Facile synthesis of surface N-doped Bi2O2CO3: Origin of visible light photocatalytic activity and in situ DRIFTS studies

Bi2O2CO3 nanosheets with exposed {001} facets were prepared by a facile room temperature chemical method. Due to the high oxygen atom density in {001} facets of Bi2O2CO3, the addition of cetyltrimethylammonium bromide (CTAB) does not only influence the growth of crystalline Bi2O2CO3, but also modifi...
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Autor*in:	Zhou, Ying [verfasserIn] Zhao, Ziyan Wang, Fang Cao, Kun Doronkin, Dmitry E Dong, Fan Grunwaldt, Jan-Dierk

Format:	Artikel
Sprache:	Englisch

Erschienen:	2016

Rechteinformationen:	Nutzungsrecht: Copyright © 2016 Elsevier B.V. All rights reserved.

Übergeordnetes Werk:	Enthalten in: Journal of hazardous materials - Amsterdam : Elsevier, 1975, 307(2016), Seite 163-172
Übergeordnetes Werk:	volume:307 ; year:2016 ; pages:163-172

Links:	Volltext Link aufrufen

DOI / URN:	10.1016/j.jhazmat.2015.12.072

Katalog-ID:	OLC1973494515

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520			\|a Bi2O2CO3 nanosheets with exposed {001} facets were prepared by a facile room temperature chemical method. Due to the high oxygen atom density in {001} facets of Bi2O2CO3, the addition of cetyltrimethylammonium bromide (CTAB) does not only influence the growth of crystalline Bi2O2CO3, but also modifies the surface properties of Bi2O2CO3 through the interaction between CTAB and Bi2O2CO3. Nitrogen from CTAB as dopant interstitially incorporates in the Bi2O2CO3 surface evidenced by both experimental and theoretical investigations. Hence, the formation of localized states from NO bond improves the visible light absorption and charge separation efficiency, which leads to an enhancement of visible light photocatalytic activity toward to the degradation of Rhodamine B (RhB) and oxidation of NO. In addition, the photocatalytic NO oxidation over Bi2O2CO3 nanosheets was successfully monitored for the first time using in situ diffuse reflectance infrared Fourier-transform spectroscopy (DRIFTS). Both bidentate and monodentate nitrates were identified on the surface of catalysts during the photocatalytic reaction process. The application of this strategy to another relevant bismuth based photocatalyst, BiOCl, demonstrated that surface interstitial N doping could also be achieved in this case. Therefore, our current route seems to be a general option to modify the surface properties of bismuth based photocatalysts.
540			\|a Nutzungsrecht: Copyright © 2016 Elsevier B.V. All rights reserved.
700	1		\|a Zhao, Ziyan \|4 oth
700	1		\|a Wang, Fang \|4 oth
700	1		\|a Cao, Kun \|4 oth
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700	1		\|a Dong, Fan \|4 oth
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allfields	10.1016/j.jhazmat.2015.12.072 doi PQ20160610 (DE-627)OLC1973494515 (DE-599)GBVOLC1973494515 (PRQ)c2232-a2ed9efdff4a13f95502ef4b7f43bc856d0d2f017478a9117fb8ca59457b4bc60 (KEY)0002474020160000307000000163facilesynthesisofsurfacendopedbi2o2co3originofvisi DE-627 ger DE-627 rakwb eng 530 DNB 43.13 bkl 50.17 bkl 58.53 bkl Zhou, Ying verfasserin aut Facile synthesis of surface N-doped Bi2O2CO3: Origin of visible light photocatalytic activity and in situ DRIFTS studies 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier Bi2O2CO3 nanosheets with exposed {001} facets were prepared by a facile room temperature chemical method. Due to the high oxygen atom density in {001} facets of Bi2O2CO3, the addition of cetyltrimethylammonium bromide (CTAB) does not only influence the growth of crystalline Bi2O2CO3, but also modifies the surface properties of Bi2O2CO3 through the interaction between CTAB and Bi2O2CO3. Nitrogen from CTAB as dopant interstitially incorporates in the Bi2O2CO3 surface evidenced by both experimental and theoretical investigations. Hence, the formation of localized states from NO bond improves the visible light absorption and charge separation efficiency, which leads to an enhancement of visible light photocatalytic activity toward to the degradation of Rhodamine B (RhB) and oxidation of NO. In addition, the photocatalytic NO oxidation over Bi2O2CO3 nanosheets was successfully monitored for the first time using in situ diffuse reflectance infrared Fourier-transform spectroscopy (DRIFTS). Both bidentate and monodentate nitrates were identified on the surface of catalysts during the photocatalytic reaction process. The application of this strategy to another relevant bismuth based photocatalyst, BiOCl, demonstrated that surface interstitial N doping could also be achieved in this case. Therefore, our current route seems to be a general option to modify the surface properties of bismuth based photocatalysts. Nutzungsrecht: Copyright © 2016 Elsevier B.V. All rights reserved. Zhao, Ziyan oth Wang, Fang oth Cao, Kun oth Doronkin, Dmitry E oth Dong, Fan oth Grunwaldt, Jan-Dierk oth Enthalten in Journal of hazardous materials Amsterdam : Elsevier, 1975 307(2016), Seite 163-172 (DE-627)129442305 (DE-600)195278-X (DE-576)9129442303 0304-3894 nnns volume:307 year:2016 pages:163-172 http://dx.doi.org/10.1016/j.jhazmat.2015.12.072 Volltext http://www.ncbi.nlm.nih.gov/pubmed/26780703 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-UMW SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_70 43.13 AVZ 50.17 AVZ 58.53 AVZ AR 307 2016 163-172
spelling	10.1016/j.jhazmat.2015.12.072 doi PQ20160610 (DE-627)OLC1973494515 (DE-599)GBVOLC1973494515 (PRQ)c2232-a2ed9efdff4a13f95502ef4b7f43bc856d0d2f017478a9117fb8ca59457b4bc60 (KEY)0002474020160000307000000163facilesynthesisofsurfacendopedbi2o2co3originofvisi DE-627 ger DE-627 rakwb eng 530 DNB 43.13 bkl 50.17 bkl 58.53 bkl Zhou, Ying verfasserin aut Facile synthesis of surface N-doped Bi2O2CO3: Origin of visible light photocatalytic activity and in situ DRIFTS studies 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier Bi2O2CO3 nanosheets with exposed {001} facets were prepared by a facile room temperature chemical method. Due to the high oxygen atom density in {001} facets of Bi2O2CO3, the addition of cetyltrimethylammonium bromide (CTAB) does not only influence the growth of crystalline Bi2O2CO3, but also modifies the surface properties of Bi2O2CO3 through the interaction between CTAB and Bi2O2CO3. Nitrogen from CTAB as dopant interstitially incorporates in the Bi2O2CO3 surface evidenced by both experimental and theoretical investigations. Hence, the formation of localized states from NO bond improves the visible light absorption and charge separation efficiency, which leads to an enhancement of visible light photocatalytic activity toward to the degradation of Rhodamine B (RhB) and oxidation of NO. In addition, the photocatalytic NO oxidation over Bi2O2CO3 nanosheets was successfully monitored for the first time using in situ diffuse reflectance infrared Fourier-transform spectroscopy (DRIFTS). Both bidentate and monodentate nitrates were identified on the surface of catalysts during the photocatalytic reaction process. The application of this strategy to another relevant bismuth based photocatalyst, BiOCl, demonstrated that surface interstitial N doping could also be achieved in this case. Therefore, our current route seems to be a general option to modify the surface properties of bismuth based photocatalysts. Nutzungsrecht: Copyright © 2016 Elsevier B.V. All rights reserved. Zhao, Ziyan oth Wang, Fang oth Cao, Kun oth Doronkin, Dmitry E oth Dong, Fan oth Grunwaldt, Jan-Dierk oth Enthalten in Journal of hazardous materials Amsterdam : Elsevier, 1975 307(2016), Seite 163-172 (DE-627)129442305 (DE-600)195278-X (DE-576)9129442303 0304-3894 nnns volume:307 year:2016 pages:163-172 http://dx.doi.org/10.1016/j.jhazmat.2015.12.072 Volltext http://www.ncbi.nlm.nih.gov/pubmed/26780703 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-UMW SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_70 43.13 AVZ 50.17 AVZ 58.53 AVZ AR 307 2016 163-172
allfields_unstemmed	10.1016/j.jhazmat.2015.12.072 doi PQ20160610 (DE-627)OLC1973494515 (DE-599)GBVOLC1973494515 (PRQ)c2232-a2ed9efdff4a13f95502ef4b7f43bc856d0d2f017478a9117fb8ca59457b4bc60 (KEY)0002474020160000307000000163facilesynthesisofsurfacendopedbi2o2co3originofvisi DE-627 ger DE-627 rakwb eng 530 DNB 43.13 bkl 50.17 bkl 58.53 bkl Zhou, Ying verfasserin aut Facile synthesis of surface N-doped Bi2O2CO3: Origin of visible light photocatalytic activity and in situ DRIFTS studies 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier Bi2O2CO3 nanosheets with exposed {001} facets were prepared by a facile room temperature chemical method. Due to the high oxygen atom density in {001} facets of Bi2O2CO3, the addition of cetyltrimethylammonium bromide (CTAB) does not only influence the growth of crystalline Bi2O2CO3, but also modifies the surface properties of Bi2O2CO3 through the interaction between CTAB and Bi2O2CO3. Nitrogen from CTAB as dopant interstitially incorporates in the Bi2O2CO3 surface evidenced by both experimental and theoretical investigations. Hence, the formation of localized states from NO bond improves the visible light absorption and charge separation efficiency, which leads to an enhancement of visible light photocatalytic activity toward to the degradation of Rhodamine B (RhB) and oxidation of NO. In addition, the photocatalytic NO oxidation over Bi2O2CO3 nanosheets was successfully monitored for the first time using in situ diffuse reflectance infrared Fourier-transform spectroscopy (DRIFTS). Both bidentate and monodentate nitrates were identified on the surface of catalysts during the photocatalytic reaction process. The application of this strategy to another relevant bismuth based photocatalyst, BiOCl, demonstrated that surface interstitial N doping could also be achieved in this case. Therefore, our current route seems to be a general option to modify the surface properties of bismuth based photocatalysts. Nutzungsrecht: Copyright © 2016 Elsevier B.V. All rights reserved. Zhao, Ziyan oth Wang, Fang oth Cao, Kun oth Doronkin, Dmitry E oth Dong, Fan oth Grunwaldt, Jan-Dierk oth Enthalten in Journal of hazardous materials Amsterdam : Elsevier, 1975 307(2016), Seite 163-172 (DE-627)129442305 (DE-600)195278-X (DE-576)9129442303 0304-3894 nnns volume:307 year:2016 pages:163-172 http://dx.doi.org/10.1016/j.jhazmat.2015.12.072 Volltext http://www.ncbi.nlm.nih.gov/pubmed/26780703 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-UMW SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_70 43.13 AVZ 50.17 AVZ 58.53 AVZ AR 307 2016 163-172
allfieldsGer	10.1016/j.jhazmat.2015.12.072 doi PQ20160610 (DE-627)OLC1973494515 (DE-599)GBVOLC1973494515 (PRQ)c2232-a2ed9efdff4a13f95502ef4b7f43bc856d0d2f017478a9117fb8ca59457b4bc60 (KEY)0002474020160000307000000163facilesynthesisofsurfacendopedbi2o2co3originofvisi DE-627 ger DE-627 rakwb eng 530 DNB 43.13 bkl 50.17 bkl 58.53 bkl Zhou, Ying verfasserin aut Facile synthesis of surface N-doped Bi2O2CO3: Origin of visible light photocatalytic activity and in situ DRIFTS studies 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier Bi2O2CO3 nanosheets with exposed {001} facets were prepared by a facile room temperature chemical method. Due to the high oxygen atom density in {001} facets of Bi2O2CO3, the addition of cetyltrimethylammonium bromide (CTAB) does not only influence the growth of crystalline Bi2O2CO3, but also modifies the surface properties of Bi2O2CO3 through the interaction between CTAB and Bi2O2CO3. Nitrogen from CTAB as dopant interstitially incorporates in the Bi2O2CO3 surface evidenced by both experimental and theoretical investigations. Hence, the formation of localized states from NO bond improves the visible light absorption and charge separation efficiency, which leads to an enhancement of visible light photocatalytic activity toward to the degradation of Rhodamine B (RhB) and oxidation of NO. In addition, the photocatalytic NO oxidation over Bi2O2CO3 nanosheets was successfully monitored for the first time using in situ diffuse reflectance infrared Fourier-transform spectroscopy (DRIFTS). Both bidentate and monodentate nitrates were identified on the surface of catalysts during the photocatalytic reaction process. The application of this strategy to another relevant bismuth based photocatalyst, BiOCl, demonstrated that surface interstitial N doping could also be achieved in this case. Therefore, our current route seems to be a general option to modify the surface properties of bismuth based photocatalysts. Nutzungsrecht: Copyright © 2016 Elsevier B.V. All rights reserved. Zhao, Ziyan oth Wang, Fang oth Cao, Kun oth Doronkin, Dmitry E oth Dong, Fan oth Grunwaldt, Jan-Dierk oth Enthalten in Journal of hazardous materials Amsterdam : Elsevier, 1975 307(2016), Seite 163-172 (DE-627)129442305 (DE-600)195278-X (DE-576)9129442303 0304-3894 nnns volume:307 year:2016 pages:163-172 http://dx.doi.org/10.1016/j.jhazmat.2015.12.072 Volltext http://www.ncbi.nlm.nih.gov/pubmed/26780703 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-UMW SSG-OLC-TEC SSG-OLC-PHY GBV_ILN_70 43.13 AVZ 50.17 AVZ 58.53 AVZ AR 307 2016 163-172
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Due to the high oxygen atom density in {001} facets of Bi2O2CO3, the addition of cetyltrimethylammonium bromide (CTAB) does not only influence the growth of crystalline Bi2O2CO3, but also modifies the surface properties of Bi2O2CO3 through the interaction between CTAB and Bi2O2CO3. Nitrogen from CTAB as dopant interstitially incorporates in the Bi2O2CO3 surface evidenced by both experimental and theoretical investigations. Hence, the formation of localized states from NO bond improves the visible light absorption and charge separation efficiency, which leads to an enhancement of visible light photocatalytic activity toward to the degradation of Rhodamine B (RhB) and oxidation of NO. In addition, the photocatalytic NO oxidation over Bi2O2CO3 nanosheets was successfully monitored for the first time using in situ diffuse reflectance infrared Fourier-transform spectroscopy (DRIFTS). Both bidentate and monodentate nitrates were identified on the surface of catalysts during the photocatalytic reaction process. The application of this strategy to another relevant bismuth based photocatalyst, BiOCl, demonstrated that surface interstitial N doping could also be achieved in this case. Therefore, our current route seems to be a general option to modify the surface properties of bismuth based photocatalysts.</subfield></datafield><datafield tag="540" ind1=" " ind2=" "><subfield code="a">Nutzungsrecht: Copyright © 2016 Elsevier B.V. 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author	Zhou, Ying
spellingShingle	Zhou, Ying ddc 530 bkl 43.13 bkl 50.17 bkl 58.53 Facile synthesis of surface N-doped Bi2O2CO3: Origin of visible light photocatalytic activity and in situ DRIFTS studies
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topic_title	530 DNB 43.13 bkl 50.17 bkl 58.53 bkl Facile synthesis of surface N-doped Bi2O2CO3: Origin of visible light photocatalytic activity and in situ DRIFTS studies
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title	Facile synthesis of surface N-doped Bi2O2CO3: Origin of visible light photocatalytic activity and in situ DRIFTS studies
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title_full	Facile synthesis of surface N-doped Bi2O2CO3: Origin of visible light photocatalytic activity and in situ DRIFTS studies
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title_sort	facile synthesis of surface n-doped bi2o2co3: origin of visible light photocatalytic activity and in situ drifts studies
title_auth	Facile synthesis of surface N-doped Bi2O2CO3: Origin of visible light photocatalytic activity and in situ DRIFTS studies
abstract	Bi2O2CO3 nanosheets with exposed {001} facets were prepared by a facile room temperature chemical method. Due to the high oxygen atom density in {001} facets of Bi2O2CO3, the addition of cetyltrimethylammonium bromide (CTAB) does not only influence the growth of crystalline Bi2O2CO3, but also modifies the surface properties of Bi2O2CO3 through the interaction between CTAB and Bi2O2CO3. Nitrogen from CTAB as dopant interstitially incorporates in the Bi2O2CO3 surface evidenced by both experimental and theoretical investigations. Hence, the formation of localized states from NO bond improves the visible light absorption and charge separation efficiency, which leads to an enhancement of visible light photocatalytic activity toward to the degradation of Rhodamine B (RhB) and oxidation of NO. In addition, the photocatalytic NO oxidation over Bi2O2CO3 nanosheets was successfully monitored for the first time using in situ diffuse reflectance infrared Fourier-transform spectroscopy (DRIFTS). Both bidentate and monodentate nitrates were identified on the surface of catalysts during the photocatalytic reaction process. The application of this strategy to another relevant bismuth based photocatalyst, BiOCl, demonstrated that surface interstitial N doping could also be achieved in this case. Therefore, our current route seems to be a general option to modify the surface properties of bismuth based photocatalysts.
abstractGer	Bi2O2CO3 nanosheets with exposed {001} facets were prepared by a facile room temperature chemical method. Due to the high oxygen atom density in {001} facets of Bi2O2CO3, the addition of cetyltrimethylammonium bromide (CTAB) does not only influence the growth of crystalline Bi2O2CO3, but also modifies the surface properties of Bi2O2CO3 through the interaction between CTAB and Bi2O2CO3. Nitrogen from CTAB as dopant interstitially incorporates in the Bi2O2CO3 surface evidenced by both experimental and theoretical investigations. Hence, the formation of localized states from NO bond improves the visible light absorption and charge separation efficiency, which leads to an enhancement of visible light photocatalytic activity toward to the degradation of Rhodamine B (RhB) and oxidation of NO. In addition, the photocatalytic NO oxidation over Bi2O2CO3 nanosheets was successfully monitored for the first time using in situ diffuse reflectance infrared Fourier-transform spectroscopy (DRIFTS). Both bidentate and monodentate nitrates were identified on the surface of catalysts during the photocatalytic reaction process. The application of this strategy to another relevant bismuth based photocatalyst, BiOCl, demonstrated that surface interstitial N doping could also be achieved in this case. Therefore, our current route seems to be a general option to modify the surface properties of bismuth based photocatalysts.
abstract_unstemmed	Bi2O2CO3 nanosheets with exposed {001} facets were prepared by a facile room temperature chemical method. Due to the high oxygen atom density in {001} facets of Bi2O2CO3, the addition of cetyltrimethylammonium bromide (CTAB) does not only influence the growth of crystalline Bi2O2CO3, but also modifies the surface properties of Bi2O2CO3 through the interaction between CTAB and Bi2O2CO3. Nitrogen from CTAB as dopant interstitially incorporates in the Bi2O2CO3 surface evidenced by both experimental and theoretical investigations. Hence, the formation of localized states from NO bond improves the visible light absorption and charge separation efficiency, which leads to an enhancement of visible light photocatalytic activity toward to the degradation of Rhodamine B (RhB) and oxidation of NO. In addition, the photocatalytic NO oxidation over Bi2O2CO3 nanosheets was successfully monitored for the first time using in situ diffuse reflectance infrared Fourier-transform spectroscopy (DRIFTS). Both bidentate and monodentate nitrates were identified on the surface of catalysts during the photocatalytic reaction process. The application of this strategy to another relevant bismuth based photocatalyst, BiOCl, demonstrated that surface interstitial N doping could also be achieved in this case. Therefore, our current route seems to be a general option to modify the surface properties of bismuth based photocatalysts.
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title_short	Facile synthesis of surface N-doped Bi2O2CO3: Origin of visible light photocatalytic activity and in situ DRIFTS studies
url	http://dx.doi.org/10.1016/j.jhazmat.2015.12.072 http://www.ncbi.nlm.nih.gov/pubmed/26780703
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author2	Zhao, Ziyan Wang, Fang Cao, Kun Doronkin, Dmitry E Dong, Fan Grunwaldt, Jan-Dierk
author2Str	Zhao, Ziyan Wang, Fang Cao, Kun Doronkin, Dmitry E Dong, Fan Grunwaldt, Jan-Dierk
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doi_str	10.1016/j.jhazmat.2015.12.072
up_date	2024-07-04T02:34:05.604Z
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