Effect of particle size, iron ligands and anions on ciprofloxacin degradation in zero‐valent iron process: application to sewage treatment plant effluent
BACKGROUND Ciprofloxacin (CIP) is an antibiotic largely used to treat bacterial infections and found in sewage treatment plant (STP) effluent. Zero valent iron (ZVI, Fe0) technology has great potential for the degradation of residual pharmaceuticals. The effect of some parameters (anaerobic/aerobic,...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
de Lima Perini, João Angelo [verfasserIn] |
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| Format: |
Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2017 |
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| Rechteinformationen: |
Nutzungsrecht: © 2017 Society of Chemical Industry |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Journal of chemical technology and biotechnology - Chichester, Sussex : Wiley, 1979, 92(2017), 9, Seite 2300-2308 |
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| Übergeordnetes Werk: |
volume:92 ; year:2017 ; number:9 ; pages:2300-2308 |
| Links: |
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| DOI / URN: |
10.1002/jctb.5227 |
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OLC1997497360 |
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| 245 | 1 | 0 | |a Effect of particle size, iron ligands and anions on ciprofloxacin degradation in zero‐valent iron process: application to sewage treatment plant effluent |
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| 520 | |a BACKGROUND Ciprofloxacin (CIP) is an antibiotic largely used to treat bacterial infections and found in sewage treatment plant (STP) effluent. Zero valent iron (ZVI, Fe0) technology has great potential for the degradation of residual pharmaceuticals. The effect of some parameters (anaerobic/aerobic, particle size, iron ligands and anions) were evaluated for CIP degradation in distilled water (DW) and finally compared to that obtained in STP effluent. RESULTS The smaller ZVI particle (200 mesh) resulted in a lower degradation rate than the larger particle (20 mesh) in both anaerobic and aerobic treatment. This is due mainly to the fast generation of Fe2+, hindering the degradation process due to *OH scavenging. A linear increase of CIP degradation rate was observed when the reaction was carried out with increasing EDTA concentrations. The Cl- anions had a positive effect on CIP degradation in the ZVI process. On the other hand, the presence of NO3- resulted in a decrease of degradation rate, both with 20 and 200 mesh particles. CIP could be degraded in two STP effluents mediated by ZVI (20 mesh). CONCLUSIONS The ZVI process can be used efficiently for the degradation of CIP in two types of STP effluent (anaerobic treatment or anaerobic/aerobic treatment), revealing a possible applicability of the ZVI process to this type of matrix. © 2017 Society of Chemical Industry | ||
| 540 | |a Nutzungsrecht: © 2017 Society of Chemical Industry | ||
| 650 | 4 | |a STP effluent | |
| 650 | 4 | |a DOC removal | |
| 650 | 4 | |a degradation | |
| 650 | 4 | |a Fenton | |
| 650 | 4 | |a Anions | |
| 650 | 4 | |a Biodegradation | |
| 650 | 4 | |a Degradation | |
| 650 | 4 | |a Aerobic treatment | |
| 650 | 4 | |a Chloride | |
| 650 | 4 | |a Antibiotics | |
| 650 | 4 | |a Sewage treatment plants | |
| 650 | 4 | |a Wastewater treatment | |
| 650 | 4 | |a Sewage disposal | |
| 650 | 4 | |a Ciprofloxacin | |
| 650 | 4 | |a Sewage treatment | |
| 650 | 4 | |a Drugs | |
| 650 | 4 | |a Particle size | |
| 650 | 4 | |a Bacteria | |
| 650 | 4 | |a Waste treatment | |
| 650 | 4 | |a Effluents | |
| 650 | 4 | |a Anaerobic processes | |
| 650 | 4 | |a Anaerobic digestion | |
| 650 | 4 | |a Anaerobic treatment | |
| 650 | 4 | |a Sewage | |
| 650 | 4 | |a Ethylenediaminetetraacetic acids | |
| 650 | 4 | |a Distilled water | |
| 650 | 4 | |a Scavenging | |
| 650 | 4 | |a Iron | |
| 650 | 4 | |a Ligands | |
| 700 | 1 | |a Nogueira, Raquel Fernandes Pupo |4 oth | |
| 773 | 0 | 8 | |i Enthalten in |t Journal of chemical technology and biotechnology |d Chichester, Sussex : Wiley, 1979 |g 92(2017), 9, Seite 2300-2308 |w (DE-627)12909546X |w (DE-600)7483-4 |w (DE-576)014431602 |x 0142-0356 |7 nnns |
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10.1002/jctb.5227 doi PQ20171228 (DE-627)OLC1997497360 (DE-599)GBVOLC1997497360 (PRQ)c2279-af899e8d9a3bfd7fc5bd22321c4a58695a828faaf028d8bf9a706d2b8e5409a23 (KEY)0074631220170000092000902300effectofparticlesizeironligandsandanionsonciproflo DE-627 ger DE-627 rakwb eng 660 620 DE-600 de Lima Perini, João Angelo verfasserin aut Effect of particle size, iron ligands and anions on ciprofloxacin degradation in zero‐valent iron process: application to sewage treatment plant effluent 2017 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier BACKGROUND Ciprofloxacin (CIP) is an antibiotic largely used to treat bacterial infections and found in sewage treatment plant (STP) effluent. Zero valent iron (ZVI, Fe0) technology has great potential for the degradation of residual pharmaceuticals. The effect of some parameters (anaerobic/aerobic, particle size, iron ligands and anions) were evaluated for CIP degradation in distilled water (DW) and finally compared to that obtained in STP effluent. RESULTS The smaller ZVI particle (200 mesh) resulted in a lower degradation rate than the larger particle (20 mesh) in both anaerobic and aerobic treatment. This is due mainly to the fast generation of Fe2+, hindering the degradation process due to *OH scavenging. A linear increase of CIP degradation rate was observed when the reaction was carried out with increasing EDTA concentrations. The Cl- anions had a positive effect on CIP degradation in the ZVI process. On the other hand, the presence of NO3- resulted in a decrease of degradation rate, both with 20 and 200 mesh particles. CIP could be degraded in two STP effluents mediated by ZVI (20 mesh). CONCLUSIONS The ZVI process can be used efficiently for the degradation of CIP in two types of STP effluent (anaerobic treatment or anaerobic/aerobic treatment), revealing a possible applicability of the ZVI process to this type of matrix. © 2017 Society of Chemical Industry Nutzungsrecht: © 2017 Society of Chemical Industry STP effluent DOC removal degradation Fenton Anions Biodegradation Degradation Aerobic treatment Chloride Antibiotics Sewage treatment plants Wastewater treatment Sewage disposal Ciprofloxacin Sewage treatment Drugs Particle size Bacteria Waste treatment Effluents Anaerobic processes Anaerobic digestion Anaerobic treatment Sewage Ethylenediaminetetraacetic acids Distilled water Scavenging Iron Ligands Nogueira, Raquel Fernandes Pupo oth Enthalten in Journal of chemical technology and biotechnology Chichester, Sussex : Wiley, 1979 92(2017), 9, Seite 2300-2308 (DE-627)12909546X (DE-600)7483-4 (DE-576)014431602 0142-0356 nnns volume:92 year:2017 number:9 pages:2300-2308 http://dx.doi.org/10.1002/jctb.5227 Volltext http://onlinelibrary.wiley.com/doi/10.1002/jctb.5227/abstract https://search.proquest.com/docview/1929830579 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-PHA SSG-OLC-DE-84 GBV_ILN_70 AR 92 2017 9 2300-2308 |
| spelling |
10.1002/jctb.5227 doi PQ20171228 (DE-627)OLC1997497360 (DE-599)GBVOLC1997497360 (PRQ)c2279-af899e8d9a3bfd7fc5bd22321c4a58695a828faaf028d8bf9a706d2b8e5409a23 (KEY)0074631220170000092000902300effectofparticlesizeironligandsandanionsonciproflo DE-627 ger DE-627 rakwb eng 660 620 DE-600 de Lima Perini, João Angelo verfasserin aut Effect of particle size, iron ligands and anions on ciprofloxacin degradation in zero‐valent iron process: application to sewage treatment plant effluent 2017 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier BACKGROUND Ciprofloxacin (CIP) is an antibiotic largely used to treat bacterial infections and found in sewage treatment plant (STP) effluent. Zero valent iron (ZVI, Fe0) technology has great potential for the degradation of residual pharmaceuticals. The effect of some parameters (anaerobic/aerobic, particle size, iron ligands and anions) were evaluated for CIP degradation in distilled water (DW) and finally compared to that obtained in STP effluent. RESULTS The smaller ZVI particle (200 mesh) resulted in a lower degradation rate than the larger particle (20 mesh) in both anaerobic and aerobic treatment. This is due mainly to the fast generation of Fe2+, hindering the degradation process due to *OH scavenging. A linear increase of CIP degradation rate was observed when the reaction was carried out with increasing EDTA concentrations. The Cl- anions had a positive effect on CIP degradation in the ZVI process. On the other hand, the presence of NO3- resulted in a decrease of degradation rate, both with 20 and 200 mesh particles. CIP could be degraded in two STP effluents mediated by ZVI (20 mesh). CONCLUSIONS The ZVI process can be used efficiently for the degradation of CIP in two types of STP effluent (anaerobic treatment or anaerobic/aerobic treatment), revealing a possible applicability of the ZVI process to this type of matrix. © 2017 Society of Chemical Industry Nutzungsrecht: © 2017 Society of Chemical Industry STP effluent DOC removal degradation Fenton Anions Biodegradation Degradation Aerobic treatment Chloride Antibiotics Sewage treatment plants Wastewater treatment Sewage disposal Ciprofloxacin Sewage treatment Drugs Particle size Bacteria Waste treatment Effluents Anaerobic processes Anaerobic digestion Anaerobic treatment Sewage Ethylenediaminetetraacetic acids Distilled water Scavenging Iron Ligands Nogueira, Raquel Fernandes Pupo oth Enthalten in Journal of chemical technology and biotechnology Chichester, Sussex : Wiley, 1979 92(2017), 9, Seite 2300-2308 (DE-627)12909546X (DE-600)7483-4 (DE-576)014431602 0142-0356 nnns volume:92 year:2017 number:9 pages:2300-2308 http://dx.doi.org/10.1002/jctb.5227 Volltext http://onlinelibrary.wiley.com/doi/10.1002/jctb.5227/abstract https://search.proquest.com/docview/1929830579 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-PHA SSG-OLC-DE-84 GBV_ILN_70 AR 92 2017 9 2300-2308 |
| allfields_unstemmed |
10.1002/jctb.5227 doi PQ20171228 (DE-627)OLC1997497360 (DE-599)GBVOLC1997497360 (PRQ)c2279-af899e8d9a3bfd7fc5bd22321c4a58695a828faaf028d8bf9a706d2b8e5409a23 (KEY)0074631220170000092000902300effectofparticlesizeironligandsandanionsonciproflo DE-627 ger DE-627 rakwb eng 660 620 DE-600 de Lima Perini, João Angelo verfasserin aut Effect of particle size, iron ligands and anions on ciprofloxacin degradation in zero‐valent iron process: application to sewage treatment plant effluent 2017 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier BACKGROUND Ciprofloxacin (CIP) is an antibiotic largely used to treat bacterial infections and found in sewage treatment plant (STP) effluent. Zero valent iron (ZVI, Fe0) technology has great potential for the degradation of residual pharmaceuticals. The effect of some parameters (anaerobic/aerobic, particle size, iron ligands and anions) were evaluated for CIP degradation in distilled water (DW) and finally compared to that obtained in STP effluent. RESULTS The smaller ZVI particle (200 mesh) resulted in a lower degradation rate than the larger particle (20 mesh) in both anaerobic and aerobic treatment. This is due mainly to the fast generation of Fe2+, hindering the degradation process due to *OH scavenging. A linear increase of CIP degradation rate was observed when the reaction was carried out with increasing EDTA concentrations. The Cl- anions had a positive effect on CIP degradation in the ZVI process. On the other hand, the presence of NO3- resulted in a decrease of degradation rate, both with 20 and 200 mesh particles. CIP could be degraded in two STP effluents mediated by ZVI (20 mesh). CONCLUSIONS The ZVI process can be used efficiently for the degradation of CIP in two types of STP effluent (anaerobic treatment or anaerobic/aerobic treatment), revealing a possible applicability of the ZVI process to this type of matrix. © 2017 Society of Chemical Industry Nutzungsrecht: © 2017 Society of Chemical Industry STP effluent DOC removal degradation Fenton Anions Biodegradation Degradation Aerobic treatment Chloride Antibiotics Sewage treatment plants Wastewater treatment Sewage disposal Ciprofloxacin Sewage treatment Drugs Particle size Bacteria Waste treatment Effluents Anaerobic processes Anaerobic digestion Anaerobic treatment Sewage Ethylenediaminetetraacetic acids Distilled water Scavenging Iron Ligands Nogueira, Raquel Fernandes Pupo oth Enthalten in Journal of chemical technology and biotechnology Chichester, Sussex : Wiley, 1979 92(2017), 9, Seite 2300-2308 (DE-627)12909546X (DE-600)7483-4 (DE-576)014431602 0142-0356 nnns volume:92 year:2017 number:9 pages:2300-2308 http://dx.doi.org/10.1002/jctb.5227 Volltext http://onlinelibrary.wiley.com/doi/10.1002/jctb.5227/abstract https://search.proquest.com/docview/1929830579 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-PHA SSG-OLC-DE-84 GBV_ILN_70 AR 92 2017 9 2300-2308 |
| allfieldsGer |
10.1002/jctb.5227 doi PQ20171228 (DE-627)OLC1997497360 (DE-599)GBVOLC1997497360 (PRQ)c2279-af899e8d9a3bfd7fc5bd22321c4a58695a828faaf028d8bf9a706d2b8e5409a23 (KEY)0074631220170000092000902300effectofparticlesizeironligandsandanionsonciproflo DE-627 ger DE-627 rakwb eng 660 620 DE-600 de Lima Perini, João Angelo verfasserin aut Effect of particle size, iron ligands and anions on ciprofloxacin degradation in zero‐valent iron process: application to sewage treatment plant effluent 2017 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier BACKGROUND Ciprofloxacin (CIP) is an antibiotic largely used to treat bacterial infections and found in sewage treatment plant (STP) effluent. Zero valent iron (ZVI, Fe0) technology has great potential for the degradation of residual pharmaceuticals. The effect of some parameters (anaerobic/aerobic, particle size, iron ligands and anions) were evaluated for CIP degradation in distilled water (DW) and finally compared to that obtained in STP effluent. RESULTS The smaller ZVI particle (200 mesh) resulted in a lower degradation rate than the larger particle (20 mesh) in both anaerobic and aerobic treatment. This is due mainly to the fast generation of Fe2+, hindering the degradation process due to *OH scavenging. A linear increase of CIP degradation rate was observed when the reaction was carried out with increasing EDTA concentrations. The Cl- anions had a positive effect on CIP degradation in the ZVI process. On the other hand, the presence of NO3- resulted in a decrease of degradation rate, both with 20 and 200 mesh particles. CIP could be degraded in two STP effluents mediated by ZVI (20 mesh). CONCLUSIONS The ZVI process can be used efficiently for the degradation of CIP in two types of STP effluent (anaerobic treatment or anaerobic/aerobic treatment), revealing a possible applicability of the ZVI process to this type of matrix. © 2017 Society of Chemical Industry Nutzungsrecht: © 2017 Society of Chemical Industry STP effluent DOC removal degradation Fenton Anions Biodegradation Degradation Aerobic treatment Chloride Antibiotics Sewage treatment plants Wastewater treatment Sewage disposal Ciprofloxacin Sewage treatment Drugs Particle size Bacteria Waste treatment Effluents Anaerobic processes Anaerobic digestion Anaerobic treatment Sewage Ethylenediaminetetraacetic acids Distilled water Scavenging Iron Ligands Nogueira, Raquel Fernandes Pupo oth Enthalten in Journal of chemical technology and biotechnology Chichester, Sussex : Wiley, 1979 92(2017), 9, Seite 2300-2308 (DE-627)12909546X (DE-600)7483-4 (DE-576)014431602 0142-0356 nnns volume:92 year:2017 number:9 pages:2300-2308 http://dx.doi.org/10.1002/jctb.5227 Volltext http://onlinelibrary.wiley.com/doi/10.1002/jctb.5227/abstract https://search.proquest.com/docview/1929830579 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-PHA SSG-OLC-DE-84 GBV_ILN_70 AR 92 2017 9 2300-2308 |
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10.1002/jctb.5227 doi PQ20171228 (DE-627)OLC1997497360 (DE-599)GBVOLC1997497360 (PRQ)c2279-af899e8d9a3bfd7fc5bd22321c4a58695a828faaf028d8bf9a706d2b8e5409a23 (KEY)0074631220170000092000902300effectofparticlesizeironligandsandanionsonciproflo DE-627 ger DE-627 rakwb eng 660 620 DE-600 de Lima Perini, João Angelo verfasserin aut Effect of particle size, iron ligands and anions on ciprofloxacin degradation in zero‐valent iron process: application to sewage treatment plant effluent 2017 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier BACKGROUND Ciprofloxacin (CIP) is an antibiotic largely used to treat bacterial infections and found in sewage treatment plant (STP) effluent. Zero valent iron (ZVI, Fe0) technology has great potential for the degradation of residual pharmaceuticals. The effect of some parameters (anaerobic/aerobic, particle size, iron ligands and anions) were evaluated for CIP degradation in distilled water (DW) and finally compared to that obtained in STP effluent. RESULTS The smaller ZVI particle (200 mesh) resulted in a lower degradation rate than the larger particle (20 mesh) in both anaerobic and aerobic treatment. This is due mainly to the fast generation of Fe2+, hindering the degradation process due to *OH scavenging. A linear increase of CIP degradation rate was observed when the reaction was carried out with increasing EDTA concentrations. The Cl- anions had a positive effect on CIP degradation in the ZVI process. On the other hand, the presence of NO3- resulted in a decrease of degradation rate, both with 20 and 200 mesh particles. CIP could be degraded in two STP effluents mediated by ZVI (20 mesh). CONCLUSIONS The ZVI process can be used efficiently for the degradation of CIP in two types of STP effluent (anaerobic treatment or anaerobic/aerobic treatment), revealing a possible applicability of the ZVI process to this type of matrix. © 2017 Society of Chemical Industry Nutzungsrecht: © 2017 Society of Chemical Industry STP effluent DOC removal degradation Fenton Anions Biodegradation Degradation Aerobic treatment Chloride Antibiotics Sewage treatment plants Wastewater treatment Sewage disposal Ciprofloxacin Sewage treatment Drugs Particle size Bacteria Waste treatment Effluents Anaerobic processes Anaerobic digestion Anaerobic treatment Sewage Ethylenediaminetetraacetic acids Distilled water Scavenging Iron Ligands Nogueira, Raquel Fernandes Pupo oth Enthalten in Journal of chemical technology and biotechnology Chichester, Sussex : Wiley, 1979 92(2017), 9, Seite 2300-2308 (DE-627)12909546X (DE-600)7483-4 (DE-576)014431602 0142-0356 nnns volume:92 year:2017 number:9 pages:2300-2308 http://dx.doi.org/10.1002/jctb.5227 Volltext http://onlinelibrary.wiley.com/doi/10.1002/jctb.5227/abstract https://search.proquest.com/docview/1929830579 GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-PHA SSG-OLC-DE-84 GBV_ILN_70 AR 92 2017 9 2300-2308 |
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Zero valent iron (ZVI, Fe0) technology has great potential for the degradation of residual pharmaceuticals. The effect of some parameters (anaerobic/aerobic, particle size, iron ligands and anions) were evaluated for CIP degradation in distilled water (DW) and finally compared to that obtained in STP effluent. RESULTS The smaller ZVI particle (200 mesh) resulted in a lower degradation rate than the larger particle (20 mesh) in both anaerobic and aerobic treatment. This is due mainly to the fast generation of Fe2+, hindering the degradation process due to *OH scavenging. A linear increase of CIP degradation rate was observed when the reaction was carried out with increasing EDTA concentrations. The Cl- anions had a positive effect on CIP degradation in the ZVI process. On the other hand, the presence of NO3- resulted in a decrease of degradation rate, both with 20 and 200 mesh particles. CIP could be degraded in two STP effluents mediated by ZVI (20 mesh). 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de Lima Perini, João Angelo ddc 660 misc STP effluent misc DOC removal misc degradation misc Fenton misc Anions misc Biodegradation misc Degradation misc Aerobic treatment misc Chloride misc Antibiotics misc Sewage treatment plants misc Wastewater treatment misc Sewage disposal misc Ciprofloxacin misc Sewage treatment misc Drugs misc Particle size misc Bacteria misc Waste treatment misc Effluents misc Anaerobic processes misc Anaerobic digestion misc Anaerobic treatment misc Sewage misc Ethylenediaminetetraacetic acids misc Distilled water misc Scavenging misc Iron misc Ligands Effect of particle size, iron ligands and anions on ciprofloxacin degradation in zero‐valent iron process: application to sewage treatment plant effluent |
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660 620 DE-600 Effect of particle size, iron ligands and anions on ciprofloxacin degradation in zero‐valent iron process: application to sewage treatment plant effluent STP effluent DOC removal degradation Fenton Anions Biodegradation Degradation Aerobic treatment Chloride Antibiotics Sewage treatment plants Wastewater treatment Sewage disposal Ciprofloxacin Sewage treatment Drugs Particle size Bacteria Waste treatment Effluents Anaerobic processes Anaerobic digestion Anaerobic treatment Sewage Ethylenediaminetetraacetic acids Distilled water Scavenging Iron Ligands |
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ddc 660 misc STP effluent misc DOC removal misc degradation misc Fenton misc Anions misc Biodegradation misc Degradation misc Aerobic treatment misc Chloride misc Antibiotics misc Sewage treatment plants misc Wastewater treatment misc Sewage disposal misc Ciprofloxacin misc Sewage treatment misc Drugs misc Particle size misc Bacteria misc Waste treatment misc Effluents misc Anaerobic processes misc Anaerobic digestion misc Anaerobic treatment misc Sewage misc Ethylenediaminetetraacetic acids misc Distilled water misc Scavenging misc Iron misc Ligands |
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Effect of particle size, iron ligands and anions on ciprofloxacin degradation in zero‐valent iron process: application to sewage treatment plant effluent |
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Effect of particle size, iron ligands and anions on ciprofloxacin degradation in zero‐valent iron process: application to sewage treatment plant effluent |
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de Lima Perini, João Angelo |
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effect of particle size, iron ligands and anions on ciprofloxacin degradation in zero‐valent iron process: application to sewage treatment plant effluent |
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Effect of particle size, iron ligands and anions on ciprofloxacin degradation in zero‐valent iron process: application to sewage treatment plant effluent |
| abstract |
BACKGROUND Ciprofloxacin (CIP) is an antibiotic largely used to treat bacterial infections and found in sewage treatment plant (STP) effluent. Zero valent iron (ZVI, Fe0) technology has great potential for the degradation of residual pharmaceuticals. The effect of some parameters (anaerobic/aerobic, particle size, iron ligands and anions) were evaluated for CIP degradation in distilled water (DW) and finally compared to that obtained in STP effluent. RESULTS The smaller ZVI particle (200 mesh) resulted in a lower degradation rate than the larger particle (20 mesh) in both anaerobic and aerobic treatment. This is due mainly to the fast generation of Fe2+, hindering the degradation process due to *OH scavenging. A linear increase of CIP degradation rate was observed when the reaction was carried out with increasing EDTA concentrations. The Cl- anions had a positive effect on CIP degradation in the ZVI process. On the other hand, the presence of NO3- resulted in a decrease of degradation rate, both with 20 and 200 mesh particles. CIP could be degraded in two STP effluents mediated by ZVI (20 mesh). CONCLUSIONS The ZVI process can be used efficiently for the degradation of CIP in two types of STP effluent (anaerobic treatment or anaerobic/aerobic treatment), revealing a possible applicability of the ZVI process to this type of matrix. © 2017 Society of Chemical Industry |
| abstractGer |
BACKGROUND Ciprofloxacin (CIP) is an antibiotic largely used to treat bacterial infections and found in sewage treatment plant (STP) effluent. Zero valent iron (ZVI, Fe0) technology has great potential for the degradation of residual pharmaceuticals. The effect of some parameters (anaerobic/aerobic, particle size, iron ligands and anions) were evaluated for CIP degradation in distilled water (DW) and finally compared to that obtained in STP effluent. RESULTS The smaller ZVI particle (200 mesh) resulted in a lower degradation rate than the larger particle (20 mesh) in both anaerobic and aerobic treatment. This is due mainly to the fast generation of Fe2+, hindering the degradation process due to *OH scavenging. A linear increase of CIP degradation rate was observed when the reaction was carried out with increasing EDTA concentrations. The Cl- anions had a positive effect on CIP degradation in the ZVI process. On the other hand, the presence of NO3- resulted in a decrease of degradation rate, both with 20 and 200 mesh particles. CIP could be degraded in two STP effluents mediated by ZVI (20 mesh). CONCLUSIONS The ZVI process can be used efficiently for the degradation of CIP in two types of STP effluent (anaerobic treatment or anaerobic/aerobic treatment), revealing a possible applicability of the ZVI process to this type of matrix. © 2017 Society of Chemical Industry |
| abstract_unstemmed |
BACKGROUND Ciprofloxacin (CIP) is an antibiotic largely used to treat bacterial infections and found in sewage treatment plant (STP) effluent. Zero valent iron (ZVI, Fe0) technology has great potential for the degradation of residual pharmaceuticals. The effect of some parameters (anaerobic/aerobic, particle size, iron ligands and anions) were evaluated for CIP degradation in distilled water (DW) and finally compared to that obtained in STP effluent. RESULTS The smaller ZVI particle (200 mesh) resulted in a lower degradation rate than the larger particle (20 mesh) in both anaerobic and aerobic treatment. This is due mainly to the fast generation of Fe2+, hindering the degradation process due to *OH scavenging. A linear increase of CIP degradation rate was observed when the reaction was carried out with increasing EDTA concentrations. The Cl- anions had a positive effect on CIP degradation in the ZVI process. On the other hand, the presence of NO3- resulted in a decrease of degradation rate, both with 20 and 200 mesh particles. CIP could be degraded in two STP effluents mediated by ZVI (20 mesh). CONCLUSIONS The ZVI process can be used efficiently for the degradation of CIP in two types of STP effluent (anaerobic treatment or anaerobic/aerobic treatment), revealing a possible applicability of the ZVI process to this type of matrix. © 2017 Society of Chemical Industry |
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Effect of particle size, iron ligands and anions on ciprofloxacin degradation in zero‐valent iron process: application to sewage treatment plant effluent |
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http://dx.doi.org/10.1002/jctb.5227 http://onlinelibrary.wiley.com/doi/10.1002/jctb.5227/abstract https://search.proquest.com/docview/1929830579 |
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