Ion migration mediated high Seebeck effect in halide perovskites and application in infrared detection
Thermoelectric materials play an important role in thermopower systems, thermal sensing and infrared photo-thermoelectric imaging. Ionic thermoelectric materials have recently attracted attentions considering their relatively high Seebeck coefficient. However, the ionic thermoelectric materials have...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Xiong, Yan [verfasserIn] Shen, Zixi [verfasserIn] Yuan, Shunsheng [verfasserIn] Liu, Yuting [verfasserIn] Jin, Tong [verfasserIn] Liang, Yudong [verfasserIn] Masrour, Rachid [verfasserIn] Niu, Guangda [verfasserIn] Xu, Ling [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2023 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: The chemical engineering journal - Amsterdam : Elsevier, 1997, 477 |
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| Übergeordnetes Werk: |
volume:477 |
| DOI / URN: |
10.1016/j.cej.2023.147168 |
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| Katalog-ID: |
ELV065755332 |
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| 245 | 1 | 0 | |a Ion migration mediated high Seebeck effect in halide perovskites and application in infrared detection |
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| 520 | |a Thermoelectric materials play an important role in thermopower systems, thermal sensing and infrared photo-thermoelectric imaging. Ionic thermoelectric materials have recently attracted attentions considering their relatively high Seebeck coefficient. However, the ionic thermoelectric materials have to use liquid or hydrogels for ion conduction, and are susceptible to leakage, evaporation and portability issues. Metal halide perovskites possess low thermal conductivity and prominent ion migration characteristics, making them theoretically suitable candidates for thermoelectric conversion. Here we present the first-ever study of the ionic thermoelectric properties in typical solid perovskite composition MAPbI3, revealing an extremely high Seebeck coefficient of 35.7 mV/K. Furthermore, the assembled photo-thermoelectric detector of carbon/MAPbI3 single crystal/carbon demonstrated a high response (0.58 V/W) toward infrared light and the imaging test was well resolved. This research provides a novel avenue to investigate efficient thermoelectric devices based on ionic and electronic mixed conductors and develop photo-thermoelectric applications. | ||
| 650 | 4 | |a Perovskite | |
| 650 | 4 | |a Ionic Seebeck coefficient | |
| 650 | 4 | |a Ion migration | |
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| 700 | 1 | |a Shen, Zixi |e verfasserin |4 aut | |
| 700 | 1 | |a Yuan, Shunsheng |e verfasserin |0 (orcid)0009-0005-4435-6273 |4 aut | |
| 700 | 1 | |a Liu, Yuting |e verfasserin |4 aut | |
| 700 | 1 | |a Jin, Tong |e verfasserin |0 (orcid)0009-0003-0366-3731 |4 aut | |
| 700 | 1 | |a Liang, Yudong |e verfasserin |4 aut | |
| 700 | 1 | |a Masrour, Rachid |e verfasserin |4 aut | |
| 700 | 1 | |a Niu, Guangda |e verfasserin |4 aut | |
| 700 | 1 | |a Xu, Ling |e verfasserin |0 (orcid)0000-0001-9676-5769 |4 aut | |
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10.1016/j.cej.2023.147168 doi (DE-627)ELV065755332 (ELSEVIER)S1385-8947(23)05899-0 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Xiong, Yan verfasserin aut Ion migration mediated high Seebeck effect in halide perovskites and application in infrared detection 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Thermoelectric materials play an important role in thermopower systems, thermal sensing and infrared photo-thermoelectric imaging. Ionic thermoelectric materials have recently attracted attentions considering their relatively high Seebeck coefficient. However, the ionic thermoelectric materials have to use liquid or hydrogels for ion conduction, and are susceptible to leakage, evaporation and portability issues. Metal halide perovskites possess low thermal conductivity and prominent ion migration characteristics, making them theoretically suitable candidates for thermoelectric conversion. Here we present the first-ever study of the ionic thermoelectric properties in typical solid perovskite composition MAPbI3, revealing an extremely high Seebeck coefficient of 35.7 mV/K. Furthermore, the assembled photo-thermoelectric detector of carbon/MAPbI3 single crystal/carbon demonstrated a high response (0.58 V/W) toward infrared light and the imaging test was well resolved. This research provides a novel avenue to investigate efficient thermoelectric devices based on ionic and electronic mixed conductors and develop photo-thermoelectric applications. Perovskite Ionic Seebeck coefficient Ion migration Photo-thermoelectric detection Shen, Zixi verfasserin aut Yuan, Shunsheng verfasserin (orcid)0009-0005-4435-6273 aut Liu, Yuting verfasserin aut Jin, Tong verfasserin (orcid)0009-0003-0366-3731 aut Liang, Yudong verfasserin aut Masrour, Rachid verfasserin aut Niu, Guangda verfasserin aut Xu, Ling verfasserin (orcid)0000-0001-9676-5769 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 477 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:477 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 477 |
| spelling |
10.1016/j.cej.2023.147168 doi (DE-627)ELV065755332 (ELSEVIER)S1385-8947(23)05899-0 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Xiong, Yan verfasserin aut Ion migration mediated high Seebeck effect in halide perovskites and application in infrared detection 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Thermoelectric materials play an important role in thermopower systems, thermal sensing and infrared photo-thermoelectric imaging. Ionic thermoelectric materials have recently attracted attentions considering their relatively high Seebeck coefficient. However, the ionic thermoelectric materials have to use liquid or hydrogels for ion conduction, and are susceptible to leakage, evaporation and portability issues. Metal halide perovskites possess low thermal conductivity and prominent ion migration characteristics, making them theoretically suitable candidates for thermoelectric conversion. Here we present the first-ever study of the ionic thermoelectric properties in typical solid perovskite composition MAPbI3, revealing an extremely high Seebeck coefficient of 35.7 mV/K. Furthermore, the assembled photo-thermoelectric detector of carbon/MAPbI3 single crystal/carbon demonstrated a high response (0.58 V/W) toward infrared light and the imaging test was well resolved. This research provides a novel avenue to investigate efficient thermoelectric devices based on ionic and electronic mixed conductors and develop photo-thermoelectric applications. Perovskite Ionic Seebeck coefficient Ion migration Photo-thermoelectric detection Shen, Zixi verfasserin aut Yuan, Shunsheng verfasserin (orcid)0009-0005-4435-6273 aut Liu, Yuting verfasserin aut Jin, Tong verfasserin (orcid)0009-0003-0366-3731 aut Liang, Yudong verfasserin aut Masrour, Rachid verfasserin aut Niu, Guangda verfasserin aut Xu, Ling verfasserin (orcid)0000-0001-9676-5769 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 477 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:477 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 477 |
| allfields_unstemmed |
10.1016/j.cej.2023.147168 doi (DE-627)ELV065755332 (ELSEVIER)S1385-8947(23)05899-0 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Xiong, Yan verfasserin aut Ion migration mediated high Seebeck effect in halide perovskites and application in infrared detection 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Thermoelectric materials play an important role in thermopower systems, thermal sensing and infrared photo-thermoelectric imaging. Ionic thermoelectric materials have recently attracted attentions considering their relatively high Seebeck coefficient. However, the ionic thermoelectric materials have to use liquid or hydrogels for ion conduction, and are susceptible to leakage, evaporation and portability issues. Metal halide perovskites possess low thermal conductivity and prominent ion migration characteristics, making them theoretically suitable candidates for thermoelectric conversion. Here we present the first-ever study of the ionic thermoelectric properties in typical solid perovskite composition MAPbI3, revealing an extremely high Seebeck coefficient of 35.7 mV/K. Furthermore, the assembled photo-thermoelectric detector of carbon/MAPbI3 single crystal/carbon demonstrated a high response (0.58 V/W) toward infrared light and the imaging test was well resolved. This research provides a novel avenue to investigate efficient thermoelectric devices based on ionic and electronic mixed conductors and develop photo-thermoelectric applications. Perovskite Ionic Seebeck coefficient Ion migration Photo-thermoelectric detection Shen, Zixi verfasserin aut Yuan, Shunsheng verfasserin (orcid)0009-0005-4435-6273 aut Liu, Yuting verfasserin aut Jin, Tong verfasserin (orcid)0009-0003-0366-3731 aut Liang, Yudong verfasserin aut Masrour, Rachid verfasserin aut Niu, Guangda verfasserin aut Xu, Ling verfasserin (orcid)0000-0001-9676-5769 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 477 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:477 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 477 |
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10.1016/j.cej.2023.147168 doi (DE-627)ELV065755332 (ELSEVIER)S1385-8947(23)05899-0 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Xiong, Yan verfasserin aut Ion migration mediated high Seebeck effect in halide perovskites and application in infrared detection 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Thermoelectric materials play an important role in thermopower systems, thermal sensing and infrared photo-thermoelectric imaging. Ionic thermoelectric materials have recently attracted attentions considering their relatively high Seebeck coefficient. However, the ionic thermoelectric materials have to use liquid or hydrogels for ion conduction, and are susceptible to leakage, evaporation and portability issues. Metal halide perovskites possess low thermal conductivity and prominent ion migration characteristics, making them theoretically suitable candidates for thermoelectric conversion. Here we present the first-ever study of the ionic thermoelectric properties in typical solid perovskite composition MAPbI3, revealing an extremely high Seebeck coefficient of 35.7 mV/K. Furthermore, the assembled photo-thermoelectric detector of carbon/MAPbI3 single crystal/carbon demonstrated a high response (0.58 V/W) toward infrared light and the imaging test was well resolved. This research provides a novel avenue to investigate efficient thermoelectric devices based on ionic and electronic mixed conductors and develop photo-thermoelectric applications. Perovskite Ionic Seebeck coefficient Ion migration Photo-thermoelectric detection Shen, Zixi verfasserin aut Yuan, Shunsheng verfasserin (orcid)0009-0005-4435-6273 aut Liu, Yuting verfasserin aut Jin, Tong verfasserin (orcid)0009-0003-0366-3731 aut Liang, Yudong verfasserin aut Masrour, Rachid verfasserin aut Niu, Guangda verfasserin aut Xu, Ling verfasserin (orcid)0000-0001-9676-5769 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 477 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:477 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 477 |
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10.1016/j.cej.2023.147168 doi (DE-627)ELV065755332 (ELSEVIER)S1385-8947(23)05899-0 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Xiong, Yan verfasserin aut Ion migration mediated high Seebeck effect in halide perovskites and application in infrared detection 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Thermoelectric materials play an important role in thermopower systems, thermal sensing and infrared photo-thermoelectric imaging. Ionic thermoelectric materials have recently attracted attentions considering their relatively high Seebeck coefficient. However, the ionic thermoelectric materials have to use liquid or hydrogels for ion conduction, and are susceptible to leakage, evaporation and portability issues. Metal halide perovskites possess low thermal conductivity and prominent ion migration characteristics, making them theoretically suitable candidates for thermoelectric conversion. Here we present the first-ever study of the ionic thermoelectric properties in typical solid perovskite composition MAPbI3, revealing an extremely high Seebeck coefficient of 35.7 mV/K. Furthermore, the assembled photo-thermoelectric detector of carbon/MAPbI3 single crystal/carbon demonstrated a high response (0.58 V/W) toward infrared light and the imaging test was well resolved. This research provides a novel avenue to investigate efficient thermoelectric devices based on ionic and electronic mixed conductors and develop photo-thermoelectric applications. Perovskite Ionic Seebeck coefficient Ion migration Photo-thermoelectric detection Shen, Zixi verfasserin aut Yuan, Shunsheng verfasserin (orcid)0009-0005-4435-6273 aut Liu, Yuting verfasserin aut Jin, Tong verfasserin (orcid)0009-0003-0366-3731 aut Liang, Yudong verfasserin aut Masrour, Rachid verfasserin aut Niu, Guangda verfasserin aut Xu, Ling verfasserin (orcid)0000-0001-9676-5769 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 477 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:477 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 477 |
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ion migration mediated high seebeck effect in halide perovskites and application in infrared detection |
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Ion migration mediated high Seebeck effect in halide perovskites and application in infrared detection |
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Thermoelectric materials play an important role in thermopower systems, thermal sensing and infrared photo-thermoelectric imaging. Ionic thermoelectric materials have recently attracted attentions considering their relatively high Seebeck coefficient. However, the ionic thermoelectric materials have to use liquid or hydrogels for ion conduction, and are susceptible to leakage, evaporation and portability issues. Metal halide perovskites possess low thermal conductivity and prominent ion migration characteristics, making them theoretically suitable candidates for thermoelectric conversion. Here we present the first-ever study of the ionic thermoelectric properties in typical solid perovskite composition MAPbI3, revealing an extremely high Seebeck coefficient of 35.7 mV/K. Furthermore, the assembled photo-thermoelectric detector of carbon/MAPbI3 single crystal/carbon demonstrated a high response (0.58 V/W) toward infrared light and the imaging test was well resolved. This research provides a novel avenue to investigate efficient thermoelectric devices based on ionic and electronic mixed conductors and develop photo-thermoelectric applications. |
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Thermoelectric materials play an important role in thermopower systems, thermal sensing and infrared photo-thermoelectric imaging. Ionic thermoelectric materials have recently attracted attentions considering their relatively high Seebeck coefficient. However, the ionic thermoelectric materials have to use liquid or hydrogels for ion conduction, and are susceptible to leakage, evaporation and portability issues. Metal halide perovskites possess low thermal conductivity and prominent ion migration characteristics, making them theoretically suitable candidates for thermoelectric conversion. Here we present the first-ever study of the ionic thermoelectric properties in typical solid perovskite composition MAPbI3, revealing an extremely high Seebeck coefficient of 35.7 mV/K. Furthermore, the assembled photo-thermoelectric detector of carbon/MAPbI3 single crystal/carbon demonstrated a high response (0.58 V/W) toward infrared light and the imaging test was well resolved. This research provides a novel avenue to investigate efficient thermoelectric devices based on ionic and electronic mixed conductors and develop photo-thermoelectric applications. |
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Thermoelectric materials play an important role in thermopower systems, thermal sensing and infrared photo-thermoelectric imaging. Ionic thermoelectric materials have recently attracted attentions considering their relatively high Seebeck coefficient. However, the ionic thermoelectric materials have to use liquid or hydrogels for ion conduction, and are susceptible to leakage, evaporation and portability issues. Metal halide perovskites possess low thermal conductivity and prominent ion migration characteristics, making them theoretically suitable candidates for thermoelectric conversion. Here we present the first-ever study of the ionic thermoelectric properties in typical solid perovskite composition MAPbI3, revealing an extremely high Seebeck coefficient of 35.7 mV/K. Furthermore, the assembled photo-thermoelectric detector of carbon/MAPbI3 single crystal/carbon demonstrated a high response (0.58 V/W) toward infrared light and the imaging test was well resolved. This research provides a novel avenue to investigate efficient thermoelectric devices based on ionic and electronic mixed conductors and develop photo-thermoelectric applications. |
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| score |
7.3998547 |