extends the photo-reaction to the infrared region but also increases the carrier residence time, and this is the fundamental reason for the excellent photocatalytic performance of the composite material. The h+ is the main reactive radical of the reaction, and •O2 − also plays a role. Based on the above characterization study, we propose a possible photoreaction mechanism for the synergistic oxygen vacancy and Bi metal of Bi/Bi3TaO7. Photocatalysis Oxygen vacancy Bi/Bi Bismuth metal Plasma resonance Li, Yueyi verfasserin aut Liu, Xuguang verfasserin aut Li, Jiaxin verfasserin aut Feng, Yanjie verfasserin aut Li, Xia verfasserin aut Enthalten in International journal of hydrogen energy New York, NY [u.a.] : Elsevier, 1976 48 Online-Ressource (DE-627)301511357 (DE-600)1484487-4 (DE-576)096806397 1879-3487 nnns volume:48 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.56 Regenerative Energieformen alternative Energieformen VZ AR 48
spelling	10.1016/j.ijhydene.2023.04.259 doi (DE-627)ELV062136488 (ELSEVIER)S0360-3199(23)02088-8 DE-627 ger DE-627 rda eng 660 620 VZ 52.56 bkl Liu, Yuehui verfasserin aut In situ construction of rich oxygen vacancy Bi/Bi 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Oxygen vacancy-rich Bi/Bi3TaO7 binary nanomaterials were obtained by a simple in situ reduction. The as-prepared composite exhibited superior photocatalytic activity for the degradation of RhB compared to the single material under the visible light range. The degradation rate of the optimal sample reached 92% within 120 min, 12.25 times that of the pure Bi3TaO7. XRD and HRTEM characterization showed that the Bi metal obtained through in situ reduction was loaded on the Bi3TaO7 nanostructure. In addition, XPS and EPR indicated a significant increase in the oxygen vacancy content of the composites. The time-resolved transient fluorescence spectroscopy and photocurrent results proved that the separation rate of photoexcited carriers and the corresponding ability of photoelectrons are greatly increased. It is due to the synergistic effect of the unique photo-reaction excitation pathway induced by bismuth metal plasma resonance and oxygen vacancies, which not only extends the photo-reaction to the infrared region but also increases the carrier residence time, and this is the fundamental reason for the excellent photocatalytic performance of the composite material. The h+ is the main reactive radical of the reaction, and •O2 − also plays a role. Based on the above characterization study, we propose a possible photoreaction mechanism for the synergistic oxygen vacancy and Bi metal of Bi/Bi3TaO7. Photocatalysis Oxygen vacancy Bi/Bi Bismuth metal Plasma resonance Li, Yueyi verfasserin aut Liu, Xuguang verfasserin aut Li, Jiaxin verfasserin aut Feng, Yanjie verfasserin aut Li, Xia verfasserin aut Enthalten in International journal of hydrogen energy New York, NY [u.a.] : Elsevier, 1976 48 Online-Ressource (DE-627)301511357 (DE-600)1484487-4 (DE-576)096806397 1879-3487 nnns volume:48 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.56 Regenerative Energieformen alternative Energieformen VZ AR 48
allfields_unstemmed	10.1016/j.ijhydene.2023.04.259 doi (DE-627)ELV062136488 (ELSEVIER)S0360-3199(23)02088-8 DE-627 ger DE-627 rda eng 660 620 VZ 52.56 bkl Liu, Yuehui verfasserin aut In situ construction of rich oxygen vacancy Bi/Bi 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Oxygen vacancy-rich Bi/Bi3TaO7 binary nanomaterials were obtained by a simple in situ reduction. The as-prepared composite exhibited superior photocatalytic activity for the degradation of RhB compared to the single material under the visible light range. The degradation rate of the optimal sample reached 92% within 120 min, 12.25 times that of the pure Bi3TaO7. XRD and HRTEM characterization showed that the Bi metal obtained through in situ reduction was loaded on the Bi3TaO7 nanostructure. In addition, XPS and EPR indicated a significant increase in the oxygen vacancy content of the composites. The time-resolved transient fluorescence spectroscopy and photocurrent results proved that the separation rate of photoexcited carriers and the corresponding ability of photoelectrons are greatly increased. It is due to the synergistic effect of the unique photo-reaction excitation pathway induced by bismuth metal plasma resonance and oxygen vacancies, which not only extends the photo-reaction to the infrared region but also increases the carrier residence time, and this is the fundamental reason for the excellent photocatalytic performance of the composite material. The h+ is the main reactive radical of the reaction, and •O2 − also plays a role. Based on the above characterization study, we propose a possible photoreaction mechanism for the synergistic oxygen vacancy and Bi metal of Bi/Bi3TaO7. Photocatalysis Oxygen vacancy Bi/Bi Bismuth metal Plasma resonance Li, Yueyi verfasserin aut Liu, Xuguang verfasserin aut Li, Jiaxin verfasserin aut Feng, Yanjie verfasserin aut Li, Xia verfasserin aut Enthalten in International journal of hydrogen energy New York, NY [u.a.] : Elsevier, 1976 48 Online-Ressource (DE-627)301511357 (DE-600)1484487-4 (DE-576)096806397 1879-3487 nnns volume:48 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.56 Regenerative Energieformen alternative Energieformen VZ AR 48
allfieldsGer	10.1016/j.ijhydene.2023.04.259 doi (DE-627)ELV062136488 (ELSEVIER)S0360-3199(23)02088-8 DE-627 ger DE-627 rda eng 660 620 VZ 52.56 bkl Liu, Yuehui verfasserin aut In situ construction of rich oxygen vacancy Bi/Bi 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Oxygen vacancy-rich Bi/Bi3TaO7 binary nanomaterials were obtained by a simple in situ reduction. The as-prepared composite exhibited superior photocatalytic activity for the degradation of RhB compared to the single material under the visible light range. The degradation rate of the optimal sample reached 92% within 120 min, 12.25 times that of the pure Bi3TaO7. XRD and HRTEM characterization showed that the Bi metal obtained through in situ reduction was loaded on the Bi3TaO7 nanostructure. In addition, XPS and EPR indicated a significant increase in the oxygen vacancy content of the composites. The time-resolved transient fluorescence spectroscopy and photocurrent results proved that the separation rate of photoexcited carriers and the corresponding ability of photoelectrons are greatly increased. It is due to the synergistic effect of the unique photo-reaction excitation pathway induced by bismuth metal plasma resonance and oxygen vacancies, which not only extends the photo-reaction to the infrared region but also increases the carrier residence time, and this is the fundamental reason for the excellent photocatalytic performance of the composite material. The h+ is the main reactive radical of the reaction, and •O2 − also plays a role. Based on the above characterization study, we propose a possible photoreaction mechanism for the synergistic oxygen vacancy and Bi metal of Bi/Bi3TaO7. Photocatalysis Oxygen vacancy Bi/Bi Bismuth metal Plasma resonance Li, Yueyi verfasserin aut Liu, Xuguang verfasserin aut Li, Jiaxin verfasserin aut Feng, Yanjie verfasserin aut Li, Xia verfasserin aut Enthalten in International journal of hydrogen energy New York, NY [u.a.] : Elsevier, 1976 48 Online-Ressource (DE-627)301511357 (DE-600)1484487-4 (DE-576)096806397 1879-3487 nnns volume:48 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.56 Regenerative Energieformen alternative Energieformen VZ AR 48
allfieldsSound	10.1016/j.ijhydene.2023.04.259 doi (DE-627)ELV062136488 (ELSEVIER)S0360-3199(23)02088-8 DE-627 ger DE-627 rda eng 660 620 VZ 52.56 bkl Liu, Yuehui verfasserin aut In situ construction of rich oxygen vacancy Bi/Bi 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Oxygen vacancy-rich Bi/Bi3TaO7 binary nanomaterials were obtained by a simple in situ reduction. The as-prepared composite exhibited superior photocatalytic activity for the degradation of RhB compared to the single material under the visible light range. The degradation rate of the optimal sample reached 92% within 120 min, 12.25 times that of the pure Bi3TaO7. XRD and HRTEM characterization showed that the Bi metal obtained through in situ reduction was loaded on the Bi3TaO7 nanostructure. In addition, XPS and EPR indicated a significant increase in the oxygen vacancy content of the composites. The time-resolved transient fluorescence spectroscopy and photocurrent results proved that the separation rate of photoexcited carriers and the corresponding ability of photoelectrons are greatly increased. It is due to the synergistic effect of the unique photo-reaction excitation pathway induced by bismuth metal plasma resonance and oxygen vacancies, which not only extends the photo-reaction to the infrared region but also increases the carrier residence time, and this is the fundamental reason for the excellent photocatalytic performance of the composite material. The h+ is the main reactive radical of the reaction, and •O2 − also plays a role. Based on the above characterization study, we propose a possible photoreaction mechanism for the synergistic oxygen vacancy and Bi metal of Bi/Bi3TaO7. Photocatalysis Oxygen vacancy Bi/Bi Bismuth metal Plasma resonance Li, Yueyi verfasserin aut Liu, Xuguang verfasserin aut Li, Jiaxin verfasserin aut Feng, Yanjie verfasserin aut Li, Xia verfasserin aut Enthalten in International journal of hydrogen energy New York, NY [u.a.] : Elsevier, 1976 48 Online-Ressource (DE-627)301511357 (DE-600)1484487-4 (DE-576)096806397 1879-3487 nnns volume:48 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.56 Regenerative Energieformen alternative Energieformen VZ AR 48
language	English
source	Enthalten in International journal of hydrogen energy 48 volume:48
sourceStr	Enthalten in International journal of hydrogen energy 48 volume:48
format_phy_str_mv	Article
bklname	Regenerative Energieformen alternative Energieformen
institution	findex.gbv.de
topic_facet	Photocatalysis Oxygen vacancy Bi/Bi Bismuth metal Plasma resonance
dewey-raw	660
isfreeaccess_bool	false
container_title	International journal of hydrogen energy
authorswithroles_txt_mv	Liu, Yuehui @@aut@@ Li, Yueyi @@aut@@ Liu, Xuguang @@aut@@ Li, Jiaxin @@aut@@ Feng, Yanjie @@aut@@ Li, Xia @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	301511357
dewey-sort	3660
id	ELV062136488
language_de	englisch
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author	Liu, Yuehui
spellingShingle	Liu, Yuehui ddc 660 bkl 52.56 misc Photocatalysis misc Oxygen vacancy misc Bi/Bi misc Bismuth metal misc Plasma resonance In situ construction of rich oxygen vacancy Bi/Bi
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topic_title	660 620 VZ 52.56 bkl In situ construction of rich oxygen vacancy Bi/Bi Photocatalysis Oxygen vacancy Bi/Bi Bismuth metal Plasma resonance
topic	ddc 660 bkl 52.56 misc Photocatalysis misc Oxygen vacancy misc Bi/Bi misc Bismuth metal misc Plasma resonance
topic_unstemmed	ddc 660 bkl 52.56 misc Photocatalysis misc Oxygen vacancy misc Bi/Bi misc Bismuth metal misc Plasma resonance
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title	In situ construction of rich oxygen vacancy Bi/Bi
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title_full	In situ construction of rich oxygen vacancy Bi/Bi
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author-letter	Liu, Yuehui
doi_str_mv	10.1016/j.ijhydene.2023.04.259
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title_sort	in situ construction of rich oxygen vacancy bi/bi
title_auth	In situ construction of rich oxygen vacancy Bi/Bi
abstract	Oxygen vacancy-rich Bi/Bi3TaO7 binary nanomaterials were obtained by a simple in situ reduction. The as-prepared composite exhibited superior photocatalytic activity for the degradation of RhB compared to the single material under the visible light range. The degradation rate of the optimal sample reached 92% within 120 min, 12.25 times that of the pure Bi3TaO7. XRD and HRTEM characterization showed that the Bi metal obtained through in situ reduction was loaded on the Bi3TaO7 nanostructure. In addition, XPS and EPR indicated a significant increase in the oxygen vacancy content of the composites. The time-resolved transient fluorescence spectroscopy and photocurrent results proved that the separation rate of photoexcited carriers and the corresponding ability of photoelectrons are greatly increased. It is due to the synergistic effect of the unique photo-reaction excitation pathway induced by bismuth metal plasma resonance and oxygen vacancies, which not only extends the photo-reaction to the infrared region but also increases the carrier residence time, and this is the fundamental reason for the excellent photocatalytic performance of the composite material. The h+ is the main reactive radical of the reaction, and •O2 − also plays a role. Based on the above characterization study, we propose a possible photoreaction mechanism for the synergistic oxygen vacancy and Bi metal of Bi/Bi3TaO7.
abstractGer	Oxygen vacancy-rich Bi/Bi3TaO7 binary nanomaterials were obtained by a simple in situ reduction. The as-prepared composite exhibited superior photocatalytic activity for the degradation of RhB compared to the single material under the visible light range. The degradation rate of the optimal sample reached 92% within 120 min, 12.25 times that of the pure Bi3TaO7. XRD and HRTEM characterization showed that the Bi metal obtained through in situ reduction was loaded on the Bi3TaO7 nanostructure. In addition, XPS and EPR indicated a significant increase in the oxygen vacancy content of the composites. The time-resolved transient fluorescence spectroscopy and photocurrent results proved that the separation rate of photoexcited carriers and the corresponding ability of photoelectrons are greatly increased. It is due to the synergistic effect of the unique photo-reaction excitation pathway induced by bismuth metal plasma resonance and oxygen vacancies, which not only extends the photo-reaction to the infrared region but also increases the carrier residence time, and this is the fundamental reason for the excellent photocatalytic performance of the composite material. The h+ is the main reactive radical of the reaction, and •O2 − also plays a role. Based on the above characterization study, we propose a possible photoreaction mechanism for the synergistic oxygen vacancy and Bi metal of Bi/Bi3TaO7.
abstract_unstemmed	Oxygen vacancy-rich Bi/Bi3TaO7 binary nanomaterials were obtained by a simple in situ reduction. The as-prepared composite exhibited superior photocatalytic activity for the degradation of RhB compared to the single material under the visible light range. The degradation rate of the optimal sample reached 92% within 120 min, 12.25 times that of the pure Bi3TaO7. XRD and HRTEM characterization showed that the Bi metal obtained through in situ reduction was loaded on the Bi3TaO7 nanostructure. In addition, XPS and EPR indicated a significant increase in the oxygen vacancy content of the composites. The time-resolved transient fluorescence spectroscopy and photocurrent results proved that the separation rate of photoexcited carriers and the corresponding ability of photoelectrons are greatly increased. It is due to the synergistic effect of the unique photo-reaction excitation pathway induced by bismuth metal plasma resonance and oxygen vacancies, which not only extends the photo-reaction to the infrared region but also increases the carrier residence time, and this is the fundamental reason for the excellent photocatalytic performance of the composite material. The h+ is the main reactive radical of the reaction, and •O2 − also plays a role. Based on the above characterization study, we propose a possible photoreaction mechanism for the synergistic oxygen vacancy and Bi metal of Bi/Bi3TaO7.
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title_short	In situ construction of rich oxygen vacancy Bi/Bi
remote_bool	true
author2	Li, Yueyi Liu, Xuguang Li, Jiaxin Feng, Yanjie Li, Xia
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doi_str	10.1016/j.ijhydene.2023.04.259
up_date	2024-07-06T18:26:53.732Z
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score	7.40075

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In situ construction of rich oxygen vacancy Bi/Bi

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