An ultrahigh-resolution multicolor sensing platform via target-induced etching of gold nanorods for multi-colorimetric analysis of trace silver ions
Heavy metal ion pollution is a pressing global concern with detrimental effects on the environment and human health. To address this issue, we have developed an ultrahigh-resolution multicolor sensing platform for the specific detection of silver ions (Ag(I)). The method employs the nanozyme of plat...
Ausführliche Beschreibung
Autor*in: |
Ma, Xiaoming [verfasserIn] Zhang, Hui [verfasserIn] Liu, Jin [verfasserIn] Zhang, Huifang [verfasserIn] Hu, Xuan [verfasserIn] Wang, Yu [verfasserIn] Li, Xun [verfasserIn] Xu, Jianguo [verfasserIn] |
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Format: |
E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2023 |
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Schlagwörter: |
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Übergeordnetes Werk: |
Enthalten in: Sensors and actuators |
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Übergeordnetes Werk: |
volume:397 |
DOI / URN: |
10.1016/j.snb.2023.134658 |
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Katalog-ID: |
ELV065111087 |
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245 | 1 | 0 | |a An ultrahigh-resolution multicolor sensing platform via target-induced etching of gold nanorods for multi-colorimetric analysis of trace silver ions |
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520 | |a Heavy metal ion pollution is a pressing global concern with detrimental effects on the environment and human health. To address this issue, we have developed an ultrahigh-resolution multicolor sensing platform for the specific detection of silver ions (Ag(I)). The method employs the nanozyme of platinum nanoparticles (PtNPs) as a link to control the etching of gold nanorods (AuNRs). Through specific binding with Ag(I), the PtNPs hinder the catalase-like activity responsible for hydrogen peroxide (H2O2) decomposition. This inhibition enables the Fenton reaction between H2O2 and ferrous ions, generating highly oxidizing hydroxyl free radicals (·OH). The resulting etching of AuNRs induces a blue-shift in their local surface plasmon resonance (LSPR) absorption spectra. The degree of blue-shift is directly proportional to the Ag(I) concentration, facilitating trace-level detection. Furthermore, the aspect ratio change of the AuNRs yields distinguishable colors. In contrast to common multicolor sensors relying on nanozyme horseradish peroxidase (HRP) activity, which exhibits an inverse relationship between AuNR etching and target concentration, our approach demonstrates a proportional response. This unique characteristic enables ultrahigh-resolution multicolor detection of Ag(I) visible to the naked eye. We anticipate that this innovative sensing platform will pave the way for nanosensor development in environmental monitoring and food safety detection. | ||
650 | 4 | |a Ultrahigh resolution | |
650 | 4 | |a Multicolor sensor | |
650 | 4 | |a Silver ion detection | |
650 | 4 | |a Gold nanorod | |
650 | 4 | |a Nanozyme | |
700 | 1 | |a Zhang, Hui |e verfasserin |4 aut | |
700 | 1 | |a Liu, Jin |e verfasserin |4 aut | |
700 | 1 | |a Zhang, Huifang |e verfasserin |4 aut | |
700 | 1 | |a Hu, Xuan |e verfasserin |4 aut | |
700 | 1 | |a Wang, Yu |e verfasserin |4 aut | |
700 | 1 | |a Li, Xun |e verfasserin |4 aut | |
700 | 1 | |a Xu, Jianguo |e verfasserin |4 aut | |
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2023 |
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10.1016/j.snb.2023.134658 doi (DE-627)ELV065111087 (ELSEVIER)S0925-4005(23)01373-4 DE-627 ger DE-627 rda eng 530 620 VZ 50.22 bkl 35.07 bkl Ma, Xiaoming verfasserin aut An ultrahigh-resolution multicolor sensing platform via target-induced etching of gold nanorods for multi-colorimetric analysis of trace silver ions 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Heavy metal ion pollution is a pressing global concern with detrimental effects on the environment and human health. To address this issue, we have developed an ultrahigh-resolution multicolor sensing platform for the specific detection of silver ions (Ag(I)). The method employs the nanozyme of platinum nanoparticles (PtNPs) as a link to control the etching of gold nanorods (AuNRs). Through specific binding with Ag(I), the PtNPs hinder the catalase-like activity responsible for hydrogen peroxide (H2O2) decomposition. This inhibition enables the Fenton reaction between H2O2 and ferrous ions, generating highly oxidizing hydroxyl free radicals (·OH). The resulting etching of AuNRs induces a blue-shift in their local surface plasmon resonance (LSPR) absorption spectra. The degree of blue-shift is directly proportional to the Ag(I) concentration, facilitating trace-level detection. Furthermore, the aspect ratio change of the AuNRs yields distinguishable colors. In contrast to common multicolor sensors relying on nanozyme horseradish peroxidase (HRP) activity, which exhibits an inverse relationship between AuNR etching and target concentration, our approach demonstrates a proportional response. This unique characteristic enables ultrahigh-resolution multicolor detection of Ag(I) visible to the naked eye. We anticipate that this innovative sensing platform will pave the way for nanosensor development in environmental monitoring and food safety detection. Ultrahigh resolution Multicolor sensor Silver ion detection Gold nanorod Nanozyme Zhang, Hui verfasserin aut Liu, Jin verfasserin aut Zhang, Huifang verfasserin aut Hu, Xuan verfasserin aut Wang, Yu verfasserin aut Li, Xun verfasserin aut Xu, Jianguo verfasserin aut Enthalten in Sensors and actuators <Lausanne> / B Amsterdam [u.a.] : Elsevier Science, 1990 397 Online-Ressource (DE-627)306710358 (DE-600)1500731-5 (DE-576)082435855 0925-4005 nnns volume:397 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 50.22 Sensorik VZ 35.07 Chemisches Labor chemische Methoden VZ AR 397 |
spelling |
10.1016/j.snb.2023.134658 doi (DE-627)ELV065111087 (ELSEVIER)S0925-4005(23)01373-4 DE-627 ger DE-627 rda eng 530 620 VZ 50.22 bkl 35.07 bkl Ma, Xiaoming verfasserin aut An ultrahigh-resolution multicolor sensing platform via target-induced etching of gold nanorods for multi-colorimetric analysis of trace silver ions 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Heavy metal ion pollution is a pressing global concern with detrimental effects on the environment and human health. To address this issue, we have developed an ultrahigh-resolution multicolor sensing platform for the specific detection of silver ions (Ag(I)). The method employs the nanozyme of platinum nanoparticles (PtNPs) as a link to control the etching of gold nanorods (AuNRs). Through specific binding with Ag(I), the PtNPs hinder the catalase-like activity responsible for hydrogen peroxide (H2O2) decomposition. This inhibition enables the Fenton reaction between H2O2 and ferrous ions, generating highly oxidizing hydroxyl free radicals (·OH). The resulting etching of AuNRs induces a blue-shift in their local surface plasmon resonance (LSPR) absorption spectra. The degree of blue-shift is directly proportional to the Ag(I) concentration, facilitating trace-level detection. Furthermore, the aspect ratio change of the AuNRs yields distinguishable colors. In contrast to common multicolor sensors relying on nanozyme horseradish peroxidase (HRP) activity, which exhibits an inverse relationship between AuNR etching and target concentration, our approach demonstrates a proportional response. This unique characteristic enables ultrahigh-resolution multicolor detection of Ag(I) visible to the naked eye. We anticipate that this innovative sensing platform will pave the way for nanosensor development in environmental monitoring and food safety detection. Ultrahigh resolution Multicolor sensor Silver ion detection Gold nanorod Nanozyme Zhang, Hui verfasserin aut Liu, Jin verfasserin aut Zhang, Huifang verfasserin aut Hu, Xuan verfasserin aut Wang, Yu verfasserin aut Li, Xun verfasserin aut Xu, Jianguo verfasserin aut Enthalten in Sensors and actuators <Lausanne> / B Amsterdam [u.a.] : Elsevier Science, 1990 397 Online-Ressource (DE-627)306710358 (DE-600)1500731-5 (DE-576)082435855 0925-4005 nnns volume:397 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 50.22 Sensorik VZ 35.07 Chemisches Labor chemische Methoden VZ AR 397 |
allfields_unstemmed |
10.1016/j.snb.2023.134658 doi (DE-627)ELV065111087 (ELSEVIER)S0925-4005(23)01373-4 DE-627 ger DE-627 rda eng 530 620 VZ 50.22 bkl 35.07 bkl Ma, Xiaoming verfasserin aut An ultrahigh-resolution multicolor sensing platform via target-induced etching of gold nanorods for multi-colorimetric analysis of trace silver ions 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Heavy metal ion pollution is a pressing global concern with detrimental effects on the environment and human health. To address this issue, we have developed an ultrahigh-resolution multicolor sensing platform for the specific detection of silver ions (Ag(I)). The method employs the nanozyme of platinum nanoparticles (PtNPs) as a link to control the etching of gold nanorods (AuNRs). Through specific binding with Ag(I), the PtNPs hinder the catalase-like activity responsible for hydrogen peroxide (H2O2) decomposition. This inhibition enables the Fenton reaction between H2O2 and ferrous ions, generating highly oxidizing hydroxyl free radicals (·OH). The resulting etching of AuNRs induces a blue-shift in their local surface plasmon resonance (LSPR) absorption spectra. The degree of blue-shift is directly proportional to the Ag(I) concentration, facilitating trace-level detection. Furthermore, the aspect ratio change of the AuNRs yields distinguishable colors. In contrast to common multicolor sensors relying on nanozyme horseradish peroxidase (HRP) activity, which exhibits an inverse relationship between AuNR etching and target concentration, our approach demonstrates a proportional response. This unique characteristic enables ultrahigh-resolution multicolor detection of Ag(I) visible to the naked eye. We anticipate that this innovative sensing platform will pave the way for nanosensor development in environmental monitoring and food safety detection. Ultrahigh resolution Multicolor sensor Silver ion detection Gold nanorod Nanozyme Zhang, Hui verfasserin aut Liu, Jin verfasserin aut Zhang, Huifang verfasserin aut Hu, Xuan verfasserin aut Wang, Yu verfasserin aut Li, Xun verfasserin aut Xu, Jianguo verfasserin aut Enthalten in Sensors and actuators <Lausanne> / B Amsterdam [u.a.] : Elsevier Science, 1990 397 Online-Ressource (DE-627)306710358 (DE-600)1500731-5 (DE-576)082435855 0925-4005 nnns volume:397 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 50.22 Sensorik VZ 35.07 Chemisches Labor chemische Methoden VZ AR 397 |
allfieldsGer |
10.1016/j.snb.2023.134658 doi (DE-627)ELV065111087 (ELSEVIER)S0925-4005(23)01373-4 DE-627 ger DE-627 rda eng 530 620 VZ 50.22 bkl 35.07 bkl Ma, Xiaoming verfasserin aut An ultrahigh-resolution multicolor sensing platform via target-induced etching of gold nanorods for multi-colorimetric analysis of trace silver ions 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Heavy metal ion pollution is a pressing global concern with detrimental effects on the environment and human health. To address this issue, we have developed an ultrahigh-resolution multicolor sensing platform for the specific detection of silver ions (Ag(I)). The method employs the nanozyme of platinum nanoparticles (PtNPs) as a link to control the etching of gold nanorods (AuNRs). Through specific binding with Ag(I), the PtNPs hinder the catalase-like activity responsible for hydrogen peroxide (H2O2) decomposition. This inhibition enables the Fenton reaction between H2O2 and ferrous ions, generating highly oxidizing hydroxyl free radicals (·OH). The resulting etching of AuNRs induces a blue-shift in their local surface plasmon resonance (LSPR) absorption spectra. The degree of blue-shift is directly proportional to the Ag(I) concentration, facilitating trace-level detection. Furthermore, the aspect ratio change of the AuNRs yields distinguishable colors. In contrast to common multicolor sensors relying on nanozyme horseradish peroxidase (HRP) activity, which exhibits an inverse relationship between AuNR etching and target concentration, our approach demonstrates a proportional response. This unique characteristic enables ultrahigh-resolution multicolor detection of Ag(I) visible to the naked eye. We anticipate that this innovative sensing platform will pave the way for nanosensor development in environmental monitoring and food safety detection. Ultrahigh resolution Multicolor sensor Silver ion detection Gold nanorod Nanozyme Zhang, Hui verfasserin aut Liu, Jin verfasserin aut Zhang, Huifang verfasserin aut Hu, Xuan verfasserin aut Wang, Yu verfasserin aut Li, Xun verfasserin aut Xu, Jianguo verfasserin aut Enthalten in Sensors and actuators <Lausanne> / B Amsterdam [u.a.] : Elsevier Science, 1990 397 Online-Ressource (DE-627)306710358 (DE-600)1500731-5 (DE-576)082435855 0925-4005 nnns volume:397 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 50.22 Sensorik VZ 35.07 Chemisches Labor chemische Methoden VZ AR 397 |
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10.1016/j.snb.2023.134658 doi (DE-627)ELV065111087 (ELSEVIER)S0925-4005(23)01373-4 DE-627 ger DE-627 rda eng 530 620 VZ 50.22 bkl 35.07 bkl Ma, Xiaoming verfasserin aut An ultrahigh-resolution multicolor sensing platform via target-induced etching of gold nanorods for multi-colorimetric analysis of trace silver ions 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Heavy metal ion pollution is a pressing global concern with detrimental effects on the environment and human health. To address this issue, we have developed an ultrahigh-resolution multicolor sensing platform for the specific detection of silver ions (Ag(I)). The method employs the nanozyme of platinum nanoparticles (PtNPs) as a link to control the etching of gold nanorods (AuNRs). Through specific binding with Ag(I), the PtNPs hinder the catalase-like activity responsible for hydrogen peroxide (H2O2) decomposition. This inhibition enables the Fenton reaction between H2O2 and ferrous ions, generating highly oxidizing hydroxyl free radicals (·OH). The resulting etching of AuNRs induces a blue-shift in their local surface plasmon resonance (LSPR) absorption spectra. The degree of blue-shift is directly proportional to the Ag(I) concentration, facilitating trace-level detection. Furthermore, the aspect ratio change of the AuNRs yields distinguishable colors. In contrast to common multicolor sensors relying on nanozyme horseradish peroxidase (HRP) activity, which exhibits an inverse relationship between AuNR etching and target concentration, our approach demonstrates a proportional response. This unique characteristic enables ultrahigh-resolution multicolor detection of Ag(I) visible to the naked eye. We anticipate that this innovative sensing platform will pave the way for nanosensor development in environmental monitoring and food safety detection. Ultrahigh resolution Multicolor sensor Silver ion detection Gold nanorod Nanozyme Zhang, Hui verfasserin aut Liu, Jin verfasserin aut Zhang, Huifang verfasserin aut Hu, Xuan verfasserin aut Wang, Yu verfasserin aut Li, Xun verfasserin aut Xu, Jianguo verfasserin aut Enthalten in Sensors and actuators <Lausanne> / B Amsterdam [u.a.] : Elsevier Science, 1990 397 Online-Ressource (DE-627)306710358 (DE-600)1500731-5 (DE-576)082435855 0925-4005 nnns volume:397 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 50.22 Sensorik VZ 35.07 Chemisches Labor chemische Methoden VZ AR 397 |
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Ma, Xiaoming @@aut@@ Zhang, Hui @@aut@@ Liu, Jin @@aut@@ Zhang, Huifang @@aut@@ Hu, Xuan @@aut@@ Wang, Yu @@aut@@ Li, Xun @@aut@@ Xu, Jianguo @@aut@@ |
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2023-01-01T00:00:00Z |
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Ma, Xiaoming |
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Ma, Xiaoming ddc 530 bkl 50.22 bkl 35.07 misc Ultrahigh resolution misc Multicolor sensor misc Silver ion detection misc Gold nanorod misc Nanozyme An ultrahigh-resolution multicolor sensing platform via target-induced etching of gold nanorods for multi-colorimetric analysis of trace silver ions |
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530 620 VZ 50.22 bkl 35.07 bkl An ultrahigh-resolution multicolor sensing platform via target-induced etching of gold nanorods for multi-colorimetric analysis of trace silver ions Ultrahigh resolution Multicolor sensor Silver ion detection Gold nanorod Nanozyme |
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an ultrahigh-resolution multicolor sensing platform via target-induced etching of gold nanorods for multi-colorimetric analysis of trace silver ions |
title_auth |
An ultrahigh-resolution multicolor sensing platform via target-induced etching of gold nanorods for multi-colorimetric analysis of trace silver ions |
abstract |
Heavy metal ion pollution is a pressing global concern with detrimental effects on the environment and human health. To address this issue, we have developed an ultrahigh-resolution multicolor sensing platform for the specific detection of silver ions (Ag(I)). The method employs the nanozyme of platinum nanoparticles (PtNPs) as a link to control the etching of gold nanorods (AuNRs). Through specific binding with Ag(I), the PtNPs hinder the catalase-like activity responsible for hydrogen peroxide (H2O2) decomposition. This inhibition enables the Fenton reaction between H2O2 and ferrous ions, generating highly oxidizing hydroxyl free radicals (·OH). The resulting etching of AuNRs induces a blue-shift in their local surface plasmon resonance (LSPR) absorption spectra. The degree of blue-shift is directly proportional to the Ag(I) concentration, facilitating trace-level detection. Furthermore, the aspect ratio change of the AuNRs yields distinguishable colors. In contrast to common multicolor sensors relying on nanozyme horseradish peroxidase (HRP) activity, which exhibits an inverse relationship between AuNR etching and target concentration, our approach demonstrates a proportional response. This unique characteristic enables ultrahigh-resolution multicolor detection of Ag(I) visible to the naked eye. We anticipate that this innovative sensing platform will pave the way for nanosensor development in environmental monitoring and food safety detection. |
abstractGer |
Heavy metal ion pollution is a pressing global concern with detrimental effects on the environment and human health. To address this issue, we have developed an ultrahigh-resolution multicolor sensing platform for the specific detection of silver ions (Ag(I)). The method employs the nanozyme of platinum nanoparticles (PtNPs) as a link to control the etching of gold nanorods (AuNRs). Through specific binding with Ag(I), the PtNPs hinder the catalase-like activity responsible for hydrogen peroxide (H2O2) decomposition. This inhibition enables the Fenton reaction between H2O2 and ferrous ions, generating highly oxidizing hydroxyl free radicals (·OH). The resulting etching of AuNRs induces a blue-shift in their local surface plasmon resonance (LSPR) absorption spectra. The degree of blue-shift is directly proportional to the Ag(I) concentration, facilitating trace-level detection. Furthermore, the aspect ratio change of the AuNRs yields distinguishable colors. In contrast to common multicolor sensors relying on nanozyme horseradish peroxidase (HRP) activity, which exhibits an inverse relationship between AuNR etching and target concentration, our approach demonstrates a proportional response. This unique characteristic enables ultrahigh-resolution multicolor detection of Ag(I) visible to the naked eye. We anticipate that this innovative sensing platform will pave the way for nanosensor development in environmental monitoring and food safety detection. |
abstract_unstemmed |
Heavy metal ion pollution is a pressing global concern with detrimental effects on the environment and human health. To address this issue, we have developed an ultrahigh-resolution multicolor sensing platform for the specific detection of silver ions (Ag(I)). The method employs the nanozyme of platinum nanoparticles (PtNPs) as a link to control the etching of gold nanorods (AuNRs). Through specific binding with Ag(I), the PtNPs hinder the catalase-like activity responsible for hydrogen peroxide (H2O2) decomposition. This inhibition enables the Fenton reaction between H2O2 and ferrous ions, generating highly oxidizing hydroxyl free radicals (·OH). The resulting etching of AuNRs induces a blue-shift in their local surface plasmon resonance (LSPR) absorption spectra. The degree of blue-shift is directly proportional to the Ag(I) concentration, facilitating trace-level detection. Furthermore, the aspect ratio change of the AuNRs yields distinguishable colors. In contrast to common multicolor sensors relying on nanozyme horseradish peroxidase (HRP) activity, which exhibits an inverse relationship between AuNR etching and target concentration, our approach demonstrates a proportional response. This unique characteristic enables ultrahigh-resolution multicolor detection of Ag(I) visible to the naked eye. We anticipate that this innovative sensing platform will pave the way for nanosensor development in environmental monitoring and food safety detection. |
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An ultrahigh-resolution multicolor sensing platform via target-induced etching of gold nanorods for multi-colorimetric analysis of trace silver ions |
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|
score |
7.399987 |