Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell
Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much...
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Gespeichert in:
| Autor*in: |
Li, Wan [verfasserIn] |
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| Format: |
Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2016 |
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| Schlagwörter: |
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| Systematik: |
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| Anmerkung: |
© Springer Science+Business Media New York 2016 |
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| Übergeordnetes Werk: |
Enthalten in: Catalysis letters - Springer US, 1988, 146(2016), 12 vom: 28. Okt., Seite 2585-2595 |
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| Übergeordnetes Werk: |
volume:146 ; year:2016 ; number:12 ; day:28 ; month:10 ; pages:2585-2595 |
| Links: |
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| DOI / URN: |
10.1007/s10562-016-1894-3 |
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| Katalog-ID: |
OLC2040190856 |
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| 520 | |a Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. Graphical Abstract | ||
| 650 | 4 | |a Nitrate | |
| 650 | 4 | |a Electrochemical reduction | |
| 650 | 4 | |a Dual-chamber cell | |
| 650 | 4 | |a Ti/TiO | |
| 650 | 4 | |a nanotube array anode | |
| 650 | 4 | |a Fe | |
| 700 | 1 | |a Xiao, Chengwei |4 aut | |
| 700 | 1 | |a Zhao, Yuan |4 aut | |
| 700 | 1 | |a Zhao, Qingqing |4 aut | |
| 700 | 1 | |a Fan, Rong |4 aut | |
| 700 | 1 | |a Xue, Jianjun |4 aut | |
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10.1007/s10562-016-1894-3 doi (DE-627)OLC2040190856 (DE-He213)s10562-016-1894-3-p DE-627 ger DE-627 rakwb eng 540 660 VZ VA 2890 VZ rvk Li, Wan verfasserin aut Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer Science+Business Media New York 2016 Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. Graphical Abstract Nitrate Electrochemical reduction Dual-chamber cell Ti/TiO nanotube array anode Fe Xiao, Chengwei aut Zhao, Yuan aut Zhao, Qingqing aut Fan, Rong aut Xue, Jianjun aut Enthalten in Catalysis letters Springer US, 1988 146(2016), 12 vom: 28. Okt., Seite 2585-2595 (DE-627)130436550 (DE-600)644234-1 (DE-576)025720724 1011-372X nnns volume:146 year:2016 number:12 day:28 month:10 pages:2585-2595 https://doi.org/10.1007/s10562-016-1894-3 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE GBV_ILN_70 GBV_ILN_4012 VA 2890 AR 146 2016 12 28 10 2585-2595 |
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10.1007/s10562-016-1894-3 doi (DE-627)OLC2040190856 (DE-He213)s10562-016-1894-3-p DE-627 ger DE-627 rakwb eng 540 660 VZ VA 2890 VZ rvk Li, Wan verfasserin aut Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer Science+Business Media New York 2016 Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. Graphical Abstract Nitrate Electrochemical reduction Dual-chamber cell Ti/TiO nanotube array anode Fe Xiao, Chengwei aut Zhao, Yuan aut Zhao, Qingqing aut Fan, Rong aut Xue, Jianjun aut Enthalten in Catalysis letters Springer US, 1988 146(2016), 12 vom: 28. Okt., Seite 2585-2595 (DE-627)130436550 (DE-600)644234-1 (DE-576)025720724 1011-372X nnns volume:146 year:2016 number:12 day:28 month:10 pages:2585-2595 https://doi.org/10.1007/s10562-016-1894-3 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE GBV_ILN_70 GBV_ILN_4012 VA 2890 AR 146 2016 12 28 10 2585-2595 |
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10.1007/s10562-016-1894-3 doi (DE-627)OLC2040190856 (DE-He213)s10562-016-1894-3-p DE-627 ger DE-627 rakwb eng 540 660 VZ VA 2890 VZ rvk Li, Wan verfasserin aut Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer Science+Business Media New York 2016 Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. Graphical Abstract Nitrate Electrochemical reduction Dual-chamber cell Ti/TiO nanotube array anode Fe Xiao, Chengwei aut Zhao, Yuan aut Zhao, Qingqing aut Fan, Rong aut Xue, Jianjun aut Enthalten in Catalysis letters Springer US, 1988 146(2016), 12 vom: 28. Okt., Seite 2585-2595 (DE-627)130436550 (DE-600)644234-1 (DE-576)025720724 1011-372X nnns volume:146 year:2016 number:12 day:28 month:10 pages:2585-2595 https://doi.org/10.1007/s10562-016-1894-3 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE GBV_ILN_70 GBV_ILN_4012 VA 2890 AR 146 2016 12 28 10 2585-2595 |
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10.1007/s10562-016-1894-3 doi (DE-627)OLC2040190856 (DE-He213)s10562-016-1894-3-p DE-627 ger DE-627 rakwb eng 540 660 VZ VA 2890 VZ rvk Li, Wan verfasserin aut Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer Science+Business Media New York 2016 Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. Graphical Abstract Nitrate Electrochemical reduction Dual-chamber cell Ti/TiO nanotube array anode Fe Xiao, Chengwei aut Zhao, Yuan aut Zhao, Qingqing aut Fan, Rong aut Xue, Jianjun aut Enthalten in Catalysis letters Springer US, 1988 146(2016), 12 vom: 28. Okt., Seite 2585-2595 (DE-627)130436550 (DE-600)644234-1 (DE-576)025720724 1011-372X nnns volume:146 year:2016 number:12 day:28 month:10 pages:2585-2595 https://doi.org/10.1007/s10562-016-1894-3 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE GBV_ILN_70 GBV_ILN_4012 VA 2890 AR 146 2016 12 28 10 2585-2595 |
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10.1007/s10562-016-1894-3 doi (DE-627)OLC2040190856 (DE-He213)s10562-016-1894-3-p DE-627 ger DE-627 rakwb eng 540 660 VZ VA 2890 VZ rvk Li, Wan verfasserin aut Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell 2016 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer Science+Business Media New York 2016 Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. Graphical Abstract Nitrate Electrochemical reduction Dual-chamber cell Ti/TiO nanotube array anode Fe Xiao, Chengwei aut Zhao, Yuan aut Zhao, Qingqing aut Fan, Rong aut Xue, Jianjun aut Enthalten in Catalysis letters Springer US, 1988 146(2016), 12 vom: 28. Okt., Seite 2585-2595 (DE-627)130436550 (DE-600)644234-1 (DE-576)025720724 1011-372X nnns volume:146 year:2016 number:12 day:28 month:10 pages:2585-2595 https://doi.org/10.1007/s10562-016-1894-3 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC SSG-OLC-TEC SSG-OLC-CHE GBV_ILN_70 GBV_ILN_4012 VA 2890 AR 146 2016 12 28 10 2585-2595 |
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Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell |
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(DE-627)OLC2040190856 (DE-He213)s10562-016-1894-3-p |
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Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell |
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Li, Wan |
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2016 |
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Li, Wan Xiao, Chengwei Zhao, Yuan Zhao, Qingqing Fan, Rong Xue, Jianjun |
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10.1007/s10562-016-1894-3 |
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540 660 |
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electrochemical reduction of high-concentrated nitrate using ti/$ tio_{2} $ nanotube array anode and fe cathode in dual-chamber cell |
| title_auth |
Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell |
| abstract |
Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. Graphical Abstract © Springer Science+Business Media New York 2016 |
| abstractGer |
Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. Graphical Abstract © Springer Science+Business Media New York 2016 |
| abstract_unstemmed |
Abstract Electrochemical reduction of nitrate using Fe cathode and Ti/$ TiO_{2} $ nanotube array anode in dual-chamber cell was investigated. The performance of different cathodes for nitrate removal were in the order of Fe>Al>Cu>Ni. The nitrate removal in dual-chamber cell (99.8%) was much higher than that in single-chamber cell (84.3%) with Fe cathode in 2.5 h. In dual-chamber cell, the highest nitrate removal was obtained at the current density of 15 mA/$ cm^{2} $. The nitrate reduction followed first-order kinetics. With increasing initial nitrate concentration, the reduction rate constant slightly decreased from 2.2 $ h^{−1} $ (100.0 mg/L) to 0.9 $ h^{−1} $ (1000.0 mg/L), of which a remarkable nitrate removal of 88.3% could still be achieved with 1000.0 mg/L nitrate. In the presence of 0.5 g/L NaCl, simultaneous reduction of nitrate and oxidation of by-products of ammonia and nitrite were achieved in dual-chamber cell with Fe cathode, of which the nitrate removal rate was 94.3% and no by-products were detected in the solution. Graphical Abstract © Springer Science+Business Media New York 2016 |
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Electrochemical Reduction of High-Concentrated Nitrate Using Ti/$ TiO_{2} $ Nanotube Array Anode and Fe Cathode in Dual-Chamber Cell |
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Xiao, Chengwei Zhao, Yuan Zhao, Qingqing Fan, Rong Xue, Jianjun |
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