Partial oxidation of methane catalyzed by YBa2Cu3Ox in a solid state electrochemical reactor
Abstract The catalytic oxidation of methane was studied between 840 and 1110 K on a YBa2Cu3O* mixed-conducting electrode deposited on an yttria stabilized zirconia solid electrolyte. The lattice oxygen supplied electrochermically to the catalyst surface actively participated in the oxidation reactio...
Ausführliche Beschreibung
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
1994 |
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| Umfang: |
7 |
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| Reproduktion: |
Springer Online Journal Archives 1860-2002 |
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| Übergeordnetes Werk: |
in: Catalysis letters - 1988, 23(1994) vom: März/Apr., Seite 387-393 |
| Übergeordnetes Werk: |
volume:23 ; year:1994 ; month:03/04 ; pages:387-393 ; extent:7 |
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NLEJ196764645 |
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| 245 | 1 | 0 | |a Partial oxidation of methane catalyzed by YBa2Cu3Ox in a solid state electrochemical reactor |
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| 520 | |a Abstract The catalytic oxidation of methane was studied between 840 and 1110 K on a YBa2Cu3O* mixed-conducting electrode deposited on an yttria stabilized zirconia solid electrolyte. The lattice oxygen supplied electrochermically to the catalyst surface actively participated in the oxidation reaction, with CO as the major product, and CO2, CH3OH and HCHO as the minor products. The reaction rate was found to be of first order with respect to methane. The rate constant depended strongly on the electrochemically imposed bias. Under DC bias condition, the reaction rate was enhanced by as much as two orders of magnitude over that observed under open-circuit conditions. An Eley-Rideal mechanism for the interaction of CH4 with surface oxygen is proposed as the rate-determining step. | ||
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| 700 | 1 | |a Huggins, Robert A. |4 oth | |
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(DE-627)NLEJ196764645 DE-627 ger DE-627 rakwb eng Partial oxidation of methane catalyzed by YBa2Cu3Ox in a solid state electrochemical reactor 1994 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Abstract The catalytic oxidation of methane was studied between 840 and 1110 K on a YBa2Cu3O* mixed-conducting electrode deposited on an yttria stabilized zirconia solid electrolyte. The lattice oxygen supplied electrochermically to the catalyst surface actively participated in the oxidation reaction, with CO as the major product, and CO2, CH3OH and HCHO as the minor products. The reaction rate was found to be of first order with respect to methane. The rate constant depended strongly on the electrochemically imposed bias. Under DC bias condition, the reaction rate was enhanced by as much as two orders of magnitude over that observed under open-circuit conditions. An Eley-Rideal mechanism for the interaction of CH4 with surface oxygen is proposed as the rate-determining step. Springer Online Journal Archives 1860-2002 Gür, Turgut M. oth Wise, Henry oth Huggins, Robert A. oth in Catalysis letters 1988 23(1994) vom: März/Apr., Seite 387-393 (DE-627)NLEJ188994181 (DE-600)1501518-x 1572-879X nnns volume:23 year:1994 month:03/04 pages:387-393 extent:7 http://dx.doi.org/10.1007/BF00811373 GBV_USEFLAG_U ZDB-1-SOJ GBV_NL_ARTICLE AR 23 1994 3/4 387-393 7 |
| spelling |
(DE-627)NLEJ196764645 DE-627 ger DE-627 rakwb eng Partial oxidation of methane catalyzed by YBa2Cu3Ox in a solid state electrochemical reactor 1994 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Abstract The catalytic oxidation of methane was studied between 840 and 1110 K on a YBa2Cu3O* mixed-conducting electrode deposited on an yttria stabilized zirconia solid electrolyte. The lattice oxygen supplied electrochermically to the catalyst surface actively participated in the oxidation reaction, with CO as the major product, and CO2, CH3OH and HCHO as the minor products. The reaction rate was found to be of first order with respect to methane. The rate constant depended strongly on the electrochemically imposed bias. Under DC bias condition, the reaction rate was enhanced by as much as two orders of magnitude over that observed under open-circuit conditions. An Eley-Rideal mechanism for the interaction of CH4 with surface oxygen is proposed as the rate-determining step. Springer Online Journal Archives 1860-2002 Gür, Turgut M. oth Wise, Henry oth Huggins, Robert A. oth in Catalysis letters 1988 23(1994) vom: März/Apr., Seite 387-393 (DE-627)NLEJ188994181 (DE-600)1501518-x 1572-879X nnns volume:23 year:1994 month:03/04 pages:387-393 extent:7 http://dx.doi.org/10.1007/BF00811373 GBV_USEFLAG_U ZDB-1-SOJ GBV_NL_ARTICLE AR 23 1994 3/4 387-393 7 |
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(DE-627)NLEJ196764645 DE-627 ger DE-627 rakwb eng Partial oxidation of methane catalyzed by YBa2Cu3Ox in a solid state electrochemical reactor 1994 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Abstract The catalytic oxidation of methane was studied between 840 and 1110 K on a YBa2Cu3O* mixed-conducting electrode deposited on an yttria stabilized zirconia solid electrolyte. The lattice oxygen supplied electrochermically to the catalyst surface actively participated in the oxidation reaction, with CO as the major product, and CO2, CH3OH and HCHO as the minor products. The reaction rate was found to be of first order with respect to methane. The rate constant depended strongly on the electrochemically imposed bias. Under DC bias condition, the reaction rate was enhanced by as much as two orders of magnitude over that observed under open-circuit conditions. An Eley-Rideal mechanism for the interaction of CH4 with surface oxygen is proposed as the rate-determining step. Springer Online Journal Archives 1860-2002 Gür, Turgut M. oth Wise, Henry oth Huggins, Robert A. oth in Catalysis letters 1988 23(1994) vom: März/Apr., Seite 387-393 (DE-627)NLEJ188994181 (DE-600)1501518-x 1572-879X nnns volume:23 year:1994 month:03/04 pages:387-393 extent:7 http://dx.doi.org/10.1007/BF00811373 GBV_USEFLAG_U ZDB-1-SOJ GBV_NL_ARTICLE AR 23 1994 3/4 387-393 7 |
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(DE-627)NLEJ196764645 DE-627 ger DE-627 rakwb eng Partial oxidation of methane catalyzed by YBa2Cu3Ox in a solid state electrochemical reactor 1994 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Abstract The catalytic oxidation of methane was studied between 840 and 1110 K on a YBa2Cu3O* mixed-conducting electrode deposited on an yttria stabilized zirconia solid electrolyte. The lattice oxygen supplied electrochermically to the catalyst surface actively participated in the oxidation reaction, with CO as the major product, and CO2, CH3OH and HCHO as the minor products. The reaction rate was found to be of first order with respect to methane. The rate constant depended strongly on the electrochemically imposed bias. Under DC bias condition, the reaction rate was enhanced by as much as two orders of magnitude over that observed under open-circuit conditions. An Eley-Rideal mechanism for the interaction of CH4 with surface oxygen is proposed as the rate-determining step. Springer Online Journal Archives 1860-2002 Gür, Turgut M. oth Wise, Henry oth Huggins, Robert A. oth in Catalysis letters 1988 23(1994) vom: März/Apr., Seite 387-393 (DE-627)NLEJ188994181 (DE-600)1501518-x 1572-879X nnns volume:23 year:1994 month:03/04 pages:387-393 extent:7 http://dx.doi.org/10.1007/BF00811373 GBV_USEFLAG_U ZDB-1-SOJ GBV_NL_ARTICLE AR 23 1994 3/4 387-393 7 |
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(DE-627)NLEJ196764645 DE-627 ger DE-627 rakwb eng Partial oxidation of methane catalyzed by YBa2Cu3Ox in a solid state electrochemical reactor 1994 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Abstract The catalytic oxidation of methane was studied between 840 and 1110 K on a YBa2Cu3O* mixed-conducting electrode deposited on an yttria stabilized zirconia solid electrolyte. The lattice oxygen supplied electrochermically to the catalyst surface actively participated in the oxidation reaction, with CO as the major product, and CO2, CH3OH and HCHO as the minor products. The reaction rate was found to be of first order with respect to methane. The rate constant depended strongly on the electrochemically imposed bias. Under DC bias condition, the reaction rate was enhanced by as much as two orders of magnitude over that observed under open-circuit conditions. An Eley-Rideal mechanism for the interaction of CH4 with surface oxygen is proposed as the rate-determining step. Springer Online Journal Archives 1860-2002 Gür, Turgut M. oth Wise, Henry oth Huggins, Robert A. oth in Catalysis letters 1988 23(1994) vom: März/Apr., Seite 387-393 (DE-627)NLEJ188994181 (DE-600)1501518-x 1572-879X nnns volume:23 year:1994 month:03/04 pages:387-393 extent:7 http://dx.doi.org/10.1007/BF00811373 GBV_USEFLAG_U ZDB-1-SOJ GBV_NL_ARTICLE AR 23 1994 3/4 387-393 7 |
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partial oxidation of methane catalyzed by yba2cu3ox in a solid state electrochemical reactor |
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Partial oxidation of methane catalyzed by YBa2Cu3Ox in a solid state electrochemical reactor |
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Abstract The catalytic oxidation of methane was studied between 840 and 1110 K on a YBa2Cu3O* mixed-conducting electrode deposited on an yttria stabilized zirconia solid electrolyte. The lattice oxygen supplied electrochermically to the catalyst surface actively participated in the oxidation reaction, with CO as the major product, and CO2, CH3OH and HCHO as the minor products. The reaction rate was found to be of first order with respect to methane. The rate constant depended strongly on the electrochemically imposed bias. Under DC bias condition, the reaction rate was enhanced by as much as two orders of magnitude over that observed under open-circuit conditions. An Eley-Rideal mechanism for the interaction of CH4 with surface oxygen is proposed as the rate-determining step. |
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Abstract The catalytic oxidation of methane was studied between 840 and 1110 K on a YBa2Cu3O* mixed-conducting electrode deposited on an yttria stabilized zirconia solid electrolyte. The lattice oxygen supplied electrochermically to the catalyst surface actively participated in the oxidation reaction, with CO as the major product, and CO2, CH3OH and HCHO as the minor products. The reaction rate was found to be of first order with respect to methane. The rate constant depended strongly on the electrochemically imposed bias. Under DC bias condition, the reaction rate was enhanced by as much as two orders of magnitude over that observed under open-circuit conditions. An Eley-Rideal mechanism for the interaction of CH4 with surface oxygen is proposed as the rate-determining step. |
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Abstract The catalytic oxidation of methane was studied between 840 and 1110 K on a YBa2Cu3O* mixed-conducting electrode deposited on an yttria stabilized zirconia solid electrolyte. The lattice oxygen supplied electrochermically to the catalyst surface actively participated in the oxidation reaction, with CO as the major product, and CO2, CH3OH and HCHO as the minor products. The reaction rate was found to be of first order with respect to methane. The rate constant depended strongly on the electrochemically imposed bias. Under DC bias condition, the reaction rate was enhanced by as much as two orders of magnitude over that observed under open-circuit conditions. An Eley-Rideal mechanism for the interaction of CH4 with surface oxygen is proposed as the rate-determining step. |
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