Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries

A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determinin...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Kennedy, Ssendagire [verfasserIn] Kim, Jungmin [verfasserIn] Kim, Jeongtae [verfasserIn] Phiri, Isheunesu [verfasserIn] Ryou, Sun-Yul [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Lithium-ion batteries Al Aqueous slurry Microporous polyolefin separators

Übergeordnetes Werk:	Enthalten in: Journal of industrial and engineering chemistry - Seoul : KSIEC, 1995, 130, Seite 638-647
Übergeordnetes Werk:	volume:130 ; pages:638-647

DOI / URN:	10.1016/j.jiec.2023.10.017

Katalog-ID:	ELV066203961

Internformat


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245	1	0	\|a Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries
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520			\|a A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determining the polymer binders (CMC/PVA) content in the ceramic slurry and studying the interaction between the polymer binders and Al2O3 ceramic particles by changing the mixing order of the slurry components. CMC effectively controls the viscosity of the slurry to maintain a stable slurry dispersion. In contrast, PVA significantly influences the formation of a uniform ceramic coating layer on the polyethylene (PE) separator. This results in a synergistic effect to produce an optimal ceramic-coated composite separator (CCS). Compared to the bare PE separators, the prepared Al2O3 CCSs display improved physical properties, such as high adhesion strength of the ceramic coating layer, thermal stability, electrolyte wettability, and increased ionic conductivity. Moreover, the CCSs exhibit enhanced electrochemical performance. Half cells (LiMn2O4/Li metal) comprising CCSs retained 96.5% (144.8 mAh g−1) of the initial discharge capacity even after 200 cycles, while bare PE separators lose their capacity rapidly after 150 cycles, retaining only 22.62% (33.5 mAh g−1) at the 200th cycle.
650		4	\|a Lithium-ion batteries
650		4	\|a Al
650		4	\|a Aqueous slurry
650		4	\|a Microporous polyolefin separators
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700	1		\|a Kim, Jeongtae \|e verfasserin \|4 aut
700	1		\|a Phiri, Isheunesu \|e verfasserin \|0 (orcid)0000-0001-5186-566X \|4 aut
700	1		\|a Ryou, Sun-Yul \|e verfasserin \|0 (orcid)0000-0001-8899-019X \|4 aut
773	0	8	\|i Enthalten in \|t Journal of industrial and engineering chemistry \|d Seoul : KSIEC, 1995 \|g 130, Seite 638-647 \|w (DE-627)391337238 \|w (DE-600)2152565-1 \|w (DE-576)28474784X \|x 1226-086X \|7 nnns
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912			\|a GBV_ILN_40
912			\|a GBV_ILN_60
912			\|a GBV_ILN_62
912			\|a GBV_ILN_65
912			\|a GBV_ILN_69
912			\|a GBV_ILN_70
912			\|a GBV_ILN_73
912			\|a GBV_ILN_74
912			\|a GBV_ILN_90
912			\|a GBV_ILN_95
912			\|a GBV_ILN_100
912			\|a GBV_ILN_101
912			\|a GBV_ILN_105
912			\|a GBV_ILN_110
912			\|a GBV_ILN_150
912			\|a GBV_ILN_151
912			\|a GBV_ILN_187
912			\|a GBV_ILN_213
912			\|a GBV_ILN_224
912			\|a GBV_ILN_230
912			\|a GBV_ILN_370
912			\|a GBV_ILN_602
912			\|a GBV_ILN_702
912			\|a GBV_ILN_2001
912			\|a GBV_ILN_2003
912			\|a GBV_ILN_2004
912			\|a GBV_ILN_2005
912			\|a GBV_ILN_2007
912			\|a GBV_ILN_2009
912			\|a GBV_ILN_2010
912			\|a GBV_ILN_2011
912			\|a GBV_ILN_2014
912			\|a GBV_ILN_2015
912			\|a GBV_ILN_2020
912			\|a GBV_ILN_2021
912			\|a GBV_ILN_2025
912			\|a GBV_ILN_2026
912			\|a GBV_ILN_2027
912			\|a GBV_ILN_2034
912			\|a GBV_ILN_2044
912			\|a GBV_ILN_2048
912			\|a GBV_ILN_2049
912			\|a GBV_ILN_2050
912			\|a GBV_ILN_2055
912			\|a GBV_ILN_2056
912			\|a GBV_ILN_2059
912			\|a GBV_ILN_2061
912			\|a GBV_ILN_2064
912			\|a GBV_ILN_2106
912			\|a GBV_ILN_2110
912			\|a GBV_ILN_2111
912			\|a GBV_ILN_2112
912			\|a GBV_ILN_2122
912			\|a GBV_ILN_2129
912			\|a GBV_ILN_2143
912			\|a GBV_ILN_2152
912			\|a GBV_ILN_2153
912			\|a GBV_ILN_2190
912			\|a GBV_ILN_2232
912			\|a GBV_ILN_2336
912			\|a GBV_ILN_2470
912			\|a GBV_ILN_2507
912			\|a GBV_ILN_4035
912			\|a GBV_ILN_4037
912			\|a GBV_ILN_4112
912			\|a GBV_ILN_4125
912			\|a GBV_ILN_4242
912			\|a GBV_ILN_4249
912			\|a GBV_ILN_4251
912			\|a GBV_ILN_4305
912			\|a GBV_ILN_4306
912			\|a GBV_ILN_4307
912			\|a GBV_ILN_4313
912			\|a GBV_ILN_4322
912			\|a GBV_ILN_4323
912			\|a GBV_ILN_4324
912			\|a GBV_ILN_4325
912			\|a GBV_ILN_4326
912			\|a GBV_ILN_4333
912			\|a GBV_ILN_4334
912			\|a GBV_ILN_4338
912			\|a GBV_ILN_4393
912			\|a GBV_ILN_4700
951			\|a AR
952			\|d 130 \|h 638-647

Indexfelder

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publishDate	2023
allfields	10.1016/j.jiec.2023.10.017 doi (DE-627)ELV066203961 (ELSEVIER)S1226-086X(23)00638-X DE-627 ger DE-627 rda eng 600 540 VZ Kennedy, Ssendagire verfasserin aut Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determining the polymer binders (CMC/PVA) content in the ceramic slurry and studying the interaction between the polymer binders and Al2O3 ceramic particles by changing the mixing order of the slurry components. CMC effectively controls the viscosity of the slurry to maintain a stable slurry dispersion. In contrast, PVA significantly influences the formation of a uniform ceramic coating layer on the polyethylene (PE) separator. This results in a synergistic effect to produce an optimal ceramic-coated composite separator (CCS). Compared to the bare PE separators, the prepared Al2O3 CCSs display improved physical properties, such as high adhesion strength of the ceramic coating layer, thermal stability, electrolyte wettability, and increased ionic conductivity. Moreover, the CCSs exhibit enhanced electrochemical performance. Half cells (LiMn2O4/Li metal) comprising CCSs retained 96.5% (144.8 mAh g−1) of the initial discharge capacity even after 200 cycles, while bare PE separators lose their capacity rapidly after 150 cycles, retaining only 22.62% (33.5 mAh g−1) at the 200th cycle. Lithium-ion batteries Al Aqueous slurry Microporous polyolefin separators Kim, Jungmin verfasserin aut Kim, Jeongtae verfasserin aut Phiri, Isheunesu verfasserin (orcid)0000-0001-5186-566X aut Ryou, Sun-Yul verfasserin (orcid)0000-0001-8899-019X aut Enthalten in Journal of industrial and engineering chemistry Seoul : KSIEC, 1995 130, Seite 638-647 (DE-627)391337238 (DE-600)2152565-1 (DE-576)28474784X 1226-086X nnns volume:130 pages:638-647 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 130 638-647
spelling	10.1016/j.jiec.2023.10.017 doi (DE-627)ELV066203961 (ELSEVIER)S1226-086X(23)00638-X DE-627 ger DE-627 rda eng 600 540 VZ Kennedy, Ssendagire verfasserin aut Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determining the polymer binders (CMC/PVA) content in the ceramic slurry and studying the interaction between the polymer binders and Al2O3 ceramic particles by changing the mixing order of the slurry components. CMC effectively controls the viscosity of the slurry to maintain a stable slurry dispersion. In contrast, PVA significantly influences the formation of a uniform ceramic coating layer on the polyethylene (PE) separator. This results in a synergistic effect to produce an optimal ceramic-coated composite separator (CCS). Compared to the bare PE separators, the prepared Al2O3 CCSs display improved physical properties, such as high adhesion strength of the ceramic coating layer, thermal stability, electrolyte wettability, and increased ionic conductivity. Moreover, the CCSs exhibit enhanced electrochemical performance. Half cells (LiMn2O4/Li metal) comprising CCSs retained 96.5% (144.8 mAh g−1) of the initial discharge capacity even after 200 cycles, while bare PE separators lose their capacity rapidly after 150 cycles, retaining only 22.62% (33.5 mAh g−1) at the 200th cycle. Lithium-ion batteries Al Aqueous slurry Microporous polyolefin separators Kim, Jungmin verfasserin aut Kim, Jeongtae verfasserin aut Phiri, Isheunesu verfasserin (orcid)0000-0001-5186-566X aut Ryou, Sun-Yul verfasserin (orcid)0000-0001-8899-019X aut Enthalten in Journal of industrial and engineering chemistry Seoul : KSIEC, 1995 130, Seite 638-647 (DE-627)391337238 (DE-600)2152565-1 (DE-576)28474784X 1226-086X nnns volume:130 pages:638-647 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 130 638-647
allfields_unstemmed	10.1016/j.jiec.2023.10.017 doi (DE-627)ELV066203961 (ELSEVIER)S1226-086X(23)00638-X DE-627 ger DE-627 rda eng 600 540 VZ Kennedy, Ssendagire verfasserin aut Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determining the polymer binders (CMC/PVA) content in the ceramic slurry and studying the interaction between the polymer binders and Al2O3 ceramic particles by changing the mixing order of the slurry components. CMC effectively controls the viscosity of the slurry to maintain a stable slurry dispersion. In contrast, PVA significantly influences the formation of a uniform ceramic coating layer on the polyethylene (PE) separator. This results in a synergistic effect to produce an optimal ceramic-coated composite separator (CCS). Compared to the bare PE separators, the prepared Al2O3 CCSs display improved physical properties, such as high adhesion strength of the ceramic coating layer, thermal stability, electrolyte wettability, and increased ionic conductivity. Moreover, the CCSs exhibit enhanced electrochemical performance. Half cells (LiMn2O4/Li metal) comprising CCSs retained 96.5% (144.8 mAh g−1) of the initial discharge capacity even after 200 cycles, while bare PE separators lose their capacity rapidly after 150 cycles, retaining only 22.62% (33.5 mAh g−1) at the 200th cycle. Lithium-ion batteries Al Aqueous slurry Microporous polyolefin separators Kim, Jungmin verfasserin aut Kim, Jeongtae verfasserin aut Phiri, Isheunesu verfasserin (orcid)0000-0001-5186-566X aut Ryou, Sun-Yul verfasserin (orcid)0000-0001-8899-019X aut Enthalten in Journal of industrial and engineering chemistry Seoul : KSIEC, 1995 130, Seite 638-647 (DE-627)391337238 (DE-600)2152565-1 (DE-576)28474784X 1226-086X nnns volume:130 pages:638-647 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 130 638-647
allfieldsGer	10.1016/j.jiec.2023.10.017 doi (DE-627)ELV066203961 (ELSEVIER)S1226-086X(23)00638-X DE-627 ger DE-627 rda eng 600 540 VZ Kennedy, Ssendagire verfasserin aut Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determining the polymer binders (CMC/PVA) content in the ceramic slurry and studying the interaction between the polymer binders and Al2O3 ceramic particles by changing the mixing order of the slurry components. CMC effectively controls the viscosity of the slurry to maintain a stable slurry dispersion. In contrast, PVA significantly influences the formation of a uniform ceramic coating layer on the polyethylene (PE) separator. This results in a synergistic effect to produce an optimal ceramic-coated composite separator (CCS). Compared to the bare PE separators, the prepared Al2O3 CCSs display improved physical properties, such as high adhesion strength of the ceramic coating layer, thermal stability, electrolyte wettability, and increased ionic conductivity. Moreover, the CCSs exhibit enhanced electrochemical performance. Half cells (LiMn2O4/Li metal) comprising CCSs retained 96.5% (144.8 mAh g−1) of the initial discharge capacity even after 200 cycles, while bare PE separators lose their capacity rapidly after 150 cycles, retaining only 22.62% (33.5 mAh g−1) at the 200th cycle. Lithium-ion batteries Al Aqueous slurry Microporous polyolefin separators Kim, Jungmin verfasserin aut Kim, Jeongtae verfasserin aut Phiri, Isheunesu verfasserin (orcid)0000-0001-5186-566X aut Ryou, Sun-Yul verfasserin (orcid)0000-0001-8899-019X aut Enthalten in Journal of industrial and engineering chemistry Seoul : KSIEC, 1995 130, Seite 638-647 (DE-627)391337238 (DE-600)2152565-1 (DE-576)28474784X 1226-086X nnns volume:130 pages:638-647 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 130 638-647
allfieldsSound	10.1016/j.jiec.2023.10.017 doi (DE-627)ELV066203961 (ELSEVIER)S1226-086X(23)00638-X DE-627 ger DE-627 rda eng 600 540 VZ Kennedy, Ssendagire verfasserin aut Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determining the polymer binders (CMC/PVA) content in the ceramic slurry and studying the interaction between the polymer binders and Al2O3 ceramic particles by changing the mixing order of the slurry components. CMC effectively controls the viscosity of the slurry to maintain a stable slurry dispersion. In contrast, PVA significantly influences the formation of a uniform ceramic coating layer on the polyethylene (PE) separator. This results in a synergistic effect to produce an optimal ceramic-coated composite separator (CCS). Compared to the bare PE separators, the prepared Al2O3 CCSs display improved physical properties, such as high adhesion strength of the ceramic coating layer, thermal stability, electrolyte wettability, and increased ionic conductivity. Moreover, the CCSs exhibit enhanced electrochemical performance. Half cells (LiMn2O4/Li metal) comprising CCSs retained 96.5% (144.8 mAh g−1) of the initial discharge capacity even after 200 cycles, while bare PE separators lose their capacity rapidly after 150 cycles, retaining only 22.62% (33.5 mAh g−1) at the 200th cycle. Lithium-ion batteries Al Aqueous slurry Microporous polyolefin separators Kim, Jungmin verfasserin aut Kim, Jeongtae verfasserin aut Phiri, Isheunesu verfasserin (orcid)0000-0001-5186-566X aut Ryou, Sun-Yul verfasserin (orcid)0000-0001-8899-019X aut Enthalten in Journal of industrial and engineering chemistry Seoul : KSIEC, 1995 130, Seite 638-647 (DE-627)391337238 (DE-600)2152565-1 (DE-576)28474784X 1226-086X nnns volume:130 pages:638-647 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 130 638-647
language	English
source	Enthalten in Journal of industrial and engineering chemistry 130, Seite 638-647 volume:130 pages:638-647
sourceStr	Enthalten in Journal of industrial and engineering chemistry 130, Seite 638-647 volume:130 pages:638-647
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	Lithium-ion batteries Al Aqueous slurry Microporous polyolefin separators
dewey-raw	600
isfreeaccess_bool	false
container_title	Journal of industrial and engineering chemistry
authorswithroles_txt_mv	Kennedy, Ssendagire @@aut@@ Kim, Jungmin @@aut@@ Kim, Jeongtae @@aut@@ Phiri, Isheunesu @@aut@@ Ryou, Sun-Yul @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	391337238
dewey-sort	3600
id	ELV066203961
language_de	englisch
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author	Kennedy, Ssendagire
spellingShingle	Kennedy, Ssendagire ddc 600 misc Lithium-ion batteries misc Al misc Aqueous slurry misc Microporous polyolefin separators Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries
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topic_title	600 540 VZ Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries Lithium-ion batteries Al Aqueous slurry Microporous polyolefin separators
topic	ddc 600 misc Lithium-ion batteries misc Al misc Aqueous slurry misc Microporous polyolefin separators
topic_unstemmed	ddc 600 misc Lithium-ion batteries misc Al misc Aqueous slurry misc Microporous polyolefin separators
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title	Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries
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title_full	Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries
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author_browse	Kennedy, Ssendagire Kim, Jungmin Kim, Jeongtae Phiri, Isheunesu Ryou, Sun-Yul
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title_sort	water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries
title_auth	Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries
abstract	A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determining the polymer binders (CMC/PVA) content in the ceramic slurry and studying the interaction between the polymer binders and Al2O3 ceramic particles by changing the mixing order of the slurry components. CMC effectively controls the viscosity of the slurry to maintain a stable slurry dispersion. In contrast, PVA significantly influences the formation of a uniform ceramic coating layer on the polyethylene (PE) separator. This results in a synergistic effect to produce an optimal ceramic-coated composite separator (CCS). Compared to the bare PE separators, the prepared Al2O3 CCSs display improved physical properties, such as high adhesion strength of the ceramic coating layer, thermal stability, electrolyte wettability, and increased ionic conductivity. Moreover, the CCSs exhibit enhanced electrochemical performance. Half cells (LiMn2O4/Li metal) comprising CCSs retained 96.5% (144.8 mAh g−1) of the initial discharge capacity even after 200 cycles, while bare PE separators lose their capacity rapidly after 150 cycles, retaining only 22.62% (33.5 mAh g−1) at the 200th cycle.
abstractGer	A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determining the polymer binders (CMC/PVA) content in the ceramic slurry and studying the interaction between the polymer binders and Al2O3 ceramic particles by changing the mixing order of the slurry components. CMC effectively controls the viscosity of the slurry to maintain a stable slurry dispersion. In contrast, PVA significantly influences the formation of a uniform ceramic coating layer on the polyethylene (PE) separator. This results in a synergistic effect to produce an optimal ceramic-coated composite separator (CCS). Compared to the bare PE separators, the prepared Al2O3 CCSs display improved physical properties, such as high adhesion strength of the ceramic coating layer, thermal stability, electrolyte wettability, and increased ionic conductivity. Moreover, the CCSs exhibit enhanced electrochemical performance. Half cells (LiMn2O4/Li metal) comprising CCSs retained 96.5% (144.8 mAh g−1) of the initial discharge capacity even after 200 cycles, while bare PE separators lose their capacity rapidly after 150 cycles, retaining only 22.62% (33.5 mAh g−1) at the 200th cycle.
abstract_unstemmed	A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determining the polymer binders (CMC/PVA) content in the ceramic slurry and studying the interaction between the polymer binders and Al2O3 ceramic particles by changing the mixing order of the slurry components. CMC effectively controls the viscosity of the slurry to maintain a stable slurry dispersion. In contrast, PVA significantly influences the formation of a uniform ceramic coating layer on the polyethylene (PE) separator. This results in a synergistic effect to produce an optimal ceramic-coated composite separator (CCS). Compared to the bare PE separators, the prepared Al2O3 CCSs display improved physical properties, such as high adhesion strength of the ceramic coating layer, thermal stability, electrolyte wettability, and increased ionic conductivity. Moreover, the CCSs exhibit enhanced electrochemical performance. Half cells (LiMn2O4/Li metal) comprising CCSs retained 96.5% (144.8 mAh g−1) of the initial discharge capacity even after 200 cycles, while bare PE separators lose their capacity rapidly after 150 cycles, retaining only 22.62% (33.5 mAh g−1) at the 200th cycle.
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title_short	Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries
remote_bool	true
author2	Kim, Jungmin Kim, Jeongtae Phiri, Isheunesu Ryou, Sun-Yul
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doi_str	10.1016/j.jiec.2023.10.017
up_date	2024-07-06T16:56:42.327Z
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Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries

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