Transboundary transport and deposition of Hg emission from springtime biomass burning in the Indo‐China Peninsula

Biomass burning from the Indo‐China Peninsula region is an important source of atmospheric mercury (Hg). We isolated 18 unique transport events over 2 years using observations of Hg and CO at a high‐altitude background site in southwestern China (Mount Ailao Observatory Station) to assess the transp...
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Autor*in:	Wang, Xun [verfasserIn] Zhang, Hui Lin, Che‐Jen Fu, Xuewu Zhang, Yiping Feng, Xinbin

Format:	Artikel
Sprache:	Englisch

Erschienen:	2015

Rechteinformationen:	Nutzungsrecht: © 2015. American Geophysical Union. All Rights Reserved.

Schlagwörter:	transport mercury biomass burning Emissions Mercury Biomass Atmospheric chemistry

Übergeordnetes Werk:	Enthalten in: Journal of geophysical research / D - Washington, DC : Union, 1984, 120(2015), 18, Seite 9758-9771
Übergeordnetes Werk:	volume:120 ; year:2015 ; number:18 ; pages:9758-9771

Links:	Volltext Link aufrufen Link aufrufen

DOI / URN:	10.1002/2015JD023525

Katalog-ID:	OLC1957059494

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520			\|a Biomass burning from the Indo‐China Peninsula region is an important source of atmospheric mercury (Hg). We isolated 18 unique transport events over 2 years using observations of Hg and CO at a high‐altitude background site in southwestern China (Mount Ailao Observatory Station) to assess the transport and impact of Hg emissions from biomass burning. The quantity of Hg emission and the source regions were determined using ΔTGM/ΔCO slopes coupled with backward trajectory analysis and CO emission inventories. The slopes of ΔTGM/ΔCO appeared to be a useful chemical indicator for source identification. Industrial emission sources exhibited slopes in the range of 5.1–61.0 × 10 −7 (parts per trillion by volume, pptv/pptv), in contrast to a slope of 2.0–6.0 × 10 −7 for typical biomass burning. Transboundary transport of Hg from biomass burning led to episodically elevated atmospheric Hg concentrations during springtime. Hg emissions from biomass burning in the Indo‐China Peninsula region from 2001 to 2008 were estimated to be 11.4 ± 2.1 Mg yr −1 , equivalent to 40% of annual anthropogenic emissions in the region. In addition, Hg emissions from biomass burning contained a substantial fraction of particulate bound Hg (PBM). Assuming that PBM readily deposits locally (within 50 km), the local Hg deposition caused by the PBM was estimated to be 2.2 ± 0.4 Mg yr −1 , up to 1 order of magnitude higher than the PBM deposition caused by anthropogenic emissions during springtime in the region. The strong springtime emissions potentially pose a threat to the ecosystems of the Indo‐China Peninsula and southwest China. ΔTGM/ΔCO slope can be an indicator for source identification ΔTGM/ΔCO slope for biomass burning is about of 2.0 × 10−7 Hg emission from biomass burning was estimated
540			\|a Nutzungsrecht: © 2015. American Geophysical Union. All Rights Reserved.
650		4	\|a transport
650		4	\|a mercury
650		4	\|a biomass burning
650		4	\|a Emissions
650		4	\|a Mercury
650		4	\|a Biomass
650		4	\|a Atmospheric chemistry
700	1		\|a Zhang, Hui \|4 oth
700	1		\|a Lin, Che‐Jen \|4 oth
700	1		\|a Fu, Xuewu \|4 oth
700	1		\|a Zhang, Yiping \|4 oth
700	1		\|a Feng, Xinbin \|4 oth
773	0	8	\|i Enthalten in \|t Journal of geophysical research / D \|d Washington, DC : Union, 1984 \|g 120(2015), 18, Seite 9758-9771 \|w (DE-627)130444391 \|w (DE-600)710256-2 \|w (DE-576)015978818 \|x 2169-897X \|7 nnns
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856	4	1	\|u http://dx.doi.org/10.1002/2015JD023525 \|3 Volltext
856	4	2	\|u http://onlinelibrary.wiley.com/doi/10.1002/2015JD023525/abstract
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allfields	10.1002/2015JD023525 doi PQ20160617 (DE-627)OLC1957059494 (DE-599)GBVOLC1957059494 (PRQ)p1847-8ef8ea2ff55840fe96d163fe7a45f2995f835141c6591168ab6d68f9193c94000 (KEY)0137985220150000120001809758transboundarytransportanddepositionofhgemissionfro DE-627 ger DE-627 rakwb eng 550 DNB Wang, Xun verfasserin aut Transboundary transport and deposition of Hg emission from springtime biomass burning in the Indo‐China Peninsula 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier Biomass burning from the Indo‐China Peninsula region is an important source of atmospheric mercury (Hg). We isolated 18 unique transport events over 2 years using observations of Hg and CO at a high‐altitude background site in southwestern China (Mount Ailao Observatory Station) to assess the transport and impact of Hg emissions from biomass burning. The quantity of Hg emission and the source regions were determined using ΔTGM/ΔCO slopes coupled with backward trajectory analysis and CO emission inventories. The slopes of ΔTGM/ΔCO appeared to be a useful chemical indicator for source identification. Industrial emission sources exhibited slopes in the range of 5.1–61.0 × 10 −7 (parts per trillion by volume, pptv/pptv), in contrast to a slope of 2.0–6.0 × 10 −7 for typical biomass burning. Transboundary transport of Hg from biomass burning led to episodically elevated atmospheric Hg concentrations during springtime. Hg emissions from biomass burning in the Indo‐China Peninsula region from 2001 to 2008 were estimated to be 11.4 ± 2.1 Mg yr −1 , equivalent to 40% of annual anthropogenic emissions in the region. In addition, Hg emissions from biomass burning contained a substantial fraction of particulate bound Hg (PBM). Assuming that PBM readily deposits locally (within 50 km), the local Hg deposition caused by the PBM was estimated to be 2.2 ± 0.4 Mg yr −1 , up to 1 order of magnitude higher than the PBM deposition caused by anthropogenic emissions during springtime in the region. The strong springtime emissions potentially pose a threat to the ecosystems of the Indo‐China Peninsula and southwest China. ΔTGM/ΔCO slope can be an indicator for source identification ΔTGM/ΔCO slope for biomass burning is about of 2.0 × 10−7 Hg emission from biomass burning was estimated Nutzungsrecht: © 2015. American Geophysical Union. All Rights Reserved. transport mercury biomass burning Emissions Mercury Biomass Atmospheric chemistry Zhang, Hui oth Lin, Che‐Jen oth Fu, Xuewu oth Zhang, Yiping oth Feng, Xinbin oth Enthalten in Journal of geophysical research / D Washington, DC : Union, 1984 120(2015), 18, Seite 9758-9771 (DE-627)130444391 (DE-600)710256-2 (DE-576)015978818 2169-897X nnns volume:120 year:2015 number:18 pages:9758-9771 http://dx.doi.org/10.1002/2015JD023525 Volltext http://onlinelibrary.wiley.com/doi/10.1002/2015JD023525/abstract http://search.proquest.com/docview/1724667783 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY SSG-OLC-GEO SSG-OLC-PHA SSG-OLC-DE-84 SSG-OPC-GGO SSG-OPC-GEO GBV_ILN_62 GBV_ILN_154 AR 120 2015 18 9758-9771
spelling	10.1002/2015JD023525 doi PQ20160617 (DE-627)OLC1957059494 (DE-599)GBVOLC1957059494 (PRQ)p1847-8ef8ea2ff55840fe96d163fe7a45f2995f835141c6591168ab6d68f9193c94000 (KEY)0137985220150000120001809758transboundarytransportanddepositionofhgemissionfro DE-627 ger DE-627 rakwb eng 550 DNB Wang, Xun verfasserin aut Transboundary transport and deposition of Hg emission from springtime biomass burning in the Indo‐China Peninsula 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier Biomass burning from the Indo‐China Peninsula region is an important source of atmospheric mercury (Hg). We isolated 18 unique transport events over 2 years using observations of Hg and CO at a high‐altitude background site in southwestern China (Mount Ailao Observatory Station) to assess the transport and impact of Hg emissions from biomass burning. The quantity of Hg emission and the source regions were determined using ΔTGM/ΔCO slopes coupled with backward trajectory analysis and CO emission inventories. The slopes of ΔTGM/ΔCO appeared to be a useful chemical indicator for source identification. Industrial emission sources exhibited slopes in the range of 5.1–61.0 × 10 −7 (parts per trillion by volume, pptv/pptv), in contrast to a slope of 2.0–6.0 × 10 −7 for typical biomass burning. Transboundary transport of Hg from biomass burning led to episodically elevated atmospheric Hg concentrations during springtime. Hg emissions from biomass burning in the Indo‐China Peninsula region from 2001 to 2008 were estimated to be 11.4 ± 2.1 Mg yr −1 , equivalent to 40% of annual anthropogenic emissions in the region. In addition, Hg emissions from biomass burning contained a substantial fraction of particulate bound Hg (PBM). Assuming that PBM readily deposits locally (within 50 km), the local Hg deposition caused by the PBM was estimated to be 2.2 ± 0.4 Mg yr −1 , up to 1 order of magnitude higher than the PBM deposition caused by anthropogenic emissions during springtime in the region. The strong springtime emissions potentially pose a threat to the ecosystems of the Indo‐China Peninsula and southwest China. ΔTGM/ΔCO slope can be an indicator for source identification ΔTGM/ΔCO slope for biomass burning is about of 2.0 × 10−7 Hg emission from biomass burning was estimated Nutzungsrecht: © 2015. American Geophysical Union. All Rights Reserved. transport mercury biomass burning Emissions Mercury Biomass Atmospheric chemistry Zhang, Hui oth Lin, Che‐Jen oth Fu, Xuewu oth Zhang, Yiping oth Feng, Xinbin oth Enthalten in Journal of geophysical research / D Washington, DC : Union, 1984 120(2015), 18, Seite 9758-9771 (DE-627)130444391 (DE-600)710256-2 (DE-576)015978818 2169-897X nnns volume:120 year:2015 number:18 pages:9758-9771 http://dx.doi.org/10.1002/2015JD023525 Volltext http://onlinelibrary.wiley.com/doi/10.1002/2015JD023525/abstract http://search.proquest.com/docview/1724667783 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY SSG-OLC-GEO SSG-OLC-PHA SSG-OLC-DE-84 SSG-OPC-GGO SSG-OPC-GEO GBV_ILN_62 GBV_ILN_154 AR 120 2015 18 9758-9771
allfields_unstemmed	10.1002/2015JD023525 doi PQ20160617 (DE-627)OLC1957059494 (DE-599)GBVOLC1957059494 (PRQ)p1847-8ef8ea2ff55840fe96d163fe7a45f2995f835141c6591168ab6d68f9193c94000 (KEY)0137985220150000120001809758transboundarytransportanddepositionofhgemissionfro DE-627 ger DE-627 rakwb eng 550 DNB Wang, Xun verfasserin aut Transboundary transport and deposition of Hg emission from springtime biomass burning in the Indo‐China Peninsula 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier Biomass burning from the Indo‐China Peninsula region is an important source of atmospheric mercury (Hg). We isolated 18 unique transport events over 2 years using observations of Hg and CO at a high‐altitude background site in southwestern China (Mount Ailao Observatory Station) to assess the transport and impact of Hg emissions from biomass burning. The quantity of Hg emission and the source regions were determined using ΔTGM/ΔCO slopes coupled with backward trajectory analysis and CO emission inventories. The slopes of ΔTGM/ΔCO appeared to be a useful chemical indicator for source identification. Industrial emission sources exhibited slopes in the range of 5.1–61.0 × 10 −7 (parts per trillion by volume, pptv/pptv), in contrast to a slope of 2.0–6.0 × 10 −7 for typical biomass burning. Transboundary transport of Hg from biomass burning led to episodically elevated atmospheric Hg concentrations during springtime. Hg emissions from biomass burning in the Indo‐China Peninsula region from 2001 to 2008 were estimated to be 11.4 ± 2.1 Mg yr −1 , equivalent to 40% of annual anthropogenic emissions in the region. In addition, Hg emissions from biomass burning contained a substantial fraction of particulate bound Hg (PBM). Assuming that PBM readily deposits locally (within 50 km), the local Hg deposition caused by the PBM was estimated to be 2.2 ± 0.4 Mg yr −1 , up to 1 order of magnitude higher than the PBM deposition caused by anthropogenic emissions during springtime in the region. The strong springtime emissions potentially pose a threat to the ecosystems of the Indo‐China Peninsula and southwest China. ΔTGM/ΔCO slope can be an indicator for source identification ΔTGM/ΔCO slope for biomass burning is about of 2.0 × 10−7 Hg emission from biomass burning was estimated Nutzungsrecht: © 2015. American Geophysical Union. All Rights Reserved. transport mercury biomass burning Emissions Mercury Biomass Atmospheric chemistry Zhang, Hui oth Lin, Che‐Jen oth Fu, Xuewu oth Zhang, Yiping oth Feng, Xinbin oth Enthalten in Journal of geophysical research / D Washington, DC : Union, 1984 120(2015), 18, Seite 9758-9771 (DE-627)130444391 (DE-600)710256-2 (DE-576)015978818 2169-897X nnns volume:120 year:2015 number:18 pages:9758-9771 http://dx.doi.org/10.1002/2015JD023525 Volltext http://onlinelibrary.wiley.com/doi/10.1002/2015JD023525/abstract http://search.proquest.com/docview/1724667783 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY SSG-OLC-GEO SSG-OLC-PHA SSG-OLC-DE-84 SSG-OPC-GGO SSG-OPC-GEO GBV_ILN_62 GBV_ILN_154 AR 120 2015 18 9758-9771
allfieldsGer	10.1002/2015JD023525 doi PQ20160617 (DE-627)OLC1957059494 (DE-599)GBVOLC1957059494 (PRQ)p1847-8ef8ea2ff55840fe96d163fe7a45f2995f835141c6591168ab6d68f9193c94000 (KEY)0137985220150000120001809758transboundarytransportanddepositionofhgemissionfro DE-627 ger DE-627 rakwb eng 550 DNB Wang, Xun verfasserin aut Transboundary transport and deposition of Hg emission from springtime biomass burning in the Indo‐China Peninsula 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier Biomass burning from the Indo‐China Peninsula region is an important source of atmospheric mercury (Hg). We isolated 18 unique transport events over 2 years using observations of Hg and CO at a high‐altitude background site in southwestern China (Mount Ailao Observatory Station) to assess the transport and impact of Hg emissions from biomass burning. The quantity of Hg emission and the source regions were determined using ΔTGM/ΔCO slopes coupled with backward trajectory analysis and CO emission inventories. The slopes of ΔTGM/ΔCO appeared to be a useful chemical indicator for source identification. Industrial emission sources exhibited slopes in the range of 5.1–61.0 × 10 −7 (parts per trillion by volume, pptv/pptv), in contrast to a slope of 2.0–6.0 × 10 −7 for typical biomass burning. Transboundary transport of Hg from biomass burning led to episodically elevated atmospheric Hg concentrations during springtime. Hg emissions from biomass burning in the Indo‐China Peninsula region from 2001 to 2008 were estimated to be 11.4 ± 2.1 Mg yr −1 , equivalent to 40% of annual anthropogenic emissions in the region. In addition, Hg emissions from biomass burning contained a substantial fraction of particulate bound Hg (PBM). Assuming that PBM readily deposits locally (within 50 km), the local Hg deposition caused by the PBM was estimated to be 2.2 ± 0.4 Mg yr −1 , up to 1 order of magnitude higher than the PBM deposition caused by anthropogenic emissions during springtime in the region. The strong springtime emissions potentially pose a threat to the ecosystems of the Indo‐China Peninsula and southwest China. ΔTGM/ΔCO slope can be an indicator for source identification ΔTGM/ΔCO slope for biomass burning is about of 2.0 × 10−7 Hg emission from biomass burning was estimated Nutzungsrecht: © 2015. American Geophysical Union. All Rights Reserved. transport mercury biomass burning Emissions Mercury Biomass Atmospheric chemistry Zhang, Hui oth Lin, Che‐Jen oth Fu, Xuewu oth Zhang, Yiping oth Feng, Xinbin oth Enthalten in Journal of geophysical research / D Washington, DC : Union, 1984 120(2015), 18, Seite 9758-9771 (DE-627)130444391 (DE-600)710256-2 (DE-576)015978818 2169-897X nnns volume:120 year:2015 number:18 pages:9758-9771 http://dx.doi.org/10.1002/2015JD023525 Volltext http://onlinelibrary.wiley.com/doi/10.1002/2015JD023525/abstract http://search.proquest.com/docview/1724667783 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY SSG-OLC-GEO SSG-OLC-PHA SSG-OLC-DE-84 SSG-OPC-GGO SSG-OPC-GEO GBV_ILN_62 GBV_ILN_154 AR 120 2015 18 9758-9771
allfieldsSound	10.1002/2015JD023525 doi PQ20160617 (DE-627)OLC1957059494 (DE-599)GBVOLC1957059494 (PRQ)p1847-8ef8ea2ff55840fe96d163fe7a45f2995f835141c6591168ab6d68f9193c94000 (KEY)0137985220150000120001809758transboundarytransportanddepositionofhgemissionfro DE-627 ger DE-627 rakwb eng 550 DNB Wang, Xun verfasserin aut Transboundary transport and deposition of Hg emission from springtime biomass burning in the Indo‐China Peninsula 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier Biomass burning from the Indo‐China Peninsula region is an important source of atmospheric mercury (Hg). We isolated 18 unique transport events over 2 years using observations of Hg and CO at a high‐altitude background site in southwestern China (Mount Ailao Observatory Station) to assess the transport and impact of Hg emissions from biomass burning. The quantity of Hg emission and the source regions were determined using ΔTGM/ΔCO slopes coupled with backward trajectory analysis and CO emission inventories. The slopes of ΔTGM/ΔCO appeared to be a useful chemical indicator for source identification. Industrial emission sources exhibited slopes in the range of 5.1–61.0 × 10 −7 (parts per trillion by volume, pptv/pptv), in contrast to a slope of 2.0–6.0 × 10 −7 for typical biomass burning. Transboundary transport of Hg from biomass burning led to episodically elevated atmospheric Hg concentrations during springtime. Hg emissions from biomass burning in the Indo‐China Peninsula region from 2001 to 2008 were estimated to be 11.4 ± 2.1 Mg yr −1 , equivalent to 40% of annual anthropogenic emissions in the region. In addition, Hg emissions from biomass burning contained a substantial fraction of particulate bound Hg (PBM). Assuming that PBM readily deposits locally (within 50 km), the local Hg deposition caused by the PBM was estimated to be 2.2 ± 0.4 Mg yr −1 , up to 1 order of magnitude higher than the PBM deposition caused by anthropogenic emissions during springtime in the region. The strong springtime emissions potentially pose a threat to the ecosystems of the Indo‐China Peninsula and southwest China. ΔTGM/ΔCO slope can be an indicator for source identification ΔTGM/ΔCO slope for biomass burning is about of 2.0 × 10−7 Hg emission from biomass burning was estimated Nutzungsrecht: © 2015. American Geophysical Union. All Rights Reserved. transport mercury biomass burning Emissions Mercury Biomass Atmospheric chemistry Zhang, Hui oth Lin, Che‐Jen oth Fu, Xuewu oth Zhang, Yiping oth Feng, Xinbin oth Enthalten in Journal of geophysical research / D Washington, DC : Union, 1984 120(2015), 18, Seite 9758-9771 (DE-627)130444391 (DE-600)710256-2 (DE-576)015978818 2169-897X nnns volume:120 year:2015 number:18 pages:9758-9771 http://dx.doi.org/10.1002/2015JD023525 Volltext http://onlinelibrary.wiley.com/doi/10.1002/2015JD023525/abstract http://search.proquest.com/docview/1724667783 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY SSG-OLC-GEO SSG-OLC-PHA SSG-OLC-DE-84 SSG-OPC-GGO SSG-OPC-GEO GBV_ILN_62 GBV_ILN_154 AR 120 2015 18 9758-9771
language	English
source	Enthalten in Journal of geophysical research / D 120(2015), 18, Seite 9758-9771 volume:120 year:2015 number:18 pages:9758-9771
sourceStr	Enthalten in Journal of geophysical research / D 120(2015), 18, Seite 9758-9771 volume:120 year:2015 number:18 pages:9758-9771
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	transport mercury biomass burning Emissions Mercury Biomass Atmospheric chemistry
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container_title	Journal of geophysical research / D
authorswithroles_txt_mv	Wang, Xun @@aut@@ Zhang, Hui @@oth@@ Lin, Che‐Jen @@oth@@ Fu, Xuewu @@oth@@ Zhang, Yiping @@oth@@ Feng, Xinbin @@oth@@
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We isolated 18 unique transport events over 2 years using observations of Hg and CO at a high‐altitude background site in southwestern China (Mount Ailao Observatory Station) to assess the transport and impact of Hg emissions from biomass burning. The quantity of Hg emission and the source regions were determined using ΔTGM/ΔCO slopes coupled with backward trajectory analysis and CO emission inventories. The slopes of ΔTGM/ΔCO appeared to be a useful chemical indicator for source identification. Industrial emission sources exhibited slopes in the range of 5.1–61.0 × 10 −7 (parts per trillion by volume, pptv/pptv), in contrast to a slope of 2.0–6.0 × 10 −7 for typical biomass burning. Transboundary transport of Hg from biomass burning led to episodically elevated atmospheric Hg concentrations during springtime. Hg emissions from biomass burning in the Indo‐China Peninsula region from 2001 to 2008 were estimated to be 11.4 ± 2.1 Mg yr −1 , equivalent to 40% of annual anthropogenic emissions in the region. In addition, Hg emissions from biomass burning contained a substantial fraction of particulate bound Hg (PBM). Assuming that PBM readily deposits locally (within 50 km), the local Hg deposition caused by the PBM was estimated to be 2.2 ± 0.4 Mg yr −1 , up to 1 order of magnitude higher than the PBM deposition caused by anthropogenic emissions during springtime in the region. The strong springtime emissions potentially pose a threat to the ecosystems of the Indo‐China Peninsula and southwest China. ΔTGM/ΔCO slope can be an indicator for source identification ΔTGM/ΔCO slope for biomass burning is about of 2.0 × 10−7 Hg emission from biomass burning was estimated</subfield></datafield><datafield tag="540" ind1=" " ind2=" "><subfield code="a">Nutzungsrecht: © 2015. American Geophysical Union. 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author	Wang, Xun
spellingShingle	Wang, Xun ddc 550 misc transport misc mercury misc biomass burning misc Emissions misc Mercury misc Biomass misc Atmospheric chemistry Transboundary transport and deposition of Hg emission from springtime biomass burning in the Indo‐China Peninsula
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topic_title	550 DNB Transboundary transport and deposition of Hg emission from springtime biomass burning in the Indo‐China Peninsula transport mercury biomass burning Emissions Mercury Biomass Atmospheric chemistry
topic	ddc 550 misc transport misc mercury misc biomass burning misc Emissions misc Mercury misc Biomass misc Atmospheric chemistry
topic_unstemmed	ddc 550 misc transport misc mercury misc biomass burning misc Emissions misc Mercury misc Biomass misc Atmospheric chemistry
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title	Transboundary transport and deposition of Hg emission from springtime biomass burning in the Indo‐China Peninsula
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title_full	Transboundary transport and deposition of Hg emission from springtime biomass burning in the Indo‐China Peninsula
author_sort	Wang, Xun
journal	Journal of geophysical research / D
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title_sort	transboundary transport and deposition of hg emission from springtime biomass burning in the indo‐china peninsula
title_auth	Transboundary transport and deposition of Hg emission from springtime biomass burning in the Indo‐China Peninsula
abstract	Biomass burning from the Indo‐China Peninsula region is an important source of atmospheric mercury (Hg). We isolated 18 unique transport events over 2 years using observations of Hg and CO at a high‐altitude background site in southwestern China (Mount Ailao Observatory Station) to assess the transport and impact of Hg emissions from biomass burning. The quantity of Hg emission and the source regions were determined using ΔTGM/ΔCO slopes coupled with backward trajectory analysis and CO emission inventories. The slopes of ΔTGM/ΔCO appeared to be a useful chemical indicator for source identification. Industrial emission sources exhibited slopes in the range of 5.1–61.0 × 10 −7 (parts per trillion by volume, pptv/pptv), in contrast to a slope of 2.0–6.0 × 10 −7 for typical biomass burning. Transboundary transport of Hg from biomass burning led to episodically elevated atmospheric Hg concentrations during springtime. Hg emissions from biomass burning in the Indo‐China Peninsula region from 2001 to 2008 were estimated to be 11.4 ± 2.1 Mg yr −1 , equivalent to 40% of annual anthropogenic emissions in the region. In addition, Hg emissions from biomass burning contained a substantial fraction of particulate bound Hg (PBM). Assuming that PBM readily deposits locally (within 50 km), the local Hg deposition caused by the PBM was estimated to be 2.2 ± 0.4 Mg yr −1 , up to 1 order of magnitude higher than the PBM deposition caused by anthropogenic emissions during springtime in the region. The strong springtime emissions potentially pose a threat to the ecosystems of the Indo‐China Peninsula and southwest China. ΔTGM/ΔCO slope can be an indicator for source identification ΔTGM/ΔCO slope for biomass burning is about of 2.0 × 10−7 Hg emission from biomass burning was estimated
abstractGer	Biomass burning from the Indo‐China Peninsula region is an important source of atmospheric mercury (Hg). We isolated 18 unique transport events over 2 years using observations of Hg and CO at a high‐altitude background site in southwestern China (Mount Ailao Observatory Station) to assess the transport and impact of Hg emissions from biomass burning. The quantity of Hg emission and the source regions were determined using ΔTGM/ΔCO slopes coupled with backward trajectory analysis and CO emission inventories. The slopes of ΔTGM/ΔCO appeared to be a useful chemical indicator for source identification. Industrial emission sources exhibited slopes in the range of 5.1–61.0 × 10 −7 (parts per trillion by volume, pptv/pptv), in contrast to a slope of 2.0–6.0 × 10 −7 for typical biomass burning. Transboundary transport of Hg from biomass burning led to episodically elevated atmospheric Hg concentrations during springtime. Hg emissions from biomass burning in the Indo‐China Peninsula region from 2001 to 2008 were estimated to be 11.4 ± 2.1 Mg yr −1 , equivalent to 40% of annual anthropogenic emissions in the region. In addition, Hg emissions from biomass burning contained a substantial fraction of particulate bound Hg (PBM). Assuming that PBM readily deposits locally (within 50 km), the local Hg deposition caused by the PBM was estimated to be 2.2 ± 0.4 Mg yr −1 , up to 1 order of magnitude higher than the PBM deposition caused by anthropogenic emissions during springtime in the region. The strong springtime emissions potentially pose a threat to the ecosystems of the Indo‐China Peninsula and southwest China. ΔTGM/ΔCO slope can be an indicator for source identification ΔTGM/ΔCO slope for biomass burning is about of 2.0 × 10−7 Hg emission from biomass burning was estimated
abstract_unstemmed	Biomass burning from the Indo‐China Peninsula region is an important source of atmospheric mercury (Hg). We isolated 18 unique transport events over 2 years using observations of Hg and CO at a high‐altitude background site in southwestern China (Mount Ailao Observatory Station) to assess the transport and impact of Hg emissions from biomass burning. The quantity of Hg emission and the source regions were determined using ΔTGM/ΔCO slopes coupled with backward trajectory analysis and CO emission inventories. The slopes of ΔTGM/ΔCO appeared to be a useful chemical indicator for source identification. Industrial emission sources exhibited slopes in the range of 5.1–61.0 × 10 −7 (parts per trillion by volume, pptv/pptv), in contrast to a slope of 2.0–6.0 × 10 −7 for typical biomass burning. Transboundary transport of Hg from biomass burning led to episodically elevated atmospheric Hg concentrations during springtime. Hg emissions from biomass burning in the Indo‐China Peninsula region from 2001 to 2008 were estimated to be 11.4 ± 2.1 Mg yr −1 , equivalent to 40% of annual anthropogenic emissions in the region. In addition, Hg emissions from biomass burning contained a substantial fraction of particulate bound Hg (PBM). Assuming that PBM readily deposits locally (within 50 km), the local Hg deposition caused by the PBM was estimated to be 2.2 ± 0.4 Mg yr −1 , up to 1 order of magnitude higher than the PBM deposition caused by anthropogenic emissions during springtime in the region. The strong springtime emissions potentially pose a threat to the ecosystems of the Indo‐China Peninsula and southwest China. ΔTGM/ΔCO slope can be an indicator for source identification ΔTGM/ΔCO slope for biomass burning is about of 2.0 × 10−7 Hg emission from biomass burning was estimated
collection_details	GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY SSG-OLC-GEO SSG-OLC-PHA SSG-OLC-DE-84 SSG-OPC-GGO SSG-OPC-GEO GBV_ILN_62 GBV_ILN_154
container_issue	18
title_short	Transboundary transport and deposition of Hg emission from springtime biomass burning in the Indo‐China Peninsula
url	http://dx.doi.org/10.1002/2015JD023525 http://onlinelibrary.wiley.com/doi/10.1002/2015JD023525/abstract http://search.proquest.com/docview/1724667783
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author2	Zhang, Hui Lin, Che‐Jen Fu, Xuewu Zhang, Yiping Feng, Xinbin
author2Str	Zhang, Hui Lin, Che‐Jen Fu, Xuewu Zhang, Yiping Feng, Xinbin
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up_date	2024-07-03T23:01:28.244Z
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