Remobilization of trace metals from contaminated marine sediment in a simulated dynamic environment
Abstract In this study, release and redistribution of sediment bound trace metals due to resuspension were investigated by a lid-driven elongated annular flume (LEAF). The total suspended particulate matters (SPMs) increased significantly in quantity with the raised resuspension energies and varied...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Xu, Weihai [verfasserIn] |
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| Format: |
Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2015 |
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| Schlagwörter: |
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| Anmerkung: |
© Springer-Verlag Berlin Heidelberg 2015 |
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| Übergeordnetes Werk: |
Enthalten in: Environmental science and pollution research - Springer Berlin Heidelberg, 1994, 22(2015), 24 vom: 21. Aug., Seite 19905-19911 |
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| Übergeordnetes Werk: |
volume:22 ; year:2015 ; number:24 ; day:21 ; month:08 ; pages:19905-19911 |
| Links: |
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| DOI / URN: |
10.1007/s11356-015-5228-6 |
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| Katalog-ID: |
OLC2040454101 |
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| 520 | |a Abstract In this study, release and redistribution of sediment bound trace metals due to resuspension were investigated by a lid-driven elongated annular flume (LEAF). The total suspended particulate matters (SPMs) increased significantly in quantity with the raised resuspension energies and varied distinctively in particle size and mineral composition. Except for Cu, Ni, Cd, Pb, and Zn showed an increase in dissolved phase as the resuspension energy increased. Relatively low Cu was observed in dissolved phase whereas it owned the highest original concentration in the sediment. This is primarily due to the very low solubility of Cu sulfide. In comparison to sediment, all metals were evidently enriched in SPMs which primarily contributed to the much more fine particles (silt/clay fraction) contained in the SPMs. Metals enrichment followed the Irving-Williams order of complex stability. However, metals content varied indistinctively in the SPMs among the three selected resuspension levels. The distribution coefficients (Kd) exhibited opposite trend with the increasing resuspension level with the exception of Cu. It indicated that physical and chemical characters of sediment such as grain composition, Fe/Mn, and organic matter content may also act as major factors in the release of metals and control their phase distribution in the water column. | ||
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10.1007/s11356-015-5228-6 doi (DE-627)OLC2040454101 (DE-He213)s11356-015-5228-6-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Xu, Weihai verfasserin aut Remobilization of trace metals from contaminated marine sediment in a simulated dynamic environment 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag Berlin Heidelberg 2015 Abstract In this study, release and redistribution of sediment bound trace metals due to resuspension were investigated by a lid-driven elongated annular flume (LEAF). The total suspended particulate matters (SPMs) increased significantly in quantity with the raised resuspension energies and varied distinctively in particle size and mineral composition. Except for Cu, Ni, Cd, Pb, and Zn showed an increase in dissolved phase as the resuspension energy increased. Relatively low Cu was observed in dissolved phase whereas it owned the highest original concentration in the sediment. This is primarily due to the very low solubility of Cu sulfide. In comparison to sediment, all metals were evidently enriched in SPMs which primarily contributed to the much more fine particles (silt/clay fraction) contained in the SPMs. Metals enrichment followed the Irving-Williams order of complex stability. However, metals content varied indistinctively in the SPMs among the three selected resuspension levels. The distribution coefficients (Kd) exhibited opposite trend with the increasing resuspension level with the exception of Cu. It indicated that physical and chemical characters of sediment such as grain composition, Fe/Mn, and organic matter content may also act as major factors in the release of metals and control their phase distribution in the water column. Heavy metals Sediment resuspension Simulated coastal system LEAF Li, Xiangdong aut Wai, Onyx W. H. aut Huang, Weilin aut Yan, Wen aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 22(2015), 24 vom: 21. Aug., Seite 19905-19911 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:22 year:2015 number:24 day:21 month:08 pages:19905-19911 https://doi.org/10.1007/s11356-015-5228-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR SSG-OLC-DE-84 GBV_ILN_70 GBV_ILN_252 GBV_ILN_267 GBV_ILN_370 GBV_ILN_2018 GBV_ILN_2057 GBV_ILN_4012 GBV_ILN_4046 GBV_ILN_4219 GBV_ILN_4266 GBV_ILN_4277 AR 22 2015 24 21 08 19905-19911 |
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10.1007/s11356-015-5228-6 doi (DE-627)OLC2040454101 (DE-He213)s11356-015-5228-6-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Xu, Weihai verfasserin aut Remobilization of trace metals from contaminated marine sediment in a simulated dynamic environment 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag Berlin Heidelberg 2015 Abstract In this study, release and redistribution of sediment bound trace metals due to resuspension were investigated by a lid-driven elongated annular flume (LEAF). The total suspended particulate matters (SPMs) increased significantly in quantity with the raised resuspension energies and varied distinctively in particle size and mineral composition. Except for Cu, Ni, Cd, Pb, and Zn showed an increase in dissolved phase as the resuspension energy increased. Relatively low Cu was observed in dissolved phase whereas it owned the highest original concentration in the sediment. This is primarily due to the very low solubility of Cu sulfide. In comparison to sediment, all metals were evidently enriched in SPMs which primarily contributed to the much more fine particles (silt/clay fraction) contained in the SPMs. Metals enrichment followed the Irving-Williams order of complex stability. However, metals content varied indistinctively in the SPMs among the three selected resuspension levels. The distribution coefficients (Kd) exhibited opposite trend with the increasing resuspension level with the exception of Cu. It indicated that physical and chemical characters of sediment such as grain composition, Fe/Mn, and organic matter content may also act as major factors in the release of metals and control their phase distribution in the water column. Heavy metals Sediment resuspension Simulated coastal system LEAF Li, Xiangdong aut Wai, Onyx W. H. aut Huang, Weilin aut Yan, Wen aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 22(2015), 24 vom: 21. Aug., Seite 19905-19911 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:22 year:2015 number:24 day:21 month:08 pages:19905-19911 https://doi.org/10.1007/s11356-015-5228-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR SSG-OLC-DE-84 GBV_ILN_70 GBV_ILN_252 GBV_ILN_267 GBV_ILN_370 GBV_ILN_2018 GBV_ILN_2057 GBV_ILN_4012 GBV_ILN_4046 GBV_ILN_4219 GBV_ILN_4266 GBV_ILN_4277 AR 22 2015 24 21 08 19905-19911 |
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10.1007/s11356-015-5228-6 doi (DE-627)OLC2040454101 (DE-He213)s11356-015-5228-6-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Xu, Weihai verfasserin aut Remobilization of trace metals from contaminated marine sediment in a simulated dynamic environment 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag Berlin Heidelberg 2015 Abstract In this study, release and redistribution of sediment bound trace metals due to resuspension were investigated by a lid-driven elongated annular flume (LEAF). The total suspended particulate matters (SPMs) increased significantly in quantity with the raised resuspension energies and varied distinctively in particle size and mineral composition. Except for Cu, Ni, Cd, Pb, and Zn showed an increase in dissolved phase as the resuspension energy increased. Relatively low Cu was observed in dissolved phase whereas it owned the highest original concentration in the sediment. This is primarily due to the very low solubility of Cu sulfide. In comparison to sediment, all metals were evidently enriched in SPMs which primarily contributed to the much more fine particles (silt/clay fraction) contained in the SPMs. Metals enrichment followed the Irving-Williams order of complex stability. However, metals content varied indistinctively in the SPMs among the three selected resuspension levels. The distribution coefficients (Kd) exhibited opposite trend with the increasing resuspension level with the exception of Cu. It indicated that physical and chemical characters of sediment such as grain composition, Fe/Mn, and organic matter content may also act as major factors in the release of metals and control their phase distribution in the water column. Heavy metals Sediment resuspension Simulated coastal system LEAF Li, Xiangdong aut Wai, Onyx W. H. aut Huang, Weilin aut Yan, Wen aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 22(2015), 24 vom: 21. Aug., Seite 19905-19911 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:22 year:2015 number:24 day:21 month:08 pages:19905-19911 https://doi.org/10.1007/s11356-015-5228-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR SSG-OLC-DE-84 GBV_ILN_70 GBV_ILN_252 GBV_ILN_267 GBV_ILN_370 GBV_ILN_2018 GBV_ILN_2057 GBV_ILN_4012 GBV_ILN_4046 GBV_ILN_4219 GBV_ILN_4266 GBV_ILN_4277 AR 22 2015 24 21 08 19905-19911 |
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10.1007/s11356-015-5228-6 doi (DE-627)OLC2040454101 (DE-He213)s11356-015-5228-6-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Xu, Weihai verfasserin aut Remobilization of trace metals from contaminated marine sediment in a simulated dynamic environment 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag Berlin Heidelberg 2015 Abstract In this study, release and redistribution of sediment bound trace metals due to resuspension were investigated by a lid-driven elongated annular flume (LEAF). The total suspended particulate matters (SPMs) increased significantly in quantity with the raised resuspension energies and varied distinctively in particle size and mineral composition. Except for Cu, Ni, Cd, Pb, and Zn showed an increase in dissolved phase as the resuspension energy increased. Relatively low Cu was observed in dissolved phase whereas it owned the highest original concentration in the sediment. This is primarily due to the very low solubility of Cu sulfide. In comparison to sediment, all metals were evidently enriched in SPMs which primarily contributed to the much more fine particles (silt/clay fraction) contained in the SPMs. Metals enrichment followed the Irving-Williams order of complex stability. However, metals content varied indistinctively in the SPMs among the three selected resuspension levels. The distribution coefficients (Kd) exhibited opposite trend with the increasing resuspension level with the exception of Cu. It indicated that physical and chemical characters of sediment such as grain composition, Fe/Mn, and organic matter content may also act as major factors in the release of metals and control their phase distribution in the water column. Heavy metals Sediment resuspension Simulated coastal system LEAF Li, Xiangdong aut Wai, Onyx W. H. aut Huang, Weilin aut Yan, Wen aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 22(2015), 24 vom: 21. Aug., Seite 19905-19911 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:22 year:2015 number:24 day:21 month:08 pages:19905-19911 https://doi.org/10.1007/s11356-015-5228-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR SSG-OLC-DE-84 GBV_ILN_70 GBV_ILN_252 GBV_ILN_267 GBV_ILN_370 GBV_ILN_2018 GBV_ILN_2057 GBV_ILN_4012 GBV_ILN_4046 GBV_ILN_4219 GBV_ILN_4266 GBV_ILN_4277 AR 22 2015 24 21 08 19905-19911 |
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10.1007/s11356-015-5228-6 doi (DE-627)OLC2040454101 (DE-He213)s11356-015-5228-6-p DE-627 ger DE-627 rakwb eng 570 360 333.7 VZ 690 333.7 540 VZ BIODIV DE-30 fid Xu, Weihai verfasserin aut Remobilization of trace metals from contaminated marine sediment in a simulated dynamic environment 2015 Text txt rdacontent ohne Hilfsmittel zu benutzen n rdamedia Band nc rdacarrier © Springer-Verlag Berlin Heidelberg 2015 Abstract In this study, release and redistribution of sediment bound trace metals due to resuspension were investigated by a lid-driven elongated annular flume (LEAF). The total suspended particulate matters (SPMs) increased significantly in quantity with the raised resuspension energies and varied distinctively in particle size and mineral composition. Except for Cu, Ni, Cd, Pb, and Zn showed an increase in dissolved phase as the resuspension energy increased. Relatively low Cu was observed in dissolved phase whereas it owned the highest original concentration in the sediment. This is primarily due to the very low solubility of Cu sulfide. In comparison to sediment, all metals were evidently enriched in SPMs which primarily contributed to the much more fine particles (silt/clay fraction) contained in the SPMs. Metals enrichment followed the Irving-Williams order of complex stability. However, metals content varied indistinctively in the SPMs among the three selected resuspension levels. The distribution coefficients (Kd) exhibited opposite trend with the increasing resuspension level with the exception of Cu. It indicated that physical and chemical characters of sediment such as grain composition, Fe/Mn, and organic matter content may also act as major factors in the release of metals and control their phase distribution in the water column. Heavy metals Sediment resuspension Simulated coastal system LEAF Li, Xiangdong aut Wai, Onyx W. H. aut Huang, Weilin aut Yan, Wen aut Enthalten in Environmental science and pollution research Springer Berlin Heidelberg, 1994 22(2015), 24 vom: 21. Aug., Seite 19905-19911 (DE-627)171335805 (DE-600)1178791-0 (DE-576)038875101 0944-1344 nnns volume:22 year:2015 number:24 day:21 month:08 pages:19905-19911 https://doi.org/10.1007/s11356-015-5228-6 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_OLC FID-BIODIV SSG-OLC-UMW SSG-OLC-ARC SSG-OLC-TEC SSG-OLC-CHE SSG-OLC-FOR SSG-OLC-DE-84 GBV_ILN_70 GBV_ILN_252 GBV_ILN_267 GBV_ILN_370 GBV_ILN_2018 GBV_ILN_2057 GBV_ILN_4012 GBV_ILN_4046 GBV_ILN_4219 GBV_ILN_4266 GBV_ILN_4277 AR 22 2015 24 21 08 19905-19911 |
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remobilization of trace metals from contaminated marine sediment in a simulated dynamic environment |
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Remobilization of trace metals from contaminated marine sediment in a simulated dynamic environment |
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Abstract In this study, release and redistribution of sediment bound trace metals due to resuspension were investigated by a lid-driven elongated annular flume (LEAF). The total suspended particulate matters (SPMs) increased significantly in quantity with the raised resuspension energies and varied distinctively in particle size and mineral composition. Except for Cu, Ni, Cd, Pb, and Zn showed an increase in dissolved phase as the resuspension energy increased. Relatively low Cu was observed in dissolved phase whereas it owned the highest original concentration in the sediment. This is primarily due to the very low solubility of Cu sulfide. In comparison to sediment, all metals were evidently enriched in SPMs which primarily contributed to the much more fine particles (silt/clay fraction) contained in the SPMs. Metals enrichment followed the Irving-Williams order of complex stability. However, metals content varied indistinctively in the SPMs among the three selected resuspension levels. The distribution coefficients (Kd) exhibited opposite trend with the increasing resuspension level with the exception of Cu. It indicated that physical and chemical characters of sediment such as grain composition, Fe/Mn, and organic matter content may also act as major factors in the release of metals and control their phase distribution in the water column. © Springer-Verlag Berlin Heidelberg 2015 |
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Abstract In this study, release and redistribution of sediment bound trace metals due to resuspension were investigated by a lid-driven elongated annular flume (LEAF). The total suspended particulate matters (SPMs) increased significantly in quantity with the raised resuspension energies and varied distinctively in particle size and mineral composition. Except for Cu, Ni, Cd, Pb, and Zn showed an increase in dissolved phase as the resuspension energy increased. Relatively low Cu was observed in dissolved phase whereas it owned the highest original concentration in the sediment. This is primarily due to the very low solubility of Cu sulfide. In comparison to sediment, all metals were evidently enriched in SPMs which primarily contributed to the much more fine particles (silt/clay fraction) contained in the SPMs. Metals enrichment followed the Irving-Williams order of complex stability. However, metals content varied indistinctively in the SPMs among the three selected resuspension levels. The distribution coefficients (Kd) exhibited opposite trend with the increasing resuspension level with the exception of Cu. It indicated that physical and chemical characters of sediment such as grain composition, Fe/Mn, and organic matter content may also act as major factors in the release of metals and control their phase distribution in the water column. © Springer-Verlag Berlin Heidelberg 2015 |
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Abstract In this study, release and redistribution of sediment bound trace metals due to resuspension were investigated by a lid-driven elongated annular flume (LEAF). The total suspended particulate matters (SPMs) increased significantly in quantity with the raised resuspension energies and varied distinctively in particle size and mineral composition. Except for Cu, Ni, Cd, Pb, and Zn showed an increase in dissolved phase as the resuspension energy increased. Relatively low Cu was observed in dissolved phase whereas it owned the highest original concentration in the sediment. This is primarily due to the very low solubility of Cu sulfide. In comparison to sediment, all metals were evidently enriched in SPMs which primarily contributed to the much more fine particles (silt/clay fraction) contained in the SPMs. Metals enrichment followed the Irving-Williams order of complex stability. However, metals content varied indistinctively in the SPMs among the three selected resuspension levels. The distribution coefficients (Kd) exhibited opposite trend with the increasing resuspension level with the exception of Cu. It indicated that physical and chemical characters of sediment such as grain composition, Fe/Mn, and organic matter content may also act as major factors in the release of metals and control their phase distribution in the water column. © Springer-Verlag Berlin Heidelberg 2015 |
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