Regulating B-N moieties in carbon anode toward stable and fast potassium-storage

Boron (B) and nitrogen (N) co-doped hard carbons usually tend to deliver an excellent rate and ultra-long cycle lifespan, because of the formed B-N moieties can accelerate both ion/electron transfer. However, the rational regulation of B-N moieties content is rarely mentioned, and correlating rate a...
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Autor*in:	Song, Fan [verfasserIn] Li, Zihan [verfasserIn] Zhang, Di [verfasserIn] Sun, Huilan [verfasserIn] Li, Zhaojin [verfasserIn] Wang, Qiujun [verfasserIn] Sun, Qujiang [verfasserIn] Yuan, Fei [verfasserIn] Wang, Bo [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2024

Schlagwörter:	B-N moieties Hard carbon Potassium ion battery Anode

Übergeordnetes Werk:	Enthalten in: Electrochimica acta - New York, NY [u.a.] : Elsevier, 1959, 480
Übergeordnetes Werk:	volume:480

DOI / URN:	10.1016/j.electacta.2024.143883

Katalog-ID:	ELV067124429

Internformat


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520			\|a Boron (B) and nitrogen (N) co-doped hard carbons usually tend to deliver an excellent rate and ultra-long cycle lifespan, because of the formed B-N moieties can accelerate both ion/electron transfer. However, the rational regulation of B-N moieties content is rarely mentioned, and correlating rate and reversible capacity with B-N moieties content is still lacking yet. Hence, a series of B/N co-doped hard carbons are designed based on varied carbonization temperatures. Systematic characterizations prove that the introduced B-heteroatoms can create more defects and form well-developed pore channels. Besides, with increasing carbonization temperatures, B-N moieties content first increases and then decreases, which is in accordance with the evolution of defect degree of carbon matrix. Therefore, rich B-N moieties can induce more defect sites to greatly improve capacitive contribution, and as a result both rate and reversible capacity are strongly correlated with B-N moieties content. Based on this, the electrode with the highest B-N moieties content (79.6 %) realizes an excellent rate (220.9 mAh g−1 at 2 A g−1) and cycling stability (over 2000 cycles). Note that the storage of B-N moieties on K + only occurs in a high potential region (>0.5 V), and this process is highly reversible.
650		4	\|a B-N moieties
650		4	\|a Hard carbon
650		4	\|a Potassium ion battery
650		4	\|a Anode
700	1		\|a Li, Zihan \|e verfasserin \|4 aut
700	1		\|a Zhang, Di \|e verfasserin \|4 aut
700	1		\|a Sun, Huilan \|e verfasserin \|4 aut
700	1		\|a Li, Zhaojin \|e verfasserin \|4 aut
700	1		\|a Wang, Qiujun \|e verfasserin \|4 aut
700	1		\|a Sun, Qujiang \|e verfasserin \|4 aut
700	1		\|a Yuan, Fei \|e verfasserin \|4 aut
700	1		\|a Wang, Bo \|e verfasserin \|0 (orcid)0000-0002-0466-6323 \|4 aut
773	0	8	\|i Enthalten in \|t Electrochimica acta \|d New York, NY [u.a.] : Elsevier, 1959 \|g 480 \|h Online-Ressource \|w (DE-627)300897561 \|w (DE-600)1483548-4 \|w (DE-576)094752451 \|x 1873-3859 \|7 nnns
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912			\|a GBV_ILN_2021
912			\|a GBV_ILN_2025
912			\|a GBV_ILN_2026
912			\|a GBV_ILN_2027
912			\|a GBV_ILN_2034
912			\|a GBV_ILN_2044
912			\|a GBV_ILN_2048
912			\|a GBV_ILN_2049
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912			\|a GBV_ILN_4305
912			\|a GBV_ILN_4306
912			\|a GBV_ILN_4307
912			\|a GBV_ILN_4313
912			\|a GBV_ILN_4322
912			\|a GBV_ILN_4323
912			\|a GBV_ILN_4324
912			\|a GBV_ILN_4326
912			\|a GBV_ILN_4333
912			\|a GBV_ILN_4334
912			\|a GBV_ILN_4338
912			\|a GBV_ILN_4393
912			\|a GBV_ILN_4700
936	b	k	\|a 35.00 \|j Chemie: Allgemeines \|q VZ
951			\|a AR
952			\|d 480

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allfields	10.1016/j.electacta.2024.143883 doi (DE-627)ELV067124429 (ELSEVIER)S0013-4686(24)00127-0 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Song, Fan verfasserin aut Regulating B-N moieties in carbon anode toward stable and fast potassium-storage 2024 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Boron (B) and nitrogen (N) co-doped hard carbons usually tend to deliver an excellent rate and ultra-long cycle lifespan, because of the formed B-N moieties can accelerate both ion/electron transfer. However, the rational regulation of B-N moieties content is rarely mentioned, and correlating rate and reversible capacity with B-N moieties content is still lacking yet. Hence, a series of B/N co-doped hard carbons are designed based on varied carbonization temperatures. Systematic characterizations prove that the introduced B-heteroatoms can create more defects and form well-developed pore channels. Besides, with increasing carbonization temperatures, B-N moieties content first increases and then decreases, which is in accordance with the evolution of defect degree of carbon matrix. Therefore, rich B-N moieties can induce more defect sites to greatly improve capacitive contribution, and as a result both rate and reversible capacity are strongly correlated with B-N moieties content. Based on this, the electrode with the highest B-N moieties content (79.6 %) realizes an excellent rate (220.9 mAh g−1 at 2 A g−1) and cycling stability (over 2000 cycles). Note that the storage of B-N moieties on K + only occurs in a high potential region (>0.5 V), and this process is highly reversible. B-N moieties Hard carbon Potassium ion battery Anode Li, Zihan verfasserin aut Zhang, Di verfasserin aut Sun, Huilan verfasserin aut Li, Zhaojin verfasserin aut Wang, Qiujun verfasserin aut Sun, Qujiang verfasserin aut Yuan, Fei verfasserin aut Wang, Bo verfasserin (orcid)0000-0002-0466-6323 aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 480 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:480 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 480
spelling	10.1016/j.electacta.2024.143883 doi (DE-627)ELV067124429 (ELSEVIER)S0013-4686(24)00127-0 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Song, Fan verfasserin aut Regulating B-N moieties in carbon anode toward stable and fast potassium-storage 2024 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Boron (B) and nitrogen (N) co-doped hard carbons usually tend to deliver an excellent rate and ultra-long cycle lifespan, because of the formed B-N moieties can accelerate both ion/electron transfer. However, the rational regulation of B-N moieties content is rarely mentioned, and correlating rate and reversible capacity with B-N moieties content is still lacking yet. Hence, a series of B/N co-doped hard carbons are designed based on varied carbonization temperatures. Systematic characterizations prove that the introduced B-heteroatoms can create more defects and form well-developed pore channels. Besides, with increasing carbonization temperatures, B-N moieties content first increases and then decreases, which is in accordance with the evolution of defect degree of carbon matrix. Therefore, rich B-N moieties can induce more defect sites to greatly improve capacitive contribution, and as a result both rate and reversible capacity are strongly correlated with B-N moieties content. Based on this, the electrode with the highest B-N moieties content (79.6 %) realizes an excellent rate (220.9 mAh g−1 at 2 A g−1) and cycling stability (over 2000 cycles). Note that the storage of B-N moieties on K + only occurs in a high potential region (>0.5 V), and this process is highly reversible. B-N moieties Hard carbon Potassium ion battery Anode Li, Zihan verfasserin aut Zhang, Di verfasserin aut Sun, Huilan verfasserin aut Li, Zhaojin verfasserin aut Wang, Qiujun verfasserin aut Sun, Qujiang verfasserin aut Yuan, Fei verfasserin aut Wang, Bo verfasserin (orcid)0000-0002-0466-6323 aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 480 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:480 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 480
allfields_unstemmed	10.1016/j.electacta.2024.143883 doi (DE-627)ELV067124429 (ELSEVIER)S0013-4686(24)00127-0 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Song, Fan verfasserin aut Regulating B-N moieties in carbon anode toward stable and fast potassium-storage 2024 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Boron (B) and nitrogen (N) co-doped hard carbons usually tend to deliver an excellent rate and ultra-long cycle lifespan, because of the formed B-N moieties can accelerate both ion/electron transfer. However, the rational regulation of B-N moieties content is rarely mentioned, and correlating rate and reversible capacity with B-N moieties content is still lacking yet. Hence, a series of B/N co-doped hard carbons are designed based on varied carbonization temperatures. Systematic characterizations prove that the introduced B-heteroatoms can create more defects and form well-developed pore channels. Besides, with increasing carbonization temperatures, B-N moieties content first increases and then decreases, which is in accordance with the evolution of defect degree of carbon matrix. Therefore, rich B-N moieties can induce more defect sites to greatly improve capacitive contribution, and as a result both rate and reversible capacity are strongly correlated with B-N moieties content. Based on this, the electrode with the highest B-N moieties content (79.6 %) realizes an excellent rate (220.9 mAh g−1 at 2 A g−1) and cycling stability (over 2000 cycles). Note that the storage of B-N moieties on K + only occurs in a high potential region (>0.5 V), and this process is highly reversible. B-N moieties Hard carbon Potassium ion battery Anode Li, Zihan verfasserin aut Zhang, Di verfasserin aut Sun, Huilan verfasserin aut Li, Zhaojin verfasserin aut Wang, Qiujun verfasserin aut Sun, Qujiang verfasserin aut Yuan, Fei verfasserin aut Wang, Bo verfasserin (orcid)0000-0002-0466-6323 aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 480 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:480 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 480
allfieldsGer	10.1016/j.electacta.2024.143883 doi (DE-627)ELV067124429 (ELSEVIER)S0013-4686(24)00127-0 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Song, Fan verfasserin aut Regulating B-N moieties in carbon anode toward stable and fast potassium-storage 2024 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Boron (B) and nitrogen (N) co-doped hard carbons usually tend to deliver an excellent rate and ultra-long cycle lifespan, because of the formed B-N moieties can accelerate both ion/electron transfer. However, the rational regulation of B-N moieties content is rarely mentioned, and correlating rate and reversible capacity with B-N moieties content is still lacking yet. Hence, a series of B/N co-doped hard carbons are designed based on varied carbonization temperatures. Systematic characterizations prove that the introduced B-heteroatoms can create more defects and form well-developed pore channels. Besides, with increasing carbonization temperatures, B-N moieties content first increases and then decreases, which is in accordance with the evolution of defect degree of carbon matrix. Therefore, rich B-N moieties can induce more defect sites to greatly improve capacitive contribution, and as a result both rate and reversible capacity are strongly correlated with B-N moieties content. Based on this, the electrode with the highest B-N moieties content (79.6 %) realizes an excellent rate (220.9 mAh g−1 at 2 A g−1) and cycling stability (over 2000 cycles). Note that the storage of B-N moieties on K + only occurs in a high potential region (>0.5 V), and this process is highly reversible. B-N moieties Hard carbon Potassium ion battery Anode Li, Zihan verfasserin aut Zhang, Di verfasserin aut Sun, Huilan verfasserin aut Li, Zhaojin verfasserin aut Wang, Qiujun verfasserin aut Sun, Qujiang verfasserin aut Yuan, Fei verfasserin aut Wang, Bo verfasserin (orcid)0000-0002-0466-6323 aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 480 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:480 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 480
allfieldsSound	10.1016/j.electacta.2024.143883 doi (DE-627)ELV067124429 (ELSEVIER)S0013-4686(24)00127-0 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Song, Fan verfasserin aut Regulating B-N moieties in carbon anode toward stable and fast potassium-storage 2024 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Boron (B) and nitrogen (N) co-doped hard carbons usually tend to deliver an excellent rate and ultra-long cycle lifespan, because of the formed B-N moieties can accelerate both ion/electron transfer. However, the rational regulation of B-N moieties content is rarely mentioned, and correlating rate and reversible capacity with B-N moieties content is still lacking yet. Hence, a series of B/N co-doped hard carbons are designed based on varied carbonization temperatures. Systematic characterizations prove that the introduced B-heteroatoms can create more defects and form well-developed pore channels. Besides, with increasing carbonization temperatures, B-N moieties content first increases and then decreases, which is in accordance with the evolution of defect degree of carbon matrix. Therefore, rich B-N moieties can induce more defect sites to greatly improve capacitive contribution, and as a result both rate and reversible capacity are strongly correlated with B-N moieties content. Based on this, the electrode with the highest B-N moieties content (79.6 %) realizes an excellent rate (220.9 mAh g−1 at 2 A g−1) and cycling stability (over 2000 cycles). Note that the storage of B-N moieties on K + only occurs in a high potential region (>0.5 V), and this process is highly reversible. B-N moieties Hard carbon Potassium ion battery Anode Li, Zihan verfasserin aut Zhang, Di verfasserin aut Sun, Huilan verfasserin aut Li, Zhaojin verfasserin aut Wang, Qiujun verfasserin aut Sun, Qujiang verfasserin aut Yuan, Fei verfasserin aut Wang, Bo verfasserin (orcid)0000-0002-0466-6323 aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 480 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:480 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.00 Chemie: Allgemeines VZ AR 480
language	English
source	Enthalten in Electrochimica acta 480 volume:480
sourceStr	Enthalten in Electrochimica acta 480 volume:480
format_phy_str_mv	Article
bklname	Chemie: Allgemeines
institution	findex.gbv.de
topic_facet	B-N moieties Hard carbon Potassium ion battery Anode
dewey-raw	540
isfreeaccess_bool	false
container_title	Electrochimica acta
authorswithroles_txt_mv	Song, Fan @@aut@@ Li, Zihan @@aut@@ Zhang, Di @@aut@@ Sun, Huilan @@aut@@ Li, Zhaojin @@aut@@ Wang, Qiujun @@aut@@ Sun, Qujiang @@aut@@ Yuan, Fei @@aut@@ Wang, Bo @@aut@@
publishDateDaySort_date	2024-01-01T00:00:00Z
hierarchy_top_id	300897561
dewey-sort	3540
id	ELV067124429
language_de	englisch
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author	Song, Fan
spellingShingle	Song, Fan ddc 540 bkl 35.00 misc B-N moieties misc Hard carbon misc Potassium ion battery misc Anode Regulating B-N moieties in carbon anode toward stable and fast potassium-storage
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topic_title	540 VZ 35.00 bkl Regulating B-N moieties in carbon anode toward stable and fast potassium-storage B-N moieties Hard carbon Potassium ion battery Anode
topic	ddc 540 bkl 35.00 misc B-N moieties misc Hard carbon misc Potassium ion battery misc Anode
topic_unstemmed	ddc 540 bkl 35.00 misc B-N moieties misc Hard carbon misc Potassium ion battery misc Anode
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title	Regulating B-N moieties in carbon anode toward stable and fast potassium-storage
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title_full	Regulating B-N moieties in carbon anode toward stable and fast potassium-storage
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author_browse	Song, Fan Li, Zihan Zhang, Di Sun, Huilan Li, Zhaojin Wang, Qiujun Sun, Qujiang Yuan, Fei Wang, Bo
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title_sort	regulating b-n moieties in carbon anode toward stable and fast potassium-storage
title_auth	Regulating B-N moieties in carbon anode toward stable and fast potassium-storage
abstract	Boron (B) and nitrogen (N) co-doped hard carbons usually tend to deliver an excellent rate and ultra-long cycle lifespan, because of the formed B-N moieties can accelerate both ion/electron transfer. However, the rational regulation of B-N moieties content is rarely mentioned, and correlating rate and reversible capacity with B-N moieties content is still lacking yet. Hence, a series of B/N co-doped hard carbons are designed based on varied carbonization temperatures. Systematic characterizations prove that the introduced B-heteroatoms can create more defects and form well-developed pore channels. Besides, with increasing carbonization temperatures, B-N moieties content first increases and then decreases, which is in accordance with the evolution of defect degree of carbon matrix. Therefore, rich B-N moieties can induce more defect sites to greatly improve capacitive contribution, and as a result both rate and reversible capacity are strongly correlated with B-N moieties content. Based on this, the electrode with the highest B-N moieties content (79.6 %) realizes an excellent rate (220.9 mAh g−1 at 2 A g−1) and cycling stability (over 2000 cycles). Note that the storage of B-N moieties on K + only occurs in a high potential region (>0.5 V), and this process is highly reversible.
abstractGer	Boron (B) and nitrogen (N) co-doped hard carbons usually tend to deliver an excellent rate and ultra-long cycle lifespan, because of the formed B-N moieties can accelerate both ion/electron transfer. However, the rational regulation of B-N moieties content is rarely mentioned, and correlating rate and reversible capacity with B-N moieties content is still lacking yet. Hence, a series of B/N co-doped hard carbons are designed based on varied carbonization temperatures. Systematic characterizations prove that the introduced B-heteroatoms can create more defects and form well-developed pore channels. Besides, with increasing carbonization temperatures, B-N moieties content first increases and then decreases, which is in accordance with the evolution of defect degree of carbon matrix. Therefore, rich B-N moieties can induce more defect sites to greatly improve capacitive contribution, and as a result both rate and reversible capacity are strongly correlated with B-N moieties content. Based on this, the electrode with the highest B-N moieties content (79.6 %) realizes an excellent rate (220.9 mAh g−1 at 2 A g−1) and cycling stability (over 2000 cycles). Note that the storage of B-N moieties on K + only occurs in a high potential region (>0.5 V), and this process is highly reversible.
abstract_unstemmed	Boron (B) and nitrogen (N) co-doped hard carbons usually tend to deliver an excellent rate and ultra-long cycle lifespan, because of the formed B-N moieties can accelerate both ion/electron transfer. However, the rational regulation of B-N moieties content is rarely mentioned, and correlating rate and reversible capacity with B-N moieties content is still lacking yet. Hence, a series of B/N co-doped hard carbons are designed based on varied carbonization temperatures. Systematic characterizations prove that the introduced B-heteroatoms can create more defects and form well-developed pore channels. Besides, with increasing carbonization temperatures, B-N moieties content first increases and then decreases, which is in accordance with the evolution of defect degree of carbon matrix. Therefore, rich B-N moieties can induce more defect sites to greatly improve capacitive contribution, and as a result both rate and reversible capacity are strongly correlated with B-N moieties content. Based on this, the electrode with the highest B-N moieties content (79.6 %) realizes an excellent rate (220.9 mAh g−1 at 2 A g−1) and cycling stability (over 2000 cycles). Note that the storage of B-N moieties on K + only occurs in a high potential region (>0.5 V), and this process is highly reversible.
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title_short	Regulating B-N moieties in carbon anode toward stable and fast potassium-storage
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author2	Li, Zihan Zhang, Di Sun, Huilan Li, Zhaojin Wang, Qiujun Sun, Qujiang Yuan, Fei Wang, Bo
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doi_str	10.1016/j.electacta.2024.143883
up_date	2024-07-06T20:10:54.275Z
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Regulating B-N moieties in carbon anode toward stable and fast potassium-storage

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