Long-cycling and high-loading lithium-sulfur battery enabled by free-standing three-dimensional porous NiCo 2 O 4 nanosheets
The lithium-sulfur (Li-S) battery is a promising electrochemical energy storage system with ultrahigh theoretical energy density and abundant raw material, however, issues of “shuttle effect”, low sulfur utilization and dendrite of lithium anode restrict its wide applications. Herein, hierarchical p...
Ausführliche Beschreibung
Autor*in: |
Tian, Xiaohui [verfasserIn] Cheng, Yunnian [verfasserIn] Zhou, Yingke [verfasserIn] Zhang, Bingyin [verfasserIn] Wang, Guiru [verfasserIn] |
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E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2023 |
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Schlagwörter: |
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Übergeordnetes Werk: |
Enthalten in: Applied energy - Amsterdam [u.a.] : Elsevier Science, 1975, 334 |
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Übergeordnetes Werk: |
volume:334 |
DOI / URN: |
10.1016/j.apenergy.2023.120694 |
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Katalog-ID: |
ELV06274741X |
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520 | |a The lithium-sulfur (Li-S) battery is a promising electrochemical energy storage system with ultrahigh theoretical energy density and abundant raw material, however, issues of “shuttle effect”, low sulfur utilization and dendrite of lithium anode restrict its wide applications. Herein, hierarchical porous NiCo2O4 nanosheets anchored on carbon cloth framework (NCO-CC) have been prepared and applied as highly efficient sulfur host for Li-S battery. NiCo2O4 nanosheets are composed of interconnected nanoparticles and mesopores of about 300–600 nm. The porous NCO-CC can offer adequate space to increase sulfur loading and relieve the volumetric change during charge/discharge processes, and provide strong chemisorption for trapping lithium polysulfides, to effectively increase utilization and redox kinetics. The three-dimensional conductive carbon cloth substrate can be directly used as current collector, and the free-standing cathode without any carbon black and binder displays high specific capacities of 1275.1 and 732.1 mAh/g at respectively 0.1 and 5 C, and a low capacity decay rate (∼0.022 %/cycle) over 1500 cycles at 2 C. The novel porous NiCo2O4 nanosheet based sulfur cathode is promising to construct highly efficient and long cycling Li-S battery, and the rational design of flexible CC based hierarchical porous composites might be extended for various applications of energy and catalysis. | ||
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700 | 1 | |a Cheng, Yunnian |e verfasserin |4 aut | |
700 | 1 | |a Zhou, Yingke |e verfasserin |0 (orcid)0000-0002-6310-8831 |4 aut | |
700 | 1 | |a Zhang, Bingyin |e verfasserin |4 aut | |
700 | 1 | |a Wang, Guiru |e verfasserin |4 aut | |
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10.1016/j.apenergy.2023.120694 doi (DE-627)ELV06274741X (ELSEVIER)S0306-2619(23)00058-2 DE-627 ger DE-627 rda eng 620 VZ 52.50 bkl Tian, Xiaohui verfasserin aut Long-cycling and high-loading lithium-sulfur battery enabled by free-standing three-dimensional porous NiCo 2 O 4 nanosheets 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The lithium-sulfur (Li-S) battery is a promising electrochemical energy storage system with ultrahigh theoretical energy density and abundant raw material, however, issues of “shuttle effect”, low sulfur utilization and dendrite of lithium anode restrict its wide applications. Herein, hierarchical porous NiCo2O4 nanosheets anchored on carbon cloth framework (NCO-CC) have been prepared and applied as highly efficient sulfur host for Li-S battery. NiCo2O4 nanosheets are composed of interconnected nanoparticles and mesopores of about 300–600 nm. The porous NCO-CC can offer adequate space to increase sulfur loading and relieve the volumetric change during charge/discharge processes, and provide strong chemisorption for trapping lithium polysulfides, to effectively increase utilization and redox kinetics. The three-dimensional conductive carbon cloth substrate can be directly used as current collector, and the free-standing cathode without any carbon black and binder displays high specific capacities of 1275.1 and 732.1 mAh/g at respectively 0.1 and 5 C, and a low capacity decay rate (∼0.022 %/cycle) over 1500 cycles at 2 C. The novel porous NiCo2O4 nanosheet based sulfur cathode is promising to construct highly efficient and long cycling Li-S battery, and the rational design of flexible CC based hierarchical porous composites might be extended for various applications of energy and catalysis. Hierarchical porous architecture Polar NiCo High sulfur loading Free-standing cathode Lithium-sulfur battery Cheng, Yunnian verfasserin aut Zhou, Yingke verfasserin (orcid)0000-0002-6310-8831 aut Zhang, Bingyin verfasserin aut Wang, Guiru verfasserin aut Enthalten in Applied energy Amsterdam [u.a.] : Elsevier Science, 1975 334 Online-Ressource (DE-627)320406709 (DE-600)2000772-3 (DE-576)256140251 1872-9118 nnns volume:334 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.50 Energietechnik: Allgemeines VZ AR 334 |
spelling |
10.1016/j.apenergy.2023.120694 doi (DE-627)ELV06274741X (ELSEVIER)S0306-2619(23)00058-2 DE-627 ger DE-627 rda eng 620 VZ 52.50 bkl Tian, Xiaohui verfasserin aut Long-cycling and high-loading lithium-sulfur battery enabled by free-standing three-dimensional porous NiCo 2 O 4 nanosheets 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The lithium-sulfur (Li-S) battery is a promising electrochemical energy storage system with ultrahigh theoretical energy density and abundant raw material, however, issues of “shuttle effect”, low sulfur utilization and dendrite of lithium anode restrict its wide applications. Herein, hierarchical porous NiCo2O4 nanosheets anchored on carbon cloth framework (NCO-CC) have been prepared and applied as highly efficient sulfur host for Li-S battery. NiCo2O4 nanosheets are composed of interconnected nanoparticles and mesopores of about 300–600 nm. The porous NCO-CC can offer adequate space to increase sulfur loading and relieve the volumetric change during charge/discharge processes, and provide strong chemisorption for trapping lithium polysulfides, to effectively increase utilization and redox kinetics. The three-dimensional conductive carbon cloth substrate can be directly used as current collector, and the free-standing cathode without any carbon black and binder displays high specific capacities of 1275.1 and 732.1 mAh/g at respectively 0.1 and 5 C, and a low capacity decay rate (∼0.022 %/cycle) over 1500 cycles at 2 C. The novel porous NiCo2O4 nanosheet based sulfur cathode is promising to construct highly efficient and long cycling Li-S battery, and the rational design of flexible CC based hierarchical porous composites might be extended for various applications of energy and catalysis. Hierarchical porous architecture Polar NiCo High sulfur loading Free-standing cathode Lithium-sulfur battery Cheng, Yunnian verfasserin aut Zhou, Yingke verfasserin (orcid)0000-0002-6310-8831 aut Zhang, Bingyin verfasserin aut Wang, Guiru verfasserin aut Enthalten in Applied energy Amsterdam [u.a.] : Elsevier Science, 1975 334 Online-Ressource (DE-627)320406709 (DE-600)2000772-3 (DE-576)256140251 1872-9118 nnns volume:334 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.50 Energietechnik: Allgemeines VZ AR 334 |
allfields_unstemmed |
10.1016/j.apenergy.2023.120694 doi (DE-627)ELV06274741X (ELSEVIER)S0306-2619(23)00058-2 DE-627 ger DE-627 rda eng 620 VZ 52.50 bkl Tian, Xiaohui verfasserin aut Long-cycling and high-loading lithium-sulfur battery enabled by free-standing three-dimensional porous NiCo 2 O 4 nanosheets 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The lithium-sulfur (Li-S) battery is a promising electrochemical energy storage system with ultrahigh theoretical energy density and abundant raw material, however, issues of “shuttle effect”, low sulfur utilization and dendrite of lithium anode restrict its wide applications. Herein, hierarchical porous NiCo2O4 nanosheets anchored on carbon cloth framework (NCO-CC) have been prepared and applied as highly efficient sulfur host for Li-S battery. NiCo2O4 nanosheets are composed of interconnected nanoparticles and mesopores of about 300–600 nm. The porous NCO-CC can offer adequate space to increase sulfur loading and relieve the volumetric change during charge/discharge processes, and provide strong chemisorption for trapping lithium polysulfides, to effectively increase utilization and redox kinetics. The three-dimensional conductive carbon cloth substrate can be directly used as current collector, and the free-standing cathode without any carbon black and binder displays high specific capacities of 1275.1 and 732.1 mAh/g at respectively 0.1 and 5 C, and a low capacity decay rate (∼0.022 %/cycle) over 1500 cycles at 2 C. The novel porous NiCo2O4 nanosheet based sulfur cathode is promising to construct highly efficient and long cycling Li-S battery, and the rational design of flexible CC based hierarchical porous composites might be extended for various applications of energy and catalysis. Hierarchical porous architecture Polar NiCo High sulfur loading Free-standing cathode Lithium-sulfur battery Cheng, Yunnian verfasserin aut Zhou, Yingke verfasserin (orcid)0000-0002-6310-8831 aut Zhang, Bingyin verfasserin aut Wang, Guiru verfasserin aut Enthalten in Applied energy Amsterdam [u.a.] : Elsevier Science, 1975 334 Online-Ressource (DE-627)320406709 (DE-600)2000772-3 (DE-576)256140251 1872-9118 nnns volume:334 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.50 Energietechnik: Allgemeines VZ AR 334 |
allfieldsGer |
10.1016/j.apenergy.2023.120694 doi (DE-627)ELV06274741X (ELSEVIER)S0306-2619(23)00058-2 DE-627 ger DE-627 rda eng 620 VZ 52.50 bkl Tian, Xiaohui verfasserin aut Long-cycling and high-loading lithium-sulfur battery enabled by free-standing three-dimensional porous NiCo 2 O 4 nanosheets 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The lithium-sulfur (Li-S) battery is a promising electrochemical energy storage system with ultrahigh theoretical energy density and abundant raw material, however, issues of “shuttle effect”, low sulfur utilization and dendrite of lithium anode restrict its wide applications. Herein, hierarchical porous NiCo2O4 nanosheets anchored on carbon cloth framework (NCO-CC) have been prepared and applied as highly efficient sulfur host for Li-S battery. NiCo2O4 nanosheets are composed of interconnected nanoparticles and mesopores of about 300–600 nm. The porous NCO-CC can offer adequate space to increase sulfur loading and relieve the volumetric change during charge/discharge processes, and provide strong chemisorption for trapping lithium polysulfides, to effectively increase utilization and redox kinetics. The three-dimensional conductive carbon cloth substrate can be directly used as current collector, and the free-standing cathode without any carbon black and binder displays high specific capacities of 1275.1 and 732.1 mAh/g at respectively 0.1 and 5 C, and a low capacity decay rate (∼0.022 %/cycle) over 1500 cycles at 2 C. The novel porous NiCo2O4 nanosheet based sulfur cathode is promising to construct highly efficient and long cycling Li-S battery, and the rational design of flexible CC based hierarchical porous composites might be extended for various applications of energy and catalysis. Hierarchical porous architecture Polar NiCo High sulfur loading Free-standing cathode Lithium-sulfur battery Cheng, Yunnian verfasserin aut Zhou, Yingke verfasserin (orcid)0000-0002-6310-8831 aut Zhang, Bingyin verfasserin aut Wang, Guiru verfasserin aut Enthalten in Applied energy Amsterdam [u.a.] : Elsevier Science, 1975 334 Online-Ressource (DE-627)320406709 (DE-600)2000772-3 (DE-576)256140251 1872-9118 nnns volume:334 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.50 Energietechnik: Allgemeines VZ AR 334 |
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10.1016/j.apenergy.2023.120694 doi (DE-627)ELV06274741X (ELSEVIER)S0306-2619(23)00058-2 DE-627 ger DE-627 rda eng 620 VZ 52.50 bkl Tian, Xiaohui verfasserin aut Long-cycling and high-loading lithium-sulfur battery enabled by free-standing three-dimensional porous NiCo 2 O 4 nanosheets 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The lithium-sulfur (Li-S) battery is a promising electrochemical energy storage system with ultrahigh theoretical energy density and abundant raw material, however, issues of “shuttle effect”, low sulfur utilization and dendrite of lithium anode restrict its wide applications. Herein, hierarchical porous NiCo2O4 nanosheets anchored on carbon cloth framework (NCO-CC) have been prepared and applied as highly efficient sulfur host for Li-S battery. NiCo2O4 nanosheets are composed of interconnected nanoparticles and mesopores of about 300–600 nm. The porous NCO-CC can offer adequate space to increase sulfur loading and relieve the volumetric change during charge/discharge processes, and provide strong chemisorption for trapping lithium polysulfides, to effectively increase utilization and redox kinetics. The three-dimensional conductive carbon cloth substrate can be directly used as current collector, and the free-standing cathode without any carbon black and binder displays high specific capacities of 1275.1 and 732.1 mAh/g at respectively 0.1 and 5 C, and a low capacity decay rate (∼0.022 %/cycle) over 1500 cycles at 2 C. The novel porous NiCo2O4 nanosheet based sulfur cathode is promising to construct highly efficient and long cycling Li-S battery, and the rational design of flexible CC based hierarchical porous composites might be extended for various applications of energy and catalysis. Hierarchical porous architecture Polar NiCo High sulfur loading Free-standing cathode Lithium-sulfur battery Cheng, Yunnian verfasserin aut Zhou, Yingke verfasserin (orcid)0000-0002-6310-8831 aut Zhang, Bingyin verfasserin aut Wang, Guiru verfasserin aut Enthalten in Applied energy Amsterdam [u.a.] : Elsevier Science, 1975 334 Online-Ressource (DE-627)320406709 (DE-600)2000772-3 (DE-576)256140251 1872-9118 nnns volume:334 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.50 Energietechnik: Allgemeines VZ AR 334 |
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Tian, Xiaohui @@aut@@ Cheng, Yunnian @@aut@@ Zhou, Yingke @@aut@@ Zhang, Bingyin @@aut@@ Wang, Guiru @@aut@@ |
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620 VZ 52.50 bkl Long-cycling and high-loading lithium-sulfur battery enabled by free-standing three-dimensional porous NiCo 2 O 4 nanosheets Hierarchical porous architecture Polar NiCo High sulfur loading Free-standing cathode Lithium-sulfur battery |
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ddc 620 bkl 52.50 misc Hierarchical porous architecture misc Polar NiCo misc High sulfur loading misc Free-standing cathode misc Lithium-sulfur battery |
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Long-cycling and high-loading lithium-sulfur battery enabled by free-standing three-dimensional porous NiCo 2 O 4 nanosheets |
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Long-cycling and high-loading lithium-sulfur battery enabled by free-standing three-dimensional porous NiCo 2 O 4 nanosheets |
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Tian, Xiaohui Cheng, Yunnian Zhou, Yingke Zhang, Bingyin Wang, Guiru |
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long-cycling and high-loading lithium-sulfur battery enabled by free-standing three-dimensional porous nico 2 o 4 nanosheets |
title_auth |
Long-cycling and high-loading lithium-sulfur battery enabled by free-standing three-dimensional porous NiCo 2 O 4 nanosheets |
abstract |
The lithium-sulfur (Li-S) battery is a promising electrochemical energy storage system with ultrahigh theoretical energy density and abundant raw material, however, issues of “shuttle effect”, low sulfur utilization and dendrite of lithium anode restrict its wide applications. Herein, hierarchical porous NiCo2O4 nanosheets anchored on carbon cloth framework (NCO-CC) have been prepared and applied as highly efficient sulfur host for Li-S battery. NiCo2O4 nanosheets are composed of interconnected nanoparticles and mesopores of about 300–600 nm. The porous NCO-CC can offer adequate space to increase sulfur loading and relieve the volumetric change during charge/discharge processes, and provide strong chemisorption for trapping lithium polysulfides, to effectively increase utilization and redox kinetics. The three-dimensional conductive carbon cloth substrate can be directly used as current collector, and the free-standing cathode without any carbon black and binder displays high specific capacities of 1275.1 and 732.1 mAh/g at respectively 0.1 and 5 C, and a low capacity decay rate (∼0.022 %/cycle) over 1500 cycles at 2 C. The novel porous NiCo2O4 nanosheet based sulfur cathode is promising to construct highly efficient and long cycling Li-S battery, and the rational design of flexible CC based hierarchical porous composites might be extended for various applications of energy and catalysis. |
abstractGer |
The lithium-sulfur (Li-S) battery is a promising electrochemical energy storage system with ultrahigh theoretical energy density and abundant raw material, however, issues of “shuttle effect”, low sulfur utilization and dendrite of lithium anode restrict its wide applications. Herein, hierarchical porous NiCo2O4 nanosheets anchored on carbon cloth framework (NCO-CC) have been prepared and applied as highly efficient sulfur host for Li-S battery. NiCo2O4 nanosheets are composed of interconnected nanoparticles and mesopores of about 300–600 nm. The porous NCO-CC can offer adequate space to increase sulfur loading and relieve the volumetric change during charge/discharge processes, and provide strong chemisorption for trapping lithium polysulfides, to effectively increase utilization and redox kinetics. The three-dimensional conductive carbon cloth substrate can be directly used as current collector, and the free-standing cathode without any carbon black and binder displays high specific capacities of 1275.1 and 732.1 mAh/g at respectively 0.1 and 5 C, and a low capacity decay rate (∼0.022 %/cycle) over 1500 cycles at 2 C. The novel porous NiCo2O4 nanosheet based sulfur cathode is promising to construct highly efficient and long cycling Li-S battery, and the rational design of flexible CC based hierarchical porous composites might be extended for various applications of energy and catalysis. |
abstract_unstemmed |
The lithium-sulfur (Li-S) battery is a promising electrochemical energy storage system with ultrahigh theoretical energy density and abundant raw material, however, issues of “shuttle effect”, low sulfur utilization and dendrite of lithium anode restrict its wide applications. Herein, hierarchical porous NiCo2O4 nanosheets anchored on carbon cloth framework (NCO-CC) have been prepared and applied as highly efficient sulfur host for Li-S battery. NiCo2O4 nanosheets are composed of interconnected nanoparticles and mesopores of about 300–600 nm. The porous NCO-CC can offer adequate space to increase sulfur loading and relieve the volumetric change during charge/discharge processes, and provide strong chemisorption for trapping lithium polysulfides, to effectively increase utilization and redox kinetics. The three-dimensional conductive carbon cloth substrate can be directly used as current collector, and the free-standing cathode without any carbon black and binder displays high specific capacities of 1275.1 and 732.1 mAh/g at respectively 0.1 and 5 C, and a low capacity decay rate (∼0.022 %/cycle) over 1500 cycles at 2 C. The novel porous NiCo2O4 nanosheet based sulfur cathode is promising to construct highly efficient and long cycling Li-S battery, and the rational design of flexible CC based hierarchical porous composites might be extended for various applications of energy and catalysis. |
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Long-cycling and high-loading lithium-sulfur battery enabled by free-standing three-dimensional porous NiCo 2 O 4 nanosheets |
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