Carbon/iron co-product from clean hydrogen production as a tri-functional adsorbent and catalyst for efficient wastewater treatment

Clean hydrogen production via methane pyrolysis (CH4 → 2H2 + C) generates large quantities of solid carbon. Realizing their applications is a critical gap to enable its broader adoption. Here, we show that carbon nano onions encapsulated with iron cores (FeCNO) produced in CH4 pyrolysis using low-co...
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Autor*in:	Yao, Yuanyuan [verfasserIn] Pan, Yuqi [verfasserIn] Lai, Leo [verfasserIn] Yu, Zixun [verfasserIn] Chen, Jiaxiang [verfasserIn] Yu, Yanxi [verfasserIn] Darma, Terrence [verfasserIn] Tao, Yongwen [verfasserIn] Cao, Liuyue [verfasserIn] Chivers, Benjamin [verfasserIn] Zhong, Xia [verfasserIn] Wei, Li [verfasserIn] Chen, Yuan [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Sustainable hydrogen production Carbon adsorbent Hydrogen peroxide synthesis Heterogeneous Fenton catalyst Recyclable catalyst

Übergeordnetes Werk:	Enthalten in: Applied catalysis / B - Amsterdam : Elsevier, 1992, 342
Übergeordnetes Werk:	volume:342

DOI / URN:	10.1016/j.apcatb.2023.123380

Katalog-ID:	ELV06562808X

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520			\|a Clean hydrogen production via methane pyrolysis (CH4 → 2H2 + C) generates large quantities of solid carbon. Realizing their applications is a critical gap to enable its broader adoption. Here, we show that carbon nano onions encapsulated with iron cores (FeCNO) produced in CH4 pyrolysis using low-cost Fe ore catalysts can serve as a tri-functional adsorbent and catalyst for organic contaminant degradation. Fe@CNO has a high adsorption capacity and fast pseudo-second-order adsorption kinetics for antibiotics in wastewater. Surface oxidized Fe@CNO presents a high catalytic activity for in situ hydrogen peroxide production. Fe@CNO is also an efficient heterogeneous Fenton catalyst to degrade adsorbed antibiotics. Further, the Fe core is magnetic, enabling easy separation from solvents as reusable adsorbents and catalysts. We demonstrate that the adsorption and electro-Fenton process applies to various organic pollutants in different water matrices. This opens a new strategy for utilizing co-products from H2 production for sustainable environmental applications.
650		4	\|a Sustainable hydrogen production
650		4	\|a Carbon adsorbent
650		4	\|a Hydrogen peroxide synthesis
650		4	\|a Heterogeneous Fenton catalyst
650		4	\|a Recyclable catalyst
700	1		\|a Pan, Yuqi \|e verfasserin \|4 aut
700	1		\|a Lai, Leo \|e verfasserin \|4 aut
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700	1		\|a Chen, Jiaxiang \|e verfasserin \|0 (orcid)0000-0002-4525-0981 \|4 aut
700	1		\|a Yu, Yanxi \|e verfasserin \|4 aut
700	1		\|a Darma, Terrence \|e verfasserin \|0 (orcid)0009-0008-6885-4914 \|4 aut
700	1		\|a Tao, Yongwen \|e verfasserin \|4 aut
700	1		\|a Cao, Liuyue \|e verfasserin \|0 (orcid)0000-0002-4635-5187 \|4 aut
700	1		\|a Chivers, Benjamin \|e verfasserin \|4 aut
700	1		\|a Zhong, Xia \|e verfasserin \|4 aut
700	1		\|a Wei, Li \|e verfasserin \|0 (orcid)0000-0001-8771-2921 \|4 aut
700	1		\|a Chen, Yuan \|e verfasserin \|0 (orcid)0000-0001-9059-3839 \|4 aut
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allfields	10.1016/j.apcatb.2023.123380 doi (DE-627)ELV06562808X (ELSEVIER)S0926-3373(23)01023-8 DE-627 ger DE-627 rda eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Yao, Yuanyuan verfasserin aut Carbon/iron co-product from clean hydrogen production as a tri-functional adsorbent and catalyst for efficient wastewater treatment 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Clean hydrogen production via methane pyrolysis (CH4 → 2H2 + C) generates large quantities of solid carbon. Realizing their applications is a critical gap to enable its broader adoption. Here, we show that carbon nano onions encapsulated with iron cores (FeCNO) produced in CH4 pyrolysis using low-cost Fe ore catalysts can serve as a tri-functional adsorbent and catalyst for organic contaminant degradation. Fe@CNO has a high adsorption capacity and fast pseudo-second-order adsorption kinetics for antibiotics in wastewater. Surface oxidized Fe@CNO presents a high catalytic activity for in situ hydrogen peroxide production. Fe@CNO is also an efficient heterogeneous Fenton catalyst to degrade adsorbed antibiotics. Further, the Fe core is magnetic, enabling easy separation from solvents as reusable adsorbents and catalysts. We demonstrate that the adsorption and electro-Fenton process applies to various organic pollutants in different water matrices. This opens a new strategy for utilizing co-products from H2 production for sustainable environmental applications. Sustainable hydrogen production Carbon adsorbent Hydrogen peroxide synthesis Heterogeneous Fenton catalyst Recyclable catalyst Pan, Yuqi verfasserin aut Lai, Leo verfasserin aut Yu, Zixun verfasserin aut Chen, Jiaxiang verfasserin (orcid)0000-0002-4525-0981 aut Yu, Yanxi verfasserin aut Darma, Terrence verfasserin (orcid)0009-0008-6885-4914 aut Tao, Yongwen verfasserin aut Cao, Liuyue verfasserin (orcid)0000-0002-4635-5187 aut Chivers, Benjamin verfasserin aut Zhong, Xia verfasserin aut Wei, Li verfasserin (orcid)0000-0001-8771-2921 aut Chen, Yuan verfasserin (orcid)0000-0001-9059-3839 aut Enthalten in Applied catalysis / B Amsterdam : Elsevier, 1992 342 Online-Ressource (DE-627)320578658 (DE-600)2017331-3 (DE-576)095956344 0926-3373 nnns volume:342 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 342
spelling	10.1016/j.apcatb.2023.123380 doi (DE-627)ELV06562808X (ELSEVIER)S0926-3373(23)01023-8 DE-627 ger DE-627 rda eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Yao, Yuanyuan verfasserin aut Carbon/iron co-product from clean hydrogen production as a tri-functional adsorbent and catalyst for efficient wastewater treatment 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Clean hydrogen production via methane pyrolysis (CH4 → 2H2 + C) generates large quantities of solid carbon. Realizing their applications is a critical gap to enable its broader adoption. Here, we show that carbon nano onions encapsulated with iron cores (FeCNO) produced in CH4 pyrolysis using low-cost Fe ore catalysts can serve as a tri-functional adsorbent and catalyst for organic contaminant degradation. Fe@CNO has a high adsorption capacity and fast pseudo-second-order adsorption kinetics for antibiotics in wastewater. Surface oxidized Fe@CNO presents a high catalytic activity for in situ hydrogen peroxide production. Fe@CNO is also an efficient heterogeneous Fenton catalyst to degrade adsorbed antibiotics. Further, the Fe core is magnetic, enabling easy separation from solvents as reusable adsorbents and catalysts. We demonstrate that the adsorption and electro-Fenton process applies to various organic pollutants in different water matrices. This opens a new strategy for utilizing co-products from H2 production for sustainable environmental applications. Sustainable hydrogen production Carbon adsorbent Hydrogen peroxide synthesis Heterogeneous Fenton catalyst Recyclable catalyst Pan, Yuqi verfasserin aut Lai, Leo verfasserin aut Yu, Zixun verfasserin aut Chen, Jiaxiang verfasserin (orcid)0000-0002-4525-0981 aut Yu, Yanxi verfasserin aut Darma, Terrence verfasserin (orcid)0009-0008-6885-4914 aut Tao, Yongwen verfasserin aut Cao, Liuyue verfasserin (orcid)0000-0002-4635-5187 aut Chivers, Benjamin verfasserin aut Zhong, Xia verfasserin aut Wei, Li verfasserin (orcid)0000-0001-8771-2921 aut Chen, Yuan verfasserin (orcid)0000-0001-9059-3839 aut Enthalten in Applied catalysis / B Amsterdam : Elsevier, 1992 342 Online-Ressource (DE-627)320578658 (DE-600)2017331-3 (DE-576)095956344 0926-3373 nnns volume:342 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 342
allfields_unstemmed	10.1016/j.apcatb.2023.123380 doi (DE-627)ELV06562808X (ELSEVIER)S0926-3373(23)01023-8 DE-627 ger DE-627 rda eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Yao, Yuanyuan verfasserin aut Carbon/iron co-product from clean hydrogen production as a tri-functional adsorbent and catalyst for efficient wastewater treatment 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Clean hydrogen production via methane pyrolysis (CH4 → 2H2 + C) generates large quantities of solid carbon. Realizing their applications is a critical gap to enable its broader adoption. Here, we show that carbon nano onions encapsulated with iron cores (FeCNO) produced in CH4 pyrolysis using low-cost Fe ore catalysts can serve as a tri-functional adsorbent and catalyst for organic contaminant degradation. Fe@CNO has a high adsorption capacity and fast pseudo-second-order adsorption kinetics for antibiotics in wastewater. Surface oxidized Fe@CNO presents a high catalytic activity for in situ hydrogen peroxide production. Fe@CNO is also an efficient heterogeneous Fenton catalyst to degrade adsorbed antibiotics. Further, the Fe core is magnetic, enabling easy separation from solvents as reusable adsorbents and catalysts. We demonstrate that the adsorption and electro-Fenton process applies to various organic pollutants in different water matrices. This opens a new strategy for utilizing co-products from H2 production for sustainable environmental applications. Sustainable hydrogen production Carbon adsorbent Hydrogen peroxide synthesis Heterogeneous Fenton catalyst Recyclable catalyst Pan, Yuqi verfasserin aut Lai, Leo verfasserin aut Yu, Zixun verfasserin aut Chen, Jiaxiang verfasserin (orcid)0000-0002-4525-0981 aut Yu, Yanxi verfasserin aut Darma, Terrence verfasserin (orcid)0009-0008-6885-4914 aut Tao, Yongwen verfasserin aut Cao, Liuyue verfasserin (orcid)0000-0002-4635-5187 aut Chivers, Benjamin verfasserin aut Zhong, Xia verfasserin aut Wei, Li verfasserin (orcid)0000-0001-8771-2921 aut Chen, Yuan verfasserin (orcid)0000-0001-9059-3839 aut Enthalten in Applied catalysis / B Amsterdam : Elsevier, 1992 342 Online-Ressource (DE-627)320578658 (DE-600)2017331-3 (DE-576)095956344 0926-3373 nnns volume:342 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 342
allfieldsGer	10.1016/j.apcatb.2023.123380 doi (DE-627)ELV06562808X (ELSEVIER)S0926-3373(23)01023-8 DE-627 ger DE-627 rda eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Yao, Yuanyuan verfasserin aut Carbon/iron co-product from clean hydrogen production as a tri-functional adsorbent and catalyst for efficient wastewater treatment 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Clean hydrogen production via methane pyrolysis (CH4 → 2H2 + C) generates large quantities of solid carbon. Realizing their applications is a critical gap to enable its broader adoption. Here, we show that carbon nano onions encapsulated with iron cores (FeCNO) produced in CH4 pyrolysis using low-cost Fe ore catalysts can serve as a tri-functional adsorbent and catalyst for organic contaminant degradation. Fe@CNO has a high adsorption capacity and fast pseudo-second-order adsorption kinetics for antibiotics in wastewater. Surface oxidized Fe@CNO presents a high catalytic activity for in situ hydrogen peroxide production. Fe@CNO is also an efficient heterogeneous Fenton catalyst to degrade adsorbed antibiotics. Further, the Fe core is magnetic, enabling easy separation from solvents as reusable adsorbents and catalysts. We demonstrate that the adsorption and electro-Fenton process applies to various organic pollutants in different water matrices. This opens a new strategy for utilizing co-products from H2 production for sustainable environmental applications. Sustainable hydrogen production Carbon adsorbent Hydrogen peroxide synthesis Heterogeneous Fenton catalyst Recyclable catalyst Pan, Yuqi verfasserin aut Lai, Leo verfasserin aut Yu, Zixun verfasserin aut Chen, Jiaxiang verfasserin (orcid)0000-0002-4525-0981 aut Yu, Yanxi verfasserin aut Darma, Terrence verfasserin (orcid)0009-0008-6885-4914 aut Tao, Yongwen verfasserin aut Cao, Liuyue verfasserin (orcid)0000-0002-4635-5187 aut Chivers, Benjamin verfasserin aut Zhong, Xia verfasserin aut Wei, Li verfasserin (orcid)0000-0001-8771-2921 aut Chen, Yuan verfasserin (orcid)0000-0001-9059-3839 aut Enthalten in Applied catalysis / B Amsterdam : Elsevier, 1992 342 Online-Ressource (DE-627)320578658 (DE-600)2017331-3 (DE-576)095956344 0926-3373 nnns volume:342 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 342
allfieldsSound	10.1016/j.apcatb.2023.123380 doi (DE-627)ELV06562808X (ELSEVIER)S0926-3373(23)01023-8 DE-627 ger DE-627 rda eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Yao, Yuanyuan verfasserin aut Carbon/iron co-product from clean hydrogen production as a tri-functional adsorbent and catalyst for efficient wastewater treatment 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Clean hydrogen production via methane pyrolysis (CH4 → 2H2 + C) generates large quantities of solid carbon. Realizing their applications is a critical gap to enable its broader adoption. Here, we show that carbon nano onions encapsulated with iron cores (FeCNO) produced in CH4 pyrolysis using low-cost Fe ore catalysts can serve as a tri-functional adsorbent and catalyst for organic contaminant degradation. Fe@CNO has a high adsorption capacity and fast pseudo-second-order adsorption kinetics for antibiotics in wastewater. Surface oxidized Fe@CNO presents a high catalytic activity for in situ hydrogen peroxide production. Fe@CNO is also an efficient heterogeneous Fenton catalyst to degrade adsorbed antibiotics. Further, the Fe core is magnetic, enabling easy separation from solvents as reusable adsorbents and catalysts. We demonstrate that the adsorption and electro-Fenton process applies to various organic pollutants in different water matrices. This opens a new strategy for utilizing co-products from H2 production for sustainable environmental applications. Sustainable hydrogen production Carbon adsorbent Hydrogen peroxide synthesis Heterogeneous Fenton catalyst Recyclable catalyst Pan, Yuqi verfasserin aut Lai, Leo verfasserin aut Yu, Zixun verfasserin aut Chen, Jiaxiang verfasserin (orcid)0000-0002-4525-0981 aut Yu, Yanxi verfasserin aut Darma, Terrence verfasserin (orcid)0009-0008-6885-4914 aut Tao, Yongwen verfasserin aut Cao, Liuyue verfasserin (orcid)0000-0002-4635-5187 aut Chivers, Benjamin verfasserin aut Zhong, Xia verfasserin aut Wei, Li verfasserin (orcid)0000-0001-8771-2921 aut Chen, Yuan verfasserin (orcid)0000-0001-9059-3839 aut Enthalten in Applied catalysis / B Amsterdam : Elsevier, 1992 342 Online-Ressource (DE-627)320578658 (DE-600)2017331-3 (DE-576)095956344 0926-3373 nnns volume:342 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 342
language	English
source	Enthalten in Applied catalysis / B 342 volume:342
sourceStr	Enthalten in Applied catalysis / B 342 volume:342
format_phy_str_mv	Article
bklname	Katalyse Umwelttechnik: Allgemeines Umweltchemie
institution	findex.gbv.de
topic_facet	Sustainable hydrogen production Carbon adsorbent Hydrogen peroxide synthesis Heterogeneous Fenton catalyst Recyclable catalyst
dewey-raw	540
isfreeaccess_bool	false
container_title	Applied catalysis / B
authorswithroles_txt_mv	Yao, Yuanyuan @@aut@@ Pan, Yuqi @@aut@@ Lai, Leo @@aut@@ Yu, Zixun @@aut@@ Chen, Jiaxiang @@aut@@ Yu, Yanxi @@aut@@ Darma, Terrence @@aut@@ Tao, Yongwen @@aut@@ Cao, Liuyue @@aut@@ Chivers, Benjamin @@aut@@ Zhong, Xia @@aut@@ Wei, Li @@aut@@ Chen, Yuan @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	320578658
dewey-sort	3540
id	ELV06562808X
language_de	englisch
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author	Yao, Yuanyuan
spellingShingle	Yao, Yuanyuan ddc 540 bkl 35.17 bkl 58.50 bkl 43.12 misc Sustainable hydrogen production misc Carbon adsorbent misc Hydrogen peroxide synthesis misc Heterogeneous Fenton catalyst misc Recyclable catalyst Carbon/iron co-product from clean hydrogen production as a tri-functional adsorbent and catalyst for efficient wastewater treatment
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topic_title	540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Carbon/iron co-product from clean hydrogen production as a tri-functional adsorbent and catalyst for efficient wastewater treatment Sustainable hydrogen production Carbon adsorbent Hydrogen peroxide synthesis Heterogeneous Fenton catalyst Recyclable catalyst
topic	ddc 540 bkl 35.17 bkl 58.50 bkl 43.12 misc Sustainable hydrogen production misc Carbon adsorbent misc Hydrogen peroxide synthesis misc Heterogeneous Fenton catalyst misc Recyclable catalyst
topic_unstemmed	ddc 540 bkl 35.17 bkl 58.50 bkl 43.12 misc Sustainable hydrogen production misc Carbon adsorbent misc Hydrogen peroxide synthesis misc Heterogeneous Fenton catalyst misc Recyclable catalyst
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title	Carbon/iron co-product from clean hydrogen production as a tri-functional adsorbent and catalyst for efficient wastewater treatment
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title_full	Carbon/iron co-product from clean hydrogen production as a tri-functional adsorbent and catalyst for efficient wastewater treatment
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author_browse	Yao, Yuanyuan Pan, Yuqi Lai, Leo Yu, Zixun Chen, Jiaxiang Yu, Yanxi Darma, Terrence Tao, Yongwen Cao, Liuyue Chivers, Benjamin Zhong, Xia Wei, Li Chen, Yuan
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title_sort	carbon/iron co-product from clean hydrogen production as a tri-functional adsorbent and catalyst for efficient wastewater treatment
title_auth	Carbon/iron co-product from clean hydrogen production as a tri-functional adsorbent and catalyst for efficient wastewater treatment
abstract	Clean hydrogen production via methane pyrolysis (CH4 → 2H2 + C) generates large quantities of solid carbon. Realizing their applications is a critical gap to enable its broader adoption. Here, we show that carbon nano onions encapsulated with iron cores (FeCNO) produced in CH4 pyrolysis using low-cost Fe ore catalysts can serve as a tri-functional adsorbent and catalyst for organic contaminant degradation. Fe@CNO has a high adsorption capacity and fast pseudo-second-order adsorption kinetics for antibiotics in wastewater. Surface oxidized Fe@CNO presents a high catalytic activity for in situ hydrogen peroxide production. Fe@CNO is also an efficient heterogeneous Fenton catalyst to degrade adsorbed antibiotics. Further, the Fe core is magnetic, enabling easy separation from solvents as reusable adsorbents and catalysts. We demonstrate that the adsorption and electro-Fenton process applies to various organic pollutants in different water matrices. This opens a new strategy for utilizing co-products from H2 production for sustainable environmental applications.
abstractGer	Clean hydrogen production via methane pyrolysis (CH4 → 2H2 + C) generates large quantities of solid carbon. Realizing their applications is a critical gap to enable its broader adoption. Here, we show that carbon nano onions encapsulated with iron cores (FeCNO) produced in CH4 pyrolysis using low-cost Fe ore catalysts can serve as a tri-functional adsorbent and catalyst for organic contaminant degradation. Fe@CNO has a high adsorption capacity and fast pseudo-second-order adsorption kinetics for antibiotics in wastewater. Surface oxidized Fe@CNO presents a high catalytic activity for in situ hydrogen peroxide production. Fe@CNO is also an efficient heterogeneous Fenton catalyst to degrade adsorbed antibiotics. Further, the Fe core is magnetic, enabling easy separation from solvents as reusable adsorbents and catalysts. We demonstrate that the adsorption and electro-Fenton process applies to various organic pollutants in different water matrices. This opens a new strategy for utilizing co-products from H2 production for sustainable environmental applications.
abstract_unstemmed	Clean hydrogen production via methane pyrolysis (CH4 → 2H2 + C) generates large quantities of solid carbon. Realizing their applications is a critical gap to enable its broader adoption. Here, we show that carbon nano onions encapsulated with iron cores (FeCNO) produced in CH4 pyrolysis using low-cost Fe ore catalysts can serve as a tri-functional adsorbent and catalyst for organic contaminant degradation. Fe@CNO has a high adsorption capacity and fast pseudo-second-order adsorption kinetics for antibiotics in wastewater. Surface oxidized Fe@CNO presents a high catalytic activity for in situ hydrogen peroxide production. Fe@CNO is also an efficient heterogeneous Fenton catalyst to degrade adsorbed antibiotics. Further, the Fe core is magnetic, enabling easy separation from solvents as reusable adsorbents and catalysts. We demonstrate that the adsorption and electro-Fenton process applies to various organic pollutants in different water matrices. This opens a new strategy for utilizing co-products from H2 production for sustainable environmental applications.
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title_short	Carbon/iron co-product from clean hydrogen production as a tri-functional adsorbent and catalyst for efficient wastewater treatment
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author2	Pan, Yuqi Lai, Leo Yu, Zixun Chen, Jiaxiang Yu, Yanxi Darma, Terrence Tao, Yongwen Cao, Liuyue Chivers, Benjamin Zhong, Xia Wei, Li Chen, Yuan
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doi_str	10.1016/j.apcatb.2023.123380
up_date	2024-07-06T23:41:38.185Z
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Realizing their applications is a critical gap to enable its broader adoption. Here, we show that carbon nano onions encapsulated with iron cores (FeCNO) produced in CH4 pyrolysis using low-cost Fe ore catalysts can serve as a tri-functional adsorbent and catalyst for organic contaminant degradation. Fe@CNO has a high adsorption capacity and fast pseudo-second-order adsorption kinetics for antibiotics in wastewater. Surface oxidized Fe@CNO presents a high catalytic activity for in situ hydrogen peroxide production. Fe@CNO is also an efficient heterogeneous Fenton catalyst to degrade adsorbed antibiotics. Further, the Fe core is magnetic, enabling easy separation from solvents as reusable adsorbents and catalysts. We demonstrate that the adsorption and electro-Fenton process applies to various organic pollutants in different water matrices. 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Carbon/iron co-product from clean hydrogen production as a tri-functional adsorbent and catalyst for efficient wastewater treatment

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