Theory of Long-Range Ultracold Atom-Molecule Photoassociation
The creation of ultracold molecules is currently limited to diatomic species. In this Letter, we present a theoretical description of the photoassociation of ultracold atoms and molecules to create ultracold excited triatomic molecules, thus being a novel example of a light-assisted ultracold chemic...
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Gespeichert in:
| Autor*in: |
Pérez-Ríos, Jesús [verfasserIn] |
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| Format: |
Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2015 |
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| Übergeordnetes Werk: |
Enthalten in: Physical review letters - Ridge, NY : American Physical Society, 1958, 115(2015), 7 |
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| Übergeordnetes Werk: |
volume:115 ; year:2015 ; number:7 |
| Links: |
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| DOI / URN: |
10.1103/PhysRevLett.115.073201 |
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OLC1969293683 |
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| 520 | |a The creation of ultracold molecules is currently limited to diatomic species. In this Letter, we present a theoretical description of the photoassociation of ultracold atoms and molecules to create ultracold excited triatomic molecules, thus being a novel example of a light-assisted ultracold chemical reaction. The calculation of the photoassociation rate of an ultracold Cs_{2} molecule in its rovibrational ground state with an ultracold Cs atom at frequencies close to its resonant excitation is reported, based on the solution of the quantum dynamics involving the atom-molecule long-range interactions and assuming a model potential for the short-range physics. The rate for the formation of excited Cs_{3} molecules is predicted to be comparable with currently observed atom-atom photoassociation rates. We formulate an experimental proposal to observe this process relying on the available techniques of optical lattices and standard photoassociation spectroscopy. | ||
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10.1103/PhysRevLett.115.073201 doi PQ20160211 (DE-627)OLC1969293683 (DE-599)GBVOLC1969293683 (PRQ)a1689-f876bd00a024e4fb9346cce37a84666764c3a1b8c4161796a8992261de07e4ac0 (KEY)0009201020150000115000700000theoryoflongrangeultracoldatommoleculephotoassocia DE-627 ger DE-627 rakwb eng 550 DNB UA 1000 AVZ rvk Pérez-Ríos, Jesús verfasserin aut Theory of Long-Range Ultracold Atom-Molecule Photoassociation 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The creation of ultracold molecules is currently limited to diatomic species. In this Letter, we present a theoretical description of the photoassociation of ultracold atoms and molecules to create ultracold excited triatomic molecules, thus being a novel example of a light-assisted ultracold chemical reaction. The calculation of the photoassociation rate of an ultracold Cs_{2} molecule in its rovibrational ground state with an ultracold Cs atom at frequencies close to its resonant excitation is reported, based on the solution of the quantum dynamics involving the atom-molecule long-range interactions and assuming a model potential for the short-range physics. The rate for the formation of excited Cs_{3} molecules is predicted to be comparable with currently observed atom-atom photoassociation rates. We formulate an experimental proposal to observe this process relying on the available techniques of optical lattices and standard photoassociation spectroscopy. Quantum Gases Quantum Physics Atomic Physics Physics Condensed Matter Lepers, Maxence oth Dulieu, Olivier oth Enthalten in Physical review letters Ridge, NY : American Physical Society, 1958 115(2015), 7 (DE-627)129503959 (DE-600)208853-8 (DE-576)014907267 0031-9007 nnns volume:115 year:2015 number:7 http://dx.doi.org/10.1103/PhysRevLett.115.073201 Volltext http://www.ncbi.nlm.nih.gov/pubmed/26317720 http://arxiv.org/abs/1505.03288 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY GBV_ILN_21 GBV_ILN_22 GBV_ILN_40 GBV_ILN_47 GBV_ILN_55 GBV_ILN_59 GBV_ILN_60 GBV_ILN_70 GBV_ILN_130 GBV_ILN_2004 GBV_ILN_2016 GBV_ILN_2095 GBV_ILN_2192 GBV_ILN_2279 GBV_ILN_2286 UA 1000 AR 115 2015 7 |
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10.1103/PhysRevLett.115.073201 doi PQ20160211 (DE-627)OLC1969293683 (DE-599)GBVOLC1969293683 (PRQ)a1689-f876bd00a024e4fb9346cce37a84666764c3a1b8c4161796a8992261de07e4ac0 (KEY)0009201020150000115000700000theoryoflongrangeultracoldatommoleculephotoassocia DE-627 ger DE-627 rakwb eng 550 DNB UA 1000 AVZ rvk Pérez-Ríos, Jesús verfasserin aut Theory of Long-Range Ultracold Atom-Molecule Photoassociation 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The creation of ultracold molecules is currently limited to diatomic species. In this Letter, we present a theoretical description of the photoassociation of ultracold atoms and molecules to create ultracold excited triatomic molecules, thus being a novel example of a light-assisted ultracold chemical reaction. The calculation of the photoassociation rate of an ultracold Cs_{2} molecule in its rovibrational ground state with an ultracold Cs atom at frequencies close to its resonant excitation is reported, based on the solution of the quantum dynamics involving the atom-molecule long-range interactions and assuming a model potential for the short-range physics. The rate for the formation of excited Cs_{3} molecules is predicted to be comparable with currently observed atom-atom photoassociation rates. We formulate an experimental proposal to observe this process relying on the available techniques of optical lattices and standard photoassociation spectroscopy. Quantum Gases Quantum Physics Atomic Physics Physics Condensed Matter Lepers, Maxence oth Dulieu, Olivier oth Enthalten in Physical review letters Ridge, NY : American Physical Society, 1958 115(2015), 7 (DE-627)129503959 (DE-600)208853-8 (DE-576)014907267 0031-9007 nnns volume:115 year:2015 number:7 http://dx.doi.org/10.1103/PhysRevLett.115.073201 Volltext http://www.ncbi.nlm.nih.gov/pubmed/26317720 http://arxiv.org/abs/1505.03288 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY GBV_ILN_21 GBV_ILN_22 GBV_ILN_40 GBV_ILN_47 GBV_ILN_55 GBV_ILN_59 GBV_ILN_60 GBV_ILN_70 GBV_ILN_130 GBV_ILN_2004 GBV_ILN_2016 GBV_ILN_2095 GBV_ILN_2192 GBV_ILN_2279 GBV_ILN_2286 UA 1000 AR 115 2015 7 |
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10.1103/PhysRevLett.115.073201 doi PQ20160211 (DE-627)OLC1969293683 (DE-599)GBVOLC1969293683 (PRQ)a1689-f876bd00a024e4fb9346cce37a84666764c3a1b8c4161796a8992261de07e4ac0 (KEY)0009201020150000115000700000theoryoflongrangeultracoldatommoleculephotoassocia DE-627 ger DE-627 rakwb eng 550 DNB UA 1000 AVZ rvk Pérez-Ríos, Jesús verfasserin aut Theory of Long-Range Ultracold Atom-Molecule Photoassociation 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The creation of ultracold molecules is currently limited to diatomic species. In this Letter, we present a theoretical description of the photoassociation of ultracold atoms and molecules to create ultracold excited triatomic molecules, thus being a novel example of a light-assisted ultracold chemical reaction. The calculation of the photoassociation rate of an ultracold Cs_{2} molecule in its rovibrational ground state with an ultracold Cs atom at frequencies close to its resonant excitation is reported, based on the solution of the quantum dynamics involving the atom-molecule long-range interactions and assuming a model potential for the short-range physics. The rate for the formation of excited Cs_{3} molecules is predicted to be comparable with currently observed atom-atom photoassociation rates. We formulate an experimental proposal to observe this process relying on the available techniques of optical lattices and standard photoassociation spectroscopy. Quantum Gases Quantum Physics Atomic Physics Physics Condensed Matter Lepers, Maxence oth Dulieu, Olivier oth Enthalten in Physical review letters Ridge, NY : American Physical Society, 1958 115(2015), 7 (DE-627)129503959 (DE-600)208853-8 (DE-576)014907267 0031-9007 nnns volume:115 year:2015 number:7 http://dx.doi.org/10.1103/PhysRevLett.115.073201 Volltext http://www.ncbi.nlm.nih.gov/pubmed/26317720 http://arxiv.org/abs/1505.03288 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY GBV_ILN_21 GBV_ILN_22 GBV_ILN_40 GBV_ILN_47 GBV_ILN_55 GBV_ILN_59 GBV_ILN_60 GBV_ILN_70 GBV_ILN_130 GBV_ILN_2004 GBV_ILN_2016 GBV_ILN_2095 GBV_ILN_2192 GBV_ILN_2279 GBV_ILN_2286 UA 1000 AR 115 2015 7 |
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10.1103/PhysRevLett.115.073201 doi PQ20160211 (DE-627)OLC1969293683 (DE-599)GBVOLC1969293683 (PRQ)a1689-f876bd00a024e4fb9346cce37a84666764c3a1b8c4161796a8992261de07e4ac0 (KEY)0009201020150000115000700000theoryoflongrangeultracoldatommoleculephotoassocia DE-627 ger DE-627 rakwb eng 550 DNB UA 1000 AVZ rvk Pérez-Ríos, Jesús verfasserin aut Theory of Long-Range Ultracold Atom-Molecule Photoassociation 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The creation of ultracold molecules is currently limited to diatomic species. In this Letter, we present a theoretical description of the photoassociation of ultracold atoms and molecules to create ultracold excited triatomic molecules, thus being a novel example of a light-assisted ultracold chemical reaction. The calculation of the photoassociation rate of an ultracold Cs_{2} molecule in its rovibrational ground state with an ultracold Cs atom at frequencies close to its resonant excitation is reported, based on the solution of the quantum dynamics involving the atom-molecule long-range interactions and assuming a model potential for the short-range physics. The rate for the formation of excited Cs_{3} molecules is predicted to be comparable with currently observed atom-atom photoassociation rates. We formulate an experimental proposal to observe this process relying on the available techniques of optical lattices and standard photoassociation spectroscopy. Quantum Gases Quantum Physics Atomic Physics Physics Condensed Matter Lepers, Maxence oth Dulieu, Olivier oth Enthalten in Physical review letters Ridge, NY : American Physical Society, 1958 115(2015), 7 (DE-627)129503959 (DE-600)208853-8 (DE-576)014907267 0031-9007 nnns volume:115 year:2015 number:7 http://dx.doi.org/10.1103/PhysRevLett.115.073201 Volltext http://www.ncbi.nlm.nih.gov/pubmed/26317720 http://arxiv.org/abs/1505.03288 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY GBV_ILN_21 GBV_ILN_22 GBV_ILN_40 GBV_ILN_47 GBV_ILN_55 GBV_ILN_59 GBV_ILN_60 GBV_ILN_70 GBV_ILN_130 GBV_ILN_2004 GBV_ILN_2016 GBV_ILN_2095 GBV_ILN_2192 GBV_ILN_2279 GBV_ILN_2286 UA 1000 AR 115 2015 7 |
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10.1103/PhysRevLett.115.073201 doi PQ20160211 (DE-627)OLC1969293683 (DE-599)GBVOLC1969293683 (PRQ)a1689-f876bd00a024e4fb9346cce37a84666764c3a1b8c4161796a8992261de07e4ac0 (KEY)0009201020150000115000700000theoryoflongrangeultracoldatommoleculephotoassocia DE-627 ger DE-627 rakwb eng 550 DNB UA 1000 AVZ rvk Pérez-Ríos, Jesús verfasserin aut Theory of Long-Range Ultracold Atom-Molecule Photoassociation 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The creation of ultracold molecules is currently limited to diatomic species. In this Letter, we present a theoretical description of the photoassociation of ultracold atoms and molecules to create ultracold excited triatomic molecules, thus being a novel example of a light-assisted ultracold chemical reaction. The calculation of the photoassociation rate of an ultracold Cs_{2} molecule in its rovibrational ground state with an ultracold Cs atom at frequencies close to its resonant excitation is reported, based on the solution of the quantum dynamics involving the atom-molecule long-range interactions and assuming a model potential for the short-range physics. The rate for the formation of excited Cs_{3} molecules is predicted to be comparable with currently observed atom-atom photoassociation rates. We formulate an experimental proposal to observe this process relying on the available techniques of optical lattices and standard photoassociation spectroscopy. Quantum Gases Quantum Physics Atomic Physics Physics Condensed Matter Lepers, Maxence oth Dulieu, Olivier oth Enthalten in Physical review letters Ridge, NY : American Physical Society, 1958 115(2015), 7 (DE-627)129503959 (DE-600)208853-8 (DE-576)014907267 0031-9007 nnns volume:115 year:2015 number:7 http://dx.doi.org/10.1103/PhysRevLett.115.073201 Volltext http://www.ncbi.nlm.nih.gov/pubmed/26317720 http://arxiv.org/abs/1505.03288 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY GBV_ILN_21 GBV_ILN_22 GBV_ILN_40 GBV_ILN_47 GBV_ILN_55 GBV_ILN_59 GBV_ILN_60 GBV_ILN_70 GBV_ILN_130 GBV_ILN_2004 GBV_ILN_2016 GBV_ILN_2095 GBV_ILN_2192 GBV_ILN_2279 GBV_ILN_2286 UA 1000 AR 115 2015 7 |
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Theory of Long-Range Ultracold Atom-Molecule Photoassociation |
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Theory of Long-Range Ultracold Atom-Molecule Photoassociation |
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The creation of ultracold molecules is currently limited to diatomic species. In this Letter, we present a theoretical description of the photoassociation of ultracold atoms and molecules to create ultracold excited triatomic molecules, thus being a novel example of a light-assisted ultracold chemical reaction. The calculation of the photoassociation rate of an ultracold Cs_{2} molecule in its rovibrational ground state with an ultracold Cs atom at frequencies close to its resonant excitation is reported, based on the solution of the quantum dynamics involving the atom-molecule long-range interactions and assuming a model potential for the short-range physics. The rate for the formation of excited Cs_{3} molecules is predicted to be comparable with currently observed atom-atom photoassociation rates. We formulate an experimental proposal to observe this process relying on the available techniques of optical lattices and standard photoassociation spectroscopy. |
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The creation of ultracold molecules is currently limited to diatomic species. In this Letter, we present a theoretical description of the photoassociation of ultracold atoms and molecules to create ultracold excited triatomic molecules, thus being a novel example of a light-assisted ultracold chemical reaction. The calculation of the photoassociation rate of an ultracold Cs_{2} molecule in its rovibrational ground state with an ultracold Cs atom at frequencies close to its resonant excitation is reported, based on the solution of the quantum dynamics involving the atom-molecule long-range interactions and assuming a model potential for the short-range physics. The rate for the formation of excited Cs_{3} molecules is predicted to be comparable with currently observed atom-atom photoassociation rates. We formulate an experimental proposal to observe this process relying on the available techniques of optical lattices and standard photoassociation spectroscopy. |
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The creation of ultracold molecules is currently limited to diatomic species. In this Letter, we present a theoretical description of the photoassociation of ultracold atoms and molecules to create ultracold excited triatomic molecules, thus being a novel example of a light-assisted ultracold chemical reaction. The calculation of the photoassociation rate of an ultracold Cs_{2} molecule in its rovibrational ground state with an ultracold Cs atom at frequencies close to its resonant excitation is reported, based on the solution of the quantum dynamics involving the atom-molecule long-range interactions and assuming a model potential for the short-range physics. The rate for the formation of excited Cs_{3} molecules is predicted to be comparable with currently observed atom-atom photoassociation rates. We formulate an experimental proposal to observe this process relying on the available techniques of optical lattices and standard photoassociation spectroscopy. |
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