Phosphate-decorated Ni

Direct seawater splitting technique can produce clean hydrogen energy without a complicated water desalination process. However, the oxygen evolution reaction (OER) confronts with selectivity challenge in competing with chlorine evolution and severe corrosion issues of the electrode. In this work, p...
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Autor*in:	Li, Tianshui [verfasserIn] Zhao, Xiuping [verfasserIn] Getaye Sendeku, Marshet [verfasserIn] Zhang, Xingheng [verfasserIn] Xu, Ling [verfasserIn] Wang, Zhaolei [verfasserIn] Wang, Shiyuan [verfasserIn] Duan, Xinxuan [verfasserIn] Liu, Hai [verfasserIn] Liu, Wei [verfasserIn] Zhou, Daojin [verfasserIn] Xu, Haijun [verfasserIn] Kuang, Yun [verfasserIn] Sun, Xiaoming [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Seawater splitting Near-neutral solutions Oxygen evolution reaction Non-precious metals Phosphate-decorated

Übergeordnetes Werk:	Enthalten in: The chemical engineering journal - Amsterdam : Elsevier, 1997, 460
Übergeordnetes Werk:	volume:460

DOI / URN:	10.1016/j.cej.2023.141413

Katalog-ID:	ELV062643754

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520			\|a Direct seawater splitting technique can produce clean hydrogen energy without a complicated water desalination process. However, the oxygen evolution reaction (OER) confronts with selectivity challenge in competing with chlorine evolution and severe corrosion issues of the electrode. In this work, phosphate-decorated Ni3Fe-layered double hydroxides grown on cobalt phosphide nanoarray with both high intrinsic activity and 100 % selectivity towards seawater oxidation in a near neutral electrolyte is reported. The as-prepared electrode shows a low overpotential of 370 mV10 mA cm−2 with high durability in near-neutral seawater oxidation for 350 h. The phosphate layer on the catalyst surface contributes to the enhanced selectivity by weakening the adsorption of Cl–, and thus avoiding the competing chlorine evolution. Meanwhile, the phosphate layer with a strong proton accepting ability can resist the local pH change on the electrode surface in the neutral electrolyte, affording highly stable seawater splitting for prolonged operations in neutral seawater electrolyte.
650		4	\|a Seawater splitting
650		4	\|a Near-neutral solutions
650		4	\|a Oxygen evolution reaction
650		4	\|a Non-precious metals
650		4	\|a Phosphate-decorated
700	1		\|a Zhao, Xiuping \|e verfasserin \|4 aut
700	1		\|a Getaye Sendeku, Marshet \|e verfasserin \|4 aut
700	1		\|a Zhang, Xingheng \|e verfasserin \|4 aut
700	1		\|a Xu, Ling \|e verfasserin \|4 aut
700	1		\|a Wang, Zhaolei \|e verfasserin \|4 aut
700	1		\|a Wang, Shiyuan \|e verfasserin \|4 aut
700	1		\|a Duan, Xinxuan \|e verfasserin \|4 aut
700	1		\|a Liu, Hai \|e verfasserin \|4 aut
700	1		\|a Liu, Wei \|e verfasserin \|4 aut
700	1		\|a Zhou, Daojin \|e verfasserin \|4 aut
700	1		\|a Xu, Haijun \|e verfasserin \|4 aut
700	1		\|a Kuang, Yun \|e verfasserin \|4 aut
700	1		\|a Sun, Xiaoming \|e verfasserin \|4 aut
773	0	8	\|i Enthalten in \|t The chemical engineering journal \|d Amsterdam : Elsevier, 1997 \|g 460 \|h Online-Ressource \|w (DE-627)320500322 \|w (DE-600)2012137-4 \|w (DE-576)098330152 \|x 1873-3212 \|7 nnns
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912			\|a GBV_ILN_2048
912			\|a GBV_ILN_2049
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912			\|a GBV_ILN_4325
912			\|a GBV_ILN_4326
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912			\|a GBV_ILN_4334
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allfields	10.1016/j.cej.2023.141413 doi (DE-627)ELV062643754 (ELSEVIER)S1385-8947(23)00144-4 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Li, Tianshui verfasserin aut Phosphate-decorated Ni 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Direct seawater splitting technique can produce clean hydrogen energy without a complicated water desalination process. However, the oxygen evolution reaction (OER) confronts with selectivity challenge in competing with chlorine evolution and severe corrosion issues of the electrode. In this work, phosphate-decorated Ni3Fe-layered double hydroxides grown on cobalt phosphide nanoarray with both high intrinsic activity and 100 % selectivity towards seawater oxidation in a near neutral electrolyte is reported. The as-prepared electrode shows a low overpotential of 370 mV10 mA cm−2 with high durability in near-neutral seawater oxidation for 350 h. The phosphate layer on the catalyst surface contributes to the enhanced selectivity by weakening the adsorption of Cl–, and thus avoiding the competing chlorine evolution. Meanwhile, the phosphate layer with a strong proton accepting ability can resist the local pH change on the electrode surface in the neutral electrolyte, affording highly stable seawater splitting for prolonged operations in neutral seawater electrolyte. Seawater splitting Near-neutral solutions Oxygen evolution reaction Non-precious metals Phosphate-decorated Zhao, Xiuping verfasserin aut Getaye Sendeku, Marshet verfasserin aut Zhang, Xingheng verfasserin aut Xu, Ling verfasserin aut Wang, Zhaolei verfasserin aut Wang, Shiyuan verfasserin aut Duan, Xinxuan verfasserin aut Liu, Hai verfasserin aut Liu, Wei verfasserin aut Zhou, Daojin verfasserin aut Xu, Haijun verfasserin aut Kuang, Yun verfasserin aut Sun, Xiaoming verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 460 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:460 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 460
spelling	10.1016/j.cej.2023.141413 doi (DE-627)ELV062643754 (ELSEVIER)S1385-8947(23)00144-4 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Li, Tianshui verfasserin aut Phosphate-decorated Ni 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Direct seawater splitting technique can produce clean hydrogen energy without a complicated water desalination process. However, the oxygen evolution reaction (OER) confronts with selectivity challenge in competing with chlorine evolution and severe corrosion issues of the electrode. In this work, phosphate-decorated Ni3Fe-layered double hydroxides grown on cobalt phosphide nanoarray with both high intrinsic activity and 100 % selectivity towards seawater oxidation in a near neutral electrolyte is reported. The as-prepared electrode shows a low overpotential of 370 mV10 mA cm−2 with high durability in near-neutral seawater oxidation for 350 h. The phosphate layer on the catalyst surface contributes to the enhanced selectivity by weakening the adsorption of Cl–, and thus avoiding the competing chlorine evolution. Meanwhile, the phosphate layer with a strong proton accepting ability can resist the local pH change on the electrode surface in the neutral electrolyte, affording highly stable seawater splitting for prolonged operations in neutral seawater electrolyte. Seawater splitting Near-neutral solutions Oxygen evolution reaction Non-precious metals Phosphate-decorated Zhao, Xiuping verfasserin aut Getaye Sendeku, Marshet verfasserin aut Zhang, Xingheng verfasserin aut Xu, Ling verfasserin aut Wang, Zhaolei verfasserin aut Wang, Shiyuan verfasserin aut Duan, Xinxuan verfasserin aut Liu, Hai verfasserin aut Liu, Wei verfasserin aut Zhou, Daojin verfasserin aut Xu, Haijun verfasserin aut Kuang, Yun verfasserin aut Sun, Xiaoming verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 460 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:460 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 460
allfields_unstemmed	10.1016/j.cej.2023.141413 doi (DE-627)ELV062643754 (ELSEVIER)S1385-8947(23)00144-4 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Li, Tianshui verfasserin aut Phosphate-decorated Ni 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Direct seawater splitting technique can produce clean hydrogen energy without a complicated water desalination process. However, the oxygen evolution reaction (OER) confronts with selectivity challenge in competing with chlorine evolution and severe corrosion issues of the electrode. In this work, phosphate-decorated Ni3Fe-layered double hydroxides grown on cobalt phosphide nanoarray with both high intrinsic activity and 100 % selectivity towards seawater oxidation in a near neutral electrolyte is reported. The as-prepared electrode shows a low overpotential of 370 mV10 mA cm−2 with high durability in near-neutral seawater oxidation for 350 h. The phosphate layer on the catalyst surface contributes to the enhanced selectivity by weakening the adsorption of Cl–, and thus avoiding the competing chlorine evolution. Meanwhile, the phosphate layer with a strong proton accepting ability can resist the local pH change on the electrode surface in the neutral electrolyte, affording highly stable seawater splitting for prolonged operations in neutral seawater electrolyte. Seawater splitting Near-neutral solutions Oxygen evolution reaction Non-precious metals Phosphate-decorated Zhao, Xiuping verfasserin aut Getaye Sendeku, Marshet verfasserin aut Zhang, Xingheng verfasserin aut Xu, Ling verfasserin aut Wang, Zhaolei verfasserin aut Wang, Shiyuan verfasserin aut Duan, Xinxuan verfasserin aut Liu, Hai verfasserin aut Liu, Wei verfasserin aut Zhou, Daojin verfasserin aut Xu, Haijun verfasserin aut Kuang, Yun verfasserin aut Sun, Xiaoming verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 460 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:460 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 460
allfieldsGer	10.1016/j.cej.2023.141413 doi (DE-627)ELV062643754 (ELSEVIER)S1385-8947(23)00144-4 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Li, Tianshui verfasserin aut Phosphate-decorated Ni 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Direct seawater splitting technique can produce clean hydrogen energy without a complicated water desalination process. However, the oxygen evolution reaction (OER) confronts with selectivity challenge in competing with chlorine evolution and severe corrosion issues of the electrode. In this work, phosphate-decorated Ni3Fe-layered double hydroxides grown on cobalt phosphide nanoarray with both high intrinsic activity and 100 % selectivity towards seawater oxidation in a near neutral electrolyte is reported. The as-prepared electrode shows a low overpotential of 370 mV10 mA cm−2 with high durability in near-neutral seawater oxidation for 350 h. The phosphate layer on the catalyst surface contributes to the enhanced selectivity by weakening the adsorption of Cl–, and thus avoiding the competing chlorine evolution. Meanwhile, the phosphate layer with a strong proton accepting ability can resist the local pH change on the electrode surface in the neutral electrolyte, affording highly stable seawater splitting for prolonged operations in neutral seawater electrolyte. Seawater splitting Near-neutral solutions Oxygen evolution reaction Non-precious metals Phosphate-decorated Zhao, Xiuping verfasserin aut Getaye Sendeku, Marshet verfasserin aut Zhang, Xingheng verfasserin aut Xu, Ling verfasserin aut Wang, Zhaolei verfasserin aut Wang, Shiyuan verfasserin aut Duan, Xinxuan verfasserin aut Liu, Hai verfasserin aut Liu, Wei verfasserin aut Zhou, Daojin verfasserin aut Xu, Haijun verfasserin aut Kuang, Yun verfasserin aut Sun, Xiaoming verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 460 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:460 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 460
allfieldsSound	10.1016/j.cej.2023.141413 doi (DE-627)ELV062643754 (ELSEVIER)S1385-8947(23)00144-4 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Li, Tianshui verfasserin aut Phosphate-decorated Ni 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Direct seawater splitting technique can produce clean hydrogen energy without a complicated water desalination process. However, the oxygen evolution reaction (OER) confronts with selectivity challenge in competing with chlorine evolution and severe corrosion issues of the electrode. In this work, phosphate-decorated Ni3Fe-layered double hydroxides grown on cobalt phosphide nanoarray with both high intrinsic activity and 100 % selectivity towards seawater oxidation in a near neutral electrolyte is reported. The as-prepared electrode shows a low overpotential of 370 mV10 mA cm−2 with high durability in near-neutral seawater oxidation for 350 h. The phosphate layer on the catalyst surface contributes to the enhanced selectivity by weakening the adsorption of Cl–, and thus avoiding the competing chlorine evolution. Meanwhile, the phosphate layer with a strong proton accepting ability can resist the local pH change on the electrode surface in the neutral electrolyte, affording highly stable seawater splitting for prolonged operations in neutral seawater electrolyte. Seawater splitting Near-neutral solutions Oxygen evolution reaction Non-precious metals Phosphate-decorated Zhao, Xiuping verfasserin aut Getaye Sendeku, Marshet verfasserin aut Zhang, Xingheng verfasserin aut Xu, Ling verfasserin aut Wang, Zhaolei verfasserin aut Wang, Shiyuan verfasserin aut Duan, Xinxuan verfasserin aut Liu, Hai verfasserin aut Liu, Wei verfasserin aut Zhou, Daojin verfasserin aut Xu, Haijun verfasserin aut Kuang, Yun verfasserin aut Sun, Xiaoming verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 460 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:460 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 460
language	English
source	Enthalten in The chemical engineering journal 460 volume:460
sourceStr	Enthalten in The chemical engineering journal 460 volume:460
format_phy_str_mv	Article
bklname	Verfahrenstechnik: Allgemeines
institution	findex.gbv.de
topic_facet	Seawater splitting Near-neutral solutions Oxygen evolution reaction Non-precious metals Phosphate-decorated
dewey-raw	660
isfreeaccess_bool	false
container_title	The chemical engineering journal
authorswithroles_txt_mv	Li, Tianshui @@aut@@ Zhao, Xiuping @@aut@@ Getaye Sendeku, Marshet @@aut@@ Zhang, Xingheng @@aut@@ Xu, Ling @@aut@@ Wang, Zhaolei @@aut@@ Wang, Shiyuan @@aut@@ Duan, Xinxuan @@aut@@ Liu, Hai @@aut@@ Liu, Wei @@aut@@ Zhou, Daojin @@aut@@ Xu, Haijun @@aut@@ Kuang, Yun @@aut@@ Sun, Xiaoming @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	320500322
dewey-sort	3660
id	ELV062643754
language_de	englisch
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author	Li, Tianshui
spellingShingle	Li, Tianshui ddc 660 bkl 58.10 misc Seawater splitting misc Near-neutral solutions misc Oxygen evolution reaction misc Non-precious metals misc Phosphate-decorated Phosphate-decorated Ni
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topic_title	660 VZ 58.10 bkl Phosphate-decorated Ni Seawater splitting Near-neutral solutions Oxygen evolution reaction Non-precious metals Phosphate-decorated
topic	ddc 660 bkl 58.10 misc Seawater splitting misc Near-neutral solutions misc Oxygen evolution reaction misc Non-precious metals misc Phosphate-decorated
topic_unstemmed	ddc 660 bkl 58.10 misc Seawater splitting misc Near-neutral solutions misc Oxygen evolution reaction misc Non-precious metals misc Phosphate-decorated
topic_browse	ddc 660 bkl 58.10 misc Seawater splitting misc Near-neutral solutions misc Oxygen evolution reaction misc Non-precious metals misc Phosphate-decorated
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title	Phosphate-decorated Ni
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title_full	Phosphate-decorated Ni
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author_browse	Li, Tianshui Zhao, Xiuping Getaye Sendeku, Marshet Zhang, Xingheng Xu, Ling Wang, Zhaolei Wang, Shiyuan Duan, Xinxuan Liu, Hai Liu, Wei Zhou, Daojin Xu, Haijun Kuang, Yun Sun, Xiaoming
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author-letter	Li, Tianshui
doi_str_mv	10.1016/j.cej.2023.141413
dewey-full	660
author2-role	verfasserin
title_sort	phosphate-decorated ni
title_auth	Phosphate-decorated Ni
abstract	Direct seawater splitting technique can produce clean hydrogen energy without a complicated water desalination process. However, the oxygen evolution reaction (OER) confronts with selectivity challenge in competing with chlorine evolution and severe corrosion issues of the electrode. In this work, phosphate-decorated Ni3Fe-layered double hydroxides grown on cobalt phosphide nanoarray with both high intrinsic activity and 100 % selectivity towards seawater oxidation in a near neutral electrolyte is reported. The as-prepared electrode shows a low overpotential of 370 mV10 mA cm−2 with high durability in near-neutral seawater oxidation for 350 h. The phosphate layer on the catalyst surface contributes to the enhanced selectivity by weakening the adsorption of Cl–, and thus avoiding the competing chlorine evolution. Meanwhile, the phosphate layer with a strong proton accepting ability can resist the local pH change on the electrode surface in the neutral electrolyte, affording highly stable seawater splitting for prolonged operations in neutral seawater electrolyte.
abstractGer	Direct seawater splitting technique can produce clean hydrogen energy without a complicated water desalination process. However, the oxygen evolution reaction (OER) confronts with selectivity challenge in competing with chlorine evolution and severe corrosion issues of the electrode. In this work, phosphate-decorated Ni3Fe-layered double hydroxides grown on cobalt phosphide nanoarray with both high intrinsic activity and 100 % selectivity towards seawater oxidation in a near neutral electrolyte is reported. The as-prepared electrode shows a low overpotential of 370 mV10 mA cm−2 with high durability in near-neutral seawater oxidation for 350 h. The phosphate layer on the catalyst surface contributes to the enhanced selectivity by weakening the adsorption of Cl–, and thus avoiding the competing chlorine evolution. Meanwhile, the phosphate layer with a strong proton accepting ability can resist the local pH change on the electrode surface in the neutral electrolyte, affording highly stable seawater splitting for prolonged operations in neutral seawater electrolyte.
abstract_unstemmed	Direct seawater splitting technique can produce clean hydrogen energy without a complicated water desalination process. However, the oxygen evolution reaction (OER) confronts with selectivity challenge in competing with chlorine evolution and severe corrosion issues of the electrode. In this work, phosphate-decorated Ni3Fe-layered double hydroxides grown on cobalt phosphide nanoarray with both high intrinsic activity and 100 % selectivity towards seawater oxidation in a near neutral electrolyte is reported. The as-prepared electrode shows a low overpotential of 370 mV10 mA cm−2 with high durability in near-neutral seawater oxidation for 350 h. The phosphate layer on the catalyst surface contributes to the enhanced selectivity by weakening the adsorption of Cl–, and thus avoiding the competing chlorine evolution. Meanwhile, the phosphate layer with a strong proton accepting ability can resist the local pH change on the electrode surface in the neutral electrolyte, affording highly stable seawater splitting for prolonged operations in neutral seawater electrolyte.
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title_short	Phosphate-decorated Ni
remote_bool	true
author2	Zhao, Xiuping Getaye Sendeku, Marshet Zhang, Xingheng Xu, Ling Wang, Zhaolei Wang, Shiyuan Duan, Xinxuan Liu, Hai Liu, Wei Zhou, Daojin Xu, Haijun Kuang, Yun Sun, Xiaoming
author2Str	Zhao, Xiuping Getaye Sendeku, Marshet Zhang, Xingheng Xu, Ling Wang, Zhaolei Wang, Shiyuan Duan, Xinxuan Liu, Hai Liu, Wei Zhou, Daojin Xu, Haijun Kuang, Yun Sun, Xiaoming
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doi_str	10.1016/j.cej.2023.141413
up_date	2024-07-06T19:01:49.220Z
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