Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries
A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determinin...
Ausführliche Beschreibung
Autor*in: |
Kennedy, Ssendagire [verfasserIn] Kim, Jungmin [verfasserIn] Kim, Jeongtae [verfasserIn] Phiri, Isheunesu [verfasserIn] Ryou, Sun-Yul [verfasserIn] |
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E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2023 |
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Schlagwörter: |
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Übergeordnetes Werk: |
Enthalten in: Journal of industrial and engineering chemistry - Seoul : KSIEC, 1995, 130, Seite 638-647 |
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Übergeordnetes Werk: |
volume:130 ; pages:638-647 |
DOI / URN: |
10.1016/j.jiec.2023.10.017 |
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Katalog-ID: |
ELV066203961 |
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520 | |a A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determining the polymer binders (CMC/PVA) content in the ceramic slurry and studying the interaction between the polymer binders and Al2O3 ceramic particles by changing the mixing order of the slurry components. CMC effectively controls the viscosity of the slurry to maintain a stable slurry dispersion. In contrast, PVA significantly influences the formation of a uniform ceramic coating layer on the polyethylene (PE) separator. This results in a synergistic effect to produce an optimal ceramic-coated composite separator (CCS). Compared to the bare PE separators, the prepared Al2O3 CCSs display improved physical properties, such as high adhesion strength of the ceramic coating layer, thermal stability, electrolyte wettability, and increased ionic conductivity. Moreover, the CCSs exhibit enhanced electrochemical performance. Half cells (LiMn2O4/Li metal) comprising CCSs retained 96.5% (144.8 mAh g−1) of the initial discharge capacity even after 200 cycles, while bare PE separators lose their capacity rapidly after 150 cycles, retaining only 22.62% (33.5 mAh g−1) at the 200th cycle. | ||
650 | 4 | |a Lithium-ion batteries | |
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650 | 4 | |a Aqueous slurry | |
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700 | 1 | |a Kim, Jungmin |e verfasserin |4 aut | |
700 | 1 | |a Kim, Jeongtae |e verfasserin |4 aut | |
700 | 1 | |a Phiri, Isheunesu |e verfasserin |0 (orcid)0000-0001-5186-566X |4 aut | |
700 | 1 | |a Ryou, Sun-Yul |e verfasserin |0 (orcid)0000-0001-8899-019X |4 aut | |
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10.1016/j.jiec.2023.10.017 doi (DE-627)ELV066203961 (ELSEVIER)S1226-086X(23)00638-X DE-627 ger DE-627 rda eng 600 540 VZ Kennedy, Ssendagire verfasserin aut Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determining the polymer binders (CMC/PVA) content in the ceramic slurry and studying the interaction between the polymer binders and Al2O3 ceramic particles by changing the mixing order of the slurry components. CMC effectively controls the viscosity of the slurry to maintain a stable slurry dispersion. In contrast, PVA significantly influences the formation of a uniform ceramic coating layer on the polyethylene (PE) separator. This results in a synergistic effect to produce an optimal ceramic-coated composite separator (CCS). Compared to the bare PE separators, the prepared Al2O3 CCSs display improved physical properties, such as high adhesion strength of the ceramic coating layer, thermal stability, electrolyte wettability, and increased ionic conductivity. Moreover, the CCSs exhibit enhanced electrochemical performance. Half cells (LiMn2O4/Li metal) comprising CCSs retained 96.5% (144.8 mAh g−1) of the initial discharge capacity even after 200 cycles, while bare PE separators lose their capacity rapidly after 150 cycles, retaining only 22.62% (33.5 mAh g−1) at the 200th cycle. Lithium-ion batteries Al Aqueous slurry Microporous polyolefin separators Kim, Jungmin verfasserin aut Kim, Jeongtae verfasserin aut Phiri, Isheunesu verfasserin (orcid)0000-0001-5186-566X aut Ryou, Sun-Yul verfasserin (orcid)0000-0001-8899-019X aut Enthalten in Journal of industrial and engineering chemistry Seoul : KSIEC, 1995 130, Seite 638-647 (DE-627)391337238 (DE-600)2152565-1 (DE-576)28474784X 1226-086X nnns volume:130 pages:638-647 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 130 638-647 |
spelling |
10.1016/j.jiec.2023.10.017 doi (DE-627)ELV066203961 (ELSEVIER)S1226-086X(23)00638-X DE-627 ger DE-627 rda eng 600 540 VZ Kennedy, Ssendagire verfasserin aut Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determining the polymer binders (CMC/PVA) content in the ceramic slurry and studying the interaction between the polymer binders and Al2O3 ceramic particles by changing the mixing order of the slurry components. CMC effectively controls the viscosity of the slurry to maintain a stable slurry dispersion. In contrast, PVA significantly influences the formation of a uniform ceramic coating layer on the polyethylene (PE) separator. This results in a synergistic effect to produce an optimal ceramic-coated composite separator (CCS). Compared to the bare PE separators, the prepared Al2O3 CCSs display improved physical properties, such as high adhesion strength of the ceramic coating layer, thermal stability, electrolyte wettability, and increased ionic conductivity. Moreover, the CCSs exhibit enhanced electrochemical performance. Half cells (LiMn2O4/Li metal) comprising CCSs retained 96.5% (144.8 mAh g−1) of the initial discharge capacity even after 200 cycles, while bare PE separators lose their capacity rapidly after 150 cycles, retaining only 22.62% (33.5 mAh g−1) at the 200th cycle. Lithium-ion batteries Al Aqueous slurry Microporous polyolefin separators Kim, Jungmin verfasserin aut Kim, Jeongtae verfasserin aut Phiri, Isheunesu verfasserin (orcid)0000-0001-5186-566X aut Ryou, Sun-Yul verfasserin (orcid)0000-0001-8899-019X aut Enthalten in Journal of industrial and engineering chemistry Seoul : KSIEC, 1995 130, Seite 638-647 (DE-627)391337238 (DE-600)2152565-1 (DE-576)28474784X 1226-086X nnns volume:130 pages:638-647 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 130 638-647 |
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10.1016/j.jiec.2023.10.017 doi (DE-627)ELV066203961 (ELSEVIER)S1226-086X(23)00638-X DE-627 ger DE-627 rda eng 600 540 VZ Kennedy, Ssendagire verfasserin aut Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determining the polymer binders (CMC/PVA) content in the ceramic slurry and studying the interaction between the polymer binders and Al2O3 ceramic particles by changing the mixing order of the slurry components. CMC effectively controls the viscosity of the slurry to maintain a stable slurry dispersion. In contrast, PVA significantly influences the formation of a uniform ceramic coating layer on the polyethylene (PE) separator. This results in a synergistic effect to produce an optimal ceramic-coated composite separator (CCS). Compared to the bare PE separators, the prepared Al2O3 CCSs display improved physical properties, such as high adhesion strength of the ceramic coating layer, thermal stability, electrolyte wettability, and increased ionic conductivity. Moreover, the CCSs exhibit enhanced electrochemical performance. Half cells (LiMn2O4/Li metal) comprising CCSs retained 96.5% (144.8 mAh g−1) of the initial discharge capacity even after 200 cycles, while bare PE separators lose their capacity rapidly after 150 cycles, retaining only 22.62% (33.5 mAh g−1) at the 200th cycle. Lithium-ion batteries Al Aqueous slurry Microporous polyolefin separators Kim, Jungmin verfasserin aut Kim, Jeongtae verfasserin aut Phiri, Isheunesu verfasserin (orcid)0000-0001-5186-566X aut Ryou, Sun-Yul verfasserin (orcid)0000-0001-8899-019X aut Enthalten in Journal of industrial and engineering chemistry Seoul : KSIEC, 1995 130, Seite 638-647 (DE-627)391337238 (DE-600)2152565-1 (DE-576)28474784X 1226-086X nnns volume:130 pages:638-647 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 130 638-647 |
allfieldsGer |
10.1016/j.jiec.2023.10.017 doi (DE-627)ELV066203961 (ELSEVIER)S1226-086X(23)00638-X DE-627 ger DE-627 rda eng 600 540 VZ Kennedy, Ssendagire verfasserin aut Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determining the polymer binders (CMC/PVA) content in the ceramic slurry and studying the interaction between the polymer binders and Al2O3 ceramic particles by changing the mixing order of the slurry components. CMC effectively controls the viscosity of the slurry to maintain a stable slurry dispersion. In contrast, PVA significantly influences the formation of a uniform ceramic coating layer on the polyethylene (PE) separator. This results in a synergistic effect to produce an optimal ceramic-coated composite separator (CCS). Compared to the bare PE separators, the prepared Al2O3 CCSs display improved physical properties, such as high adhesion strength of the ceramic coating layer, thermal stability, electrolyte wettability, and increased ionic conductivity. Moreover, the CCSs exhibit enhanced electrochemical performance. Half cells (LiMn2O4/Li metal) comprising CCSs retained 96.5% (144.8 mAh g−1) of the initial discharge capacity even after 200 cycles, while bare PE separators lose their capacity rapidly after 150 cycles, retaining only 22.62% (33.5 mAh g−1) at the 200th cycle. Lithium-ion batteries Al Aqueous slurry Microporous polyolefin separators Kim, Jungmin verfasserin aut Kim, Jeongtae verfasserin aut Phiri, Isheunesu verfasserin (orcid)0000-0001-5186-566X aut Ryou, Sun-Yul verfasserin (orcid)0000-0001-8899-019X aut Enthalten in Journal of industrial and engineering chemistry Seoul : KSIEC, 1995 130, Seite 638-647 (DE-627)391337238 (DE-600)2152565-1 (DE-576)28474784X 1226-086X nnns volume:130 pages:638-647 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 130 638-647 |
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10.1016/j.jiec.2023.10.017 doi (DE-627)ELV066203961 (ELSEVIER)S1226-086X(23)00638-X DE-627 ger DE-627 rda eng 600 540 VZ Kennedy, Ssendagire verfasserin aut Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determining the polymer binders (CMC/PVA) content in the ceramic slurry and studying the interaction between the polymer binders and Al2O3 ceramic particles by changing the mixing order of the slurry components. CMC effectively controls the viscosity of the slurry to maintain a stable slurry dispersion. In contrast, PVA significantly influences the formation of a uniform ceramic coating layer on the polyethylene (PE) separator. This results in a synergistic effect to produce an optimal ceramic-coated composite separator (CCS). Compared to the bare PE separators, the prepared Al2O3 CCSs display improved physical properties, such as high adhesion strength of the ceramic coating layer, thermal stability, electrolyte wettability, and increased ionic conductivity. Moreover, the CCSs exhibit enhanced electrochemical performance. Half cells (LiMn2O4/Li metal) comprising CCSs retained 96.5% (144.8 mAh g−1) of the initial discharge capacity even after 200 cycles, while bare PE separators lose their capacity rapidly after 150 cycles, retaining only 22.62% (33.5 mAh g−1) at the 200th cycle. Lithium-ion batteries Al Aqueous slurry Microporous polyolefin separators Kim, Jungmin verfasserin aut Kim, Jeongtae verfasserin aut Phiri, Isheunesu verfasserin (orcid)0000-0001-5186-566X aut Ryou, Sun-Yul verfasserin (orcid)0000-0001-8899-019X aut Enthalten in Journal of industrial and engineering chemistry Seoul : KSIEC, 1995 130, Seite 638-647 (DE-627)391337238 (DE-600)2152565-1 (DE-576)28474784X 1226-086X nnns volume:130 pages:638-647 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 130 638-647 |
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600 540 VZ Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries Lithium-ion batteries Al Aqueous slurry Microporous polyolefin separators |
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Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries |
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Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries |
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Kennedy, Ssendagire |
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Kennedy, Ssendagire Kim, Jungmin Kim, Jeongtae Phiri, Isheunesu Ryou, Sun-Yul |
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water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries |
title_auth |
Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries |
abstract |
A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determining the polymer binders (CMC/PVA) content in the ceramic slurry and studying the interaction between the polymer binders and Al2O3 ceramic particles by changing the mixing order of the slurry components. CMC effectively controls the viscosity of the slurry to maintain a stable slurry dispersion. In contrast, PVA significantly influences the formation of a uniform ceramic coating layer on the polyethylene (PE) separator. This results in a synergistic effect to produce an optimal ceramic-coated composite separator (CCS). Compared to the bare PE separators, the prepared Al2O3 CCSs display improved physical properties, such as high adhesion strength of the ceramic coating layer, thermal stability, electrolyte wettability, and increased ionic conductivity. Moreover, the CCSs exhibit enhanced electrochemical performance. Half cells (LiMn2O4/Li metal) comprising CCSs retained 96.5% (144.8 mAh g−1) of the initial discharge capacity even after 200 cycles, while bare PE separators lose their capacity rapidly after 150 cycles, retaining only 22.62% (33.5 mAh g−1) at the 200th cycle. |
abstractGer |
A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determining the polymer binders (CMC/PVA) content in the ceramic slurry and studying the interaction between the polymer binders and Al2O3 ceramic particles by changing the mixing order of the slurry components. CMC effectively controls the viscosity of the slurry to maintain a stable slurry dispersion. In contrast, PVA significantly influences the formation of a uniform ceramic coating layer on the polyethylene (PE) separator. This results in a synergistic effect to produce an optimal ceramic-coated composite separator (CCS). Compared to the bare PE separators, the prepared Al2O3 CCSs display improved physical properties, such as high adhesion strength of the ceramic coating layer, thermal stability, electrolyte wettability, and increased ionic conductivity. Moreover, the CCSs exhibit enhanced electrochemical performance. Half cells (LiMn2O4/Li metal) comprising CCSs retained 96.5% (144.8 mAh g−1) of the initial discharge capacity even after 200 cycles, while bare PE separators lose their capacity rapidly after 150 cycles, retaining only 22.62% (33.5 mAh g−1) at the 200th cycle. |
abstract_unstemmed |
A simple, eco-friendly, and effective additive-free technique for stabilizing a coating slurry, using alumina (Al2O3) inorganic particles and aqueous dual polymers—sodium carboxymethyl cellulose (CMC) and polyvinyl alcohol (PVA) is developed. The slurry preparation process is optimized by determining the polymer binders (CMC/PVA) content in the ceramic slurry and studying the interaction between the polymer binders and Al2O3 ceramic particles by changing the mixing order of the slurry components. CMC effectively controls the viscosity of the slurry to maintain a stable slurry dispersion. In contrast, PVA significantly influences the formation of a uniform ceramic coating layer on the polyethylene (PE) separator. This results in a synergistic effect to produce an optimal ceramic-coated composite separator (CCS). Compared to the bare PE separators, the prepared Al2O3 CCSs display improved physical properties, such as high adhesion strength of the ceramic coating layer, thermal stability, electrolyte wettability, and increased ionic conductivity. Moreover, the CCSs exhibit enhanced electrochemical performance. Half cells (LiMn2O4/Li metal) comprising CCSs retained 96.5% (144.8 mAh g−1) of the initial discharge capacity even after 200 cycles, while bare PE separators lose their capacity rapidly after 150 cycles, retaining only 22.62% (33.5 mAh g−1) at the 200th cycle. |
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Water-based dual polymer ceramic-coated composite separator for high-energy-density lithium secondary batteries |
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