Femtosecond electron-phonon lock-in by photoemission and x-ray free-electron laser
The interactions that lead to the emergence of superconductivity in iron-based materials remain a subject of debate. It has been suggested that electron-electron correlations enhance electron-phonon coupling in iron selenide (FeSe) and related pnictides, but direct experimental verification has been...
Ausführliche Beschreibung
Autor*in: |
Gerber, S [verfasserIn] |
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Artikel |
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Englisch |
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2017 |
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Rechteinformationen: |
Nutzungsrecht: © COPYRIGHT 2017 American Association for the Advancement of Science |
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Übergeordnetes Werk: |
Enthalten in: Science - Washington, DC : AAAS, American Assoc. for the Advancement of Science, 1883, 357(2017), 6346, Seite 71 |
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Übergeordnetes Werk: |
volume:357 ; year:2017 ; number:6346 ; pages:71 |
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DOI / URN: |
10.1126/science.aak9946 |
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520 | |a The interactions that lead to the emergence of superconductivity in iron-based materials remain a subject of debate. It has been suggested that electron-electron correlations enhance electron-phonon coupling in iron selenide (FeSe) and related pnictides, but direct experimental verification has been lacking. Here we show that the electron-phonon coupling strength in FeSe can be quantified by combining two time-domain experiments into a "coherent lock-in" measurement in the terahertz regime. X-ray diffraction tracks the light-induced femtosecond coherent lattice motion at a single phonon frequency, and photoemission monitors the subsequent coherent changes in the electronic band structure. Comparison with theory reveals a strong enhancement of the coupling strength in FeSe owing to correlation effects. Given that the electron-phonon coupling affects superconductivity exponentially, this enhancement highlights the importance of the cooperative interplay between electron-electron and electron-phonon interactions. | ||
540 | |a Nutzungsrecht: © COPYRIGHT 2017 American Association for the Advancement of Science | ||
650 | 4 | |a Electron-electron interactions | |
650 | 4 | |a Spin coupling | |
650 | 4 | |a Iron compounds | |
650 | 4 | |a Electric properties | |
650 | 4 | |a Research | |
650 | 4 | |a Free electron lasers | |
650 | 4 | |a Selenides | |
650 | 4 | |a Superconductivity | |
650 | 4 | |a Usage | |
700 | 1 | |a Yang, S.-L |4 oth | |
700 | 1 | |a Zhu, S |4 oth | |
700 | 1 | |a Soifer, H |4 oth | |
700 | 1 | |a Sobota, J.A |4 oth | |
700 | 1 | |a Rebec, S |4 oth | |
700 | 1 | |a Lee, J.J |4 oth | |
700 | 1 | |a Jia, T |4 oth | |
700 | 1 | |a Moritz, B |4 oth | |
700 | 1 | |a Jia, C |4 oth | |
700 | 1 | |a Gauthier, A |4 oth | |
700 | 1 | |a Li, Y |4 oth | |
700 | 1 | |a Leuenberger, D |4 oth | |
700 | 1 | |a Zhang, Y |4 oth | |
700 | 1 | |a Chaix, L |4 oth | |
700 | 1 | |a Li, W |4 oth | |
700 | 1 | |a Jang, H |4 oth | |
700 | 1 | |a Lee, J.-s |4 oth | |
700 | 1 | |a Yi, M |4 oth | |
700 | 1 | |a Dakovski, G.L |4 oth | |
700 | 1 | |a Song, S |4 oth | |
700 | 1 | |a Glownia, J.M |4 oth | |
700 | 1 | |a Nelson, S |4 oth | |
700 | 1 | |a Kim, K.W |4 oth | |
700 | 1 | |a Chuang, Y.-d |4 oth | |
700 | 1 | |a Hussain, Z |4 oth | |
700 | 1 | |a Moore, R.G |4 oth | |
700 | 1 | |a Devereaux, T.P |4 oth | |
700 | 1 | |a Lee, W.-s |4 oth | |
700 | 1 | |a Kirchmann, P.S |4 oth | |
700 | 1 | |a Shen, Z.-X |4 oth | |
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10.1126/science.aak9946 doi PQ20170901 (DE-627)OLC1995981524 (DE-599)GBVOLC1995981524 (PRQ)gale_infotrac_4998631720 (KEY)0063888920170000357634600071femtosecondelectronphononlockinbyphotoemissionandx DE-627 ger DE-627 rakwb eng 500 DE-600 LING fid Gerber, S verfasserin aut Femtosecond electron-phonon lock-in by photoemission and x-ray free-electron laser 2017 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The interactions that lead to the emergence of superconductivity in iron-based materials remain a subject of debate. It has been suggested that electron-electron correlations enhance electron-phonon coupling in iron selenide (FeSe) and related pnictides, but direct experimental verification has been lacking. Here we show that the electron-phonon coupling strength in FeSe can be quantified by combining two time-domain experiments into a "coherent lock-in" measurement in the terahertz regime. X-ray diffraction tracks the light-induced femtosecond coherent lattice motion at a single phonon frequency, and photoemission monitors the subsequent coherent changes in the electronic band structure. Comparison with theory reveals a strong enhancement of the coupling strength in FeSe owing to correlation effects. Given that the electron-phonon coupling affects superconductivity exponentially, this enhancement highlights the importance of the cooperative interplay between electron-electron and electron-phonon interactions. Nutzungsrecht: © COPYRIGHT 2017 American Association for the Advancement of Science Electron-electron interactions Spin coupling Iron compounds Electric properties Research Free electron lasers Selenides Superconductivity Usage Yang, S.-L oth Zhu, S oth Soifer, H oth Sobota, J.A oth Rebec, S oth Lee, J.J oth Jia, T oth Moritz, B oth Jia, C oth Gauthier, A oth Li, Y oth Leuenberger, D oth Zhang, Y oth Chaix, L oth Li, W oth Jang, H oth Lee, J.-s oth Yi, M oth Dakovski, G.L oth Song, S oth Glownia, J.M oth Nelson, S oth Kim, K.W oth Chuang, Y.-d oth Hussain, Z oth Moore, R.G oth Devereaux, T.P oth Lee, W.-s oth Kirchmann, P.S oth Shen, Z.-X oth Enthalten in Science Washington, DC : AAAS, American Assoc. for the Advancement of Science, 1883 357(2017), 6346, Seite 71 (DE-627)12931482X (DE-600)128410-1 (DE-576)014533189 0036-8075 nnns volume:357 year:2017 number:6346 pages:71 http://dx.doi.org/10.1126/science.aak9946 Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-LING SSG-OLC-PHY SSG-OLC-CHE SSG-OLC-MAT SSG-OLC-FOR SSG-OLC-SPO SSG-OLC-IBL SSG-OLC-PHA SSG-OLC-DE-84 SSG-OPC-FOR GBV_ILN_11 GBV_ILN_20 GBV_ILN_21 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_47 GBV_ILN_55 GBV_ILN_59 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_92 GBV_ILN_101 GBV_ILN_110 GBV_ILN_120 GBV_ILN_131 GBV_ILN_170 GBV_ILN_171 GBV_ILN_179 GBV_ILN_181 GBV_ILN_211 GBV_ILN_252 GBV_ILN_259 GBV_ILN_290 GBV_ILN_600 GBV_ILN_601 GBV_ILN_647 GBV_ILN_754 GBV_ILN_2001 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2012 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2116 GBV_ILN_2120 GBV_ILN_2121 GBV_ILN_2173 GBV_ILN_2219 GBV_ILN_2221 GBV_ILN_2279 GBV_ILN_2286 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4036 GBV_ILN_4125 GBV_ILN_4219 GBV_ILN_4251 GBV_ILN_4277 GBV_ILN_4302 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4310 GBV_ILN_4314 GBV_ILN_4317 GBV_ILN_4318 GBV_ILN_4320 GBV_ILN_4328 GBV_ILN_4333 AR 357 2017 6346 71 |
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10.1126/science.aak9946 doi PQ20170901 (DE-627)OLC1995981524 (DE-599)GBVOLC1995981524 (PRQ)gale_infotrac_4998631720 (KEY)0063888920170000357634600071femtosecondelectronphononlockinbyphotoemissionandx DE-627 ger DE-627 rakwb eng 500 DE-600 LING fid Gerber, S verfasserin aut Femtosecond electron-phonon lock-in by photoemission and x-ray free-electron laser 2017 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The interactions that lead to the emergence of superconductivity in iron-based materials remain a subject of debate. It has been suggested that electron-electron correlations enhance electron-phonon coupling in iron selenide (FeSe) and related pnictides, but direct experimental verification has been lacking. Here we show that the electron-phonon coupling strength in FeSe can be quantified by combining two time-domain experiments into a "coherent lock-in" measurement in the terahertz regime. X-ray diffraction tracks the light-induced femtosecond coherent lattice motion at a single phonon frequency, and photoemission monitors the subsequent coherent changes in the electronic band structure. Comparison with theory reveals a strong enhancement of the coupling strength in FeSe owing to correlation effects. Given that the electron-phonon coupling affects superconductivity exponentially, this enhancement highlights the importance of the cooperative interplay between electron-electron and electron-phonon interactions. Nutzungsrecht: © COPYRIGHT 2017 American Association for the Advancement of Science Electron-electron interactions Spin coupling Iron compounds Electric properties Research Free electron lasers Selenides Superconductivity Usage Yang, S.-L oth Zhu, S oth Soifer, H oth Sobota, J.A oth Rebec, S oth Lee, J.J oth Jia, T oth Moritz, B oth Jia, C oth Gauthier, A oth Li, Y oth Leuenberger, D oth Zhang, Y oth Chaix, L oth Li, W oth Jang, H oth Lee, J.-s oth Yi, M oth Dakovski, G.L oth Song, S oth Glownia, J.M oth Nelson, S oth Kim, K.W oth Chuang, Y.-d oth Hussain, Z oth Moore, R.G oth Devereaux, T.P oth Lee, W.-s oth Kirchmann, P.S oth Shen, Z.-X oth Enthalten in Science Washington, DC : AAAS, American Assoc. for the Advancement of Science, 1883 357(2017), 6346, Seite 71 (DE-627)12931482X (DE-600)128410-1 (DE-576)014533189 0036-8075 nnns volume:357 year:2017 number:6346 pages:71 http://dx.doi.org/10.1126/science.aak9946 Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-LING SSG-OLC-PHY SSG-OLC-CHE SSG-OLC-MAT SSG-OLC-FOR SSG-OLC-SPO SSG-OLC-IBL SSG-OLC-PHA SSG-OLC-DE-84 SSG-OPC-FOR GBV_ILN_11 GBV_ILN_20 GBV_ILN_21 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_47 GBV_ILN_55 GBV_ILN_59 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_92 GBV_ILN_101 GBV_ILN_110 GBV_ILN_120 GBV_ILN_131 GBV_ILN_170 GBV_ILN_171 GBV_ILN_179 GBV_ILN_181 GBV_ILN_211 GBV_ILN_252 GBV_ILN_259 GBV_ILN_290 GBV_ILN_600 GBV_ILN_601 GBV_ILN_647 GBV_ILN_754 GBV_ILN_2001 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2012 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2116 GBV_ILN_2120 GBV_ILN_2121 GBV_ILN_2173 GBV_ILN_2219 GBV_ILN_2221 GBV_ILN_2279 GBV_ILN_2286 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4036 GBV_ILN_4125 GBV_ILN_4219 GBV_ILN_4251 GBV_ILN_4277 GBV_ILN_4302 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4310 GBV_ILN_4314 GBV_ILN_4317 GBV_ILN_4318 GBV_ILN_4320 GBV_ILN_4328 GBV_ILN_4333 AR 357 2017 6346 71 |
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10.1126/science.aak9946 doi PQ20170901 (DE-627)OLC1995981524 (DE-599)GBVOLC1995981524 (PRQ)gale_infotrac_4998631720 (KEY)0063888920170000357634600071femtosecondelectronphononlockinbyphotoemissionandx DE-627 ger DE-627 rakwb eng 500 DE-600 LING fid Gerber, S verfasserin aut Femtosecond electron-phonon lock-in by photoemission and x-ray free-electron laser 2017 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The interactions that lead to the emergence of superconductivity in iron-based materials remain a subject of debate. It has been suggested that electron-electron correlations enhance electron-phonon coupling in iron selenide (FeSe) and related pnictides, but direct experimental verification has been lacking. Here we show that the electron-phonon coupling strength in FeSe can be quantified by combining two time-domain experiments into a "coherent lock-in" measurement in the terahertz regime. X-ray diffraction tracks the light-induced femtosecond coherent lattice motion at a single phonon frequency, and photoemission monitors the subsequent coherent changes in the electronic band structure. Comparison with theory reveals a strong enhancement of the coupling strength in FeSe owing to correlation effects. Given that the electron-phonon coupling affects superconductivity exponentially, this enhancement highlights the importance of the cooperative interplay between electron-electron and electron-phonon interactions. Nutzungsrecht: © COPYRIGHT 2017 American Association for the Advancement of Science Electron-electron interactions Spin coupling Iron compounds Electric properties Research Free electron lasers Selenides Superconductivity Usage Yang, S.-L oth Zhu, S oth Soifer, H oth Sobota, J.A oth Rebec, S oth Lee, J.J oth Jia, T oth Moritz, B oth Jia, C oth Gauthier, A oth Li, Y oth Leuenberger, D oth Zhang, Y oth Chaix, L oth Li, W oth Jang, H oth Lee, J.-s oth Yi, M oth Dakovski, G.L oth Song, S oth Glownia, J.M oth Nelson, S oth Kim, K.W oth Chuang, Y.-d oth Hussain, Z oth Moore, R.G oth Devereaux, T.P oth Lee, W.-s oth Kirchmann, P.S oth Shen, Z.-X oth Enthalten in Science Washington, DC : AAAS, American Assoc. for the Advancement of Science, 1883 357(2017), 6346, Seite 71 (DE-627)12931482X (DE-600)128410-1 (DE-576)014533189 0036-8075 nnns volume:357 year:2017 number:6346 pages:71 http://dx.doi.org/10.1126/science.aak9946 Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-LING SSG-OLC-PHY SSG-OLC-CHE SSG-OLC-MAT SSG-OLC-FOR SSG-OLC-SPO SSG-OLC-IBL SSG-OLC-PHA SSG-OLC-DE-84 SSG-OPC-FOR GBV_ILN_11 GBV_ILN_20 GBV_ILN_21 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_47 GBV_ILN_55 GBV_ILN_59 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_92 GBV_ILN_101 GBV_ILN_110 GBV_ILN_120 GBV_ILN_131 GBV_ILN_170 GBV_ILN_171 GBV_ILN_179 GBV_ILN_181 GBV_ILN_211 GBV_ILN_252 GBV_ILN_259 GBV_ILN_290 GBV_ILN_600 GBV_ILN_601 GBV_ILN_647 GBV_ILN_754 GBV_ILN_2001 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2012 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2116 GBV_ILN_2120 GBV_ILN_2121 GBV_ILN_2173 GBV_ILN_2219 GBV_ILN_2221 GBV_ILN_2279 GBV_ILN_2286 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4036 GBV_ILN_4125 GBV_ILN_4219 GBV_ILN_4251 GBV_ILN_4277 GBV_ILN_4302 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4310 GBV_ILN_4314 GBV_ILN_4317 GBV_ILN_4318 GBV_ILN_4320 GBV_ILN_4328 GBV_ILN_4333 AR 357 2017 6346 71 |
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10.1126/science.aak9946 doi PQ20170901 (DE-627)OLC1995981524 (DE-599)GBVOLC1995981524 (PRQ)gale_infotrac_4998631720 (KEY)0063888920170000357634600071femtosecondelectronphononlockinbyphotoemissionandx DE-627 ger DE-627 rakwb eng 500 DE-600 LING fid Gerber, S verfasserin aut Femtosecond electron-phonon lock-in by photoemission and x-ray free-electron laser 2017 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The interactions that lead to the emergence of superconductivity in iron-based materials remain a subject of debate. It has been suggested that electron-electron correlations enhance electron-phonon coupling in iron selenide (FeSe) and related pnictides, but direct experimental verification has been lacking. Here we show that the electron-phonon coupling strength in FeSe can be quantified by combining two time-domain experiments into a "coherent lock-in" measurement in the terahertz regime. X-ray diffraction tracks the light-induced femtosecond coherent lattice motion at a single phonon frequency, and photoemission monitors the subsequent coherent changes in the electronic band structure. Comparison with theory reveals a strong enhancement of the coupling strength in FeSe owing to correlation effects. Given that the electron-phonon coupling affects superconductivity exponentially, this enhancement highlights the importance of the cooperative interplay between electron-electron and electron-phonon interactions. Nutzungsrecht: © COPYRIGHT 2017 American Association for the Advancement of Science Electron-electron interactions Spin coupling Iron compounds Electric properties Research Free electron lasers Selenides Superconductivity Usage Yang, S.-L oth Zhu, S oth Soifer, H oth Sobota, J.A oth Rebec, S oth Lee, J.J oth Jia, T oth Moritz, B oth Jia, C oth Gauthier, A oth Li, Y oth Leuenberger, D oth Zhang, Y oth Chaix, L oth Li, W oth Jang, H oth Lee, J.-s oth Yi, M oth Dakovski, G.L oth Song, S oth Glownia, J.M oth Nelson, S oth Kim, K.W oth Chuang, Y.-d oth Hussain, Z oth Moore, R.G oth Devereaux, T.P oth Lee, W.-s oth Kirchmann, P.S oth Shen, Z.-X oth Enthalten in Science Washington, DC : AAAS, American Assoc. for the Advancement of Science, 1883 357(2017), 6346, Seite 71 (DE-627)12931482X (DE-600)128410-1 (DE-576)014533189 0036-8075 nnns volume:357 year:2017 number:6346 pages:71 http://dx.doi.org/10.1126/science.aak9946 Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-LING SSG-OLC-PHY SSG-OLC-CHE SSG-OLC-MAT SSG-OLC-FOR SSG-OLC-SPO SSG-OLC-IBL SSG-OLC-PHA SSG-OLC-DE-84 SSG-OPC-FOR GBV_ILN_11 GBV_ILN_20 GBV_ILN_21 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_47 GBV_ILN_55 GBV_ILN_59 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_92 GBV_ILN_101 GBV_ILN_110 GBV_ILN_120 GBV_ILN_131 GBV_ILN_170 GBV_ILN_171 GBV_ILN_179 GBV_ILN_181 GBV_ILN_211 GBV_ILN_252 GBV_ILN_259 GBV_ILN_290 GBV_ILN_600 GBV_ILN_601 GBV_ILN_647 GBV_ILN_754 GBV_ILN_2001 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2012 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2116 GBV_ILN_2120 GBV_ILN_2121 GBV_ILN_2173 GBV_ILN_2219 GBV_ILN_2221 GBV_ILN_2279 GBV_ILN_2286 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4036 GBV_ILN_4125 GBV_ILN_4219 GBV_ILN_4251 GBV_ILN_4277 GBV_ILN_4302 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4310 GBV_ILN_4314 GBV_ILN_4317 GBV_ILN_4318 GBV_ILN_4320 GBV_ILN_4328 GBV_ILN_4333 AR 357 2017 6346 71 |
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10.1126/science.aak9946 doi PQ20170901 (DE-627)OLC1995981524 (DE-599)GBVOLC1995981524 (PRQ)gale_infotrac_4998631720 (KEY)0063888920170000357634600071femtosecondelectronphononlockinbyphotoemissionandx DE-627 ger DE-627 rakwb eng 500 DE-600 LING fid Gerber, S verfasserin aut Femtosecond electron-phonon lock-in by photoemission and x-ray free-electron laser 2017 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier The interactions that lead to the emergence of superconductivity in iron-based materials remain a subject of debate. It has been suggested that electron-electron correlations enhance electron-phonon coupling in iron selenide (FeSe) and related pnictides, but direct experimental verification has been lacking. Here we show that the electron-phonon coupling strength in FeSe can be quantified by combining two time-domain experiments into a "coherent lock-in" measurement in the terahertz regime. X-ray diffraction tracks the light-induced femtosecond coherent lattice motion at a single phonon frequency, and photoemission monitors the subsequent coherent changes in the electronic band structure. Comparison with theory reveals a strong enhancement of the coupling strength in FeSe owing to correlation effects. Given that the electron-phonon coupling affects superconductivity exponentially, this enhancement highlights the importance of the cooperative interplay between electron-electron and electron-phonon interactions. Nutzungsrecht: © COPYRIGHT 2017 American Association for the Advancement of Science Electron-electron interactions Spin coupling Iron compounds Electric properties Research Free electron lasers Selenides Superconductivity Usage Yang, S.-L oth Zhu, S oth Soifer, H oth Sobota, J.A oth Rebec, S oth Lee, J.J oth Jia, T oth Moritz, B oth Jia, C oth Gauthier, A oth Li, Y oth Leuenberger, D oth Zhang, Y oth Chaix, L oth Li, W oth Jang, H oth Lee, J.-s oth Yi, M oth Dakovski, G.L oth Song, S oth Glownia, J.M oth Nelson, S oth Kim, K.W oth Chuang, Y.-d oth Hussain, Z oth Moore, R.G oth Devereaux, T.P oth Lee, W.-s oth Kirchmann, P.S oth Shen, Z.-X oth Enthalten in Science Washington, DC : AAAS, American Assoc. for the Advancement of Science, 1883 357(2017), 6346, Seite 71 (DE-627)12931482X (DE-600)128410-1 (DE-576)014533189 0036-8075 nnns volume:357 year:2017 number:6346 pages:71 http://dx.doi.org/10.1126/science.aak9946 Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-LING SSG-OLC-PHY SSG-OLC-CHE SSG-OLC-MAT SSG-OLC-FOR SSG-OLC-SPO SSG-OLC-IBL SSG-OLC-PHA SSG-OLC-DE-84 SSG-OPC-FOR GBV_ILN_11 GBV_ILN_20 GBV_ILN_21 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_47 GBV_ILN_55 GBV_ILN_59 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_92 GBV_ILN_101 GBV_ILN_110 GBV_ILN_120 GBV_ILN_131 GBV_ILN_170 GBV_ILN_171 GBV_ILN_179 GBV_ILN_181 GBV_ILN_211 GBV_ILN_252 GBV_ILN_259 GBV_ILN_290 GBV_ILN_600 GBV_ILN_601 GBV_ILN_647 GBV_ILN_754 GBV_ILN_2001 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2012 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2018 GBV_ILN_2020 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2116 GBV_ILN_2120 GBV_ILN_2121 GBV_ILN_2173 GBV_ILN_2219 GBV_ILN_2221 GBV_ILN_2279 GBV_ILN_2286 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4036 GBV_ILN_4125 GBV_ILN_4219 GBV_ILN_4251 GBV_ILN_4277 GBV_ILN_4302 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4310 GBV_ILN_4314 GBV_ILN_4317 GBV_ILN_4318 GBV_ILN_4320 GBV_ILN_4328 GBV_ILN_4333 AR 357 2017 6346 71 |
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Gerber, S @@aut@@ Yang, S.-L @@oth@@ Zhu, S @@oth@@ Soifer, H @@oth@@ Sobota, J.A @@oth@@ Rebec, S @@oth@@ Lee, J.J @@oth@@ Jia, T @@oth@@ Moritz, B @@oth@@ Jia, C @@oth@@ Gauthier, A @@oth@@ Li, Y @@oth@@ Leuenberger, D @@oth@@ Zhang, Y @@oth@@ Chaix, L @@oth@@ Li, W @@oth@@ Jang, H @@oth@@ Lee, J.-s @@oth@@ Yi, M @@oth@@ Dakovski, G.L @@oth@@ Song, S @@oth@@ Glownia, J.M @@oth@@ Nelson, S @@oth@@ Kim, K.W @@oth@@ Chuang, Y.-d @@oth@@ Hussain, Z @@oth@@ Moore, R.G @@oth@@ Devereaux, T.P @@oth@@ Lee, W.-s @@oth@@ Kirchmann, P.S @@oth@@ Shen, Z.-X @@oth@@ |
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2017-01-01T00:00:00Z |
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femtosecond electron-phonon lock-in by photoemission and x-ray free-electron laser |
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Femtosecond electron-phonon lock-in by photoemission and x-ray free-electron laser |
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The interactions that lead to the emergence of superconductivity in iron-based materials remain a subject of debate. It has been suggested that electron-electron correlations enhance electron-phonon coupling in iron selenide (FeSe) and related pnictides, but direct experimental verification has been lacking. Here we show that the electron-phonon coupling strength in FeSe can be quantified by combining two time-domain experiments into a "coherent lock-in" measurement in the terahertz regime. X-ray diffraction tracks the light-induced femtosecond coherent lattice motion at a single phonon frequency, and photoemission monitors the subsequent coherent changes in the electronic band structure. Comparison with theory reveals a strong enhancement of the coupling strength in FeSe owing to correlation effects. Given that the electron-phonon coupling affects superconductivity exponentially, this enhancement highlights the importance of the cooperative interplay between electron-electron and electron-phonon interactions. |
abstractGer |
The interactions that lead to the emergence of superconductivity in iron-based materials remain a subject of debate. It has been suggested that electron-electron correlations enhance electron-phonon coupling in iron selenide (FeSe) and related pnictides, but direct experimental verification has been lacking. Here we show that the electron-phonon coupling strength in FeSe can be quantified by combining two time-domain experiments into a "coherent lock-in" measurement in the terahertz regime. X-ray diffraction tracks the light-induced femtosecond coherent lattice motion at a single phonon frequency, and photoemission monitors the subsequent coherent changes in the electronic band structure. Comparison with theory reveals a strong enhancement of the coupling strength in FeSe owing to correlation effects. Given that the electron-phonon coupling affects superconductivity exponentially, this enhancement highlights the importance of the cooperative interplay between electron-electron and electron-phonon interactions. |
abstract_unstemmed |
The interactions that lead to the emergence of superconductivity in iron-based materials remain a subject of debate. It has been suggested that electron-electron correlations enhance electron-phonon coupling in iron selenide (FeSe) and related pnictides, but direct experimental verification has been lacking. Here we show that the electron-phonon coupling strength in FeSe can be quantified by combining two time-domain experiments into a "coherent lock-in" measurement in the terahertz regime. X-ray diffraction tracks the light-induced femtosecond coherent lattice motion at a single phonon frequency, and photoemission monitors the subsequent coherent changes in the electronic band structure. Comparison with theory reveals a strong enhancement of the coupling strength in FeSe owing to correlation effects. Given that the electron-phonon coupling affects superconductivity exponentially, this enhancement highlights the importance of the cooperative interplay between electron-electron and electron-phonon interactions. |
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Femtosecond electron-phonon lock-in by photoemission and x-ray free-electron laser |
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Yang, S.-L Zhu, S Soifer, H Sobota, J.A Rebec, S Lee, J.J Jia, T Moritz, B Jia, C Gauthier, A Li, Y Leuenberger, D Zhang, Y Chaix, L Li, W Jang, H Lee, J.-s Yi, M Dakovski, G.L Song, S Glownia, J.M Nelson, S Kim, K.W Chuang, Y.-d Hussain, Z Moore, R.G Devereaux, T.P Lee, W.-s Kirchmann, P.S Shen, Z.-X |
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