Solid–solid thermal synthesis of bimetallic Ni/Zn embedded in N-doped porous carbon for efficient adsorptive separation based on CO

High-efficient adsorptive materials for carbon dioxide (CO2) capture and separation of a gas mixture are vital for energy consumption and emission reduction but are still a substantial challenge. A facile synthesis of bimetallic nickel/zinc embedded in N-doped carbon (Ni/ZnNC) through the solid–soli...
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Gespeichert in:

Autor*in:	Chaemchuen, Somboon [verfasserIn] Cheng, Zhonghan [verfasserIn] Hou, Xiaotong [verfasserIn] Verpoort, Francis [verfasserIn] Kumsi, Jakkapan [verfasserIn] Klomkliang, Nikom [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Solid–solid thermal method Ni/Zn@NC Solvent-free synthesis Carbon adsorbent CO

Übergeordnetes Werk:	Enthalten in: Fuel - New York, NY [u.a.] : Elsevier, 1970, 356
Übergeordnetes Werk:	volume:356

DOI / URN:	10.1016/j.fuel.2023.129608

Katalog-ID:	ELV065394208

Internformat


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024	7		\|a 10.1016/j.fuel.2023.129608 \|2 doi
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100	1		\|a Chaemchuen, Somboon \|e verfasserin \|0 (orcid)0000-0001-9936-0919 \|4 aut
245	1	0	\|a Solid–solid thermal synthesis of bimetallic Ni/Zn embedded in N-doped porous carbon for efficient adsorptive separation based on CO
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520			\|a High-efficient adsorptive materials for carbon dioxide (CO2) capture and separation of a gas mixture are vital for energy consumption and emission reduction but are still a substantial challenge. A facile synthesis of bimetallic nickel/zinc embedded in N-doped carbon (Ni/ZnNC) through the solid–solid thermal method (SST) is developed herein. The SST method is a straightforward procedure with the advantage that the materials are obtained in a single step and solvent-free conditions. Thermal analysis and material characterization were used to investigate the synthesis mechanism during the SST process. The results revealed that an intermediate material, initially obtained at a low thermal temperature, was sacrificed to generate Ni/Zn@NC at high temperatures of the SST method. The resulting robust carbon structure, decorated with heteroatoms (Ni, Zn, N), exhibits a potential for efficient CO2 adsorption during the capture and separation of biogas (CO2/CH4), off-gas (CO2/N2), and natural gas (CH4/ N2). The synergetic effect of Ni in the materials enhances the selectivity of SCO2/CH4 , SCO2/N2, and SCH4/N2 . The improved selectivities by effective sites were confirmed by computational modeling. Significantly, the Ni/Zn@NC material obtained through a mild yet simple synthesis method (SST) exhibits substantially higher CO2 adsorption capacity and selectivity when compared to commercial carbon (activated charcoal).
650		4	\|a Solid–solid thermal method
650		4	\|a Ni/Zn@NC
650		4	\|a Solvent-free synthesis
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650		4	\|a CO
650		4	\|a CO
700	1		\|a Cheng, Zhonghan \|e verfasserin \|4 aut
700	1		\|a Hou, Xiaotong \|e verfasserin \|4 aut
700	1		\|a Verpoort, Francis \|e verfasserin \|0 (orcid)0000-0002-5184-5500 \|4 aut
700	1		\|a Kumsi, Jakkapan \|e verfasserin \|4 aut
700	1		\|a Klomkliang, Nikom \|e verfasserin \|0 (orcid)0000-0001-8834-6011 \|4 aut
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936	b	k	\|a 58.21 \|j Brennstoffe \|j Kraftstoffe \|j Explosivstoffe \|q VZ
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publishDate	2023
allfields	10.1016/j.fuel.2023.129608 doi (DE-627)ELV065394208 (ELSEVIER)S0016-2361(23)02222-6 DE-627 ger DE-627 rda eng 660 VZ 58.21 bkl Chaemchuen, Somboon verfasserin (orcid)0000-0001-9936-0919 aut Solid–solid thermal synthesis of bimetallic Ni/Zn embedded in N-doped porous carbon for efficient adsorptive separation based on CO 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier High-efficient adsorptive materials for carbon dioxide (CO2) capture and separation of a gas mixture are vital for energy consumption and emission reduction but are still a substantial challenge. A facile synthesis of bimetallic nickel/zinc embedded in N-doped carbon (Ni/ZnNC) through the solid–solid thermal method (SST) is developed herein. The SST method is a straightforward procedure with the advantage that the materials are obtained in a single step and solvent-free conditions. Thermal analysis and material characterization were used to investigate the synthesis mechanism during the SST process. The results revealed that an intermediate material, initially obtained at a low thermal temperature, was sacrificed to generate Ni/Zn@NC at high temperatures of the SST method. The resulting robust carbon structure, decorated with heteroatoms (Ni, Zn, N), exhibits a potential for efficient CO2 adsorption during the capture and separation of biogas (CO2/CH4), off-gas (CO2/N2), and natural gas (CH4/ N2). The synergetic effect of Ni in the materials enhances the selectivity of SCO2/CH4 , SCO2/N2, and SCH4/N2 . The improved selectivities by effective sites were confirmed by computational modeling. Significantly, the Ni/Zn@NC material obtained through a mild yet simple synthesis method (SST) exhibits substantially higher CO2 adsorption capacity and selectivity when compared to commercial carbon (activated charcoal). Solid–solid thermal method Ni/Zn@NC Solvent-free synthesis Carbon adsorbent CO CO Cheng, Zhonghan verfasserin aut Hou, Xiaotong verfasserin aut Verpoort, Francis verfasserin (orcid)0000-0002-5184-5500 aut Kumsi, Jakkapan verfasserin aut Klomkliang, Nikom verfasserin (orcid)0000-0001-8834-6011 aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 356 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:356 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.21 Brennstoffe Kraftstoffe Explosivstoffe VZ AR 356
spelling	10.1016/j.fuel.2023.129608 doi (DE-627)ELV065394208 (ELSEVIER)S0016-2361(23)02222-6 DE-627 ger DE-627 rda eng 660 VZ 58.21 bkl Chaemchuen, Somboon verfasserin (orcid)0000-0001-9936-0919 aut Solid–solid thermal synthesis of bimetallic Ni/Zn embedded in N-doped porous carbon for efficient adsorptive separation based on CO 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier High-efficient adsorptive materials for carbon dioxide (CO2) capture and separation of a gas mixture are vital for energy consumption and emission reduction but are still a substantial challenge. A facile synthesis of bimetallic nickel/zinc embedded in N-doped carbon (Ni/ZnNC) through the solid–solid thermal method (SST) is developed herein. The SST method is a straightforward procedure with the advantage that the materials are obtained in a single step and solvent-free conditions. Thermal analysis and material characterization were used to investigate the synthesis mechanism during the SST process. The results revealed that an intermediate material, initially obtained at a low thermal temperature, was sacrificed to generate Ni/Zn@NC at high temperatures of the SST method. The resulting robust carbon structure, decorated with heteroatoms (Ni, Zn, N), exhibits a potential for efficient CO2 adsorption during the capture and separation of biogas (CO2/CH4), off-gas (CO2/N2), and natural gas (CH4/ N2). The synergetic effect of Ni in the materials enhances the selectivity of SCO2/CH4 , SCO2/N2, and SCH4/N2 . The improved selectivities by effective sites were confirmed by computational modeling. Significantly, the Ni/Zn@NC material obtained through a mild yet simple synthesis method (SST) exhibits substantially higher CO2 adsorption capacity and selectivity when compared to commercial carbon (activated charcoal). Solid–solid thermal method Ni/Zn@NC Solvent-free synthesis Carbon adsorbent CO CO Cheng, Zhonghan verfasserin aut Hou, Xiaotong verfasserin aut Verpoort, Francis verfasserin (orcid)0000-0002-5184-5500 aut Kumsi, Jakkapan verfasserin aut Klomkliang, Nikom verfasserin (orcid)0000-0001-8834-6011 aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 356 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:356 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.21 Brennstoffe Kraftstoffe Explosivstoffe VZ AR 356
allfields_unstemmed	10.1016/j.fuel.2023.129608 doi (DE-627)ELV065394208 (ELSEVIER)S0016-2361(23)02222-6 DE-627 ger DE-627 rda eng 660 VZ 58.21 bkl Chaemchuen, Somboon verfasserin (orcid)0000-0001-9936-0919 aut Solid–solid thermal synthesis of bimetallic Ni/Zn embedded in N-doped porous carbon for efficient adsorptive separation based on CO 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier High-efficient adsorptive materials for carbon dioxide (CO2) capture and separation of a gas mixture are vital for energy consumption and emission reduction but are still a substantial challenge. A facile synthesis of bimetallic nickel/zinc embedded in N-doped carbon (Ni/ZnNC) through the solid–solid thermal method (SST) is developed herein. The SST method is a straightforward procedure with the advantage that the materials are obtained in a single step and solvent-free conditions. Thermal analysis and material characterization were used to investigate the synthesis mechanism during the SST process. The results revealed that an intermediate material, initially obtained at a low thermal temperature, was sacrificed to generate Ni/Zn@NC at high temperatures of the SST method. The resulting robust carbon structure, decorated with heteroatoms (Ni, Zn, N), exhibits a potential for efficient CO2 adsorption during the capture and separation of biogas (CO2/CH4), off-gas (CO2/N2), and natural gas (CH4/ N2). The synergetic effect of Ni in the materials enhances the selectivity of SCO2/CH4 , SCO2/N2, and SCH4/N2 . The improved selectivities by effective sites were confirmed by computational modeling. Significantly, the Ni/Zn@NC material obtained through a mild yet simple synthesis method (SST) exhibits substantially higher CO2 adsorption capacity and selectivity when compared to commercial carbon (activated charcoal). Solid–solid thermal method Ni/Zn@NC Solvent-free synthesis Carbon adsorbent CO CO Cheng, Zhonghan verfasserin aut Hou, Xiaotong verfasserin aut Verpoort, Francis verfasserin (orcid)0000-0002-5184-5500 aut Kumsi, Jakkapan verfasserin aut Klomkliang, Nikom verfasserin (orcid)0000-0001-8834-6011 aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 356 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:356 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.21 Brennstoffe Kraftstoffe Explosivstoffe VZ AR 356
allfieldsGer	10.1016/j.fuel.2023.129608 doi (DE-627)ELV065394208 (ELSEVIER)S0016-2361(23)02222-6 DE-627 ger DE-627 rda eng 660 VZ 58.21 bkl Chaemchuen, Somboon verfasserin (orcid)0000-0001-9936-0919 aut Solid–solid thermal synthesis of bimetallic Ni/Zn embedded in N-doped porous carbon for efficient adsorptive separation based on CO 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier High-efficient adsorptive materials for carbon dioxide (CO2) capture and separation of a gas mixture are vital for energy consumption and emission reduction but are still a substantial challenge. A facile synthesis of bimetallic nickel/zinc embedded in N-doped carbon (Ni/ZnNC) through the solid–solid thermal method (SST) is developed herein. The SST method is a straightforward procedure with the advantage that the materials are obtained in a single step and solvent-free conditions. Thermal analysis and material characterization were used to investigate the synthesis mechanism during the SST process. The results revealed that an intermediate material, initially obtained at a low thermal temperature, was sacrificed to generate Ni/Zn@NC at high temperatures of the SST method. The resulting robust carbon structure, decorated with heteroatoms (Ni, Zn, N), exhibits a potential for efficient CO2 adsorption during the capture and separation of biogas (CO2/CH4), off-gas (CO2/N2), and natural gas (CH4/ N2). The synergetic effect of Ni in the materials enhances the selectivity of SCO2/CH4 , SCO2/N2, and SCH4/N2 . The improved selectivities by effective sites were confirmed by computational modeling. Significantly, the Ni/Zn@NC material obtained through a mild yet simple synthesis method (SST) exhibits substantially higher CO2 adsorption capacity and selectivity when compared to commercial carbon (activated charcoal). Solid–solid thermal method Ni/Zn@NC Solvent-free synthesis Carbon adsorbent CO CO Cheng, Zhonghan verfasserin aut Hou, Xiaotong verfasserin aut Verpoort, Francis verfasserin (orcid)0000-0002-5184-5500 aut Kumsi, Jakkapan verfasserin aut Klomkliang, Nikom verfasserin (orcid)0000-0001-8834-6011 aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 356 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:356 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.21 Brennstoffe Kraftstoffe Explosivstoffe VZ AR 356
allfieldsSound	10.1016/j.fuel.2023.129608 doi (DE-627)ELV065394208 (ELSEVIER)S0016-2361(23)02222-6 DE-627 ger DE-627 rda eng 660 VZ 58.21 bkl Chaemchuen, Somboon verfasserin (orcid)0000-0001-9936-0919 aut Solid–solid thermal synthesis of bimetallic Ni/Zn embedded in N-doped porous carbon for efficient adsorptive separation based on CO 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier High-efficient adsorptive materials for carbon dioxide (CO2) capture and separation of a gas mixture are vital for energy consumption and emission reduction but are still a substantial challenge. A facile synthesis of bimetallic nickel/zinc embedded in N-doped carbon (Ni/ZnNC) through the solid–solid thermal method (SST) is developed herein. The SST method is a straightforward procedure with the advantage that the materials are obtained in a single step and solvent-free conditions. Thermal analysis and material characterization were used to investigate the synthesis mechanism during the SST process. The results revealed that an intermediate material, initially obtained at a low thermal temperature, was sacrificed to generate Ni/Zn@NC at high temperatures of the SST method. The resulting robust carbon structure, decorated with heteroatoms (Ni, Zn, N), exhibits a potential for efficient CO2 adsorption during the capture and separation of biogas (CO2/CH4), off-gas (CO2/N2), and natural gas (CH4/ N2). The synergetic effect of Ni in the materials enhances the selectivity of SCO2/CH4 , SCO2/N2, and SCH4/N2 . The improved selectivities by effective sites were confirmed by computational modeling. Significantly, the Ni/Zn@NC material obtained through a mild yet simple synthesis method (SST) exhibits substantially higher CO2 adsorption capacity and selectivity when compared to commercial carbon (activated charcoal). Solid–solid thermal method Ni/Zn@NC Solvent-free synthesis Carbon adsorbent CO CO Cheng, Zhonghan verfasserin aut Hou, Xiaotong verfasserin aut Verpoort, Francis verfasserin (orcid)0000-0002-5184-5500 aut Kumsi, Jakkapan verfasserin aut Klomkliang, Nikom verfasserin (orcid)0000-0001-8834-6011 aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 356 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:356 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.21 Brennstoffe Kraftstoffe Explosivstoffe VZ AR 356
language	English
source	Enthalten in Fuel 356 volume:356
sourceStr	Enthalten in Fuel 356 volume:356
format_phy_str_mv	Article
bklname	Brennstoffe Kraftstoffe Explosivstoffe
institution	findex.gbv.de
topic_facet	Solid–solid thermal method Ni/Zn@NC Solvent-free synthesis Carbon adsorbent CO
dewey-raw	660
isfreeaccess_bool	false
container_title	Fuel
authorswithroles_txt_mv	Chaemchuen, Somboon @@aut@@ Cheng, Zhonghan @@aut@@ Hou, Xiaotong @@aut@@ Verpoort, Francis @@aut@@ Kumsi, Jakkapan @@aut@@ Klomkliang, Nikom @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	300898584
dewey-sort	3660
id	ELV065394208
language_de	englisch
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author	Chaemchuen, Somboon
spellingShingle	Chaemchuen, Somboon ddc 660 bkl 58.21 misc Solid–solid thermal method misc Ni/Zn@NC misc Solvent-free synthesis misc Carbon adsorbent misc CO Solid–solid thermal synthesis of bimetallic Ni/Zn embedded in N-doped porous carbon for efficient adsorptive separation based on CO
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topic_title	660 VZ 58.21 bkl Solid–solid thermal synthesis of bimetallic Ni/Zn embedded in N-doped porous carbon for efficient adsorptive separation based on CO Solid–solid thermal method Ni/Zn@NC Solvent-free synthesis Carbon adsorbent CO
topic	ddc 660 bkl 58.21 misc Solid–solid thermal method misc Ni/Zn@NC misc Solvent-free synthesis misc Carbon adsorbent misc CO
topic_unstemmed	ddc 660 bkl 58.21 misc Solid–solid thermal method misc Ni/Zn@NC misc Solvent-free synthesis misc Carbon adsorbent misc CO
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title	Solid–solid thermal synthesis of bimetallic Ni/Zn embedded in N-doped porous carbon for efficient adsorptive separation based on CO
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title_full	Solid–solid thermal synthesis of bimetallic Ni/Zn embedded in N-doped porous carbon for efficient adsorptive separation based on CO
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author_browse	Chaemchuen, Somboon Cheng, Zhonghan Hou, Xiaotong Verpoort, Francis Kumsi, Jakkapan Klomkliang, Nikom
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title_sort	solid–solid thermal synthesis of bimetallic ni/zn embedded in n-doped porous carbon for efficient adsorptive separation based on co
title_auth	Solid–solid thermal synthesis of bimetallic Ni/Zn embedded in N-doped porous carbon for efficient adsorptive separation based on CO
abstract	High-efficient adsorptive materials for carbon dioxide (CO2) capture and separation of a gas mixture are vital for energy consumption and emission reduction but are still a substantial challenge. A facile synthesis of bimetallic nickel/zinc embedded in N-doped carbon (Ni/ZnNC) through the solid–solid thermal method (SST) is developed herein. The SST method is a straightforward procedure with the advantage that the materials are obtained in a single step and solvent-free conditions. Thermal analysis and material characterization were used to investigate the synthesis mechanism during the SST process. The results revealed that an intermediate material, initially obtained at a low thermal temperature, was sacrificed to generate Ni/Zn@NC at high temperatures of the SST method. The resulting robust carbon structure, decorated with heteroatoms (Ni, Zn, N), exhibits a potential for efficient CO2 adsorption during the capture and separation of biogas (CO2/CH4), off-gas (CO2/N2), and natural gas (CH4/ N2). The synergetic effect of Ni in the materials enhances the selectivity of SCO2/CH4 , SCO2/N2, and SCH4/N2 . The improved selectivities by effective sites were confirmed by computational modeling. Significantly, the Ni/Zn@NC material obtained through a mild yet simple synthesis method (SST) exhibits substantially higher CO2 adsorption capacity and selectivity when compared to commercial carbon (activated charcoal).
abstractGer	High-efficient adsorptive materials for carbon dioxide (CO2) capture and separation of a gas mixture are vital for energy consumption and emission reduction but are still a substantial challenge. A facile synthesis of bimetallic nickel/zinc embedded in N-doped carbon (Ni/ZnNC) through the solid–solid thermal method (SST) is developed herein. The SST method is a straightforward procedure with the advantage that the materials are obtained in a single step and solvent-free conditions. Thermal analysis and material characterization were used to investigate the synthesis mechanism during the SST process. The results revealed that an intermediate material, initially obtained at a low thermal temperature, was sacrificed to generate Ni/Zn@NC at high temperatures of the SST method. The resulting robust carbon structure, decorated with heteroatoms (Ni, Zn, N), exhibits a potential for efficient CO2 adsorption during the capture and separation of biogas (CO2/CH4), off-gas (CO2/N2), and natural gas (CH4/ N2). The synergetic effect of Ni in the materials enhances the selectivity of SCO2/CH4 , SCO2/N2, and SCH4/N2 . The improved selectivities by effective sites were confirmed by computational modeling. Significantly, the Ni/Zn@NC material obtained through a mild yet simple synthesis method (SST) exhibits substantially higher CO2 adsorption capacity and selectivity when compared to commercial carbon (activated charcoal).
abstract_unstemmed	High-efficient adsorptive materials for carbon dioxide (CO2) capture and separation of a gas mixture are vital for energy consumption and emission reduction but are still a substantial challenge. A facile synthesis of bimetallic nickel/zinc embedded in N-doped carbon (Ni/ZnNC) through the solid–solid thermal method (SST) is developed herein. The SST method is a straightforward procedure with the advantage that the materials are obtained in a single step and solvent-free conditions. Thermal analysis and material characterization were used to investigate the synthesis mechanism during the SST process. The results revealed that an intermediate material, initially obtained at a low thermal temperature, was sacrificed to generate Ni/Zn@NC at high temperatures of the SST method. The resulting robust carbon structure, decorated with heteroatoms (Ni, Zn, N), exhibits a potential for efficient CO2 adsorption during the capture and separation of biogas (CO2/CH4), off-gas (CO2/N2), and natural gas (CH4/ N2). The synergetic effect of Ni in the materials enhances the selectivity of SCO2/CH4 , SCO2/N2, and SCH4/N2 . The improved selectivities by effective sites were confirmed by computational modeling. Significantly, the Ni/Zn@NC material obtained through a mild yet simple synthesis method (SST) exhibits substantially higher CO2 adsorption capacity and selectivity when compared to commercial carbon (activated charcoal).
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title_short	Solid–solid thermal synthesis of bimetallic Ni/Zn embedded in N-doped porous carbon for efficient adsorptive separation based on CO
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author2	Cheng, Zhonghan Hou, Xiaotong Verpoort, Francis Kumsi, Jakkapan Klomkliang, Nikom
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doi_str	10.1016/j.fuel.2023.129608
up_date	2024-07-06T22:52:54.786Z
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Solid–solid thermal synthesis of bimetallic Ni/Zn embedded in N-doped porous carbon for efficient adsorptive separation based on CO

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