Interface engineering of FeOF/FeF 2 heterostructure for ultrastable Li-ion/Na-ion storage
Iron fluoride is a prospective cathode material for Li-ion batteries (LIBs) and Na-ion batteries (SIBs) due to their high theoretical capacity and working voltage, whereas the practical applicability is inhibited by its slow reaction kinetics and poor cycling stability. Herein, the FeOF/FeF2 heteros...
Ausführliche Beschreibung
Autor*in: |
Zhou, Hongyan [verfasserIn] Zhao, Yanming [verfasserIn] Li, Yunbo [verfasserIn] Kuang, Quan [verfasserIn] Dong, Youzhong [verfasserIn] Fan, Qinghua [verfasserIn] |
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E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2023 |
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Schlagwörter: |
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Übergeordnetes Werk: |
Enthalten in: Journal of power sources - New York, NY [u.a.] : Elsevier, 1976, 592 |
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Übergeordnetes Werk: |
volume:592 |
DOI / URN: |
10.1016/j.jpowsour.2023.233911 |
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Katalog-ID: |
ELV066272238 |
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520 | |a Iron fluoride is a prospective cathode material for Li-ion batteries (LIBs) and Na-ion batteries (SIBs) due to their high theoretical capacity and working voltage, whereas the practical applicability is inhibited by its slow reaction kinetics and poor cycling stability. Herein, the FeOF/FeF2 heterostructure is constructed to address the aforementioned issues and obtain ultrastable Li-ion/Na-ion storage. The FeOF/FeF2 heterostructure possesses a built-in electric field, oxygen vacancies and a homo-tetragonal phase, which can considerably improve the charge transfer kinetics, increase the ion storage sites and strengthen the structural stability. As expected, the FeOF/FeF2 cathode delivers remarkable cycle stability: 134.7 mAh g−1 after 1000 cycles at 1000 mA g− 1 for LIBs, and 124.8 mAh g−1 after 200 cycles at 500 mA g− 1 for SIBs. Furthermore, the Li-ion/Na-ion storage mechanism of the FeOF/FeF2 heterostructure during the electrochemical process is revealed through in-situ X-ray diffraction and ex-situ characterizations. This method of constructing heterostructure opens a way for other conversion materials to achieve high-performance LIBs/SIBs. | ||
650 | 4 | |a FeOF/FeF | |
650 | 4 | |a Heterostructure | |
650 | 4 | |a Li-ion batteries | |
650 | 4 | |a Na-ion batteries | |
700 | 1 | |a Zhao, Yanming |e verfasserin |0 (orcid)0000-0002-0056-7248 |4 aut | |
700 | 1 | |a Li, Yunbo |e verfasserin |4 aut | |
700 | 1 | |a Kuang, Quan |e verfasserin |4 aut | |
700 | 1 | |a Dong, Youzhong |e verfasserin |4 aut | |
700 | 1 | |a Fan, Qinghua |e verfasserin |4 aut | |
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allfields |
10.1016/j.jpowsour.2023.233911 doi (DE-627)ELV066272238 (ELSEVIER)S0378-7753(23)01287-9 DE-627 ger DE-627 rda eng 620 VZ 52.57 bkl 53.36 bkl Zhou, Hongyan verfasserin aut Interface engineering of FeOF/FeF 2 heterostructure for ultrastable Li-ion/Na-ion storage 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Iron fluoride is a prospective cathode material for Li-ion batteries (LIBs) and Na-ion batteries (SIBs) due to their high theoretical capacity and working voltage, whereas the practical applicability is inhibited by its slow reaction kinetics and poor cycling stability. Herein, the FeOF/FeF2 heterostructure is constructed to address the aforementioned issues and obtain ultrastable Li-ion/Na-ion storage. The FeOF/FeF2 heterostructure possesses a built-in electric field, oxygen vacancies and a homo-tetragonal phase, which can considerably improve the charge transfer kinetics, increase the ion storage sites and strengthen the structural stability. As expected, the FeOF/FeF2 cathode delivers remarkable cycle stability: 134.7 mAh g−1 after 1000 cycles at 1000 mA g− 1 for LIBs, and 124.8 mAh g−1 after 200 cycles at 500 mA g− 1 for SIBs. Furthermore, the Li-ion/Na-ion storage mechanism of the FeOF/FeF2 heterostructure during the electrochemical process is revealed through in-situ X-ray diffraction and ex-situ characterizations. This method of constructing heterostructure opens a way for other conversion materials to achieve high-performance LIBs/SIBs. FeOF/FeF Heterostructure Li-ion batteries Na-ion batteries Zhao, Yanming verfasserin (orcid)0000-0002-0056-7248 aut Li, Yunbo verfasserin aut Kuang, Quan verfasserin aut Dong, Youzhong verfasserin aut Fan, Qinghua verfasserin aut Enthalten in Journal of power sources New York, NY [u.a.] : Elsevier, 1976 592 Online-Ressource (DE-627)302718923 (DE-600)1491915-1 (DE-576)259483958 1873-2755 nnns volume:592 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.57 Energiespeicherung VZ 53.36 Energiedirektumwandler elektrische Energiespeicher VZ AR 592 |
spelling |
10.1016/j.jpowsour.2023.233911 doi (DE-627)ELV066272238 (ELSEVIER)S0378-7753(23)01287-9 DE-627 ger DE-627 rda eng 620 VZ 52.57 bkl 53.36 bkl Zhou, Hongyan verfasserin aut Interface engineering of FeOF/FeF 2 heterostructure for ultrastable Li-ion/Na-ion storage 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Iron fluoride is a prospective cathode material for Li-ion batteries (LIBs) and Na-ion batteries (SIBs) due to their high theoretical capacity and working voltage, whereas the practical applicability is inhibited by its slow reaction kinetics and poor cycling stability. Herein, the FeOF/FeF2 heterostructure is constructed to address the aforementioned issues and obtain ultrastable Li-ion/Na-ion storage. The FeOF/FeF2 heterostructure possesses a built-in electric field, oxygen vacancies and a homo-tetragonal phase, which can considerably improve the charge transfer kinetics, increase the ion storage sites and strengthen the structural stability. As expected, the FeOF/FeF2 cathode delivers remarkable cycle stability: 134.7 mAh g−1 after 1000 cycles at 1000 mA g− 1 for LIBs, and 124.8 mAh g−1 after 200 cycles at 500 mA g− 1 for SIBs. Furthermore, the Li-ion/Na-ion storage mechanism of the FeOF/FeF2 heterostructure during the electrochemical process is revealed through in-situ X-ray diffraction and ex-situ characterizations. This method of constructing heterostructure opens a way for other conversion materials to achieve high-performance LIBs/SIBs. FeOF/FeF Heterostructure Li-ion batteries Na-ion batteries Zhao, Yanming verfasserin (orcid)0000-0002-0056-7248 aut Li, Yunbo verfasserin aut Kuang, Quan verfasserin aut Dong, Youzhong verfasserin aut Fan, Qinghua verfasserin aut Enthalten in Journal of power sources New York, NY [u.a.] : Elsevier, 1976 592 Online-Ressource (DE-627)302718923 (DE-600)1491915-1 (DE-576)259483958 1873-2755 nnns volume:592 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.57 Energiespeicherung VZ 53.36 Energiedirektumwandler elektrische Energiespeicher VZ AR 592 |
allfields_unstemmed |
10.1016/j.jpowsour.2023.233911 doi (DE-627)ELV066272238 (ELSEVIER)S0378-7753(23)01287-9 DE-627 ger DE-627 rda eng 620 VZ 52.57 bkl 53.36 bkl Zhou, Hongyan verfasserin aut Interface engineering of FeOF/FeF 2 heterostructure for ultrastable Li-ion/Na-ion storage 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Iron fluoride is a prospective cathode material for Li-ion batteries (LIBs) and Na-ion batteries (SIBs) due to their high theoretical capacity and working voltage, whereas the practical applicability is inhibited by its slow reaction kinetics and poor cycling stability. Herein, the FeOF/FeF2 heterostructure is constructed to address the aforementioned issues and obtain ultrastable Li-ion/Na-ion storage. The FeOF/FeF2 heterostructure possesses a built-in electric field, oxygen vacancies and a homo-tetragonal phase, which can considerably improve the charge transfer kinetics, increase the ion storage sites and strengthen the structural stability. As expected, the FeOF/FeF2 cathode delivers remarkable cycle stability: 134.7 mAh g−1 after 1000 cycles at 1000 mA g− 1 for LIBs, and 124.8 mAh g−1 after 200 cycles at 500 mA g− 1 for SIBs. Furthermore, the Li-ion/Na-ion storage mechanism of the FeOF/FeF2 heterostructure during the electrochemical process is revealed through in-situ X-ray diffraction and ex-situ characterizations. This method of constructing heterostructure opens a way for other conversion materials to achieve high-performance LIBs/SIBs. FeOF/FeF Heterostructure Li-ion batteries Na-ion batteries Zhao, Yanming verfasserin (orcid)0000-0002-0056-7248 aut Li, Yunbo verfasserin aut Kuang, Quan verfasserin aut Dong, Youzhong verfasserin aut Fan, Qinghua verfasserin aut Enthalten in Journal of power sources New York, NY [u.a.] : Elsevier, 1976 592 Online-Ressource (DE-627)302718923 (DE-600)1491915-1 (DE-576)259483958 1873-2755 nnns volume:592 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.57 Energiespeicherung VZ 53.36 Energiedirektumwandler elektrische Energiespeicher VZ AR 592 |
allfieldsGer |
10.1016/j.jpowsour.2023.233911 doi (DE-627)ELV066272238 (ELSEVIER)S0378-7753(23)01287-9 DE-627 ger DE-627 rda eng 620 VZ 52.57 bkl 53.36 bkl Zhou, Hongyan verfasserin aut Interface engineering of FeOF/FeF 2 heterostructure for ultrastable Li-ion/Na-ion storage 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Iron fluoride is a prospective cathode material for Li-ion batteries (LIBs) and Na-ion batteries (SIBs) due to their high theoretical capacity and working voltage, whereas the practical applicability is inhibited by its slow reaction kinetics and poor cycling stability. Herein, the FeOF/FeF2 heterostructure is constructed to address the aforementioned issues and obtain ultrastable Li-ion/Na-ion storage. The FeOF/FeF2 heterostructure possesses a built-in electric field, oxygen vacancies and a homo-tetragonal phase, which can considerably improve the charge transfer kinetics, increase the ion storage sites and strengthen the structural stability. As expected, the FeOF/FeF2 cathode delivers remarkable cycle stability: 134.7 mAh g−1 after 1000 cycles at 1000 mA g− 1 for LIBs, and 124.8 mAh g−1 after 200 cycles at 500 mA g− 1 for SIBs. Furthermore, the Li-ion/Na-ion storage mechanism of the FeOF/FeF2 heterostructure during the electrochemical process is revealed through in-situ X-ray diffraction and ex-situ characterizations. This method of constructing heterostructure opens a way for other conversion materials to achieve high-performance LIBs/SIBs. FeOF/FeF Heterostructure Li-ion batteries Na-ion batteries Zhao, Yanming verfasserin (orcid)0000-0002-0056-7248 aut Li, Yunbo verfasserin aut Kuang, Quan verfasserin aut Dong, Youzhong verfasserin aut Fan, Qinghua verfasserin aut Enthalten in Journal of power sources New York, NY [u.a.] : Elsevier, 1976 592 Online-Ressource (DE-627)302718923 (DE-600)1491915-1 (DE-576)259483958 1873-2755 nnns volume:592 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.57 Energiespeicherung VZ 53.36 Energiedirektumwandler elektrische Energiespeicher VZ AR 592 |
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10.1016/j.jpowsour.2023.233911 doi (DE-627)ELV066272238 (ELSEVIER)S0378-7753(23)01287-9 DE-627 ger DE-627 rda eng 620 VZ 52.57 bkl 53.36 bkl Zhou, Hongyan verfasserin aut Interface engineering of FeOF/FeF 2 heterostructure for ultrastable Li-ion/Na-ion storage 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Iron fluoride is a prospective cathode material for Li-ion batteries (LIBs) and Na-ion batteries (SIBs) due to their high theoretical capacity and working voltage, whereas the practical applicability is inhibited by its slow reaction kinetics and poor cycling stability. Herein, the FeOF/FeF2 heterostructure is constructed to address the aforementioned issues and obtain ultrastable Li-ion/Na-ion storage. The FeOF/FeF2 heterostructure possesses a built-in electric field, oxygen vacancies and a homo-tetragonal phase, which can considerably improve the charge transfer kinetics, increase the ion storage sites and strengthen the structural stability. As expected, the FeOF/FeF2 cathode delivers remarkable cycle stability: 134.7 mAh g−1 after 1000 cycles at 1000 mA g− 1 for LIBs, and 124.8 mAh g−1 after 200 cycles at 500 mA g− 1 for SIBs. Furthermore, the Li-ion/Na-ion storage mechanism of the FeOF/FeF2 heterostructure during the electrochemical process is revealed through in-situ X-ray diffraction and ex-situ characterizations. This method of constructing heterostructure opens a way for other conversion materials to achieve high-performance LIBs/SIBs. FeOF/FeF Heterostructure Li-ion batteries Na-ion batteries Zhao, Yanming verfasserin (orcid)0000-0002-0056-7248 aut Li, Yunbo verfasserin aut Kuang, Quan verfasserin aut Dong, Youzhong verfasserin aut Fan, Qinghua verfasserin aut Enthalten in Journal of power sources New York, NY [u.a.] : Elsevier, 1976 592 Online-Ressource (DE-627)302718923 (DE-600)1491915-1 (DE-576)259483958 1873-2755 nnns volume:592 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.57 Energiespeicherung VZ 53.36 Energiedirektumwandler elektrische Energiespeicher VZ AR 592 |
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Zhou, Hongyan @@aut@@ Zhao, Yanming @@aut@@ Li, Yunbo @@aut@@ Kuang, Quan @@aut@@ Dong, Youzhong @@aut@@ Fan, Qinghua @@aut@@ |
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Zhou, Hongyan |
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Zhou, Hongyan ddc 620 bkl 52.57 bkl 53.36 misc FeOF/FeF misc Heterostructure misc Li-ion batteries misc Na-ion batteries Interface engineering of FeOF/FeF 2 heterostructure for ultrastable Li-ion/Na-ion storage |
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620 VZ 52.57 bkl 53.36 bkl Interface engineering of FeOF/FeF 2 heterostructure for ultrastable Li-ion/Na-ion storage FeOF/FeF Heterostructure Li-ion batteries Na-ion batteries |
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Interface engineering of FeOF/FeF 2 heterostructure for ultrastable Li-ion/Na-ion storage |
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interface engineering of feof/fef 2 heterostructure for ultrastable li-ion/na-ion storage |
title_auth |
Interface engineering of FeOF/FeF 2 heterostructure for ultrastable Li-ion/Na-ion storage |
abstract |
Iron fluoride is a prospective cathode material for Li-ion batteries (LIBs) and Na-ion batteries (SIBs) due to their high theoretical capacity and working voltage, whereas the practical applicability is inhibited by its slow reaction kinetics and poor cycling stability. Herein, the FeOF/FeF2 heterostructure is constructed to address the aforementioned issues and obtain ultrastable Li-ion/Na-ion storage. The FeOF/FeF2 heterostructure possesses a built-in electric field, oxygen vacancies and a homo-tetragonal phase, which can considerably improve the charge transfer kinetics, increase the ion storage sites and strengthen the structural stability. As expected, the FeOF/FeF2 cathode delivers remarkable cycle stability: 134.7 mAh g−1 after 1000 cycles at 1000 mA g− 1 for LIBs, and 124.8 mAh g−1 after 200 cycles at 500 mA g− 1 for SIBs. Furthermore, the Li-ion/Na-ion storage mechanism of the FeOF/FeF2 heterostructure during the electrochemical process is revealed through in-situ X-ray diffraction and ex-situ characterizations. This method of constructing heterostructure opens a way for other conversion materials to achieve high-performance LIBs/SIBs. |
abstractGer |
Iron fluoride is a prospective cathode material for Li-ion batteries (LIBs) and Na-ion batteries (SIBs) due to their high theoretical capacity and working voltage, whereas the practical applicability is inhibited by its slow reaction kinetics and poor cycling stability. Herein, the FeOF/FeF2 heterostructure is constructed to address the aforementioned issues and obtain ultrastable Li-ion/Na-ion storage. The FeOF/FeF2 heterostructure possesses a built-in electric field, oxygen vacancies and a homo-tetragonal phase, which can considerably improve the charge transfer kinetics, increase the ion storage sites and strengthen the structural stability. As expected, the FeOF/FeF2 cathode delivers remarkable cycle stability: 134.7 mAh g−1 after 1000 cycles at 1000 mA g− 1 for LIBs, and 124.8 mAh g−1 after 200 cycles at 500 mA g− 1 for SIBs. Furthermore, the Li-ion/Na-ion storage mechanism of the FeOF/FeF2 heterostructure during the electrochemical process is revealed through in-situ X-ray diffraction and ex-situ characterizations. This method of constructing heterostructure opens a way for other conversion materials to achieve high-performance LIBs/SIBs. |
abstract_unstemmed |
Iron fluoride is a prospective cathode material for Li-ion batteries (LIBs) and Na-ion batteries (SIBs) due to their high theoretical capacity and working voltage, whereas the practical applicability is inhibited by its slow reaction kinetics and poor cycling stability. Herein, the FeOF/FeF2 heterostructure is constructed to address the aforementioned issues and obtain ultrastable Li-ion/Na-ion storage. The FeOF/FeF2 heterostructure possesses a built-in electric field, oxygen vacancies and a homo-tetragonal phase, which can considerably improve the charge transfer kinetics, increase the ion storage sites and strengthen the structural stability. As expected, the FeOF/FeF2 cathode delivers remarkable cycle stability: 134.7 mAh g−1 after 1000 cycles at 1000 mA g− 1 for LIBs, and 124.8 mAh g−1 after 200 cycles at 500 mA g− 1 for SIBs. Furthermore, the Li-ion/Na-ion storage mechanism of the FeOF/FeF2 heterostructure during the electrochemical process is revealed through in-situ X-ray diffraction and ex-situ characterizations. This method of constructing heterostructure opens a way for other conversion materials to achieve high-performance LIBs/SIBs. |
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title_short |
Interface engineering of FeOF/FeF 2 heterostructure for ultrastable Li-ion/Na-ion storage |
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Zhao, Yanming Li, Yunbo Kuang, Quan Dong, Youzhong Fan, Qinghua |
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up_date |
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|
score |
7.401354 |