A hybrid anaerobic osmotic membrane bioreactor - membrane distillation for water reclamation: aquatic toxicity, membrane fouling characterization, and economic assessment
The incomplete removal of pharmaceutically active compounds (PhACs) by conventional wastewater treatment has been challenging due to their ecological implications. Therefore, advanced technologies are necessary to remove PhACs efficiently. In the present study, an anaerobic osmotic membrane bioreact...
Ausführliche Beschreibung
Autor*in: |
Santos, Carolina Rodrigues [verfasserIn] Arcanjo, Gemima Santos [verfasserIn] Santos, Lucilaine Valéria de Souza [verfasserIn] Silva, Priscila Romana [verfasserIn] Mounteer, Ann H. [verfasserIn] Silva, Ubiana de Cássia Mourão [verfasserIn] Santos, Vera Lúcia [verfasserIn] Amaral, Míriam Cristina Santos [verfasserIn] |
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E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2023 |
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Übergeordnetes Werk: |
Enthalten in: The chemical engineering journal - Amsterdam : Elsevier, 1997, 477 |
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Übergeordnetes Werk: |
volume:477 |
DOI / URN: |
10.1016/j.cej.2023.146283 |
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Katalog-ID: |
ELV065752201 |
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245 | 1 | 0 | |a A hybrid anaerobic osmotic membrane bioreactor - membrane distillation for water reclamation: aquatic toxicity, membrane fouling characterization, and economic assessment |
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520 | |a The incomplete removal of pharmaceutically active compounds (PhACs) by conventional wastewater treatment has been challenging due to their ecological implications. Therefore, advanced technologies are necessary to remove PhACs efficiently. In the present study, an anaerobic osmotic membrane bioreactor - membrane distillation (AnOMBR-MD), aiming to remove seven PhACs, was evaluated by an integrated approach, considering the environmental toxicity, fouling characterization, and economic assessment. PhACs removal was evaluated using liquid chromatography coupled with mass spectrometry. Besides, organic matter and nutrient removal were evaluated. The FO and MD membrane fouling was characterized with scanning electron microscopy and energy dispersive spectroscopy. Toxic effects were analyzed for Aliivibrio fischeri, Daphnia similis, and Raphidocelis subcapitata. Furthermore, a preliminary economic assessment was carried out using capital and operating expenditures. The results showed a DOC, N-NH4 +, and P-PO4 3- removal of 92%, 97%, and 99.9%, respectively, while removal of PhACs was >96%. However, the distillate was classified as very toxic for R. subcapitata, and a strong correlation was found between toxicity and the Mg2+ originating from the draw solution (DS). This result showed the importance of including toxicity tests in the selection of DS. The economic evaluation indicated that the higher cost is related to the membrane replacement due to the decrease in the permeate flux, pointing out the need for future studies that address cleaning strategies to solve the organic and inorganic fouling on the membrane's surface. In this sense, this study promoted an improvement in understanding the AnOMBR-MD technical-economic viability aiming at full-scale application. | ||
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700 | 1 | |a Arcanjo, Gemima Santos |e verfasserin |4 aut | |
700 | 1 | |a Santos, Lucilaine Valéria de Souza |e verfasserin |4 aut | |
700 | 1 | |a Silva, Priscila Romana |e verfasserin |4 aut | |
700 | 1 | |a Mounteer, Ann H. |e verfasserin |4 aut | |
700 | 1 | |a Silva, Ubiana de Cássia Mourão |e verfasserin |4 aut | |
700 | 1 | |a Santos, Vera Lúcia |e verfasserin |4 aut | |
700 | 1 | |a Amaral, Míriam Cristina Santos |e verfasserin |4 aut | |
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10.1016/j.cej.2023.146283 doi (DE-627)ELV065752201 (ELSEVIER)S1385-8947(23)05014-3 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Santos, Carolina Rodrigues verfasserin aut A hybrid anaerobic osmotic membrane bioreactor - membrane distillation for water reclamation: aquatic toxicity, membrane fouling characterization, and economic assessment 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The incomplete removal of pharmaceutically active compounds (PhACs) by conventional wastewater treatment has been challenging due to their ecological implications. Therefore, advanced technologies are necessary to remove PhACs efficiently. In the present study, an anaerobic osmotic membrane bioreactor - membrane distillation (AnOMBR-MD), aiming to remove seven PhACs, was evaluated by an integrated approach, considering the environmental toxicity, fouling characterization, and economic assessment. PhACs removal was evaluated using liquid chromatography coupled with mass spectrometry. Besides, organic matter and nutrient removal were evaluated. The FO and MD membrane fouling was characterized with scanning electron microscopy and energy dispersive spectroscopy. Toxic effects were analyzed for Aliivibrio fischeri, Daphnia similis, and Raphidocelis subcapitata. Furthermore, a preliminary economic assessment was carried out using capital and operating expenditures. The results showed a DOC, N-NH4 +, and P-PO4 3- removal of 92%, 97%, and 99.9%, respectively, while removal of PhACs was >96%. However, the distillate was classified as very toxic for R. subcapitata, and a strong correlation was found between toxicity and the Mg2+ originating from the draw solution (DS). This result showed the importance of including toxicity tests in the selection of DS. The economic evaluation indicated that the higher cost is related to the membrane replacement due to the decrease in the permeate flux, pointing out the need for future studies that address cleaning strategies to solve the organic and inorganic fouling on the membrane's surface. In this sense, this study promoted an improvement in understanding the AnOMBR-MD technical-economic viability aiming at full-scale application. Osmotic membrane bioreactor Membrane distillation Toxicity Pharmaceutical Cost Arcanjo, Gemima Santos verfasserin aut Santos, Lucilaine Valéria de Souza verfasserin aut Silva, Priscila Romana verfasserin aut Mounteer, Ann H. verfasserin aut Silva, Ubiana de Cássia Mourão verfasserin aut Santos, Vera Lúcia verfasserin aut Amaral, Míriam Cristina Santos verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 477 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:477 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 477 |
spelling |
10.1016/j.cej.2023.146283 doi (DE-627)ELV065752201 (ELSEVIER)S1385-8947(23)05014-3 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Santos, Carolina Rodrigues verfasserin aut A hybrid anaerobic osmotic membrane bioreactor - membrane distillation for water reclamation: aquatic toxicity, membrane fouling characterization, and economic assessment 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The incomplete removal of pharmaceutically active compounds (PhACs) by conventional wastewater treatment has been challenging due to their ecological implications. Therefore, advanced technologies are necessary to remove PhACs efficiently. In the present study, an anaerobic osmotic membrane bioreactor - membrane distillation (AnOMBR-MD), aiming to remove seven PhACs, was evaluated by an integrated approach, considering the environmental toxicity, fouling characterization, and economic assessment. PhACs removal was evaluated using liquid chromatography coupled with mass spectrometry. Besides, organic matter and nutrient removal were evaluated. The FO and MD membrane fouling was characterized with scanning electron microscopy and energy dispersive spectroscopy. Toxic effects were analyzed for Aliivibrio fischeri, Daphnia similis, and Raphidocelis subcapitata. Furthermore, a preliminary economic assessment was carried out using capital and operating expenditures. The results showed a DOC, N-NH4 +, and P-PO4 3- removal of 92%, 97%, and 99.9%, respectively, while removal of PhACs was >96%. However, the distillate was classified as very toxic for R. subcapitata, and a strong correlation was found between toxicity and the Mg2+ originating from the draw solution (DS). This result showed the importance of including toxicity tests in the selection of DS. The economic evaluation indicated that the higher cost is related to the membrane replacement due to the decrease in the permeate flux, pointing out the need for future studies that address cleaning strategies to solve the organic and inorganic fouling on the membrane's surface. In this sense, this study promoted an improvement in understanding the AnOMBR-MD technical-economic viability aiming at full-scale application. Osmotic membrane bioreactor Membrane distillation Toxicity Pharmaceutical Cost Arcanjo, Gemima Santos verfasserin aut Santos, Lucilaine Valéria de Souza verfasserin aut Silva, Priscila Romana verfasserin aut Mounteer, Ann H. verfasserin aut Silva, Ubiana de Cássia Mourão verfasserin aut Santos, Vera Lúcia verfasserin aut Amaral, Míriam Cristina Santos verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 477 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:477 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 477 |
allfields_unstemmed |
10.1016/j.cej.2023.146283 doi (DE-627)ELV065752201 (ELSEVIER)S1385-8947(23)05014-3 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Santos, Carolina Rodrigues verfasserin aut A hybrid anaerobic osmotic membrane bioreactor - membrane distillation for water reclamation: aquatic toxicity, membrane fouling characterization, and economic assessment 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The incomplete removal of pharmaceutically active compounds (PhACs) by conventional wastewater treatment has been challenging due to their ecological implications. Therefore, advanced technologies are necessary to remove PhACs efficiently. In the present study, an anaerobic osmotic membrane bioreactor - membrane distillation (AnOMBR-MD), aiming to remove seven PhACs, was evaluated by an integrated approach, considering the environmental toxicity, fouling characterization, and economic assessment. PhACs removal was evaluated using liquid chromatography coupled with mass spectrometry. Besides, organic matter and nutrient removal were evaluated. The FO and MD membrane fouling was characterized with scanning electron microscopy and energy dispersive spectroscopy. Toxic effects were analyzed for Aliivibrio fischeri, Daphnia similis, and Raphidocelis subcapitata. Furthermore, a preliminary economic assessment was carried out using capital and operating expenditures. The results showed a DOC, N-NH4 +, and P-PO4 3- removal of 92%, 97%, and 99.9%, respectively, while removal of PhACs was >96%. However, the distillate was classified as very toxic for R. subcapitata, and a strong correlation was found between toxicity and the Mg2+ originating from the draw solution (DS). This result showed the importance of including toxicity tests in the selection of DS. The economic evaluation indicated that the higher cost is related to the membrane replacement due to the decrease in the permeate flux, pointing out the need for future studies that address cleaning strategies to solve the organic and inorganic fouling on the membrane's surface. In this sense, this study promoted an improvement in understanding the AnOMBR-MD technical-economic viability aiming at full-scale application. Osmotic membrane bioreactor Membrane distillation Toxicity Pharmaceutical Cost Arcanjo, Gemima Santos verfasserin aut Santos, Lucilaine Valéria de Souza verfasserin aut Silva, Priscila Romana verfasserin aut Mounteer, Ann H. verfasserin aut Silva, Ubiana de Cássia Mourão verfasserin aut Santos, Vera Lúcia verfasserin aut Amaral, Míriam Cristina Santos verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 477 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:477 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 477 |
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10.1016/j.cej.2023.146283 doi (DE-627)ELV065752201 (ELSEVIER)S1385-8947(23)05014-3 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Santos, Carolina Rodrigues verfasserin aut A hybrid anaerobic osmotic membrane bioreactor - membrane distillation for water reclamation: aquatic toxicity, membrane fouling characterization, and economic assessment 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The incomplete removal of pharmaceutically active compounds (PhACs) by conventional wastewater treatment has been challenging due to their ecological implications. Therefore, advanced technologies are necessary to remove PhACs efficiently. In the present study, an anaerobic osmotic membrane bioreactor - membrane distillation (AnOMBR-MD), aiming to remove seven PhACs, was evaluated by an integrated approach, considering the environmental toxicity, fouling characterization, and economic assessment. PhACs removal was evaluated using liquid chromatography coupled with mass spectrometry. Besides, organic matter and nutrient removal were evaluated. The FO and MD membrane fouling was characterized with scanning electron microscopy and energy dispersive spectroscopy. Toxic effects were analyzed for Aliivibrio fischeri, Daphnia similis, and Raphidocelis subcapitata. Furthermore, a preliminary economic assessment was carried out using capital and operating expenditures. The results showed a DOC, N-NH4 +, and P-PO4 3- removal of 92%, 97%, and 99.9%, respectively, while removal of PhACs was >96%. However, the distillate was classified as very toxic for R. subcapitata, and a strong correlation was found between toxicity and the Mg2+ originating from the draw solution (DS). This result showed the importance of including toxicity tests in the selection of DS. The economic evaluation indicated that the higher cost is related to the membrane replacement due to the decrease in the permeate flux, pointing out the need for future studies that address cleaning strategies to solve the organic and inorganic fouling on the membrane's surface. In this sense, this study promoted an improvement in understanding the AnOMBR-MD technical-economic viability aiming at full-scale application. Osmotic membrane bioreactor Membrane distillation Toxicity Pharmaceutical Cost Arcanjo, Gemima Santos verfasserin aut Santos, Lucilaine Valéria de Souza verfasserin aut Silva, Priscila Romana verfasserin aut Mounteer, Ann H. verfasserin aut Silva, Ubiana de Cássia Mourão verfasserin aut Santos, Vera Lúcia verfasserin aut Amaral, Míriam Cristina Santos verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 477 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:477 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 477 |
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10.1016/j.cej.2023.146283 doi (DE-627)ELV065752201 (ELSEVIER)S1385-8947(23)05014-3 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Santos, Carolina Rodrigues verfasserin aut A hybrid anaerobic osmotic membrane bioreactor - membrane distillation for water reclamation: aquatic toxicity, membrane fouling characterization, and economic assessment 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The incomplete removal of pharmaceutically active compounds (PhACs) by conventional wastewater treatment has been challenging due to their ecological implications. Therefore, advanced technologies are necessary to remove PhACs efficiently. In the present study, an anaerobic osmotic membrane bioreactor - membrane distillation (AnOMBR-MD), aiming to remove seven PhACs, was evaluated by an integrated approach, considering the environmental toxicity, fouling characterization, and economic assessment. PhACs removal was evaluated using liquid chromatography coupled with mass spectrometry. Besides, organic matter and nutrient removal were evaluated. The FO and MD membrane fouling was characterized with scanning electron microscopy and energy dispersive spectroscopy. Toxic effects were analyzed for Aliivibrio fischeri, Daphnia similis, and Raphidocelis subcapitata. Furthermore, a preliminary economic assessment was carried out using capital and operating expenditures. The results showed a DOC, N-NH4 +, and P-PO4 3- removal of 92%, 97%, and 99.9%, respectively, while removal of PhACs was >96%. However, the distillate was classified as very toxic for R. subcapitata, and a strong correlation was found between toxicity and the Mg2+ originating from the draw solution (DS). This result showed the importance of including toxicity tests in the selection of DS. The economic evaluation indicated that the higher cost is related to the membrane replacement due to the decrease in the permeate flux, pointing out the need for future studies that address cleaning strategies to solve the organic and inorganic fouling on the membrane's surface. In this sense, this study promoted an improvement in understanding the AnOMBR-MD technical-economic viability aiming at full-scale application. Osmotic membrane bioreactor Membrane distillation Toxicity Pharmaceutical Cost Arcanjo, Gemima Santos verfasserin aut Santos, Lucilaine Valéria de Souza verfasserin aut Silva, Priscila Romana verfasserin aut Mounteer, Ann H. verfasserin aut Silva, Ubiana de Cássia Mourão verfasserin aut Santos, Vera Lúcia verfasserin aut Amaral, Míriam Cristina Santos verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 477 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:477 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 477 |
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Santos, Carolina Rodrigues @@aut@@ Arcanjo, Gemima Santos @@aut@@ Santos, Lucilaine Valéria de Souza @@aut@@ Silva, Priscila Romana @@aut@@ Mounteer, Ann H. @@aut@@ Silva, Ubiana de Cássia Mourão @@aut@@ Santos, Vera Lúcia @@aut@@ Amaral, Míriam Cristina Santos @@aut@@ |
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Santos, Carolina Rodrigues |
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660 VZ 58.10 bkl A hybrid anaerobic osmotic membrane bioreactor - membrane distillation for water reclamation: aquatic toxicity, membrane fouling characterization, and economic assessment Osmotic membrane bioreactor Membrane distillation Toxicity Pharmaceutical Cost |
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Santos, Carolina Rodrigues Arcanjo, Gemima Santos Santos, Lucilaine Valéria de Souza Silva, Priscila Romana Mounteer, Ann H. Silva, Ubiana de Cássia Mourão Santos, Vera Lúcia Amaral, Míriam Cristina Santos |
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a hybrid anaerobic osmotic membrane bioreactor - membrane distillation for water reclamation: aquatic toxicity, membrane fouling characterization, and economic assessment |
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A hybrid anaerobic osmotic membrane bioreactor - membrane distillation for water reclamation: aquatic toxicity, membrane fouling characterization, and economic assessment |
abstract |
The incomplete removal of pharmaceutically active compounds (PhACs) by conventional wastewater treatment has been challenging due to their ecological implications. Therefore, advanced technologies are necessary to remove PhACs efficiently. In the present study, an anaerobic osmotic membrane bioreactor - membrane distillation (AnOMBR-MD), aiming to remove seven PhACs, was evaluated by an integrated approach, considering the environmental toxicity, fouling characterization, and economic assessment. PhACs removal was evaluated using liquid chromatography coupled with mass spectrometry. Besides, organic matter and nutrient removal were evaluated. The FO and MD membrane fouling was characterized with scanning electron microscopy and energy dispersive spectroscopy. Toxic effects were analyzed for Aliivibrio fischeri, Daphnia similis, and Raphidocelis subcapitata. Furthermore, a preliminary economic assessment was carried out using capital and operating expenditures. The results showed a DOC, N-NH4 +, and P-PO4 3- removal of 92%, 97%, and 99.9%, respectively, while removal of PhACs was >96%. However, the distillate was classified as very toxic for R. subcapitata, and a strong correlation was found between toxicity and the Mg2+ originating from the draw solution (DS). This result showed the importance of including toxicity tests in the selection of DS. The economic evaluation indicated that the higher cost is related to the membrane replacement due to the decrease in the permeate flux, pointing out the need for future studies that address cleaning strategies to solve the organic and inorganic fouling on the membrane's surface. In this sense, this study promoted an improvement in understanding the AnOMBR-MD technical-economic viability aiming at full-scale application. |
abstractGer |
The incomplete removal of pharmaceutically active compounds (PhACs) by conventional wastewater treatment has been challenging due to their ecological implications. Therefore, advanced technologies are necessary to remove PhACs efficiently. In the present study, an anaerobic osmotic membrane bioreactor - membrane distillation (AnOMBR-MD), aiming to remove seven PhACs, was evaluated by an integrated approach, considering the environmental toxicity, fouling characterization, and economic assessment. PhACs removal was evaluated using liquid chromatography coupled with mass spectrometry. Besides, organic matter and nutrient removal were evaluated. The FO and MD membrane fouling was characterized with scanning electron microscopy and energy dispersive spectroscopy. Toxic effects were analyzed for Aliivibrio fischeri, Daphnia similis, and Raphidocelis subcapitata. Furthermore, a preliminary economic assessment was carried out using capital and operating expenditures. The results showed a DOC, N-NH4 +, and P-PO4 3- removal of 92%, 97%, and 99.9%, respectively, while removal of PhACs was >96%. However, the distillate was classified as very toxic for R. subcapitata, and a strong correlation was found between toxicity and the Mg2+ originating from the draw solution (DS). This result showed the importance of including toxicity tests in the selection of DS. The economic evaluation indicated that the higher cost is related to the membrane replacement due to the decrease in the permeate flux, pointing out the need for future studies that address cleaning strategies to solve the organic and inorganic fouling on the membrane's surface. In this sense, this study promoted an improvement in understanding the AnOMBR-MD technical-economic viability aiming at full-scale application. |
abstract_unstemmed |
The incomplete removal of pharmaceutically active compounds (PhACs) by conventional wastewater treatment has been challenging due to their ecological implications. Therefore, advanced technologies are necessary to remove PhACs efficiently. In the present study, an anaerobic osmotic membrane bioreactor - membrane distillation (AnOMBR-MD), aiming to remove seven PhACs, was evaluated by an integrated approach, considering the environmental toxicity, fouling characterization, and economic assessment. PhACs removal was evaluated using liquid chromatography coupled with mass spectrometry. Besides, organic matter and nutrient removal were evaluated. The FO and MD membrane fouling was characterized with scanning electron microscopy and energy dispersive spectroscopy. Toxic effects were analyzed for Aliivibrio fischeri, Daphnia similis, and Raphidocelis subcapitata. Furthermore, a preliminary economic assessment was carried out using capital and operating expenditures. The results showed a DOC, N-NH4 +, and P-PO4 3- removal of 92%, 97%, and 99.9%, respectively, while removal of PhACs was >96%. However, the distillate was classified as very toxic for R. subcapitata, and a strong correlation was found between toxicity and the Mg2+ originating from the draw solution (DS). This result showed the importance of including toxicity tests in the selection of DS. The economic evaluation indicated that the higher cost is related to the membrane replacement due to the decrease in the permeate flux, pointing out the need for future studies that address cleaning strategies to solve the organic and inorganic fouling on the membrane's surface. In this sense, this study promoted an improvement in understanding the AnOMBR-MD technical-economic viability aiming at full-scale application. |
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title_short |
A hybrid anaerobic osmotic membrane bioreactor - membrane distillation for water reclamation: aquatic toxicity, membrane fouling characterization, and economic assessment |
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Arcanjo, Gemima Santos Santos, Lucilaine Valéria de Souza Silva, Priscila Romana Mounteer, Ann H. Silva, Ubiana de Cássia Mourão Santos, Vera Lúcia Amaral, Míriam Cristina Santos |
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