Relaxation of the 4d→5p resonance in atomic iodine
Iodine atoms, produced by laser-induced dissociation of molecular iodine, have been photoexcited with synchrotron radiation in the region of the 4d-shell excitation. A strong resonance is observed below the 4d ionization threshold, which is assigned to the 4d→5p(2D5/2) transition. Photoelectron spec...
Ausführliche Beschreibung
Gespeichert in:
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E-Artikel |
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| Erschienen: |
1990 |
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Online-Ressource 10 |
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APS Digital Backfile Archive 1893-2003 |
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Enthalten in: Physical review / A - College Park, Md., 1970, 41(1990), 9, Seite 4879-4888 |
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volume:41 ; year:1990 ; number:9 ; pages:4879-4888 ; extent:10 |
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| 520 | |a Iodine atoms, produced by laser-induced dissociation of molecular iodine, have been photoexcited with synchrotron radiation in the region of the 4d-shell excitation. A strong resonance is observed below the 4d ionization threshold, which is assigned to the 4d→5p(2D5/2) transition. Photoelectron spectra reveal that the main decay of such an excited state is through direct autoionization into outer shells, especially into singlet states. Above the 5s-1 threshold, numerous lines are observed, which cannot be understood in a single-particle framework. Indeed, ab initio calculations point out that the 5s-1 configuration is strongly mixed with the 5p3(2P)5d and 5p3(2D)5d configurations, so that observed lines cannot be separated into main and satellite lines. Moreover, strong dynamic correlation effects are observed via a strong variation of the Auger decay rate with the kinetic energy of the Auger electron. | ||
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(DE-627)NLEJ248464906 (DE-601)aps:a2316130555d70f84e09984121271b7d8060a016 DE-627 ger DE-627 rakwb Relaxation of the 4d→5p resonance in atomic iodine 1990 Online-Ressource 10 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Iodine atoms, produced by laser-induced dissociation of molecular iodine, have been photoexcited with synchrotron radiation in the region of the 4d-shell excitation. A strong resonance is observed below the 4d ionization threshold, which is assigned to the 4d→5p(2D5/2) transition. Photoelectron spectra reveal that the main decay of such an excited state is through direct autoionization into outer shells, especially into singlet states. Above the 5s-1 threshold, numerous lines are observed, which cannot be understood in a single-particle framework. Indeed, ab initio calculations point out that the 5s-1 configuration is strongly mixed with the 5p3(2P)5d and 5p3(2D)5d configurations, so that observed lines cannot be separated into main and satellite lines. Moreover, strong dynamic correlation effects are observed via a strong variation of the Auger decay rate with the kinetic energy of the Auger electron. APS Digital Backfile Archive 1893-2003 Nahon, L. oth Duffy, L. oth Morin, P. oth Enthalten in Physical review / A College Park, Md., 1970 41(1990), 9, Seite 4879-4888 Online-Ressource (DE-627)NLEJ248237853 (DE-600)1472694-4 1094-1622 nnns volume:41 year:1990 number:9 pages:4879-4888 extent:10 https://www.tib.eu/de/suchen/id/aps%3Aa2316130555d70f84e09984121271b7d8060a016 Verlag Deutschlandweit zugänglich GBV_USEFLAG_U ZDB-1-APS GBV_NL_ARTICLE AR 41 1990 9 4879-4888 10 |
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(DE-627)NLEJ248464906 (DE-601)aps:a2316130555d70f84e09984121271b7d8060a016 DE-627 ger DE-627 rakwb Relaxation of the 4d→5p resonance in atomic iodine 1990 Online-Ressource 10 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Iodine atoms, produced by laser-induced dissociation of molecular iodine, have been photoexcited with synchrotron radiation in the region of the 4d-shell excitation. A strong resonance is observed below the 4d ionization threshold, which is assigned to the 4d→5p(2D5/2) transition. Photoelectron spectra reveal that the main decay of such an excited state is through direct autoionization into outer shells, especially into singlet states. Above the 5s-1 threshold, numerous lines are observed, which cannot be understood in a single-particle framework. Indeed, ab initio calculations point out that the 5s-1 configuration is strongly mixed with the 5p3(2P)5d and 5p3(2D)5d configurations, so that observed lines cannot be separated into main and satellite lines. Moreover, strong dynamic correlation effects are observed via a strong variation of the Auger decay rate with the kinetic energy of the Auger electron. APS Digital Backfile Archive 1893-2003 Nahon, L. oth Duffy, L. oth Morin, P. oth Enthalten in Physical review / A College Park, Md., 1970 41(1990), 9, Seite 4879-4888 Online-Ressource (DE-627)NLEJ248237853 (DE-600)1472694-4 1094-1622 nnns volume:41 year:1990 number:9 pages:4879-4888 extent:10 https://www.tib.eu/de/suchen/id/aps%3Aa2316130555d70f84e09984121271b7d8060a016 Verlag Deutschlandweit zugänglich GBV_USEFLAG_U ZDB-1-APS GBV_NL_ARTICLE AR 41 1990 9 4879-4888 10 |
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(DE-627)NLEJ248464906 (DE-601)aps:a2316130555d70f84e09984121271b7d8060a016 DE-627 ger DE-627 rakwb Relaxation of the 4d→5p resonance in atomic iodine 1990 Online-Ressource 10 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Iodine atoms, produced by laser-induced dissociation of molecular iodine, have been photoexcited with synchrotron radiation in the region of the 4d-shell excitation. A strong resonance is observed below the 4d ionization threshold, which is assigned to the 4d→5p(2D5/2) transition. Photoelectron spectra reveal that the main decay of such an excited state is through direct autoionization into outer shells, especially into singlet states. Above the 5s-1 threshold, numerous lines are observed, which cannot be understood in a single-particle framework. Indeed, ab initio calculations point out that the 5s-1 configuration is strongly mixed with the 5p3(2P)5d and 5p3(2D)5d configurations, so that observed lines cannot be separated into main and satellite lines. Moreover, strong dynamic correlation effects are observed via a strong variation of the Auger decay rate with the kinetic energy of the Auger electron. APS Digital Backfile Archive 1893-2003 Nahon, L. oth Duffy, L. oth Morin, P. oth Enthalten in Physical review / A College Park, Md., 1970 41(1990), 9, Seite 4879-4888 Online-Ressource (DE-627)NLEJ248237853 (DE-600)1472694-4 1094-1622 nnns volume:41 year:1990 number:9 pages:4879-4888 extent:10 https://www.tib.eu/de/suchen/id/aps%3Aa2316130555d70f84e09984121271b7d8060a016 Verlag Deutschlandweit zugänglich GBV_USEFLAG_U ZDB-1-APS GBV_NL_ARTICLE AR 41 1990 9 4879-4888 10 |
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(DE-627)NLEJ248464906 (DE-601)aps:a2316130555d70f84e09984121271b7d8060a016 DE-627 ger DE-627 rakwb Relaxation of the 4d→5p resonance in atomic iodine 1990 Online-Ressource 10 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Iodine atoms, produced by laser-induced dissociation of molecular iodine, have been photoexcited with synchrotron radiation in the region of the 4d-shell excitation. A strong resonance is observed below the 4d ionization threshold, which is assigned to the 4d→5p(2D5/2) transition. Photoelectron spectra reveal that the main decay of such an excited state is through direct autoionization into outer shells, especially into singlet states. Above the 5s-1 threshold, numerous lines are observed, which cannot be understood in a single-particle framework. Indeed, ab initio calculations point out that the 5s-1 configuration is strongly mixed with the 5p3(2P)5d and 5p3(2D)5d configurations, so that observed lines cannot be separated into main and satellite lines. Moreover, strong dynamic correlation effects are observed via a strong variation of the Auger decay rate with the kinetic energy of the Auger electron. APS Digital Backfile Archive 1893-2003 Nahon, L. oth Duffy, L. oth Morin, P. oth Enthalten in Physical review / A College Park, Md., 1970 41(1990), 9, Seite 4879-4888 Online-Ressource (DE-627)NLEJ248237853 (DE-600)1472694-4 1094-1622 nnns volume:41 year:1990 number:9 pages:4879-4888 extent:10 https://www.tib.eu/de/suchen/id/aps%3Aa2316130555d70f84e09984121271b7d8060a016 Verlag Deutschlandweit zugänglich GBV_USEFLAG_U ZDB-1-APS GBV_NL_ARTICLE AR 41 1990 9 4879-4888 10 |
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(DE-627)NLEJ248464906 (DE-601)aps:a2316130555d70f84e09984121271b7d8060a016 DE-627 ger DE-627 rakwb Relaxation of the 4d→5p resonance in atomic iodine 1990 Online-Ressource 10 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Iodine atoms, produced by laser-induced dissociation of molecular iodine, have been photoexcited with synchrotron radiation in the region of the 4d-shell excitation. A strong resonance is observed below the 4d ionization threshold, which is assigned to the 4d→5p(2D5/2) transition. Photoelectron spectra reveal that the main decay of such an excited state is through direct autoionization into outer shells, especially into singlet states. Above the 5s-1 threshold, numerous lines are observed, which cannot be understood in a single-particle framework. Indeed, ab initio calculations point out that the 5s-1 configuration is strongly mixed with the 5p3(2P)5d and 5p3(2D)5d configurations, so that observed lines cannot be separated into main and satellite lines. Moreover, strong dynamic correlation effects are observed via a strong variation of the Auger decay rate with the kinetic energy of the Auger electron. APS Digital Backfile Archive 1893-2003 Nahon, L. oth Duffy, L. oth Morin, P. oth Enthalten in Physical review / A College Park, Md., 1970 41(1990), 9, Seite 4879-4888 Online-Ressource (DE-627)NLEJ248237853 (DE-600)1472694-4 1094-1622 nnns volume:41 year:1990 number:9 pages:4879-4888 extent:10 https://www.tib.eu/de/suchen/id/aps%3Aa2316130555d70f84e09984121271b7d8060a016 Verlag Deutschlandweit zugänglich GBV_USEFLAG_U ZDB-1-APS GBV_NL_ARTICLE AR 41 1990 9 4879-4888 10 |
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relaxation of the 4d→5p resonance in atomic iodine |
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Relaxation of the 4d→5p resonance in atomic iodine |
| abstract |
Iodine atoms, produced by laser-induced dissociation of molecular iodine, have been photoexcited with synchrotron radiation in the region of the 4d-shell excitation. A strong resonance is observed below the 4d ionization threshold, which is assigned to the 4d→5p(2D5/2) transition. Photoelectron spectra reveal that the main decay of such an excited state is through direct autoionization into outer shells, especially into singlet states. Above the 5s-1 threshold, numerous lines are observed, which cannot be understood in a single-particle framework. Indeed, ab initio calculations point out that the 5s-1 configuration is strongly mixed with the 5p3(2P)5d and 5p3(2D)5d configurations, so that observed lines cannot be separated into main and satellite lines. Moreover, strong dynamic correlation effects are observed via a strong variation of the Auger decay rate with the kinetic energy of the Auger electron. |
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Iodine atoms, produced by laser-induced dissociation of molecular iodine, have been photoexcited with synchrotron radiation in the region of the 4d-shell excitation. A strong resonance is observed below the 4d ionization threshold, which is assigned to the 4d→5p(2D5/2) transition. Photoelectron spectra reveal that the main decay of such an excited state is through direct autoionization into outer shells, especially into singlet states. Above the 5s-1 threshold, numerous lines are observed, which cannot be understood in a single-particle framework. Indeed, ab initio calculations point out that the 5s-1 configuration is strongly mixed with the 5p3(2P)5d and 5p3(2D)5d configurations, so that observed lines cannot be separated into main and satellite lines. Moreover, strong dynamic correlation effects are observed via a strong variation of the Auger decay rate with the kinetic energy of the Auger electron. |
| abstract_unstemmed |
Iodine atoms, produced by laser-induced dissociation of molecular iodine, have been photoexcited with synchrotron radiation in the region of the 4d-shell excitation. A strong resonance is observed below the 4d ionization threshold, which is assigned to the 4d→5p(2D5/2) transition. Photoelectron spectra reveal that the main decay of such an excited state is through direct autoionization into outer shells, especially into singlet states. Above the 5s-1 threshold, numerous lines are observed, which cannot be understood in a single-particle framework. Indeed, ab initio calculations point out that the 5s-1 configuration is strongly mixed with the 5p3(2P)5d and 5p3(2D)5d configurations, so that observed lines cannot be separated into main and satellite lines. Moreover, strong dynamic correlation effects are observed via a strong variation of the Auger decay rate with the kinetic energy of the Auger electron. |
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<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000naa a22002652 4500</leader><controlfield tag="001">NLEJ248464906</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20231114095413.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">231114s1990 xx |||||o 00| ||und c</controlfield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)NLEJ248464906</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-601)aps:a2316130555d70f84e09984121271b7d8060a016</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rakwb</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Relaxation of the 4d→5p resonance in atomic iodine</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">1990</subfield></datafield><datafield tag="300" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield></datafield><datafield tag="300" ind1=" " ind2=" "><subfield code="a">10</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">Text</subfield><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Iodine atoms, produced by laser-induced dissociation of molecular iodine, have been photoexcited with synchrotron radiation in the region of the 4d-shell excitation. A strong resonance is observed below the 4d ionization threshold, which is assigned to the 4d→5p(2D5/2) transition. Photoelectron spectra reveal that the main decay of such an excited state is through direct autoionization into outer shells, especially into singlet states. Above the 5s-1 threshold, numerous lines are observed, which cannot be understood in a single-particle framework. Indeed, ab initio calculations point out that the 5s-1 configuration is strongly mixed with the 5p3(2P)5d and 5p3(2D)5d configurations, so that observed lines cannot be separated into main and satellite lines. Moreover, strong dynamic correlation effects are observed via a strong variation of the Auger decay rate with the kinetic energy of the Auger electron.</subfield></datafield><datafield tag="533" ind1=" " ind2=" "><subfield code="f">APS Digital Backfile Archive 1893-2003</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Nahon, L.</subfield><subfield code="4">oth</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Duffy, L.</subfield><subfield code="4">oth</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Morin, P.</subfield><subfield code="4">oth</subfield></datafield><datafield tag="773" ind1="0" ind2="8"><subfield code="i">Enthalten in</subfield><subfield code="t">Physical review / A</subfield><subfield code="d">College Park, Md., 1970</subfield><subfield code="g">41(1990), 9, Seite 4879-4888</subfield><subfield code="h">Online-Ressource</subfield><subfield code="w">(DE-627)NLEJ248237853</subfield><subfield code="w">(DE-600)1472694-4</subfield><subfield code="x">1094-1622</subfield><subfield code="7">nnns</subfield></datafield><datafield tag="773" ind1="1" ind2="8"><subfield code="g">volume:41</subfield><subfield code="g">year:1990</subfield><subfield code="g">number:9</subfield><subfield code="g">pages:4879-4888</subfield><subfield code="g">extent:10</subfield></datafield><datafield tag="856" ind1="4" ind2="0"><subfield code="u">https://www.tib.eu/de/suchen/id/aps%3Aa2316130555d70f84e09984121271b7d8060a016</subfield><subfield code="x">Verlag</subfield><subfield code="z">Deutschlandweit zugänglich</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_USEFLAG_U</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">ZDB-1-APS</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_NL_ARTICLE</subfield></datafield><datafield tag="951" ind1=" " ind2=" "><subfield code="a">AR</subfield></datafield><datafield tag="952" ind1=" " ind2=" "><subfield code="d">41</subfield><subfield code="j">1990</subfield><subfield code="e">9</subfield><subfield code="h">4879-4888</subfield><subfield code="g">10</subfield></datafield></record></collection>
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