Reduced Fe, Mn-based catalyst with dual reaction sites for rapid decolorization treatment via Fenton-like reactions

Ferromanganese oxides are promising efficient catalysts for peroxymonosulfate (PMS) activation. In this study, a novel porous ferromanganese oxides (FeMnOx) nanocubes derived from prussian blue analogues was prepared via a successive codeposition-calcination method, and the reduced Fe, Mn-based cata...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Su, Yiping [verfasserIn] Long, Yangke [verfasserIn] Zhao, Shiyin [verfasserIn] Wang, Pengju [verfasserIn] Xie, Feng [verfasserIn] Huang, Junyi [verfasserIn] Han, Bing [verfasserIn] Zhang, Zuotai [verfasserIn] Zhang, Bo-Ping [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Ferromanganese oxides Hydrogenation Oxygen vacancies Peroxymonosulfate Decolorization

Übergeordnetes Werk:	Enthalten in: Applied surface science - Amsterdam : Elsevier, 1985, 616
Übergeordnetes Werk:	volume:616

DOI / URN:	10.1016/j.apsusc.2023.156522

Katalog-ID:	ELV063892405

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520			\|a Ferromanganese oxides are promising efficient catalysts for peroxymonosulfate (PMS) activation. In this study, a novel porous ferromanganese oxides (FeMnOx) nanocubes derived from prussian blue analogues was prepared via a successive codeposition-calcination method, and the reduced Fe, Mn-based catalysts were further synthesized by a hydrogenation process. Their catalytic performance was evaluated in a Fenton-like degradation of Rhodamine B (RhB) and other dyes in the presence of PMS. It was found that FeMnOx showed outstanding catalytic activity in dyes elimination, which benefited by the synergetic effect of dual reaction sites, reductive Fe-Mn binary oxides and oxygen vacancies (OVs) for PMS activation. The optimized sample (H2 annealed at 260 °C, FMO-260) exhibited high degradation efficiency to RhB within 5 cycles and after regeneration, implying the strong stability and reusability. Moreover, the influences of PMS and FMO-260 dosages, pH values, coexist anions for the degradation efficiency to RhB were also carried out. According to inhibitor experiments and EPR (electron paramagnetic resonance) tests, a possible catalytic mechanism and degradation pathway of RhB was proposed. This study provides a novel fabrication strategy to design Fe, Mn-based catalysts and demonstrates more potential in the decolorization field.
650		4	\|a Ferromanganese oxides
650		4	\|a Hydrogenation
650		4	\|a Oxygen vacancies
650		4	\|a Peroxymonosulfate
650		4	\|a Decolorization
700	1		\|a Long, Yangke \|e verfasserin \|4 aut
700	1		\|a Zhao, Shiyin \|e verfasserin \|4 aut
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700	1		\|a Xie, Feng \|e verfasserin \|0 (orcid)0000-0002-6861-8267 \|4 aut
700	1		\|a Huang, Junyi \|e verfasserin \|4 aut
700	1		\|a Han, Bing \|e verfasserin \|0 (orcid)0000-0001-8143-3964 \|4 aut
700	1		\|a Zhang, Zuotai \|e verfasserin \|4 aut
700	1		\|a Zhang, Bo-Ping \|e verfasserin \|4 aut
773	0	8	\|i Enthalten in \|t Applied surface science \|d Amsterdam : Elsevier, 1985 \|g 616 \|h Online-Ressource \|w (DE-627)312151128 \|w (DE-600)2002520-8 \|w (DE-576)094476985 \|7 nnns
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publishDate	2023
allfields	10.1016/j.apsusc.2023.156522 doi (DE-627)ELV063892405 (ELSEVIER)S0169-4332(23)00198-8 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Su, Yiping verfasserin aut Reduced Fe, Mn-based catalyst with dual reaction sites for rapid decolorization treatment via Fenton-like reactions 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Ferromanganese oxides are promising efficient catalysts for peroxymonosulfate (PMS) activation. In this study, a novel porous ferromanganese oxides (FeMnOx) nanocubes derived from prussian blue analogues was prepared via a successive codeposition-calcination method, and the reduced Fe, Mn-based catalysts were further synthesized by a hydrogenation process. Their catalytic performance was evaluated in a Fenton-like degradation of Rhodamine B (RhB) and other dyes in the presence of PMS. It was found that FeMnOx showed outstanding catalytic activity in dyes elimination, which benefited by the synergetic effect of dual reaction sites, reductive Fe-Mn binary oxides and oxygen vacancies (OVs) for PMS activation. The optimized sample (H2 annealed at 260 °C, FMO-260) exhibited high degradation efficiency to RhB within 5 cycles and after regeneration, implying the strong stability and reusability. Moreover, the influences of PMS and FMO-260 dosages, pH values, coexist anions for the degradation efficiency to RhB were also carried out. According to inhibitor experiments and EPR (electron paramagnetic resonance) tests, a possible catalytic mechanism and degradation pathway of RhB was proposed. This study provides a novel fabrication strategy to design Fe, Mn-based catalysts and demonstrates more potential in the decolorization field. Ferromanganese oxides Hydrogenation Oxygen vacancies Peroxymonosulfate Decolorization Long, Yangke verfasserin aut Zhao, Shiyin verfasserin aut Wang, Pengju verfasserin (orcid)0000-0002-1046-6360 aut Xie, Feng verfasserin (orcid)0000-0002-6861-8267 aut Huang, Junyi verfasserin aut Han, Bing verfasserin (orcid)0000-0001-8143-3964 aut Zhang, Zuotai verfasserin aut Zhang, Bo-Ping verfasserin aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 616 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:616 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 616
spelling	10.1016/j.apsusc.2023.156522 doi (DE-627)ELV063892405 (ELSEVIER)S0169-4332(23)00198-8 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Su, Yiping verfasserin aut Reduced Fe, Mn-based catalyst with dual reaction sites for rapid decolorization treatment via Fenton-like reactions 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Ferromanganese oxides are promising efficient catalysts for peroxymonosulfate (PMS) activation. In this study, a novel porous ferromanganese oxides (FeMnOx) nanocubes derived from prussian blue analogues was prepared via a successive codeposition-calcination method, and the reduced Fe, Mn-based catalysts were further synthesized by a hydrogenation process. Their catalytic performance was evaluated in a Fenton-like degradation of Rhodamine B (RhB) and other dyes in the presence of PMS. It was found that FeMnOx showed outstanding catalytic activity in dyes elimination, which benefited by the synergetic effect of dual reaction sites, reductive Fe-Mn binary oxides and oxygen vacancies (OVs) for PMS activation. The optimized sample (H2 annealed at 260 °C, FMO-260) exhibited high degradation efficiency to RhB within 5 cycles and after regeneration, implying the strong stability and reusability. Moreover, the influences of PMS and FMO-260 dosages, pH values, coexist anions for the degradation efficiency to RhB were also carried out. According to inhibitor experiments and EPR (electron paramagnetic resonance) tests, a possible catalytic mechanism and degradation pathway of RhB was proposed. This study provides a novel fabrication strategy to design Fe, Mn-based catalysts and demonstrates more potential in the decolorization field. Ferromanganese oxides Hydrogenation Oxygen vacancies Peroxymonosulfate Decolorization Long, Yangke verfasserin aut Zhao, Shiyin verfasserin aut Wang, Pengju verfasserin (orcid)0000-0002-1046-6360 aut Xie, Feng verfasserin (orcid)0000-0002-6861-8267 aut Huang, Junyi verfasserin aut Han, Bing verfasserin (orcid)0000-0001-8143-3964 aut Zhang, Zuotai verfasserin aut Zhang, Bo-Ping verfasserin aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 616 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:616 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 616
allfields_unstemmed	10.1016/j.apsusc.2023.156522 doi (DE-627)ELV063892405 (ELSEVIER)S0169-4332(23)00198-8 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Su, Yiping verfasserin aut Reduced Fe, Mn-based catalyst with dual reaction sites for rapid decolorization treatment via Fenton-like reactions 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Ferromanganese oxides are promising efficient catalysts for peroxymonosulfate (PMS) activation. In this study, a novel porous ferromanganese oxides (FeMnOx) nanocubes derived from prussian blue analogues was prepared via a successive codeposition-calcination method, and the reduced Fe, Mn-based catalysts were further synthesized by a hydrogenation process. Their catalytic performance was evaluated in a Fenton-like degradation of Rhodamine B (RhB) and other dyes in the presence of PMS. It was found that FeMnOx showed outstanding catalytic activity in dyes elimination, which benefited by the synergetic effect of dual reaction sites, reductive Fe-Mn binary oxides and oxygen vacancies (OVs) for PMS activation. The optimized sample (H2 annealed at 260 °C, FMO-260) exhibited high degradation efficiency to RhB within 5 cycles and after regeneration, implying the strong stability and reusability. Moreover, the influences of PMS and FMO-260 dosages, pH values, coexist anions for the degradation efficiency to RhB were also carried out. According to inhibitor experiments and EPR (electron paramagnetic resonance) tests, a possible catalytic mechanism and degradation pathway of RhB was proposed. This study provides a novel fabrication strategy to design Fe, Mn-based catalysts and demonstrates more potential in the decolorization field. Ferromanganese oxides Hydrogenation Oxygen vacancies Peroxymonosulfate Decolorization Long, Yangke verfasserin aut Zhao, Shiyin verfasserin aut Wang, Pengju verfasserin (orcid)0000-0002-1046-6360 aut Xie, Feng verfasserin (orcid)0000-0002-6861-8267 aut Huang, Junyi verfasserin aut Han, Bing verfasserin (orcid)0000-0001-8143-3964 aut Zhang, Zuotai verfasserin aut Zhang, Bo-Ping verfasserin aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 616 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:616 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 616
allfieldsGer	10.1016/j.apsusc.2023.156522 doi (DE-627)ELV063892405 (ELSEVIER)S0169-4332(23)00198-8 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Su, Yiping verfasserin aut Reduced Fe, Mn-based catalyst with dual reaction sites for rapid decolorization treatment via Fenton-like reactions 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Ferromanganese oxides are promising efficient catalysts for peroxymonosulfate (PMS) activation. In this study, a novel porous ferromanganese oxides (FeMnOx) nanocubes derived from prussian blue analogues was prepared via a successive codeposition-calcination method, and the reduced Fe, Mn-based catalysts were further synthesized by a hydrogenation process. Their catalytic performance was evaluated in a Fenton-like degradation of Rhodamine B (RhB) and other dyes in the presence of PMS. It was found that FeMnOx showed outstanding catalytic activity in dyes elimination, which benefited by the synergetic effect of dual reaction sites, reductive Fe-Mn binary oxides and oxygen vacancies (OVs) for PMS activation. The optimized sample (H2 annealed at 260 °C, FMO-260) exhibited high degradation efficiency to RhB within 5 cycles and after regeneration, implying the strong stability and reusability. Moreover, the influences of PMS and FMO-260 dosages, pH values, coexist anions for the degradation efficiency to RhB were also carried out. According to inhibitor experiments and EPR (electron paramagnetic resonance) tests, a possible catalytic mechanism and degradation pathway of RhB was proposed. This study provides a novel fabrication strategy to design Fe, Mn-based catalysts and demonstrates more potential in the decolorization field. Ferromanganese oxides Hydrogenation Oxygen vacancies Peroxymonosulfate Decolorization Long, Yangke verfasserin aut Zhao, Shiyin verfasserin aut Wang, Pengju verfasserin (orcid)0000-0002-1046-6360 aut Xie, Feng verfasserin (orcid)0000-0002-6861-8267 aut Huang, Junyi verfasserin aut Han, Bing verfasserin (orcid)0000-0001-8143-3964 aut Zhang, Zuotai verfasserin aut Zhang, Bo-Ping verfasserin aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 616 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:616 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 616
allfieldsSound	10.1016/j.apsusc.2023.156522 doi (DE-627)ELV063892405 (ELSEVIER)S0169-4332(23)00198-8 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Su, Yiping verfasserin aut Reduced Fe, Mn-based catalyst with dual reaction sites for rapid decolorization treatment via Fenton-like reactions 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Ferromanganese oxides are promising efficient catalysts for peroxymonosulfate (PMS) activation. In this study, a novel porous ferromanganese oxides (FeMnOx) nanocubes derived from prussian blue analogues was prepared via a successive codeposition-calcination method, and the reduced Fe, Mn-based catalysts were further synthesized by a hydrogenation process. Their catalytic performance was evaluated in a Fenton-like degradation of Rhodamine B (RhB) and other dyes in the presence of PMS. It was found that FeMnOx showed outstanding catalytic activity in dyes elimination, which benefited by the synergetic effect of dual reaction sites, reductive Fe-Mn binary oxides and oxygen vacancies (OVs) for PMS activation. The optimized sample (H2 annealed at 260 °C, FMO-260) exhibited high degradation efficiency to RhB within 5 cycles and after regeneration, implying the strong stability and reusability. Moreover, the influences of PMS and FMO-260 dosages, pH values, coexist anions for the degradation efficiency to RhB were also carried out. According to inhibitor experiments and EPR (electron paramagnetic resonance) tests, a possible catalytic mechanism and degradation pathway of RhB was proposed. This study provides a novel fabrication strategy to design Fe, Mn-based catalysts and demonstrates more potential in the decolorization field. Ferromanganese oxides Hydrogenation Oxygen vacancies Peroxymonosulfate Decolorization Long, Yangke verfasserin aut Zhao, Shiyin verfasserin aut Wang, Pengju verfasserin (orcid)0000-0002-1046-6360 aut Xie, Feng verfasserin (orcid)0000-0002-6861-8267 aut Huang, Junyi verfasserin aut Han, Bing verfasserin (orcid)0000-0001-8143-3964 aut Zhang, Zuotai verfasserin aut Zhang, Bo-Ping verfasserin aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 616 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:616 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 616
language	English
source	Enthalten in Applied surface science 616 volume:616
sourceStr	Enthalten in Applied surface science 616 volume:616
format_phy_str_mv	Article
bklname	Oberflächen Dünne Schichten Grenzflächen Kolloidchemie Grenzflächenchemie Oberflächentechnik Wärmebehandlung
institution	findex.gbv.de
topic_facet	Ferromanganese oxides Hydrogenation Oxygen vacancies Peroxymonosulfate Decolorization
dewey-raw	670
isfreeaccess_bool	false
container_title	Applied surface science
authorswithroles_txt_mv	Su, Yiping @@aut@@ Long, Yangke @@aut@@ Zhao, Shiyin @@aut@@ Wang, Pengju @@aut@@ Xie, Feng @@aut@@ Huang, Junyi @@aut@@ Han, Bing @@aut@@ Zhang, Zuotai @@aut@@ Zhang, Bo-Ping @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	312151128
dewey-sort	3670
id	ELV063892405
language_de	englisch
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author	Su, Yiping
spellingShingle	Su, Yiping ddc 670 bkl 33.68 bkl 35.18 bkl 52.78 misc Ferromanganese oxides misc Hydrogenation misc Oxygen vacancies misc Peroxymonosulfate misc Decolorization Reduced Fe, Mn-based catalyst with dual reaction sites for rapid decolorization treatment via Fenton-like reactions
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topic_title	670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Reduced Fe, Mn-based catalyst with dual reaction sites for rapid decolorization treatment via Fenton-like reactions Ferromanganese oxides Hydrogenation Oxygen vacancies Peroxymonosulfate Decolorization
topic	ddc 670 bkl 33.68 bkl 35.18 bkl 52.78 misc Ferromanganese oxides misc Hydrogenation misc Oxygen vacancies misc Peroxymonosulfate misc Decolorization
topic_unstemmed	ddc 670 bkl 33.68 bkl 35.18 bkl 52.78 misc Ferromanganese oxides misc Hydrogenation misc Oxygen vacancies misc Peroxymonosulfate misc Decolorization
topic_browse	ddc 670 bkl 33.68 bkl 35.18 bkl 52.78 misc Ferromanganese oxides misc Hydrogenation misc Oxygen vacancies misc Peroxymonosulfate misc Decolorization
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title	Reduced Fe, Mn-based catalyst with dual reaction sites for rapid decolorization treatment via Fenton-like reactions
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title_full	Reduced Fe, Mn-based catalyst with dual reaction sites for rapid decolorization treatment via Fenton-like reactions
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author-letter	Su, Yiping
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title_sort	reduced fe, mn-based catalyst with dual reaction sites for rapid decolorization treatment via fenton-like reactions
title_auth	Reduced Fe, Mn-based catalyst with dual reaction sites for rapid decolorization treatment via Fenton-like reactions
abstract	Ferromanganese oxides are promising efficient catalysts for peroxymonosulfate (PMS) activation. In this study, a novel porous ferromanganese oxides (FeMnOx) nanocubes derived from prussian blue analogues was prepared via a successive codeposition-calcination method, and the reduced Fe, Mn-based catalysts were further synthesized by a hydrogenation process. Their catalytic performance was evaluated in a Fenton-like degradation of Rhodamine B (RhB) and other dyes in the presence of PMS. It was found that FeMnOx showed outstanding catalytic activity in dyes elimination, which benefited by the synergetic effect of dual reaction sites, reductive Fe-Mn binary oxides and oxygen vacancies (OVs) for PMS activation. The optimized sample (H2 annealed at 260 °C, FMO-260) exhibited high degradation efficiency to RhB within 5 cycles and after regeneration, implying the strong stability and reusability. Moreover, the influences of PMS and FMO-260 dosages, pH values, coexist anions for the degradation efficiency to RhB were also carried out. According to inhibitor experiments and EPR (electron paramagnetic resonance) tests, a possible catalytic mechanism and degradation pathway of RhB was proposed. This study provides a novel fabrication strategy to design Fe, Mn-based catalysts and demonstrates more potential in the decolorization field.
abstractGer	Ferromanganese oxides are promising efficient catalysts for peroxymonosulfate (PMS) activation. In this study, a novel porous ferromanganese oxides (FeMnOx) nanocubes derived from prussian blue analogues was prepared via a successive codeposition-calcination method, and the reduced Fe, Mn-based catalysts were further synthesized by a hydrogenation process. Their catalytic performance was evaluated in a Fenton-like degradation of Rhodamine B (RhB) and other dyes in the presence of PMS. It was found that FeMnOx showed outstanding catalytic activity in dyes elimination, which benefited by the synergetic effect of dual reaction sites, reductive Fe-Mn binary oxides and oxygen vacancies (OVs) for PMS activation. The optimized sample (H2 annealed at 260 °C, FMO-260) exhibited high degradation efficiency to RhB within 5 cycles and after regeneration, implying the strong stability and reusability. Moreover, the influences of PMS and FMO-260 dosages, pH values, coexist anions for the degradation efficiency to RhB were also carried out. According to inhibitor experiments and EPR (electron paramagnetic resonance) tests, a possible catalytic mechanism and degradation pathway of RhB was proposed. This study provides a novel fabrication strategy to design Fe, Mn-based catalysts and demonstrates more potential in the decolorization field.
abstract_unstemmed	Ferromanganese oxides are promising efficient catalysts for peroxymonosulfate (PMS) activation. In this study, a novel porous ferromanganese oxides (FeMnOx) nanocubes derived from prussian blue analogues was prepared via a successive codeposition-calcination method, and the reduced Fe, Mn-based catalysts were further synthesized by a hydrogenation process. Their catalytic performance was evaluated in a Fenton-like degradation of Rhodamine B (RhB) and other dyes in the presence of PMS. It was found that FeMnOx showed outstanding catalytic activity in dyes elimination, which benefited by the synergetic effect of dual reaction sites, reductive Fe-Mn binary oxides and oxygen vacancies (OVs) for PMS activation. The optimized sample (H2 annealed at 260 °C, FMO-260) exhibited high degradation efficiency to RhB within 5 cycles and after regeneration, implying the strong stability and reusability. Moreover, the influences of PMS and FMO-260 dosages, pH values, coexist anions for the degradation efficiency to RhB were also carried out. According to inhibitor experiments and EPR (electron paramagnetic resonance) tests, a possible catalytic mechanism and degradation pathway of RhB was proposed. This study provides a novel fabrication strategy to design Fe, Mn-based catalysts and demonstrates more potential in the decolorization field.
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title_short	Reduced Fe, Mn-based catalyst with dual reaction sites for rapid decolorization treatment via Fenton-like reactions
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author2	Long, Yangke Zhao, Shiyin Wang, Pengju Xie, Feng Huang, Junyi Han, Bing Zhang, Zuotai Zhang, Bo-Ping
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up_date	2024-07-06T20:02:39.493Z
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In this study, a novel porous ferromanganese oxides (FeMnOx) nanocubes derived from prussian blue analogues was prepared via a successive codeposition-calcination method, and the reduced Fe, Mn-based catalysts were further synthesized by a hydrogenation process. Their catalytic performance was evaluated in a Fenton-like degradation of Rhodamine B (RhB) and other dyes in the presence of PMS. It was found that FeMnOx showed outstanding catalytic activity in dyes elimination, which benefited by the synergetic effect of dual reaction sites, reductive Fe-Mn binary oxides and oxygen vacancies (OVs) for PMS activation. The optimized sample (H2 annealed at 260 °C, FMO-260) exhibited high degradation efficiency to RhB within 5 cycles and after regeneration, implying the strong stability and reusability. Moreover, the influences of PMS and FMO-260 dosages, pH values, coexist anions for the degradation efficiency to RhB were also carried out. According to inhibitor experiments and EPR (electron paramagnetic resonance) tests, a possible catalytic mechanism and degradation pathway of RhB was proposed. 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Reduced Fe, Mn-based catalyst with dual reaction sites for rapid decolorization treatment via Fenton-like reactions

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