Nitrogen, phosphorus co-doped holey rGO as a cathode material for Li-ion capacitors (LICs)

Graphene-based materials are considered as ideal cathode materials for lithium-ion capacitors (LICs). However, the ion-accessible surface area of graphene is restricted by the restacking of graphene nanosheets, resulting in a limited specific capacity. Fabricating porous graphene with an appropriate...
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Gespeichert in:

Autor*in:	Alomari, Suaad A. [verfasserIn] Dubal, Deepak P. [verfasserIn] MacLeod, Jennifer [verfasserIn] Jadhav, Sagar [verfasserIn] Padwal, Chinmayee [verfasserIn] Motta, Nunzio [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	rGO Holey rGO Heteroatom-doped rGO Lithium-ion capacitors Energy storage devices

Übergeordnetes Werk:	Enthalten in: Applied surface science - Amsterdam : Elsevier, 1985, 641
Übergeordnetes Werk:	volume:641

DOI / URN:	10.1016/j.apsusc.2023.158452

Katalog-ID:	ELV065077520

Internformat


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245	1	0	\|a Nitrogen, phosphorus co-doped holey rGO as a cathode material for Li-ion capacitors (LICs)
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520			\|a Graphene-based materials are considered as ideal cathode materials for lithium-ion capacitors (LICs). However, the ion-accessible surface area of graphene is restricted by the restacking of graphene nanosheets, resulting in a limited specific capacity. Fabricating porous graphene with an appropriate pore structure and introducing heteroatom doping can improve the capacity of graphene and increase the energy outputs of graphene-based LICs. Herein, we use an easy and low-cost hydrothermal method to create a 3D nitrogen and phosphorus co-doped holey rGO (NPHG) aerogel. In a half-cell system, NPHG delivers a specific capacity of ∼120 mAh/g at 0.1 A/g and maintains 92% of its initial capacity after 1000 cycles at 1 Ag−1. Moreover, when used as a cathode with a pre-lithiated nitrogen-doped rGO-siloxene (NGSil-4) anode to construct an NGSil-4//NPHG LIC, a high energy density of 145.86 Wh Kg−1 is obtained at a power density of 200.2 W Kg−1, while retaining 15.35 Wh Kg−1 at 14550 W Kg−1.This work demonstrates the great potential of NPHG cathodes, with the integration of the appropriate porosity and N and P co-doping using a simple and low cost hydrothermal method, for high-performance LICs.
650		4	\|a rGO
650		4	\|a Holey rGO
650		4	\|a Heteroatom-doped rGO
650		4	\|a Lithium-ion capacitors
650		4	\|a Energy storage devices
700	1		\|a Dubal, Deepak P. \|e verfasserin \|4 aut
700	1		\|a MacLeod, Jennifer \|e verfasserin \|0 (orcid)0000-0002-2138-8716 \|4 aut
700	1		\|a Jadhav, Sagar \|e verfasserin \|0 (orcid)0000-0001-7259-5435 \|4 aut
700	1		\|a Padwal, Chinmayee \|e verfasserin \|0 (orcid)0009-0008-4487-7054 \|4 aut
700	1		\|a Motta, Nunzio \|e verfasserin \|0 (orcid)0000-0002-3857-1031 \|4 aut
773	0	8	\|i Enthalten in \|t Applied surface science \|d Amsterdam : Elsevier, 1985 \|g 641 \|h Online-Ressource \|w (DE-627)312151128 \|w (DE-600)2002520-8 \|w (DE-576)094476985 \|7 nnns
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912			\|a GBV_ILN_602
912			\|a GBV_ILN_702
912			\|a GBV_ILN_2001
912			\|a GBV_ILN_2003
912			\|a GBV_ILN_2004
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912			\|a GBV_ILN_2025
912			\|a GBV_ILN_2026
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912			\|a GBV_ILN_4323
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912			\|a GBV_ILN_4334
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matchkey_str	alomarisuaadadubaldeepakpmacleodjennifer:2023----:irgnhshrsooehlygaaahdmtrafr
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publishDate	2023
allfields	10.1016/j.apsusc.2023.158452 doi (DE-627)ELV065077520 (ELSEVIER)S0169-4332(23)02132-3 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Alomari, Suaad A. verfasserin (orcid)0000-0002-0315-7105 aut Nitrogen, phosphorus co-doped holey rGO as a cathode material for Li-ion capacitors (LICs) 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Graphene-based materials are considered as ideal cathode materials for lithium-ion capacitors (LICs). However, the ion-accessible surface area of graphene is restricted by the restacking of graphene nanosheets, resulting in a limited specific capacity. Fabricating porous graphene with an appropriate pore structure and introducing heteroatom doping can improve the capacity of graphene and increase the energy outputs of graphene-based LICs. Herein, we use an easy and low-cost hydrothermal method to create a 3D nitrogen and phosphorus co-doped holey rGO (NPHG) aerogel. In a half-cell system, NPHG delivers a specific capacity of ∼120 mAh/g at 0.1 A/g and maintains 92% of its initial capacity after 1000 cycles at 1 Ag−1. Moreover, when used as a cathode with a pre-lithiated nitrogen-doped rGO-siloxene (NGSil-4) anode to construct an NGSil-4//NPHG LIC, a high energy density of 145.86 Wh Kg−1 is obtained at a power density of 200.2 W Kg−1, while retaining 15.35 Wh Kg−1 at 14550 W Kg−1.This work demonstrates the great potential of NPHG cathodes, with the integration of the appropriate porosity and N and P co-doping using a simple and low cost hydrothermal method, for high-performance LICs. rGO Holey rGO Heteroatom-doped rGO Lithium-ion capacitors Energy storage devices Dubal, Deepak P. verfasserin aut MacLeod, Jennifer verfasserin (orcid)0000-0002-2138-8716 aut Jadhav, Sagar verfasserin (orcid)0000-0001-7259-5435 aut Padwal, Chinmayee verfasserin (orcid)0009-0008-4487-7054 aut Motta, Nunzio verfasserin (orcid)0000-0002-3857-1031 aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 641 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:641 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 641
spelling	10.1016/j.apsusc.2023.158452 doi (DE-627)ELV065077520 (ELSEVIER)S0169-4332(23)02132-3 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Alomari, Suaad A. verfasserin (orcid)0000-0002-0315-7105 aut Nitrogen, phosphorus co-doped holey rGO as a cathode material for Li-ion capacitors (LICs) 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Graphene-based materials are considered as ideal cathode materials for lithium-ion capacitors (LICs). However, the ion-accessible surface area of graphene is restricted by the restacking of graphene nanosheets, resulting in a limited specific capacity. Fabricating porous graphene with an appropriate pore structure and introducing heteroatom doping can improve the capacity of graphene and increase the energy outputs of graphene-based LICs. Herein, we use an easy and low-cost hydrothermal method to create a 3D nitrogen and phosphorus co-doped holey rGO (NPHG) aerogel. In a half-cell system, NPHG delivers a specific capacity of ∼120 mAh/g at 0.1 A/g and maintains 92% of its initial capacity after 1000 cycles at 1 Ag−1. Moreover, when used as a cathode with a pre-lithiated nitrogen-doped rGO-siloxene (NGSil-4) anode to construct an NGSil-4//NPHG LIC, a high energy density of 145.86 Wh Kg−1 is obtained at a power density of 200.2 W Kg−1, while retaining 15.35 Wh Kg−1 at 14550 W Kg−1.This work demonstrates the great potential of NPHG cathodes, with the integration of the appropriate porosity and N and P co-doping using a simple and low cost hydrothermal method, for high-performance LICs. rGO Holey rGO Heteroatom-doped rGO Lithium-ion capacitors Energy storage devices Dubal, Deepak P. verfasserin aut MacLeod, Jennifer verfasserin (orcid)0000-0002-2138-8716 aut Jadhav, Sagar verfasserin (orcid)0000-0001-7259-5435 aut Padwal, Chinmayee verfasserin (orcid)0009-0008-4487-7054 aut Motta, Nunzio verfasserin (orcid)0000-0002-3857-1031 aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 641 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:641 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 641
allfields_unstemmed	10.1016/j.apsusc.2023.158452 doi (DE-627)ELV065077520 (ELSEVIER)S0169-4332(23)02132-3 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Alomari, Suaad A. verfasserin (orcid)0000-0002-0315-7105 aut Nitrogen, phosphorus co-doped holey rGO as a cathode material for Li-ion capacitors (LICs) 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Graphene-based materials are considered as ideal cathode materials for lithium-ion capacitors (LICs). However, the ion-accessible surface area of graphene is restricted by the restacking of graphene nanosheets, resulting in a limited specific capacity. Fabricating porous graphene with an appropriate pore structure and introducing heteroatom doping can improve the capacity of graphene and increase the energy outputs of graphene-based LICs. Herein, we use an easy and low-cost hydrothermal method to create a 3D nitrogen and phosphorus co-doped holey rGO (NPHG) aerogel. In a half-cell system, NPHG delivers a specific capacity of ∼120 mAh/g at 0.1 A/g and maintains 92% of its initial capacity after 1000 cycles at 1 Ag−1. Moreover, when used as a cathode with a pre-lithiated nitrogen-doped rGO-siloxene (NGSil-4) anode to construct an NGSil-4//NPHG LIC, a high energy density of 145.86 Wh Kg−1 is obtained at a power density of 200.2 W Kg−1, while retaining 15.35 Wh Kg−1 at 14550 W Kg−1.This work demonstrates the great potential of NPHG cathodes, with the integration of the appropriate porosity and N and P co-doping using a simple and low cost hydrothermal method, for high-performance LICs. rGO Holey rGO Heteroatom-doped rGO Lithium-ion capacitors Energy storage devices Dubal, Deepak P. verfasserin aut MacLeod, Jennifer verfasserin (orcid)0000-0002-2138-8716 aut Jadhav, Sagar verfasserin (orcid)0000-0001-7259-5435 aut Padwal, Chinmayee verfasserin (orcid)0009-0008-4487-7054 aut Motta, Nunzio verfasserin (orcid)0000-0002-3857-1031 aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 641 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:641 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 641
allfieldsGer	10.1016/j.apsusc.2023.158452 doi (DE-627)ELV065077520 (ELSEVIER)S0169-4332(23)02132-3 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Alomari, Suaad A. verfasserin (orcid)0000-0002-0315-7105 aut Nitrogen, phosphorus co-doped holey rGO as a cathode material for Li-ion capacitors (LICs) 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Graphene-based materials are considered as ideal cathode materials for lithium-ion capacitors (LICs). However, the ion-accessible surface area of graphene is restricted by the restacking of graphene nanosheets, resulting in a limited specific capacity. Fabricating porous graphene with an appropriate pore structure and introducing heteroatom doping can improve the capacity of graphene and increase the energy outputs of graphene-based LICs. Herein, we use an easy and low-cost hydrothermal method to create a 3D nitrogen and phosphorus co-doped holey rGO (NPHG) aerogel. In a half-cell system, NPHG delivers a specific capacity of ∼120 mAh/g at 0.1 A/g and maintains 92% of its initial capacity after 1000 cycles at 1 Ag−1. Moreover, when used as a cathode with a pre-lithiated nitrogen-doped rGO-siloxene (NGSil-4) anode to construct an NGSil-4//NPHG LIC, a high energy density of 145.86 Wh Kg−1 is obtained at a power density of 200.2 W Kg−1, while retaining 15.35 Wh Kg−1 at 14550 W Kg−1.This work demonstrates the great potential of NPHG cathodes, with the integration of the appropriate porosity and N and P co-doping using a simple and low cost hydrothermal method, for high-performance LICs. rGO Holey rGO Heteroatom-doped rGO Lithium-ion capacitors Energy storage devices Dubal, Deepak P. verfasserin aut MacLeod, Jennifer verfasserin (orcid)0000-0002-2138-8716 aut Jadhav, Sagar verfasserin (orcid)0000-0001-7259-5435 aut Padwal, Chinmayee verfasserin (orcid)0009-0008-4487-7054 aut Motta, Nunzio verfasserin (orcid)0000-0002-3857-1031 aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 641 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:641 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 641
allfieldsSound	10.1016/j.apsusc.2023.158452 doi (DE-627)ELV065077520 (ELSEVIER)S0169-4332(23)02132-3 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Alomari, Suaad A. verfasserin (orcid)0000-0002-0315-7105 aut Nitrogen, phosphorus co-doped holey rGO as a cathode material for Li-ion capacitors (LICs) 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Graphene-based materials are considered as ideal cathode materials for lithium-ion capacitors (LICs). However, the ion-accessible surface area of graphene is restricted by the restacking of graphene nanosheets, resulting in a limited specific capacity. Fabricating porous graphene with an appropriate pore structure and introducing heteroatom doping can improve the capacity of graphene and increase the energy outputs of graphene-based LICs. Herein, we use an easy and low-cost hydrothermal method to create a 3D nitrogen and phosphorus co-doped holey rGO (NPHG) aerogel. In a half-cell system, NPHG delivers a specific capacity of ∼120 mAh/g at 0.1 A/g and maintains 92% of its initial capacity after 1000 cycles at 1 Ag−1. Moreover, when used as a cathode with a pre-lithiated nitrogen-doped rGO-siloxene (NGSil-4) anode to construct an NGSil-4//NPHG LIC, a high energy density of 145.86 Wh Kg−1 is obtained at a power density of 200.2 W Kg−1, while retaining 15.35 Wh Kg−1 at 14550 W Kg−1.This work demonstrates the great potential of NPHG cathodes, with the integration of the appropriate porosity and N and P co-doping using a simple and low cost hydrothermal method, for high-performance LICs. rGO Holey rGO Heteroatom-doped rGO Lithium-ion capacitors Energy storage devices Dubal, Deepak P. verfasserin aut MacLeod, Jennifer verfasserin (orcid)0000-0002-2138-8716 aut Jadhav, Sagar verfasserin (orcid)0000-0001-7259-5435 aut Padwal, Chinmayee verfasserin (orcid)0009-0008-4487-7054 aut Motta, Nunzio verfasserin (orcid)0000-0002-3857-1031 aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 641 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:641 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 641
language	English
source	Enthalten in Applied surface science 641 volume:641
sourceStr	Enthalten in Applied surface science 641 volume:641
format_phy_str_mv	Article
bklname	Oberflächen Dünne Schichten Grenzflächen Kolloidchemie Grenzflächenchemie Oberflächentechnik Wärmebehandlung
institution	findex.gbv.de
topic_facet	rGO Holey rGO Heteroatom-doped rGO Lithium-ion capacitors Energy storage devices
dewey-raw	670
isfreeaccess_bool	false
container_title	Applied surface science
authorswithroles_txt_mv	Alomari, Suaad A. @@aut@@ Dubal, Deepak P. @@aut@@ MacLeod, Jennifer @@aut@@ Jadhav, Sagar @@aut@@ Padwal, Chinmayee @@aut@@ Motta, Nunzio @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	312151128
dewey-sort	3670
id	ELV065077520
language_de	englisch
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author	Alomari, Suaad A.
spellingShingle	Alomari, Suaad A. ddc 670 bkl 33.68 bkl 35.18 bkl 52.78 misc rGO misc Holey rGO misc Heteroatom-doped rGO misc Lithium-ion capacitors misc Energy storage devices Nitrogen, phosphorus co-doped holey rGO as a cathode material for Li-ion capacitors (LICs)
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topic_title	670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Nitrogen, phosphorus co-doped holey rGO as a cathode material for Li-ion capacitors (LICs) rGO Holey rGO Heteroatom-doped rGO Lithium-ion capacitors Energy storage devices
topic	ddc 670 bkl 33.68 bkl 35.18 bkl 52.78 misc rGO misc Holey rGO misc Heteroatom-doped rGO misc Lithium-ion capacitors misc Energy storage devices
topic_unstemmed	ddc 670 bkl 33.68 bkl 35.18 bkl 52.78 misc rGO misc Holey rGO misc Heteroatom-doped rGO misc Lithium-ion capacitors misc Energy storage devices
topic_browse	ddc 670 bkl 33.68 bkl 35.18 bkl 52.78 misc rGO misc Holey rGO misc Heteroatom-doped rGO misc Lithium-ion capacitors misc Energy storage devices
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title	Nitrogen, phosphorus co-doped holey rGO as a cathode material for Li-ion capacitors (LICs)
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title_full	Nitrogen, phosphorus co-doped holey rGO as a cathode material for Li-ion capacitors (LICs)
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title_sort	nitrogen, phosphorus co-doped holey rgo as a cathode material for li-ion capacitors (lics)
title_auth	Nitrogen, phosphorus co-doped holey rGO as a cathode material for Li-ion capacitors (LICs)
abstract	Graphene-based materials are considered as ideal cathode materials for lithium-ion capacitors (LICs). However, the ion-accessible surface area of graphene is restricted by the restacking of graphene nanosheets, resulting in a limited specific capacity. Fabricating porous graphene with an appropriate pore structure and introducing heteroatom doping can improve the capacity of graphene and increase the energy outputs of graphene-based LICs. Herein, we use an easy and low-cost hydrothermal method to create a 3D nitrogen and phosphorus co-doped holey rGO (NPHG) aerogel. In a half-cell system, NPHG delivers a specific capacity of ∼120 mAh/g at 0.1 A/g and maintains 92% of its initial capacity after 1000 cycles at 1 Ag−1. Moreover, when used as a cathode with a pre-lithiated nitrogen-doped rGO-siloxene (NGSil-4) anode to construct an NGSil-4//NPHG LIC, a high energy density of 145.86 Wh Kg−1 is obtained at a power density of 200.2 W Kg−1, while retaining 15.35 Wh Kg−1 at 14550 W Kg−1.This work demonstrates the great potential of NPHG cathodes, with the integration of the appropriate porosity and N and P co-doping using a simple and low cost hydrothermal method, for high-performance LICs.
abstractGer	Graphene-based materials are considered as ideal cathode materials for lithium-ion capacitors (LICs). However, the ion-accessible surface area of graphene is restricted by the restacking of graphene nanosheets, resulting in a limited specific capacity. Fabricating porous graphene with an appropriate pore structure and introducing heteroatom doping can improve the capacity of graphene and increase the energy outputs of graphene-based LICs. Herein, we use an easy and low-cost hydrothermal method to create a 3D nitrogen and phosphorus co-doped holey rGO (NPHG) aerogel. In a half-cell system, NPHG delivers a specific capacity of ∼120 mAh/g at 0.1 A/g and maintains 92% of its initial capacity after 1000 cycles at 1 Ag−1. Moreover, when used as a cathode with a pre-lithiated nitrogen-doped rGO-siloxene (NGSil-4) anode to construct an NGSil-4//NPHG LIC, a high energy density of 145.86 Wh Kg−1 is obtained at a power density of 200.2 W Kg−1, while retaining 15.35 Wh Kg−1 at 14550 W Kg−1.This work demonstrates the great potential of NPHG cathodes, with the integration of the appropriate porosity and N and P co-doping using a simple and low cost hydrothermal method, for high-performance LICs.
abstract_unstemmed	Graphene-based materials are considered as ideal cathode materials for lithium-ion capacitors (LICs). However, the ion-accessible surface area of graphene is restricted by the restacking of graphene nanosheets, resulting in a limited specific capacity. Fabricating porous graphene with an appropriate pore structure and introducing heteroatom doping can improve the capacity of graphene and increase the energy outputs of graphene-based LICs. Herein, we use an easy and low-cost hydrothermal method to create a 3D nitrogen and phosphorus co-doped holey rGO (NPHG) aerogel. In a half-cell system, NPHG delivers a specific capacity of ∼120 mAh/g at 0.1 A/g and maintains 92% of its initial capacity after 1000 cycles at 1 Ag−1. Moreover, when used as a cathode with a pre-lithiated nitrogen-doped rGO-siloxene (NGSil-4) anode to construct an NGSil-4//NPHG LIC, a high energy density of 145.86 Wh Kg−1 is obtained at a power density of 200.2 W Kg−1, while retaining 15.35 Wh Kg−1 at 14550 W Kg−1.This work demonstrates the great potential of NPHG cathodes, with the integration of the appropriate porosity and N and P co-doping using a simple and low cost hydrothermal method, for high-performance LICs.
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title_short	Nitrogen, phosphorus co-doped holey rGO as a cathode material for Li-ion capacitors (LICs)
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author2	Dubal, Deepak P. MacLeod, Jennifer Jadhav, Sagar Padwal, Chinmayee Motta, Nunzio
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up_date	2024-07-06T21:45:03.350Z
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However, the ion-accessible surface area of graphene is restricted by the restacking of graphene nanosheets, resulting in a limited specific capacity. Fabricating porous graphene with an appropriate pore structure and introducing heteroatom doping can improve the capacity of graphene and increase the energy outputs of graphene-based LICs. Herein, we use an easy and low-cost hydrothermal method to create a 3D nitrogen and phosphorus co-doped holey rGO (NPHG) aerogel. In a half-cell system, NPHG delivers a specific capacity of ∼120 mAh/g at 0.1 A/g and maintains 92% of its initial capacity after 1000 cycles at 1 Ag−1. Moreover, when used as a cathode with a pre-lithiated nitrogen-doped rGO-siloxene (NGSil-4) anode to construct an NGSil-4//NPHG LIC, a high energy density of 145.86 Wh Kg−1 is obtained at a power density of 200.2 W Kg−1, while retaining 15.35 Wh Kg−1 at 14550 W Kg−1.This work demonstrates the great potential of NPHG cathodes, with the integration of the appropriate porosity and N and P co-doping using a simple and low cost hydrothermal method, for high-performance LICs.</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">rGO</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Holey rGO</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Heteroatom-doped rGO</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Lithium-ion capacitors</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Energy storage devices</subfield></datafield><datafield tag="700" 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Nitrogen, phosphorus co-doped holey rGO as a cathode material for Li-ion capacitors (LICs)

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