Experimental simulation of bubble nucleation and magma ascent in basaltic systems: Implications for Stromboli volcano
The ascent of H O- and H O-CO -bearing basaltic melts from the deeper to the shallower part of the Stromboli magmatic system and their vesiculation were simulated from decompression experiments. A well-studied “golden” pumice produced during an intermediate- to a large-scale paroxysm was used as sta...
Ausführliche Beschreibung
Autor*in: |
Nolwenn Le Gall [verfasserIn] |
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Format: |
Artikel |
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Sprache: |
Englisch |
Erschienen: |
2016 |
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Schlagwörter: |
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Übergeordnetes Werk: |
Enthalten in: American mineralogist - Washington, DC [u.a.] : Soc., 1916, 101(2016), 9, Seite 1967-1985 |
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Übergeordnetes Werk: |
volume:101 ; year:2016 ; number:9 ; pages:1967-1985 |
Links: |
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DOI / URN: |
10.2138/am-2016-5639 |
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Katalog-ID: |
OLC1982561084 |
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520 | |a The ascent of H O- and H O-CO -bearing basaltic melts from the deeper to the shallower part of the Stromboli magmatic system and their vesiculation were simulated from decompression experiments. A well-studied “golden” pumice produced during an intermediate- to a large-scale paroxysm was used as starting material. Volatile-bearing glasses were synthesized at an oxygen fugacity ranging from NNO-1.4 to +0.9, 1200 °C and 200 MPa. The resulting crystal- and bubble-free glasses were then isothermally (1200 °C) decompressed to final pressures ranging between 200 and 25 MPa, at a linear ascent rate of 1.5 m/s (or 39 kPa/s) prior to be rapidly quenched. Textures of post-decompression glasses that were characterized by X-ray computed tomography result from different mechanisms of degassing that include bubble nucleation, growth, coalescence, and outgassing, as well as fragmentation. Homogeneous bubble nucleation occurs for supersaturation pressures (difference between saturation pressure and pressure at which bubbles start to form homogeneously, Δ ) ≤ 50 MPa. In the CO -free melts, homogeneous nucleation occurs as two distinct events, the first at high (200–150 MPa) and the second at low (50–25 MPa) near the fragmentation level. In contrast, in the CO -bearing melts, multiple events of homogeneous bubble nucleation occur over a substantial interval along the decompression path. Bubble coalescence occurs in both H O- and H O-CO -bearing melts and is the more strongly marked between 100 and 50 MPa P . The CO -free melts follow equilibrium degassing until 100 MPa and are slightly supersaturated at 60 and 50 MPa , thus providing the driving force for the second bubble nucleation event. In comparison, disequilibrium degassing occurs systematically in the CO -bearing melts that retain high CO concentrations. Fragmentation was observed in some CO2-free charges decompressed to 25 MPa and is intimately associated with the occurrence of the second bubble nucleation event. Textures of H O-CO -bearing glasses reproduce certain critical aspects of the Stromboli natural textures (bubble number densities, shapes, sizes, and distributions) and chemistries (residual volatile concentrations). Average bubble sizes, bubble size distribution (BSD), and bubble number density (BND) data are used together to estimate that the “golden” pumice magmas ascend from their source region in 43 to 128 min. | ||
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10.2138/am-2016-5639 doi PQ20161012 (DE-627)OLC1982561084 (DE-599)GBVOLC1982561084 (PRQ)c907-8f93a9ed415b6baa77c183c5490a3542df7aee48c79ccc0331044c6c4b4672580 (KEY)0120180820160000101000901967experimentalsimulationofbubblenucleationandmagmaas DE-627 ger DE-627 rakwb eng 550 540 DNB 38.30 bkl Nolwenn Le Gall verfasserin aut Experimental simulation of bubble nucleation and magma ascent in basaltic systems: Implications for Stromboli volcano 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The ascent of H O- and H O-CO -bearing basaltic melts from the deeper to the shallower part of the Stromboli magmatic system and their vesiculation were simulated from decompression experiments. A well-studied “golden” pumice produced during an intermediate- to a large-scale paroxysm was used as starting material. Volatile-bearing glasses were synthesized at an oxygen fugacity ranging from NNO-1.4 to +0.9, 1200 °C and 200 MPa. The resulting crystal- and bubble-free glasses were then isothermally (1200 °C) decompressed to final pressures ranging between 200 and 25 MPa, at a linear ascent rate of 1.5 m/s (or 39 kPa/s) prior to be rapidly quenched. Textures of post-decompression glasses that were characterized by X-ray computed tomography result from different mechanisms of degassing that include bubble nucleation, growth, coalescence, and outgassing, as well as fragmentation. Homogeneous bubble nucleation occurs for supersaturation pressures (difference between saturation pressure and pressure at which bubbles start to form homogeneously, Δ ) ≤ 50 MPa. In the CO -free melts, homogeneous nucleation occurs as two distinct events, the first at high (200–150 MPa) and the second at low (50–25 MPa) near the fragmentation level. In contrast, in the CO -bearing melts, multiple events of homogeneous bubble nucleation occur over a substantial interval along the decompression path. Bubble coalescence occurs in both H O- and H O-CO -bearing melts and is the more strongly marked between 100 and 50 MPa P . The CO -free melts follow equilibrium degassing until 100 MPa and are slightly supersaturated at 60 and 50 MPa , thus providing the driving force for the second bubble nucleation event. In comparison, disequilibrium degassing occurs systematically in the CO -bearing melts that retain high CO concentrations. Fragmentation was observed in some CO2-free charges decompressed to 25 MPa and is intimately associated with the occurrence of the second bubble nucleation event. Textures of H O-CO -bearing glasses reproduce certain critical aspects of the Stromboli natural textures (bubble number densities, shapes, sizes, and distributions) and chemistries (residual volatile concentrations). Average bubble sizes, bubble size distribution (BSD), and bubble number density (BND) data are used together to estimate that the “golden” pumice magmas ascend from their source region in 43 to 128 min. volatiles fragmentation bubble nucleation magma ascent Stromboli magma degassing Basalt Michel Pichavant oth Enthalten in American mineralogist Washington, DC [u.a.] : Soc., 1916 101(2016), 9, Seite 1967-1985 (DE-627)129081795 (DE-600)3514-2 (DE-576)014414716 0003-004X nnns volume:101 year:2016 number:9 pages:1967-1985 http://dx.doi.org/10.2138/am-2016-5639 Volltext http://www.degruyter.com/doi/10.2138/am-2016-5639 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-CHE SSG-OLC-GEO SSG-OLC-PHA SSG-OLC-DE-84 SSG-OPC-GGO GBV_ILN_21 GBV_ILN_22 GBV_ILN_40 GBV_ILN_65 GBV_ILN_70 GBV_ILN_188 GBV_ILN_2010 GBV_ILN_2015 GBV_ILN_4012 GBV_ILN_4112 GBV_ILN_4323 38.30 AVZ AR 101 2016 9 1967-1985 |
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10.2138/am-2016-5639 doi PQ20161012 (DE-627)OLC1982561084 (DE-599)GBVOLC1982561084 (PRQ)c907-8f93a9ed415b6baa77c183c5490a3542df7aee48c79ccc0331044c6c4b4672580 (KEY)0120180820160000101000901967experimentalsimulationofbubblenucleationandmagmaas DE-627 ger DE-627 rakwb eng 550 540 DNB 38.30 bkl Nolwenn Le Gall verfasserin aut Experimental simulation of bubble nucleation and magma ascent in basaltic systems: Implications for Stromboli volcano 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The ascent of H O- and H O-CO -bearing basaltic melts from the deeper to the shallower part of the Stromboli magmatic system and their vesiculation were simulated from decompression experiments. A well-studied “golden” pumice produced during an intermediate- to a large-scale paroxysm was used as starting material. Volatile-bearing glasses were synthesized at an oxygen fugacity ranging from NNO-1.4 to +0.9, 1200 °C and 200 MPa. The resulting crystal- and bubble-free glasses were then isothermally (1200 °C) decompressed to final pressures ranging between 200 and 25 MPa, at a linear ascent rate of 1.5 m/s (or 39 kPa/s) prior to be rapidly quenched. Textures of post-decompression glasses that were characterized by X-ray computed tomography result from different mechanisms of degassing that include bubble nucleation, growth, coalescence, and outgassing, as well as fragmentation. Homogeneous bubble nucleation occurs for supersaturation pressures (difference between saturation pressure and pressure at which bubbles start to form homogeneously, Δ ) ≤ 50 MPa. In the CO -free melts, homogeneous nucleation occurs as two distinct events, the first at high (200–150 MPa) and the second at low (50–25 MPa) near the fragmentation level. In contrast, in the CO -bearing melts, multiple events of homogeneous bubble nucleation occur over a substantial interval along the decompression path. Bubble coalescence occurs in both H O- and H O-CO -bearing melts and is the more strongly marked between 100 and 50 MPa P . The CO -free melts follow equilibrium degassing until 100 MPa and are slightly supersaturated at 60 and 50 MPa , thus providing the driving force for the second bubble nucleation event. In comparison, disequilibrium degassing occurs systematically in the CO -bearing melts that retain high CO concentrations. Fragmentation was observed in some CO2-free charges decompressed to 25 MPa and is intimately associated with the occurrence of the second bubble nucleation event. Textures of H O-CO -bearing glasses reproduce certain critical aspects of the Stromboli natural textures (bubble number densities, shapes, sizes, and distributions) and chemistries (residual volatile concentrations). Average bubble sizes, bubble size distribution (BSD), and bubble number density (BND) data are used together to estimate that the “golden” pumice magmas ascend from their source region in 43 to 128 min. volatiles fragmentation bubble nucleation magma ascent Stromboli magma degassing Basalt Michel Pichavant oth Enthalten in American mineralogist Washington, DC [u.a.] : Soc., 1916 101(2016), 9, Seite 1967-1985 (DE-627)129081795 (DE-600)3514-2 (DE-576)014414716 0003-004X nnns volume:101 year:2016 number:9 pages:1967-1985 http://dx.doi.org/10.2138/am-2016-5639 Volltext http://www.degruyter.com/doi/10.2138/am-2016-5639 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-CHE SSG-OLC-GEO SSG-OLC-PHA SSG-OLC-DE-84 SSG-OPC-GGO GBV_ILN_21 GBV_ILN_22 GBV_ILN_40 GBV_ILN_65 GBV_ILN_70 GBV_ILN_188 GBV_ILN_2010 GBV_ILN_2015 GBV_ILN_4012 GBV_ILN_4112 GBV_ILN_4323 38.30 AVZ AR 101 2016 9 1967-1985 |
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10.2138/am-2016-5639 doi PQ20161012 (DE-627)OLC1982561084 (DE-599)GBVOLC1982561084 (PRQ)c907-8f93a9ed415b6baa77c183c5490a3542df7aee48c79ccc0331044c6c4b4672580 (KEY)0120180820160000101000901967experimentalsimulationofbubblenucleationandmagmaas DE-627 ger DE-627 rakwb eng 550 540 DNB 38.30 bkl Nolwenn Le Gall verfasserin aut Experimental simulation of bubble nucleation and magma ascent in basaltic systems: Implications for Stromboli volcano 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The ascent of H O- and H O-CO -bearing basaltic melts from the deeper to the shallower part of the Stromboli magmatic system and their vesiculation were simulated from decompression experiments. A well-studied “golden” pumice produced during an intermediate- to a large-scale paroxysm was used as starting material. Volatile-bearing glasses were synthesized at an oxygen fugacity ranging from NNO-1.4 to +0.9, 1200 °C and 200 MPa. The resulting crystal- and bubble-free glasses were then isothermally (1200 °C) decompressed to final pressures ranging between 200 and 25 MPa, at a linear ascent rate of 1.5 m/s (or 39 kPa/s) prior to be rapidly quenched. Textures of post-decompression glasses that were characterized by X-ray computed tomography result from different mechanisms of degassing that include bubble nucleation, growth, coalescence, and outgassing, as well as fragmentation. Homogeneous bubble nucleation occurs for supersaturation pressures (difference between saturation pressure and pressure at which bubbles start to form homogeneously, Δ ) ≤ 50 MPa. In the CO -free melts, homogeneous nucleation occurs as two distinct events, the first at high (200–150 MPa) and the second at low (50–25 MPa) near the fragmentation level. In contrast, in the CO -bearing melts, multiple events of homogeneous bubble nucleation occur over a substantial interval along the decompression path. Bubble coalescence occurs in both H O- and H O-CO -bearing melts and is the more strongly marked between 100 and 50 MPa P . The CO -free melts follow equilibrium degassing until 100 MPa and are slightly supersaturated at 60 and 50 MPa , thus providing the driving force for the second bubble nucleation event. In comparison, disequilibrium degassing occurs systematically in the CO -bearing melts that retain high CO concentrations. Fragmentation was observed in some CO2-free charges decompressed to 25 MPa and is intimately associated with the occurrence of the second bubble nucleation event. Textures of H O-CO -bearing glasses reproduce certain critical aspects of the Stromboli natural textures (bubble number densities, shapes, sizes, and distributions) and chemistries (residual volatile concentrations). Average bubble sizes, bubble size distribution (BSD), and bubble number density (BND) data are used together to estimate that the “golden” pumice magmas ascend from their source region in 43 to 128 min. volatiles fragmentation bubble nucleation magma ascent Stromboli magma degassing Basalt Michel Pichavant oth Enthalten in American mineralogist Washington, DC [u.a.] : Soc., 1916 101(2016), 9, Seite 1967-1985 (DE-627)129081795 (DE-600)3514-2 (DE-576)014414716 0003-004X nnns volume:101 year:2016 number:9 pages:1967-1985 http://dx.doi.org/10.2138/am-2016-5639 Volltext http://www.degruyter.com/doi/10.2138/am-2016-5639 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-CHE SSG-OLC-GEO SSG-OLC-PHA SSG-OLC-DE-84 SSG-OPC-GGO GBV_ILN_21 GBV_ILN_22 GBV_ILN_40 GBV_ILN_65 GBV_ILN_70 GBV_ILN_188 GBV_ILN_2010 GBV_ILN_2015 GBV_ILN_4012 GBV_ILN_4112 GBV_ILN_4323 38.30 AVZ AR 101 2016 9 1967-1985 |
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10.2138/am-2016-5639 doi PQ20161012 (DE-627)OLC1982561084 (DE-599)GBVOLC1982561084 (PRQ)c907-8f93a9ed415b6baa77c183c5490a3542df7aee48c79ccc0331044c6c4b4672580 (KEY)0120180820160000101000901967experimentalsimulationofbubblenucleationandmagmaas DE-627 ger DE-627 rakwb eng 550 540 DNB 38.30 bkl Nolwenn Le Gall verfasserin aut Experimental simulation of bubble nucleation and magma ascent in basaltic systems: Implications for Stromboli volcano 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The ascent of H O- and H O-CO -bearing basaltic melts from the deeper to the shallower part of the Stromboli magmatic system and their vesiculation were simulated from decompression experiments. A well-studied “golden” pumice produced during an intermediate- to a large-scale paroxysm was used as starting material. Volatile-bearing glasses were synthesized at an oxygen fugacity ranging from NNO-1.4 to +0.9, 1200 °C and 200 MPa. The resulting crystal- and bubble-free glasses were then isothermally (1200 °C) decompressed to final pressures ranging between 200 and 25 MPa, at a linear ascent rate of 1.5 m/s (or 39 kPa/s) prior to be rapidly quenched. Textures of post-decompression glasses that were characterized by X-ray computed tomography result from different mechanisms of degassing that include bubble nucleation, growth, coalescence, and outgassing, as well as fragmentation. Homogeneous bubble nucleation occurs for supersaturation pressures (difference between saturation pressure and pressure at which bubbles start to form homogeneously, Δ ) ≤ 50 MPa. In the CO -free melts, homogeneous nucleation occurs as two distinct events, the first at high (200–150 MPa) and the second at low (50–25 MPa) near the fragmentation level. In contrast, in the CO -bearing melts, multiple events of homogeneous bubble nucleation occur over a substantial interval along the decompression path. Bubble coalescence occurs in both H O- and H O-CO -bearing melts and is the more strongly marked between 100 and 50 MPa P . The CO -free melts follow equilibrium degassing until 100 MPa and are slightly supersaturated at 60 and 50 MPa , thus providing the driving force for the second bubble nucleation event. In comparison, disequilibrium degassing occurs systematically in the CO -bearing melts that retain high CO concentrations. Fragmentation was observed in some CO2-free charges decompressed to 25 MPa and is intimately associated with the occurrence of the second bubble nucleation event. Textures of H O-CO -bearing glasses reproduce certain critical aspects of the Stromboli natural textures (bubble number densities, shapes, sizes, and distributions) and chemistries (residual volatile concentrations). Average bubble sizes, bubble size distribution (BSD), and bubble number density (BND) data are used together to estimate that the “golden” pumice magmas ascend from their source region in 43 to 128 min. volatiles fragmentation bubble nucleation magma ascent Stromboli magma degassing Basalt Michel Pichavant oth Enthalten in American mineralogist Washington, DC [u.a.] : Soc., 1916 101(2016), 9, Seite 1967-1985 (DE-627)129081795 (DE-600)3514-2 (DE-576)014414716 0003-004X nnns volume:101 year:2016 number:9 pages:1967-1985 http://dx.doi.org/10.2138/am-2016-5639 Volltext http://www.degruyter.com/doi/10.2138/am-2016-5639 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-CHE SSG-OLC-GEO SSG-OLC-PHA SSG-OLC-DE-84 SSG-OPC-GGO GBV_ILN_21 GBV_ILN_22 GBV_ILN_40 GBV_ILN_65 GBV_ILN_70 GBV_ILN_188 GBV_ILN_2010 GBV_ILN_2015 GBV_ILN_4012 GBV_ILN_4112 GBV_ILN_4323 38.30 AVZ AR 101 2016 9 1967-1985 |
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10.2138/am-2016-5639 doi PQ20161012 (DE-627)OLC1982561084 (DE-599)GBVOLC1982561084 (PRQ)c907-8f93a9ed415b6baa77c183c5490a3542df7aee48c79ccc0331044c6c4b4672580 (KEY)0120180820160000101000901967experimentalsimulationofbubblenucleationandmagmaas DE-627 ger DE-627 rakwb eng 550 540 DNB 38.30 bkl Nolwenn Le Gall verfasserin aut Experimental simulation of bubble nucleation and magma ascent in basaltic systems: Implications for Stromboli volcano 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The ascent of H O- and H O-CO -bearing basaltic melts from the deeper to the shallower part of the Stromboli magmatic system and their vesiculation were simulated from decompression experiments. A well-studied “golden” pumice produced during an intermediate- to a large-scale paroxysm was used as starting material. Volatile-bearing glasses were synthesized at an oxygen fugacity ranging from NNO-1.4 to +0.9, 1200 °C and 200 MPa. The resulting crystal- and bubble-free glasses were then isothermally (1200 °C) decompressed to final pressures ranging between 200 and 25 MPa, at a linear ascent rate of 1.5 m/s (or 39 kPa/s) prior to be rapidly quenched. Textures of post-decompression glasses that were characterized by X-ray computed tomography result from different mechanisms of degassing that include bubble nucleation, growth, coalescence, and outgassing, as well as fragmentation. Homogeneous bubble nucleation occurs for supersaturation pressures (difference between saturation pressure and pressure at which bubbles start to form homogeneously, Δ ) ≤ 50 MPa. In the CO -free melts, homogeneous nucleation occurs as two distinct events, the first at high (200–150 MPa) and the second at low (50–25 MPa) near the fragmentation level. In contrast, in the CO -bearing melts, multiple events of homogeneous bubble nucleation occur over a substantial interval along the decompression path. Bubble coalescence occurs in both H O- and H O-CO -bearing melts and is the more strongly marked between 100 and 50 MPa P . The CO -free melts follow equilibrium degassing until 100 MPa and are slightly supersaturated at 60 and 50 MPa , thus providing the driving force for the second bubble nucleation event. In comparison, disequilibrium degassing occurs systematically in the CO -bearing melts that retain high CO concentrations. Fragmentation was observed in some CO2-free charges decompressed to 25 MPa and is intimately associated with the occurrence of the second bubble nucleation event. Textures of H O-CO -bearing glasses reproduce certain critical aspects of the Stromboli natural textures (bubble number densities, shapes, sizes, and distributions) and chemistries (residual volatile concentrations). Average bubble sizes, bubble size distribution (BSD), and bubble number density (BND) data are used together to estimate that the “golden” pumice magmas ascend from their source region in 43 to 128 min. volatiles fragmentation bubble nucleation magma ascent Stromboli magma degassing Basalt Michel Pichavant oth Enthalten in American mineralogist Washington, DC [u.a.] : Soc., 1916 101(2016), 9, Seite 1967-1985 (DE-627)129081795 (DE-600)3514-2 (DE-576)014414716 0003-004X nnns volume:101 year:2016 number:9 pages:1967-1985 http://dx.doi.org/10.2138/am-2016-5639 Volltext http://www.degruyter.com/doi/10.2138/am-2016-5639 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-CHE SSG-OLC-GEO SSG-OLC-PHA SSG-OLC-DE-84 SSG-OPC-GGO GBV_ILN_21 GBV_ILN_22 GBV_ILN_40 GBV_ILN_65 GBV_ILN_70 GBV_ILN_188 GBV_ILN_2010 GBV_ILN_2015 GBV_ILN_4012 GBV_ILN_4112 GBV_ILN_4323 38.30 AVZ AR 101 2016 9 1967-1985 |
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550 540 DNB 38.30 bkl Experimental simulation of bubble nucleation and magma ascent in basaltic systems: Implications for Stromboli volcano volatiles fragmentation bubble nucleation magma ascent Stromboli magma degassing Basalt |
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Experimental simulation of bubble nucleation and magma ascent in basaltic systems: Implications for Stromboli volcano |
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Experimental simulation of bubble nucleation and magma ascent in basaltic systems: Implications for Stromboli volcano |
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experimental simulation of bubble nucleation and magma ascent in basaltic systems: implications for stromboli volcano |
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Experimental simulation of bubble nucleation and magma ascent in basaltic systems: Implications for Stromboli volcano |
abstract |
The ascent of H O- and H O-CO -bearing basaltic melts from the deeper to the shallower part of the Stromboli magmatic system and their vesiculation were simulated from decompression experiments. A well-studied “golden” pumice produced during an intermediate- to a large-scale paroxysm was used as starting material. Volatile-bearing glasses were synthesized at an oxygen fugacity ranging from NNO-1.4 to +0.9, 1200 °C and 200 MPa. The resulting crystal- and bubble-free glasses were then isothermally (1200 °C) decompressed to final pressures ranging between 200 and 25 MPa, at a linear ascent rate of 1.5 m/s (or 39 kPa/s) prior to be rapidly quenched. Textures of post-decompression glasses that were characterized by X-ray computed tomography result from different mechanisms of degassing that include bubble nucleation, growth, coalescence, and outgassing, as well as fragmentation. Homogeneous bubble nucleation occurs for supersaturation pressures (difference between saturation pressure and pressure at which bubbles start to form homogeneously, Δ ) ≤ 50 MPa. In the CO -free melts, homogeneous nucleation occurs as two distinct events, the first at high (200–150 MPa) and the second at low (50–25 MPa) near the fragmentation level. In contrast, in the CO -bearing melts, multiple events of homogeneous bubble nucleation occur over a substantial interval along the decompression path. Bubble coalescence occurs in both H O- and H O-CO -bearing melts and is the more strongly marked between 100 and 50 MPa P . The CO -free melts follow equilibrium degassing until 100 MPa and are slightly supersaturated at 60 and 50 MPa , thus providing the driving force for the second bubble nucleation event. In comparison, disequilibrium degassing occurs systematically in the CO -bearing melts that retain high CO concentrations. Fragmentation was observed in some CO2-free charges decompressed to 25 MPa and is intimately associated with the occurrence of the second bubble nucleation event. Textures of H O-CO -bearing glasses reproduce certain critical aspects of the Stromboli natural textures (bubble number densities, shapes, sizes, and distributions) and chemistries (residual volatile concentrations). Average bubble sizes, bubble size distribution (BSD), and bubble number density (BND) data are used together to estimate that the “golden” pumice magmas ascend from their source region in 43 to 128 min. |
abstractGer |
The ascent of H O- and H O-CO -bearing basaltic melts from the deeper to the shallower part of the Stromboli magmatic system and their vesiculation were simulated from decompression experiments. A well-studied “golden” pumice produced during an intermediate- to a large-scale paroxysm was used as starting material. Volatile-bearing glasses were synthesized at an oxygen fugacity ranging from NNO-1.4 to +0.9, 1200 °C and 200 MPa. The resulting crystal- and bubble-free glasses were then isothermally (1200 °C) decompressed to final pressures ranging between 200 and 25 MPa, at a linear ascent rate of 1.5 m/s (or 39 kPa/s) prior to be rapidly quenched. Textures of post-decompression glasses that were characterized by X-ray computed tomography result from different mechanisms of degassing that include bubble nucleation, growth, coalescence, and outgassing, as well as fragmentation. Homogeneous bubble nucleation occurs for supersaturation pressures (difference between saturation pressure and pressure at which bubbles start to form homogeneously, Δ ) ≤ 50 MPa. In the CO -free melts, homogeneous nucleation occurs as two distinct events, the first at high (200–150 MPa) and the second at low (50–25 MPa) near the fragmentation level. In contrast, in the CO -bearing melts, multiple events of homogeneous bubble nucleation occur over a substantial interval along the decompression path. Bubble coalescence occurs in both H O- and H O-CO -bearing melts and is the more strongly marked between 100 and 50 MPa P . The CO -free melts follow equilibrium degassing until 100 MPa and are slightly supersaturated at 60 and 50 MPa , thus providing the driving force for the second bubble nucleation event. In comparison, disequilibrium degassing occurs systematically in the CO -bearing melts that retain high CO concentrations. Fragmentation was observed in some CO2-free charges decompressed to 25 MPa and is intimately associated with the occurrence of the second bubble nucleation event. Textures of H O-CO -bearing glasses reproduce certain critical aspects of the Stromboli natural textures (bubble number densities, shapes, sizes, and distributions) and chemistries (residual volatile concentrations). Average bubble sizes, bubble size distribution (BSD), and bubble number density (BND) data are used together to estimate that the “golden” pumice magmas ascend from their source region in 43 to 128 min. |
abstract_unstemmed |
The ascent of H O- and H O-CO -bearing basaltic melts from the deeper to the shallower part of the Stromboli magmatic system and their vesiculation were simulated from decompression experiments. A well-studied “golden” pumice produced during an intermediate- to a large-scale paroxysm was used as starting material. Volatile-bearing glasses were synthesized at an oxygen fugacity ranging from NNO-1.4 to +0.9, 1200 °C and 200 MPa. The resulting crystal- and bubble-free glasses were then isothermally (1200 °C) decompressed to final pressures ranging between 200 and 25 MPa, at a linear ascent rate of 1.5 m/s (or 39 kPa/s) prior to be rapidly quenched. Textures of post-decompression glasses that were characterized by X-ray computed tomography result from different mechanisms of degassing that include bubble nucleation, growth, coalescence, and outgassing, as well as fragmentation. Homogeneous bubble nucleation occurs for supersaturation pressures (difference between saturation pressure and pressure at which bubbles start to form homogeneously, Δ ) ≤ 50 MPa. In the CO -free melts, homogeneous nucleation occurs as two distinct events, the first at high (200–150 MPa) and the second at low (50–25 MPa) near the fragmentation level. In contrast, in the CO -bearing melts, multiple events of homogeneous bubble nucleation occur over a substantial interval along the decompression path. Bubble coalescence occurs in both H O- and H O-CO -bearing melts and is the more strongly marked between 100 and 50 MPa P . The CO -free melts follow equilibrium degassing until 100 MPa and are slightly supersaturated at 60 and 50 MPa , thus providing the driving force for the second bubble nucleation event. In comparison, disequilibrium degassing occurs systematically in the CO -bearing melts that retain high CO concentrations. Fragmentation was observed in some CO2-free charges decompressed to 25 MPa and is intimately associated with the occurrence of the second bubble nucleation event. Textures of H O-CO -bearing glasses reproduce certain critical aspects of the Stromboli natural textures (bubble number densities, shapes, sizes, and distributions) and chemistries (residual volatile concentrations). Average bubble sizes, bubble size distribution (BSD), and bubble number density (BND) data are used together to estimate that the “golden” pumice magmas ascend from their source region in 43 to 128 min. |
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title_short |
Experimental simulation of bubble nucleation and magma ascent in basaltic systems: Implications for Stromboli volcano |
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In the CO -free melts, homogeneous nucleation occurs as two distinct events, the first at high (200–150 MPa) and the second at low (50–25 MPa) near the fragmentation level. In contrast, in the CO -bearing melts, multiple events of homogeneous bubble nucleation occur over a substantial interval along the decompression path. Bubble coalescence occurs in both H O- and H O-CO -bearing melts and is the more strongly marked between 100 and 50 MPa P . The CO -free melts follow equilibrium degassing until 100 MPa and are slightly supersaturated at 60 and 50 MPa , thus providing the driving force for the second bubble nucleation event. In comparison, disequilibrium degassing occurs systematically in the CO -bearing melts that retain high CO concentrations. Fragmentation was observed in some CO2-free charges decompressed to 25 MPa and is intimately associated with the occurrence of the second bubble nucleation event. Textures of H O-CO -bearing glasses reproduce certain critical aspects of the Stromboli natural textures (bubble number densities, shapes, sizes, and distributions) and chemistries (residual volatile concentrations). Average bubble sizes, bubble size distribution (BSD), and bubble number density (BND) data are used together to estimate that the “golden” pumice magmas ascend from their source region in 43 to 128 min.</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">volatiles</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">fragmentation</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">bubble nucleation</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">magma ascent</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Stromboli</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">magma degassing</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Basalt</subfield></datafield><datafield tag="700" ind1="0" ind2=" "><subfield code="a">Michel Pichavant</subfield><subfield code="4">oth</subfield></datafield><datafield tag="773" ind1="0" ind2="8"><subfield code="i">Enthalten in</subfield><subfield code="t">American mineralogist</subfield><subfield code="d">Washington, DC [u.a.] : Soc., 1916</subfield><subfield code="g">101(2016), 9, Seite 1967-1985</subfield><subfield code="w">(DE-627)129081795</subfield><subfield code="w">(DE-600)3514-2</subfield><subfield code="w">(DE-576)014414716</subfield><subfield code="x">0003-004X</subfield><subfield code="7">nnns</subfield></datafield><datafield tag="773" ind1="1" ind2="8"><subfield code="g">volume:101</subfield><subfield code="g">year:2016</subfield><subfield code="g">number:9</subfield><subfield code="g">pages:1967-1985</subfield></datafield><datafield tag="856" ind1="4" ind2="1"><subfield code="u">http://dx.doi.org/10.2138/am-2016-5639</subfield><subfield code="3">Volltext</subfield></datafield><datafield tag="856" ind1="4" ind2="2"><subfield code="u">http://www.degruyter.com/doi/10.2138/am-2016-5639</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_USEFLAG_A</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SYSFLAG_A</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_OLC</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SSG-OLC-CHE</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SSG-OLC-GEO</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SSG-OLC-PHA</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SSG-OLC-DE-84</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SSG-OPC-GGO</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_21</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_22</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_40</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_65</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_70</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_188</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2010</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2015</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4012</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4112</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4323</subfield></datafield><datafield tag="936" ind1="b" ind2="k"><subfield code="a">38.30</subfield><subfield code="q">AVZ</subfield></datafield><datafield tag="951" ind1=" " ind2=" "><subfield code="a">AR</subfield></datafield><datafield tag="952" ind1=" " ind2=" "><subfield code="d">101</subfield><subfield code="j">2016</subfield><subfield code="e">9</subfield><subfield code="h">1967-1985</subfield></datafield></record></collection>
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