Three new Zn (II)-based coordination polymers: Optical properties and dye degradation against RhB

Three newly developed coordination polymers (CPs), denoted as [Zn2(HL)(ptp)2]n (1), [Zn(HL)(bpz)·0.25H2O]n (2) and [Zn(HL)(bic)·H2O]n (3), have been synthesized using hydrothermal methods. These CPs are composed of zinc ions and specific ligands with 3-(4-ca...
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Gespeichert in:

Autor*in:	Liu, Qiang-Qiang [verfasserIn] Ghosh, Mithun Kumar [verfasserIn] Cai, Shu-Lan [verfasserIn] Liu, Xiao-Hong [verfasserIn] Lu, Lu [verfasserIn] Muddassir, Mohd. [verfasserIn] Ghorai, Tanmay Kumar [verfasserIn] Wang, Jun [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Zn (II) Coordination polymer Photocatalyst RhB

Übergeordnetes Werk:	Enthalten in: Polyhedron - Amsterdam [u.a.] : Elsevier Science, 1982, 247
Übergeordnetes Werk:	volume:247

DOI / URN:	10.1016/j.poly.2023.116731

Katalog-ID:	ELV065975537

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520			\|a Three newly developed coordination polymers (CPs), denoted as [Zn2(HL)(ptp)2]n (1), [Zn(HL)(bpz)·0.25H2O]n (2) and [Zn(HL)(bic)·H2O]n (3), have been synthesized using hydrothermal methods. These CPs are composed of zinc ions and specific ligands with 3-(4-carboxyphenoxy)-5-methylbenzoic acid (H3L); 3,5-bis(4-pyridyl)-1,2,4-triazolyl (ptp); 3,3ʹ,5,5ʹ-tetramethyl-4,4ʹ-bipyrazole (bpz) and 3,6-bis(imidazol-1-yl)-9H-carbazole (bic) which provide oxygen and nitrogen donor sites. The molecular structures of the CPs were determined through single X-ray diffraction analysis, revealing a tetrahedral geometry. The CPs 1–3 have distorted tetrahedral geometry. The layered structural progression, starting from the tetrahedral complex and moving towards 1D, 2D, and potentially 3D networks, showcases the intricacies and hierarchical nature of CP 1–3’s molecular architecture. An interesting property of these CPs is their semiconducting nature. They exhibit the ability to serve as photocatalysts, especially against organic pollutants such as Acid chrome blue (ACB), Methyl blue (MB), Methyl orange (MO), and Rhodamine B (RhB). Among the CPs, CP 1 demonstrates superior photocatalytic activity against RhB (RhB) at a concentration of 25 mg/L. This suggests that CP 1, when used in a quantity of 25 mg, exhibits enhanced efficiency in degrading RhB through photocatalysis. The optimal conditions, where 25 mg/L RhB and 25 mg of CP 1 are employed, result in the degradation of an impressive 97.51 % of RhB.
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700	1		\|a Ghorai, Tanmay Kumar \|e verfasserin \|4 aut
700	1		\|a Wang, Jun \|e verfasserin \|4 aut
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Indexfelder

author_variant	q q l qql m k g mk mkg s l c slc x h l xhl l l ll m m mm t k g tk tkg j w jw
matchkey_str	liuqiangqiangghoshmithunkumarcaishulanli:2023----:henwniaecodntoplmrotclrprisnde
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publishDate	2023
allfields	10.1016/j.poly.2023.116731 doi (DE-627)ELV065975537 (ELSEVIER)S0277-5387(23)00453-9 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Liu, Qiang-Qiang verfasserin aut Three new Zn (II)-based coordination polymers: Optical properties and dye degradation against RhB 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Three newly developed coordination polymers (CPs), denoted as [Zn2(HL)(ptp)2]n (1), [Zn(HL)(bpz)·0.25H2O]n (2) and [Zn(HL)(bic)·H2O]n (3), have been synthesized using hydrothermal methods. These CPs are composed of zinc ions and specific ligands with 3-(4-carboxyphenoxy)-5-methylbenzoic acid (H3L); 3,5-bis(4-pyridyl)-1,2,4-triazolyl (ptp); 3,3ʹ,5,5ʹ-tetramethyl-4,4ʹ-bipyrazole (bpz) and 3,6-bis(imidazol-1-yl)-9H-carbazole (bic) which provide oxygen and nitrogen donor sites. The molecular structures of the CPs were determined through single X-ray diffraction analysis, revealing a tetrahedral geometry. The CPs 1–3 have distorted tetrahedral geometry. The layered structural progression, starting from the tetrahedral complex and moving towards 1D, 2D, and potentially 3D networks, showcases the intricacies and hierarchical nature of CP 1–3’s molecular architecture. An interesting property of these CPs is their semiconducting nature. They exhibit the ability to serve as photocatalysts, especially against organic pollutants such as Acid chrome blue (ACB), Methyl blue (MB), Methyl orange (MO), and Rhodamine B (RhB). Among the CPs, CP 1 demonstrates superior photocatalytic activity against RhB (RhB) at a concentration of 25 mg/L. This suggests that CP 1, when used in a quantity of 25 mg, exhibits enhanced efficiency in degrading RhB through photocatalysis. The optimal conditions, where 25 mg/L RhB and 25 mg of CP 1 are employed, result in the degradation of an impressive 97.51 % of RhB. Zn (II) Coordination polymer Photocatalyst RhB Ghosh, Mithun Kumar verfasserin aut Cai, Shu-Lan verfasserin aut Liu, Xiao-Hong verfasserin aut Lu, Lu verfasserin aut Muddassir, Mohd. verfasserin aut Ghorai, Tanmay Kumar verfasserin aut Wang, Jun verfasserin aut Enthalten in Polyhedron Amsterdam [u.a.] : Elsevier Science, 1982 247 Online-Ressource (DE-627)320402967 (DE-600)2000326-2 (DE-576)096704209 nnns volume:247 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 247
spelling	10.1016/j.poly.2023.116731 doi (DE-627)ELV065975537 (ELSEVIER)S0277-5387(23)00453-9 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Liu, Qiang-Qiang verfasserin aut Three new Zn (II)-based coordination polymers: Optical properties and dye degradation against RhB 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Three newly developed coordination polymers (CPs), denoted as [Zn2(HL)(ptp)2]n (1), [Zn(HL)(bpz)·0.25H2O]n (2) and [Zn(HL)(bic)·H2O]n (3), have been synthesized using hydrothermal methods. These CPs are composed of zinc ions and specific ligands with 3-(4-carboxyphenoxy)-5-methylbenzoic acid (H3L); 3,5-bis(4-pyridyl)-1,2,4-triazolyl (ptp); 3,3ʹ,5,5ʹ-tetramethyl-4,4ʹ-bipyrazole (bpz) and 3,6-bis(imidazol-1-yl)-9H-carbazole (bic) which provide oxygen and nitrogen donor sites. The molecular structures of the CPs were determined through single X-ray diffraction analysis, revealing a tetrahedral geometry. The CPs 1–3 have distorted tetrahedral geometry. The layered structural progression, starting from the tetrahedral complex and moving towards 1D, 2D, and potentially 3D networks, showcases the intricacies and hierarchical nature of CP 1–3’s molecular architecture. An interesting property of these CPs is their semiconducting nature. They exhibit the ability to serve as photocatalysts, especially against organic pollutants such as Acid chrome blue (ACB), Methyl blue (MB), Methyl orange (MO), and Rhodamine B (RhB). Among the CPs, CP 1 demonstrates superior photocatalytic activity against RhB (RhB) at a concentration of 25 mg/L. This suggests that CP 1, when used in a quantity of 25 mg, exhibits enhanced efficiency in degrading RhB through photocatalysis. The optimal conditions, where 25 mg/L RhB and 25 mg of CP 1 are employed, result in the degradation of an impressive 97.51 % of RhB. Zn (II) Coordination polymer Photocatalyst RhB Ghosh, Mithun Kumar verfasserin aut Cai, Shu-Lan verfasserin aut Liu, Xiao-Hong verfasserin aut Lu, Lu verfasserin aut Muddassir, Mohd. verfasserin aut Ghorai, Tanmay Kumar verfasserin aut Wang, Jun verfasserin aut Enthalten in Polyhedron Amsterdam [u.a.] : Elsevier Science, 1982 247 Online-Ressource (DE-627)320402967 (DE-600)2000326-2 (DE-576)096704209 nnns volume:247 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 247
allfields_unstemmed	10.1016/j.poly.2023.116731 doi (DE-627)ELV065975537 (ELSEVIER)S0277-5387(23)00453-9 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Liu, Qiang-Qiang verfasserin aut Three new Zn (II)-based coordination polymers: Optical properties and dye degradation against RhB 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Three newly developed coordination polymers (CPs), denoted as [Zn2(HL)(ptp)2]n (1), [Zn(HL)(bpz)·0.25H2O]n (2) and [Zn(HL)(bic)·H2O]n (3), have been synthesized using hydrothermal methods. These CPs are composed of zinc ions and specific ligands with 3-(4-carboxyphenoxy)-5-methylbenzoic acid (H3L); 3,5-bis(4-pyridyl)-1,2,4-triazolyl (ptp); 3,3ʹ,5,5ʹ-tetramethyl-4,4ʹ-bipyrazole (bpz) and 3,6-bis(imidazol-1-yl)-9H-carbazole (bic) which provide oxygen and nitrogen donor sites. The molecular structures of the CPs were determined through single X-ray diffraction analysis, revealing a tetrahedral geometry. The CPs 1–3 have distorted tetrahedral geometry. The layered structural progression, starting from the tetrahedral complex and moving towards 1D, 2D, and potentially 3D networks, showcases the intricacies and hierarchical nature of CP 1–3’s molecular architecture. An interesting property of these CPs is their semiconducting nature. They exhibit the ability to serve as photocatalysts, especially against organic pollutants such as Acid chrome blue (ACB), Methyl blue (MB), Methyl orange (MO), and Rhodamine B (RhB). Among the CPs, CP 1 demonstrates superior photocatalytic activity against RhB (RhB) at a concentration of 25 mg/L. This suggests that CP 1, when used in a quantity of 25 mg, exhibits enhanced efficiency in degrading RhB through photocatalysis. The optimal conditions, where 25 mg/L RhB and 25 mg of CP 1 are employed, result in the degradation of an impressive 97.51 % of RhB. Zn (II) Coordination polymer Photocatalyst RhB Ghosh, Mithun Kumar verfasserin aut Cai, Shu-Lan verfasserin aut Liu, Xiao-Hong verfasserin aut Lu, Lu verfasserin aut Muddassir, Mohd. verfasserin aut Ghorai, Tanmay Kumar verfasserin aut Wang, Jun verfasserin aut Enthalten in Polyhedron Amsterdam [u.a.] : Elsevier Science, 1982 247 Online-Ressource (DE-627)320402967 (DE-600)2000326-2 (DE-576)096704209 nnns volume:247 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 247
allfieldsGer	10.1016/j.poly.2023.116731 doi (DE-627)ELV065975537 (ELSEVIER)S0277-5387(23)00453-9 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Liu, Qiang-Qiang verfasserin aut Three new Zn (II)-based coordination polymers: Optical properties and dye degradation against RhB 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Three newly developed coordination polymers (CPs), denoted as [Zn2(HL)(ptp)2]n (1), [Zn(HL)(bpz)·0.25H2O]n (2) and [Zn(HL)(bic)·H2O]n (3), have been synthesized using hydrothermal methods. These CPs are composed of zinc ions and specific ligands with 3-(4-carboxyphenoxy)-5-methylbenzoic acid (H3L); 3,5-bis(4-pyridyl)-1,2,4-triazolyl (ptp); 3,3ʹ,5,5ʹ-tetramethyl-4,4ʹ-bipyrazole (bpz) and 3,6-bis(imidazol-1-yl)-9H-carbazole (bic) which provide oxygen and nitrogen donor sites. The molecular structures of the CPs were determined through single X-ray diffraction analysis, revealing a tetrahedral geometry. The CPs 1–3 have distorted tetrahedral geometry. The layered structural progression, starting from the tetrahedral complex and moving towards 1D, 2D, and potentially 3D networks, showcases the intricacies and hierarchical nature of CP 1–3’s molecular architecture. An interesting property of these CPs is their semiconducting nature. They exhibit the ability to serve as photocatalysts, especially against organic pollutants such as Acid chrome blue (ACB), Methyl blue (MB), Methyl orange (MO), and Rhodamine B (RhB). Among the CPs, CP 1 demonstrates superior photocatalytic activity against RhB (RhB) at a concentration of 25 mg/L. This suggests that CP 1, when used in a quantity of 25 mg, exhibits enhanced efficiency in degrading RhB through photocatalysis. The optimal conditions, where 25 mg/L RhB and 25 mg of CP 1 are employed, result in the degradation of an impressive 97.51 % of RhB. Zn (II) Coordination polymer Photocatalyst RhB Ghosh, Mithun Kumar verfasserin aut Cai, Shu-Lan verfasserin aut Liu, Xiao-Hong verfasserin aut Lu, Lu verfasserin aut Muddassir, Mohd. verfasserin aut Ghorai, Tanmay Kumar verfasserin aut Wang, Jun verfasserin aut Enthalten in Polyhedron Amsterdam [u.a.] : Elsevier Science, 1982 247 Online-Ressource (DE-627)320402967 (DE-600)2000326-2 (DE-576)096704209 nnns volume:247 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 247
allfieldsSound	10.1016/j.poly.2023.116731 doi (DE-627)ELV065975537 (ELSEVIER)S0277-5387(23)00453-9 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Liu, Qiang-Qiang verfasserin aut Three new Zn (II)-based coordination polymers: Optical properties and dye degradation against RhB 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Three newly developed coordination polymers (CPs), denoted as [Zn2(HL)(ptp)2]n (1), [Zn(HL)(bpz)·0.25H2O]n (2) and [Zn(HL)(bic)·H2O]n (3), have been synthesized using hydrothermal methods. These CPs are composed of zinc ions and specific ligands with 3-(4-carboxyphenoxy)-5-methylbenzoic acid (H3L); 3,5-bis(4-pyridyl)-1,2,4-triazolyl (ptp); 3,3ʹ,5,5ʹ-tetramethyl-4,4ʹ-bipyrazole (bpz) and 3,6-bis(imidazol-1-yl)-9H-carbazole (bic) which provide oxygen and nitrogen donor sites. The molecular structures of the CPs were determined through single X-ray diffraction analysis, revealing a tetrahedral geometry. The CPs 1–3 have distorted tetrahedral geometry. The layered structural progression, starting from the tetrahedral complex and moving towards 1D, 2D, and potentially 3D networks, showcases the intricacies and hierarchical nature of CP 1–3’s molecular architecture. An interesting property of these CPs is their semiconducting nature. They exhibit the ability to serve as photocatalysts, especially against organic pollutants such as Acid chrome blue (ACB), Methyl blue (MB), Methyl orange (MO), and Rhodamine B (RhB). Among the CPs, CP 1 demonstrates superior photocatalytic activity against RhB (RhB) at a concentration of 25 mg/L. This suggests that CP 1, when used in a quantity of 25 mg, exhibits enhanced efficiency in degrading RhB through photocatalysis. The optimal conditions, where 25 mg/L RhB and 25 mg of CP 1 are employed, result in the degradation of an impressive 97.51 % of RhB. Zn (II) Coordination polymer Photocatalyst RhB Ghosh, Mithun Kumar verfasserin aut Cai, Shu-Lan verfasserin aut Liu, Xiao-Hong verfasserin aut Lu, Lu verfasserin aut Muddassir, Mohd. verfasserin aut Ghorai, Tanmay Kumar verfasserin aut Wang, Jun verfasserin aut Enthalten in Polyhedron Amsterdam [u.a.] : Elsevier Science, 1982 247 Online-Ressource (DE-627)320402967 (DE-600)2000326-2 (DE-576)096704209 nnns volume:247 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 247
language	English
source	Enthalten in Polyhedron 247 volume:247
sourceStr	Enthalten in Polyhedron 247 volume:247
format_phy_str_mv	Article
bklname	Chemie: Allgemeines
institution	findex.gbv.de
topic_facet	Zn (II) Coordination polymer Photocatalyst RhB
dewey-raw	540
isfreeaccess_bool	false
container_title	Polyhedron
authorswithroles_txt_mv	Liu, Qiang-Qiang @@aut@@ Ghosh, Mithun Kumar @@aut@@ Cai, Shu-Lan @@aut@@ Liu, Xiao-Hong @@aut@@ Lu, Lu @@aut@@ Muddassir, Mohd. @@aut@@ Ghorai, Tanmay Kumar @@aut@@ Wang, Jun @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	320402967
dewey-sort	3540
id	ELV065975537
language_de	englisch
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author	Liu, Qiang-Qiang
spellingShingle	Liu, Qiang-Qiang ddc 540 bkl 35.00 misc Zn (II) misc Coordination polymer misc Photocatalyst misc RhB Three new Zn (II)-based coordination polymers: Optical properties and dye degradation against RhB
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topic_title	540 VZ 35.00 bkl Three new Zn (II)-based coordination polymers: Optical properties and dye degradation against RhB Zn (II) Coordination polymer Photocatalyst RhB
topic	ddc 540 bkl 35.00 misc Zn (II) misc Coordination polymer misc Photocatalyst misc RhB
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title	Three new Zn (II)-based coordination polymers: Optical properties and dye degradation against RhB
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title_full	Three new Zn (II)-based coordination polymers: Optical properties and dye degradation against RhB
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author_browse	Liu, Qiang-Qiang Ghosh, Mithun Kumar Cai, Shu-Lan Liu, Xiao-Hong Lu, Lu Muddassir, Mohd. Ghorai, Tanmay Kumar Wang, Jun
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title_sort	three new zn (ii)-based coordination polymers: optical properties and dye degradation against rhb
title_auth	Three new Zn (II)-based coordination polymers: Optical properties and dye degradation against RhB
abstract	Three newly developed coordination polymers (CPs), denoted as [Zn2(HL)(ptp)2]n (1), [Zn(HL)(bpz)·0.25H2O]n (2) and [Zn(HL)(bic)·H2O]n (3), have been synthesized using hydrothermal methods. These CPs are composed of zinc ions and specific ligands with 3-(4-carboxyphenoxy)-5-methylbenzoic acid (H3L); 3,5-bis(4-pyridyl)-1,2,4-triazolyl (ptp); 3,3ʹ,5,5ʹ-tetramethyl-4,4ʹ-bipyrazole (bpz) and 3,6-bis(imidazol-1-yl)-9H-carbazole (bic) which provide oxygen and nitrogen donor sites. The molecular structures of the CPs were determined through single X-ray diffraction analysis, revealing a tetrahedral geometry. The CPs 1–3 have distorted tetrahedral geometry. The layered structural progression, starting from the tetrahedral complex and moving towards 1D, 2D, and potentially 3D networks, showcases the intricacies and hierarchical nature of CP 1–3’s molecular architecture. An interesting property of these CPs is their semiconducting nature. They exhibit the ability to serve as photocatalysts, especially against organic pollutants such as Acid chrome blue (ACB), Methyl blue (MB), Methyl orange (MO), and Rhodamine B (RhB). Among the CPs, CP 1 demonstrates superior photocatalytic activity against RhB (RhB) at a concentration of 25 mg/L. This suggests that CP 1, when used in a quantity of 25 mg, exhibits enhanced efficiency in degrading RhB through photocatalysis. The optimal conditions, where 25 mg/L RhB and 25 mg of CP 1 are employed, result in the degradation of an impressive 97.51 % of RhB.
abstractGer	Three newly developed coordination polymers (CPs), denoted as [Zn2(HL)(ptp)2]n (1), [Zn(HL)(bpz)·0.25H2O]n (2) and [Zn(HL)(bic)·H2O]n (3), have been synthesized using hydrothermal methods. These CPs are composed of zinc ions and specific ligands with 3-(4-carboxyphenoxy)-5-methylbenzoic acid (H3L); 3,5-bis(4-pyridyl)-1,2,4-triazolyl (ptp); 3,3ʹ,5,5ʹ-tetramethyl-4,4ʹ-bipyrazole (bpz) and 3,6-bis(imidazol-1-yl)-9H-carbazole (bic) which provide oxygen and nitrogen donor sites. The molecular structures of the CPs were determined through single X-ray diffraction analysis, revealing a tetrahedral geometry. The CPs 1–3 have distorted tetrahedral geometry. The layered structural progression, starting from the tetrahedral complex and moving towards 1D, 2D, and potentially 3D networks, showcases the intricacies and hierarchical nature of CP 1–3’s molecular architecture. An interesting property of these CPs is their semiconducting nature. They exhibit the ability to serve as photocatalysts, especially against organic pollutants such as Acid chrome blue (ACB), Methyl blue (MB), Methyl orange (MO), and Rhodamine B (RhB). Among the CPs, CP 1 demonstrates superior photocatalytic activity against RhB (RhB) at a concentration of 25 mg/L. This suggests that CP 1, when used in a quantity of 25 mg, exhibits enhanced efficiency in degrading RhB through photocatalysis. The optimal conditions, where 25 mg/L RhB and 25 mg of CP 1 are employed, result in the degradation of an impressive 97.51 % of RhB.
abstract_unstemmed	Three newly developed coordination polymers (CPs), denoted as [Zn2(HL)(ptp)2]n (1), [Zn(HL)(bpz)·0.25H2O]n (2) and [Zn(HL)(bic)·H2O]n (3), have been synthesized using hydrothermal methods. These CPs are composed of zinc ions and specific ligands with 3-(4-carboxyphenoxy)-5-methylbenzoic acid (H3L); 3,5-bis(4-pyridyl)-1,2,4-triazolyl (ptp); 3,3ʹ,5,5ʹ-tetramethyl-4,4ʹ-bipyrazole (bpz) and 3,6-bis(imidazol-1-yl)-9H-carbazole (bic) which provide oxygen and nitrogen donor sites. The molecular structures of the CPs were determined through single X-ray diffraction analysis, revealing a tetrahedral geometry. The CPs 1–3 have distorted tetrahedral geometry. The layered structural progression, starting from the tetrahedral complex and moving towards 1D, 2D, and potentially 3D networks, showcases the intricacies and hierarchical nature of CP 1–3’s molecular architecture. An interesting property of these CPs is their semiconducting nature. They exhibit the ability to serve as photocatalysts, especially against organic pollutants such as Acid chrome blue (ACB), Methyl blue (MB), Methyl orange (MO), and Rhodamine B (RhB). Among the CPs, CP 1 demonstrates superior photocatalytic activity against RhB (RhB) at a concentration of 25 mg/L. This suggests that CP 1, when used in a quantity of 25 mg, exhibits enhanced efficiency in degrading RhB through photocatalysis. The optimal conditions, where 25 mg/L RhB and 25 mg of CP 1 are employed, result in the degradation of an impressive 97.51 % of RhB.
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title_short	Three new Zn (II)-based coordination polymers: Optical properties and dye degradation against RhB
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author2	Ghosh, Mithun Kumar Cai, Shu-Lan Liu, Xiao-Hong Lu, Lu Muddassir, Mohd Ghorai, Tanmay Kumar Wang, Jun
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doi_str	10.1016/j.poly.2023.116731
up_date	2024-07-07T00:53:56.725Z
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These CPs are composed of zinc ions and specific ligands with 3-(4-carboxyphenoxy)-5-methylbenzoic acid (H3L); 3,5-bis(4-pyridyl)-1,2,4-triazolyl (ptp); 3,3ʹ,5,5ʹ-tetramethyl-4,4ʹ-bipyrazole (bpz) and 3,6-bis(imidazol-1-yl)-9H-carbazole (bic) which provide oxygen and nitrogen donor sites. The molecular structures of the CPs were determined through single X-ray diffraction analysis, revealing a tetrahedral geometry. The CPs 1–3 have distorted tetrahedral geometry. The layered structural progression, starting from the tetrahedral complex and moving towards 1D, 2D, and potentially 3D networks, showcases the intricacies and hierarchical nature of CP 1–3’s molecular architecture. An interesting property of these CPs is their semiconducting nature. They exhibit the ability to serve as photocatalysts, especially against organic pollutants such as Acid chrome blue (ACB), Methyl blue (MB), Methyl orange (MO), and Rhodamine B (RhB). Among the CPs, CP 1 demonstrates superior photocatalytic activity against RhB (RhB) at a concentration of 25 mg/L. This suggests that CP 1, when used in a quantity of 25 mg, exhibits enhanced efficiency in degrading RhB through photocatalysis. The optimal conditions, where 25 mg/L RhB and 25 mg of CP 1 are employed, result in the degradation of an impressive 97.51 % of RhB.</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Zn (II)</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Coordination polymer</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Photocatalyst</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">RhB</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Ghosh, Mithun Kumar</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Cai, Shu-Lan</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Liu, Xiao-Hong</subfield><subfield code="e">verfasserin</subfield><subfield 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Three new Zn (II)-based coordination polymers: Optical properties and dye degradation against RhB

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