Mo 2 C regulated by cobalt components in N-doped carbon networks as pH-universal electrocatalyst for hydrogen evolution reaction
Developing non-noble and high-performance electrocatalysts that are suitable for a wide pH range is viable for hydrogen evolution reaction (HER), whereas it has a great challenge to design suitable catalyst to overcome the slow water dissociation kinetics. Herein, we report a novel and large-scale t...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Kang, Qiaoling [verfasserIn] Wang, Ru [verfasserIn] Lu, Yao [verfasserIn] Wang, Rui [verfasserIn] Yuan, Mingjian [verfasserIn] Gao, Feng [verfasserIn] Ma, Tingli [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2024 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: International journal of hydrogen energy - New York, NY [u.a.] : Elsevier, 1976, 57, Seite 1325-1331 |
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| Übergeordnetes Werk: |
volume:57 ; pages:1325-1331 |
| DOI / URN: |
10.1016/j.ijhydene.2024.01.109 |
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| Katalog-ID: |
ELV067143938 |
|---|
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| 520 | |a Developing non-noble and high-performance electrocatalysts that are suitable for a wide pH range is viable for hydrogen evolution reaction (HER), whereas it has a great challenge to design suitable catalyst to overcome the slow water dissociation kinetics. Herein, we report a novel and large-scale tactics using natural kelp as a precursor by utilizing the super high water-absorption capacity to construct Co/Mo2C nanoparticles dispersed in N-doped carbon matrix with lamellar-crossing networks (Co/Mo2CN-CKNs). Benefiting from synergistic advantages of Co-doped, Mo2C, as well as on the N-doped carbon, the Co/Mo2C@N-CKNs show superior HER performance in different pH condition with low overpotential of 63, 338 and 98mV at the current density of 10 mA·cm−2 in 0.5 M H2SO4, 0.1 M PBS and 1 M KOH respectively, and remaining stable even after 50 h of testing. This work may supply a common and hopeful strategy to realize non-noble and high-performance HER electrocatalysts with pH-universal work condition. | ||
| 650 | 4 | |a Molybdenum carbide | |
| 650 | 4 | |a pH-universal electrocatalyst | |
| 650 | 4 | |a Hydrogen evolution reaction | |
| 700 | 1 | |a Wang, Ru |e verfasserin |4 aut | |
| 700 | 1 | |a Lu, Yao |e verfasserin |4 aut | |
| 700 | 1 | |a Wang, Rui |e verfasserin |4 aut | |
| 700 | 1 | |a Yuan, Mingjian |e verfasserin |4 aut | |
| 700 | 1 | |a Gao, Feng |e verfasserin |4 aut | |
| 700 | 1 | |a Ma, Tingli |e verfasserin |4 aut | |
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10.1016/j.ijhydene.2024.01.109 doi (DE-627)ELV067143938 (ELSEVIER)S0360-3199(24)00112-5 DE-627 ger DE-627 rda eng 660 620 VZ 52.56 bkl Kang, Qiaoling verfasserin (orcid)0000-0001-7584-1582 aut Mo 2 C regulated by cobalt components in N-doped carbon networks as pH-universal electrocatalyst for hydrogen evolution reaction 2024 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Developing non-noble and high-performance electrocatalysts that are suitable for a wide pH range is viable for hydrogen evolution reaction (HER), whereas it has a great challenge to design suitable catalyst to overcome the slow water dissociation kinetics. Herein, we report a novel and large-scale tactics using natural kelp as a precursor by utilizing the super high water-absorption capacity to construct Co/Mo2C nanoparticles dispersed in N-doped carbon matrix with lamellar-crossing networks (Co/Mo2CN-CKNs). Benefiting from synergistic advantages of Co-doped, Mo2C, as well as on the N-doped carbon, the Co/Mo2C@N-CKNs show superior HER performance in different pH condition with low overpotential of 63, 338 and 98mV at the current density of 10 mA·cm−2 in 0.5 M H2SO4, 0.1 M PBS and 1 M KOH respectively, and remaining stable even after 50 h of testing. This work may supply a common and hopeful strategy to realize non-noble and high-performance HER electrocatalysts with pH-universal work condition. Molybdenum carbide pH-universal electrocatalyst Hydrogen evolution reaction Wang, Ru verfasserin aut Lu, Yao verfasserin aut Wang, Rui verfasserin aut Yuan, Mingjian verfasserin aut Gao, Feng verfasserin aut Ma, Tingli verfasserin aut Enthalten in International journal of hydrogen energy New York, NY [u.a.] : Elsevier, 1976 57, Seite 1325-1331 Online-Ressource (DE-627)301511357 (DE-600)1484487-4 (DE-576)096806397 1879-3487 nnns volume:57 pages:1325-1331 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.56 Regenerative Energieformen alternative Energieformen VZ AR 57 1325-1331 |
| spelling |
10.1016/j.ijhydene.2024.01.109 doi (DE-627)ELV067143938 (ELSEVIER)S0360-3199(24)00112-5 DE-627 ger DE-627 rda eng 660 620 VZ 52.56 bkl Kang, Qiaoling verfasserin (orcid)0000-0001-7584-1582 aut Mo 2 C regulated by cobalt components in N-doped carbon networks as pH-universal electrocatalyst for hydrogen evolution reaction 2024 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Developing non-noble and high-performance electrocatalysts that are suitable for a wide pH range is viable for hydrogen evolution reaction (HER), whereas it has a great challenge to design suitable catalyst to overcome the slow water dissociation kinetics. Herein, we report a novel and large-scale tactics using natural kelp as a precursor by utilizing the super high water-absorption capacity to construct Co/Mo2C nanoparticles dispersed in N-doped carbon matrix with lamellar-crossing networks (Co/Mo2CN-CKNs). Benefiting from synergistic advantages of Co-doped, Mo2C, as well as on the N-doped carbon, the Co/Mo2C@N-CKNs show superior HER performance in different pH condition with low overpotential of 63, 338 and 98mV at the current density of 10 mA·cm−2 in 0.5 M H2SO4, 0.1 M PBS and 1 M KOH respectively, and remaining stable even after 50 h of testing. This work may supply a common and hopeful strategy to realize non-noble and high-performance HER electrocatalysts with pH-universal work condition. Molybdenum carbide pH-universal electrocatalyst Hydrogen evolution reaction Wang, Ru verfasserin aut Lu, Yao verfasserin aut Wang, Rui verfasserin aut Yuan, Mingjian verfasserin aut Gao, Feng verfasserin aut Ma, Tingli verfasserin aut Enthalten in International journal of hydrogen energy New York, NY [u.a.] : Elsevier, 1976 57, Seite 1325-1331 Online-Ressource (DE-627)301511357 (DE-600)1484487-4 (DE-576)096806397 1879-3487 nnns volume:57 pages:1325-1331 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.56 Regenerative Energieformen alternative Energieformen VZ AR 57 1325-1331 |
| allfields_unstemmed |
10.1016/j.ijhydene.2024.01.109 doi (DE-627)ELV067143938 (ELSEVIER)S0360-3199(24)00112-5 DE-627 ger DE-627 rda eng 660 620 VZ 52.56 bkl Kang, Qiaoling verfasserin (orcid)0000-0001-7584-1582 aut Mo 2 C regulated by cobalt components in N-doped carbon networks as pH-universal electrocatalyst for hydrogen evolution reaction 2024 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Developing non-noble and high-performance electrocatalysts that are suitable for a wide pH range is viable for hydrogen evolution reaction (HER), whereas it has a great challenge to design suitable catalyst to overcome the slow water dissociation kinetics. Herein, we report a novel and large-scale tactics using natural kelp as a precursor by utilizing the super high water-absorption capacity to construct Co/Mo2C nanoparticles dispersed in N-doped carbon matrix with lamellar-crossing networks (Co/Mo2CN-CKNs). Benefiting from synergistic advantages of Co-doped, Mo2C, as well as on the N-doped carbon, the Co/Mo2C@N-CKNs show superior HER performance in different pH condition with low overpotential of 63, 338 and 98mV at the current density of 10 mA·cm−2 in 0.5 M H2SO4, 0.1 M PBS and 1 M KOH respectively, and remaining stable even after 50 h of testing. This work may supply a common and hopeful strategy to realize non-noble and high-performance HER electrocatalysts with pH-universal work condition. Molybdenum carbide pH-universal electrocatalyst Hydrogen evolution reaction Wang, Ru verfasserin aut Lu, Yao verfasserin aut Wang, Rui verfasserin aut Yuan, Mingjian verfasserin aut Gao, Feng verfasserin aut Ma, Tingli verfasserin aut Enthalten in International journal of hydrogen energy New York, NY [u.a.] : Elsevier, 1976 57, Seite 1325-1331 Online-Ressource (DE-627)301511357 (DE-600)1484487-4 (DE-576)096806397 1879-3487 nnns volume:57 pages:1325-1331 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.56 Regenerative Energieformen alternative Energieformen VZ AR 57 1325-1331 |
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10.1016/j.ijhydene.2024.01.109 doi (DE-627)ELV067143938 (ELSEVIER)S0360-3199(24)00112-5 DE-627 ger DE-627 rda eng 660 620 VZ 52.56 bkl Kang, Qiaoling verfasserin (orcid)0000-0001-7584-1582 aut Mo 2 C regulated by cobalt components in N-doped carbon networks as pH-universal electrocatalyst for hydrogen evolution reaction 2024 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Developing non-noble and high-performance electrocatalysts that are suitable for a wide pH range is viable for hydrogen evolution reaction (HER), whereas it has a great challenge to design suitable catalyst to overcome the slow water dissociation kinetics. Herein, we report a novel and large-scale tactics using natural kelp as a precursor by utilizing the super high water-absorption capacity to construct Co/Mo2C nanoparticles dispersed in N-doped carbon matrix with lamellar-crossing networks (Co/Mo2CN-CKNs). Benefiting from synergistic advantages of Co-doped, Mo2C, as well as on the N-doped carbon, the Co/Mo2C@N-CKNs show superior HER performance in different pH condition with low overpotential of 63, 338 and 98mV at the current density of 10 mA·cm−2 in 0.5 M H2SO4, 0.1 M PBS and 1 M KOH respectively, and remaining stable even after 50 h of testing. This work may supply a common and hopeful strategy to realize non-noble and high-performance HER electrocatalysts with pH-universal work condition. Molybdenum carbide pH-universal electrocatalyst Hydrogen evolution reaction Wang, Ru verfasserin aut Lu, Yao verfasserin aut Wang, Rui verfasserin aut Yuan, Mingjian verfasserin aut Gao, Feng verfasserin aut Ma, Tingli verfasserin aut Enthalten in International journal of hydrogen energy New York, NY [u.a.] : Elsevier, 1976 57, Seite 1325-1331 Online-Ressource (DE-627)301511357 (DE-600)1484487-4 (DE-576)096806397 1879-3487 nnns volume:57 pages:1325-1331 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 52.56 Regenerative Energieformen alternative Energieformen VZ AR 57 1325-1331 |
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Enthalten in International journal of hydrogen energy 57, Seite 1325-1331 volume:57 pages:1325-1331 |
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Molybdenum carbide pH-universal electrocatalyst Hydrogen evolution reaction |
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Kang, Qiaoling @@aut@@ Wang, Ru @@aut@@ Lu, Yao @@aut@@ Wang, Rui @@aut@@ Yuan, Mingjian @@aut@@ Gao, Feng @@aut@@ Ma, Tingli @@aut@@ |
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Kang, Qiaoling |
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Kang, Qiaoling ddc 660 bkl 52.56 misc Molybdenum carbide misc pH-universal electrocatalyst misc Hydrogen evolution reaction Mo 2 C regulated by cobalt components in N-doped carbon networks as pH-universal electrocatalyst for hydrogen evolution reaction |
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660 620 VZ 52.56 bkl Mo 2 C regulated by cobalt components in N-doped carbon networks as pH-universal electrocatalyst for hydrogen evolution reaction Molybdenum carbide pH-universal electrocatalyst Hydrogen evolution reaction |
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Mo 2 C regulated by cobalt components in N-doped carbon networks as pH-universal electrocatalyst for hydrogen evolution reaction |
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mo 2 c regulated by cobalt components in n-doped carbon networks as ph-universal electrocatalyst for hydrogen evolution reaction |
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Mo 2 C regulated by cobalt components in N-doped carbon networks as pH-universal electrocatalyst for hydrogen evolution reaction |
| abstract |
Developing non-noble and high-performance electrocatalysts that are suitable for a wide pH range is viable for hydrogen evolution reaction (HER), whereas it has a great challenge to design suitable catalyst to overcome the slow water dissociation kinetics. Herein, we report a novel and large-scale tactics using natural kelp as a precursor by utilizing the super high water-absorption capacity to construct Co/Mo2C nanoparticles dispersed in N-doped carbon matrix with lamellar-crossing networks (Co/Mo2CN-CKNs). Benefiting from synergistic advantages of Co-doped, Mo2C, as well as on the N-doped carbon, the Co/Mo2C@N-CKNs show superior HER performance in different pH condition with low overpotential of 63, 338 and 98mV at the current density of 10 mA·cm−2 in 0.5 M H2SO4, 0.1 M PBS and 1 M KOH respectively, and remaining stable even after 50 h of testing. This work may supply a common and hopeful strategy to realize non-noble and high-performance HER electrocatalysts with pH-universal work condition. |
| abstractGer |
Developing non-noble and high-performance electrocatalysts that are suitable for a wide pH range is viable for hydrogen evolution reaction (HER), whereas it has a great challenge to design suitable catalyst to overcome the slow water dissociation kinetics. Herein, we report a novel and large-scale tactics using natural kelp as a precursor by utilizing the super high water-absorption capacity to construct Co/Mo2C nanoparticles dispersed in N-doped carbon matrix with lamellar-crossing networks (Co/Mo2CN-CKNs). Benefiting from synergistic advantages of Co-doped, Mo2C, as well as on the N-doped carbon, the Co/Mo2C@N-CKNs show superior HER performance in different pH condition with low overpotential of 63, 338 and 98mV at the current density of 10 mA·cm−2 in 0.5 M H2SO4, 0.1 M PBS and 1 M KOH respectively, and remaining stable even after 50 h of testing. This work may supply a common and hopeful strategy to realize non-noble and high-performance HER electrocatalysts with pH-universal work condition. |
| abstract_unstemmed |
Developing non-noble and high-performance electrocatalysts that are suitable for a wide pH range is viable for hydrogen evolution reaction (HER), whereas it has a great challenge to design suitable catalyst to overcome the slow water dissociation kinetics. Herein, we report a novel and large-scale tactics using natural kelp as a precursor by utilizing the super high water-absorption capacity to construct Co/Mo2C nanoparticles dispersed in N-doped carbon matrix with lamellar-crossing networks (Co/Mo2CN-CKNs). Benefiting from synergistic advantages of Co-doped, Mo2C, as well as on the N-doped carbon, the Co/Mo2C@N-CKNs show superior HER performance in different pH condition with low overpotential of 63, 338 and 98mV at the current density of 10 mA·cm−2 in 0.5 M H2SO4, 0.1 M PBS and 1 M KOH respectively, and remaining stable even after 50 h of testing. This work may supply a common and hopeful strategy to realize non-noble and high-performance HER electrocatalysts with pH-universal work condition. |
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Mo 2 C regulated by cobalt components in N-doped carbon networks as pH-universal electrocatalyst for hydrogen evolution reaction |
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| score |
7.4005814 |