Distribution of anionic and nonionic surfactants in a sewage-impacted Mediterranean coastal lagoon: inputs and seasonal variations
In this work we have monitored the seasonal inputs, occurrence and distribution of the world's most widely used surfactants (linear alkylbenzene sulfonates, LAS, nonylphenol polyethoxylates, NPEOs, and alcohol polyethoxylates, AEOs) in Mar Menor lagoon (SE Spain) and its main tributary (El Albu...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Traverso-Soto, Juan M [verfasserIn] |
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| Format: |
Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2015 |
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| Rechteinformationen: |
Nutzungsrecht: Copyright © 2014 Elsevier B.V. All rights reserved. |
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| Schlagwörter: |
Geologic Sediments - chemistry Surface-Active Agents - analysis |
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| Übergeordnetes Werk: |
Enthalten in: The science of the total environment - Amsterdam : Elsevier, 1972, 503-504(2015), Seite 87-96 |
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| Übergeordnetes Werk: |
volume:503-504 ; year:2015 ; pages:87-96 |
| Links: |
|---|
| DOI / URN: |
10.1016/j.scitotenv.2014.06.107 |
|---|
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OLC1967431361 |
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| 520 | |a In this work we have monitored the seasonal inputs, occurrence and distribution of the world's most widely used surfactants (linear alkylbenzene sulfonates, LAS, nonylphenol polyethoxylates, NPEOs, and alcohol polyethoxylates, AEOs) in Mar Menor lagoon (SE Spain) and its main tributary (El Albujón) for the first time. Concentration of target compounds was determined in both surface waters and sediments after solid phase extraction and pressurized liquid extraction, respectively, followed by liquid chromatography-mass spectrometry (LC-MS). There were significant differences in surfactant fluxes from El Albujón towards Mar Menor depending on the season and the day of the week, with maximum estimated annual inputs being detected for LAS (406 kg) and their metabolites, sulfophenyl carboxylic acids (482 kg). Average concentrations of surfactants in the lagoon were between 44 and 1665 μg/kg in sediment, and between 0.3 and 63 μg/L in water. These levels were significantly higher for samples collected near the shore than for those measured inside the lagoon itself. Overall, the occurrence and distribution of surfactants in the system could be explained due to a combination of different sources (surface and groundwater inputs, treated and untreated wastewater effluents, towns, ports, etc.) and simultaneous in-situ physicochemical and biological processes, with an special emphasis on degradation during warmer months. | ||
| 540 | |a Nutzungsrecht: Copyright © 2014 Elsevier B.V. All rights reserved. | ||
| 650 | 4 | |a Geologic Sediments - chemistry | |
| 650 | 4 | |a Groundwater - chemistry | |
| 650 | 4 | |a Surface-Active Agents - analysis | |
| 650 | 4 | |a Sewage - analysis | |
| 650 | 4 | |a Water Pollutants, Chemical - analysis | |
| 650 | 4 | |a Sewage - statistics & numerical data | |
| 700 | 1 | |a Lara-Martín, Pablo A |4 oth | |
| 700 | 1 | |a González-Mazo, Eduardo |4 oth | |
| 700 | 1 | |a León, Víctor M |4 oth | |
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10.1016/j.scitotenv.2014.06.107 doi PQ20160617 (DE-627)OLC1967431361 (DE-599)GBVOLC1967431361 (PRQ)c2068-b6ae2363b928bae2faa6bf91a836fa18753fe38f15679d5495f90b26726e2e2c0 (KEY)0073664320150000503000000087distributionofanionicandnonionicsurfactantsinasewa DE-627 ger DE-627 rakwb eng 570 333.7 610 DNB Traverso-Soto, Juan M verfasserin aut Distribution of anionic and nonionic surfactants in a sewage-impacted Mediterranean coastal lagoon: inputs and seasonal variations 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier In this work we have monitored the seasonal inputs, occurrence and distribution of the world's most widely used surfactants (linear alkylbenzene sulfonates, LAS, nonylphenol polyethoxylates, NPEOs, and alcohol polyethoxylates, AEOs) in Mar Menor lagoon (SE Spain) and its main tributary (El Albujón) for the first time. Concentration of target compounds was determined in both surface waters and sediments after solid phase extraction and pressurized liquid extraction, respectively, followed by liquid chromatography-mass spectrometry (LC-MS). There were significant differences in surfactant fluxes from El Albujón towards Mar Menor depending on the season and the day of the week, with maximum estimated annual inputs being detected for LAS (406 kg) and their metabolites, sulfophenyl carboxylic acids (482 kg). Average concentrations of surfactants in the lagoon were between 44 and 1665 μg/kg in sediment, and between 0.3 and 63 μg/L in water. These levels were significantly higher for samples collected near the shore than for those measured inside the lagoon itself. Overall, the occurrence and distribution of surfactants in the system could be explained due to a combination of different sources (surface and groundwater inputs, treated and untreated wastewater effluents, towns, ports, etc.) and simultaneous in-situ physicochemical and biological processes, with an special emphasis on degradation during warmer months. Nutzungsrecht: Copyright © 2014 Elsevier B.V. All rights reserved. Geologic Sediments - chemistry Groundwater - chemistry Surface-Active Agents - analysis Sewage - analysis Water Pollutants, Chemical - analysis Sewage - statistics & numerical data Lara-Martín, Pablo A oth González-Mazo, Eduardo oth León, Víctor M oth Enthalten in The science of the total environment Amsterdam : Elsevier, 1972 503-504(2015), Seite 87-96 (DE-627)129297917 (DE-600)121506-1 (DE-576)014490919 0048-9697 nnns volume:503-504 year:2015 pages:87-96 http://dx.doi.org/10.1016/j.scitotenv.2014.06.107 Volltext http://www.ncbi.nlm.nih.gov/pubmed/25046983 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-UMW SSG-OLC-FOR SSG-OPC-GGO GBV_ILN_21 GBV_ILN_70 GBV_ILN_4012 AR 503-504 2015 87-96 |
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10.1016/j.scitotenv.2014.06.107 doi PQ20160617 (DE-627)OLC1967431361 (DE-599)GBVOLC1967431361 (PRQ)c2068-b6ae2363b928bae2faa6bf91a836fa18753fe38f15679d5495f90b26726e2e2c0 (KEY)0073664320150000503000000087distributionofanionicandnonionicsurfactantsinasewa DE-627 ger DE-627 rakwb eng 570 333.7 610 DNB Traverso-Soto, Juan M verfasserin aut Distribution of anionic and nonionic surfactants in a sewage-impacted Mediterranean coastal lagoon: inputs and seasonal variations 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier In this work we have monitored the seasonal inputs, occurrence and distribution of the world's most widely used surfactants (linear alkylbenzene sulfonates, LAS, nonylphenol polyethoxylates, NPEOs, and alcohol polyethoxylates, AEOs) in Mar Menor lagoon (SE Spain) and its main tributary (El Albujón) for the first time. Concentration of target compounds was determined in both surface waters and sediments after solid phase extraction and pressurized liquid extraction, respectively, followed by liquid chromatography-mass spectrometry (LC-MS). There were significant differences in surfactant fluxes from El Albujón towards Mar Menor depending on the season and the day of the week, with maximum estimated annual inputs being detected for LAS (406 kg) and their metabolites, sulfophenyl carboxylic acids (482 kg). Average concentrations of surfactants in the lagoon were between 44 and 1665 μg/kg in sediment, and between 0.3 and 63 μg/L in water. These levels were significantly higher for samples collected near the shore than for those measured inside the lagoon itself. Overall, the occurrence and distribution of surfactants in the system could be explained due to a combination of different sources (surface and groundwater inputs, treated and untreated wastewater effluents, towns, ports, etc.) and simultaneous in-situ physicochemical and biological processes, with an special emphasis on degradation during warmer months. Nutzungsrecht: Copyright © 2014 Elsevier B.V. All rights reserved. Geologic Sediments - chemistry Groundwater - chemistry Surface-Active Agents - analysis Sewage - analysis Water Pollutants, Chemical - analysis Sewage - statistics & numerical data Lara-Martín, Pablo A oth González-Mazo, Eduardo oth León, Víctor M oth Enthalten in The science of the total environment Amsterdam : Elsevier, 1972 503-504(2015), Seite 87-96 (DE-627)129297917 (DE-600)121506-1 (DE-576)014490919 0048-9697 nnns volume:503-504 year:2015 pages:87-96 http://dx.doi.org/10.1016/j.scitotenv.2014.06.107 Volltext http://www.ncbi.nlm.nih.gov/pubmed/25046983 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-UMW SSG-OLC-FOR SSG-OPC-GGO GBV_ILN_21 GBV_ILN_70 GBV_ILN_4012 AR 503-504 2015 87-96 |
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10.1016/j.scitotenv.2014.06.107 doi PQ20160617 (DE-627)OLC1967431361 (DE-599)GBVOLC1967431361 (PRQ)c2068-b6ae2363b928bae2faa6bf91a836fa18753fe38f15679d5495f90b26726e2e2c0 (KEY)0073664320150000503000000087distributionofanionicandnonionicsurfactantsinasewa DE-627 ger DE-627 rakwb eng 570 333.7 610 DNB Traverso-Soto, Juan M verfasserin aut Distribution of anionic and nonionic surfactants in a sewage-impacted Mediterranean coastal lagoon: inputs and seasonal variations 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier In this work we have monitored the seasonal inputs, occurrence and distribution of the world's most widely used surfactants (linear alkylbenzene sulfonates, LAS, nonylphenol polyethoxylates, NPEOs, and alcohol polyethoxylates, AEOs) in Mar Menor lagoon (SE Spain) and its main tributary (El Albujón) for the first time. Concentration of target compounds was determined in both surface waters and sediments after solid phase extraction and pressurized liquid extraction, respectively, followed by liquid chromatography-mass spectrometry (LC-MS). There were significant differences in surfactant fluxes from El Albujón towards Mar Menor depending on the season and the day of the week, with maximum estimated annual inputs being detected for LAS (406 kg) and their metabolites, sulfophenyl carboxylic acids (482 kg). Average concentrations of surfactants in the lagoon were between 44 and 1665 μg/kg in sediment, and between 0.3 and 63 μg/L in water. These levels were significantly higher for samples collected near the shore than for those measured inside the lagoon itself. Overall, the occurrence and distribution of surfactants in the system could be explained due to a combination of different sources (surface and groundwater inputs, treated and untreated wastewater effluents, towns, ports, etc.) and simultaneous in-situ physicochemical and biological processes, with an special emphasis on degradation during warmer months. Nutzungsrecht: Copyright © 2014 Elsevier B.V. All rights reserved. Geologic Sediments - chemistry Groundwater - chemistry Surface-Active Agents - analysis Sewage - analysis Water Pollutants, Chemical - analysis Sewage - statistics & numerical data Lara-Martín, Pablo A oth González-Mazo, Eduardo oth León, Víctor M oth Enthalten in The science of the total environment Amsterdam : Elsevier, 1972 503-504(2015), Seite 87-96 (DE-627)129297917 (DE-600)121506-1 (DE-576)014490919 0048-9697 nnns volume:503-504 year:2015 pages:87-96 http://dx.doi.org/10.1016/j.scitotenv.2014.06.107 Volltext http://www.ncbi.nlm.nih.gov/pubmed/25046983 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-UMW SSG-OLC-FOR SSG-OPC-GGO GBV_ILN_21 GBV_ILN_70 GBV_ILN_4012 AR 503-504 2015 87-96 |
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10.1016/j.scitotenv.2014.06.107 doi PQ20160617 (DE-627)OLC1967431361 (DE-599)GBVOLC1967431361 (PRQ)c2068-b6ae2363b928bae2faa6bf91a836fa18753fe38f15679d5495f90b26726e2e2c0 (KEY)0073664320150000503000000087distributionofanionicandnonionicsurfactantsinasewa DE-627 ger DE-627 rakwb eng 570 333.7 610 DNB Traverso-Soto, Juan M verfasserin aut Distribution of anionic and nonionic surfactants in a sewage-impacted Mediterranean coastal lagoon: inputs and seasonal variations 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier In this work we have monitored the seasonal inputs, occurrence and distribution of the world's most widely used surfactants (linear alkylbenzene sulfonates, LAS, nonylphenol polyethoxylates, NPEOs, and alcohol polyethoxylates, AEOs) in Mar Menor lagoon (SE Spain) and its main tributary (El Albujón) for the first time. Concentration of target compounds was determined in both surface waters and sediments after solid phase extraction and pressurized liquid extraction, respectively, followed by liquid chromatography-mass spectrometry (LC-MS). There were significant differences in surfactant fluxes from El Albujón towards Mar Menor depending on the season and the day of the week, with maximum estimated annual inputs being detected for LAS (406 kg) and their metabolites, sulfophenyl carboxylic acids (482 kg). Average concentrations of surfactants in the lagoon were between 44 and 1665 μg/kg in sediment, and between 0.3 and 63 μg/L in water. These levels were significantly higher for samples collected near the shore than for those measured inside the lagoon itself. Overall, the occurrence and distribution of surfactants in the system could be explained due to a combination of different sources (surface and groundwater inputs, treated and untreated wastewater effluents, towns, ports, etc.) and simultaneous in-situ physicochemical and biological processes, with an special emphasis on degradation during warmer months. Nutzungsrecht: Copyright © 2014 Elsevier B.V. All rights reserved. Geologic Sediments - chemistry Groundwater - chemistry Surface-Active Agents - analysis Sewage - analysis Water Pollutants, Chemical - analysis Sewage - statistics & numerical data Lara-Martín, Pablo A oth González-Mazo, Eduardo oth León, Víctor M oth Enthalten in The science of the total environment Amsterdam : Elsevier, 1972 503-504(2015), Seite 87-96 (DE-627)129297917 (DE-600)121506-1 (DE-576)014490919 0048-9697 nnns volume:503-504 year:2015 pages:87-96 http://dx.doi.org/10.1016/j.scitotenv.2014.06.107 Volltext http://www.ncbi.nlm.nih.gov/pubmed/25046983 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-UMW SSG-OLC-FOR SSG-OPC-GGO GBV_ILN_21 GBV_ILN_70 GBV_ILN_4012 AR 503-504 2015 87-96 |
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10.1016/j.scitotenv.2014.06.107 doi PQ20160617 (DE-627)OLC1967431361 (DE-599)GBVOLC1967431361 (PRQ)c2068-b6ae2363b928bae2faa6bf91a836fa18753fe38f15679d5495f90b26726e2e2c0 (KEY)0073664320150000503000000087distributionofanionicandnonionicsurfactantsinasewa DE-627 ger DE-627 rakwb eng 570 333.7 610 DNB Traverso-Soto, Juan M verfasserin aut Distribution of anionic and nonionic surfactants in a sewage-impacted Mediterranean coastal lagoon: inputs and seasonal variations 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier In this work we have monitored the seasonal inputs, occurrence and distribution of the world's most widely used surfactants (linear alkylbenzene sulfonates, LAS, nonylphenol polyethoxylates, NPEOs, and alcohol polyethoxylates, AEOs) in Mar Menor lagoon (SE Spain) and its main tributary (El Albujón) for the first time. Concentration of target compounds was determined in both surface waters and sediments after solid phase extraction and pressurized liquid extraction, respectively, followed by liquid chromatography-mass spectrometry (LC-MS). There were significant differences in surfactant fluxes from El Albujón towards Mar Menor depending on the season and the day of the week, with maximum estimated annual inputs being detected for LAS (406 kg) and their metabolites, sulfophenyl carboxylic acids (482 kg). Average concentrations of surfactants in the lagoon were between 44 and 1665 μg/kg in sediment, and between 0.3 and 63 μg/L in water. These levels were significantly higher for samples collected near the shore than for those measured inside the lagoon itself. Overall, the occurrence and distribution of surfactants in the system could be explained due to a combination of different sources (surface and groundwater inputs, treated and untreated wastewater effluents, towns, ports, etc.) and simultaneous in-situ physicochemical and biological processes, with an special emphasis on degradation during warmer months. Nutzungsrecht: Copyright © 2014 Elsevier B.V. All rights reserved. Geologic Sediments - chemistry Groundwater - chemistry Surface-Active Agents - analysis Sewage - analysis Water Pollutants, Chemical - analysis Sewage - statistics & numerical data Lara-Martín, Pablo A oth González-Mazo, Eduardo oth León, Víctor M oth Enthalten in The science of the total environment Amsterdam : Elsevier, 1972 503-504(2015), Seite 87-96 (DE-627)129297917 (DE-600)121506-1 (DE-576)014490919 0048-9697 nnns volume:503-504 year:2015 pages:87-96 http://dx.doi.org/10.1016/j.scitotenv.2014.06.107 Volltext http://www.ncbi.nlm.nih.gov/pubmed/25046983 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-UMW SSG-OLC-FOR SSG-OPC-GGO GBV_ILN_21 GBV_ILN_70 GBV_ILN_4012 AR 503-504 2015 87-96 |
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Distribution of anionic and nonionic surfactants in a sewage-impacted Mediterranean coastal lagoon: inputs and seasonal variations |
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distribution of anionic and nonionic surfactants in a sewage-impacted mediterranean coastal lagoon: inputs and seasonal variations |
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Distribution of anionic and nonionic surfactants in a sewage-impacted Mediterranean coastal lagoon: inputs and seasonal variations |
| abstract |
In this work we have monitored the seasonal inputs, occurrence and distribution of the world's most widely used surfactants (linear alkylbenzene sulfonates, LAS, nonylphenol polyethoxylates, NPEOs, and alcohol polyethoxylates, AEOs) in Mar Menor lagoon (SE Spain) and its main tributary (El Albujón) for the first time. Concentration of target compounds was determined in both surface waters and sediments after solid phase extraction and pressurized liquid extraction, respectively, followed by liquid chromatography-mass spectrometry (LC-MS). There were significant differences in surfactant fluxes from El Albujón towards Mar Menor depending on the season and the day of the week, with maximum estimated annual inputs being detected for LAS (406 kg) and their metabolites, sulfophenyl carboxylic acids (482 kg). Average concentrations of surfactants in the lagoon were between 44 and 1665 μg/kg in sediment, and between 0.3 and 63 μg/L in water. These levels were significantly higher for samples collected near the shore than for those measured inside the lagoon itself. Overall, the occurrence and distribution of surfactants in the system could be explained due to a combination of different sources (surface and groundwater inputs, treated and untreated wastewater effluents, towns, ports, etc.) and simultaneous in-situ physicochemical and biological processes, with an special emphasis on degradation during warmer months. |
| abstractGer |
In this work we have monitored the seasonal inputs, occurrence and distribution of the world's most widely used surfactants (linear alkylbenzene sulfonates, LAS, nonylphenol polyethoxylates, NPEOs, and alcohol polyethoxylates, AEOs) in Mar Menor lagoon (SE Spain) and its main tributary (El Albujón) for the first time. Concentration of target compounds was determined in both surface waters and sediments after solid phase extraction and pressurized liquid extraction, respectively, followed by liquid chromatography-mass spectrometry (LC-MS). There were significant differences in surfactant fluxes from El Albujón towards Mar Menor depending on the season and the day of the week, with maximum estimated annual inputs being detected for LAS (406 kg) and their metabolites, sulfophenyl carboxylic acids (482 kg). Average concentrations of surfactants in the lagoon were between 44 and 1665 μg/kg in sediment, and between 0.3 and 63 μg/L in water. These levels were significantly higher for samples collected near the shore than for those measured inside the lagoon itself. Overall, the occurrence and distribution of surfactants in the system could be explained due to a combination of different sources (surface and groundwater inputs, treated and untreated wastewater effluents, towns, ports, etc.) and simultaneous in-situ physicochemical and biological processes, with an special emphasis on degradation during warmer months. |
| abstract_unstemmed |
In this work we have monitored the seasonal inputs, occurrence and distribution of the world's most widely used surfactants (linear alkylbenzene sulfonates, LAS, nonylphenol polyethoxylates, NPEOs, and alcohol polyethoxylates, AEOs) in Mar Menor lagoon (SE Spain) and its main tributary (El Albujón) for the first time. Concentration of target compounds was determined in both surface waters and sediments after solid phase extraction and pressurized liquid extraction, respectively, followed by liquid chromatography-mass spectrometry (LC-MS). There were significant differences in surfactant fluxes from El Albujón towards Mar Menor depending on the season and the day of the week, with maximum estimated annual inputs being detected for LAS (406 kg) and their metabolites, sulfophenyl carboxylic acids (482 kg). Average concentrations of surfactants in the lagoon were between 44 and 1665 μg/kg in sediment, and between 0.3 and 63 μg/L in water. These levels were significantly higher for samples collected near the shore than for those measured inside the lagoon itself. Overall, the occurrence and distribution of surfactants in the system could be explained due to a combination of different sources (surface and groundwater inputs, treated and untreated wastewater effluents, towns, ports, etc.) and simultaneous in-situ physicochemical and biological processes, with an special emphasis on degradation during warmer months. |
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| title_short |
Distribution of anionic and nonionic surfactants in a sewage-impacted Mediterranean coastal lagoon: inputs and seasonal variations |
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