Atomic‐Scale Origin of Long‐Term Stability and High Performance of p‐GaN Nanowire Arrays for Photocatalytic Overall Pure Water Splitting
The atomic‐scale origin of the unusually high performance and long‐term stability of wurtzite p ‐GaN oriented nanowire arrays is revealed. Nitrogen termination of both the polar ( 000 1 ¯ ) top face and the nonpolar ( 10 1 ¯ 0 ) side faces of the nanowires is essential for long‐term stability and hi...
Ausführliche Beschreibung
Autor*in: |
Kibria, Md Golam [verfasserIn] |
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Artikel |
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Sprache: |
Englisch |
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2016 |
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Rechteinformationen: |
Nutzungsrecht: © 2016 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim |
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Schlagwörter: |
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Systematik: |
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Übergeordnetes Werk: |
Enthalten in: Advanced materials - Weinheim : Wiley-VCH Verl., 1988, 28(2016), 38, Seite 8388-8397 |
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Übergeordnetes Werk: |
volume:28 ; year:2016 ; number:38 ; pages:8388-8397 |
Links: |
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DOI / URN: |
10.1002/adma.201602274 |
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Katalog-ID: |
OLC198299780X |
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520 | |a The atomic‐scale origin of the unusually high performance and long‐term stability of wurtzite p ‐GaN oriented nanowire arrays is revealed. Nitrogen termination of both the polar ( 000 1 ¯ ) top face and the nonpolar ( 10 1 ¯ 0 ) side faces of the nanowires is essential for long‐term stability and high efficiency. Such a distinct atomic configuration ensures not only stability against (photo) oxidation in air and in water/electrolyte but, as importantly, also provides the necessary overall reverse crystal polarization needed for efficient hole extraction in p ‐GaN. | ||
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650 | 4 | |a wurtzite structure | |
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10.1002/adma.201602274 doi PQ20161012 (DE-627)OLC198299780X (DE-599)GBVOLC198299780X (PRQ)wiley_primary_10_1002_adma_201602274_ADMA2016022743 (KEY)0178503620160000028003808388atomicscaleoriginoflongtermstabilityandhighperform DE-627 ger DE-627 rakwb eng 620 540 DE-101 540 AVZ UA 1538 AVZ rvk Kibria, Md Golam verfasserin aut Atomic‐Scale Origin of Long‐Term Stability and High Performance of p‐GaN Nanowire Arrays for Photocatalytic Overall Pure Water Splitting 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The atomic‐scale origin of the unusually high performance and long‐term stability of wurtzite p ‐GaN oriented nanowire arrays is revealed. Nitrogen termination of both the polar ( 000 1 ¯ ) top face and the nonpolar ( 10 1 ¯ 0 ) side faces of the nanowires is essential for long‐term stability and high efficiency. Such a distinct atomic configuration ensures not only stability against (photo) oxidation in air and in water/electrolyte but, as importantly, also provides the necessary overall reverse crystal polarization needed for efficient hole extraction in p ‐GaN. Nutzungsrecht: © 2016 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim wurtzite structure artificial photosynthesis polarization dependence X‐ray spectroscopy metal nitride N‐terminated surfaces Qiao, Ruimin oth Yang, Wanli oth Boukahil, Idris oth Kong, Xianghua oth Chowdhury, Faqrul Alam oth Trudeau, Michel L oth Ji, Wei oth Guo, Hong oth Himpsel, F. J oth Vayssieres, Lionel oth Mi, Zetian oth Enthalten in Advanced materials Weinheim : Wiley-VCH Verl., 1988 28(2016), 38, Seite 8388-8397 (DE-627)130815152 (DE-600)1012489-5 (DE-576)023057149 0935-9648 nnns volume:28 year:2016 number:38 pages:8388-8397 http://dx.doi.org/10.1002/adma.201602274 Volltext http://onlinelibrary.wiley.com/doi/10.1002/adma.201602274/abstract GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-DE-84 GBV_ILN_70 GBV_ILN_95 GBV_ILN_267 GBV_ILN_2004 GBV_ILN_2016 GBV_ILN_2018 GBV_ILN_2095 GBV_ILN_4012 GBV_ILN_4306 UA 1538 AR 28 2016 38 8388-8397 |
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10.1002/adma.201602274 doi PQ20161012 (DE-627)OLC198299780X (DE-599)GBVOLC198299780X (PRQ)wiley_primary_10_1002_adma_201602274_ADMA2016022743 (KEY)0178503620160000028003808388atomicscaleoriginoflongtermstabilityandhighperform DE-627 ger DE-627 rakwb eng 620 540 DE-101 540 AVZ UA 1538 AVZ rvk Kibria, Md Golam verfasserin aut Atomic‐Scale Origin of Long‐Term Stability and High Performance of p‐GaN Nanowire Arrays for Photocatalytic Overall Pure Water Splitting 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The atomic‐scale origin of the unusually high performance and long‐term stability of wurtzite p ‐GaN oriented nanowire arrays is revealed. Nitrogen termination of both the polar ( 000 1 ¯ ) top face and the nonpolar ( 10 1 ¯ 0 ) side faces of the nanowires is essential for long‐term stability and high efficiency. Such a distinct atomic configuration ensures not only stability against (photo) oxidation in air and in water/electrolyte but, as importantly, also provides the necessary overall reverse crystal polarization needed for efficient hole extraction in p ‐GaN. Nutzungsrecht: © 2016 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim wurtzite structure artificial photosynthesis polarization dependence X‐ray spectroscopy metal nitride N‐terminated surfaces Qiao, Ruimin oth Yang, Wanli oth Boukahil, Idris oth Kong, Xianghua oth Chowdhury, Faqrul Alam oth Trudeau, Michel L oth Ji, Wei oth Guo, Hong oth Himpsel, F. J oth Vayssieres, Lionel oth Mi, Zetian oth Enthalten in Advanced materials Weinheim : Wiley-VCH Verl., 1988 28(2016), 38, Seite 8388-8397 (DE-627)130815152 (DE-600)1012489-5 (DE-576)023057149 0935-9648 nnns volume:28 year:2016 number:38 pages:8388-8397 http://dx.doi.org/10.1002/adma.201602274 Volltext http://onlinelibrary.wiley.com/doi/10.1002/adma.201602274/abstract GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-DE-84 GBV_ILN_70 GBV_ILN_95 GBV_ILN_267 GBV_ILN_2004 GBV_ILN_2016 GBV_ILN_2018 GBV_ILN_2095 GBV_ILN_4012 GBV_ILN_4306 UA 1538 AR 28 2016 38 8388-8397 |
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10.1002/adma.201602274 doi PQ20161012 (DE-627)OLC198299780X (DE-599)GBVOLC198299780X (PRQ)wiley_primary_10_1002_adma_201602274_ADMA2016022743 (KEY)0178503620160000028003808388atomicscaleoriginoflongtermstabilityandhighperform DE-627 ger DE-627 rakwb eng 620 540 DE-101 540 AVZ UA 1538 AVZ rvk Kibria, Md Golam verfasserin aut Atomic‐Scale Origin of Long‐Term Stability and High Performance of p‐GaN Nanowire Arrays for Photocatalytic Overall Pure Water Splitting 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The atomic‐scale origin of the unusually high performance and long‐term stability of wurtzite p ‐GaN oriented nanowire arrays is revealed. Nitrogen termination of both the polar ( 000 1 ¯ ) top face and the nonpolar ( 10 1 ¯ 0 ) side faces of the nanowires is essential for long‐term stability and high efficiency. Such a distinct atomic configuration ensures not only stability against (photo) oxidation in air and in water/electrolyte but, as importantly, also provides the necessary overall reverse crystal polarization needed for efficient hole extraction in p ‐GaN. Nutzungsrecht: © 2016 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim wurtzite structure artificial photosynthesis polarization dependence X‐ray spectroscopy metal nitride N‐terminated surfaces Qiao, Ruimin oth Yang, Wanli oth Boukahil, Idris oth Kong, Xianghua oth Chowdhury, Faqrul Alam oth Trudeau, Michel L oth Ji, Wei oth Guo, Hong oth Himpsel, F. J oth Vayssieres, Lionel oth Mi, Zetian oth Enthalten in Advanced materials Weinheim : Wiley-VCH Verl., 1988 28(2016), 38, Seite 8388-8397 (DE-627)130815152 (DE-600)1012489-5 (DE-576)023057149 0935-9648 nnns volume:28 year:2016 number:38 pages:8388-8397 http://dx.doi.org/10.1002/adma.201602274 Volltext http://onlinelibrary.wiley.com/doi/10.1002/adma.201602274/abstract GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-DE-84 GBV_ILN_70 GBV_ILN_95 GBV_ILN_267 GBV_ILN_2004 GBV_ILN_2016 GBV_ILN_2018 GBV_ILN_2095 GBV_ILN_4012 GBV_ILN_4306 UA 1538 AR 28 2016 38 8388-8397 |
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10.1002/adma.201602274 doi PQ20161012 (DE-627)OLC198299780X (DE-599)GBVOLC198299780X (PRQ)wiley_primary_10_1002_adma_201602274_ADMA2016022743 (KEY)0178503620160000028003808388atomicscaleoriginoflongtermstabilityandhighperform DE-627 ger DE-627 rakwb eng 620 540 DE-101 540 AVZ UA 1538 AVZ rvk Kibria, Md Golam verfasserin aut Atomic‐Scale Origin of Long‐Term Stability and High Performance of p‐GaN Nanowire Arrays for Photocatalytic Overall Pure Water Splitting 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The atomic‐scale origin of the unusually high performance and long‐term stability of wurtzite p ‐GaN oriented nanowire arrays is revealed. Nitrogen termination of both the polar ( 000 1 ¯ ) top face and the nonpolar ( 10 1 ¯ 0 ) side faces of the nanowires is essential for long‐term stability and high efficiency. Such a distinct atomic configuration ensures not only stability against (photo) oxidation in air and in water/electrolyte but, as importantly, also provides the necessary overall reverse crystal polarization needed for efficient hole extraction in p ‐GaN. Nutzungsrecht: © 2016 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim wurtzite structure artificial photosynthesis polarization dependence X‐ray spectroscopy metal nitride N‐terminated surfaces Qiao, Ruimin oth Yang, Wanli oth Boukahil, Idris oth Kong, Xianghua oth Chowdhury, Faqrul Alam oth Trudeau, Michel L oth Ji, Wei oth Guo, Hong oth Himpsel, F. J oth Vayssieres, Lionel oth Mi, Zetian oth Enthalten in Advanced materials Weinheim : Wiley-VCH Verl., 1988 28(2016), 38, Seite 8388-8397 (DE-627)130815152 (DE-600)1012489-5 (DE-576)023057149 0935-9648 nnns volume:28 year:2016 number:38 pages:8388-8397 http://dx.doi.org/10.1002/adma.201602274 Volltext http://onlinelibrary.wiley.com/doi/10.1002/adma.201602274/abstract GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-DE-84 GBV_ILN_70 GBV_ILN_95 GBV_ILN_267 GBV_ILN_2004 GBV_ILN_2016 GBV_ILN_2018 GBV_ILN_2095 GBV_ILN_4012 GBV_ILN_4306 UA 1538 AR 28 2016 38 8388-8397 |
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10.1002/adma.201602274 doi PQ20161012 (DE-627)OLC198299780X (DE-599)GBVOLC198299780X (PRQ)wiley_primary_10_1002_adma_201602274_ADMA2016022743 (KEY)0178503620160000028003808388atomicscaleoriginoflongtermstabilityandhighperform DE-627 ger DE-627 rakwb eng 620 540 DE-101 540 AVZ UA 1538 AVZ rvk Kibria, Md Golam verfasserin aut Atomic‐Scale Origin of Long‐Term Stability and High Performance of p‐GaN Nanowire Arrays for Photocatalytic Overall Pure Water Splitting 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The atomic‐scale origin of the unusually high performance and long‐term stability of wurtzite p ‐GaN oriented nanowire arrays is revealed. Nitrogen termination of both the polar ( 000 1 ¯ ) top face and the nonpolar ( 10 1 ¯ 0 ) side faces of the nanowires is essential for long‐term stability and high efficiency. Such a distinct atomic configuration ensures not only stability against (photo) oxidation in air and in water/electrolyte but, as importantly, also provides the necessary overall reverse crystal polarization needed for efficient hole extraction in p ‐GaN. Nutzungsrecht: © 2016 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim wurtzite structure artificial photosynthesis polarization dependence X‐ray spectroscopy metal nitride N‐terminated surfaces Qiao, Ruimin oth Yang, Wanli oth Boukahil, Idris oth Kong, Xianghua oth Chowdhury, Faqrul Alam oth Trudeau, Michel L oth Ji, Wei oth Guo, Hong oth Himpsel, F. J oth Vayssieres, Lionel oth Mi, Zetian oth Enthalten in Advanced materials Weinheim : Wiley-VCH Verl., 1988 28(2016), 38, Seite 8388-8397 (DE-627)130815152 (DE-600)1012489-5 (DE-576)023057149 0935-9648 nnns volume:28 year:2016 number:38 pages:8388-8397 http://dx.doi.org/10.1002/adma.201602274 Volltext http://onlinelibrary.wiley.com/doi/10.1002/adma.201602274/abstract GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-DE-84 GBV_ILN_70 GBV_ILN_95 GBV_ILN_267 GBV_ILN_2004 GBV_ILN_2016 GBV_ILN_2018 GBV_ILN_2095 GBV_ILN_4012 GBV_ILN_4306 UA 1538 AR 28 2016 38 8388-8397 |
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Kibria, Md Golam @@aut@@ Qiao, Ruimin @@oth@@ Yang, Wanli @@oth@@ Boukahil, Idris @@oth@@ Kong, Xianghua @@oth@@ Chowdhury, Faqrul Alam @@oth@@ Trudeau, Michel L @@oth@@ Ji, Wei @@oth@@ Guo, Hong @@oth@@ Himpsel, F. J @@oth@@ Vayssieres, Lionel @@oth@@ Mi, Zetian @@oth@@ |
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Atomic‐Scale Origin of Long‐Term Stability and High Performance of p‐GaN Nanowire Arrays for Photocatalytic Overall Pure Water Splitting |
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Atomic‐Scale Origin of Long‐Term Stability and High Performance of p‐GaN Nanowire Arrays for Photocatalytic Overall Pure Water Splitting |
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atomic‐scale origin of long‐term stability and high performance of p‐gan nanowire arrays for photocatalytic overall pure water splitting |
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Atomic‐Scale Origin of Long‐Term Stability and High Performance of p‐GaN Nanowire Arrays for Photocatalytic Overall Pure Water Splitting |
abstract |
The atomic‐scale origin of the unusually high performance and long‐term stability of wurtzite p ‐GaN oriented nanowire arrays is revealed. Nitrogen termination of both the polar ( 000 1 ¯ ) top face and the nonpolar ( 10 1 ¯ 0 ) side faces of the nanowires is essential for long‐term stability and high efficiency. Such a distinct atomic configuration ensures not only stability against (photo) oxidation in air and in water/electrolyte but, as importantly, also provides the necessary overall reverse crystal polarization needed for efficient hole extraction in p ‐GaN. |
abstractGer |
The atomic‐scale origin of the unusually high performance and long‐term stability of wurtzite p ‐GaN oriented nanowire arrays is revealed. Nitrogen termination of both the polar ( 000 1 ¯ ) top face and the nonpolar ( 10 1 ¯ 0 ) side faces of the nanowires is essential for long‐term stability and high efficiency. Such a distinct atomic configuration ensures not only stability against (photo) oxidation in air and in water/electrolyte but, as importantly, also provides the necessary overall reverse crystal polarization needed for efficient hole extraction in p ‐GaN. |
abstract_unstemmed |
The atomic‐scale origin of the unusually high performance and long‐term stability of wurtzite p ‐GaN oriented nanowire arrays is revealed. Nitrogen termination of both the polar ( 000 1 ¯ ) top face and the nonpolar ( 10 1 ¯ 0 ) side faces of the nanowires is essential for long‐term stability and high efficiency. Such a distinct atomic configuration ensures not only stability against (photo) oxidation in air and in water/electrolyte but, as importantly, also provides the necessary overall reverse crystal polarization needed for efficient hole extraction in p ‐GaN. |
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38 |
title_short |
Atomic‐Scale Origin of Long‐Term Stability and High Performance of p‐GaN Nanowire Arrays for Photocatalytic Overall Pure Water Splitting |
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http://dx.doi.org/10.1002/adma.201602274 http://onlinelibrary.wiley.com/doi/10.1002/adma.201602274/abstract |
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Qiao, Ruimin Yang, Wanli Boukahil, Idris Kong, Xianghua Chowdhury, Faqrul Alam Trudeau, Michel L Ji, Wei Guo, Hong Himpsel, F. J Vayssieres, Lionel Mi, Zetian |
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