Microstructure engineering in sulfuretted coal tar pitch by varying the Cross-Link state for enhanced sodium storage
Sulfur (S) is an efficient dopant to enhance the sodium storage of carbon, yet the conventional in-situ/post treatments cause unstable S configuration or lower S content, and hence unsatisfied electrochemical performance. Herein, we investigate sulfurization at various cross-link state of coal tar p...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Zhao, Dan [verfasserIn] Zheng, Huiling [verfasserIn] Huang, Cheng [verfasserIn] Chang, Gaobo [verfasserIn] Li, Zhong [verfasserIn] Zhao, Hanqing [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2024 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Journal of colloid and interface science - Amsterdam [u.a.] : Elsevier, 1966, 660, Seite 845-858 |
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| Übergeordnetes Werk: |
volume:660 ; pages:845-858 |
| DOI / URN: |
10.1016/j.jcis.2024.01.095 |
|---|
| Katalog-ID: |
ELV066976146 |
|---|
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| 245 | 1 | 0 | |a Microstructure engineering in sulfuretted coal tar pitch by varying the Cross-Link state for enhanced sodium storage |
| 264 | 1 | |c 2024 | |
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| 520 | |a Sulfur (S) is an efficient dopant to enhance the sodium storage of carbon, yet the conventional in-situ/post treatments cause unstable S configuration or lower S content, and hence unsatisfied electrochemical performance. Herein, we investigate sulfurization at various cross-link state of coal tar pitch (CTP) (pristine, coke, and carbonized states), and the microstructure of the products (SCTP). Experimental and calculational results reveal that introducing S in the coke state of CTP is essential for achieving abundant and stable C-Sx-C bonds between carbon layers. Moreover, this innovative strategy not only achieves a high S content, but also avoids the liquid carbonization, resulting in a hierarchically porous structure with a small particle size. As a result, the SCTP delivers a sodium storage capacity of 318 mA h g−1 at 0.1 A g−1 after 200th cycle, and the capacity maintains 207 mA h g−1 with capacity retention of 99 % after 1000th cycle at 2.0 A g−1, in half-cells. Moreover, the sample shows a considerable discharge capacity of 328 mA h g-1 anode at 0.05 A g−1 in full-cells. Consequently, this approach offers a novel pathway for large-scale production of thermoplastic-derived carbons in battery industry. | ||
| 650 | 4 | |a Coal tar pitch | |
| 650 | 4 | |a Sulfur doping | |
| 650 | 4 | |a Microstructure regulation | |
| 650 | 4 | |a Anode | |
| 650 | 4 | |a Sodium storage | |
| 700 | 1 | |a Zheng, Huiling |e verfasserin |0 (orcid)0000-0001-8347-3724 |4 aut | |
| 700 | 1 | |a Huang, Cheng |e verfasserin |4 aut | |
| 700 | 1 | |a Chang, Gaobo |e verfasserin |4 aut | |
| 700 | 1 | |a Li, Zhong |e verfasserin |4 aut | |
| 700 | 1 | |a Zhao, Hanqing |e verfasserin |0 (orcid)0000-0003-0327-3699 |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |t Journal of colloid and interface science |d Amsterdam [u.a.] : Elsevier, 1966 |g 660, Seite 845-858 |h Online-Ressource |w (DE-627)266891136 |w (DE-600)1469021-4 |w (DE-576)103373160 |x 1095-7103 |7 nnns |
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10.1016/j.jcis.2024.01.095 doi (DE-627)ELV066976146 (ELSEVIER)S0021-9797(24)00104-8 DE-627 ger DE-627 rda eng 540 VZ 35.18 bkl Zhao, Dan verfasserin aut Microstructure engineering in sulfuretted coal tar pitch by varying the Cross-Link state for enhanced sodium storage 2024 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Sulfur (S) is an efficient dopant to enhance the sodium storage of carbon, yet the conventional in-situ/post treatments cause unstable S configuration or lower S content, and hence unsatisfied electrochemical performance. Herein, we investigate sulfurization at various cross-link state of coal tar pitch (CTP) (pristine, coke, and carbonized states), and the microstructure of the products (SCTP). Experimental and calculational results reveal that introducing S in the coke state of CTP is essential for achieving abundant and stable C-Sx-C bonds between carbon layers. Moreover, this innovative strategy not only achieves a high S content, but also avoids the liquid carbonization, resulting in a hierarchically porous structure with a small particle size. As a result, the SCTP delivers a sodium storage capacity of 318 mA h g−1 at 0.1 A g−1 after 200th cycle, and the capacity maintains 207 mA h g−1 with capacity retention of 99 % after 1000th cycle at 2.0 A g−1, in half-cells. Moreover, the sample shows a considerable discharge capacity of 328 mA h g-1 anode at 0.05 A g−1 in full-cells. Consequently, this approach offers a novel pathway for large-scale production of thermoplastic-derived carbons in battery industry. Coal tar pitch Sulfur doping Microstructure regulation Anode Sodium storage Zheng, Huiling verfasserin (orcid)0000-0001-8347-3724 aut Huang, Cheng verfasserin aut Chang, Gaobo verfasserin aut Li, Zhong verfasserin aut Zhao, Hanqing verfasserin (orcid)0000-0003-0327-3699 aut Enthalten in Journal of colloid and interface science Amsterdam [u.a.] : Elsevier, 1966 660, Seite 845-858 Online-Ressource (DE-627)266891136 (DE-600)1469021-4 (DE-576)103373160 1095-7103 nnns volume:660 pages:845-858 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.18 Kolloidchemie Grenzflächenchemie VZ AR 660 845-858 |
| spelling |
10.1016/j.jcis.2024.01.095 doi (DE-627)ELV066976146 (ELSEVIER)S0021-9797(24)00104-8 DE-627 ger DE-627 rda eng 540 VZ 35.18 bkl Zhao, Dan verfasserin aut Microstructure engineering in sulfuretted coal tar pitch by varying the Cross-Link state for enhanced sodium storage 2024 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Sulfur (S) is an efficient dopant to enhance the sodium storage of carbon, yet the conventional in-situ/post treatments cause unstable S configuration or lower S content, and hence unsatisfied electrochemical performance. Herein, we investigate sulfurization at various cross-link state of coal tar pitch (CTP) (pristine, coke, and carbonized states), and the microstructure of the products (SCTP). Experimental and calculational results reveal that introducing S in the coke state of CTP is essential for achieving abundant and stable C-Sx-C bonds between carbon layers. Moreover, this innovative strategy not only achieves a high S content, but also avoids the liquid carbonization, resulting in a hierarchically porous structure with a small particle size. As a result, the SCTP delivers a sodium storage capacity of 318 mA h g−1 at 0.1 A g−1 after 200th cycle, and the capacity maintains 207 mA h g−1 with capacity retention of 99 % after 1000th cycle at 2.0 A g−1, in half-cells. Moreover, the sample shows a considerable discharge capacity of 328 mA h g-1 anode at 0.05 A g−1 in full-cells. Consequently, this approach offers a novel pathway for large-scale production of thermoplastic-derived carbons in battery industry. Coal tar pitch Sulfur doping Microstructure regulation Anode Sodium storage Zheng, Huiling verfasserin (orcid)0000-0001-8347-3724 aut Huang, Cheng verfasserin aut Chang, Gaobo verfasserin aut Li, Zhong verfasserin aut Zhao, Hanqing verfasserin (orcid)0000-0003-0327-3699 aut Enthalten in Journal of colloid and interface science Amsterdam [u.a.] : Elsevier, 1966 660, Seite 845-858 Online-Ressource (DE-627)266891136 (DE-600)1469021-4 (DE-576)103373160 1095-7103 nnns volume:660 pages:845-858 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.18 Kolloidchemie Grenzflächenchemie VZ AR 660 845-858 |
| allfields_unstemmed |
10.1016/j.jcis.2024.01.095 doi (DE-627)ELV066976146 (ELSEVIER)S0021-9797(24)00104-8 DE-627 ger DE-627 rda eng 540 VZ 35.18 bkl Zhao, Dan verfasserin aut Microstructure engineering in sulfuretted coal tar pitch by varying the Cross-Link state for enhanced sodium storage 2024 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Sulfur (S) is an efficient dopant to enhance the sodium storage of carbon, yet the conventional in-situ/post treatments cause unstable S configuration or lower S content, and hence unsatisfied electrochemical performance. Herein, we investigate sulfurization at various cross-link state of coal tar pitch (CTP) (pristine, coke, and carbonized states), and the microstructure of the products (SCTP). Experimental and calculational results reveal that introducing S in the coke state of CTP is essential for achieving abundant and stable C-Sx-C bonds between carbon layers. Moreover, this innovative strategy not only achieves a high S content, but also avoids the liquid carbonization, resulting in a hierarchically porous structure with a small particle size. As a result, the SCTP delivers a sodium storage capacity of 318 mA h g−1 at 0.1 A g−1 after 200th cycle, and the capacity maintains 207 mA h g−1 with capacity retention of 99 % after 1000th cycle at 2.0 A g−1, in half-cells. Moreover, the sample shows a considerable discharge capacity of 328 mA h g-1 anode at 0.05 A g−1 in full-cells. Consequently, this approach offers a novel pathway for large-scale production of thermoplastic-derived carbons in battery industry. Coal tar pitch Sulfur doping Microstructure regulation Anode Sodium storage Zheng, Huiling verfasserin (orcid)0000-0001-8347-3724 aut Huang, Cheng verfasserin aut Chang, Gaobo verfasserin aut Li, Zhong verfasserin aut Zhao, Hanqing verfasserin (orcid)0000-0003-0327-3699 aut Enthalten in Journal of colloid and interface science Amsterdam [u.a.] : Elsevier, 1966 660, Seite 845-858 Online-Ressource (DE-627)266891136 (DE-600)1469021-4 (DE-576)103373160 1095-7103 nnns volume:660 pages:845-858 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.18 Kolloidchemie Grenzflächenchemie VZ AR 660 845-858 |
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10.1016/j.jcis.2024.01.095 doi (DE-627)ELV066976146 (ELSEVIER)S0021-9797(24)00104-8 DE-627 ger DE-627 rda eng 540 VZ 35.18 bkl Zhao, Dan verfasserin aut Microstructure engineering in sulfuretted coal tar pitch by varying the Cross-Link state for enhanced sodium storage 2024 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Sulfur (S) is an efficient dopant to enhance the sodium storage of carbon, yet the conventional in-situ/post treatments cause unstable S configuration or lower S content, and hence unsatisfied electrochemical performance. Herein, we investigate sulfurization at various cross-link state of coal tar pitch (CTP) (pristine, coke, and carbonized states), and the microstructure of the products (SCTP). Experimental and calculational results reveal that introducing S in the coke state of CTP is essential for achieving abundant and stable C-Sx-C bonds between carbon layers. Moreover, this innovative strategy not only achieves a high S content, but also avoids the liquid carbonization, resulting in a hierarchically porous structure with a small particle size. As a result, the SCTP delivers a sodium storage capacity of 318 mA h g−1 at 0.1 A g−1 after 200th cycle, and the capacity maintains 207 mA h g−1 with capacity retention of 99 % after 1000th cycle at 2.0 A g−1, in half-cells. Moreover, the sample shows a considerable discharge capacity of 328 mA h g-1 anode at 0.05 A g−1 in full-cells. Consequently, this approach offers a novel pathway for large-scale production of thermoplastic-derived carbons in battery industry. Coal tar pitch Sulfur doping Microstructure regulation Anode Sodium storage Zheng, Huiling verfasserin (orcid)0000-0001-8347-3724 aut Huang, Cheng verfasserin aut Chang, Gaobo verfasserin aut Li, Zhong verfasserin aut Zhao, Hanqing verfasserin (orcid)0000-0003-0327-3699 aut Enthalten in Journal of colloid and interface science Amsterdam [u.a.] : Elsevier, 1966 660, Seite 845-858 Online-Ressource (DE-627)266891136 (DE-600)1469021-4 (DE-576)103373160 1095-7103 nnns volume:660 pages:845-858 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.18 Kolloidchemie Grenzflächenchemie VZ AR 660 845-858 |
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10.1016/j.jcis.2024.01.095 doi (DE-627)ELV066976146 (ELSEVIER)S0021-9797(24)00104-8 DE-627 ger DE-627 rda eng 540 VZ 35.18 bkl Zhao, Dan verfasserin aut Microstructure engineering in sulfuretted coal tar pitch by varying the Cross-Link state for enhanced sodium storage 2024 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Sulfur (S) is an efficient dopant to enhance the sodium storage of carbon, yet the conventional in-situ/post treatments cause unstable S configuration or lower S content, and hence unsatisfied electrochemical performance. Herein, we investigate sulfurization at various cross-link state of coal tar pitch (CTP) (pristine, coke, and carbonized states), and the microstructure of the products (SCTP). Experimental and calculational results reveal that introducing S in the coke state of CTP is essential for achieving abundant and stable C-Sx-C bonds between carbon layers. Moreover, this innovative strategy not only achieves a high S content, but also avoids the liquid carbonization, resulting in a hierarchically porous structure with a small particle size. As a result, the SCTP delivers a sodium storage capacity of 318 mA h g−1 at 0.1 A g−1 after 200th cycle, and the capacity maintains 207 mA h g−1 with capacity retention of 99 % after 1000th cycle at 2.0 A g−1, in half-cells. Moreover, the sample shows a considerable discharge capacity of 328 mA h g-1 anode at 0.05 A g−1 in full-cells. Consequently, this approach offers a novel pathway for large-scale production of thermoplastic-derived carbons in battery industry. Coal tar pitch Sulfur doping Microstructure regulation Anode Sodium storage Zheng, Huiling verfasserin (orcid)0000-0001-8347-3724 aut Huang, Cheng verfasserin aut Chang, Gaobo verfasserin aut Li, Zhong verfasserin aut Zhao, Hanqing verfasserin (orcid)0000-0003-0327-3699 aut Enthalten in Journal of colloid and interface science Amsterdam [u.a.] : Elsevier, 1966 660, Seite 845-858 Online-Ressource (DE-627)266891136 (DE-600)1469021-4 (DE-576)103373160 1095-7103 nnns volume:660 pages:845-858 GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.18 Kolloidchemie Grenzflächenchemie VZ AR 660 845-858 |
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Enthalten in Journal of colloid and interface science 660, Seite 845-858 volume:660 pages:845-858 |
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Coal tar pitch Sulfur doping Microstructure regulation Anode Sodium storage |
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Zhao, Dan @@aut@@ Zheng, Huiling @@aut@@ Huang, Cheng @@aut@@ Chang, Gaobo @@aut@@ Li, Zhong @@aut@@ Zhao, Hanqing @@aut@@ |
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Zhao, Dan |
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Zhao, Dan ddc 540 bkl 35.18 misc Coal tar pitch misc Sulfur doping misc Microstructure regulation misc Anode misc Sodium storage Microstructure engineering in sulfuretted coal tar pitch by varying the Cross-Link state for enhanced sodium storage |
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540 VZ 35.18 bkl Microstructure engineering in sulfuretted coal tar pitch by varying the Cross-Link state for enhanced sodium storage Coal tar pitch Sulfur doping Microstructure regulation Anode Sodium storage |
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ddc 540 bkl 35.18 misc Coal tar pitch misc Sulfur doping misc Microstructure regulation misc Anode misc Sodium storage |
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Microstructure engineering in sulfuretted coal tar pitch by varying the Cross-Link state for enhanced sodium storage |
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Microstructure engineering in sulfuretted coal tar pitch by varying the Cross-Link state for enhanced sodium storage |
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Zhao, Dan Zheng, Huiling Huang, Cheng Chang, Gaobo Li, Zhong Zhao, Hanqing |
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microstructure engineering in sulfuretted coal tar pitch by varying the cross-link state for enhanced sodium storage |
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Microstructure engineering in sulfuretted coal tar pitch by varying the Cross-Link state for enhanced sodium storage |
| abstract |
Sulfur (S) is an efficient dopant to enhance the sodium storage of carbon, yet the conventional in-situ/post treatments cause unstable S configuration or lower S content, and hence unsatisfied electrochemical performance. Herein, we investigate sulfurization at various cross-link state of coal tar pitch (CTP) (pristine, coke, and carbonized states), and the microstructure of the products (SCTP). Experimental and calculational results reveal that introducing S in the coke state of CTP is essential for achieving abundant and stable C-Sx-C bonds between carbon layers. Moreover, this innovative strategy not only achieves a high S content, but also avoids the liquid carbonization, resulting in a hierarchically porous structure with a small particle size. As a result, the SCTP delivers a sodium storage capacity of 318 mA h g−1 at 0.1 A g−1 after 200th cycle, and the capacity maintains 207 mA h g−1 with capacity retention of 99 % after 1000th cycle at 2.0 A g−1, in half-cells. Moreover, the sample shows a considerable discharge capacity of 328 mA h g-1 anode at 0.05 A g−1 in full-cells. Consequently, this approach offers a novel pathway for large-scale production of thermoplastic-derived carbons in battery industry. |
| abstractGer |
Sulfur (S) is an efficient dopant to enhance the sodium storage of carbon, yet the conventional in-situ/post treatments cause unstable S configuration or lower S content, and hence unsatisfied electrochemical performance. Herein, we investigate sulfurization at various cross-link state of coal tar pitch (CTP) (pristine, coke, and carbonized states), and the microstructure of the products (SCTP). Experimental and calculational results reveal that introducing S in the coke state of CTP is essential for achieving abundant and stable C-Sx-C bonds between carbon layers. Moreover, this innovative strategy not only achieves a high S content, but also avoids the liquid carbonization, resulting in a hierarchically porous structure with a small particle size. As a result, the SCTP delivers a sodium storage capacity of 318 mA h g−1 at 0.1 A g−1 after 200th cycle, and the capacity maintains 207 mA h g−1 with capacity retention of 99 % after 1000th cycle at 2.0 A g−1, in half-cells. Moreover, the sample shows a considerable discharge capacity of 328 mA h g-1 anode at 0.05 A g−1 in full-cells. Consequently, this approach offers a novel pathway for large-scale production of thermoplastic-derived carbons in battery industry. |
| abstract_unstemmed |
Sulfur (S) is an efficient dopant to enhance the sodium storage of carbon, yet the conventional in-situ/post treatments cause unstable S configuration or lower S content, and hence unsatisfied electrochemical performance. Herein, we investigate sulfurization at various cross-link state of coal tar pitch (CTP) (pristine, coke, and carbonized states), and the microstructure of the products (SCTP). Experimental and calculational results reveal that introducing S in the coke state of CTP is essential for achieving abundant and stable C-Sx-C bonds between carbon layers. Moreover, this innovative strategy not only achieves a high S content, but also avoids the liquid carbonization, resulting in a hierarchically porous structure with a small particle size. As a result, the SCTP delivers a sodium storage capacity of 318 mA h g−1 at 0.1 A g−1 after 200th cycle, and the capacity maintains 207 mA h g−1 with capacity retention of 99 % after 1000th cycle at 2.0 A g−1, in half-cells. Moreover, the sample shows a considerable discharge capacity of 328 mA h g-1 anode at 0.05 A g−1 in full-cells. Consequently, this approach offers a novel pathway for large-scale production of thermoplastic-derived carbons in battery industry. |
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Microstructure engineering in sulfuretted coal tar pitch by varying the Cross-Link state for enhanced sodium storage |
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| score |
7.4001894 |