Selective enrichment strategy induces ultra-broadband NIR emission in Cr

Near-infrared (NIR) spectroscopy has gained widespread application in food analysis, disease diagnosis, fingerprint analysis, and security monitoring. However, the lack of efficient, broadband NIR luminescent materials hinders the full potential of this technology. Here, an ultra-broadband and high-...
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Autor*in:	Liu, Weizhen [verfasserIn] Xiao, Zongliang [verfasserIn] Li, Lei [verfasserIn] Wen, Zhiqiang [verfasserIn] Xu, Xiangwei [verfasserIn] Qin, Shikun [verfasserIn] Huang, Jianhui [verfasserIn] You, Weixiong [verfasserIn] Han, Lei [verfasserIn] Yu, Jingbo [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Cr Multi-phase glass-ceramics NIR lighting sources Ultra-broadband NIR emission

Übergeordnetes Werk:	Enthalten in: Ceramics international - Amsterdam [u.a.] : Elsevier Science, 1995, 49, Seite 38318-38330
Übergeordnetes Werk:	volume:49 ; pages:38318-38330

DOI / URN:	10.1016/j.ceramint.2023.09.164

Katalog-ID:	ELV065204085

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520			\|a Near-infrared (NIR) spectroscopy has gained widespread application in food analysis, disease diagnosis, fingerprint analysis, and security monitoring. However, the lack of efficient, broadband NIR luminescent materials hinders the full potential of this technology. Here, an ultra-broadband and high-efficiency Cr3+-doped multi-phase glass-ceramics containing MgAl2O4, Al2SiO5, and SiO2 nanocrystals was discovered, which exhibited an ultra-broadband NIR emission (λem ∼ 900 nm) with a full width at half maximum more than 300 nm and a high internal quantum yield of 50.9% under the excitation of 465 nm blue light. Moreover, the integrated emission intensity at 100 °C and 150 °C can keep 88% and 77% of that at room temperature. The ultra-broadband, high efficiency, and thermally robust luminescence of this Cr3+-doped multi-phase glass-ceramics can be attributed to the selective enrichment of Cr3+ ions into different nanocrystals with octahedral sites, and medium electron-photon coupling effect. The NIR glass-ceramics-converted light-emitting diode constructed by the glass-ceramics combined with 465 blue LED chip produced an excellent NIR output and photoelectric conversion efficiency of 274 mW/1007 mW and 3.43%/2.79% at 100 mA/320 mA drive current, which demonstrated superior overall performance to the NIR device built by using the well-known NIR phosphors. Additionally, the NIR camera can capture the image of license plate and nectarine, as well as identify the residual drug content in the bottle under the irradiation of the NIR device constructed by the glass-ceramics. This work not only presented an ultra-broadband and high-efficiency NIR material but also highlights a design strategy to effectively enhance the efficiency and broadband characteristics of NIR glass-ceramics.
650		4	\|a Cr
650		4	\|a Multi-phase glass-ceramics
650		4	\|a NIR lighting sources
650		4	\|a Ultra-broadband NIR emission
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700	1		\|a Qin, Shikun \|e verfasserin \|4 aut
700	1		\|a Huang, Jianhui \|e verfasserin \|4 aut
700	1		\|a You, Weixiong \|e verfasserin \|4 aut
700	1		\|a Han, Lei \|e verfasserin \|0 (orcid)0000-0003-1474-3131 \|4 aut
700	1		\|a Yu, Jingbo \|e verfasserin \|4 aut
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allfields	10.1016/j.ceramint.2023.09.164 doi (DE-627)ELV065204085 (ELSEVIER)S0272-8842(23)02790-6 DE-627 ger DE-627 rda eng 670 VZ 51.60 bkl 58.45 bkl Liu, Weizhen verfasserin aut Selective enrichment strategy induces ultra-broadband NIR emission in Cr 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Near-infrared (NIR) spectroscopy has gained widespread application in food analysis, disease diagnosis, fingerprint analysis, and security monitoring. However, the lack of efficient, broadband NIR luminescent materials hinders the full potential of this technology. Here, an ultra-broadband and high-efficiency Cr3+-doped multi-phase glass-ceramics containing MgAl2O4, Al2SiO5, and SiO2 nanocrystals was discovered, which exhibited an ultra-broadband NIR emission (λem ∼ 900 nm) with a full width at half maximum more than 300 nm and a high internal quantum yield of 50.9% under the excitation of 465 nm blue light. Moreover, the integrated emission intensity at 100 °C and 150 °C can keep 88% and 77% of that at room temperature. The ultra-broadband, high efficiency, and thermally robust luminescence of this Cr3+-doped multi-phase glass-ceramics can be attributed to the selective enrichment of Cr3+ ions into different nanocrystals with octahedral sites, and medium electron-photon coupling effect. The NIR glass-ceramics-converted light-emitting diode constructed by the glass-ceramics combined with 465 blue LED chip produced an excellent NIR output and photoelectric conversion efficiency of 274 mW/1007 mW and 3.43%/2.79% at 100 mA/320 mA drive current, which demonstrated superior overall performance to the NIR device built by using the well-known NIR phosphors. Additionally, the NIR camera can capture the image of license plate and nectarine, as well as identify the residual drug content in the bottle under the irradiation of the NIR device constructed by the glass-ceramics. This work not only presented an ultra-broadband and high-efficiency NIR material but also highlights a design strategy to effectively enhance the efficiency and broadband characteristics of NIR glass-ceramics. Cr Multi-phase glass-ceramics NIR lighting sources Ultra-broadband NIR emission Xiao, Zongliang verfasserin aut Li, Lei verfasserin aut Wen, Zhiqiang verfasserin aut Xu, Xiangwei verfasserin aut Qin, Shikun verfasserin aut Huang, Jianhui verfasserin aut You, Weixiong verfasserin aut Han, Lei verfasserin (orcid)0000-0003-1474-3131 aut Yu, Jingbo verfasserin aut Enthalten in Ceramics international Amsterdam [u.a.] : Elsevier Science, 1995 49, Seite 38318-38330 Online-Ressource (DE-627)320584305 (DE-600)2018052-4 (DE-576)25523063X 0272-8842 nnns volume:49 pages:38318-38330 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.60 Keramische Werkstoffe Hartstoffe Werkstoffkunde VZ 58.45 Gesteinshüttenkunde VZ AR 49 38318-38330
spelling	10.1016/j.ceramint.2023.09.164 doi (DE-627)ELV065204085 (ELSEVIER)S0272-8842(23)02790-6 DE-627 ger DE-627 rda eng 670 VZ 51.60 bkl 58.45 bkl Liu, Weizhen verfasserin aut Selective enrichment strategy induces ultra-broadband NIR emission in Cr 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Near-infrared (NIR) spectroscopy has gained widespread application in food analysis, disease diagnosis, fingerprint analysis, and security monitoring. However, the lack of efficient, broadband NIR luminescent materials hinders the full potential of this technology. Here, an ultra-broadband and high-efficiency Cr3+-doped multi-phase glass-ceramics containing MgAl2O4, Al2SiO5, and SiO2 nanocrystals was discovered, which exhibited an ultra-broadband NIR emission (λem ∼ 900 nm) with a full width at half maximum more than 300 nm and a high internal quantum yield of 50.9% under the excitation of 465 nm blue light. Moreover, the integrated emission intensity at 100 °C and 150 °C can keep 88% and 77% of that at room temperature. The ultra-broadband, high efficiency, and thermally robust luminescence of this Cr3+-doped multi-phase glass-ceramics can be attributed to the selective enrichment of Cr3+ ions into different nanocrystals with octahedral sites, and medium electron-photon coupling effect. The NIR glass-ceramics-converted light-emitting diode constructed by the glass-ceramics combined with 465 blue LED chip produced an excellent NIR output and photoelectric conversion efficiency of 274 mW/1007 mW and 3.43%/2.79% at 100 mA/320 mA drive current, which demonstrated superior overall performance to the NIR device built by using the well-known NIR phosphors. Additionally, the NIR camera can capture the image of license plate and nectarine, as well as identify the residual drug content in the bottle under the irradiation of the NIR device constructed by the glass-ceramics. This work not only presented an ultra-broadband and high-efficiency NIR material but also highlights a design strategy to effectively enhance the efficiency and broadband characteristics of NIR glass-ceramics. Cr Multi-phase glass-ceramics NIR lighting sources Ultra-broadband NIR emission Xiao, Zongliang verfasserin aut Li, Lei verfasserin aut Wen, Zhiqiang verfasserin aut Xu, Xiangwei verfasserin aut Qin, Shikun verfasserin aut Huang, Jianhui verfasserin aut You, Weixiong verfasserin aut Han, Lei verfasserin (orcid)0000-0003-1474-3131 aut Yu, Jingbo verfasserin aut Enthalten in Ceramics international Amsterdam [u.a.] : Elsevier Science, 1995 49, Seite 38318-38330 Online-Ressource (DE-627)320584305 (DE-600)2018052-4 (DE-576)25523063X 0272-8842 nnns volume:49 pages:38318-38330 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.60 Keramische Werkstoffe Hartstoffe Werkstoffkunde VZ 58.45 Gesteinshüttenkunde VZ AR 49 38318-38330
allfields_unstemmed	10.1016/j.ceramint.2023.09.164 doi (DE-627)ELV065204085 (ELSEVIER)S0272-8842(23)02790-6 DE-627 ger DE-627 rda eng 670 VZ 51.60 bkl 58.45 bkl Liu, Weizhen verfasserin aut Selective enrichment strategy induces ultra-broadband NIR emission in Cr 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Near-infrared (NIR) spectroscopy has gained widespread application in food analysis, disease diagnosis, fingerprint analysis, and security monitoring. However, the lack of efficient, broadband NIR luminescent materials hinders the full potential of this technology. Here, an ultra-broadband and high-efficiency Cr3+-doped multi-phase glass-ceramics containing MgAl2O4, Al2SiO5, and SiO2 nanocrystals was discovered, which exhibited an ultra-broadband NIR emission (λem ∼ 900 nm) with a full width at half maximum more than 300 nm and a high internal quantum yield of 50.9% under the excitation of 465 nm blue light. Moreover, the integrated emission intensity at 100 °C and 150 °C can keep 88% and 77% of that at room temperature. The ultra-broadband, high efficiency, and thermally robust luminescence of this Cr3+-doped multi-phase glass-ceramics can be attributed to the selective enrichment of Cr3+ ions into different nanocrystals with octahedral sites, and medium electron-photon coupling effect. The NIR glass-ceramics-converted light-emitting diode constructed by the glass-ceramics combined with 465 blue LED chip produced an excellent NIR output and photoelectric conversion efficiency of 274 mW/1007 mW and 3.43%/2.79% at 100 mA/320 mA drive current, which demonstrated superior overall performance to the NIR device built by using the well-known NIR phosphors. Additionally, the NIR camera can capture the image of license plate and nectarine, as well as identify the residual drug content in the bottle under the irradiation of the NIR device constructed by the glass-ceramics. This work not only presented an ultra-broadband and high-efficiency NIR material but also highlights a design strategy to effectively enhance the efficiency and broadband characteristics of NIR glass-ceramics. Cr Multi-phase glass-ceramics NIR lighting sources Ultra-broadband NIR emission Xiao, Zongliang verfasserin aut Li, Lei verfasserin aut Wen, Zhiqiang verfasserin aut Xu, Xiangwei verfasserin aut Qin, Shikun verfasserin aut Huang, Jianhui verfasserin aut You, Weixiong verfasserin aut Han, Lei verfasserin (orcid)0000-0003-1474-3131 aut Yu, Jingbo verfasserin aut Enthalten in Ceramics international Amsterdam [u.a.] : Elsevier Science, 1995 49, Seite 38318-38330 Online-Ressource (DE-627)320584305 (DE-600)2018052-4 (DE-576)25523063X 0272-8842 nnns volume:49 pages:38318-38330 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.60 Keramische Werkstoffe Hartstoffe Werkstoffkunde VZ 58.45 Gesteinshüttenkunde VZ AR 49 38318-38330
allfieldsGer	10.1016/j.ceramint.2023.09.164 doi (DE-627)ELV065204085 (ELSEVIER)S0272-8842(23)02790-6 DE-627 ger DE-627 rda eng 670 VZ 51.60 bkl 58.45 bkl Liu, Weizhen verfasserin aut Selective enrichment strategy induces ultra-broadband NIR emission in Cr 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Near-infrared (NIR) spectroscopy has gained widespread application in food analysis, disease diagnosis, fingerprint analysis, and security monitoring. However, the lack of efficient, broadband NIR luminescent materials hinders the full potential of this technology. Here, an ultra-broadband and high-efficiency Cr3+-doped multi-phase glass-ceramics containing MgAl2O4, Al2SiO5, and SiO2 nanocrystals was discovered, which exhibited an ultra-broadband NIR emission (λem ∼ 900 nm) with a full width at half maximum more than 300 nm and a high internal quantum yield of 50.9% under the excitation of 465 nm blue light. Moreover, the integrated emission intensity at 100 °C and 150 °C can keep 88% and 77% of that at room temperature. The ultra-broadband, high efficiency, and thermally robust luminescence of this Cr3+-doped multi-phase glass-ceramics can be attributed to the selective enrichment of Cr3+ ions into different nanocrystals with octahedral sites, and medium electron-photon coupling effect. The NIR glass-ceramics-converted light-emitting diode constructed by the glass-ceramics combined with 465 blue LED chip produced an excellent NIR output and photoelectric conversion efficiency of 274 mW/1007 mW and 3.43%/2.79% at 100 mA/320 mA drive current, which demonstrated superior overall performance to the NIR device built by using the well-known NIR phosphors. Additionally, the NIR camera can capture the image of license plate and nectarine, as well as identify the residual drug content in the bottle under the irradiation of the NIR device constructed by the glass-ceramics. This work not only presented an ultra-broadband and high-efficiency NIR material but also highlights a design strategy to effectively enhance the efficiency and broadband characteristics of NIR glass-ceramics. Cr Multi-phase glass-ceramics NIR lighting sources Ultra-broadband NIR emission Xiao, Zongliang verfasserin aut Li, Lei verfasserin aut Wen, Zhiqiang verfasserin aut Xu, Xiangwei verfasserin aut Qin, Shikun verfasserin aut Huang, Jianhui verfasserin aut You, Weixiong verfasserin aut Han, Lei verfasserin (orcid)0000-0003-1474-3131 aut Yu, Jingbo verfasserin aut Enthalten in Ceramics international Amsterdam [u.a.] : Elsevier Science, 1995 49, Seite 38318-38330 Online-Ressource (DE-627)320584305 (DE-600)2018052-4 (DE-576)25523063X 0272-8842 nnns volume:49 pages:38318-38330 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.60 Keramische Werkstoffe Hartstoffe Werkstoffkunde VZ 58.45 Gesteinshüttenkunde VZ AR 49 38318-38330
allfieldsSound	10.1016/j.ceramint.2023.09.164 doi (DE-627)ELV065204085 (ELSEVIER)S0272-8842(23)02790-6 DE-627 ger DE-627 rda eng 670 VZ 51.60 bkl 58.45 bkl Liu, Weizhen verfasserin aut Selective enrichment strategy induces ultra-broadband NIR emission in Cr 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Near-infrared (NIR) spectroscopy has gained widespread application in food analysis, disease diagnosis, fingerprint analysis, and security monitoring. However, the lack of efficient, broadband NIR luminescent materials hinders the full potential of this technology. Here, an ultra-broadband and high-efficiency Cr3+-doped multi-phase glass-ceramics containing MgAl2O4, Al2SiO5, and SiO2 nanocrystals was discovered, which exhibited an ultra-broadband NIR emission (λem ∼ 900 nm) with a full width at half maximum more than 300 nm and a high internal quantum yield of 50.9% under the excitation of 465 nm blue light. Moreover, the integrated emission intensity at 100 °C and 150 °C can keep 88% and 77% of that at room temperature. The ultra-broadband, high efficiency, and thermally robust luminescence of this Cr3+-doped multi-phase glass-ceramics can be attributed to the selective enrichment of Cr3+ ions into different nanocrystals with octahedral sites, and medium electron-photon coupling effect. The NIR glass-ceramics-converted light-emitting diode constructed by the glass-ceramics combined with 465 blue LED chip produced an excellent NIR output and photoelectric conversion efficiency of 274 mW/1007 mW and 3.43%/2.79% at 100 mA/320 mA drive current, which demonstrated superior overall performance to the NIR device built by using the well-known NIR phosphors. Additionally, the NIR camera can capture the image of license plate and nectarine, as well as identify the residual drug content in the bottle under the irradiation of the NIR device constructed by the glass-ceramics. This work not only presented an ultra-broadband and high-efficiency NIR material but also highlights a design strategy to effectively enhance the efficiency and broadband characteristics of NIR glass-ceramics. Cr Multi-phase glass-ceramics NIR lighting sources Ultra-broadband NIR emission Xiao, Zongliang verfasserin aut Li, Lei verfasserin aut Wen, Zhiqiang verfasserin aut Xu, Xiangwei verfasserin aut Qin, Shikun verfasserin aut Huang, Jianhui verfasserin aut You, Weixiong verfasserin aut Han, Lei verfasserin (orcid)0000-0003-1474-3131 aut Yu, Jingbo verfasserin aut Enthalten in Ceramics international Amsterdam [u.a.] : Elsevier Science, 1995 49, Seite 38318-38330 Online-Ressource (DE-627)320584305 (DE-600)2018052-4 (DE-576)25523063X 0272-8842 nnns volume:49 pages:38318-38330 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.60 Keramische Werkstoffe Hartstoffe Werkstoffkunde VZ 58.45 Gesteinshüttenkunde VZ AR 49 38318-38330
language	English
source	Enthalten in Ceramics international 49, Seite 38318-38330 volume:49 pages:38318-38330
sourceStr	Enthalten in Ceramics international 49, Seite 38318-38330 volume:49 pages:38318-38330
format_phy_str_mv	Article
bklname	Keramische Werkstoffe Hartstoffe Gesteinshüttenkunde
institution	findex.gbv.de
topic_facet	Cr Multi-phase glass-ceramics NIR lighting sources Ultra-broadband NIR emission
dewey-raw	670
isfreeaccess_bool	false
container_title	Ceramics international
authorswithroles_txt_mv	Liu, Weizhen @@aut@@ Xiao, Zongliang @@aut@@ Li, Lei @@aut@@ Wen, Zhiqiang @@aut@@ Xu, Xiangwei @@aut@@ Qin, Shikun @@aut@@ Huang, Jianhui @@aut@@ You, Weixiong @@aut@@ Han, Lei @@aut@@ Yu, Jingbo @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	320584305
dewey-sort	3670
id	ELV065204085
language_de	englisch
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author	Liu, Weizhen
spellingShingle	Liu, Weizhen ddc 670 bkl 51.60 bkl 58.45 misc Cr misc Multi-phase glass-ceramics misc NIR lighting sources misc Ultra-broadband NIR emission Selective enrichment strategy induces ultra-broadband NIR emission in Cr
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topic_title	670 VZ 51.60 bkl 58.45 bkl Selective enrichment strategy induces ultra-broadband NIR emission in Cr Cr Multi-phase glass-ceramics NIR lighting sources Ultra-broadband NIR emission
topic	ddc 670 bkl 51.60 bkl 58.45 misc Cr misc Multi-phase glass-ceramics misc NIR lighting sources misc Ultra-broadband NIR emission
topic_unstemmed	ddc 670 bkl 51.60 bkl 58.45 misc Cr misc Multi-phase glass-ceramics misc NIR lighting sources misc Ultra-broadband NIR emission
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title	Selective enrichment strategy induces ultra-broadband NIR emission in Cr
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title_full	Selective enrichment strategy induces ultra-broadband NIR emission in Cr
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title_sort	selective enrichment strategy induces ultra-broadband nir emission in cr
title_auth	Selective enrichment strategy induces ultra-broadband NIR emission in Cr
abstract	Near-infrared (NIR) spectroscopy has gained widespread application in food analysis, disease diagnosis, fingerprint analysis, and security monitoring. However, the lack of efficient, broadband NIR luminescent materials hinders the full potential of this technology. Here, an ultra-broadband and high-efficiency Cr3+-doped multi-phase glass-ceramics containing MgAl2O4, Al2SiO5, and SiO2 nanocrystals was discovered, which exhibited an ultra-broadband NIR emission (λem ∼ 900 nm) with a full width at half maximum more than 300 nm and a high internal quantum yield of 50.9% under the excitation of 465 nm blue light. Moreover, the integrated emission intensity at 100 °C and 150 °C can keep 88% and 77% of that at room temperature. The ultra-broadband, high efficiency, and thermally robust luminescence of this Cr3+-doped multi-phase glass-ceramics can be attributed to the selective enrichment of Cr3+ ions into different nanocrystals with octahedral sites, and medium electron-photon coupling effect. The NIR glass-ceramics-converted light-emitting diode constructed by the glass-ceramics combined with 465 blue LED chip produced an excellent NIR output and photoelectric conversion efficiency of 274 mW/1007 mW and 3.43%/2.79% at 100 mA/320 mA drive current, which demonstrated superior overall performance to the NIR device built by using the well-known NIR phosphors. Additionally, the NIR camera can capture the image of license plate and nectarine, as well as identify the residual drug content in the bottle under the irradiation of the NIR device constructed by the glass-ceramics. This work not only presented an ultra-broadband and high-efficiency NIR material but also highlights a design strategy to effectively enhance the efficiency and broadband characteristics of NIR glass-ceramics.
abstractGer	Near-infrared (NIR) spectroscopy has gained widespread application in food analysis, disease diagnosis, fingerprint analysis, and security monitoring. However, the lack of efficient, broadband NIR luminescent materials hinders the full potential of this technology. Here, an ultra-broadband and high-efficiency Cr3+-doped multi-phase glass-ceramics containing MgAl2O4, Al2SiO5, and SiO2 nanocrystals was discovered, which exhibited an ultra-broadband NIR emission (λem ∼ 900 nm) with a full width at half maximum more than 300 nm and a high internal quantum yield of 50.9% under the excitation of 465 nm blue light. Moreover, the integrated emission intensity at 100 °C and 150 °C can keep 88% and 77% of that at room temperature. The ultra-broadband, high efficiency, and thermally robust luminescence of this Cr3+-doped multi-phase glass-ceramics can be attributed to the selective enrichment of Cr3+ ions into different nanocrystals with octahedral sites, and medium electron-photon coupling effect. The NIR glass-ceramics-converted light-emitting diode constructed by the glass-ceramics combined with 465 blue LED chip produced an excellent NIR output and photoelectric conversion efficiency of 274 mW/1007 mW and 3.43%/2.79% at 100 mA/320 mA drive current, which demonstrated superior overall performance to the NIR device built by using the well-known NIR phosphors. Additionally, the NIR camera can capture the image of license plate and nectarine, as well as identify the residual drug content in the bottle under the irradiation of the NIR device constructed by the glass-ceramics. This work not only presented an ultra-broadband and high-efficiency NIR material but also highlights a design strategy to effectively enhance the efficiency and broadband characteristics of NIR glass-ceramics.
abstract_unstemmed	Near-infrared (NIR) spectroscopy has gained widespread application in food analysis, disease diagnosis, fingerprint analysis, and security monitoring. However, the lack of efficient, broadband NIR luminescent materials hinders the full potential of this technology. Here, an ultra-broadband and high-efficiency Cr3+-doped multi-phase glass-ceramics containing MgAl2O4, Al2SiO5, and SiO2 nanocrystals was discovered, which exhibited an ultra-broadband NIR emission (λem ∼ 900 nm) with a full width at half maximum more than 300 nm and a high internal quantum yield of 50.9% under the excitation of 465 nm blue light. Moreover, the integrated emission intensity at 100 °C and 150 °C can keep 88% and 77% of that at room temperature. The ultra-broadband, high efficiency, and thermally robust luminescence of this Cr3+-doped multi-phase glass-ceramics can be attributed to the selective enrichment of Cr3+ ions into different nanocrystals with octahedral sites, and medium electron-photon coupling effect. The NIR glass-ceramics-converted light-emitting diode constructed by the glass-ceramics combined with 465 blue LED chip produced an excellent NIR output and photoelectric conversion efficiency of 274 mW/1007 mW and 3.43%/2.79% at 100 mA/320 mA drive current, which demonstrated superior overall performance to the NIR device built by using the well-known NIR phosphors. Additionally, the NIR camera can capture the image of license plate and nectarine, as well as identify the residual drug content in the bottle under the irradiation of the NIR device constructed by the glass-ceramics. This work not only presented an ultra-broadband and high-efficiency NIR material but also highlights a design strategy to effectively enhance the efficiency and broadband characteristics of NIR glass-ceramics.
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title_short	Selective enrichment strategy induces ultra-broadband NIR emission in Cr
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author2	Xiao, Zongliang Li, Lei Wen, Zhiqiang Xu, Xiangwei Qin, Shikun Huang, Jianhui You, Weixiong Han, Lei Yu, Jingbo
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doi_str	10.1016/j.ceramint.2023.09.164
up_date	2024-07-06T22:12:13.594Z
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fullrecord_marcxml	<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000naa a22002652 4500</leader><controlfield tag="001">ELV065204085</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20231020093235.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">231020s2023 xx \|\|\|\|\|o 00\| \|\|eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1016/j.ceramint.2023.09.164</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)ELV065204085</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(ELSEVIER)S0272-8842(23)02790-6</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rda</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="082" ind1="0" ind2="4"><subfield code="a">670</subfield><subfield code="q">VZ</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">51.60</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">58.45</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Liu, Weizhen</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Selective enrichment strategy induces ultra-broadband NIR emission in Cr</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2023</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">nicht spezifiziert</subfield><subfield code="b">zzz</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Near-infrared (NIR) spectroscopy has gained widespread application in food analysis, disease diagnosis, fingerprint analysis, and security monitoring. However, the lack of efficient, broadband NIR luminescent materials hinders the full potential of this technology. Here, an ultra-broadband and high-efficiency Cr3+-doped multi-phase glass-ceramics containing MgAl2O4, Al2SiO5, and SiO2 nanocrystals was discovered, which exhibited an ultra-broadband NIR emission (λem ∼ 900 nm) with a full width at half maximum more than 300 nm and a high internal quantum yield of 50.9% under the excitation of 465 nm blue light. Moreover, the integrated emission intensity at 100 °C and 150 °C can keep 88% and 77% of that at room temperature. The ultra-broadband, high efficiency, and thermally robust luminescence of this Cr3+-doped multi-phase glass-ceramics can be attributed to the selective enrichment of Cr3+ ions into different nanocrystals with octahedral sites, and medium electron-photon coupling effect. The NIR glass-ceramics-converted light-emitting diode constructed by the glass-ceramics combined with 465 blue LED chip produced an excellent NIR output and photoelectric conversion efficiency of 274 mW/1007 mW and 3.43%/2.79% at 100 mA/320 mA drive current, which demonstrated superior overall performance to the NIR device built by using the well-known NIR phosphors. Additionally, the NIR camera can capture the image of license plate and nectarine, as well as identify the residual drug content in the bottle under the irradiation of the NIR device constructed by the glass-ceramics. This work not only presented an ultra-broadband and high-efficiency NIR material but also highlights a design strategy to effectively enhance the efficiency and broadband characteristics of NIR glass-ceramics.</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Cr</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Multi-phase glass-ceramics</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">NIR lighting sources</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Ultra-broadband NIR emission</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Xiao, Zongliang</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Li, Lei</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" 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Selective enrichment strategy induces ultra-broadband NIR emission in Cr

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