Configurational Model of Metal Ion Complex Formation in Water Solutions
A configurational model for the quantum statistical description of the process of metal ion complex formation in water solution is proposed. Special attention is paid to the formation of hydroxocomplexes. In the framework of the model determination of such chemical characteristics of reaction as Bje...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Stasyuk, I. V. [verfasserIn] Velychko, O. V. [verfasserIn] |
|---|
| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2011 |
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| Übergeordnetes Werk: |
Enthalten in: Physics and chemistry of liquids - London [u.a.] : Taylor & Francis, 1968, 38(2000), 6 vom: 01. Nov., Seite 743-757 |
|---|---|
| Übergeordnetes Werk: |
number:6 ; volume:38 ; year:2000 ; month:11 ; day:01 ; pages:743-757 |
| Links: |
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| DOI / URN: |
10.1080/00319100008030320 |
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NLEJ252230000 |
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| 520 | |a A configurational model for the quantum statistical description of the process of metal ion complex formation in water solution is proposed. Special attention is paid to the formation of hydroxocomplexes. In the framework of the model determination of such chemical characteristics of reaction as Bjerrum function, partial mole fraction and formation constants is made. It is established that regions of existence of different complex forms at variation of solution pH reaction depend on differences of configuration energies and temperature. Existence of a saturation effect which leads to a sharp change of ligand concentration in solution when the metal ion concentration crosses a certain value is established. Dependence of this effect on temperature and other parameters of the system is investigated. | ||
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10.1080/00319100008030320 doi (DE-627)NLEJ252230000 (TFO)757034127 DE-627 ger DE-627 rda eng Stasyuk, I. V. verfasserin aut Configurational Model of Metal Ion Complex Formation in Water Solutions 2011 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A configurational model for the quantum statistical description of the process of metal ion complex formation in water solution is proposed. Special attention is paid to the formation of hydroxocomplexes. In the framework of the model determination of such chemical characteristics of reaction as Bjerrum function, partial mole fraction and formation constants is made. It is established that regions of existence of different complex forms at variation of solution pH reaction depend on differences of configuration energies and temperature. Existence of a saturation effect which leads to a sharp change of ligand concentration in solution when the metal ion concentration crosses a certain value is established. Dependence of this effect on temperature and other parameters of the system is investigated. Velychko, O. V. verfasserin aut Enthalten in Physics and chemistry of liquids London [u.a.] : Taylor & Francis, 1968 38(2000), 6 vom: 01. Nov., Seite 743-757 Online-Ressource (DE-627)NLEJ252219635 (DE-600)2022959-8 (DE-576)263253651 1029-0451 nnns number:6 volume:38 year:2000 month:11 day:01 pages:743-757 https://www.tib.eu/de/suchen/id/tandf%3A557ba005168689833886c1d6e1e6838dd529b7f3 Digitalisierung Deutschlandweit zugänglich ZDB-1-TFO GBV_NL_ARTICLE AR 6 38 2000 11 01 743-757 |
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10.1080/00319100008030320 doi (DE-627)NLEJ252230000 (TFO)757034127 DE-627 ger DE-627 rda eng Stasyuk, I. V. verfasserin aut Configurational Model of Metal Ion Complex Formation in Water Solutions 2011 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A configurational model for the quantum statistical description of the process of metal ion complex formation in water solution is proposed. Special attention is paid to the formation of hydroxocomplexes. In the framework of the model determination of such chemical characteristics of reaction as Bjerrum function, partial mole fraction and formation constants is made. It is established that regions of existence of different complex forms at variation of solution pH reaction depend on differences of configuration energies and temperature. Existence of a saturation effect which leads to a sharp change of ligand concentration in solution when the metal ion concentration crosses a certain value is established. Dependence of this effect on temperature and other parameters of the system is investigated. Velychko, O. V. verfasserin aut Enthalten in Physics and chemistry of liquids London [u.a.] : Taylor & Francis, 1968 38(2000), 6 vom: 01. Nov., Seite 743-757 Online-Ressource (DE-627)NLEJ252219635 (DE-600)2022959-8 (DE-576)263253651 1029-0451 nnns number:6 volume:38 year:2000 month:11 day:01 pages:743-757 https://www.tib.eu/de/suchen/id/tandf%3A557ba005168689833886c1d6e1e6838dd529b7f3 Digitalisierung Deutschlandweit zugänglich ZDB-1-TFO GBV_NL_ARTICLE AR 6 38 2000 11 01 743-757 |
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10.1080/00319100008030320 doi (DE-627)NLEJ252230000 (TFO)757034127 DE-627 ger DE-627 rda eng Stasyuk, I. V. verfasserin aut Configurational Model of Metal Ion Complex Formation in Water Solutions 2011 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A configurational model for the quantum statistical description of the process of metal ion complex formation in water solution is proposed. Special attention is paid to the formation of hydroxocomplexes. In the framework of the model determination of such chemical characteristics of reaction as Bjerrum function, partial mole fraction and formation constants is made. It is established that regions of existence of different complex forms at variation of solution pH reaction depend on differences of configuration energies and temperature. Existence of a saturation effect which leads to a sharp change of ligand concentration in solution when the metal ion concentration crosses a certain value is established. Dependence of this effect on temperature and other parameters of the system is investigated. Velychko, O. V. verfasserin aut Enthalten in Physics and chemistry of liquids London [u.a.] : Taylor & Francis, 1968 38(2000), 6 vom: 01. Nov., Seite 743-757 Online-Ressource (DE-627)NLEJ252219635 (DE-600)2022959-8 (DE-576)263253651 1029-0451 nnns number:6 volume:38 year:2000 month:11 day:01 pages:743-757 https://www.tib.eu/de/suchen/id/tandf%3A557ba005168689833886c1d6e1e6838dd529b7f3 Digitalisierung Deutschlandweit zugänglich ZDB-1-TFO GBV_NL_ARTICLE AR 6 38 2000 11 01 743-757 |
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Configurational Model of Metal Ion Complex Formation in Water Solutions |
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A configurational model for the quantum statistical description of the process of metal ion complex formation in water solution is proposed. Special attention is paid to the formation of hydroxocomplexes. In the framework of the model determination of such chemical characteristics of reaction as Bjerrum function, partial mole fraction and formation constants is made. It is established that regions of existence of different complex forms at variation of solution pH reaction depend on differences of configuration energies and temperature. Existence of a saturation effect which leads to a sharp change of ligand concentration in solution when the metal ion concentration crosses a certain value is established. Dependence of this effect on temperature and other parameters of the system is investigated. |
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A configurational model for the quantum statistical description of the process of metal ion complex formation in water solution is proposed. Special attention is paid to the formation of hydroxocomplexes. In the framework of the model determination of such chemical characteristics of reaction as Bjerrum function, partial mole fraction and formation constants is made. It is established that regions of existence of different complex forms at variation of solution pH reaction depend on differences of configuration energies and temperature. Existence of a saturation effect which leads to a sharp change of ligand concentration in solution when the metal ion concentration crosses a certain value is established. Dependence of this effect on temperature and other parameters of the system is investigated. |
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A configurational model for the quantum statistical description of the process of metal ion complex formation in water solution is proposed. Special attention is paid to the formation of hydroxocomplexes. In the framework of the model determination of such chemical characteristics of reaction as Bjerrum function, partial mole fraction and formation constants is made. It is established that regions of existence of different complex forms at variation of solution pH reaction depend on differences of configuration energies and temperature. Existence of a saturation effect which leads to a sharp change of ligand concentration in solution when the metal ion concentration crosses a certain value is established. Dependence of this effect on temperature and other parameters of the system is investigated. |
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