Lignin with enhanced photothermal performance for the preparation of a sustainable solar-driven double-layer biomass evaporator
The undesirable photothermal conversion performance of lignin limits the potential for directing use as a photothermal conversion material, and no strategies have been found to enhance the photothermal conversion efficiency of lignin. Herein, three modified lignin of corn stover alkali lignin (DEHL)...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Shao, Qizhao [verfasserIn] Luo, Yu [verfasserIn] Cao, Meifang [verfasserIn] Qiu, Xueqing [verfasserIn] Zheng, Dafeng [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2023 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: The chemical engineering journal - Amsterdam : Elsevier, 1997, 476 |
|---|---|
| Übergeordnetes Werk: |
volume:476 |
| DOI / URN: |
10.1016/j.cej.2023.146678 |
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| Katalog-ID: |
ELV065580788 |
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| 520 | |a The undesirable photothermal conversion performance of lignin limits the potential for directing use as a photothermal conversion material, and no strategies have been found to enhance the photothermal conversion efficiency of lignin. Herein, three modified lignin of corn stover alkali lignin (DEHL), pine alkali lignin (DAL) and birch alkali lignin (DTAL) with excellent photothermal conversion efficiency and fast temperature response was prepared by a one-step iodocyclohexane (ICH) activation strategy. The maximum temperature of the DEHL, DAL and DTAL can reach to 138 °C, 157 °C, and 172 °C in 12 min under 0.15 W/cm2 compared to the native lignin. Moreover, the photothermal conversion efficiency of the DEHL, DAL and DTAL was calculated to be 36.52 %, 36.19 % and 43.19 % by ICH modification. The photothermal enhancement mechanism of the modified lignin was determined by various characterizations and simulation calculations, which can be summarized that the activation of lignin by ICH breaks the molecular structure and reduces the methoxy content of the lignin, which enhances the intermolecular bonding, and the hydrogen bonding between the phenolic hydroxyl groups strengthens the π-π intermolecular interactions between the benzene rings. In addition, a double-layer biomass aerogel evaporator (DAGS) with cost-friendly and superior evaporation performance was synthesized by chemical cross-linking using DTAL as the photothermal agent. The evaporation rate of 4DAGS can be as high as 2.063, 2.024, 2.259 and 2.447 kg/(m2∙h) in water, 3.5 wt% seawater, and 200 mg/L of MG or MB wastewater under 1sun. And no salt was observed on the surface of the 4DAGS after a long period of 36 h of operation in 3.5 wt% seawater, suggesting the outstanding salt-reject performance of the aerogel. Furthermore, there is no structural damage and chemical decomposition found on 4DAGS after 24 h immersion in NaOH and HCl solutions, demonstrating the excellent acid and alkali resistance of the synthesized aerogels. This work may offer a novel strategy for the photothermal performance enhancement of lignin and expand the potential application in solar-driven evaporation materials. | ||
| 650 | 4 | |a Lignin | |
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10.1016/j.cej.2023.146678 doi (DE-627)ELV065580788 (ELSEVIER)S1385-8947(23)05409-8 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Shao, Qizhao verfasserin aut Lignin with enhanced photothermal performance for the preparation of a sustainable solar-driven double-layer biomass evaporator 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The undesirable photothermal conversion performance of lignin limits the potential for directing use as a photothermal conversion material, and no strategies have been found to enhance the photothermal conversion efficiency of lignin. Herein, three modified lignin of corn stover alkali lignin (DEHL), pine alkali lignin (DAL) and birch alkali lignin (DTAL) with excellent photothermal conversion efficiency and fast temperature response was prepared by a one-step iodocyclohexane (ICH) activation strategy. The maximum temperature of the DEHL, DAL and DTAL can reach to 138 °C, 157 °C, and 172 °C in 12 min under 0.15 W/cm2 compared to the native lignin. Moreover, the photothermal conversion efficiency of the DEHL, DAL and DTAL was calculated to be 36.52 %, 36.19 % and 43.19 % by ICH modification. The photothermal enhancement mechanism of the modified lignin was determined by various characterizations and simulation calculations, which can be summarized that the activation of lignin by ICH breaks the molecular structure and reduces the methoxy content of the lignin, which enhances the intermolecular bonding, and the hydrogen bonding between the phenolic hydroxyl groups strengthens the π-π intermolecular interactions between the benzene rings. In addition, a double-layer biomass aerogel evaporator (DAGS) with cost-friendly and superior evaporation performance was synthesized by chemical cross-linking using DTAL as the photothermal agent. The evaporation rate of 4DAGS can be as high as 2.063, 2.024, 2.259 and 2.447 kg/(m2∙h) in water, 3.5 wt% seawater, and 200 mg/L of MG or MB wastewater under 1sun. And no salt was observed on the surface of the 4DAGS after a long period of 36 h of operation in 3.5 wt% seawater, suggesting the outstanding salt-reject performance of the aerogel. Furthermore, there is no structural damage and chemical decomposition found on 4DAGS after 24 h immersion in NaOH and HCl solutions, demonstrating the excellent acid and alkali resistance of the synthesized aerogels. This work may offer a novel strategy for the photothermal performance enhancement of lignin and expand the potential application in solar-driven evaporation materials. Lignin Photothermal conversion Photothermal mechanism Aerogels Water purification Luo, Yu verfasserin aut Cao, Meifang verfasserin aut Qiu, Xueqing verfasserin aut Zheng, Dafeng verfasserin (orcid)0000-0002-0353-8231 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 476 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:476 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 476 |
| spelling |
10.1016/j.cej.2023.146678 doi (DE-627)ELV065580788 (ELSEVIER)S1385-8947(23)05409-8 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Shao, Qizhao verfasserin aut Lignin with enhanced photothermal performance for the preparation of a sustainable solar-driven double-layer biomass evaporator 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The undesirable photothermal conversion performance of lignin limits the potential for directing use as a photothermal conversion material, and no strategies have been found to enhance the photothermal conversion efficiency of lignin. Herein, three modified lignin of corn stover alkali lignin (DEHL), pine alkali lignin (DAL) and birch alkali lignin (DTAL) with excellent photothermal conversion efficiency and fast temperature response was prepared by a one-step iodocyclohexane (ICH) activation strategy. The maximum temperature of the DEHL, DAL and DTAL can reach to 138 °C, 157 °C, and 172 °C in 12 min under 0.15 W/cm2 compared to the native lignin. Moreover, the photothermal conversion efficiency of the DEHL, DAL and DTAL was calculated to be 36.52 %, 36.19 % and 43.19 % by ICH modification. The photothermal enhancement mechanism of the modified lignin was determined by various characterizations and simulation calculations, which can be summarized that the activation of lignin by ICH breaks the molecular structure and reduces the methoxy content of the lignin, which enhances the intermolecular bonding, and the hydrogen bonding between the phenolic hydroxyl groups strengthens the π-π intermolecular interactions between the benzene rings. In addition, a double-layer biomass aerogel evaporator (DAGS) with cost-friendly and superior evaporation performance was synthesized by chemical cross-linking using DTAL as the photothermal agent. The evaporation rate of 4DAGS can be as high as 2.063, 2.024, 2.259 and 2.447 kg/(m2∙h) in water, 3.5 wt% seawater, and 200 mg/L of MG or MB wastewater under 1sun. And no salt was observed on the surface of the 4DAGS after a long period of 36 h of operation in 3.5 wt% seawater, suggesting the outstanding salt-reject performance of the aerogel. Furthermore, there is no structural damage and chemical decomposition found on 4DAGS after 24 h immersion in NaOH and HCl solutions, demonstrating the excellent acid and alkali resistance of the synthesized aerogels. This work may offer a novel strategy for the photothermal performance enhancement of lignin and expand the potential application in solar-driven evaporation materials. Lignin Photothermal conversion Photothermal mechanism Aerogels Water purification Luo, Yu verfasserin aut Cao, Meifang verfasserin aut Qiu, Xueqing verfasserin aut Zheng, Dafeng verfasserin (orcid)0000-0002-0353-8231 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 476 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:476 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 476 |
| allfields_unstemmed |
10.1016/j.cej.2023.146678 doi (DE-627)ELV065580788 (ELSEVIER)S1385-8947(23)05409-8 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Shao, Qizhao verfasserin aut Lignin with enhanced photothermal performance for the preparation of a sustainable solar-driven double-layer biomass evaporator 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The undesirable photothermal conversion performance of lignin limits the potential for directing use as a photothermal conversion material, and no strategies have been found to enhance the photothermal conversion efficiency of lignin. Herein, three modified lignin of corn stover alkali lignin (DEHL), pine alkali lignin (DAL) and birch alkali lignin (DTAL) with excellent photothermal conversion efficiency and fast temperature response was prepared by a one-step iodocyclohexane (ICH) activation strategy. The maximum temperature of the DEHL, DAL and DTAL can reach to 138 °C, 157 °C, and 172 °C in 12 min under 0.15 W/cm2 compared to the native lignin. Moreover, the photothermal conversion efficiency of the DEHL, DAL and DTAL was calculated to be 36.52 %, 36.19 % and 43.19 % by ICH modification. The photothermal enhancement mechanism of the modified lignin was determined by various characterizations and simulation calculations, which can be summarized that the activation of lignin by ICH breaks the molecular structure and reduces the methoxy content of the lignin, which enhances the intermolecular bonding, and the hydrogen bonding between the phenolic hydroxyl groups strengthens the π-π intermolecular interactions between the benzene rings. In addition, a double-layer biomass aerogel evaporator (DAGS) with cost-friendly and superior evaporation performance was synthesized by chemical cross-linking using DTAL as the photothermal agent. The evaporation rate of 4DAGS can be as high as 2.063, 2.024, 2.259 and 2.447 kg/(m2∙h) in water, 3.5 wt% seawater, and 200 mg/L of MG or MB wastewater under 1sun. And no salt was observed on the surface of the 4DAGS after a long period of 36 h of operation in 3.5 wt% seawater, suggesting the outstanding salt-reject performance of the aerogel. Furthermore, there is no structural damage and chemical decomposition found on 4DAGS after 24 h immersion in NaOH and HCl solutions, demonstrating the excellent acid and alkali resistance of the synthesized aerogels. This work may offer a novel strategy for the photothermal performance enhancement of lignin and expand the potential application in solar-driven evaporation materials. Lignin Photothermal conversion Photothermal mechanism Aerogels Water purification Luo, Yu verfasserin aut Cao, Meifang verfasserin aut Qiu, Xueqing verfasserin aut Zheng, Dafeng verfasserin (orcid)0000-0002-0353-8231 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 476 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:476 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 476 |
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10.1016/j.cej.2023.146678 doi (DE-627)ELV065580788 (ELSEVIER)S1385-8947(23)05409-8 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Shao, Qizhao verfasserin aut Lignin with enhanced photothermal performance for the preparation of a sustainable solar-driven double-layer biomass evaporator 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The undesirable photothermal conversion performance of lignin limits the potential for directing use as a photothermal conversion material, and no strategies have been found to enhance the photothermal conversion efficiency of lignin. Herein, three modified lignin of corn stover alkali lignin (DEHL), pine alkali lignin (DAL) and birch alkali lignin (DTAL) with excellent photothermal conversion efficiency and fast temperature response was prepared by a one-step iodocyclohexane (ICH) activation strategy. The maximum temperature of the DEHL, DAL and DTAL can reach to 138 °C, 157 °C, and 172 °C in 12 min under 0.15 W/cm2 compared to the native lignin. Moreover, the photothermal conversion efficiency of the DEHL, DAL and DTAL was calculated to be 36.52 %, 36.19 % and 43.19 % by ICH modification. The photothermal enhancement mechanism of the modified lignin was determined by various characterizations and simulation calculations, which can be summarized that the activation of lignin by ICH breaks the molecular structure and reduces the methoxy content of the lignin, which enhances the intermolecular bonding, and the hydrogen bonding between the phenolic hydroxyl groups strengthens the π-π intermolecular interactions between the benzene rings. In addition, a double-layer biomass aerogel evaporator (DAGS) with cost-friendly and superior evaporation performance was synthesized by chemical cross-linking using DTAL as the photothermal agent. The evaporation rate of 4DAGS can be as high as 2.063, 2.024, 2.259 and 2.447 kg/(m2∙h) in water, 3.5 wt% seawater, and 200 mg/L of MG or MB wastewater under 1sun. And no salt was observed on the surface of the 4DAGS after a long period of 36 h of operation in 3.5 wt% seawater, suggesting the outstanding salt-reject performance of the aerogel. Furthermore, there is no structural damage and chemical decomposition found on 4DAGS after 24 h immersion in NaOH and HCl solutions, demonstrating the excellent acid and alkali resistance of the synthesized aerogels. This work may offer a novel strategy for the photothermal performance enhancement of lignin and expand the potential application in solar-driven evaporation materials. Lignin Photothermal conversion Photothermal mechanism Aerogels Water purification Luo, Yu verfasserin aut Cao, Meifang verfasserin aut Qiu, Xueqing verfasserin aut Zheng, Dafeng verfasserin (orcid)0000-0002-0353-8231 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 476 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:476 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 476 |
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10.1016/j.cej.2023.146678 doi (DE-627)ELV065580788 (ELSEVIER)S1385-8947(23)05409-8 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Shao, Qizhao verfasserin aut Lignin with enhanced photothermal performance for the preparation of a sustainable solar-driven double-layer biomass evaporator 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The undesirable photothermal conversion performance of lignin limits the potential for directing use as a photothermal conversion material, and no strategies have been found to enhance the photothermal conversion efficiency of lignin. Herein, three modified lignin of corn stover alkali lignin (DEHL), pine alkali lignin (DAL) and birch alkali lignin (DTAL) with excellent photothermal conversion efficiency and fast temperature response was prepared by a one-step iodocyclohexane (ICH) activation strategy. The maximum temperature of the DEHL, DAL and DTAL can reach to 138 °C, 157 °C, and 172 °C in 12 min under 0.15 W/cm2 compared to the native lignin. Moreover, the photothermal conversion efficiency of the DEHL, DAL and DTAL was calculated to be 36.52 %, 36.19 % and 43.19 % by ICH modification. The photothermal enhancement mechanism of the modified lignin was determined by various characterizations and simulation calculations, which can be summarized that the activation of lignin by ICH breaks the molecular structure and reduces the methoxy content of the lignin, which enhances the intermolecular bonding, and the hydrogen bonding between the phenolic hydroxyl groups strengthens the π-π intermolecular interactions between the benzene rings. In addition, a double-layer biomass aerogel evaporator (DAGS) with cost-friendly and superior evaporation performance was synthesized by chemical cross-linking using DTAL as the photothermal agent. The evaporation rate of 4DAGS can be as high as 2.063, 2.024, 2.259 and 2.447 kg/(m2∙h) in water, 3.5 wt% seawater, and 200 mg/L of MG or MB wastewater under 1sun. And no salt was observed on the surface of the 4DAGS after a long period of 36 h of operation in 3.5 wt% seawater, suggesting the outstanding salt-reject performance of the aerogel. Furthermore, there is no structural damage and chemical decomposition found on 4DAGS after 24 h immersion in NaOH and HCl solutions, demonstrating the excellent acid and alkali resistance of the synthesized aerogels. This work may offer a novel strategy for the photothermal performance enhancement of lignin and expand the potential application in solar-driven evaporation materials. Lignin Photothermal conversion Photothermal mechanism Aerogels Water purification Luo, Yu verfasserin aut Cao, Meifang verfasserin aut Qiu, Xueqing verfasserin aut Zheng, Dafeng verfasserin (orcid)0000-0002-0353-8231 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 476 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:476 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 476 |
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Shao, Qizhao |
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Shao, Qizhao ddc 660 bkl 58.10 misc Lignin misc Photothermal conversion misc Photothermal mechanism misc Aerogels misc Water purification Lignin with enhanced photothermal performance for the preparation of a sustainable solar-driven double-layer biomass evaporator |
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660 VZ 58.10 bkl Lignin with enhanced photothermal performance for the preparation of a sustainable solar-driven double-layer biomass evaporator Lignin Photothermal conversion Photothermal mechanism Aerogels Water purification |
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lignin with enhanced photothermal performance for the preparation of a sustainable solar-driven double-layer biomass evaporator |
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Lignin with enhanced photothermal performance for the preparation of a sustainable solar-driven double-layer biomass evaporator |
| abstract |
The undesirable photothermal conversion performance of lignin limits the potential for directing use as a photothermal conversion material, and no strategies have been found to enhance the photothermal conversion efficiency of lignin. Herein, three modified lignin of corn stover alkali lignin (DEHL), pine alkali lignin (DAL) and birch alkali lignin (DTAL) with excellent photothermal conversion efficiency and fast temperature response was prepared by a one-step iodocyclohexane (ICH) activation strategy. The maximum temperature of the DEHL, DAL and DTAL can reach to 138 °C, 157 °C, and 172 °C in 12 min under 0.15 W/cm2 compared to the native lignin. Moreover, the photothermal conversion efficiency of the DEHL, DAL and DTAL was calculated to be 36.52 %, 36.19 % and 43.19 % by ICH modification. The photothermal enhancement mechanism of the modified lignin was determined by various characterizations and simulation calculations, which can be summarized that the activation of lignin by ICH breaks the molecular structure and reduces the methoxy content of the lignin, which enhances the intermolecular bonding, and the hydrogen bonding between the phenolic hydroxyl groups strengthens the π-π intermolecular interactions between the benzene rings. In addition, a double-layer biomass aerogel evaporator (DAGS) with cost-friendly and superior evaporation performance was synthesized by chemical cross-linking using DTAL as the photothermal agent. The evaporation rate of 4DAGS can be as high as 2.063, 2.024, 2.259 and 2.447 kg/(m2∙h) in water, 3.5 wt% seawater, and 200 mg/L of MG or MB wastewater under 1sun. And no salt was observed on the surface of the 4DAGS after a long period of 36 h of operation in 3.5 wt% seawater, suggesting the outstanding salt-reject performance of the aerogel. Furthermore, there is no structural damage and chemical decomposition found on 4DAGS after 24 h immersion in NaOH and HCl solutions, demonstrating the excellent acid and alkali resistance of the synthesized aerogels. This work may offer a novel strategy for the photothermal performance enhancement of lignin and expand the potential application in solar-driven evaporation materials. |
| abstractGer |
The undesirable photothermal conversion performance of lignin limits the potential for directing use as a photothermal conversion material, and no strategies have been found to enhance the photothermal conversion efficiency of lignin. Herein, three modified lignin of corn stover alkali lignin (DEHL), pine alkali lignin (DAL) and birch alkali lignin (DTAL) with excellent photothermal conversion efficiency and fast temperature response was prepared by a one-step iodocyclohexane (ICH) activation strategy. The maximum temperature of the DEHL, DAL and DTAL can reach to 138 °C, 157 °C, and 172 °C in 12 min under 0.15 W/cm2 compared to the native lignin. Moreover, the photothermal conversion efficiency of the DEHL, DAL and DTAL was calculated to be 36.52 %, 36.19 % and 43.19 % by ICH modification. The photothermal enhancement mechanism of the modified lignin was determined by various characterizations and simulation calculations, which can be summarized that the activation of lignin by ICH breaks the molecular structure and reduces the methoxy content of the lignin, which enhances the intermolecular bonding, and the hydrogen bonding between the phenolic hydroxyl groups strengthens the π-π intermolecular interactions between the benzene rings. In addition, a double-layer biomass aerogel evaporator (DAGS) with cost-friendly and superior evaporation performance was synthesized by chemical cross-linking using DTAL as the photothermal agent. The evaporation rate of 4DAGS can be as high as 2.063, 2.024, 2.259 and 2.447 kg/(m2∙h) in water, 3.5 wt% seawater, and 200 mg/L of MG or MB wastewater under 1sun. And no salt was observed on the surface of the 4DAGS after a long period of 36 h of operation in 3.5 wt% seawater, suggesting the outstanding salt-reject performance of the aerogel. Furthermore, there is no structural damage and chemical decomposition found on 4DAGS after 24 h immersion in NaOH and HCl solutions, demonstrating the excellent acid and alkali resistance of the synthesized aerogels. This work may offer a novel strategy for the photothermal performance enhancement of lignin and expand the potential application in solar-driven evaporation materials. |
| abstract_unstemmed |
The undesirable photothermal conversion performance of lignin limits the potential for directing use as a photothermal conversion material, and no strategies have been found to enhance the photothermal conversion efficiency of lignin. Herein, three modified lignin of corn stover alkali lignin (DEHL), pine alkali lignin (DAL) and birch alkali lignin (DTAL) with excellent photothermal conversion efficiency and fast temperature response was prepared by a one-step iodocyclohexane (ICH) activation strategy. The maximum temperature of the DEHL, DAL and DTAL can reach to 138 °C, 157 °C, and 172 °C in 12 min under 0.15 W/cm2 compared to the native lignin. Moreover, the photothermal conversion efficiency of the DEHL, DAL and DTAL was calculated to be 36.52 %, 36.19 % and 43.19 % by ICH modification. The photothermal enhancement mechanism of the modified lignin was determined by various characterizations and simulation calculations, which can be summarized that the activation of lignin by ICH breaks the molecular structure and reduces the methoxy content of the lignin, which enhances the intermolecular bonding, and the hydrogen bonding between the phenolic hydroxyl groups strengthens the π-π intermolecular interactions between the benzene rings. In addition, a double-layer biomass aerogel evaporator (DAGS) with cost-friendly and superior evaporation performance was synthesized by chemical cross-linking using DTAL as the photothermal agent. The evaporation rate of 4DAGS can be as high as 2.063, 2.024, 2.259 and 2.447 kg/(m2∙h) in water, 3.5 wt% seawater, and 200 mg/L of MG or MB wastewater under 1sun. And no salt was observed on the surface of the 4DAGS after a long period of 36 h of operation in 3.5 wt% seawater, suggesting the outstanding salt-reject performance of the aerogel. Furthermore, there is no structural damage and chemical decomposition found on 4DAGS after 24 h immersion in NaOH and HCl solutions, demonstrating the excellent acid and alkali resistance of the synthesized aerogels. This work may offer a novel strategy for the photothermal performance enhancement of lignin and expand the potential application in solar-driven evaporation materials. |
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