A viologen-derived luminescent material exhibiting photochromism, photocontrolled luminescence and selective detection of Cr

Stable viologen-derived multifunctional smart materials exhibit widespread practical applications in many areas. In this study, a viologen-derived material with 4-fold interpenetrating diamondoid network, {[Cd(1,4-ndc)(cpbpy)]·2H2O}n, was successfully constructed based on asymmetrical N-(3-carboxyph...
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Gespeichert in:

Autor*in:	Li, Zhao-Hao [verfasserIn] Li, Min [verfasserIn] Xu, Tian-Yu [verfasserIn] Zhao, Bang-Tun [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Viologen Coordination polymer Crystal structure Photochromism Luminescence Luminescence sensing

Übergeordnetes Werk:	Enthalten in: Spectrochimica acta / A - Amsterdam [u.a.] : Elsevier Science, 1967, 306
Übergeordnetes Werk:	volume:306

DOI / URN:	10.1016/j.saa.2023.123579

Katalog-ID:	ELV065626753

Internformat


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245	1	0	\|a A viologen-derived luminescent material exhibiting photochromism, photocontrolled luminescence and selective detection of Cr
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520			\|a Stable viologen-derived multifunctional smart materials exhibit widespread practical applications in many areas. In this study, a viologen-derived material with 4-fold interpenetrating diamondoid network, {[Cd(1,4-ndc)(cpbpy)]·2H2O}n, was successfully constructed based on asymmetrical N-(3-carboxyphenyl)-4,4′-bipyridinium (cpbpy) and 1,4-naphthalenedicarboxylic acid (1,4-H2ndc). The compound shows reversible photochromic behavior under a xenon lamp, which are proved by UV–vis spectra and EPR characterizations. Moreover, the compound with good photoluminescence properties displays photocontrolled luminescence quenching behaviors. Owing to its good water stability, the compound is then applied in luminescence sensing for the detection of Cr2O7 2− in aqueous solution. The corresponding luminescence quenching constant for Cr2O7 2− is K SV = 4.33 × 104 M−1, and the detection limit is 3.66 μM. Systematic investigations on the luminescence quenching mechanism suggest that the inner filter effect resulted in the selective detection of Cr2O7 2−. This study provides inspiration for the design and synthesis of target luminescent crystalline materials with rigid and asymmetric viologen-derived ligands.
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650		4	\|a Coordination polymer
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700	1		\|a Li, Min \|e verfasserin \|4 aut
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700	1		\|a Zhao, Bang-Tun \|e verfasserin \|4 aut
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publishDate	2023
allfields	10.1016/j.saa.2023.123579 doi (DE-627)ELV065626753 (ELSEVIER)S1386-1425(23)01264-7 DE-627 ger DE-627 rda eng 540 530 VZ 35.00 bkl Li, Zhao-Hao verfasserin aut A viologen-derived luminescent material exhibiting photochromism, photocontrolled luminescence and selective detection of Cr 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Stable viologen-derived multifunctional smart materials exhibit widespread practical applications in many areas. In this study, a viologen-derived material with 4-fold interpenetrating diamondoid network, {[Cd(1,4-ndc)(cpbpy)]·2H2O}n, was successfully constructed based on asymmetrical N-(3-carboxyphenyl)-4,4′-bipyridinium (cpbpy) and 1,4-naphthalenedicarboxylic acid (1,4-H2ndc). The compound shows reversible photochromic behavior under a xenon lamp, which are proved by UV–vis spectra and EPR characterizations. Moreover, the compound with good photoluminescence properties displays photocontrolled luminescence quenching behaviors. Owing to its good water stability, the compound is then applied in luminescence sensing for the detection of Cr2O7 2− in aqueous solution. The corresponding luminescence quenching constant for Cr2O7 2− is K SV = 4.33 × 104 M−1, and the detection limit is 3.66 μM. Systematic investigations on the luminescence quenching mechanism suggest that the inner filter effect resulted in the selective detection of Cr2O7 2−. This study provides inspiration for the design and synthesis of target luminescent crystalline materials with rigid and asymmetric viologen-derived ligands. Viologen Coordination polymer Crystal structure Photochromism Luminescence Luminescence sensing Li, Min verfasserin aut Xu, Tian-Yu verfasserin aut Zhao, Bang-Tun verfasserin aut Enthalten in Spectrochimica acta / A Amsterdam [u.a.] : Elsevier Science, 1967 306 Online-Ressource (DE-627)320570983 (DE-600)2016492-0 (DE-576)090956206 1873-3557 nnns volume:306 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 306
spelling	10.1016/j.saa.2023.123579 doi (DE-627)ELV065626753 (ELSEVIER)S1386-1425(23)01264-7 DE-627 ger DE-627 rda eng 540 530 VZ 35.00 bkl Li, Zhao-Hao verfasserin aut A viologen-derived luminescent material exhibiting photochromism, photocontrolled luminescence and selective detection of Cr 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Stable viologen-derived multifunctional smart materials exhibit widespread practical applications in many areas. In this study, a viologen-derived material with 4-fold interpenetrating diamondoid network, {[Cd(1,4-ndc)(cpbpy)]·2H2O}n, was successfully constructed based on asymmetrical N-(3-carboxyphenyl)-4,4′-bipyridinium (cpbpy) and 1,4-naphthalenedicarboxylic acid (1,4-H2ndc). The compound shows reversible photochromic behavior under a xenon lamp, which are proved by UV–vis spectra and EPR characterizations. Moreover, the compound with good photoluminescence properties displays photocontrolled luminescence quenching behaviors. Owing to its good water stability, the compound is then applied in luminescence sensing for the detection of Cr2O7 2− in aqueous solution. The corresponding luminescence quenching constant for Cr2O7 2− is K SV = 4.33 × 104 M−1, and the detection limit is 3.66 μM. Systematic investigations on the luminescence quenching mechanism suggest that the inner filter effect resulted in the selective detection of Cr2O7 2−. This study provides inspiration for the design and synthesis of target luminescent crystalline materials with rigid and asymmetric viologen-derived ligands. Viologen Coordination polymer Crystal structure Photochromism Luminescence Luminescence sensing Li, Min verfasserin aut Xu, Tian-Yu verfasserin aut Zhao, Bang-Tun verfasserin aut Enthalten in Spectrochimica acta / A Amsterdam [u.a.] : Elsevier Science, 1967 306 Online-Ressource (DE-627)320570983 (DE-600)2016492-0 (DE-576)090956206 1873-3557 nnns volume:306 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 306
allfields_unstemmed	10.1016/j.saa.2023.123579 doi (DE-627)ELV065626753 (ELSEVIER)S1386-1425(23)01264-7 DE-627 ger DE-627 rda eng 540 530 VZ 35.00 bkl Li, Zhao-Hao verfasserin aut A viologen-derived luminescent material exhibiting photochromism, photocontrolled luminescence and selective detection of Cr 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Stable viologen-derived multifunctional smart materials exhibit widespread practical applications in many areas. In this study, a viologen-derived material with 4-fold interpenetrating diamondoid network, {[Cd(1,4-ndc)(cpbpy)]·2H2O}n, was successfully constructed based on asymmetrical N-(3-carboxyphenyl)-4,4′-bipyridinium (cpbpy) and 1,4-naphthalenedicarboxylic acid (1,4-H2ndc). The compound shows reversible photochromic behavior under a xenon lamp, which are proved by UV–vis spectra and EPR characterizations. Moreover, the compound with good photoluminescence properties displays photocontrolled luminescence quenching behaviors. Owing to its good water stability, the compound is then applied in luminescence sensing for the detection of Cr2O7 2− in aqueous solution. The corresponding luminescence quenching constant for Cr2O7 2− is K SV = 4.33 × 104 M−1, and the detection limit is 3.66 μM. Systematic investigations on the luminescence quenching mechanism suggest that the inner filter effect resulted in the selective detection of Cr2O7 2−. This study provides inspiration for the design and synthesis of target luminescent crystalline materials with rigid and asymmetric viologen-derived ligands. Viologen Coordination polymer Crystal structure Photochromism Luminescence Luminescence sensing Li, Min verfasserin aut Xu, Tian-Yu verfasserin aut Zhao, Bang-Tun verfasserin aut Enthalten in Spectrochimica acta / A Amsterdam [u.a.] : Elsevier Science, 1967 306 Online-Ressource (DE-627)320570983 (DE-600)2016492-0 (DE-576)090956206 1873-3557 nnns volume:306 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 306
allfieldsGer	10.1016/j.saa.2023.123579 doi (DE-627)ELV065626753 (ELSEVIER)S1386-1425(23)01264-7 DE-627 ger DE-627 rda eng 540 530 VZ 35.00 bkl Li, Zhao-Hao verfasserin aut A viologen-derived luminescent material exhibiting photochromism, photocontrolled luminescence and selective detection of Cr 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Stable viologen-derived multifunctional smart materials exhibit widespread practical applications in many areas. In this study, a viologen-derived material with 4-fold interpenetrating diamondoid network, {[Cd(1,4-ndc)(cpbpy)]·2H2O}n, was successfully constructed based on asymmetrical N-(3-carboxyphenyl)-4,4′-bipyridinium (cpbpy) and 1,4-naphthalenedicarboxylic acid (1,4-H2ndc). The compound shows reversible photochromic behavior under a xenon lamp, which are proved by UV–vis spectra and EPR characterizations. Moreover, the compound with good photoluminescence properties displays photocontrolled luminescence quenching behaviors. Owing to its good water stability, the compound is then applied in luminescence sensing for the detection of Cr2O7 2− in aqueous solution. The corresponding luminescence quenching constant for Cr2O7 2− is K SV = 4.33 × 104 M−1, and the detection limit is 3.66 μM. Systematic investigations on the luminescence quenching mechanism suggest that the inner filter effect resulted in the selective detection of Cr2O7 2−. This study provides inspiration for the design and synthesis of target luminescent crystalline materials with rigid and asymmetric viologen-derived ligands. Viologen Coordination polymer Crystal structure Photochromism Luminescence Luminescence sensing Li, Min verfasserin aut Xu, Tian-Yu verfasserin aut Zhao, Bang-Tun verfasserin aut Enthalten in Spectrochimica acta / A Amsterdam [u.a.] : Elsevier Science, 1967 306 Online-Ressource (DE-627)320570983 (DE-600)2016492-0 (DE-576)090956206 1873-3557 nnns volume:306 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 306
allfieldsSound	10.1016/j.saa.2023.123579 doi (DE-627)ELV065626753 (ELSEVIER)S1386-1425(23)01264-7 DE-627 ger DE-627 rda eng 540 530 VZ 35.00 bkl Li, Zhao-Hao verfasserin aut A viologen-derived luminescent material exhibiting photochromism, photocontrolled luminescence and selective detection of Cr 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Stable viologen-derived multifunctional smart materials exhibit widespread practical applications in many areas. In this study, a viologen-derived material with 4-fold interpenetrating diamondoid network, {[Cd(1,4-ndc)(cpbpy)]·2H2O}n, was successfully constructed based on asymmetrical N-(3-carboxyphenyl)-4,4′-bipyridinium (cpbpy) and 1,4-naphthalenedicarboxylic acid (1,4-H2ndc). The compound shows reversible photochromic behavior under a xenon lamp, which are proved by UV–vis spectra and EPR characterizations. Moreover, the compound with good photoluminescence properties displays photocontrolled luminescence quenching behaviors. Owing to its good water stability, the compound is then applied in luminescence sensing for the detection of Cr2O7 2− in aqueous solution. The corresponding luminescence quenching constant for Cr2O7 2− is K SV = 4.33 × 104 M−1, and the detection limit is 3.66 μM. Systematic investigations on the luminescence quenching mechanism suggest that the inner filter effect resulted in the selective detection of Cr2O7 2−. This study provides inspiration for the design and synthesis of target luminescent crystalline materials with rigid and asymmetric viologen-derived ligands. Viologen Coordination polymer Crystal structure Photochromism Luminescence Luminescence sensing Li, Min verfasserin aut Xu, Tian-Yu verfasserin aut Zhao, Bang-Tun verfasserin aut Enthalten in Spectrochimica acta / A Amsterdam [u.a.] : Elsevier Science, 1967 306 Online-Ressource (DE-627)320570983 (DE-600)2016492-0 (DE-576)090956206 1873-3557 nnns volume:306 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 306
language	English
source	Enthalten in Spectrochimica acta / A 306 volume:306
sourceStr	Enthalten in Spectrochimica acta / A 306 volume:306
format_phy_str_mv	Article
bklname	Chemie: Allgemeines
institution	findex.gbv.de
topic_facet	Viologen Coordination polymer Crystal structure Photochromism Luminescence Luminescence sensing
dewey-raw	540
isfreeaccess_bool	false
container_title	Spectrochimica acta / A
authorswithroles_txt_mv	Li, Zhao-Hao @@aut@@ Li, Min @@aut@@ Xu, Tian-Yu @@aut@@ Zhao, Bang-Tun @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	320570983
dewey-sort	3540
id	ELV065626753
language_de	englisch
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author	Li, Zhao-Hao
spellingShingle	Li, Zhao-Hao ddc 540 bkl 35.00 misc Viologen misc Coordination polymer misc Crystal structure misc Photochromism misc Luminescence misc Luminescence sensing A viologen-derived luminescent material exhibiting photochromism, photocontrolled luminescence and selective detection of Cr
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topic_title	540 530 VZ 35.00 bkl A viologen-derived luminescent material exhibiting photochromism, photocontrolled luminescence and selective detection of Cr Viologen Coordination polymer Crystal structure Photochromism Luminescence Luminescence sensing
topic	ddc 540 bkl 35.00 misc Viologen misc Coordination polymer misc Crystal structure misc Photochromism misc Luminescence misc Luminescence sensing
topic_unstemmed	ddc 540 bkl 35.00 misc Viologen misc Coordination polymer misc Crystal structure misc Photochromism misc Luminescence misc Luminescence sensing
topic_browse	ddc 540 bkl 35.00 misc Viologen misc Coordination polymer misc Crystal structure misc Photochromism misc Luminescence misc Luminescence sensing
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title	A viologen-derived luminescent material exhibiting photochromism, photocontrolled luminescence and selective detection of Cr
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title_full	A viologen-derived luminescent material exhibiting photochromism, photocontrolled luminescence and selective detection of Cr
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title_sort	a viologen-derived luminescent material exhibiting photochromism, photocontrolled luminescence and selective detection of cr
title_auth	A viologen-derived luminescent material exhibiting photochromism, photocontrolled luminescence and selective detection of Cr
abstract	Stable viologen-derived multifunctional smart materials exhibit widespread practical applications in many areas. In this study, a viologen-derived material with 4-fold interpenetrating diamondoid network, {[Cd(1,4-ndc)(cpbpy)]·2H2O}n, was successfully constructed based on asymmetrical N-(3-carboxyphenyl)-4,4′-bipyridinium (cpbpy) and 1,4-naphthalenedicarboxylic acid (1,4-H2ndc). The compound shows reversible photochromic behavior under a xenon lamp, which are proved by UV–vis spectra and EPR characterizations. Moreover, the compound with good photoluminescence properties displays photocontrolled luminescence quenching behaviors. Owing to its good water stability, the compound is then applied in luminescence sensing for the detection of Cr2O7 2− in aqueous solution. The corresponding luminescence quenching constant for Cr2O7 2− is K SV = 4.33 × 104 M−1, and the detection limit is 3.66 μM. Systematic investigations on the luminescence quenching mechanism suggest that the inner filter effect resulted in the selective detection of Cr2O7 2−. This study provides inspiration for the design and synthesis of target luminescent crystalline materials with rigid and asymmetric viologen-derived ligands.
abstractGer	Stable viologen-derived multifunctional smart materials exhibit widespread practical applications in many areas. In this study, a viologen-derived material with 4-fold interpenetrating diamondoid network, {[Cd(1,4-ndc)(cpbpy)]·2H2O}n, was successfully constructed based on asymmetrical N-(3-carboxyphenyl)-4,4′-bipyridinium (cpbpy) and 1,4-naphthalenedicarboxylic acid (1,4-H2ndc). The compound shows reversible photochromic behavior under a xenon lamp, which are proved by UV–vis spectra and EPR characterizations. Moreover, the compound with good photoluminescence properties displays photocontrolled luminescence quenching behaviors. Owing to its good water stability, the compound is then applied in luminescence sensing for the detection of Cr2O7 2− in aqueous solution. The corresponding luminescence quenching constant for Cr2O7 2− is K SV = 4.33 × 104 M−1, and the detection limit is 3.66 μM. Systematic investigations on the luminescence quenching mechanism suggest that the inner filter effect resulted in the selective detection of Cr2O7 2−. This study provides inspiration for the design and synthesis of target luminescent crystalline materials with rigid and asymmetric viologen-derived ligands.
abstract_unstemmed	Stable viologen-derived multifunctional smart materials exhibit widespread practical applications in many areas. In this study, a viologen-derived material with 4-fold interpenetrating diamondoid network, {[Cd(1,4-ndc)(cpbpy)]·2H2O}n, was successfully constructed based on asymmetrical N-(3-carboxyphenyl)-4,4′-bipyridinium (cpbpy) and 1,4-naphthalenedicarboxylic acid (1,4-H2ndc). The compound shows reversible photochromic behavior under a xenon lamp, which are proved by UV–vis spectra and EPR characterizations. Moreover, the compound with good photoluminescence properties displays photocontrolled luminescence quenching behaviors. Owing to its good water stability, the compound is then applied in luminescence sensing for the detection of Cr2O7 2− in aqueous solution. The corresponding luminescence quenching constant for Cr2O7 2− is K SV = 4.33 × 104 M−1, and the detection limit is 3.66 μM. Systematic investigations on the luminescence quenching mechanism suggest that the inner filter effect resulted in the selective detection of Cr2O7 2−. This study provides inspiration for the design and synthesis of target luminescent crystalline materials with rigid and asymmetric viologen-derived ligands.
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title_short	A viologen-derived luminescent material exhibiting photochromism, photocontrolled luminescence and selective detection of Cr
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author2	Li, Min Xu, Tian-Yu Zhao, Bang-Tun
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doi_str	10.1016/j.saa.2023.123579
up_date	2024-07-06T23:41:21.619Z
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A viologen-derived luminescent material exhibiting photochromism, photocontrolled luminescence and selective detection of Cr

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