Production of jet fuel range hydrocarbons using a magnetic Ni–Fe/SAPO-11 catalyst for solvent-free hydrodeoxygenation of jatropha oil
A novel, multifunctional Nix–Fe/SAPO-11 catalyst was synthesized and characterized, and its activity was evaluated for the solvent-free hydrodeoxygenation of jatropha oil. The catalyst has a spherical structure and moderate acid strength, and exhibited excellent cyclization and deoxidation activity....
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Tang, Hongbiao [verfasserIn] Dai, Qiqi [verfasserIn] Cao, Yang [verfasserIn] Li, Jin [verfasserIn] Wei, Xiaocui [verfasserIn] Jibran, Khalil [verfasserIn] Wang, Shurong [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2023 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Biomass and bioenergy - Amsterdam [u.a.] : Elsevier Science, 1991, 177 |
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| Übergeordnetes Werk: |
volume:177 |
| DOI / URN: |
10.1016/j.biombioe.2023.106927 |
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ELV064793389 |
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| 245 | 1 | 0 | |a Production of jet fuel range hydrocarbons using a magnetic Ni–Fe/SAPO-11 catalyst for solvent-free hydrodeoxygenation of jatropha oil |
| 264 | 1 | |c 2023 | |
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| 520 | |a A novel, multifunctional Nix–Fe/SAPO-11 catalyst was synthesized and characterized, and its activity was evaluated for the solvent-free hydrodeoxygenation of jatropha oil. The catalyst has a spherical structure and moderate acid strength, and exhibited excellent cyclization and deoxidation activity. The inclusion of iron facilitated the dispersion of active components. Consequently, the iron-nickel alloy particle size remained small, resulting in an optimal distribution of the product. The composition of the products is linear alkanes (59.83%), isoparaffins (4.16%), aromatics (8.41%), and naphthenes (12.03%), where jet fuel components are relatively high, accounting for 55.04% of C8–C16 hydrocarbons. Interestingly, the iron present in the catalyst allowed the use of an external magnetic field for the rapid separation and recycling of the catalyst. Despite multiple uses, the recycled catalyst maintained high activity following five cycles, with hydrocarbon content consistently above 85%. The synergic effect of the metallic and acid sites of the catalyst, let to realize one-pot hydrodeoxygenation, isomerization, aromatization, and cracking of substrate forming bio-jet fuel range hydrocarbons. | ||
| 650 | 4 | |a Hydrodeoxygenation | |
| 650 | 4 | |a Ni–Fe/SAPO-11 | |
| 650 | 4 | |a Jatropha oil | |
| 650 | 4 | |a Jet fuel | |
| 650 | 4 | |a One-pot method | |
| 700 | 1 | |a Dai, Qiqi |e verfasserin |4 aut | |
| 700 | 1 | |a Cao, Yang |e verfasserin |4 aut | |
| 700 | 1 | |a Li, Jin |e verfasserin |4 aut | |
| 700 | 1 | |a Wei, Xiaocui |e verfasserin |4 aut | |
| 700 | 1 | |a Jibran, Khalil |e verfasserin |4 aut | |
| 700 | 1 | |a Wang, Shurong |e verfasserin |4 aut | |
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10.1016/j.biombioe.2023.106927 doi (DE-627)ELV064793389 (ELSEVIER)S0961-9534(23)00226-X DE-627 ger DE-627 rda eng 630 640 530 VZ 35.00 bkl Tang, Hongbiao verfasserin aut Production of jet fuel range hydrocarbons using a magnetic Ni–Fe/SAPO-11 catalyst for solvent-free hydrodeoxygenation of jatropha oil 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A novel, multifunctional Nix–Fe/SAPO-11 catalyst was synthesized and characterized, and its activity was evaluated for the solvent-free hydrodeoxygenation of jatropha oil. The catalyst has a spherical structure and moderate acid strength, and exhibited excellent cyclization and deoxidation activity. The inclusion of iron facilitated the dispersion of active components. Consequently, the iron-nickel alloy particle size remained small, resulting in an optimal distribution of the product. The composition of the products is linear alkanes (59.83%), isoparaffins (4.16%), aromatics (8.41%), and naphthenes (12.03%), where jet fuel components are relatively high, accounting for 55.04% of C8–C16 hydrocarbons. Interestingly, the iron present in the catalyst allowed the use of an external magnetic field for the rapid separation and recycling of the catalyst. Despite multiple uses, the recycled catalyst maintained high activity following five cycles, with hydrocarbon content consistently above 85%. The synergic effect of the metallic and acid sites of the catalyst, let to realize one-pot hydrodeoxygenation, isomerization, aromatization, and cracking of substrate forming bio-jet fuel range hydrocarbons. Hydrodeoxygenation Ni–Fe/SAPO-11 Jatropha oil Jet fuel One-pot method Dai, Qiqi verfasserin aut Cao, Yang verfasserin aut Li, Jin verfasserin aut Wei, Xiaocui verfasserin aut Jibran, Khalil verfasserin aut Wang, Shurong verfasserin aut Enthalten in Biomass and bioenergy Amsterdam [u.a.] : Elsevier Science, 1991 177 Online-Ressource (DE-627)306321661 (DE-600)1496404-1 (DE-576)109839099 0961-9534 nnns volume:177 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 177 |
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10.1016/j.biombioe.2023.106927 doi (DE-627)ELV064793389 (ELSEVIER)S0961-9534(23)00226-X DE-627 ger DE-627 rda eng 630 640 530 VZ 35.00 bkl Tang, Hongbiao verfasserin aut Production of jet fuel range hydrocarbons using a magnetic Ni–Fe/SAPO-11 catalyst for solvent-free hydrodeoxygenation of jatropha oil 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A novel, multifunctional Nix–Fe/SAPO-11 catalyst was synthesized and characterized, and its activity was evaluated for the solvent-free hydrodeoxygenation of jatropha oil. The catalyst has a spherical structure and moderate acid strength, and exhibited excellent cyclization and deoxidation activity. The inclusion of iron facilitated the dispersion of active components. Consequently, the iron-nickel alloy particle size remained small, resulting in an optimal distribution of the product. The composition of the products is linear alkanes (59.83%), isoparaffins (4.16%), aromatics (8.41%), and naphthenes (12.03%), where jet fuel components are relatively high, accounting for 55.04% of C8–C16 hydrocarbons. Interestingly, the iron present in the catalyst allowed the use of an external magnetic field for the rapid separation and recycling of the catalyst. Despite multiple uses, the recycled catalyst maintained high activity following five cycles, with hydrocarbon content consistently above 85%. The synergic effect of the metallic and acid sites of the catalyst, let to realize one-pot hydrodeoxygenation, isomerization, aromatization, and cracking of substrate forming bio-jet fuel range hydrocarbons. Hydrodeoxygenation Ni–Fe/SAPO-11 Jatropha oil Jet fuel One-pot method Dai, Qiqi verfasserin aut Cao, Yang verfasserin aut Li, Jin verfasserin aut Wei, Xiaocui verfasserin aut Jibran, Khalil verfasserin aut Wang, Shurong verfasserin aut Enthalten in Biomass and bioenergy Amsterdam [u.a.] : Elsevier Science, 1991 177 Online-Ressource (DE-627)306321661 (DE-600)1496404-1 (DE-576)109839099 0961-9534 nnns volume:177 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 177 |
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10.1016/j.biombioe.2023.106927 doi (DE-627)ELV064793389 (ELSEVIER)S0961-9534(23)00226-X DE-627 ger DE-627 rda eng 630 640 530 VZ 35.00 bkl Tang, Hongbiao verfasserin aut Production of jet fuel range hydrocarbons using a magnetic Ni–Fe/SAPO-11 catalyst for solvent-free hydrodeoxygenation of jatropha oil 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A novel, multifunctional Nix–Fe/SAPO-11 catalyst was synthesized and characterized, and its activity was evaluated for the solvent-free hydrodeoxygenation of jatropha oil. The catalyst has a spherical structure and moderate acid strength, and exhibited excellent cyclization and deoxidation activity. The inclusion of iron facilitated the dispersion of active components. Consequently, the iron-nickel alloy particle size remained small, resulting in an optimal distribution of the product. The composition of the products is linear alkanes (59.83%), isoparaffins (4.16%), aromatics (8.41%), and naphthenes (12.03%), where jet fuel components are relatively high, accounting for 55.04% of C8–C16 hydrocarbons. Interestingly, the iron present in the catalyst allowed the use of an external magnetic field for the rapid separation and recycling of the catalyst. Despite multiple uses, the recycled catalyst maintained high activity following five cycles, with hydrocarbon content consistently above 85%. The synergic effect of the metallic and acid sites of the catalyst, let to realize one-pot hydrodeoxygenation, isomerization, aromatization, and cracking of substrate forming bio-jet fuel range hydrocarbons. Hydrodeoxygenation Ni–Fe/SAPO-11 Jatropha oil Jet fuel One-pot method Dai, Qiqi verfasserin aut Cao, Yang verfasserin aut Li, Jin verfasserin aut Wei, Xiaocui verfasserin aut Jibran, Khalil verfasserin aut Wang, Shurong verfasserin aut Enthalten in Biomass and bioenergy Amsterdam [u.a.] : Elsevier Science, 1991 177 Online-Ressource (DE-627)306321661 (DE-600)1496404-1 (DE-576)109839099 0961-9534 nnns volume:177 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 177 |
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10.1016/j.biombioe.2023.106927 doi (DE-627)ELV064793389 (ELSEVIER)S0961-9534(23)00226-X DE-627 ger DE-627 rda eng 630 640 530 VZ 35.00 bkl Tang, Hongbiao verfasserin aut Production of jet fuel range hydrocarbons using a magnetic Ni–Fe/SAPO-11 catalyst for solvent-free hydrodeoxygenation of jatropha oil 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A novel, multifunctional Nix–Fe/SAPO-11 catalyst was synthesized and characterized, and its activity was evaluated for the solvent-free hydrodeoxygenation of jatropha oil. The catalyst has a spherical structure and moderate acid strength, and exhibited excellent cyclization and deoxidation activity. The inclusion of iron facilitated the dispersion of active components. Consequently, the iron-nickel alloy particle size remained small, resulting in an optimal distribution of the product. The composition of the products is linear alkanes (59.83%), isoparaffins (4.16%), aromatics (8.41%), and naphthenes (12.03%), where jet fuel components are relatively high, accounting for 55.04% of C8–C16 hydrocarbons. Interestingly, the iron present in the catalyst allowed the use of an external magnetic field for the rapid separation and recycling of the catalyst. Despite multiple uses, the recycled catalyst maintained high activity following five cycles, with hydrocarbon content consistently above 85%. The synergic effect of the metallic and acid sites of the catalyst, let to realize one-pot hydrodeoxygenation, isomerization, aromatization, and cracking of substrate forming bio-jet fuel range hydrocarbons. Hydrodeoxygenation Ni–Fe/SAPO-11 Jatropha oil Jet fuel One-pot method Dai, Qiqi verfasserin aut Cao, Yang verfasserin aut Li, Jin verfasserin aut Wei, Xiaocui verfasserin aut Jibran, Khalil verfasserin aut Wang, Shurong verfasserin aut Enthalten in Biomass and bioenergy Amsterdam [u.a.] : Elsevier Science, 1991 177 Online-Ressource (DE-627)306321661 (DE-600)1496404-1 (DE-576)109839099 0961-9534 nnns volume:177 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 177 |
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10.1016/j.biombioe.2023.106927 doi (DE-627)ELV064793389 (ELSEVIER)S0961-9534(23)00226-X DE-627 ger DE-627 rda eng 630 640 530 VZ 35.00 bkl Tang, Hongbiao verfasserin aut Production of jet fuel range hydrocarbons using a magnetic Ni–Fe/SAPO-11 catalyst for solvent-free hydrodeoxygenation of jatropha oil 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A novel, multifunctional Nix–Fe/SAPO-11 catalyst was synthesized and characterized, and its activity was evaluated for the solvent-free hydrodeoxygenation of jatropha oil. The catalyst has a spherical structure and moderate acid strength, and exhibited excellent cyclization and deoxidation activity. The inclusion of iron facilitated the dispersion of active components. Consequently, the iron-nickel alloy particle size remained small, resulting in an optimal distribution of the product. The composition of the products is linear alkanes (59.83%), isoparaffins (4.16%), aromatics (8.41%), and naphthenes (12.03%), where jet fuel components are relatively high, accounting for 55.04% of C8–C16 hydrocarbons. Interestingly, the iron present in the catalyst allowed the use of an external magnetic field for the rapid separation and recycling of the catalyst. Despite multiple uses, the recycled catalyst maintained high activity following five cycles, with hydrocarbon content consistently above 85%. The synergic effect of the metallic and acid sites of the catalyst, let to realize one-pot hydrodeoxygenation, isomerization, aromatization, and cracking of substrate forming bio-jet fuel range hydrocarbons. Hydrodeoxygenation Ni–Fe/SAPO-11 Jatropha oil Jet fuel One-pot method Dai, Qiqi verfasserin aut Cao, Yang verfasserin aut Li, Jin verfasserin aut Wei, Xiaocui verfasserin aut Jibran, Khalil verfasserin aut Wang, Shurong verfasserin aut Enthalten in Biomass and bioenergy Amsterdam [u.a.] : Elsevier Science, 1991 177 Online-Ressource (DE-627)306321661 (DE-600)1496404-1 (DE-576)109839099 0961-9534 nnns volume:177 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 177 |
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Enthalten in Biomass and bioenergy 177 volume:177 |
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Tang, Hongbiao @@aut@@ Dai, Qiqi @@aut@@ Cao, Yang @@aut@@ Li, Jin @@aut@@ Wei, Xiaocui @@aut@@ Jibran, Khalil @@aut@@ Wang, Shurong @@aut@@ |
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2023-01-01T00:00:00Z |
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Tang, Hongbiao ddc 630 bkl 35.00 misc Hydrodeoxygenation misc Ni–Fe/SAPO-11 misc Jatropha oil misc Jet fuel misc One-pot method Production of jet fuel range hydrocarbons using a magnetic Ni–Fe/SAPO-11 catalyst for solvent-free hydrodeoxygenation of jatropha oil |
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630 640 530 VZ 35.00 bkl Production of jet fuel range hydrocarbons using a magnetic Ni–Fe/SAPO-11 catalyst for solvent-free hydrodeoxygenation of jatropha oil Hydrodeoxygenation Ni–Fe/SAPO-11 Jatropha oil Jet fuel One-pot method |
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production of jet fuel range hydrocarbons using a magnetic ni–fe/sapo-11 catalyst for solvent-free hydrodeoxygenation of jatropha oil |
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Production of jet fuel range hydrocarbons using a magnetic Ni–Fe/SAPO-11 catalyst for solvent-free hydrodeoxygenation of jatropha oil |
| abstract |
A novel, multifunctional Nix–Fe/SAPO-11 catalyst was synthesized and characterized, and its activity was evaluated for the solvent-free hydrodeoxygenation of jatropha oil. The catalyst has a spherical structure and moderate acid strength, and exhibited excellent cyclization and deoxidation activity. The inclusion of iron facilitated the dispersion of active components. Consequently, the iron-nickel alloy particle size remained small, resulting in an optimal distribution of the product. The composition of the products is linear alkanes (59.83%), isoparaffins (4.16%), aromatics (8.41%), and naphthenes (12.03%), where jet fuel components are relatively high, accounting for 55.04% of C8–C16 hydrocarbons. Interestingly, the iron present in the catalyst allowed the use of an external magnetic field for the rapid separation and recycling of the catalyst. Despite multiple uses, the recycled catalyst maintained high activity following five cycles, with hydrocarbon content consistently above 85%. The synergic effect of the metallic and acid sites of the catalyst, let to realize one-pot hydrodeoxygenation, isomerization, aromatization, and cracking of substrate forming bio-jet fuel range hydrocarbons. |
| abstractGer |
A novel, multifunctional Nix–Fe/SAPO-11 catalyst was synthesized and characterized, and its activity was evaluated for the solvent-free hydrodeoxygenation of jatropha oil. The catalyst has a spherical structure and moderate acid strength, and exhibited excellent cyclization and deoxidation activity. The inclusion of iron facilitated the dispersion of active components. Consequently, the iron-nickel alloy particle size remained small, resulting in an optimal distribution of the product. The composition of the products is linear alkanes (59.83%), isoparaffins (4.16%), aromatics (8.41%), and naphthenes (12.03%), where jet fuel components are relatively high, accounting for 55.04% of C8–C16 hydrocarbons. Interestingly, the iron present in the catalyst allowed the use of an external magnetic field for the rapid separation and recycling of the catalyst. Despite multiple uses, the recycled catalyst maintained high activity following five cycles, with hydrocarbon content consistently above 85%. The synergic effect of the metallic and acid sites of the catalyst, let to realize one-pot hydrodeoxygenation, isomerization, aromatization, and cracking of substrate forming bio-jet fuel range hydrocarbons. |
| abstract_unstemmed |
A novel, multifunctional Nix–Fe/SAPO-11 catalyst was synthesized and characterized, and its activity was evaluated for the solvent-free hydrodeoxygenation of jatropha oil. The catalyst has a spherical structure and moderate acid strength, and exhibited excellent cyclization and deoxidation activity. The inclusion of iron facilitated the dispersion of active components. Consequently, the iron-nickel alloy particle size remained small, resulting in an optimal distribution of the product. The composition of the products is linear alkanes (59.83%), isoparaffins (4.16%), aromatics (8.41%), and naphthenes (12.03%), where jet fuel components are relatively high, accounting for 55.04% of C8–C16 hydrocarbons. Interestingly, the iron present in the catalyst allowed the use of an external magnetic field for the rapid separation and recycling of the catalyst. Despite multiple uses, the recycled catalyst maintained high activity following five cycles, with hydrocarbon content consistently above 85%. The synergic effect of the metallic and acid sites of the catalyst, let to realize one-pot hydrodeoxygenation, isomerization, aromatization, and cracking of substrate forming bio-jet fuel range hydrocarbons. |
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Production of jet fuel range hydrocarbons using a magnetic Ni–Fe/SAPO-11 catalyst for solvent-free hydrodeoxygenation of jatropha oil |
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|
| score |
7.398575 |