Superhydrophilic fluorinated heterogeneous membranes with boosting antifouling property and high stable permeance for efficient emulsion separation

It is yet a query that whether chemically heterogeneous superwetting surface is able to enhance the permeability and anti-fouling capability of membrane contemporaneously, heretofore which is lacking and well worth creating. Here, we propose a bio-adhesion coupled with self-assembly strategy, to con...
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Autor*in:	Wang, Lulu [verfasserIn] Liu, Jie [verfasserIn] Zhang, Ruilong [verfasserIn] Wu, Junda [verfasserIn] Tian, Xiaohua [verfasserIn] Chen, Li [verfasserIn] Dai, Xiaohui [verfasserIn] Yan, Yongsheng [verfasserIn] Pan, Jianming [verfasserIn] Dai, Jiangdong [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Chemically heterogeneous surface Superwetting membrane Improved permeance Anti-fouling self-cleaning Emulsion separation

Übergeordnetes Werk:	Enthalten in: Journal of membrane science - New York, NY [u.a.] : Elsevier, 1976, 691
Übergeordnetes Werk:	volume:691

DOI / URN:	10.1016/j.memsci.2023.122253

Katalog-ID:	ELV065830903

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245	1	0	\|a Superhydrophilic fluorinated heterogeneous membranes with boosting antifouling property and high stable permeance for efficient emulsion separation
264		1	\|c 2023
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520			\|a It is yet a query that whether chemically heterogeneous superwetting surface is able to enhance the permeability and anti-fouling capability of membrane contemporaneously, heretofore which is lacking and well worth creating. Here, we propose a bio-adhesion coupled with self-assembly strategy, to construct superhydrophilic fluorinated heterogeneous membranes, through in-situ biomimetic adhesion of the hydrophilic polyphenol-silane coating (TAT) on the porous PVDF membrane, as a secondary reaction platform, and subsequently self-assembly of amphoteric fluorocarbon surfactant (FS-50). Unsurprisingly, we find that introducing FS-50 not only significantly strengthens the permeability, but also improves the anti-fouling self-cleaning, thanks to the formation of robust hydration layer and slippery micro-domains with low friction, to realize the dual anti-fouling effects of pollution resistance and release. The champion PVDF/TAT/FS-2.0 % composite membrane exhibits superhydrophilic and underwater superoleophobic (oil contact angle above 162.3°) property with very low oil-adhesion. This composite membrane possesses an ultrahigh water permeance of 29214.6 L m−2 h−1 bar−1, which is 2.8 times larger than that of pristine PVDF membrane. The PVDF/TAT/FS-2.0 % composite membrane presents the high separation efficiencies (above 99.5 %) for various surfactant-stabilized oil-in-water emulsions and high permeances of 3193.2–4212.3 L m−2 h−1 bar−1. Especially, the membrane at continuous operation for 1.0 h can reach a high stable permeance of 2505.1 L m−2 h−1 bar−1. Moreover, this composite membrane shows strong chemical stability and robustness. This research answers the initial question, and provides the insight for further design and production of chemically heterogeneous superwetting membranes with high permeability, selectivity and antifouling ability.
650		4	\|a Chemically heterogeneous surface
650		4	\|a Superwetting membrane
650		4	\|a Improved permeance
650		4	\|a Anti-fouling self-cleaning
650		4	\|a Emulsion separation
700	1		\|a Liu, Jie \|e verfasserin \|4 aut
700	1		\|a Zhang, Ruilong \|e verfasserin \|4 aut
700	1		\|a Wu, Junda \|e verfasserin \|4 aut
700	1		\|a Tian, Xiaohua \|e verfasserin \|4 aut
700	1		\|a Chen, Li \|e verfasserin \|4 aut
700	1		\|a Dai, Xiaohui \|e verfasserin \|4 aut
700	1		\|a Yan, Yongsheng \|e verfasserin \|4 aut
700	1		\|a Pan, Jianming \|e verfasserin \|4 aut
700	1		\|a Dai, Jiangdong \|e verfasserin \|4 aut
773	0	8	\|i Enthalten in \|t Journal of membrane science \|d New York, NY [u.a.] : Elsevier, 1976 \|g 691 \|h Online-Ressource \|w (DE-627)302468927 \|w (DE-600)1491419-0 \|w (DE-576)259483907 \|x 0376-7388 \|7 nnns
773	1	8	\|g volume:691
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912			\|a GBV_ILN_32
912			\|a GBV_ILN_40
912			\|a GBV_ILN_60
912			\|a GBV_ILN_62
912			\|a GBV_ILN_65
912			\|a GBV_ILN_69
912			\|a GBV_ILN_70
912			\|a GBV_ILN_73
912			\|a GBV_ILN_74
912			\|a GBV_ILN_90
912			\|a GBV_ILN_95
912			\|a GBV_ILN_100
912			\|a GBV_ILN_101
912			\|a GBV_ILN_105
912			\|a GBV_ILN_110
912			\|a GBV_ILN_150
912			\|a GBV_ILN_151
912			\|a GBV_ILN_187
912			\|a GBV_ILN_213
912			\|a GBV_ILN_224
912			\|a GBV_ILN_230
912			\|a GBV_ILN_370
912			\|a GBV_ILN_602
912			\|a GBV_ILN_702
912			\|a GBV_ILN_2001
912			\|a GBV_ILN_2003
912			\|a GBV_ILN_2004
912			\|a GBV_ILN_2005
912			\|a GBV_ILN_2007
912			\|a GBV_ILN_2008
912			\|a GBV_ILN_2009
912			\|a GBV_ILN_2010
912			\|a GBV_ILN_2011
912			\|a GBV_ILN_2014
912			\|a GBV_ILN_2015
912			\|a GBV_ILN_2020
912			\|a GBV_ILN_2021
912			\|a GBV_ILN_2025
912			\|a GBV_ILN_2026
912			\|a GBV_ILN_2027
912			\|a GBV_ILN_2034
912			\|a GBV_ILN_2044
912			\|a GBV_ILN_2048
912			\|a GBV_ILN_2049
912			\|a GBV_ILN_2050
912			\|a GBV_ILN_2055
912			\|a GBV_ILN_2056
912			\|a GBV_ILN_2059
912			\|a GBV_ILN_2061
912			\|a GBV_ILN_2064
912			\|a GBV_ILN_2088
912			\|a GBV_ILN_2106
912			\|a GBV_ILN_2110
912			\|a GBV_ILN_2111
912			\|a GBV_ILN_2112
912			\|a GBV_ILN_2122
912			\|a GBV_ILN_2129
912			\|a GBV_ILN_2143
912			\|a GBV_ILN_2152
912			\|a GBV_ILN_2153
912			\|a GBV_ILN_2190
912			\|a GBV_ILN_2232
912			\|a GBV_ILN_2336
912			\|a GBV_ILN_2470
912			\|a GBV_ILN_2507
912			\|a GBV_ILN_4035
912			\|a GBV_ILN_4037
912			\|a GBV_ILN_4112
912			\|a GBV_ILN_4125
912			\|a GBV_ILN_4242
912			\|a GBV_ILN_4249
912			\|a GBV_ILN_4251
912			\|a GBV_ILN_4305
912			\|a GBV_ILN_4306
912			\|a GBV_ILN_4307
912			\|a GBV_ILN_4313
912			\|a GBV_ILN_4322
912			\|a GBV_ILN_4323
912			\|a GBV_ILN_4324
912			\|a GBV_ILN_4325
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912			\|a GBV_ILN_4333
912			\|a GBV_ILN_4334
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936	b	k	\|a 58.11 \|j Mechanische Verfahrenstechnik \|q VZ
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Indexfelder

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matchkey_str	article:03767388:2023----::uehdohlcloiaehtrgnosebaewtbotnatfuigrprynhgsalpre
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publishDate	2023
allfields	10.1016/j.memsci.2023.122253 doi (DE-627)ELV065830903 (ELSEVIER)S0376-7388(23)00909-2 DE-627 ger DE-627 rda eng 570 VZ 58.11 bkl Wang, Lulu verfasserin aut Superhydrophilic fluorinated heterogeneous membranes with boosting antifouling property and high stable permeance for efficient emulsion separation 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier It is yet a query that whether chemically heterogeneous superwetting surface is able to enhance the permeability and anti-fouling capability of membrane contemporaneously, heretofore which is lacking and well worth creating. Here, we propose a bio-adhesion coupled with self-assembly strategy, to construct superhydrophilic fluorinated heterogeneous membranes, through in-situ biomimetic adhesion of the hydrophilic polyphenol-silane coating (TAT) on the porous PVDF membrane, as a secondary reaction platform, and subsequently self-assembly of amphoteric fluorocarbon surfactant (FS-50). Unsurprisingly, we find that introducing FS-50 not only significantly strengthens the permeability, but also improves the anti-fouling self-cleaning, thanks to the formation of robust hydration layer and slippery micro-domains with low friction, to realize the dual anti-fouling effects of pollution resistance and release. The champion PVDF/TAT/FS-2.0 % composite membrane exhibits superhydrophilic and underwater superoleophobic (oil contact angle above 162.3°) property with very low oil-adhesion. This composite membrane possesses an ultrahigh water permeance of 29214.6 L m−2 h−1 bar−1, which is 2.8 times larger than that of pristine PVDF membrane. The PVDF/TAT/FS-2.0 % composite membrane presents the high separation efficiencies (above 99.5 %) for various surfactant-stabilized oil-in-water emulsions and high permeances of 3193.2–4212.3 L m−2 h−1 bar−1. Especially, the membrane at continuous operation for 1.0 h can reach a high stable permeance of 2505.1 L m−2 h−1 bar−1. Moreover, this composite membrane shows strong chemical stability and robustness. This research answers the initial question, and provides the insight for further design and production of chemically heterogeneous superwetting membranes with high permeability, selectivity and antifouling ability. Chemically heterogeneous surface Superwetting membrane Improved permeance Anti-fouling self-cleaning Emulsion separation Liu, Jie verfasserin aut Zhang, Ruilong verfasserin aut Wu, Junda verfasserin aut Tian, Xiaohua verfasserin aut Chen, Li verfasserin aut Dai, Xiaohui verfasserin aut Yan, Yongsheng verfasserin aut Pan, Jianming verfasserin aut Dai, Jiangdong verfasserin aut Enthalten in Journal of membrane science New York, NY [u.a.] : Elsevier, 1976 691 Online-Ressource (DE-627)302468927 (DE-600)1491419-0 (DE-576)259483907 0376-7388 nnns volume:691 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.11 Mechanische Verfahrenstechnik VZ AR 691
spelling	10.1016/j.memsci.2023.122253 doi (DE-627)ELV065830903 (ELSEVIER)S0376-7388(23)00909-2 DE-627 ger DE-627 rda eng 570 VZ 58.11 bkl Wang, Lulu verfasserin aut Superhydrophilic fluorinated heterogeneous membranes with boosting antifouling property and high stable permeance for efficient emulsion separation 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier It is yet a query that whether chemically heterogeneous superwetting surface is able to enhance the permeability and anti-fouling capability of membrane contemporaneously, heretofore which is lacking and well worth creating. Here, we propose a bio-adhesion coupled with self-assembly strategy, to construct superhydrophilic fluorinated heterogeneous membranes, through in-situ biomimetic adhesion of the hydrophilic polyphenol-silane coating (TAT) on the porous PVDF membrane, as a secondary reaction platform, and subsequently self-assembly of amphoteric fluorocarbon surfactant (FS-50). Unsurprisingly, we find that introducing FS-50 not only significantly strengthens the permeability, but also improves the anti-fouling self-cleaning, thanks to the formation of robust hydration layer and slippery micro-domains with low friction, to realize the dual anti-fouling effects of pollution resistance and release. The champion PVDF/TAT/FS-2.0 % composite membrane exhibits superhydrophilic and underwater superoleophobic (oil contact angle above 162.3°) property with very low oil-adhesion. This composite membrane possesses an ultrahigh water permeance of 29214.6 L m−2 h−1 bar−1, which is 2.8 times larger than that of pristine PVDF membrane. The PVDF/TAT/FS-2.0 % composite membrane presents the high separation efficiencies (above 99.5 %) for various surfactant-stabilized oil-in-water emulsions and high permeances of 3193.2–4212.3 L m−2 h−1 bar−1. Especially, the membrane at continuous operation for 1.0 h can reach a high stable permeance of 2505.1 L m−2 h−1 bar−1. Moreover, this composite membrane shows strong chemical stability and robustness. This research answers the initial question, and provides the insight for further design and production of chemically heterogeneous superwetting membranes with high permeability, selectivity and antifouling ability. Chemically heterogeneous surface Superwetting membrane Improved permeance Anti-fouling self-cleaning Emulsion separation Liu, Jie verfasserin aut Zhang, Ruilong verfasserin aut Wu, Junda verfasserin aut Tian, Xiaohua verfasserin aut Chen, Li verfasserin aut Dai, Xiaohui verfasserin aut Yan, Yongsheng verfasserin aut Pan, Jianming verfasserin aut Dai, Jiangdong verfasserin aut Enthalten in Journal of membrane science New York, NY [u.a.] : Elsevier, 1976 691 Online-Ressource (DE-627)302468927 (DE-600)1491419-0 (DE-576)259483907 0376-7388 nnns volume:691 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.11 Mechanische Verfahrenstechnik VZ AR 691
allfields_unstemmed	10.1016/j.memsci.2023.122253 doi (DE-627)ELV065830903 (ELSEVIER)S0376-7388(23)00909-2 DE-627 ger DE-627 rda eng 570 VZ 58.11 bkl Wang, Lulu verfasserin aut Superhydrophilic fluorinated heterogeneous membranes with boosting antifouling property and high stable permeance for efficient emulsion separation 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier It is yet a query that whether chemically heterogeneous superwetting surface is able to enhance the permeability and anti-fouling capability of membrane contemporaneously, heretofore which is lacking and well worth creating. Here, we propose a bio-adhesion coupled with self-assembly strategy, to construct superhydrophilic fluorinated heterogeneous membranes, through in-situ biomimetic adhesion of the hydrophilic polyphenol-silane coating (TAT) on the porous PVDF membrane, as a secondary reaction platform, and subsequently self-assembly of amphoteric fluorocarbon surfactant (FS-50). Unsurprisingly, we find that introducing FS-50 not only significantly strengthens the permeability, but also improves the anti-fouling self-cleaning, thanks to the formation of robust hydration layer and slippery micro-domains with low friction, to realize the dual anti-fouling effects of pollution resistance and release. The champion PVDF/TAT/FS-2.0 % composite membrane exhibits superhydrophilic and underwater superoleophobic (oil contact angle above 162.3°) property with very low oil-adhesion. This composite membrane possesses an ultrahigh water permeance of 29214.6 L m−2 h−1 bar−1, which is 2.8 times larger than that of pristine PVDF membrane. The PVDF/TAT/FS-2.0 % composite membrane presents the high separation efficiencies (above 99.5 %) for various surfactant-stabilized oil-in-water emulsions and high permeances of 3193.2–4212.3 L m−2 h−1 bar−1. Especially, the membrane at continuous operation for 1.0 h can reach a high stable permeance of 2505.1 L m−2 h−1 bar−1. Moreover, this composite membrane shows strong chemical stability and robustness. This research answers the initial question, and provides the insight for further design and production of chemically heterogeneous superwetting membranes with high permeability, selectivity and antifouling ability. Chemically heterogeneous surface Superwetting membrane Improved permeance Anti-fouling self-cleaning Emulsion separation Liu, Jie verfasserin aut Zhang, Ruilong verfasserin aut Wu, Junda verfasserin aut Tian, Xiaohua verfasserin aut Chen, Li verfasserin aut Dai, Xiaohui verfasserin aut Yan, Yongsheng verfasserin aut Pan, Jianming verfasserin aut Dai, Jiangdong verfasserin aut Enthalten in Journal of membrane science New York, NY [u.a.] : Elsevier, 1976 691 Online-Ressource (DE-627)302468927 (DE-600)1491419-0 (DE-576)259483907 0376-7388 nnns volume:691 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.11 Mechanische Verfahrenstechnik VZ AR 691
allfieldsGer	10.1016/j.memsci.2023.122253 doi (DE-627)ELV065830903 (ELSEVIER)S0376-7388(23)00909-2 DE-627 ger DE-627 rda eng 570 VZ 58.11 bkl Wang, Lulu verfasserin aut Superhydrophilic fluorinated heterogeneous membranes with boosting antifouling property and high stable permeance for efficient emulsion separation 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier It is yet a query that whether chemically heterogeneous superwetting surface is able to enhance the permeability and anti-fouling capability of membrane contemporaneously, heretofore which is lacking and well worth creating. Here, we propose a bio-adhesion coupled with self-assembly strategy, to construct superhydrophilic fluorinated heterogeneous membranes, through in-situ biomimetic adhesion of the hydrophilic polyphenol-silane coating (TAT) on the porous PVDF membrane, as a secondary reaction platform, and subsequently self-assembly of amphoteric fluorocarbon surfactant (FS-50). Unsurprisingly, we find that introducing FS-50 not only significantly strengthens the permeability, but also improves the anti-fouling self-cleaning, thanks to the formation of robust hydration layer and slippery micro-domains with low friction, to realize the dual anti-fouling effects of pollution resistance and release. The champion PVDF/TAT/FS-2.0 % composite membrane exhibits superhydrophilic and underwater superoleophobic (oil contact angle above 162.3°) property with very low oil-adhesion. This composite membrane possesses an ultrahigh water permeance of 29214.6 L m−2 h−1 bar−1, which is 2.8 times larger than that of pristine PVDF membrane. The PVDF/TAT/FS-2.0 % composite membrane presents the high separation efficiencies (above 99.5 %) for various surfactant-stabilized oil-in-water emulsions and high permeances of 3193.2–4212.3 L m−2 h−1 bar−1. Especially, the membrane at continuous operation for 1.0 h can reach a high stable permeance of 2505.1 L m−2 h−1 bar−1. Moreover, this composite membrane shows strong chemical stability and robustness. This research answers the initial question, and provides the insight for further design and production of chemically heterogeneous superwetting membranes with high permeability, selectivity and antifouling ability. Chemically heterogeneous surface Superwetting membrane Improved permeance Anti-fouling self-cleaning Emulsion separation Liu, Jie verfasserin aut Zhang, Ruilong verfasserin aut Wu, Junda verfasserin aut Tian, Xiaohua verfasserin aut Chen, Li verfasserin aut Dai, Xiaohui verfasserin aut Yan, Yongsheng verfasserin aut Pan, Jianming verfasserin aut Dai, Jiangdong verfasserin aut Enthalten in Journal of membrane science New York, NY [u.a.] : Elsevier, 1976 691 Online-Ressource (DE-627)302468927 (DE-600)1491419-0 (DE-576)259483907 0376-7388 nnns volume:691 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.11 Mechanische Verfahrenstechnik VZ AR 691
allfieldsSound	10.1016/j.memsci.2023.122253 doi (DE-627)ELV065830903 (ELSEVIER)S0376-7388(23)00909-2 DE-627 ger DE-627 rda eng 570 VZ 58.11 bkl Wang, Lulu verfasserin aut Superhydrophilic fluorinated heterogeneous membranes with boosting antifouling property and high stable permeance for efficient emulsion separation 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier It is yet a query that whether chemically heterogeneous superwetting surface is able to enhance the permeability and anti-fouling capability of membrane contemporaneously, heretofore which is lacking and well worth creating. Here, we propose a bio-adhesion coupled with self-assembly strategy, to construct superhydrophilic fluorinated heterogeneous membranes, through in-situ biomimetic adhesion of the hydrophilic polyphenol-silane coating (TAT) on the porous PVDF membrane, as a secondary reaction platform, and subsequently self-assembly of amphoteric fluorocarbon surfactant (FS-50). Unsurprisingly, we find that introducing FS-50 not only significantly strengthens the permeability, but also improves the anti-fouling self-cleaning, thanks to the formation of robust hydration layer and slippery micro-domains with low friction, to realize the dual anti-fouling effects of pollution resistance and release. The champion PVDF/TAT/FS-2.0 % composite membrane exhibits superhydrophilic and underwater superoleophobic (oil contact angle above 162.3°) property with very low oil-adhesion. This composite membrane possesses an ultrahigh water permeance of 29214.6 L m−2 h−1 bar−1, which is 2.8 times larger than that of pristine PVDF membrane. The PVDF/TAT/FS-2.0 % composite membrane presents the high separation efficiencies (above 99.5 %) for various surfactant-stabilized oil-in-water emulsions and high permeances of 3193.2–4212.3 L m−2 h−1 bar−1. Especially, the membrane at continuous operation for 1.0 h can reach a high stable permeance of 2505.1 L m−2 h−1 bar−1. Moreover, this composite membrane shows strong chemical stability and robustness. This research answers the initial question, and provides the insight for further design and production of chemically heterogeneous superwetting membranes with high permeability, selectivity and antifouling ability. Chemically heterogeneous surface Superwetting membrane Improved permeance Anti-fouling self-cleaning Emulsion separation Liu, Jie verfasserin aut Zhang, Ruilong verfasserin aut Wu, Junda verfasserin aut Tian, Xiaohua verfasserin aut Chen, Li verfasserin aut Dai, Xiaohui verfasserin aut Yan, Yongsheng verfasserin aut Pan, Jianming verfasserin aut Dai, Jiangdong verfasserin aut Enthalten in Journal of membrane science New York, NY [u.a.] : Elsevier, 1976 691 Online-Ressource (DE-627)302468927 (DE-600)1491419-0 (DE-576)259483907 0376-7388 nnns volume:691 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.11 Mechanische Verfahrenstechnik VZ AR 691
language	English
source	Enthalten in Journal of membrane science 691 volume:691
sourceStr	Enthalten in Journal of membrane science 691 volume:691
format_phy_str_mv	Article
bklname	Mechanische Verfahrenstechnik
institution	findex.gbv.de
topic_facet	Chemically heterogeneous surface Superwetting membrane Improved permeance Anti-fouling self-cleaning Emulsion separation
dewey-raw	570
isfreeaccess_bool	false
container_title	Journal of membrane science
authorswithroles_txt_mv	Wang, Lulu @@aut@@ Liu, Jie @@aut@@ Zhang, Ruilong @@aut@@ Wu, Junda @@aut@@ Tian, Xiaohua @@aut@@ Chen, Li @@aut@@ Dai, Xiaohui @@aut@@ Yan, Yongsheng @@aut@@ Pan, Jianming @@aut@@ Dai, Jiangdong @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	302468927
dewey-sort	3570
id	ELV065830903
language_de	englisch
fullrecord	<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000caa a22002652 4500</leader><controlfield tag="001">ELV065830903</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20240120093215.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">231126s2023 xx \|\|\|\|\|o 00\| \|\|eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1016/j.memsci.2023.122253</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)ELV065830903</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(ELSEVIER)S0376-7388(23)00909-2</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rda</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="082" ind1="0" ind2="4"><subfield code="a">570</subfield><subfield code="q">VZ</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">58.11</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Wang, Lulu</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Superhydrophilic fluorinated heterogeneous membranes with boosting antifouling property and high stable permeance for efficient emulsion separation</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2023</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">nicht spezifiziert</subfield><subfield code="b">zzz</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">It is yet a query that whether chemically heterogeneous superwetting surface is able to enhance the permeability and anti-fouling capability of membrane contemporaneously, heretofore which is lacking and well worth creating. Here, we propose a bio-adhesion coupled with self-assembly strategy, to construct superhydrophilic fluorinated heterogeneous membranes, through in-situ biomimetic adhesion of the hydrophilic polyphenol-silane coating (TAT) on the porous PVDF membrane, as a secondary reaction platform, and subsequently self-assembly of amphoteric fluorocarbon surfactant (FS-50). Unsurprisingly, we find that introducing FS-50 not only significantly strengthens the permeability, but also improves the anti-fouling self-cleaning, thanks to the formation of robust hydration layer and slippery micro-domains with low friction, to realize the dual anti-fouling effects of pollution resistance and release. The champion PVDF/TAT/FS-2.0 % composite membrane exhibits superhydrophilic and underwater superoleophobic (oil contact angle above 162.3°) property with very low oil-adhesion. This composite membrane possesses an ultrahigh water permeance of 29214.6 L m−2 h−1 bar−1, which is 2.8 times larger than that of pristine PVDF membrane. The PVDF/TAT/FS-2.0 % composite membrane presents the high separation efficiencies (above 99.5 %) for various surfactant-stabilized oil-in-water emulsions and high permeances of 3193.2–4212.3 L m−2 h−1 bar−1. Especially, the membrane at continuous operation for 1.0 h can reach a high stable permeance of 2505.1 L m−2 h−1 bar−1. Moreover, this composite membrane shows strong chemical stability and robustness. 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author	Wang, Lulu
spellingShingle	Wang, Lulu ddc 570 bkl 58.11 misc Chemically heterogeneous surface misc Superwetting membrane misc Improved permeance misc Anti-fouling self-cleaning misc Emulsion separation Superhydrophilic fluorinated heterogeneous membranes with boosting antifouling property and high stable permeance for efficient emulsion separation
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topic_title	570 VZ 58.11 bkl Superhydrophilic fluorinated heterogeneous membranes with boosting antifouling property and high stable permeance for efficient emulsion separation Chemically heterogeneous surface Superwetting membrane Improved permeance Anti-fouling self-cleaning Emulsion separation
topic	ddc 570 bkl 58.11 misc Chemically heterogeneous surface misc Superwetting membrane misc Improved permeance misc Anti-fouling self-cleaning misc Emulsion separation
topic_unstemmed	ddc 570 bkl 58.11 misc Chemically heterogeneous surface misc Superwetting membrane misc Improved permeance misc Anti-fouling self-cleaning misc Emulsion separation
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title	Superhydrophilic fluorinated heterogeneous membranes with boosting antifouling property and high stable permeance for efficient emulsion separation
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title_full	Superhydrophilic fluorinated heterogeneous membranes with boosting antifouling property and high stable permeance for efficient emulsion separation
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author_browse	Wang, Lulu Liu, Jie Zhang, Ruilong Wu, Junda Tian, Xiaohua Chen, Li Dai, Xiaohui Yan, Yongsheng Pan, Jianming Dai, Jiangdong
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title_sort	superhydrophilic fluorinated heterogeneous membranes with boosting antifouling property and high stable permeance for efficient emulsion separation
title_auth	Superhydrophilic fluorinated heterogeneous membranes with boosting antifouling property and high stable permeance for efficient emulsion separation
abstract	It is yet a query that whether chemically heterogeneous superwetting surface is able to enhance the permeability and anti-fouling capability of membrane contemporaneously, heretofore which is lacking and well worth creating. Here, we propose a bio-adhesion coupled with self-assembly strategy, to construct superhydrophilic fluorinated heterogeneous membranes, through in-situ biomimetic adhesion of the hydrophilic polyphenol-silane coating (TAT) on the porous PVDF membrane, as a secondary reaction platform, and subsequently self-assembly of amphoteric fluorocarbon surfactant (FS-50). Unsurprisingly, we find that introducing FS-50 not only significantly strengthens the permeability, but also improves the anti-fouling self-cleaning, thanks to the formation of robust hydration layer and slippery micro-domains with low friction, to realize the dual anti-fouling effects of pollution resistance and release. The champion PVDF/TAT/FS-2.0 % composite membrane exhibits superhydrophilic and underwater superoleophobic (oil contact angle above 162.3°) property with very low oil-adhesion. This composite membrane possesses an ultrahigh water permeance of 29214.6 L m−2 h−1 bar−1, which is 2.8 times larger than that of pristine PVDF membrane. The PVDF/TAT/FS-2.0 % composite membrane presents the high separation efficiencies (above 99.5 %) for various surfactant-stabilized oil-in-water emulsions and high permeances of 3193.2–4212.3 L m−2 h−1 bar−1. Especially, the membrane at continuous operation for 1.0 h can reach a high stable permeance of 2505.1 L m−2 h−1 bar−1. Moreover, this composite membrane shows strong chemical stability and robustness. This research answers the initial question, and provides the insight for further design and production of chemically heterogeneous superwetting membranes with high permeability, selectivity and antifouling ability.
abstractGer	It is yet a query that whether chemically heterogeneous superwetting surface is able to enhance the permeability and anti-fouling capability of membrane contemporaneously, heretofore which is lacking and well worth creating. Here, we propose a bio-adhesion coupled with self-assembly strategy, to construct superhydrophilic fluorinated heterogeneous membranes, through in-situ biomimetic adhesion of the hydrophilic polyphenol-silane coating (TAT) on the porous PVDF membrane, as a secondary reaction platform, and subsequently self-assembly of amphoteric fluorocarbon surfactant (FS-50). Unsurprisingly, we find that introducing FS-50 not only significantly strengthens the permeability, but also improves the anti-fouling self-cleaning, thanks to the formation of robust hydration layer and slippery micro-domains with low friction, to realize the dual anti-fouling effects of pollution resistance and release. The champion PVDF/TAT/FS-2.0 % composite membrane exhibits superhydrophilic and underwater superoleophobic (oil contact angle above 162.3°) property with very low oil-adhesion. This composite membrane possesses an ultrahigh water permeance of 29214.6 L m−2 h−1 bar−1, which is 2.8 times larger than that of pristine PVDF membrane. The PVDF/TAT/FS-2.0 % composite membrane presents the high separation efficiencies (above 99.5 %) for various surfactant-stabilized oil-in-water emulsions and high permeances of 3193.2–4212.3 L m−2 h−1 bar−1. Especially, the membrane at continuous operation for 1.0 h can reach a high stable permeance of 2505.1 L m−2 h−1 bar−1. Moreover, this composite membrane shows strong chemical stability and robustness. This research answers the initial question, and provides the insight for further design and production of chemically heterogeneous superwetting membranes with high permeability, selectivity and antifouling ability.
abstract_unstemmed	It is yet a query that whether chemically heterogeneous superwetting surface is able to enhance the permeability and anti-fouling capability of membrane contemporaneously, heretofore which is lacking and well worth creating. Here, we propose a bio-adhesion coupled with self-assembly strategy, to construct superhydrophilic fluorinated heterogeneous membranes, through in-situ biomimetic adhesion of the hydrophilic polyphenol-silane coating (TAT) on the porous PVDF membrane, as a secondary reaction platform, and subsequently self-assembly of amphoteric fluorocarbon surfactant (FS-50). Unsurprisingly, we find that introducing FS-50 not only significantly strengthens the permeability, but also improves the anti-fouling self-cleaning, thanks to the formation of robust hydration layer and slippery micro-domains with low friction, to realize the dual anti-fouling effects of pollution resistance and release. The champion PVDF/TAT/FS-2.0 % composite membrane exhibits superhydrophilic and underwater superoleophobic (oil contact angle above 162.3°) property with very low oil-adhesion. This composite membrane possesses an ultrahigh water permeance of 29214.6 L m−2 h−1 bar−1, which is 2.8 times larger than that of pristine PVDF membrane. The PVDF/TAT/FS-2.0 % composite membrane presents the high separation efficiencies (above 99.5 %) for various surfactant-stabilized oil-in-water emulsions and high permeances of 3193.2–4212.3 L m−2 h−1 bar−1. Especially, the membrane at continuous operation for 1.0 h can reach a high stable permeance of 2505.1 L m−2 h−1 bar−1. Moreover, this composite membrane shows strong chemical stability and robustness. This research answers the initial question, and provides the insight for further design and production of chemically heterogeneous superwetting membranes with high permeability, selectivity and antifouling ability.
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title_short	Superhydrophilic fluorinated heterogeneous membranes with boosting antifouling property and high stable permeance for efficient emulsion separation
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author2	Liu, Jie Zhang, Ruilong Wu, Junda Tian, Xiaohua Chen, Li Dai, Xiaohui Yan, Yongsheng Pan, Jianming Dai, Jiangdong
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doi_str	10.1016/j.memsci.2023.122253
up_date	2024-07-07T00:24:04.203Z
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fullrecord_marcxml	<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000caa a22002652 4500</leader><controlfield tag="001">ELV065830903</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20240120093215.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">231126s2023 xx \|\|\|\|\|o 00\| \|\|eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1016/j.memsci.2023.122253</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)ELV065830903</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(ELSEVIER)S0376-7388(23)00909-2</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rda</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="082" ind1="0" ind2="4"><subfield code="a">570</subfield><subfield code="q">VZ</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">58.11</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Wang, Lulu</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Superhydrophilic fluorinated heterogeneous membranes with boosting antifouling property and high stable permeance for efficient emulsion separation</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2023</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">nicht spezifiziert</subfield><subfield code="b">zzz</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">It is yet a query that whether chemically heterogeneous superwetting surface is able to enhance the permeability and anti-fouling capability of membrane contemporaneously, heretofore which is lacking and well worth creating. Here, we propose a bio-adhesion coupled with self-assembly strategy, to construct superhydrophilic fluorinated heterogeneous membranes, through in-situ biomimetic adhesion of the hydrophilic polyphenol-silane coating (TAT) on the porous PVDF membrane, as a secondary reaction platform, and subsequently self-assembly of amphoteric fluorocarbon surfactant (FS-50). Unsurprisingly, we find that introducing FS-50 not only significantly strengthens the permeability, but also improves the anti-fouling self-cleaning, thanks to the formation of robust hydration layer and slippery micro-domains with low friction, to realize the dual anti-fouling effects of pollution resistance and release. The champion PVDF/TAT/FS-2.0 % composite membrane exhibits superhydrophilic and underwater superoleophobic (oil contact angle above 162.3°) property with very low oil-adhesion. This composite membrane possesses an ultrahigh water permeance of 29214.6 L m−2 h−1 bar−1, which is 2.8 times larger than that of pristine PVDF membrane. The PVDF/TAT/FS-2.0 % composite membrane presents the high separation efficiencies (above 99.5 %) for various surfactant-stabilized oil-in-water emulsions and high permeances of 3193.2–4212.3 L m−2 h−1 bar−1. Especially, the membrane at continuous operation for 1.0 h can reach a high stable permeance of 2505.1 L m−2 h−1 bar−1. Moreover, this composite membrane shows strong chemical stability and robustness. 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Superhydrophilic fluorinated heterogeneous membranes with boosting antifouling property and high stable permeance for efficient emulsion separation

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