Potential sea salt aerosol sources from frost flowers in the pan-Arctic region
In order to better represent observed wintertime aerosol mass and number concentrations in the pan-Arctic (60°N-90°N) region, we implemented an observationally based parameterization for estimating sea salt production from frost flowers in the Community Earth System Model (CESM, version 1.2.1). In t...
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Gespeichert in:
| Autor*in: |
Li Xu [verfasserIn] |
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| Format: |
Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2016 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Journal of geophysical research / D - Washington, DC : Union, 1984, 121(2016), 18 |
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| Übergeordnetes Werk: |
volume:121 ; year:2016 ; number:18 |
| Links: |
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| DOI / URN: |
10.1002/2015JD024713 |
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| 520 | |a In order to better represent observed wintertime aerosol mass and number concentrations in the pan-Arctic (60°N-90°N) region, we implemented an observationally based parameterization for estimating sea salt production from frost flowers in the Community Earth System Model (CESM, version 1.2.1). In this work, we evaluate the potential influence of this sea salt source on the pan-Arctic climate. Results show that frost flower salt emissions increase the modeled surface sea salt aerosol mass concentration by roughly 200% at Barrow and 100% at Alert and accumulation-mode number concentration by about a factor of 2 at Barrow and more than a factor of 10 at Alert in the winter months when new sea ice and frost flowers are present. The magnitude of sea salt aerosol mass and number concentrations at the surface in Barrow during winter simulated by the model configuration that includes this parameterization agrees better with observations by 48% and 12%, respectively, than the standard CESM simulation without a frost flower salt particle source. At Alert, the simulation with this parameterization overestimates observed sea salt aerosol mass concentration by 150% during winter in contrast to the underestimation of 63% in the simulation without this frost flower source, while it produces particle number concentration about 14% closer to observation than the standard CESM simulation. However, because the CESM version used here underestimates transported sulfate in winter, the reference accumulation-mode number concentrations at Alert are also underestimated. Adding these frost flower salt particle emissions increases sea salt aerosol optical depth by 10% in the pan-Arctic region and results in a small cooling at the surface. The increase in salt aerosol mass concentrations of a factor of 8 provides nearly two times the cloud condensation nuclei concentration at supersaturation of 0.1%, as well as 10% increases in cloud droplet number and 40% increases in liquid water content near coastal regions adjacent to continents. These cloud changes reduce longwave cloud forcing at the top of the atmosphere by 3% and cause a small surface warming, increasing the downward longwave flux at the surface by 1.8Wm-2 in the pan-Arctic under the present-day climate. This regional average longwave warming due to the presence of clouds attributed to frost flower sea salts is roughly half of previous observed surface longwave fluxes and cloud-forcing estimates reported in Alaska, implying that the longwave enhancement due to frost flower salts may be comparable to those estimated for anthropogenic aerosol emissions. Since the potential frost flower area is parameterized as the maximum possible region on which frost flowers grow for the modeled atmospheric temperature and sea ice conditions and the model underestimates the number of accumulation-mode particles from midlatitude anthropogenic sources transported in winter, the calculated aerosol indirect effect of frost flower sea salts in this work can be regarded an upper bound. Key Points First CESM implementation of salt aerosol parameterization from frost flowers Frost flower salts reproduce observed wintertime salt mass and number concentrations Frost flower salts may serve as important aerosol mass and number sources in the pan-Arctic region | ||
| 650 | 4 | |a Ocean-atmosphere interaction | |
| 650 | 4 | |a Salinity | |
| 650 | 4 | |a Meteorology | |
| 650 | 4 | |a Atmospheric aerosols | |
| 700 | 0 | |a Lynn M Russell |4 oth | |
| 700 | 0 | |a Susannah M Burrows |4 oth | |
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10.1002/2015JD024713 doi PQ20161201 (DE-627)OLC1985460475 (DE-599)GBVOLC1985460475 (PRQ)p1170-1bdb9a17818b108464a1b1e3337f1bf4f59f46358c80b94773b0a718dcdcfdf90 (KEY)0137985220160000121001800000potentialseasaltaerosolsourcesfromfrostflowersinth DE-627 ger DE-627 rakwb eng 550 DNB Li Xu verfasserin aut Potential sea salt aerosol sources from frost flowers in the pan-Arctic region 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier In order to better represent observed wintertime aerosol mass and number concentrations in the pan-Arctic (60°N-90°N) region, we implemented an observationally based parameterization for estimating sea salt production from frost flowers in the Community Earth System Model (CESM, version 1.2.1). In this work, we evaluate the potential influence of this sea salt source on the pan-Arctic climate. Results show that frost flower salt emissions increase the modeled surface sea salt aerosol mass concentration by roughly 200% at Barrow and 100% at Alert and accumulation-mode number concentration by about a factor of 2 at Barrow and more than a factor of 10 at Alert in the winter months when new sea ice and frost flowers are present. The magnitude of sea salt aerosol mass and number concentrations at the surface in Barrow during winter simulated by the model configuration that includes this parameterization agrees better with observations by 48% and 12%, respectively, than the standard CESM simulation without a frost flower salt particle source. At Alert, the simulation with this parameterization overestimates observed sea salt aerosol mass concentration by 150% during winter in contrast to the underestimation of 63% in the simulation without this frost flower source, while it produces particle number concentration about 14% closer to observation than the standard CESM simulation. However, because the CESM version used here underestimates transported sulfate in winter, the reference accumulation-mode number concentrations at Alert are also underestimated. Adding these frost flower salt particle emissions increases sea salt aerosol optical depth by 10% in the pan-Arctic region and results in a small cooling at the surface. The increase in salt aerosol mass concentrations of a factor of 8 provides nearly two times the cloud condensation nuclei concentration at supersaturation of 0.1%, as well as 10% increases in cloud droplet number and 40% increases in liquid water content near coastal regions adjacent to continents. These cloud changes reduce longwave cloud forcing at the top of the atmosphere by 3% and cause a small surface warming, increasing the downward longwave flux at the surface by 1.8Wm-2 in the pan-Arctic under the present-day climate. This regional average longwave warming due to the presence of clouds attributed to frost flower sea salts is roughly half of previous observed surface longwave fluxes and cloud-forcing estimates reported in Alaska, implying that the longwave enhancement due to frost flower salts may be comparable to those estimated for anthropogenic aerosol emissions. Since the potential frost flower area is parameterized as the maximum possible region on which frost flowers grow for the modeled atmospheric temperature and sea ice conditions and the model underestimates the number of accumulation-mode particles from midlatitude anthropogenic sources transported in winter, the calculated aerosol indirect effect of frost flower sea salts in this work can be regarded an upper bound. Key Points First CESM implementation of salt aerosol parameterization from frost flowers Frost flower salts reproduce observed wintertime salt mass and number concentrations Frost flower salts may serve as important aerosol mass and number sources in the pan-Arctic region Ocean-atmosphere interaction Salinity Meteorology Atmospheric aerosols Lynn M Russell oth Susannah M Burrows oth Enthalten in Journal of geophysical research / D Washington, DC : Union, 1984 121(2016), 18 (DE-627)130444391 (DE-600)710256-2 (DE-576)015978818 2169-897X nnns volume:121 year:2016 number:18 http://dx.doi.org/10.1002/2015JD024713 Volltext http://search.proquest.com/docview/1828696574 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY SSG-OLC-GEO SSG-OPC-GGO SSG-OPC-GEO GBV_ILN_62 GBV_ILN_154 AR 121 2016 18 |
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10.1002/2015JD024713 doi PQ20161201 (DE-627)OLC1985460475 (DE-599)GBVOLC1985460475 (PRQ)p1170-1bdb9a17818b108464a1b1e3337f1bf4f59f46358c80b94773b0a718dcdcfdf90 (KEY)0137985220160000121001800000potentialseasaltaerosolsourcesfromfrostflowersinth DE-627 ger DE-627 rakwb eng 550 DNB Li Xu verfasserin aut Potential sea salt aerosol sources from frost flowers in the pan-Arctic region 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier In order to better represent observed wintertime aerosol mass and number concentrations in the pan-Arctic (60°N-90°N) region, we implemented an observationally based parameterization for estimating sea salt production from frost flowers in the Community Earth System Model (CESM, version 1.2.1). In this work, we evaluate the potential influence of this sea salt source on the pan-Arctic climate. Results show that frost flower salt emissions increase the modeled surface sea salt aerosol mass concentration by roughly 200% at Barrow and 100% at Alert and accumulation-mode number concentration by about a factor of 2 at Barrow and more than a factor of 10 at Alert in the winter months when new sea ice and frost flowers are present. The magnitude of sea salt aerosol mass and number concentrations at the surface in Barrow during winter simulated by the model configuration that includes this parameterization agrees better with observations by 48% and 12%, respectively, than the standard CESM simulation without a frost flower salt particle source. At Alert, the simulation with this parameterization overestimates observed sea salt aerosol mass concentration by 150% during winter in contrast to the underestimation of 63% in the simulation without this frost flower source, while it produces particle number concentration about 14% closer to observation than the standard CESM simulation. However, because the CESM version used here underestimates transported sulfate in winter, the reference accumulation-mode number concentrations at Alert are also underestimated. Adding these frost flower salt particle emissions increases sea salt aerosol optical depth by 10% in the pan-Arctic region and results in a small cooling at the surface. The increase in salt aerosol mass concentrations of a factor of 8 provides nearly two times the cloud condensation nuclei concentration at supersaturation of 0.1%, as well as 10% increases in cloud droplet number and 40% increases in liquid water content near coastal regions adjacent to continents. These cloud changes reduce longwave cloud forcing at the top of the atmosphere by 3% and cause a small surface warming, increasing the downward longwave flux at the surface by 1.8Wm-2 in the pan-Arctic under the present-day climate. This regional average longwave warming due to the presence of clouds attributed to frost flower sea salts is roughly half of previous observed surface longwave fluxes and cloud-forcing estimates reported in Alaska, implying that the longwave enhancement due to frost flower salts may be comparable to those estimated for anthropogenic aerosol emissions. Since the potential frost flower area is parameterized as the maximum possible region on which frost flowers grow for the modeled atmospheric temperature and sea ice conditions and the model underestimates the number of accumulation-mode particles from midlatitude anthropogenic sources transported in winter, the calculated aerosol indirect effect of frost flower sea salts in this work can be regarded an upper bound. Key Points First CESM implementation of salt aerosol parameterization from frost flowers Frost flower salts reproduce observed wintertime salt mass and number concentrations Frost flower salts may serve as important aerosol mass and number sources in the pan-Arctic region Ocean-atmosphere interaction Salinity Meteorology Atmospheric aerosols Lynn M Russell oth Susannah M Burrows oth Enthalten in Journal of geophysical research / D Washington, DC : Union, 1984 121(2016), 18 (DE-627)130444391 (DE-600)710256-2 (DE-576)015978818 2169-897X nnns volume:121 year:2016 number:18 http://dx.doi.org/10.1002/2015JD024713 Volltext http://search.proquest.com/docview/1828696574 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY SSG-OLC-GEO SSG-OPC-GGO SSG-OPC-GEO GBV_ILN_62 GBV_ILN_154 AR 121 2016 18 |
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10.1002/2015JD024713 doi PQ20161201 (DE-627)OLC1985460475 (DE-599)GBVOLC1985460475 (PRQ)p1170-1bdb9a17818b108464a1b1e3337f1bf4f59f46358c80b94773b0a718dcdcfdf90 (KEY)0137985220160000121001800000potentialseasaltaerosolsourcesfromfrostflowersinth DE-627 ger DE-627 rakwb eng 550 DNB Li Xu verfasserin aut Potential sea salt aerosol sources from frost flowers in the pan-Arctic region 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier In order to better represent observed wintertime aerosol mass and number concentrations in the pan-Arctic (60°N-90°N) region, we implemented an observationally based parameterization for estimating sea salt production from frost flowers in the Community Earth System Model (CESM, version 1.2.1). In this work, we evaluate the potential influence of this sea salt source on the pan-Arctic climate. Results show that frost flower salt emissions increase the modeled surface sea salt aerosol mass concentration by roughly 200% at Barrow and 100% at Alert and accumulation-mode number concentration by about a factor of 2 at Barrow and more than a factor of 10 at Alert in the winter months when new sea ice and frost flowers are present. The magnitude of sea salt aerosol mass and number concentrations at the surface in Barrow during winter simulated by the model configuration that includes this parameterization agrees better with observations by 48% and 12%, respectively, than the standard CESM simulation without a frost flower salt particle source. At Alert, the simulation with this parameterization overestimates observed sea salt aerosol mass concentration by 150% during winter in contrast to the underestimation of 63% in the simulation without this frost flower source, while it produces particle number concentration about 14% closer to observation than the standard CESM simulation. However, because the CESM version used here underestimates transported sulfate in winter, the reference accumulation-mode number concentrations at Alert are also underestimated. Adding these frost flower salt particle emissions increases sea salt aerosol optical depth by 10% in the pan-Arctic region and results in a small cooling at the surface. The increase in salt aerosol mass concentrations of a factor of 8 provides nearly two times the cloud condensation nuclei concentration at supersaturation of 0.1%, as well as 10% increases in cloud droplet number and 40% increases in liquid water content near coastal regions adjacent to continents. These cloud changes reduce longwave cloud forcing at the top of the atmosphere by 3% and cause a small surface warming, increasing the downward longwave flux at the surface by 1.8Wm-2 in the pan-Arctic under the present-day climate. This regional average longwave warming due to the presence of clouds attributed to frost flower sea salts is roughly half of previous observed surface longwave fluxes and cloud-forcing estimates reported in Alaska, implying that the longwave enhancement due to frost flower salts may be comparable to those estimated for anthropogenic aerosol emissions. Since the potential frost flower area is parameterized as the maximum possible region on which frost flowers grow for the modeled atmospheric temperature and sea ice conditions and the model underestimates the number of accumulation-mode particles from midlatitude anthropogenic sources transported in winter, the calculated aerosol indirect effect of frost flower sea salts in this work can be regarded an upper bound. Key Points First CESM implementation of salt aerosol parameterization from frost flowers Frost flower salts reproduce observed wintertime salt mass and number concentrations Frost flower salts may serve as important aerosol mass and number sources in the pan-Arctic region Ocean-atmosphere interaction Salinity Meteorology Atmospheric aerosols Lynn M Russell oth Susannah M Burrows oth Enthalten in Journal of geophysical research / D Washington, DC : Union, 1984 121(2016), 18 (DE-627)130444391 (DE-600)710256-2 (DE-576)015978818 2169-897X nnns volume:121 year:2016 number:18 http://dx.doi.org/10.1002/2015JD024713 Volltext http://search.proquest.com/docview/1828696574 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY SSG-OLC-GEO SSG-OPC-GGO SSG-OPC-GEO GBV_ILN_62 GBV_ILN_154 AR 121 2016 18 |
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10.1002/2015JD024713 doi PQ20161201 (DE-627)OLC1985460475 (DE-599)GBVOLC1985460475 (PRQ)p1170-1bdb9a17818b108464a1b1e3337f1bf4f59f46358c80b94773b0a718dcdcfdf90 (KEY)0137985220160000121001800000potentialseasaltaerosolsourcesfromfrostflowersinth DE-627 ger DE-627 rakwb eng 550 DNB Li Xu verfasserin aut Potential sea salt aerosol sources from frost flowers in the pan-Arctic region 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier In order to better represent observed wintertime aerosol mass and number concentrations in the pan-Arctic (60°N-90°N) region, we implemented an observationally based parameterization for estimating sea salt production from frost flowers in the Community Earth System Model (CESM, version 1.2.1). In this work, we evaluate the potential influence of this sea salt source on the pan-Arctic climate. Results show that frost flower salt emissions increase the modeled surface sea salt aerosol mass concentration by roughly 200% at Barrow and 100% at Alert and accumulation-mode number concentration by about a factor of 2 at Barrow and more than a factor of 10 at Alert in the winter months when new sea ice and frost flowers are present. The magnitude of sea salt aerosol mass and number concentrations at the surface in Barrow during winter simulated by the model configuration that includes this parameterization agrees better with observations by 48% and 12%, respectively, than the standard CESM simulation without a frost flower salt particle source. At Alert, the simulation with this parameterization overestimates observed sea salt aerosol mass concentration by 150% during winter in contrast to the underestimation of 63% in the simulation without this frost flower source, while it produces particle number concentration about 14% closer to observation than the standard CESM simulation. However, because the CESM version used here underestimates transported sulfate in winter, the reference accumulation-mode number concentrations at Alert are also underestimated. Adding these frost flower salt particle emissions increases sea salt aerosol optical depth by 10% in the pan-Arctic region and results in a small cooling at the surface. The increase in salt aerosol mass concentrations of a factor of 8 provides nearly two times the cloud condensation nuclei concentration at supersaturation of 0.1%, as well as 10% increases in cloud droplet number and 40% increases in liquid water content near coastal regions adjacent to continents. These cloud changes reduce longwave cloud forcing at the top of the atmosphere by 3% and cause a small surface warming, increasing the downward longwave flux at the surface by 1.8Wm-2 in the pan-Arctic under the present-day climate. This regional average longwave warming due to the presence of clouds attributed to frost flower sea salts is roughly half of previous observed surface longwave fluxes and cloud-forcing estimates reported in Alaska, implying that the longwave enhancement due to frost flower salts may be comparable to those estimated for anthropogenic aerosol emissions. Since the potential frost flower area is parameterized as the maximum possible region on which frost flowers grow for the modeled atmospheric temperature and sea ice conditions and the model underestimates the number of accumulation-mode particles from midlatitude anthropogenic sources transported in winter, the calculated aerosol indirect effect of frost flower sea salts in this work can be regarded an upper bound. Key Points First CESM implementation of salt aerosol parameterization from frost flowers Frost flower salts reproduce observed wintertime salt mass and number concentrations Frost flower salts may serve as important aerosol mass and number sources in the pan-Arctic region Ocean-atmosphere interaction Salinity Meteorology Atmospheric aerosols Lynn M Russell oth Susannah M Burrows oth Enthalten in Journal of geophysical research / D Washington, DC : Union, 1984 121(2016), 18 (DE-627)130444391 (DE-600)710256-2 (DE-576)015978818 2169-897X nnns volume:121 year:2016 number:18 http://dx.doi.org/10.1002/2015JD024713 Volltext http://search.proquest.com/docview/1828696574 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY SSG-OLC-GEO SSG-OPC-GGO SSG-OPC-GEO GBV_ILN_62 GBV_ILN_154 AR 121 2016 18 |
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10.1002/2015JD024713 doi PQ20161201 (DE-627)OLC1985460475 (DE-599)GBVOLC1985460475 (PRQ)p1170-1bdb9a17818b108464a1b1e3337f1bf4f59f46358c80b94773b0a718dcdcfdf90 (KEY)0137985220160000121001800000potentialseasaltaerosolsourcesfromfrostflowersinth DE-627 ger DE-627 rakwb eng 550 DNB Li Xu verfasserin aut Potential sea salt aerosol sources from frost flowers in the pan-Arctic region 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier In order to better represent observed wintertime aerosol mass and number concentrations in the pan-Arctic (60°N-90°N) region, we implemented an observationally based parameterization for estimating sea salt production from frost flowers in the Community Earth System Model (CESM, version 1.2.1). In this work, we evaluate the potential influence of this sea salt source on the pan-Arctic climate. Results show that frost flower salt emissions increase the modeled surface sea salt aerosol mass concentration by roughly 200% at Barrow and 100% at Alert and accumulation-mode number concentration by about a factor of 2 at Barrow and more than a factor of 10 at Alert in the winter months when new sea ice and frost flowers are present. The magnitude of sea salt aerosol mass and number concentrations at the surface in Barrow during winter simulated by the model configuration that includes this parameterization agrees better with observations by 48% and 12%, respectively, than the standard CESM simulation without a frost flower salt particle source. At Alert, the simulation with this parameterization overestimates observed sea salt aerosol mass concentration by 150% during winter in contrast to the underestimation of 63% in the simulation without this frost flower source, while it produces particle number concentration about 14% closer to observation than the standard CESM simulation. However, because the CESM version used here underestimates transported sulfate in winter, the reference accumulation-mode number concentrations at Alert are also underestimated. Adding these frost flower salt particle emissions increases sea salt aerosol optical depth by 10% in the pan-Arctic region and results in a small cooling at the surface. The increase in salt aerosol mass concentrations of a factor of 8 provides nearly two times the cloud condensation nuclei concentration at supersaturation of 0.1%, as well as 10% increases in cloud droplet number and 40% increases in liquid water content near coastal regions adjacent to continents. These cloud changes reduce longwave cloud forcing at the top of the atmosphere by 3% and cause a small surface warming, increasing the downward longwave flux at the surface by 1.8Wm-2 in the pan-Arctic under the present-day climate. This regional average longwave warming due to the presence of clouds attributed to frost flower sea salts is roughly half of previous observed surface longwave fluxes and cloud-forcing estimates reported in Alaska, implying that the longwave enhancement due to frost flower salts may be comparable to those estimated for anthropogenic aerosol emissions. Since the potential frost flower area is parameterized as the maximum possible region on which frost flowers grow for the modeled atmospheric temperature and sea ice conditions and the model underestimates the number of accumulation-mode particles from midlatitude anthropogenic sources transported in winter, the calculated aerosol indirect effect of frost flower sea salts in this work can be regarded an upper bound. Key Points First CESM implementation of salt aerosol parameterization from frost flowers Frost flower salts reproduce observed wintertime salt mass and number concentrations Frost flower salts may serve as important aerosol mass and number sources in the pan-Arctic region Ocean-atmosphere interaction Salinity Meteorology Atmospheric aerosols Lynn M Russell oth Susannah M Burrows oth Enthalten in Journal of geophysical research / D Washington, DC : Union, 1984 121(2016), 18 (DE-627)130444391 (DE-600)710256-2 (DE-576)015978818 2169-897X nnns volume:121 year:2016 number:18 http://dx.doi.org/10.1002/2015JD024713 Volltext http://search.proquest.com/docview/1828696574 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-PHY SSG-OLC-GEO SSG-OPC-GGO SSG-OPC-GEO GBV_ILN_62 GBV_ILN_154 AR 121 2016 18 |
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In this work, we evaluate the potential influence of this sea salt source on the pan-Arctic climate. Results show that frost flower salt emissions increase the modeled surface sea salt aerosol mass concentration by roughly 200% at Barrow and 100% at Alert and accumulation-mode number concentration by about a factor of 2 at Barrow and more than a factor of 10 at Alert in the winter months when new sea ice and frost flowers are present. The magnitude of sea salt aerosol mass and number concentrations at the surface in Barrow during winter simulated by the model configuration that includes this parameterization agrees better with observations by 48% and 12%, respectively, than the standard CESM simulation without a frost flower salt particle source. At Alert, the simulation with this parameterization overestimates observed sea salt aerosol mass concentration by 150% during winter in contrast to the underestimation of 63% in the simulation without this frost flower source, while it produces particle number concentration about 14% closer to observation than the standard CESM simulation. However, because the CESM version used here underestimates transported sulfate in winter, the reference accumulation-mode number concentrations at Alert are also underestimated. Adding these frost flower salt particle emissions increases sea salt aerosol optical depth by 10% in the pan-Arctic region and results in a small cooling at the surface. The increase in salt aerosol mass concentrations of a factor of 8 provides nearly two times the cloud condensation nuclei concentration at supersaturation of 0.1%, as well as 10% increases in cloud droplet number and 40% increases in liquid water content near coastal regions adjacent to continents. These cloud changes reduce longwave cloud forcing at the top of the atmosphere by 3% and cause a small surface warming, increasing the downward longwave flux at the surface by 1.8Wm-2 in the pan-Arctic under the present-day climate. This regional average longwave warming due to the presence of clouds attributed to frost flower sea salts is roughly half of previous observed surface longwave fluxes and cloud-forcing estimates reported in Alaska, implying that the longwave enhancement due to frost flower salts may be comparable to those estimated for anthropogenic aerosol emissions. Since the potential frost flower area is parameterized as the maximum possible region on which frost flowers grow for the modeled atmospheric temperature and sea ice conditions and the model underestimates the number of accumulation-mode particles from midlatitude anthropogenic sources transported in winter, the calculated aerosol indirect effect of frost flower sea salts in this work can be regarded an upper bound. 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Potential sea salt aerosol sources from frost flowers in the pan-Arctic region |
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potential sea salt aerosol sources from frost flowers in the pan-arctic region |
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Potential sea salt aerosol sources from frost flowers in the pan-Arctic region |
| abstract |
In order to better represent observed wintertime aerosol mass and number concentrations in the pan-Arctic (60°N-90°N) region, we implemented an observationally based parameterization for estimating sea salt production from frost flowers in the Community Earth System Model (CESM, version 1.2.1). In this work, we evaluate the potential influence of this sea salt source on the pan-Arctic climate. Results show that frost flower salt emissions increase the modeled surface sea salt aerosol mass concentration by roughly 200% at Barrow and 100% at Alert and accumulation-mode number concentration by about a factor of 2 at Barrow and more than a factor of 10 at Alert in the winter months when new sea ice and frost flowers are present. The magnitude of sea salt aerosol mass and number concentrations at the surface in Barrow during winter simulated by the model configuration that includes this parameterization agrees better with observations by 48% and 12%, respectively, than the standard CESM simulation without a frost flower salt particle source. At Alert, the simulation with this parameterization overestimates observed sea salt aerosol mass concentration by 150% during winter in contrast to the underestimation of 63% in the simulation without this frost flower source, while it produces particle number concentration about 14% closer to observation than the standard CESM simulation. However, because the CESM version used here underestimates transported sulfate in winter, the reference accumulation-mode number concentrations at Alert are also underestimated. Adding these frost flower salt particle emissions increases sea salt aerosol optical depth by 10% in the pan-Arctic region and results in a small cooling at the surface. The increase in salt aerosol mass concentrations of a factor of 8 provides nearly two times the cloud condensation nuclei concentration at supersaturation of 0.1%, as well as 10% increases in cloud droplet number and 40% increases in liquid water content near coastal regions adjacent to continents. These cloud changes reduce longwave cloud forcing at the top of the atmosphere by 3% and cause a small surface warming, increasing the downward longwave flux at the surface by 1.8Wm-2 in the pan-Arctic under the present-day climate. This regional average longwave warming due to the presence of clouds attributed to frost flower sea salts is roughly half of previous observed surface longwave fluxes and cloud-forcing estimates reported in Alaska, implying that the longwave enhancement due to frost flower salts may be comparable to those estimated for anthropogenic aerosol emissions. Since the potential frost flower area is parameterized as the maximum possible region on which frost flowers grow for the modeled atmospheric temperature and sea ice conditions and the model underestimates the number of accumulation-mode particles from midlatitude anthropogenic sources transported in winter, the calculated aerosol indirect effect of frost flower sea salts in this work can be regarded an upper bound. Key Points First CESM implementation of salt aerosol parameterization from frost flowers Frost flower salts reproduce observed wintertime salt mass and number concentrations Frost flower salts may serve as important aerosol mass and number sources in the pan-Arctic region |
| abstractGer |
In order to better represent observed wintertime aerosol mass and number concentrations in the pan-Arctic (60°N-90°N) region, we implemented an observationally based parameterization for estimating sea salt production from frost flowers in the Community Earth System Model (CESM, version 1.2.1). In this work, we evaluate the potential influence of this sea salt source on the pan-Arctic climate. Results show that frost flower salt emissions increase the modeled surface sea salt aerosol mass concentration by roughly 200% at Barrow and 100% at Alert and accumulation-mode number concentration by about a factor of 2 at Barrow and more than a factor of 10 at Alert in the winter months when new sea ice and frost flowers are present. The magnitude of sea salt aerosol mass and number concentrations at the surface in Barrow during winter simulated by the model configuration that includes this parameterization agrees better with observations by 48% and 12%, respectively, than the standard CESM simulation without a frost flower salt particle source. At Alert, the simulation with this parameterization overestimates observed sea salt aerosol mass concentration by 150% during winter in contrast to the underestimation of 63% in the simulation without this frost flower source, while it produces particle number concentration about 14% closer to observation than the standard CESM simulation. However, because the CESM version used here underestimates transported sulfate in winter, the reference accumulation-mode number concentrations at Alert are also underestimated. Adding these frost flower salt particle emissions increases sea salt aerosol optical depth by 10% in the pan-Arctic region and results in a small cooling at the surface. The increase in salt aerosol mass concentrations of a factor of 8 provides nearly two times the cloud condensation nuclei concentration at supersaturation of 0.1%, as well as 10% increases in cloud droplet number and 40% increases in liquid water content near coastal regions adjacent to continents. These cloud changes reduce longwave cloud forcing at the top of the atmosphere by 3% and cause a small surface warming, increasing the downward longwave flux at the surface by 1.8Wm-2 in the pan-Arctic under the present-day climate. This regional average longwave warming due to the presence of clouds attributed to frost flower sea salts is roughly half of previous observed surface longwave fluxes and cloud-forcing estimates reported in Alaska, implying that the longwave enhancement due to frost flower salts may be comparable to those estimated for anthropogenic aerosol emissions. Since the potential frost flower area is parameterized as the maximum possible region on which frost flowers grow for the modeled atmospheric temperature and sea ice conditions and the model underestimates the number of accumulation-mode particles from midlatitude anthropogenic sources transported in winter, the calculated aerosol indirect effect of frost flower sea salts in this work can be regarded an upper bound. Key Points First CESM implementation of salt aerosol parameterization from frost flowers Frost flower salts reproduce observed wintertime salt mass and number concentrations Frost flower salts may serve as important aerosol mass and number sources in the pan-Arctic region |
| abstract_unstemmed |
In order to better represent observed wintertime aerosol mass and number concentrations in the pan-Arctic (60°N-90°N) region, we implemented an observationally based parameterization for estimating sea salt production from frost flowers in the Community Earth System Model (CESM, version 1.2.1). In this work, we evaluate the potential influence of this sea salt source on the pan-Arctic climate. Results show that frost flower salt emissions increase the modeled surface sea salt aerosol mass concentration by roughly 200% at Barrow and 100% at Alert and accumulation-mode number concentration by about a factor of 2 at Barrow and more than a factor of 10 at Alert in the winter months when new sea ice and frost flowers are present. The magnitude of sea salt aerosol mass and number concentrations at the surface in Barrow during winter simulated by the model configuration that includes this parameterization agrees better with observations by 48% and 12%, respectively, than the standard CESM simulation without a frost flower salt particle source. At Alert, the simulation with this parameterization overestimates observed sea salt aerosol mass concentration by 150% during winter in contrast to the underestimation of 63% in the simulation without this frost flower source, while it produces particle number concentration about 14% closer to observation than the standard CESM simulation. However, because the CESM version used here underestimates transported sulfate in winter, the reference accumulation-mode number concentrations at Alert are also underestimated. Adding these frost flower salt particle emissions increases sea salt aerosol optical depth by 10% in the pan-Arctic region and results in a small cooling at the surface. The increase in salt aerosol mass concentrations of a factor of 8 provides nearly two times the cloud condensation nuclei concentration at supersaturation of 0.1%, as well as 10% increases in cloud droplet number and 40% increases in liquid water content near coastal regions adjacent to continents. These cloud changes reduce longwave cloud forcing at the top of the atmosphere by 3% and cause a small surface warming, increasing the downward longwave flux at the surface by 1.8Wm-2 in the pan-Arctic under the present-day climate. This regional average longwave warming due to the presence of clouds attributed to frost flower sea salts is roughly half of previous observed surface longwave fluxes and cloud-forcing estimates reported in Alaska, implying that the longwave enhancement due to frost flower salts may be comparable to those estimated for anthropogenic aerosol emissions. Since the potential frost flower area is parameterized as the maximum possible region on which frost flowers grow for the modeled atmospheric temperature and sea ice conditions and the model underestimates the number of accumulation-mode particles from midlatitude anthropogenic sources transported in winter, the calculated aerosol indirect effect of frost flower sea salts in this work can be regarded an upper bound. Key Points First CESM implementation of salt aerosol parameterization from frost flowers Frost flower salts reproduce observed wintertime salt mass and number concentrations Frost flower salts may serve as important aerosol mass and number sources in the pan-Arctic region |
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In this work, we evaluate the potential influence of this sea salt source on the pan-Arctic climate. Results show that frost flower salt emissions increase the modeled surface sea salt aerosol mass concentration by roughly 200% at Barrow and 100% at Alert and accumulation-mode number concentration by about a factor of 2 at Barrow and more than a factor of 10 at Alert in the winter months when new sea ice and frost flowers are present. The magnitude of sea salt aerosol mass and number concentrations at the surface in Barrow during winter simulated by the model configuration that includes this parameterization agrees better with observations by 48% and 12%, respectively, than the standard CESM simulation without a frost flower salt particle source. At Alert, the simulation with this parameterization overestimates observed sea salt aerosol mass concentration by 150% during winter in contrast to the underestimation of 63% in the simulation without this frost flower source, while it produces particle number concentration about 14% closer to observation than the standard CESM simulation. However, because the CESM version used here underestimates transported sulfate in winter, the reference accumulation-mode number concentrations at Alert are also underestimated. Adding these frost flower salt particle emissions increases sea salt aerosol optical depth by 10% in the pan-Arctic region and results in a small cooling at the surface. The increase in salt aerosol mass concentrations of a factor of 8 provides nearly two times the cloud condensation nuclei concentration at supersaturation of 0.1%, as well as 10% increases in cloud droplet number and 40% increases in liquid water content near coastal regions adjacent to continents. 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Since the potential frost flower area is parameterized as the maximum possible region on which frost flowers grow for the modeled atmospheric temperature and sea ice conditions and the model underestimates the number of accumulation-mode particles from midlatitude anthropogenic sources transported in winter, the calculated aerosol indirect effect of frost flower sea salts in this work can be regarded an upper bound. 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